Articles | Volume 16, issue 22
https://doi.org/10.5194/acp-16-14041-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-14041-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
15 Nov 2016
Research article |
| 15 Nov 2016
Aerosol meteorology of the Maritime Continent for the 2012 7SEAS southwest monsoon intensive study – Part 1: regional-scale phenomena
Jeffrey S. Reid
CORRESPONDING AUTHOR
Marine Meteorology Division, Naval Research Laboratory,
Monterey, CA, USA
Peng Xian
Marine Meteorology Division, Naval Research Laboratory,
Monterey, CA, USA
Brent N. Holben
NASA Goddard Space Flight Center, Greenbelt,
MD, USA
Edward J. Hyer
Marine Meteorology Division, Naval Research Laboratory,
Monterey, CA, USA
Elizabeth A. Reid
Marine Meteorology Division, Naval Research Laboratory,
Monterey, CA, USA
Santo V. Salinas
Centre for Remote Imaging Sensing and Processing,
National University of Singapore, Singapore
Jianglong Zhang
Dept. of Atmospheric Science, University of North Dakota,
Grand Forks, ND, USA
James R. Campbell
Marine Meteorology Division, Naval Research Laboratory,
Monterey, CA, USA
Boon Ning Chew
Meteorological Service, Singapore
Robert E. Holz
Space Sciences Engineering Center, University of
Wisconsin, Madison, WI, USA
Arunas P. Kuciauskas
Marine Meteorology Division, Naval Research Laboratory,
Monterey, CA, USA
Nofel Lagrosas
Manila Observatory, Manila, Philippines
Derek J. Posselt
Jet Propulsion laboratory, Pasadena, CA, USA
Charles R. Sampson
Marine Meteorology Division, Naval Research Laboratory,
Monterey, CA, USA
Annette L. Walker
Marine Meteorology Division, Naval Research Laboratory,
Monterey, CA, USA
E. Judd Welton
NASA Goddard Space Flight Center, Greenbelt,
MD, USA
Chidong Zhang
NOAA Pacific Marine Environmental Laboratory Seattle,
WA, USA
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Using near-full data records of Terra and Aqua MODIS and MISR data, we have evaluated aerosol optical depth trends over global oceans (MODIS and MISR) and land (MISR). Also, for the first time, shortwave aerosol radiative effect (SWARE) trends are estimated over global oceans with the combined use of observations from MODIS and CERES.
Jennie Bukowski, Derek J. Posselt, Jeffrey S. Reid, and Samuel A. Atwood
Atmos. Chem. Phys., 17, 4611–4626, https://doi.org/10.5194/acp-17-4611-2017, https://doi.org/10.5194/acp-17-4611-2017, 2017
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The Maritime Continent (MC) exhibits tremendous meteorological variability. In this study, multiple years of atmospheric soundings over the MC are analyzed to identify key sources of variability in the region's temperature, water vapor, and wind structure. Coherent vertical structures are found among profiles sampled from different geographic locations. The results indicate that the complex meteorology of the region can be described using a few simple structure functions.
Samuel A. Atwood, Jeffrey S. Reid, Sonia M. Kreidenweis, Donald R. Blake, Haflidi H. Jonsson, Nofel D. Lagrosas, Peng Xian, Elizabeth A. Reid, Walter R. Sessions, and James B. Simpas
Atmos. Chem. Phys., 17, 1105–1123, https://doi.org/10.5194/acp-17-1105-2017, https://doi.org/10.5194/acp-17-1105-2017, 2017
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Aerosol particles were measured by ship in remote marine regions of the South China Sea as part of the 2012 7 Southeast Asian Studies (7SEAS) experiments. As the particle populations changed throughout the experiment, the distribution of particle sizes and the amount of water that collected on them changed as well. These changes were associated with various impacts from smoke, sea salt, and pollution sources, and impact how clouds form and precipitation occurs in the region.
Jeffrey S. Reid, Nofel D. Lagrosas, Haflidi H. Jonsson, Elizabeth A. Reid, Samuel A. Atwood, Thomas J. Boyd, Virendra P. Ghate, Peng Xian, Derek J. Posselt, James B. Simpas, Sherdon N. Uy, Kimo Zaiger, Donald R. Blake, Anthony Bucholtz, James R. Campbell, Boon Ning Chew, Steven S. Cliff, Brent N. Holben, Robert E. Holz, Edward J. Hyer, Sonia M. Kreidenweis, Arunas P. Kuciauskas, Simone Lolli, Min Oo, Kevin D. Perry, Santo V. Salinas, Walter R. Sessions, Alexander Smirnov, Annette L. Walker, Qing Wang, Liya Yu, Jianglong Zhang, and Yongjing Zhao
Atmos. Chem. Phys., 16, 14057–14078, https://doi.org/10.5194/acp-16-14057-2016, https://doi.org/10.5194/acp-16-14057-2016, 2016
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This paper describes aspects of the 2012 7 Southeast Asian Studies (7SEAS) operations period, the largest within the Maritime Continent. Included were an enhanced deployment of Aerosol Robotic Network (AERONET) sun photometers, multiple lidars, and a Singapore supersite. Simultaneously, a ship was dispatched to the Palawan Archipelago and Sulu Sea of the Philippines for September 2012 to observe transported smoke and pollution as it entered the southwest monsoon trough.
Peng Lynch, Jeffrey S. Reid, Douglas L. Westphal, Jianglong Zhang, Timothy F. Hogan, Edward J. Hyer, Cynthia A. Curtis, Dean A. Hegg, Yingxi Shi, James R. Campbell, Juli I. Rubin, Walter R. Sessions, F. Joseph Turk, and Annette L. Walker
Geosci. Model Dev., 9, 1489–1522, https://doi.org/10.5194/gmd-9-1489-2016, https://doi.org/10.5194/gmd-9-1489-2016, 2016
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An 11-year, 1-degree aerosol reanalysis is presented for use in studies of aerosol effects on climate and atmospheric processes. The reanalysis uses the Navy Aerosol Analysis and Prediction System, constrained by aerosol optical thickness (AOT) data from NASA sensors. Fine and coarse mode AOT at 550 nm agrees well with ground-based measurements, and reproduces the decadal AOT trends found using standalone satellite products. This dataset is a resource for basic and applied science research.
Juli I. Rubin, Jeffrey S. Reid, James A. Hansen, Jeffrey L. Anderson, Nancy Collins, Timothy J. Hoar, Timothy Hogan, Peng Lynch, Justin McLay, Carolyn A. Reynolds, Walter R. Sessions, Douglas L. Westphal, and Jianglong Zhang
Atmos. Chem. Phys., 16, 3927–3951, https://doi.org/10.5194/acp-16-3927-2016, https://doi.org/10.5194/acp-16-3927-2016, 2016
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This work tests the use of an ensemble prediction system for aerosol forecasting, including an ensemble adjustment Kalman filter for MODIS AOT assimilation. Key findings include (1) meteorology and source-perturbed ensembles are needed to capture long-range transport and near-source aerosol events, (2) adaptive covariance inflation is recommended for assimilating spatially heterogeneous observations and (3) the ensemble system captures sharp gradients relative to a deterministic/variational system.
C. Ge, J. Wang, and J. S. Reid
Atmos. Chem. Phys., 14, 159–174, https://doi.org/10.5194/acp-14-159-2014, https://doi.org/10.5194/acp-14-159-2014, 2014
R. S. Johnson, J. Zhang, E. J. Hyer, S. D. Miller, and J. S. Reid
Atmos. Meas. Tech., 6, 1245–1255, https://doi.org/10.5194/amt-6-1245-2013, https://doi.org/10.5194/amt-6-1245-2013, 2013
Y. Shi, J. Zhang, J. S. Reid, E. J. Hyer, and N. C. Hsu
Atmos. Meas. Tech., 6, 949–969, https://doi.org/10.5194/amt-6-949-2013, https://doi.org/10.5194/amt-6-949-2013, 2013
V. M. Khade, J. A. Hansen, J. S. Reid, and D. L. Westphal
Atmos. Chem. Phys., 13, 3481–3500, https://doi.org/10.5194/acp-13-3481-2013, https://doi.org/10.5194/acp-13-3481-2013, 2013
Simone Lolli, Erica K. Dolinar, Jasper R. Lewis, Andreu Salcedo-Bosch, James R. Campbell, and Ellsworth J. Welton
EGUsphere, https://doi.org/10.5194/egusphere-2025-1237, https://doi.org/10.5194/egusphere-2025-1237, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Clouds strongly influence Earth's climate by changing how sunlight is reflected or absorbed. We studied thin, high-altitude clouds using radar-laser measurements collected over twenty years at NASA GSFC. Our findings show these clouds increasingly trap heat, partly because of shrinking snow and ice cover. This trend could further accelerate warming locally, underlining the need for accurate cloud observations to improve climate forecasts and strategies to respond to climate change.
Blake T. Sorenson, Jianglong Zhang, Jeffrey S. Reid, and Peng Xian
EGUsphere, https://doi.org/10.5194/egusphere-2025-80, https://doi.org/10.5194/egusphere-2025-80, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Plumes of wildfire smoke in the Arctic affect the Arctic radiative budget. Using a neural network and observations from satellite-based sensors, we analyzed the direct radiative forcing of smoke particles on the Arctic climate and estimated long-term forcing trends. Strong negative trends in aerosol direct radiative forcing were found in northern Russia and Canada, with positive trends found over parts of the Arctic Ocean. Overall, smoke plumes may act to counter future Arctic warming.
Abdulamid A. Fakoya, Jens Redemann, Pablo E. Saide, Lan Gao, Logan T. Mitchell, Calvin Howes, Amie Dobracki, Ian Chang, Gonzalo A. Ferrada, Kristina Pistone, Samuel E. Leblanc, Michal Segal-Rozenhaimer, Arthur J. Sedlacek III, Thomas Eck, Brent Holben, Pawan Gupta, Elena Lind, Paquita Zuidema, Gregory Carmichael, and Connor J. Flynn
EGUsphere, https://doi.org/10.5194/egusphere-2024-3197, https://doi.org/10.5194/egusphere-2024-3197, 2025
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Tiny atmospheric particles from wildfire smoke impact climate by interacting with sunlight and clouds, the extent of which is uncertain due to gaps in understanding how smoke changes over time. We developed a new method using remote sensing instruments to track how these particles evolve during atmospheric transport. Our results show that the ability of these particles to absorb sunlight increased as they travel. This discovery could help improve predictions of future climate scenarios.
Jianglong Zhang, Jeffrey S. Reid, Blake Sorenson, Steven D. Miller, Miguel O. Román, Zhuosen Wang, Robert J. D. Spurr, Shawn Jaker, Thomas F. Eck, and Juli I. Rubin
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-181, https://doi.org/10.5194/amt-2024-181, 2024
Revised manuscript accepted for AMT
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Using observations from the Visible Infrared Imaging Radiometer Suite Day-Night Band, we developed a method for constructing gridded nighttime aerosol optical thickness (AOT) data based on the spatial derivative of measured top-of-atmosphere attenuated upwelling artificial lights at night. The gridded nighttime AOT retrievals, compared against Aerosol Robotic Network data, show reasonable skill levels for potential data assimilation, air quality and climate studies of significant events.
Yenny González, María F. Sánchez-Barrero, Ioana Popovici, África Barreto, Stephane Victori, Ellsworth J. Welton, Rosa D. García, Pablo G. Sicilia, Fernando A. Almansa, Carlos Torres, and Philippe Goloub
EGUsphere, https://doi.org/10.5194/egusphere-2024-2727, https://doi.org/10.5194/egusphere-2024-2727, 2024
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We characterize the optical properties of various aerosols using a compact dual-wavelength depolarization lidar (CIMEL CE376) at 532 and 808 nm. Through a modified two-wavelength Klett inversion method, we assess the vertical distribution and temporal evolution of Saharan dust, volcanic aerosols, and wildfire smoke in the subtropical North Atlantic from August 2021 to August 2023. The study confirms the CE376 lidar's effectiveness in monitoring and characterizing atmospheric aerosols over time.
Myungje Choi, Alexei Lyapustin, Gregory L. Schuster, Sujung Go, Yujie Wang, Sergey Korkin, Ralph Kahn, Jeffrey S. Reid, Edward J. Hyer, Thomas F. Eck, Mian Chin, David J. Diner, Olga Kalashnikova, Oleg Dubovik, Jhoon Kim, and Hans Moosmüller
Atmos. Chem. Phys., 24, 10543–10565, https://doi.org/10.5194/acp-24-10543-2024, https://doi.org/10.5194/acp-24-10543-2024, 2024
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This paper introduces a retrieval algorithm to estimate two key absorbing components in smoke (black carbon and brown carbon) using DSCOVR EPIC measurements. Our analysis reveals distinct smoke properties, including spectral absorption, layer height, and black carbon and brown carbon, over North America and central Africa. The retrieved smoke properties offer valuable observational constraints for modeling radiative forcing and informing health-related studies.
Kira Zeider, Grace Betito, Anthony Bucholtz, Peng Xian, Annette Walker, and Armin Sorooshian
Atmos. Chem. Phys., 24, 9059–9083, https://doi.org/10.5194/acp-24-9059-2024, https://doi.org/10.5194/acp-24-9059-2024, 2024
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The predominant wind direction along the California coast (northerly) reverses several times during the summer (to southerly). The effects of these wind reversals on aerosol and cloud characteristics are not well understood. Using data from multiple datasets we found that southerly flow periods had enhanced signatures of anthropogenic emissions due to shipping and continental sources, and clouds had more but smaller droplets.
Zhenyu Zhang, Jing Li, Huizheng Che, Yueming Dong, Oleg Dubovik, Thomas Eck, Pawan Gupta, Brent Holben, Jhoon Kim, Elena Lind, Trailokya Saud, Sachchida Nand Tripathi, and Tong Ying
EGUsphere, https://doi.org/10.5194/egusphere-2024-2533, https://doi.org/10.5194/egusphere-2024-2533, 2024
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We used ground-based remote sensing data from the Aerosol Robotic Network to examine long-term trends in aerosol characteristics. We found aerosol loadings generally decreased globally, and aerosols became more scattering. These changes are closely related to variations in aerosol compositions, such as decreased anthropogenic emissions over East Asia, Europe, and North America, increased anthropogenic source over North India, increased dust activities over the Arabian Peninsula, etc.
Anton Lopatin, Oleg Dubovik, Georgiy Stenchikov, Ellsworth J. Welton, Illia Shevchenko, David Fuertes, Marcos Herreras-Giralda, Tatsiana Lapyonok, and Alexander Smirnov
Atmos. Meas. Tech., 17, 4445–4470, https://doi.org/10.5194/amt-17-4445-2024, https://doi.org/10.5194/amt-17-4445-2024, 2024
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We compare aerosol properties over the King Abdullah University of Science and Technology campus using Generalized Retrieval of Aerosol and Surface Properties (GRASP) and the Micro-Pulse Lidar Network (MPLNET). We focus on the impact of different aerosol retrieval assumptions on daytime and nighttime retrievals and analyze seasonal variability in aerosol properties, aiding in understanding aerosol behavior and improving retrieval. Our work has implications for climate and public health.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedetti, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
Atmos. Chem. Phys., 24, 6385–6411, https://doi.org/10.5194/acp-24-6385-2024, https://doi.org/10.5194/acp-24-6385-2024, 2024
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The study compares and evaluates monthly AOD of four reanalyses (RA) and their consensus (i.e., ensemble mean). The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where divergence and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Maria Fernanda Sanchez Barrero, Ioana Elisabeta Popovici, Philippe Goloub, Stephane Victori, Qiaoyun Hu, Benjamin Torres, Thierry Podvin, Luc Blarel, Gaël Dubois, Fabrice Ducos, Eric Bourrianne, Aliaksandr Lapionak, Lelia Proniewski, Brent Holben, David Matthew Giles, and Anthony LaRosa
Atmos. Meas. Tech., 17, 3121–3146, https://doi.org/10.5194/amt-17-3121-2024, https://doi.org/10.5194/amt-17-3121-2024, 2024
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This study showcases the use of a compact elastic lidar to monitor aerosols aboard moving platforms. By coupling dual-wavelength and depolarization measurements with photometer data, we studied aerosols during events of Saharan dust and smoke transport. Our research, conducted in various scenarios, not only validated our methods but also offered insights into the atmospheric dynamics near active fires. This study aids future research to fill observational gaps in aerosol monitoring.
Cristina Gil-Díaz, Michäel Sicard, Adolfo Comerón, Daniel Camilo Fortunato dos Santos Oliveira, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Jasper R. Lewis, Ellsworth J. Welton, and Simone Lolli
Atmos. Meas. Tech., 17, 1197–1216, https://doi.org/10.5194/amt-17-1197-2024, https://doi.org/10.5194/amt-17-1197-2024, 2024
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In this paper, a statistical study of cirrus geometrical and optical properties based on 4 years of continuous ground-based lidar measurements with the Barcelona (Spain) Micro Pulse Lidar (MPL) is analysed. The cloud optical depth, effective column lidar ratio and linear cloud depolarisation ratio have been calculated by a new approach to the two-way transmittance method, which is valid for both ground-based and spaceborne lidar systems. Their associated errors are also provided.
Xiaoxia Shang, Antti Lipponen, Maria Filioglou, Anu-Maija Sundström, Mark Parrington, Virginie Buchard, Anton S. Darmenov, Ellsworth J. Welton, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Alejandro Rodríguez-Gómez, Mika Komppula, and Tero Mielonen
Atmos. Chem. Phys., 24, 1329–1344, https://doi.org/10.5194/acp-24-1329-2024, https://doi.org/10.5194/acp-24-1329-2024, 2024
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In June 2019, smoke particles from a Canadian wildfire event were transported to Europe. The long-range-transported smoke plumes were monitored with a spaceborne lidar and reanalysis models. Based on the aerosol mass concentrations estimated from the observations, the reanalysis models had difficulties in reproducing the amount and location of the smoke aerosols during the transport event. Consequently, more spaceborne lidar missions are needed for reliable monitoring of aerosol plumes.
Blake T. Sorenson, Jeffrey S. Reid, Jianglong Zhang, Robert E. Holz, William L. Smith Sr., and Amanda Gumber
Atmos. Chem. Phys., 24, 1231–1248, https://doi.org/10.5194/acp-24-1231-2024, https://doi.org/10.5194/acp-24-1231-2024, 2024
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Smoke particles are typically submicron in size and assumed to have negligible impacts at the thermal infrared spectrum. However, we show that infrared signatures can be observed over dense smoke plumes from satellites. We found that giant particles are unlikely to be the dominant cause. Rather, co-transported water vapor injected to the middle to upper troposphere and surface cooling beneath the plume due to shadowing are significant, with the surface cooling effect being the most dominant.
Nofel Lagrosas, Kosuke Okubo, Hitoshi Irie, Yutaka Matsumi, Tomoki Nakayama, Yutaka Sugita, Takashi Okada, and Tatsuo Shiina
Atmos. Meas. Tech., 16, 5937–5951, https://doi.org/10.5194/amt-16-5937-2023, https://doi.org/10.5194/amt-16-5937-2023, 2023
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This work examines the near-ground aerosol–weather relationship from 7-month continuous lidar and weather observations in Chiba, Japan. Optical parameters from lidar data are compared with weather parameters to understand and quantify the aerosol–weather relationship and how these optical parameters are affected by the weather and season. The results provide insights into analyzing optical properties of radioactive aerosols when the lidar system is continuously operated in a radioactive area.
Genevieve Rose Lorenzo, Avelino F. Arellano, Maria Obiminda Cambaliza, Christopher Castro, Melliza Templonuevo Cruz, Larry Di Girolamo, Glenn Franco Gacal, Miguel Ricardo A. Hilario, Nofel Lagrosas, Hans Jarett Ong, James Bernard Simpas, Sherdon Niño Uy, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10579–10608, https://doi.org/10.5194/acp-23-10579-2023, https://doi.org/10.5194/acp-23-10579-2023, 2023
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Aerosol and weather interactions in Southeast Asia are complex and understudied. An emerging aerosol climatology was established in Metro Manila, the Philippines, from aerosol particle physicochemical properties and meteorology, revealing five sources. Even with local traffic, transported smoke from biomass burning, aged dust, and cloud processing, background marine particles dominate and correspond to lower aerosol optical depth in Metro Manila compared to other Southeast Asian megacities.
Qian Xiao, Jiaoshi Zhang, Yang Wang, Luke D. Ziemba, Ewan Crosbie, Edward L. Winstead, Claire E. Robinson, Joshua P. DiGangi, Glenn S. Diskin, Jeffrey S. Reid, K. Sebastian Schmidt, Armin Sorooshian, Miguel Ricardo A. Hilario, Sarah Woods, Paul Lawson, Snorre A. Stamnes, and Jian Wang
Atmos. Chem. Phys., 23, 9853–9871, https://doi.org/10.5194/acp-23-9853-2023, https://doi.org/10.5194/acp-23-9853-2023, 2023
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Using recent airborne measurements, we show that the influences of anthropogenic emissions, transport, convective clouds, and meteorology lead to new particle formation (NPF) under a variety of conditions and at different altitudes in tropical marine environments. NPF is enhanced by fresh urban emissions in convective outflow but is suppressed in air masses influenced by aged urban emissions where reactive precursors are mostly consumed while particle surface area remains relatively high.
Alia L. Khan, Peng Xian, and Joshua P. Schwarz
The Cryosphere, 17, 2909–2918, https://doi.org/10.5194/tc-17-2909-2023, https://doi.org/10.5194/tc-17-2909-2023, 2023
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Ice–albedo feedbacks in the ablation region of the Greenland Ice Sheet are difficult to constrain and model. Surface samples were collected across the 2014 summer melt season from different ice surface colors. On average, concentrations were higher in patches that were visibly dark, compared to medium patches and light patches, suggesting that black carbon aggregation contributed to snow aging, and vice versa. High concentrations are likely due to smoke transport from high-latitude wildfires.
Blake T. Sorenson, Jianglong Zhang, Jeffrey S. Reid, Peng Xian, and Shawn L. Jaker
Atmos. Chem. Phys., 23, 7161–7175, https://doi.org/10.5194/acp-23-7161-2023, https://doi.org/10.5194/acp-23-7161-2023, 2023
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We quality-control Ozone Monitoring Instrument (OMI) aerosol index data by identifying row anomalies and removing systematic biases, using the data to quantify trends in UV-absorbing aerosols over the Arctic region. We found decreasing trends in UV-absorbing aerosols in spring months and increasing trends in summer months. For the first time, observational evidence of increasing trends in UV-absorbing aerosols over the North Pole is found using the OMI data, especially over the last half decade.
Robert Pincus, Paul A. Hubanks, Steven Platnick, Kerry Meyer, Robert E. Holz, Denis Botambekov, and Casey J. Wall
Earth Syst. Sci. Data, 15, 2483–2497, https://doi.org/10.5194/essd-15-2483-2023, https://doi.org/10.5194/essd-15-2483-2023, 2023
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This paper describes a new global dataset of cloud properties observed by a specific satellite program created to facilitate comparison with a matching observational proxy used in climate models. Statistics are accumulated over daily and monthly timescales on an equal-angle grid. Statistics include cloud detection, cloud-top pressure, and cloud optical properties. Joint histograms of several variable pairs are also available.
Jianglong Zhang, Jeffrey S. Reid, Steven D. Miller, Miguel Román, Zhuosen Wang, Robert J. D. Spurr, and Shawn Jaker
Atmos. Meas. Tech., 16, 2531–2546, https://doi.org/10.5194/amt-16-2531-2023, https://doi.org/10.5194/amt-16-2531-2023, 2023
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We adapted the spherical harmonics discrete ordinate method 3-dimentional radiative transfer model (3-D RTM) and developed a nighttime 3-D RTM capability for simulating top-of-atmosphere radiances from artificial light sources for aerosol retrievals. Our study suggests that both aerosol optical depth and aerosol plume height can be effectively retrieved using nighttime observations over artificial light sources, through the newly developed radiative transfer modeling capability.
Amanda Gumber, Jeffrey S. Reid, Robert E. Holz, Thomas F. Eck, N. Christina Hsu, Robert C. Levy, Jianglong Zhang, and Paolo Veglio
Atmos. Meas. Tech., 16, 2547–2573, https://doi.org/10.5194/amt-16-2547-2023, https://doi.org/10.5194/amt-16-2547-2023, 2023
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The purpose of this study is to create and evaluate a gridded dataset composed of multiple satellite instruments and algorithms to be used for data assimilation. An important part of aerosol data assimilation is having consistent measurements, especially for severe aerosol events. This study evaluates 4 years of data from MODIS, VIIRS, and AERONET with a focus on aerosol severe event detection from a regional and global perspective.
Hong Chen, K. Sebastian Schmidt, Steven T. Massie, Vikas Nataraja, Matthew S. Norgren, Jake J. Gristey, Graham Feingold, Robert E. Holz, and Hironobu Iwabuchi
Atmos. Meas. Tech., 16, 1971–2000, https://doi.org/10.5194/amt-16-1971-2023, https://doi.org/10.5194/amt-16-1971-2023, 2023
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We introduce the Education and Research 3D Radiative Transfer Toolbox (EaR3T) and propose a radiance self-consistency approach for quantifying and mitigating 3D bias in legacy airborne and spaceborne imagery retrievals due to spatially inhomogeneous clouds and surfaces.
Juli I. Rubin, Jeffrey S. Reid, Peng Xian, Christopher M. Selman, and Thomas F. Eck
Atmos. Chem. Phys., 23, 4059–4090, https://doi.org/10.5194/acp-23-4059-2023, https://doi.org/10.5194/acp-23-4059-2023, 2023
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This work aims to quantify the covariability between aerosol optical depth/extinction with water vapor (PW) globally, using NASA AERONET observations and NAAPS model data. Findings are important for data assimilation and radiative transfer. The study shows statistically significant and positive AOD–PW relationships are found across the globe, varying in strength with location and season and tied to large-scale aerosol events. Hygroscopic growth was also found to be an important factor.
Norman T. O'Neill, Keyvan Ranjbar, Liviu Ivănescu, Thomas F. Eck, Jeffrey S. Reid, David M. Giles, Daniel Pérez-Ramírez, and Jai Prakash Chaubey
Atmos. Meas. Tech., 16, 1103–1120, https://doi.org/10.5194/amt-16-1103-2023, https://doi.org/10.5194/amt-16-1103-2023, 2023
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Aerosols are atmospheric particles that vary in size (radius) from a fraction of a micrometer (µm) to around 20 µm. They tend to be either smaller than 1 µm (like smoke or pollution) or larger than 1 µm (like dust or sea salt). Their optical effect (scattering and absorbing sunlight) can be divided into FM (fine-mode) and CM (coarse-mode) parts using a cutoff radius around 1 µm or a spectral (color) technique. We present and validate a theoretical link between the types of FM and CM divisions.
Hyungwon John Park, Jeffrey S. Reid, Livia S. Freire, Christopher Jackson, and David H. Richter
Atmos. Meas. Tech., 15, 7171–7194, https://doi.org/10.5194/amt-15-7171-2022, https://doi.org/10.5194/amt-15-7171-2022, 2022
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We use numerical models to study field measurements of sea spray aerosol particles and conclude that both the atmospheric state and the methods of instrument sampling are causes for the variation in the production rate of aerosol particles: a critical metric to learn the aerosol's effect on processes like cloud physics and radiation. This work helps field observers improve their experimental design and interpretation of measurements because of turbulence in the atmosphere.
Eva-Lou Edwards, Jeffrey S. Reid, Peng Xian, Sharon P. Burton, Anthony L. Cook, Ewan C. Crosbie, Marta A. Fenn, Richard A. Ferrare, Sean W. Freeman, John W. Hair, David B. Harper, Chris A. Hostetler, Claire E. Robinson, Amy Jo Scarino, Michael A. Shook, G. Alexander Sokolowsky, Susan C. van den Heever, Edward L. Winstead, Sarah Woods, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 12961–12983, https://doi.org/10.5194/acp-22-12961-2022, https://doi.org/10.5194/acp-22-12961-2022, 2022
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This study compares NAAPS-RA model simulations of aerosol optical thickness (AOT) and extinction to those retrieved with a high spectral resolution lidar near the Philippines. Agreement for AOT was good, and extinction agreement was strongest below 1500 m. Substituting dropsonde relative humidities into NAAPS-RA did not drastically improve agreement, and we discuss potential reasons why. Accurately modeling future conditions in this region is crucial due to its susceptibility to climate change.
Ukkyo Jeong, Si-Chee Tsay, N. Christina Hsu, David M. Giles, John W. Cooper, Jaehwa Lee, Robert J. Swap, Brent N. Holben, James J. Butler, Sheng-Hsiang Wang, Somporn Chantara, Hyunkee Hong, Donghee Kim, and Jhoon Kim
Atmos. Chem. Phys., 22, 11957–11986, https://doi.org/10.5194/acp-22-11957-2022, https://doi.org/10.5194/acp-22-11957-2022, 2022
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Ultraviolet (UV) measurements from satellite and ground are important for deriving information on several atmospheric trace and aerosol characteristics. Simultaneous retrievals of aerosol and trace gases in this study suggest that water uptake by aerosols is one of the important phenomena affecting aerosol properties over northern Thailand, which is important for regional air quality and climate. Obtained aerosol properties covering the UV are also important for various satellite algorithms.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Travis D. Toth, Blake Sorenson, Peter R. Colarco, Zak Kipling, Edward J. Hyer, James R. Campbell, Jeffrey S. Reid, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9915–9947, https://doi.org/10.5194/acp-22-9915-2022, https://doi.org/10.5194/acp-22-9915-2022, 2022
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The study provides baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Jeffrey S. Reid, Travis D. Toth, Blake Sorenson, Edward J. Hyer, James R. Campbell, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9949–9967, https://doi.org/10.5194/acp-22-9949-2022, https://doi.org/10.5194/acp-22-9949-2022, 2022
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The study provides a baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Alexander Sinyuk, Brent N. Holben, Thomas F. Eck, David M. Giles, Ilya Slutsker, Oleg Dubovik, Joel S. Schafer, Alexander Smirnov, and Mikhail Sorokin
Atmos. Meas. Tech., 15, 4135–4151, https://doi.org/10.5194/amt-15-4135-2022, https://doi.org/10.5194/amt-15-4135-2022, 2022
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This paper describes modification of smoothness constraints on the imaginary part of the refractive index employed in the AERONET aerosol retrieval algorithm. This modification is termed relaxed due to the weaker strength of this new smoothness constraint. Applying the modified version of the smoothness constraint results in a significant reduction of retrieved light absorption by brown-carbon-containing aerosols.
Joseph S. Schlosser, Connor Stahl, Armin Sorooshian, Yen Thi-Hoang Le, Ki-Joon Jeon, Peng Xian, Carolyn E. Jordan, Katherine R. Travis, James H. Crawford, Sung Yong Gong, Hye-Jung Shin, In-Ho Song, and Jong-sang Youn
Atmos. Chem. Phys., 22, 7505–7522, https://doi.org/10.5194/acp-22-7505-2022, https://doi.org/10.5194/acp-22-7505-2022, 2022
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During a major haze pollution episode in March 2019, anthropogenic emissions were dominant in the boundary layer over Incheon and Seoul, South Korea. Using supermicrometer and submicrometer size- and chemistry-resolved aerosol particle measurements taken during this haze pollution period, this work shows that local emissions and a shallow boundary layer, enhanced humidity, and low temperature promoted local heterogeneous formation of secondary inorganic and organic aerosol species.
Matthew S. Norgren, John Wood, K. Sebastian Schmidt, Bastiaan van Diedenhoven, Snorre A. Stamnes, Luke D. Ziemba, Ewan C. Crosbie, Michael A. Shook, A. Scott Kittelman, Samuel E. LeBlanc, Stephen Broccardo, Steffen Freitag, and Jeffrey S. Reid
Atmos. Meas. Tech., 15, 1373–1394, https://doi.org/10.5194/amt-15-1373-2022, https://doi.org/10.5194/amt-15-1373-2022, 2022
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A new spectral instrument (SPN-S), with the ability to partition solar radiation into direct and diffuse components, is used in airborne settings to study the optical properties of aerosols and cirrus. It is a low-cost and mechanically simple system but has higher measurement uncertainty than existing standards. This challenge is overcome by utilizing the unique measurement capabilities to develop new retrieval techniques. Validation is done with data from two NASA airborne research campaigns.
Martin J. Osborne, Johannes de Leeuw, Claire Witham, Anja Schmidt, Frances Beckett, Nina Kristiansen, Joelle Buxmann, Cameron Saint, Ellsworth J. Welton, Javier Fochesatto, Ana R. Gomes, Ulrich Bundke, Andreas Petzold, Franco Marenco, and Jim Haywood
Atmos. Chem. Phys., 22, 2975–2997, https://doi.org/10.5194/acp-22-2975-2022, https://doi.org/10.5194/acp-22-2975-2022, 2022
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Using the Met Office NAME dispersion model, supported by satellite- and ground-based remote-sensing observations, we describe the dispersion of aerosols from the 2019 Raikoke eruption and the concurrent wildfires in Alberta Canada. We show how the synergy of dispersion modelling and multiple observation sources allowed observers in the London VAAC to arrive at a more complete picture of the aerosol loading at altitudes commonly used by aviation.
Jean-Claude Roger, Eric Vermote, Sergii Skakun, Emilie Murphy, Oleg Dubovik, Natacha Kalecinski, Bruno Korgo, and Brent Holben
Atmos. Meas. Tech., 15, 1123–1144, https://doi.org/10.5194/amt-15-1123-2022, https://doi.org/10.5194/amt-15-1123-2022, 2022
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From measurements of the sky performed by AERONET, we determined the microphysical properties of the atmospheric particles (aerosols) for each AERONET site. We used the aerosol optical thickness and its variation over the visible spectrum. This allows us to determine an aerosol model useful for (but not only) the validation of the surface reflectance satellite-derived product. The impact of the aerosol model uncertainties on the surface reflectance validation has been found to be 1 % to 3 %.
Sujung Go, Alexei Lyapustin, Gregory L. Schuster, Myungje Choi, Paul Ginoux, Mian Chin, Olga Kalashnikova, Oleg Dubovik, Jhoon Kim, Arlindo da Silva, Brent Holben, and Jeffrey S. Reid
Atmos. Chem. Phys., 22, 1395–1423, https://doi.org/10.5194/acp-22-1395-2022, https://doi.org/10.5194/acp-22-1395-2022, 2022
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This paper presents a retrieval algorithm of iron-oxide species (hematite, goethite) content in the atmosphere from DSCOVR EPIC observations. Our results display variations within the published range of hematite and goethite over the main dust-source regions but show significant seasonal and spatial variability. This implies a single-viewing satellite instrument with UV–visible channels may provide essential information on shortwave dust direct radiative effects for climate modeling.
Xinxin Ye, Pargoal Arab, Ravan Ahmadov, Eric James, Georg A. Grell, Bradley Pierce, Aditya Kumar, Paul Makar, Jack Chen, Didier Davignon, Greg R. Carmichael, Gonzalo Ferrada, Jeff McQueen, Jianping Huang, Rajesh Kumar, Louisa Emmons, Farren L. Herron-Thorpe, Mark Parrington, Richard Engelen, Vincent-Henri Peuch, Arlindo da Silva, Amber Soja, Emily Gargulinski, Elizabeth Wiggins, Johnathan W. Hair, Marta Fenn, Taylor Shingler, Shobha Kondragunta, Alexei Lyapustin, Yujie Wang, Brent Holben, David M. Giles, and Pablo E. Saide
Atmos. Chem. Phys., 21, 14427–14469, https://doi.org/10.5194/acp-21-14427-2021, https://doi.org/10.5194/acp-21-14427-2021, 2021
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Wildfire smoke has crucial impacts on air quality, while uncertainties in the numerical forecasts remain significant. We present an evaluation of 12 real-time forecasting systems. Comparison of predicted smoke emissions suggests a large spread in magnitudes, with temporal patterns deviating from satellite detections. The performance for AOD and surface PM2.5 and their discrepancies highlighted the role of accurately represented spatiotemporal emission profiles in improving smoke forecasts.
Connor Stahl, Ewan Crosbie, Paola Angela Bañaga, Grace Betito, Rachel A. Braun, Zenn Marie Cainglet, Maria Obiminda Cambaliza, Melliza Templonuevo Cruz, Julie Mae Dado, Miguel Ricardo A. Hilario, Gabrielle Frances Leung, Alexander B. MacDonald, Angela Monina Magnaye, Jeffrey Reid, Claire Robinson, Michael A. Shook, James Bernard Simpas, Shane Marie Visaga, Edward Winstead, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 21, 14109–14129, https://doi.org/10.5194/acp-21-14109-2021, https://doi.org/10.5194/acp-21-14109-2021, 2021
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A total of 159 cloud water samples were collected and measured for total organic carbon (TOC) during CAMP2Ex. On average, 30 % of TOC was speciated based on carboxylic/sulfonic acids and dimethylamine. Results provide a critical constraint on cloud composition and vertical profiles of TOC and organic species ranging from ~250 m to ~ 7 km and representing a variety of cloud types and air mass source influences such as biomass burning, marine emissions, anthropogenic activity, and dust.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Hongbin Yu, Qian Tan, Lillian Zhou, Yaping Zhou, Huisheng Bian, Mian Chin, Claire L. Ryder, Robert C. Levy, Yaswant Pradhan, Yingxi Shi, Qianqian Song, Zhibo Zhang, Peter R. Colarco, Dongchul Kim, Lorraine A. Remer, Tianle Yuan, Olga Mayol-Bracero, and Brent N. Holben
Atmos. Chem. Phys., 21, 12359–12383, https://doi.org/10.5194/acp-21-12359-2021, https://doi.org/10.5194/acp-21-12359-2021, 2021
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This study characterizes a historic African dust intrusion into the Caribbean Basin in June 2020 using satellites and NASA GEOS. Dust emissions in West Africa were large albeit not extreme. However, a unique synoptic system accumulated the dust near the coast for about 4 d before it was ventilated. Although GEOS reproduced satellite-observed plume tracks well, it substantially underestimated dust emissions and did not lift up dust high enough for ensuing long-range transport.
Patricia K. Quinn, Elizabeth J. Thompson, Derek J. Coffman, Sunil Baidar, Ludovic Bariteau, Timothy S. Bates, Sebastien Bigorre, Alan Brewer, Gijs de Boer, Simon P. de Szoeke, Kyla Drushka, Gregory R. Foltz, Janet Intrieri, Suneil Iyer, Chris W. Fairall, Cassandra J. Gaston, Friedhelm Jansen, James E. Johnson, Ovid O. Krüger, Richard D. Marchbanks, Kenneth P. Moran, David Noone, Sergio Pezoa, Robert Pincus, Albert J. Plueddemann, Mira L. Pöhlker, Ulrich Pöschl, Estefania Quinones Melendez, Haley M. Royer, Malgorzata Szczodrak, Jim Thomson, Lucia M. Upchurch, Chidong Zhang, Dongxiao Zhang, and Paquita Zuidema
Earth Syst. Sci. Data, 13, 1759–1790, https://doi.org/10.5194/essd-13-1759-2021, https://doi.org/10.5194/essd-13-1759-2021, 2021
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ATOMIC took place in the northwestern tropical Atlantic during January and February of 2020 to gather information on shallow atmospheric convection, the effects of aerosols and clouds on the ocean surface energy budget, and mesoscale oceanic processes. Measurements made from the NOAA RV Ronald H. Brown and assets it deployed (instrumented mooring and uncrewed seagoing vehicles) are described herein to advance widespread use of the data by the ATOMIC and broader research communities.
Genevieve Rose Lorenzo, Paola Angela Bañaga, Maria Obiminda Cambaliza, Melliza Templonuevo Cruz, Mojtaba AzadiAghdam, Avelino Arellano, Grace Betito, Rachel Braun, Andrea F. Corral, Hossein Dadashazar, Eva-Lou Edwards, Edwin Eloranta, Robert Holz, Gabrielle Leung, Lin Ma, Alexander B. MacDonald, Jeffrey S. Reid, James Bernard Simpas, Connor Stahl, Shane Marie Visaga, and Armin Sorooshian
Atmos. Chem. Phys., 21, 6155–6173, https://doi.org/10.5194/acp-21-6155-2021, https://doi.org/10.5194/acp-21-6155-2021, 2021
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Firework emissions change the physicochemical and optical properties of water-soluble particles, which subsequently alters the background aerosol’s respirability, influence on surroundings, ability to uptake gases, and viability as cloud condensation nuclei (CCN). There was heavy aerosol loading due to fireworks in the boundary layer. The aerosol constituents were largely water-soluble and submicrometer in size due to both inorganic salts in firework materials and gas-to-particle conversion.
Miguel Ricardo A. Hilario, Ewan Crosbie, Michael Shook, Jeffrey S. Reid, Maria Obiminda L. Cambaliza, James Bernard B. Simpas, Luke Ziemba, Joshua P. DiGangi, Glenn S. Diskin, Phu Nguyen, F. Joseph Turk, Edward Winstead, Claire E. Robinson, Jian Wang, Jiaoshi Zhang, Yang Wang, Subin Yoon, James Flynn, Sergio L. Alvarez, Ali Behrangi, and Armin Sorooshian
Atmos. Chem. Phys., 21, 3777–3802, https://doi.org/10.5194/acp-21-3777-2021, https://doi.org/10.5194/acp-21-3777-2021, 2021
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This study characterizes long-range transport from major Asian pollution sources into the tropical northwest Pacific and the impact of scavenging on these air masses. We combined aircraft observations, HYSPLIT trajectories, reanalysis, and satellite retrievals to reveal distinct composition and size distribution profiles associated with specific emission sources and wet scavenging. The results of this work have implications for international policymaking related to climate and health.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Yan Yu, Olga V. Kalashnikova, Michael J. Garay, Huikyo Lee, Myungje Choi, Gregory S. Okin, John E. Yorks, James R. Campbell, and Jared Marquis
Atmos. Chem. Phys., 21, 1427–1447, https://doi.org/10.5194/acp-21-1427-2021, https://doi.org/10.5194/acp-21-1427-2021, 2021
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Given the current uncertainties in the simulated diurnal variability of global dust mobilization and concentration, observational characterization of the variations in dust mobilization and concentration will provide a valuable benchmark for evaluating and constraining such model simulations. The current study investigates the diurnal cycle of dust loading across the global tropics, subtropics, and mid-latitudes by analyzing aerosol observations from the International Space Station.
Jianglong Zhang, Robert J. D. Spurr, Jeffrey S. Reid, Peng Xian, Peter R. Colarco, James R. Campbell, Edward J. Hyer, and Nancy L. Baker
Geosci. Model Dev., 14, 27–42, https://doi.org/10.5194/gmd-14-27-2021, https://doi.org/10.5194/gmd-14-27-2021, 2021
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A first-of-its-kind scheme has been developed for assimilating Ozone Monitoring Instrument (OMI) aerosol index (AI) measurements into the Naval Aerosol Analysis and Predictive System. Improvements in model simulations demonstrate the utility of OMI AI data assimilation for improving the accuracy of aerosol model analysis over cloudy regions and bright surfaces. This study can be considered one of the first attempts at direct radiance assimilation in the UV spectrum for aerosol analyses.
Jasper R. Lewis, James R. Campbell, Sebastian A. Stewart, Ivy Tan, Ellsworth J. Welton, and Simone Lolli
Atmos. Meas. Tech., 13, 6901–6913, https://doi.org/10.5194/amt-13-6901-2020, https://doi.org/10.5194/amt-13-6901-2020, 2020
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In this work, the authors describe a process to determine the thermodynamic cloud phase using the Micro Pulse Lidar Network volume depolarization ratio measurements and temperature profiles from the Global Modeling and Assimilation Office GEOS-5 model. A multi-year analysis and comparisons to supercooled liquid water fractions derived from CALIPSO satellite measurements are used to demonstrate the efficacy of the method.
Peng Xian, Philip J. Klotzbach, Jason P. Dunion, Matthew A. Janiga, Jeffrey S. Reid, Peter R. Colarco, and Zak Kipling
Atmos. Chem. Phys., 20, 15357–15378, https://doi.org/10.5194/acp-20-15357-2020, https://doi.org/10.5194/acp-20-15357-2020, 2020
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Using dust AOD (DAOD) data from three aerosol reanalyses, we explored the correlative relationships between DAOD and multiple indices representing seasonal Atlantic TC activities. A robust negative correlation with Caribbean DAOD and Atlantic TC activity was found. We documented for the first time the regional differences of this relationship for over the Caribbean and the tropical North Atlantic. We also evaluated the impacts of potential confounding climate factors in this relationship.
Augustin Mortier, Jonas Gliß, Michael Schulz, Wenche Aas, Elisabeth Andrews, Huisheng Bian, Mian Chin, Paul Ginoux, Jenny Hand, Brent Holben, Hua Zhang, Zak Kipling, Alf Kirkevåg, Paolo Laj, Thibault Lurton, Gunnar Myhre, David Neubauer, Dirk Olivié, Knut von Salzen, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Simone Tilmes
Atmos. Chem. Phys., 20, 13355–13378, https://doi.org/10.5194/acp-20-13355-2020, https://doi.org/10.5194/acp-20-13355-2020, 2020
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We present a multiparameter analysis of the aerosol trends over the last 2 decades in the different regions of the world. In most of the regions, ground-based observations show a decrease in aerosol content in both the total atmospheric column and at the surface. The use of climate models, assessed against these observations, reveals however an increase in the total aerosol load, which is not seen with the sole use of observation due to partial coverage in space and time.
Katta Vijayakumar, Panuganti C. S. Devara, Sunil M. Sonbawne, David M. Giles, Brent N. Holben, Sarangam Vijaya Bhaskara Rao, and Chalicheemalapalli K. Jayasankar
Atmos. Meas. Tech., 13, 5569–5593, https://doi.org/10.5194/amt-13-5569-2020, https://doi.org/10.5194/amt-13-5569-2020, 2020
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The direct-Sun and inversion products of urban atmospheric aerosols, obtained from a Cimel Sun–sky radiometer in Pune, India, under the AERONET program since October 2004, have been reported in this paper. The mean seasonal variations in AOD from cloud-free days indicated greater values during the monsoon season, revealing dominance of hygroscopic aerosols over the station. Such results are sparse in India and are important for estimating aerosol radiative forcing and validating climate models.
Willem J. Marais, Robert E. Holz, Jeffrey S. Reid, and Rebecca M. Willett
Atmos. Meas. Tech., 13, 5459–5480, https://doi.org/10.5194/amt-13-5459-2020, https://doi.org/10.5194/amt-13-5459-2020, 2020
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Space agencies use moderate-resolution satellite imagery to study how smoke, dust, pollution (aerosols) and cloud types impact the Earth's climate; these space agencies include NASA, ESA and the China Meteorological Administration. We demonstrate in this paper that an algorithm with convolutional neural networks can greatly enhance the automated detection of aerosols and cloud types from satellite imagery. Our algorithm is an improvement on current aerosol and cloud detection algorithms.
Alexander Sinyuk, Brent N. Holben, Thomas F. Eck, David M. Giles, Ilya Slutsker, Sergey Korkin, Joel S. Schafer, Alexander Smirnov, Mikhail Sorokin, and Alexei Lyapustin
Atmos. Meas. Tech., 13, 3375–3411, https://doi.org/10.5194/amt-13-3375-2020, https://doi.org/10.5194/amt-13-3375-2020, 2020
Steven Albers, Stephen M. Saleeby, Sonia Kreidenweis, Qijing Bian, Peng Xian, Zoltan Toth, Ravan Ahmadov, Eric James, and Steven D. Miller
Atmos. Meas. Tech., 13, 3235–3261, https://doi.org/10.5194/amt-13-3235-2020, https://doi.org/10.5194/amt-13-3235-2020, 2020
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A fast 3D visible-light forward operator is used to realistically visualize, validate, and potentially assimilate ground- and space-based camera and satellite imagery with NWP models. Three-dimensional fields of hydrometeors, aerosols, and 2D land surface variables are considered in the generation of radiance fields and RGB imagery from a variety of vantage points.
Pablo E. Saide, Meng Gao, Zifeng Lu, Daniel L. Goldberg, David G. Streets, Jung-Hun Woo, Andreas Beyersdorf, Chelsea A. Corr, Kenneth L. Thornhill, Bruce Anderson, Johnathan W. Hair, Amin R. Nehrir, Glenn S. Diskin, Jose L. Jimenez, Benjamin A. Nault, Pedro Campuzano-Jost, Jack Dibb, Eric Heim, Kara D. Lamb, Joshua P. Schwarz, Anne E. Perring, Jhoon Kim, Myungje Choi, Brent Holben, Gabriele Pfister, Alma Hodzic, Gregory R. Carmichael, Louisa Emmons, and James H. Crawford
Atmos. Chem. Phys., 20, 6455–6478, https://doi.org/10.5194/acp-20-6455-2020, https://doi.org/10.5194/acp-20-6455-2020, 2020
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Air quality forecasts over the Korean Peninsula captured aerosol optical depth but largely overpredicted surface PM during a Chinese haze transport event. Model deficiency was related to the calculation of optical properties. In order to improve it, aerosol size representation needs to be refined in the calculations, and the representation of aerosol properties, such as size distribution, chemical composition, refractive index, hygroscopicity parameter, and density, needs to be improved.
Samuel E. LeBlanc, Jens Redemann, Connor Flynn, Kristina Pistone, Meloë Kacenelenbogen, Michal Segal-Rosenheimer, Yohei Shinozuka, Stephen Dunagan, Robert P. Dahlgren, Kerry Meyer, James Podolske, Steven G. Howell, Steffen Freitag, Jennifer Small-Griswold, Brent Holben, Michael Diamond, Robert Wood, Paola Formenti, Stuart Piketh, Gillian Maggs-Kölling, Monja Gerber, and Andreas Namwoonde
Atmos. Chem. Phys., 20, 1565–1590, https://doi.org/10.5194/acp-20-1565-2020, https://doi.org/10.5194/acp-20-1565-2020, 2020
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The southeast Atlantic during August–October experiences layers of smoke from biomass burning over marine stratocumulus clouds. Here we present the light attenuation of the smoke and its dependence in the spatial, vertical, and spectral domain through direct measurements from an airborne platform during September 2016. From our observations of this climatically important smoke, we found an average aerosol optical depth of 0.32 at 500 nm, slightly lower than comparative satellite measurements.
Miguel Ricardo A. Hilario, Melliza T. Cruz, Maria Obiminda L. Cambaliza, Jeffrey S. Reid, Peng Xian, James B. Simpas, Nofel D. Lagrosas, Sherdon Niño Y. Uy, Steve Cliff, and Yongjing Zhao
Atmos. Chem. Phys., 20, 1255–1276, https://doi.org/10.5194/acp-20-1255-2020, https://doi.org/10.5194/acp-20-1255-2020, 2020
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The research apportions size-resolved aerosol contributions from the South China Sea during the Vasco research cruise in September 2011. As aerosols can affect precipitation rates and cloud formation, identifying sources is key to characterizing the region and developing our understanding of aerosol–cloud behavior. A strong biomass burning signal was identified using elemental particulate matter in the fine and ultrafine size ranges. Oil combustion, soil dust, and sea spray were also identified.
Jeremy E. Solbrig, Steven D. Miller, Jianglong Zhang, Lewis Grasso, and Anton Kliewer
Atmos. Meas. Tech., 13, 165–190, https://doi.org/10.5194/amt-13-165-2020, https://doi.org/10.5194/amt-13-165-2020, 2020
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New satellite sensors are able to view visible light, such as that emitted by cities, at night. It may be possible to use the light from cities to assess the amount of particulate matter in the atmosphere and the thickness of clouds. To do this we must understand how light emitted from the Earth's surface changes with time and viewing conditions. This study takes a step towards understanding the characteristics of light emitted by cities and its stability in time.
Pawan Gupta, Robert C. Levy, Shana Mattoo, Lorraine A. Remer, Robert E. Holz, and Andrew K. Heidinger
Atmos. Meas. Tech., 12, 6557–6577, https://doi.org/10.5194/amt-12-6557-2019, https://doi.org/10.5194/amt-12-6557-2019, 2019
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Aerosol optical depth (AOD) from a geostationary satellite has been retrieved, and validated and diurnal cycles of aerosols are discussed over the eastern hemisphere and a 2-month period of May–June 2016. The new AOD product matches well with AERONET as well as with the standard MODIS product. Future work to make this algorithm operational will need to re-examine masking including snow masks, re-evaluate assumed aerosol models for geosynchronous geometry and address the surface characterization.
Yan Yu, Olga V. Kalashnikova, Michael J. Garay, Huikyo Lee, Myungje Choi, Gregory S. Okin, John E. Yorks, and James R. Campbell
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-975, https://doi.org/10.5194/acp-2019-975, 2019
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Given the current uncertainties in the simulated diurnal variability of global dust mobilization and concentration, observational characterization of the variations in dust mobilization and concentration will provide a valuable benchmark for evaluating and constraining such model simulations. The current study investigates the diurnal cycle of dust loading across the global tropics, sub-tropics, and mid-latitudes by analyzing aerosol observations from the International Space Station.
Logan Lee, Jianglong Zhang, Jeffrey S. Reid, and John E. Yorks
Atmos. Chem. Phys., 19, 12687–12707, https://doi.org/10.5194/acp-19-12687-2019, https://doi.org/10.5194/acp-19-12687-2019, 2019
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The study of the diurnal variation of aerosol optical depth (AOD) and aerosol vertical distribution is necessary for the monitoring and modeling of aerosol particles for various air pollution, visibility and climate-related studies. Upon evaluating 1064 nm AOD and aerosol extinction profiles from the Cloud-Aerosol Transport System (CATS) level 2 aerosol product, we studied the diurnal variation of AOD and aerosol extinction profiles on both regional and global scales.
Joel S. Schafer, Tom F. Eck, Brent N. Holben, Kenneth L. Thornhill, Luke D. Ziemba, Patricia Sawamura, Richard H. Moore, Ilya Slutsker, Bruce E. Anderson, Alexander Sinyuk, David M. Giles, Alexander Smirnov, Andreas J. Beyersdorf, and Edward L. Winstead
Atmos. Meas. Tech., 12, 5289–5301, https://doi.org/10.5194/amt-12-5289-2019, https://doi.org/10.5194/amt-12-5289-2019, 2019
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Two independent datasets of column-integrated size distributions of atmospheric aerosols were compared during four 1-month regional campaigns from 2011 to 2014 in four US states. One set of measurements was from observations at multiple locations at the surface using retrievals from sun photometers, while the other relied on in situ aircraft sampling. These campaigns represent the most extensive comparison of AERONET size distributions with aircraft sampling of particle size on record.
Steven D. Miller, Louie D. Grasso, Qijing Bian, Sonia M. Kreidenweis, Jack F. Dostalek, Jeremy E. Solbrig, Jennifer Bukowski, Susan C. van den Heever, Yi Wang, Xiaoguang Xu, Jun Wang, Annette L. Walker, Ting-Chi Wu, Milija Zupanski, Christine Chiu, and Jeffrey S. Reid
Atmos. Meas. Tech., 12, 5101–5118, https://doi.org/10.5194/amt-12-5101-2019, https://doi.org/10.5194/amt-12-5101-2019, 2019
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Satellite–based detection of lofted mineral via infrared–window channels, well established in the literature, faces significant challenges in the presence of atmospheric moisture. Here, we consider a case featuring the juxtaposition of two dust plumes embedded within dry and moist air masses. The case is considered from the vantage points of numerical modeling, multi–sensor observations, and radiative transfer theory arriving at a new method for mitigating the water vapor masking effect.
Jonathan K. P. Shonk, Jui-Yuan Christine Chiu, Alexander Marshak, David M. Giles, Chiung-Huei Huang, Gerald G. Mace, Sally Benson, Ilya Slutsker, and Brent N. Holben
Atmos. Meas. Tech., 12, 5087–5099, https://doi.org/10.5194/amt-12-5087-2019, https://doi.org/10.5194/amt-12-5087-2019, 2019
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Retrievals of cloud optical depth made using AERONET radiometers in “cloud mode” rely on the assumption that all cloud is liquid. The presence of ice cloud therefore introduces errors in the retrieved optical depth, which can be over 25 in optically thick ice clouds. However, such clouds are not frequent and the long-term mean optical depth error is about 3 for a sample of real clouds. A correction equation could improve the retrieval further, although this would require extra instrumentation.
Jeffrey S. Reid, Derek J. Posselt, Kathleen Kaku, Robert A. Holz, Gao Chen, Edwin W. Eloranta, Ralph E. Kuehn, Sarah Woods, Jianglong Zhang, Bruce Anderson, T. Paul Bui, Glenn S. Diskin, Patrick Minnis, Michael J. Newchurch, Simone Tanelli, Charles R. Trepte, K. Lee Thornhill, and Luke D. Ziemba
Atmos. Chem. Phys., 19, 11413–11442, https://doi.org/10.5194/acp-19-11413-2019, https://doi.org/10.5194/acp-19-11413-2019, 2019
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The scientific community often focuses on the vertical transport of pollutants by clouds for those with bases at the planetary boundary layer (such as typical fair-weather cumulus) and the outflow from thunderstorms at their tops. We demonstrate complex aerosol and cloud features formed in mid-level thunderstorm outflow. These layers have strong relationships to mid-level tropospheric clouds, an important but difficult to model or monitor cloud regime for climate studies.
Myungje Choi, Hyunkwang Lim, Jhoon Kim, Seoyoung Lee, Thomas F. Eck, Brent N. Holben, Michael J. Garay, Edward J. Hyer, Pablo E. Saide, and Hongqing Liu
Atmos. Meas. Tech., 12, 4619–4641, https://doi.org/10.5194/amt-12-4619-2019, https://doi.org/10.5194/amt-12-4619-2019, 2019
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Satellite-based aerosol optical depth (AOD) products have been improved continuously and available from multiple low Earth orbit sensors, such as MODIS, MISR, and VIIRS, and geostationary sensors, such as GOCI and AHI, over East Asia. These multi-satellite AOD products are validated, intercompared, analyzed, and integrated to understand different characteristics, such as quality and spatio-temporal coverage, focused on several aerosol transportation cases during the 2016 KORUS-AQ campaign.
Huizheng Che, Ke Gui, Xiangao Xia, Yaqiang Wang, Brent N. Holben, Philippe Goloub, Emilio Cuevas-Agulló, Hong Wang, Yu Zheng, Hujia Zhao, and Xiaoye Zhang
Atmos. Chem. Phys., 19, 10497–10523, https://doi.org/10.5194/acp-19-10497-2019, https://doi.org/10.5194/acp-19-10497-2019, 2019
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A comprehensive assessment of the global and regional AOD trends over the past 37 years (1980–2016) is presented. AOD observations from both AERONET and CARSNET were used for the first time to assess the performance of the MERRA-2 AOD dataset on a global scale. Based on statistical models, we found the meteorological parameters explained a larger proportion of the regional AOD variability (20.4 %–2.8 %) when compared with emission factors (0 %%–56 %).
Stephen M. Saleeby, Susan C. van den Heever, Jennie Bukowski, Annette L. Walker, Jeremy E. Solbrig, Samuel A. Atwood, Qijing Bian, Sonia M. Kreidenweis, Yi Wang, Jun Wang, and Steven D. Miller
Atmos. Chem. Phys., 19, 10279–10301, https://doi.org/10.5194/acp-19-10279-2019, https://doi.org/10.5194/acp-19-10279-2019, 2019
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This study seeks to understand how intense dust storms impact the heating and cooling of the land surface and atmosphere. Dust storms that are intense enough to substantially impact visibility can also alter how much sunlight reaches the surface during the day and how much heat is trapped in the atmosphere at night. These radiation changes can impact the temperature of the atmosphere and impact the weather in the vicinity.
Xiaoguang Xu, Jun Wang, Yi Wang, Jing Zeng, Omar Torres, Jeffrey S. Reid, Steven D. Miller, J. Vanderlei Martins, and Lorraine A. Remer
Atmos. Meas. Tech., 12, 3269–3288, https://doi.org/10.5194/amt-12-3269-2019, https://doi.org/10.5194/amt-12-3269-2019, 2019
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Detecting aerosol layer height from space is challenging. The traditional method relies on active sensors such as lidar that provide the detailed vertical structure of the aerosol profile but is costly with limited spatial coverage (more than 1 year is needed for global coverage). Here we developed a passive remote sensing technique that uses backscattered sunlight to retrieve smoke aerosol layer height over both water and vegetated surfaces from a sensor 1.5 million kilometers from the Earth.
Jianglong Zhang, Shawn L. Jaker, Jeffrey S. Reid, Steven D. Miller, Jeremy Solbrig, and Travis D. Toth
Atmos. Meas. Tech., 12, 3209–3222, https://doi.org/10.5194/amt-12-3209-2019, https://doi.org/10.5194/amt-12-3209-2019, 2019
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Using nighttime observations from the Visible Infrared Imager Radiometer Suite (VIIRS) Day/Night band (DNB), the characteristics of artificial light sources are evaluated as functions of observation conditions, and incremental improvements are documented on nighttime aerosol retrievals on a regional scale. Results from the study indicate the potential of this method to begin filling critical gaps in diurnal aerosol optical thickness information at both regional and global scales.
Travis D. Toth, Jianglong Zhang, Jeffrey S. Reid, and Mark A. Vaughan
Atmos. Meas. Tech., 12, 1739–1754, https://doi.org/10.5194/amt-12-1739-2019, https://doi.org/10.5194/amt-12-1739-2019, 2019
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An innovative method is presented for deriving particulate matter (PM) concentrations using CALIOP measurements. Deviating from conventional approaches of relying on passive satellite column-integrated aerosol measurements, PM concentrations are derived from near-surface CALIOP measurements through a bulk-mass-modeling method. This proof-of-concept study shows that, while limited in spatial and temporal coverage, CALIOP exhibits reasonable skill for PM applications.
David M. Giles, Alexander Sinyuk, Mikhail G. Sorokin, Joel S. Schafer, Alexander Smirnov, Ilya Slutsker, Thomas F. Eck, Brent N. Holben, Jasper R. Lewis, James R. Campbell, Ellsworth J. Welton, Sergey V. Korkin, and Alexei I. Lyapustin
Atmos. Meas. Tech., 12, 169–209, https://doi.org/10.5194/amt-12-169-2019, https://doi.org/10.5194/amt-12-169-2019, 2019
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Clouds or instrumental anomalies may perturb ground-based solar measurements used to calculate aerosol optical depth (AOD). This study presents a new algorithm of automated near-real-time (NRT) quality controls with improved cloud screening for AERONET AOD measurements. Results from the new and old algorithms have excellent agreement for the highest-quality AOD level, while the new algorithm provides higher-quality NRT AOD for applications such as data assimilation and satellite evaluation.
Yingxi R. Shi, Robert C. Levy, Thomas F. Eck, Brad Fisher, Shana Mattoo, Lorraine A. Remer, Ilya Slutsker, and Jianglong Zhang
Atmos. Chem. Phys., 19, 259–274, https://doi.org/10.5194/acp-19-259-2019, https://doi.org/10.5194/acp-19-259-2019, 2019
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The Indonesian fire and smoke event of 2015 was an extreme episode that affected public health and caused severe economic and environmental damage. We managed to retrieve data over very thick smoke plumes and produce a lot more high aerosol loading data that were previously missed by other satellite products. These results will benefit varieties of downstream research that use the satellite aerosol data and will influence the future development of the global satellite aerosol algorithm.
Mayra I. Oyola, James R. Campbell, Peng Xian, Anthony Bucholtz, Richard A. Ferrare, Sharon P. Burton, Olga Kalashnikova, Benjamin C. Ruston, and Simone Lolli
Atmos. Chem. Phys., 19, 205–218, https://doi.org/10.5194/acp-19-205-2019, https://doi.org/10.5194/acp-19-205-2019, 2019
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We conceptualized the aerosol radiative impact of an inline aerosol analysis field coupled with a global meteorological forecast system utilizing NAAPS and NAVGEM analysis and surface albedo fields. Model simulations were compared with in situ validation data collected during the NASA 2013 SEAC4RS experiment. Instantaneous heating rates peaked around 7 K day-1 in the lower part of the troposphere, while the HSRL profiles resulted in values of up to 18 K day-1 in the in the mid-troposphere.
Carlos Toledano, Ramiro González, David Fuertes, Emilio Cuevas, Thomas F. Eck, Stelios Kazadzis, Natalia Kouremeti, Julian Gröbner, Philippe Goloub, Luc Blarel, Roberto Román, África Barreto, Alberto Berjón, Brent N. Holben, and Victoria E. Cachorro
Atmos. Chem. Phys., 18, 14555–14567, https://doi.org/10.5194/acp-18-14555-2018, https://doi.org/10.5194/acp-18-14555-2018, 2018
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Most of the ground-based radiometric networks have their reference instruments and/or calibrate them at Mauna Loa or Izaña. The suitability of these high-mountain stations for absolute radiometric calibrations is investigated with the support of 20 years of first-class Sun photometer data from the AERONET and GAW-PFR networks. We analyze the number of calibration days at each site in a climatological sense and investigate the uncertainty of the calibrations based on long-term statistics.
Alexa D. Ross, Robert E. Holz, Gregory Quinn, Jeffrey S. Reid, Peng Xian, F. Joseph Turk, and Derek J. Posselt
Atmos. Chem. Phys., 18, 12747–12764, https://doi.org/10.5194/acp-18-12747-2018, https://doi.org/10.5194/acp-18-12747-2018, 2018
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This paper explores how clouds and aerosols interact over Southeast Asia. We introduce a new collocated dataset called the Curtain Cloud-Aerosol Regional A-Train (CCARA) product. CCARA is special because it combines satellite observations with model reanalysis. We find that increased aerosol corresponds to smaller observed liquid cloud droplets in some areas. Other areas experienced little to no change in effective radius (droplet size) when aerosol amount increased.
Angela Benedetti, Jeffrey S. Reid, Peter Knippertz, John H. Marsham, Francesca Di Giuseppe, Samuel Rémy, Sara Basart, Olivier Boucher, Ian M. Brooks, Laurent Menut, Lucia Mona, Paolo Laj, Gelsomina Pappalardo, Alfred Wiedensohler, Alexander Baklanov, Malcolm Brooks, Peter R. Colarco, Emilio Cuevas, Arlindo da Silva, Jeronimo Escribano, Johannes Flemming, Nicolas Huneeus, Oriol Jorba, Stelios Kazadzis, Stefan Kinne, Thomas Popp, Patricia K. Quinn, Thomas T. Sekiyama, Taichu Tanaka, and Enric Terradellas
Atmos. Chem. Phys., 18, 10615–10643, https://doi.org/10.5194/acp-18-10615-2018, https://doi.org/10.5194/acp-18-10615-2018, 2018
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Numerical prediction of aerosol particle properties has become an important activity at many research and operational weather centers. This development is due to growing interest from a diverse set of stakeholders, such as air quality regulatory bodies, aviation authorities, solar energy plant managers, climate service providers, and health professionals. This paper describes the advances in the field and sets out requirements for observations for the sustainability of these activities.
Jungbin Mok, Nickolay A. Krotkov, Omar Torres, Hiren Jethva, Zhanqing Li, Jhoon Kim, Ja-Ho Koo, Sujung Go, Hitoshi Irie, Gordon Labow, Thomas F. Eck, Brent N. Holben, Jay Herman, Robert P. Loughman, Elena Spinei, Seoung Soo Lee, Pradeep Khatri, and Monica Campanelli
Atmos. Meas. Tech., 11, 2295–2311, https://doi.org/10.5194/amt-11-2295-2018, https://doi.org/10.5194/amt-11-2295-2018, 2018
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Measuring aerosol absorption from the shortest ultraviolet (UV) to the near-infrared (NIR) wavelengths is important for studies of climate, tropospheric photochemistry, human health, and agricultural productivity. We estimate the accuracy and demonstrate consistency of aerosol absorption retrievals from different instruments, after accounting for spectrally varying surface albedo and gaseous absorption.
Simone Lolli, Fabio Madonna, Marco Rosoldi, James R. Campbell, Ellsworth J. Welton, Jasper R. Lewis, Yu Gu, and Gelsomina Pappalardo
Atmos. Meas. Tech., 11, 1639–1651, https://doi.org/10.5194/amt-11-1639-2018, https://doi.org/10.5194/amt-11-1639-2018, 2018
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We evaluate the comparability of aerosol and cloud vertically resolved optical properties obtained with varying lidar profiling techniques and/or data processing methodologies. The discrepancies are assessed by evaluating climate-sensitive direct radiative effects, computed by radiative transfer code means. Results show important discrepancies up to 0.8 W m−2 due to lidar data smoothing in cirrus clouds and a 0.05 W m−2 difference between Raman and elastic lidar technique on a dust layer aloft.
Travis D. Toth, James R. Campbell, Jeffrey S. Reid, Jason L. Tackett, Mark A. Vaughan, Jianglong Zhang, and Jared W. Marquis
Atmos. Meas. Tech., 11, 499–514, https://doi.org/10.5194/amt-11-499-2018, https://doi.org/10.5194/amt-11-499-2018, 2018
Brent N. Holben, Jhoon Kim, Itaru Sano, Sonoyo Mukai, Thomas F. Eck, David M. Giles, Joel S. Schafer, Aliaksandr Sinyuk, Ilya Slutsker, Alexander Smirnov, Mikhail Sorokin, Bruce E. Anderson, Huizheng Che, Myungje Choi, James H. Crawford, Richard A. Ferrare, Michael J. Garay, Ukkyo Jeong, Mijin Kim, Woogyung Kim, Nichola Knox, Zhengqiang Li, Hwee S. Lim, Yang Liu, Hal Maring, Makiko Nakata, Kenneth E. Pickering, Stuart Piketh, Jens Redemann, Jeffrey S. Reid, Santo Salinas, Sora Seo, Fuyi Tan, Sachchida N. Tripathi, Owen B. Toon, and Qingyang Xiao
Atmos. Chem. Phys., 18, 655–671, https://doi.org/10.5194/acp-18-655-2018, https://doi.org/10.5194/acp-18-655-2018, 2018
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Aerosol particles, such as smoke, vary over space and time. This paper describes a series of very high-resolution ground-based aerosol measurement networks and associated studies that contributed new understanding of aerosol processes and detailed comparisons to satellite aerosol validation. Significantly, these networks also provide an opportunity to statistically relate grab samples of an aerosol parameter to companion satellite observations, a step toward air quality assessment from space.
Myungje Choi, Jhoon Kim, Jaehwa Lee, Mijin Kim, Young-Je Park, Brent Holben, Thomas F. Eck, Zhengqiang Li, and Chul H. Song
Atmos. Meas. Tech., 11, 385–408, https://doi.org/10.5194/amt-11-385-2018, https://doi.org/10.5194/amt-11-385-2018, 2018
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This study is a major version upgrade of the aerosol product from GOCI, the first and unique ocean color imager in geostationary earth orbit. It describes the improvement of version 2 of the GOCI Yonsei aerosol retrieval algorithm for near-real-time processing with improved accuracy from the modification of cloud masking, surface reflectance, etc. The product is validated against AERONET/SONET over East Asia with analyses of various errors features, and a pixel-level uncertainty is calculated.
Ricardo Alfaro-Contreras, Jianglong Zhang, Jeffrey S. Reid, and Sundar Christopher
Atmos. Chem. Phys., 17, 13849–13868, https://doi.org/10.5194/acp-17-13849-2017, https://doi.org/10.5194/acp-17-13849-2017, 2017
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Using near-full data records of Terra and Aqua MODIS and MISR data, we have evaluated aerosol optical depth trends over global oceans (MODIS and MISR) and land (MISR). Also, for the first time, shortwave aerosol radiative effect (SWARE) trends are estimated over global oceans with the combined use of observations from MODIS and CERES.
Chaeyoon Cho, Sang-Woo Kim, Maheswar Rupakheti, Jin-Soo Park, Arnico Panday, Soon-Chang Yoon, Ji-Hyoung Kim, Hyunjae Kim, Haeun Jeon, Minyoung Sung, Bong Mann Kim, Seungkyu K. Hong, Rokjin J. Park, Dipesh Rupakheti, Khadak Singh Mahata, Puppala Siva Praveen, Mark G. Lawrence, and Brent Holben
Atmos. Chem. Phys., 17, 12617–12632, https://doi.org/10.5194/acp-17-12617-2017, https://doi.org/10.5194/acp-17-12617-2017, 2017
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We investigated the optical and chemical properties and direct radiative effects of aerosols in the Kathmandu Valley. We concluded that the ratio of light-absorbing to scattering aerosols as well as the concentration of light-absorbing aerosols is much higher at Kathmandu than other comparable regions, and it contributes to a great atmospheric absorption efficiency. This study provides unprecedented insights into aerosol optical properties and their radiative forcings in the Kathmandu Valley.
Longtao Wu, Hui Su, Olga V. Kalashnikova, Jonathan H. Jiang, Chun Zhao, Michael J. Garay, James R. Campbell, and Nanpeng Yu
Atmos. Chem. Phys., 17, 7291–7309, https://doi.org/10.5194/acp-17-7291-2017, https://doi.org/10.5194/acp-17-7291-2017, 2017
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The WRF-Chem simulation successfully captures aerosol variations in the cold season in the San Joaquin Valley (SJV) but has poor performance in the warm season. High-resolution model simulation can better resolve nonhomogeneous distribution of anthropogenic emissions in urban areas, resulting in better simulation of aerosols in the cold season in the SJV. Poor performance of the WRF-Chem model in the warm season in the SJV is mainly due to misrepresentation of dust emission and vertical mixing.
Simone Lolli, James R. Campbell, Jasper R. Lewis, Yu Gu, and Ellsworth J. Welton
Atmos. Chem. Phys., 17, 7025–7034, https://doi.org/10.5194/acp-17-7025-2017, https://doi.org/10.5194/acp-17-7025-2017, 2017
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We compare net TOA radiative forcing between the simplified Corti–Peter (CP) and relatively complex Fu–Liou–Gu models for cirrus clouds observed by NASA MPLNET at Singapore in 2010–11 and Greenbelt, Maryland, in 2012. We find daytime forcing discrepancies up to 65 % between the two, which is greater than previous studies. In some cases, the sign of net TOA daytime forcing also differs. We attribute model differences to numerical simplifications in CP via regression that are not valid globally.
Andrew M. Sayer, N. Christina Hsu, Corey Bettenhausen, Robert E. Holz, Jaehwa Lee, Greg Quinn, and Paolo Veglio
Atmos. Meas. Tech., 10, 1425–1444, https://doi.org/10.5194/amt-10-1425-2017, https://doi.org/10.5194/amt-10-1425-2017, 2017
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The satellite instrument VIIRS is being used to carry on observations of the Earth made by older satellites like MODIS. Data sets created from these satellite observations depend on the quality of the satellite instruments' calibration. This paper describes a comparison between the calibration of these two sensors. MODIS is believed to be more reliable and so VIIRS is corrected to bring it in line with MODIS. These corrections are shown to improve the quality of VIIRS aerosol data.
Jennie Bukowski, Derek J. Posselt, Jeffrey S. Reid, and Samuel A. Atwood
Atmos. Chem. Phys., 17, 4611–4626, https://doi.org/10.5194/acp-17-4611-2017, https://doi.org/10.5194/acp-17-4611-2017, 2017
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The Maritime Continent (MC) exhibits tremendous meteorological variability. In this study, multiple years of atmospheric soundings over the MC are analyzed to identify key sources of variability in the region's temperature, water vapor, and wind structure. Coherent vertical structures are found among profiles sampled from different geographic locations. The results indicate that the complex meteorology of the region can be described using a few simple structure functions.
Samuel A. Atwood, Jeffrey S. Reid, Sonia M. Kreidenweis, Donald R. Blake, Haflidi H. Jonsson, Nofel D. Lagrosas, Peng Xian, Elizabeth A. Reid, Walter R. Sessions, and James B. Simpas
Atmos. Chem. Phys., 17, 1105–1123, https://doi.org/10.5194/acp-17-1105-2017, https://doi.org/10.5194/acp-17-1105-2017, 2017
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Aerosol particles were measured by ship in remote marine regions of the South China Sea as part of the 2012 7 Southeast Asian Studies (7SEAS) experiments. As the particle populations changed throughout the experiment, the distribution of particle sizes and the amount of water that collected on them changed as well. These changes were associated with various impacts from smoke, sea salt, and pollution sources, and impact how clouds form and precipitation occurs in the region.
Tatiana B. Zhuravleva, Dmitriy M. Kabanov, Ilmir M. Nasrtdinov, Tatiana V. Russkova, Sergey M. Sakerin, Alexander Smirnov, and Brent N. Holben
Atmos. Meas. Tech., 10, 179–198, https://doi.org/10.5194/amt-10-179-2017, https://doi.org/10.5194/amt-10-179-2017, 2017
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Aerosol properties were studied during a mega-fire event in summer 2012 over Siberia using ground-based measurements of spectral solar radiation at the AERONET site in Tomsk and satellite observations. The data were analysed using multi-year measurements under background conditions and yearly observed wildfires. It is shown that the aerosol radiation characteristics during individual severe fires differ significantly from the ensemble smoke hazes which are typical for the Siberian region.
Itaru Sano, Sonoyo Mukai, Makiko Nakata, and Brent N. Holben
Atmos. Chem. Phys., 16, 14795–14803, https://doi.org/10.5194/acp-16-14795-2016, https://doi.org/10.5194/acp-16-14795-2016, 2016
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We investigated the regional and local variation of aerosols based on large and small gridded sun photometer networks. The results show that long-range transboundary aerosols strongly affect aerosol condition over Japan even at a small island in the East China Sea. A dense instrument network (DRAGON) reveals the magnitude and variation of local aerosols.
Eleonora Aruffo, Fabio Biancofiore, Piero Di Carlo, Marcella Busilacchio, Marco Verdecchia, Barbara Tomassetti, Cesare Dari-Salisburgo, Franco Giammaria, Stephane Bauguitte, James Lee, Sarah Moller, James Hopkins, Shalini Punjabi, Stephen J. Andrews, Alistair C. Lewis, Paul I. Palmer, Edward Hyer, Michael Le Breton, and Carl Percival
Atmos. Meas. Tech., 9, 5591–5606, https://doi.org/10.5194/amt-9-5591-2016, https://doi.org/10.5194/amt-9-5591-2016, 2016
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During the BORTAS aircraft campaign, we measured NO2 and their oxidtation products (as peroxy nitrates) with a custom laser-induced fluorescence instrument. Because of the high correlation between known pyrogenic tracers (i.e., carbon monoxide) and peroxy nitrates, we provide two methods to use these species for the identification of biomass burning (BB) plumes. Using an artifical neural network, we improved the BB identification taking into account of a meteorological parameter (pressure).
Jeffrey S. Reid, Nofel D. Lagrosas, Haflidi H. Jonsson, Elizabeth A. Reid, Samuel A. Atwood, Thomas J. Boyd, Virendra P. Ghate, Peng Xian, Derek J. Posselt, James B. Simpas, Sherdon N. Uy, Kimo Zaiger, Donald R. Blake, Anthony Bucholtz, James R. Campbell, Boon Ning Chew, Steven S. Cliff, Brent N. Holben, Robert E. Holz, Edward J. Hyer, Sonia M. Kreidenweis, Arunas P. Kuciauskas, Simone Lolli, Min Oo, Kevin D. Perry, Santo V. Salinas, Walter R. Sessions, Alexander Smirnov, Annette L. Walker, Qing Wang, Liya Yu, Jianglong Zhang, and Yongjing Zhao
Atmos. Chem. Phys., 16, 14057–14078, https://doi.org/10.5194/acp-16-14057-2016, https://doi.org/10.5194/acp-16-14057-2016, 2016
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This paper describes aspects of the 2012 7 Southeast Asian Studies (7SEAS) operations period, the largest within the Maritime Continent. Included were an enhanced deployment of Aerosol Robotic Network (AERONET) sun photometers, multiple lidars, and a Singapore supersite. Simultaneously, a ship was dispatched to the Palawan Archipelago and Sulu Sea of the Philippines for September 2012 to observe transported smoke and pollution as it entered the southwest monsoon trough.
Graydon Snider, Crystal L. Weagle, Kalaivani K. Murdymootoo, Amanda Ring, Yvonne Ritchie, Emily Stone, Ainsley Walsh, Clement Akoshile, Nguyen Xuan Anh, Rajasekhar Balasubramanian, Jeff Brook, Fatimah D. Qonitan, Jinlu Dong, Derek Griffith, Kebin He, Brent N. Holben, Ralph Kahn, Nofel Lagrosas, Puji Lestari, Zongwei Ma, Amit Misra, Leslie K. Norford, Eduardo J. Quel, Abdus Salam, Bret Schichtel, Lior Segev, Sachchida Tripathi, Chien Wang, Chao Yu, Qiang Zhang, Yuxuan Zhang, Michael Brauer, Aaron Cohen, Mark D. Gibson, Yang Liu, J. Vanderlei Martins, Yinon Rudich, and Randall V. Martin
Atmos. Chem. Phys., 16, 9629–9653, https://doi.org/10.5194/acp-16-9629-2016, https://doi.org/10.5194/acp-16-9629-2016, 2016
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We examine the chemical composition of fine particulate matter (PM2.5) collected on filters at traditionally undersampled, globally dispersed urban locations. Several PM2.5 chemical components (e.g. ammonium sulfate, ammonium nitrate, and black carbon) vary by more than an order of magnitude between sites while aerosol hygroscopicity varies by a factor of 2. Enhanced anthropogenic dust fractions in large urban areas are apparent from high Zn : Al ratios.
Jianglong Zhang, Jeffrey S. Reid, Matthew Christensen, and Angela Benedetti
Atmos. Chem. Phys., 16, 6475–6494, https://doi.org/10.5194/acp-16-6475-2016, https://doi.org/10.5194/acp-16-6475-2016, 2016
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Through analyzing a smoke aerosol event over the Midwestern USA, the potential impacts of aerosol particles on model/weather-station-forecasted surface temperatures are studied, and for the first time, smoke-aerosol-induced surface cooling is investigated as a function of observed aerosol properties and multiple operational models over a large network of ground stations. The potential issues of incorporating aerosol models into weather models for forecasting surface temperatures are explored.
Robert E. Holz, Steven Platnick, Kerry Meyer, Mark Vaughan, Andrew Heidinger, Ping Yang, Gala Wind, Steven Dutcher, Steven Ackerman, Nandana Amarasinghe, Fredrick Nagle, and Chenxi Wang
Atmos. Chem. Phys., 16, 5075–5090, https://doi.org/10.5194/acp-16-5075-2016, https://doi.org/10.5194/acp-16-5075-2016, 2016
Peng Lynch, Jeffrey S. Reid, Douglas L. Westphal, Jianglong Zhang, Timothy F. Hogan, Edward J. Hyer, Cynthia A. Curtis, Dean A. Hegg, Yingxi Shi, James R. Campbell, Juli I. Rubin, Walter R. Sessions, F. Joseph Turk, and Annette L. Walker
Geosci. Model Dev., 9, 1489–1522, https://doi.org/10.5194/gmd-9-1489-2016, https://doi.org/10.5194/gmd-9-1489-2016, 2016
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An 11-year, 1-degree aerosol reanalysis is presented for use in studies of aerosol effects on climate and atmospheric processes. The reanalysis uses the Navy Aerosol Analysis and Prediction System, constrained by aerosol optical thickness (AOT) data from NASA sensors. Fine and coarse mode AOT at 550 nm agrees well with ground-based measurements, and reproduces the decadal AOT trends found using standalone satellite products. This dataset is a resource for basic and applied science research.
Kerry Meyer, Steven Platnick, G. Thomas Arnold, Robert E. Holz, Paolo Veglio, John Yorks, and Chenxi Wang
Atmos. Meas. Tech., 9, 1743–1753, https://doi.org/10.5194/amt-9-1743-2016, https://doi.org/10.5194/amt-9-1743-2016, 2016
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Cirrus cloud optical and microphysical properties are retrieved from remote sensing solar reflectance measurements at two narrow wavelength channels within the broader water vapor absorption band at 1.88 µm. Results from this technique compare well with other solar reflectance, IR, and lidar-based retrievals. This approach is complementary to traditional remote sensing techniques and can extend cloud retrieval capabilities for thin cirrus clouds.
Makiko Nakata, Itaru Sano, Sonoyo Mukai, and Brent N. Holben
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-182, https://doi.org/10.5194/acp-2016-182, 2016
Revised manuscript not accepted
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We document the spatial and temporal variations of atmospheric aerosols in East Asia, specifically focusing on the NASA/AERONET-Osaka site in March 2012 during the AERONET “DRAGON-Japan” campaign. It has been shown that airborne pollutants can influence both the local atmosphere near to their source and relatively remote locations due to long-range transportation.
Myungje Choi, Jhoon Kim, Jaehwa Lee, Mijin Kim, Young-Je Park, Ukkyo Jeong, Woogyung Kim, Hyunkee Hong, Brent Holben, Thomas F. Eck, Chul H. Song, Jae-Hyun Lim, and Chang-Keun Song
Atmos. Meas. Tech., 9, 1377–1398, https://doi.org/10.5194/amt-9-1377-2016, https://doi.org/10.5194/amt-9-1377-2016, 2016
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The Geostationary Ocean Color Imager (GOCI) is the first ocean color sensor in geostationary orbit. It enables hourly aerosol optical properties to be observed in high spatial resolution. This study presents improvements of the GOCI Yonsei Aerosol Retrieval (YAER) algorithm and its validation results using ground-based and other satellite-based observation products during DRAGON-NE Asia 2012 Campaign. Retrieval errors are also analyzed according to various factors through the validation studies.
Juli I. Rubin, Jeffrey S. Reid, James A. Hansen, Jeffrey L. Anderson, Nancy Collins, Timothy J. Hoar, Timothy Hogan, Peng Lynch, Justin McLay, Carolyn A. Reynolds, Walter R. Sessions, Douglas L. Westphal, and Jianglong Zhang
Atmos. Chem. Phys., 16, 3927–3951, https://doi.org/10.5194/acp-16-3927-2016, https://doi.org/10.5194/acp-16-3927-2016, 2016
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This work tests the use of an ensemble prediction system for aerosol forecasting, including an ensemble adjustment Kalman filter for MODIS AOT assimilation. Key findings include (1) meteorology and source-perturbed ensembles are needed to capture long-range transport and near-source aerosol events, (2) adaptive covariance inflation is recommended for assimilating spatially heterogeneous observations and (3) the ensemble system captures sharp gradients relative to a deterministic/variational system.
Anatoli Chaikovsky, Oleg Dubovik, Brent Holben, Andrey Bril, Philippe Goloub, Didier Tanré, Gelsomina Pappalardo, Ulla Wandinger, Ludmila Chaikovskaya, Sergey Denisov, Jan Grudo, Anton Lopatin, Yana Karol, Tatsiana Lapyonok, Vassilis Amiridis, Albert Ansmann, Arnoud Apituley, Lucas Allados-Arboledas, Ioannis Binietoglou, Antonella Boselli, Giuseppe D'Amico, Volker Freudenthaler, David Giles, María José Granados-Muñoz, Panayotis Kokkalis, Doina Nicolae, Sergey Oshchepkov, Alex Papayannis, Maria Rita Perrone, Alexander Pietruczuk, Francesc Rocadenbosch, Michaël Sicard, Ilya Slutsker, Camelia Talianu, Ferdinando De Tomasi, Alexandra Tsekeri, Janet Wagner, and Xuan Wang
Atmos. Meas. Tech., 9, 1181–1205, https://doi.org/10.5194/amt-9-1181-2016, https://doi.org/10.5194/amt-9-1181-2016, 2016
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This paper presents a detailed description of LIRIC (LIdar-Radiometer Inversion Code) algorithm for simultaneous processing of coincident lidar and radiometric observations for the retrieval of the aerosol concentrations. As the lidar/radiometric input data we use measurements from European Aerosol Research Lidar Network (EARLINET) lidars and collocated sun-photometers of Aerosol Robotic Network (AERONET). The LIRIC software package was implemented and tested at a number of EARLINET stations.
Marcella Busilacchio, Piero Di Carlo, Eleonora Aruffo, Fabio Biancofiore, Cesare Dari Salisburgo, Franco Giammaria, Stephane Bauguitte, James Lee, Sarah Moller, James Hopkins, Shalini Punjabi, Stephen Andrews, Alistair C. Lewis, Mark Parrington, Paul I. Palmer, Edward Hyer, and Glenn M. Wolfe
Atmos. Chem. Phys., 16, 3485–3497, https://doi.org/10.5194/acp-16-3485-2016, https://doi.org/10.5194/acp-16-3485-2016, 2016
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Boreal fire emissions have little effect on ozone concentrations but evident impact on some NOx reservoirs as peroxy nitrates that we quantified. This should be taken into account since NOx reservoirs can be efficiently transported and may influence the ozone budget far away from the fire emission.
The study is based on observations carried out on board the BAe 146 aircraft during BORTAS in Canada. We used a custom laser-induced fluorescence system to measure NO2 and NOx reservoirs.
África Barreto, Emilio Cuevas, María-José Granados-Muñoz, Lucas Alados-Arboledas, Pedro M. Romero, Julian Gröbner, Natalia Kouremeti, Antonio F. Almansa, Tom Stone, Carlos Toledano, Roberto Román, Mikhail Sorokin, Brent Holben, Marius Canini, and Margarita Yela
Atmos. Meas. Tech., 9, 631–654, https://doi.org/10.5194/amt-9-631-2016, https://doi.org/10.5194/amt-9-631-2016, 2016
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This paper presents the new photometer CE318-T, able to perform daytime and
night-time photometric measurements using the sun and the moon as light
sources. This new device permits a complete cycle of diurnal aerosol and water vapour measurements to be extracted, valuable to enhance atmospheric monitoring. We have also highlighted the ability of this new device to capture short-term atmospheric variations, critical for climate studies.
M. Kim, J. Kim, U. Jeong, W. Kim, H. Hong, B. Holben, T. F. Eck, J. H. Lim, C. K. Song, S. Lee, and C.-Y. Chung
Atmos. Chem. Phys., 16, 1789–1808, https://doi.org/10.5194/acp-16-1789-2016, https://doi.org/10.5194/acp-16-1789-2016, 2016
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An aerosol model optimized for East Asia is improved by applying inversion data from the DRAGON-NE Asia 2012 campaign, and is applied to an AOD retrieval algorithm using single visible measurements from a GEO satellite. In sensitivity tests, a 4 % overestimation in SSA can cause an underestimation in AOD of over 20 %. In accordance with the test, the overestimating tendency of AOD was improved by 8 % after the modification of the aerosol model.
G. L. Schuster, O. Dubovik, A. Arola, T. F. Eck, and B. N. Holben
Atmos. Chem. Phys., 16, 1587–1602, https://doi.org/10.5194/acp-16-1587-2016, https://doi.org/10.5194/acp-16-1587-2016, 2016
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Some authors have recently suggested that the spectral dependence of aerosol absorption may be used to separate soot carbon absorption from the aerosol absorption associated with organic carbon and dust. We demonstrate that this approach is inconsistent with the underlying assumptions that are required to infer aerosol absorption through remote sensing techniques, and that carbonaceous aerosols can not be differentiated from dust by exclusively using spectral absorption signatures.
Q. Xiao, H. Zhang, M. Choi, S. Li, S. Kondragunta, J. Kim, B. Holben, R. C. Levy, and Y. Liu
Atmos. Chem. Phys., 16, 1255–1269, https://doi.org/10.5194/acp-16-1255-2016, https://doi.org/10.5194/acp-16-1255-2016, 2016
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Using ground AOD measurements from AERONET, DRAGON-Asia Campaign, and handheld sunphotometers, we evaluated emerging aerosol products from VIIRS, GOCI, and Terra and Aqua MODIS (Collection 6) in East Asia in 2012–2013. We found that satellite aerosol products performed better in tracking the day-to-day variability than the high-resolution spatial variability. VIIRS EDR and GOCI products provided the most accurate AOD retrievals, while VIIRS IP and MODIS C6 3 km products had positive biases.
U. Jeong, J. Kim, C. Ahn, O. Torres, X. Liu, P. K. Bhartia, R. J. D. Spurr, D. Haffner, K. Chance, and B. N. Holben
Atmos. Chem. Phys., 16, 177–193, https://doi.org/10.5194/acp-16-177-2016, https://doi.org/10.5194/acp-16-177-2016, 2016
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An aerosol retrieval and error analysis algorithm using OMI measurements based on an optimal-estimation method was developed in this study. The aerosol retrievals were validated using the DRAGON campaign products. The estimated errors of the retrievals represented the actual biases between retrieval and AERONET measurements well. The retrievals, with their estimated uncertainties, are expected to be valuable for relevant studies, such as trace gas retrieval and data assimilation.
R. Alfaro-Contreras, J. Zhang, J. R. Campbell, and J. S. Reid
Atmos. Chem. Phys., 16, 47–69, https://doi.org/10.5194/acp-16-47-2016, https://doi.org/10.5194/acp-16-47-2016, 2016
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The spatial distributions and trends of above-cloud aerosol (ACA) events are studied using seven and a half years of MODIS, OMI, and CALIOP data. The active- (CALIOP) and passive-based (MODIS-OMI) methods have their advantages and caveats, and thus both are used to get a thorough and robust comparison of ACA distribution and climatology. For the first time, baseline above-cloud CALIOP aerosol optical depth and OMI aerosol index thresholds are derived and examined for each sensor.
T. M. McHardy, J. Zhang, J. S. Reid, S. D. Miller, E. J. Hyer, and R. E. Kuehn
Atmos. Meas. Tech., 8, 4773–4783, https://doi.org/10.5194/amt-8-4773-2015, https://doi.org/10.5194/amt-8-4773-2015, 2015
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Using Visible Infrared Imaging Radiometer Suite (VIIRS) Day/Night Band (DNB) data, a new method is developed for retrieving nighttime aerosol optical thickness values through the examination of the dispersion of radiance values above an artificial light source. Preliminary results suggest that artificial light sources can be used for estimating regional and global nighttime aerosol distributions in the future.
R. C. Levy, L. A. Munchak, S. Mattoo, F. Patadia, L. A. Remer, and R. E. Holz
Atmos. Meas. Tech., 8, 4083–4110, https://doi.org/10.5194/amt-8-4083-2015, https://doi.org/10.5194/amt-8-4083-2015, 2015
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Aerosol optical depth (AOD) is an essential climate variable, so we seek to create a long-term AOD record. From MODIS, we have 15+ years, which we want to continue with VIIRS. Accounting for instrumental difference, we have developed a MODIS-like algorithm for VIIRS, and applied it to overlapping 2-year time period. In general, the two data sets are similar, except for VIIRS being high-biased over ocean. We discuss the impacts of calibration, resolution, and sampling on the results.
A. Chandra, C. Zhang, P. Kollias, S. Matrosov, and W. Szyrmer
Atmos. Meas. Tech., 8, 3685–3699, https://doi.org/10.5194/amt-8-3685-2015, https://doi.org/10.5194/amt-8-3685-2015, 2015
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An automated algorithm is developed for routinely retrieving rain rates from the profiling Ka-Band zenith radars. The algorithm is implemented in two steps: higher rain rates are retrieved by using the amount of attenuation in rain layers, while low rain rates are retrieved from the reflectivity-rain rate (Ze-R) relation. Observations collected by rain gauge, disdrometer and scanning precipitation radars during the DYNAMO field campaign at Gan Island are used to validate the proposed approach.
E. P. Nowottnick, P. R. Colarco, E. J. Welton, and A. da Silva
Atmos. Meas. Tech., 8, 3647–3669, https://doi.org/10.5194/amt-8-3647-2015, https://doi.org/10.5194/amt-8-3647-2015, 2015
D. Pérez-Ramírez, I. Veselovskii, D. N. Whiteman, A. Suvorina, M. Korenskiy, A. Kolgotin, B. Holben, O. Dubovik, A. Siniuk, and L. Alados-Arboledas
Atmos. Meas. Tech., 8, 3117–3133, https://doi.org/10.5194/amt-8-3117-2015, https://doi.org/10.5194/amt-8-3117-2015, 2015
H. Che, X.-Y. Zhang, X. Xia, P. Goloub, B. Holben, H. Zhao, Y. Wang, X.-C. Zhang, H. Wang, L. Blarel, B. Damiri, R. Zhang, X. Deng, Y. Ma, T. Wang, F. Geng, B. Qi, J. Zhu, J. Yu, Q. Chen, and G. Shi
Atmos. Chem. Phys., 15, 7619–7652, https://doi.org/10.5194/acp-15-7619-2015, https://doi.org/10.5194/acp-15-7619-2015, 2015
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This work studied more than 10 years of measurements of aerosol optical depths (AODs) made for 50 sites of CARSNET compiled into a climatology of aerosol optical properties for China. It lets us see a detailed full-scale description of AOD observations over China. The results would benefit us a lot in comprehending the temporal and special distribution aerosol optical property over China. Also the data would be valuable to communities of aerosol satellite retrieval, modelling, etc.
V. Buchard, A. M. da Silva, P. R. Colarco, A. Darmenov, C. A. Randles, R. Govindaraju, O. Torres, J. Campbell, and R. Spurr
Atmos. Chem. Phys., 15, 5743–5760, https://doi.org/10.5194/acp-15-5743-2015, https://doi.org/10.5194/acp-15-5743-2015, 2015
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MERRAero is an aerosol reanalysis based on the GEOS-5 earth system model that incorporates an online aerosol module and assimilation of AOD from MODIS sensors. This study assesses the quality of MERRAero absorption using independent OMI observations. In addition to comparisons to OMI absorption AOD, we have developed a radiative transfer interface to simulate the UV aerosol index from assimilated aerosol fields at OMI footprint. Also, we fully diagnose the model using MISR, AERONET and CALIPSO.
M. Christensen, J. Zhang, J. S. Reid, X. Zhang, E. J. Hyer, and A. Smirnov
Atmos. Meas. Tech., 8, 2149–2160, https://doi.org/10.5194/amt-8-2149-2015, https://doi.org/10.5194/amt-8-2149-2015, 2015
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Submerged oceanic bubbles, which could have a much longer life span than whitecaps or bubble rafts, have been hypothesized to increase the water-leaving radiance and thus affect satellite-based estimates of water-leaving radiance to non-trivial levels. This study explores this effect further to determine if such bubbles are of sufficient magnitude to impact satellite aerosol optical depth retrievals through perturbation of the lower boundary conditions.
F. Tan, H. S. Lim, K. Abdullah, T. L. Yoon, and B. Holben
Atmos. Chem. Phys., 15, 3755–3771, https://doi.org/10.5194/acp-15-3755-2015, https://doi.org/10.5194/acp-15-3755-2015, 2015
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Southeast Asia stands out globally, as it hosts one of the most complex meteorological and environmental conditions, making remote sensing difficult both for AERONET and satellites. Cloud-cleared data leave gaps in our remote sensing data record, and conversely, residual cloud contamination of remotely sensed data causes challenging tasks for scientists studying aerosols. With the main motivation of overcoming this problem, an AOD-predicting model is proposed.
K. Knobelspiesse, B. van Diedenhoven, A. Marshak, S. Dunagan, B. Holben, and I. Slutsker
Atmos. Meas. Tech., 8, 1537–1554, https://doi.org/10.5194/amt-8-1537-2015, https://doi.org/10.5194/amt-8-1537-2015, 2015
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We test if ground-based sun photometers/radiometers like those in the Aerosol Robotic Network (AERONET) can use the polarization sensitivity of some instruments for improved cloud optical property retrieval. Our radiative transfer simulations show that the direction of linear polarization indicates cloud thermodynamic phase for optically thin clouds. In practice, data analysis shows a weak response with AERONET instruments, most likely due to noise and orientation/calibration ambiguity.
J. S. Reid, N. D. Lagrosas, H. H. Jonsson, E. A. Reid, W. R. Sessions, J. B. Simpas, S. N. Uy, T. J. Boyd, S. A. Atwood, D. R. Blake, J. R. Campbell, S. S. Cliff, B. N. Holben, R. E. Holz, E. J. Hyer, P. Lynch, S. Meinardi, D. J. Posselt, K. A. Richardson, S. V. Salinas, A. Smirnov, Q. Wang, L. Yu, and J. Zhang
Atmos. Chem. Phys., 15, 1745–1768, https://doi.org/10.5194/acp-15-1745-2015, https://doi.org/10.5194/acp-15-1745-2015, 2015
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This paper reports on the first measurements of aerosol particles embedded in the convectively active southwest monsoonal flow of the South China Sea. The paper describes the research cruise and discusses how variability in aerosol characteristics relates to regional meteorological phenomena such as and the Madden Julian Oscillation, tropical cyclones, squall lines and the monsoonal flow itself. Of special interest is how aerosol transport relates to meteorological drivers of convective activity.
I. Veselovskii, D. N Whiteman, M. Korenskiy, A. Suvorina, A. Kolgotin, A. Lyapustin, Y. Wang, M. Chin, H. Bian, T. L. Kucsera, D. Pérez-Ramírez, and B. Holben
Atmos. Chem. Phys., 15, 1647–1660, https://doi.org/10.5194/acp-15-1647-2015, https://doi.org/10.5194/acp-15-1647-2015, 2015
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The multi-wavelength lidar technique was applied to the study of a smoke event near Washington, DC on 26-28 August 2013. Satellite observations combined with transport model predictions imply that the smoke plume originated mainly from Wyoming/Idaho forest fires. The NASA GSFC multi-wavelength Mie-Raman lidar was used to profile the smoke particle parameters such as volume density, effective radius and the real part of the refractive index.
G. Snider, C. L. Weagle, R. V. Martin, A. van Donkelaar, K. Conrad, D. Cunningham, C. Gordon, M. Zwicker, C. Akoshile, P. Artaxo, N. X. Anh, J. Brook, J. Dong, R. M. Garland, R. Greenwald, D. Griffith, K. He, B. N. Holben, R. Kahn, I. Koren, N. Lagrosas, P. Lestari, Z. Ma, J. Vanderlei Martins, E. J. Quel, Y. Rudich, A. Salam, S. N. Tripathi, C. Yu, Q. Zhang, Y. Zhang, M. Brauer, A. Cohen, M. D. Gibson, and Y. Liu
Atmos. Meas. Tech., 8, 505–521, https://doi.org/10.5194/amt-8-505-2015, https://doi.org/10.5194/amt-8-505-2015, 2015
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We have initiated a global network of ground-level monitoring stations to measure concentrations of fine aerosols in urban environments. Our findings include major ions species, total mass, and total scatter at three wavelengths. Results will be used to further evaluate and enhance satellite remote sensing estimates.
J. R. Campbell, M. A. Vaughan, M. Oo, R. E. Holz, J. R. Lewis, and E. J. Welton
Atmos. Meas. Tech., 8, 435–449, https://doi.org/10.5194/amt-8-435-2015, https://doi.org/10.5194/amt-8-435-2015, 2015
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Digital thresholds based on 2012 CALIOP satellite lidar measurements are investigated for distinguishing cirrus cloud presence, including cloud top temperatures and heights combined with layer depolarization and phase and optical depths. A cloud top temperature of -37 C is found to exhibit the most stable performance, owing to it being the point of homogeneous liquid-water freezing. Depolarization and phase help but are mostly ambiguous at warmer temperatures where mixed-phase clouds propagate.
W. R. Sessions, J. S. Reid, A. Benedetti, P. R. Colarco, A. da Silva, S. Lu, T. Sekiyama, T. Y. Tanaka, J. M. Baldasano, S. Basart, M. E. Brooks, T. F. Eck, M. Iredell, J. A. Hansen, O. C. Jorba, H.-M. H. Juang, P. Lynch, J.-J. Morcrette, S. Moorthi, J. Mulcahy, Y. Pradhan, M. Razinger, C. B. Sampson, J. Wang, and D. L. Westphal
Atmos. Chem. Phys., 15, 335–362, https://doi.org/10.5194/acp-15-335-2015, https://doi.org/10.5194/acp-15-335-2015, 2015
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S. Seo, J. Kim, H. Lee, U. Jeong, W. Kim, B. N. Holben, S.-W. Kim, C. H. Song, and J. H. Lim
Atmos. Chem. Phys., 15, 319–334, https://doi.org/10.5194/acp-15-319-2015, https://doi.org/10.5194/acp-15-319-2015, 2015
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The estimation of PM10 from optical measurement of AERONET and MODIS by various empirical models was evaluated for the DRAGON-Asia campaign. The results showed the importance of boundary layer height (BLH) and effective radius (Reff) in estimating PM10. The highest correlation between the estimated and measured values was found to be 0.81 in winter due to the stagnant air mass and low BLH, while the poorest values were 0.54 in spring due to the influence of long-range transport above BLH.
T. F. Eck, B. N. Holben, J. S. Reid, A. Arola, R. A. Ferrare, C. A. Hostetler, S. N. Crumeyrolle, T. A. Berkoff, E. J. Welton, S. Lolli, A. Lyapustin, Y. Wang, J. S. Schafer, D. M. Giles, B. E. Anderson, K. L. Thornhill, P. Minnis, K. E. Pickering, C. P. Loughner, A. Smirnov, and A. Sinyuk
Atmos. Chem. Phys., 14, 11633–11656, https://doi.org/10.5194/acp-14-11633-2014, https://doi.org/10.5194/acp-14-11633-2014, 2014
A. M. Sayer, N. C. Hsu, T. F. Eck, A. Smirnov, and B. N. Holben
Atmos. Chem. Phys., 14, 11493–11523, https://doi.org/10.5194/acp-14-11493-2014, https://doi.org/10.5194/acp-14-11493-2014, 2014
P. Sawamura, D. Müller, R. M. Hoff, C. A. Hostetler, R. A. Ferrare, J. W. Hair, R. R. Rogers, B. E. Anderson, L. D. Ziemba, A. J. Beyersdorf, K. L. Thornhill, E. L. Winstead, and B. N. Holben
Atmos. Meas. Tech., 7, 3095–3112, https://doi.org/10.5194/amt-7-3095-2014, https://doi.org/10.5194/amt-7-3095-2014, 2014
R. P. Aryal, K. J. Voss, P. A. Terman, W. C. Keene, J. L. Moody, E. J. Welton, and B. N. Holben
Atmos. Chem. Phys., 14, 7617–7629, https://doi.org/10.5194/acp-14-7617-2014, https://doi.org/10.5194/acp-14-7617-2014, 2014
Y. Shi, J. Zhang, J. S. Reid, B. Liu, and E. J. Hyer
Atmos. Meas. Tech., 7, 1791–1801, https://doi.org/10.5194/amt-7-1791-2014, https://doi.org/10.5194/amt-7-1791-2014, 2014
T. D. Toth, J. Zhang, J. R. Campbell, E. J. Hyer, J. S. Reid, Y. Shi, and D. L. Westphal
Atmos. Chem. Phys., 14, 6049–6062, https://doi.org/10.5194/acp-14-6049-2014, https://doi.org/10.5194/acp-14-6049-2014, 2014
M. Chin, T. Diehl, Q. Tan, J. M. Prospero, R. A. Kahn, L. A. Remer, H. Yu, A. M. Sayer, H. Bian, I. V. Geogdzhayev, B. N. Holben, S. G. Howell, B. J. Huebert, N. C. Hsu, D. Kim, T. L. Kucsera, R. C. Levy, M. I. Mishchenko, X. Pan, P. K. Quinn, G. L. Schuster, D. G. Streets, S. A. Strode, O. Torres, and X.-P. Zhao
Atmos. Chem. Phys., 14, 3657–3690, https://doi.org/10.5194/acp-14-3657-2014, https://doi.org/10.5194/acp-14-3657-2014, 2014
H. Che, X. Xia, J. Zhu, Z. Li, O. Dubovik, B. Holben, P. Goloub, H. Chen, V. Estelles, E. Cuevas-Agulló, L. Blarel, H. Wang, H. Zhao, X. Zhang, Y. Wang, J. Sun, R. Tao, X. Zhang, and G. Shi
Atmos. Chem. Phys., 14, 2125–2138, https://doi.org/10.5194/acp-14-2125-2014, https://doi.org/10.5194/acp-14-2125-2014, 2014
M. E. Park, C. H. Song, R. S. Park, J. Lee, J. Kim, S. Lee, J.-H. Woo, G. R. Carmichael, T. F. Eck, B. N. Holben, S.-S. Lee, C. K. Song, and Y. D. Hong
Atmos. Chem. Phys., 14, 659–674, https://doi.org/10.5194/acp-14-659-2014, https://doi.org/10.5194/acp-14-659-2014, 2014
J. L. Moody, W. C. Keene, O. R. Cooper, K. J. Voss, R. Aryal, S. Eckhardt, B. Holben, J. R. Maben, M. A. Izaguirre, and J. N. Galloway
Atmos. Chem. Phys., 14, 691–717, https://doi.org/10.5194/acp-14-691-2014, https://doi.org/10.5194/acp-14-691-2014, 2014
C. Ge, J. Wang, and J. S. Reid
Atmos. Chem. Phys., 14, 159–174, https://doi.org/10.5194/acp-14-159-2014, https://doi.org/10.5194/acp-14-159-2014, 2014
P. E. Saide, G. R. Carmichael, Z. Liu, C. S. Schwartz, H. C. Lin, A. M. da Silva, and E. Hyer
Atmos. Chem. Phys., 13, 10425–10444, https://doi.org/10.5194/acp-13-10425-2013, https://doi.org/10.5194/acp-13-10425-2013, 2013
D. Griffin, K. A. Walker, J. E. Franklin, M. Parrington, C. Whaley, J. Hopper, J. R. Drummond, P. I. Palmer, K. Strong, T. J. Duck, I. Abboud, P. F. Bernath, C. Clerbaux, P.-F. Coheur, K. R. Curry, L. Dan, E. Hyer, J. Kliever, G. Lesins, M. Maurice, A. Saha, K. Tereszchuk, and D. Weaver
Atmos. Chem. Phys., 13, 10227–10241, https://doi.org/10.5194/acp-13-10227-2013, https://doi.org/10.5194/acp-13-10227-2013, 2013
Y. Choi, Y. S. Ghim, and B. N. Holben
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-26627-2013, https://doi.org/10.5194/acpd-13-26627-2013, 2013
Revised manuscript not accepted
L. A. Munchak, R. C. Levy, S. Mattoo, L. A. Remer, B. N. Holben, J. S. Schafer, C. A. Hostetler, and R. A. Ferrare
Atmos. Meas. Tech., 6, 1747–1759, https://doi.org/10.5194/amt-6-1747-2013, https://doi.org/10.5194/amt-6-1747-2013, 2013
R. S. Johnson, J. Zhang, E. J. Hyer, S. D. Miller, and J. S. Reid
Atmos. Meas. Tech., 6, 1245–1255, https://doi.org/10.5194/amt-6-1245-2013, https://doi.org/10.5194/amt-6-1245-2013, 2013
Y. Shi, J. Zhang, J. S. Reid, E. J. Hyer, and N. C. Hsu
Atmos. Meas. Tech., 6, 949–969, https://doi.org/10.5194/amt-6-949-2013, https://doi.org/10.5194/amt-6-949-2013, 2013
V. M. Khade, J. A. Hansen, J. S. Reid, and D. L. Westphal
Atmos. Chem. Phys., 13, 3481–3500, https://doi.org/10.5194/acp-13-3481-2013, https://doi.org/10.5194/acp-13-3481-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Measurement report: Optical and structural properties of atmospheric water-soluble organic carbon in China – insights from multi-site spectroscopic measurements
Measurement report: The variation properties of aerosol hygroscopic growth related to chemical composition during new particle formation days in a coastal city of Southeast China
In situ vertical observations of the layered structure of air pollution in a continental high-latitude urban boundary layer during winter
Size-resolved hygroscopicity and volatility properties of ambient urban aerosol particles measured by a volatility hygroscopicity tandem differential mobility analyzer system in Beijing
Terrestrial runoff is an important source of biological ice-nucleating particles in Arctic marine systems
Characterization of aerosol over the eastern Mediterranean by polarization-sensitive Raman lidar measurements during A-LIFE – aerosol type classification and type separation
Aerosol spectral optical properties in the Paris urban area and its peri-urban and forested surroundings during summer 2022 from ACROSS surface observations
Measurement report: An investigation of the spatiotemporal variability in aerosols in the mountainous terrain of the upper Colorado River basin using SAIL-Net
Contributions of the synoptic meteorology to the seasonal cloud condensation nuclei cycle over the Southern Ocean
Measurement report: Cloud condensation nuclei (CCN) activity in the South China Sea from shipborne observations during the summer and winter of 2021 – seasonal variation and anthropogenic influence
Measurement report: A comparative analysis of an intensive incursion of fluorescing African dust particles over Puerto Rico and another over Spain
Measurement report: Analysis of aerosol optical depth variation at Zhongshan Station in Antarctica
External particle mixing influences hygroscopicity in a sub-urban area
Long-term observations of black carbon and carbon monoxide in the Poker Flat Research Range, central Alaska, with a focus on forest wildfire emissions
High ice-nucleating particle concentrations associated with Arctic haze in springtime cold-air outbreaks
CCN estimations at a high-altitude remote site: role of organic aerosol variability and hygroscopicity
Aerosol hygroscopicity over the southeast Atlantic Ocean during the biomass burning season – Part 1: From the perspective of scattering enhancement
Spatial, temporal, and meteorological impact of the 26 February 2023 dust storm: increase in particulate matter concentrations across New Mexico and West Texas
Large spatiotemporal variability in aerosol properties over central Argentina during the CACTI field campaign
Quantification and characterization of primary biological aerosol particles and microbes aerosolized from Baltic seawater
Brownness of organics in anthropogenic biomass burning aerosols over South Asia
Measurement report: size-resolved particle effective density measured by the AAC-SMPS and implications for chemical composition
Source apportionment of particle number size distribution at the street canyon and urban background sites
Long-range transport of coarse mineral dust: an evaluation of the Met Office Unified Model against aircraft observations
Extreme Saharan dust events expand northward over the Atlantic and Europe, prompting record-breaking PM10 and PM2.5 episodes
Atmospheric black carbon in the metropolitan area of La Paz and El Alto, Bolivia: concentration levels and emission sources
Changing optical properties of black carbon and brown carbon aerosols during long-range transport from the Indo-Gangetic Plain to the equatorial Indian Ocean
The evolution of aerosols mixing state derived from a field campaign in Beijing: implications to the particles aging time scale in urban atmosphere
Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic
Ice-nucleating particles active below −24 °C in a Finnish boreal forest and their relationship to bioaerosols
Measurement report: The influence of particle number size distribution and hygroscopicity on the microphysical properties of cloud droplets at a mountain site
Measurements of particle emissions of an A350-941 burning 100 % sustainable aviation fuels in cruise
Vertical distribution of ice nucleating particles over the boreal forest of Hyytiälä, Finland
Multi-year gradient measurements of sea spray fluxes over the Baltic Sea and the North Atlantic Ocean
Measurement report: In situ vertical profiles of below-cloud aerosol over the central Greenland Ice Sheet
Occurrence, abundance, and formation of atmospheric tarballs from a wide range of wildfires in the western US
Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China: Diurnal variation, vertical distribution and aerosol-cloud relationship
Measurement report: Contribution of atmospheric new particle formation to ultrafine particle concentration, cloud condensation nuclei, and radiative forcing – results from 5-year observations in central Europe
Simulated contrail-processed aviation soot aerosols are poor ice-nucleating particles at cirrus temperatures
Biological and dust aerosols as sources of ice-nucleating particles in the eastern Mediterranean: source apportionment, atmospheric processing and parameterization
Quantifying the dust direct radiative effect in the southwestern United States: findings from multiyear measurements
Hygroscopic Aerosols Amplify Longwave Downward Radiation in the Arctic
How horizontal transport and turbulent mixing impact aerosol particle and precursor concentrations at a background site in the UAE
Markedly different impacts of primary emissions and secondary aerosol formation on aerosol mixing states revealed by simultaneous measurements of CCNC, H(/V)TDMA, and SP2
Phase matrix characterization of long-range transported Saharan dust using multiwavelength polarized polar imaging nephelometry
Vertically resolved aerosol variability at the Amazon Tall Tower Observatory under wet-season conditions
Vertical structure of a springtime smoky and humid troposphere over the southeast Atlantic from aircraft and reanalysis
Measurement Report: Long-term Assessment of Primary and Secondary Organic Aerosols in Shanghai Megacity throughout China’s Clean Air Actions since 2010
Shipborne observations of black carbon aerosols in the western Arctic Ocean during summer and autumn 2016–2020: impact of boreal fires
Attribution of aerosol particle number size distributions to main sources using an 11-year urban dataset
Haibiao Chen, Caiqing Yan, Liubin Huang, Lin Du, Yang Yue, Xinfeng Wang, Qingcai Chen, Mingjie Xie, Junwen Liu, Fengwen Wang, Shuhong Fang, Qiaoyun Yang, Hongya Niu, Mei Zheng, Yan Wu, and Likun Xue
Atmos. Chem. Phys., 25, 3647–3667, https://doi.org/10.5194/acp-25-3647-2025, https://doi.org/10.5194/acp-25-3647-2025, 2025
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A comprehensive understanding of the optical properties of brown carbon (BrC) is essential to accurately assess its climatic effects. Based on multi-site spectroscopic measurements, this study demonstrated the significant spatial heterogeneity in the optical and structural properties of water-soluble organic carbon (WSOC) in different regions of China and revealed factors affecting WSOC light absorption and the relationship between fluorophores and light absorption of WSOC.
Lingjun Li, Mengren Li, Xiaolong Fan, Yuping Chen, Ziyi Lin, Anqi Hou, Siqing Zhang, Ronghua Zheng, and Jinsheng Chen
Atmos. Chem. Phys., 25, 3669–3685, https://doi.org/10.5194/acp-25-3669-2025, https://doi.org/10.5194/acp-25-3669-2025, 2025
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Here, we show differences and variations in the aerosol scattering hygroscopic growth factor (f(RH)) between new particle formation (NPF) and non-NPF days and the effect of aerosol chemical compositions on f(RH) in Xiamen with in situ observations. The findings are helpful for the further understanding of aerosol hygroscopicity in a coastal city and the use of hygroscopic growth factors in models of air quality and climate change.
Roman Pohorsky, Andrea Baccarini, Natalie Brett, Brice Barret, Slimane Bekki, Gianluca Pappaccogli, Elsa Dieudonné, Brice Temime-Roussel, Barbara D'Anna, Meeta Cesler-Maloney, Antonio Donateo, Stefano Decesari, Kathy S. Law, William R. Simpson, Javier Fochesatto, Steve R. Arnold, and Julia Schmale
Atmos. Chem. Phys., 25, 3687–3715, https://doi.org/10.5194/acp-25-3687-2025, https://doi.org/10.5194/acp-25-3687-2025, 2025
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This study presents an analysis of vertical measurements of pollution in an Alaskan city during winter. It investigates the relationship between the atmospheric structure and the layering of aerosols and trace gases. Results indicate an overall very shallow surface mixing layer. The height of this layer is strongly influenced by a local shallow wind. The study also provides information on the pollution chemical composition at different altitudes, including pollution signatures from power plants.
Aoyuan Yu, Xiaojing Shen, Qianli Ma, Jiayuan Lu, Xinyao Hu, Yangmei Zhang, Quan Liu, Linlin Liang, Lei Liu, Shuo Liu, Hongfei Tong, Huizheng Che, Xiaoye Zhang, and Junying Sun
Atmos. Chem. Phys., 25, 3389–3412, https://doi.org/10.5194/acp-25-3389-2025, https://doi.org/10.5194/acp-25-3389-2025, 2025
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In this work, we utilized a volatility hygroscopicity tandem differential mobility analyzer (VH-TDMA) to investigate, for the first time, the hygroscopicity and volatility of submicron aerosols, as well as their hygroscopicity after heating, in urban Beijing during the autumn of 2023. We analyzed the size-resolved characteristics of hygroscopicity and volatility, the relationship between hygroscopic and volatile properties, and the hygroscopicity of heated submicron aerosols.
Corina Wieber, Lasse Z. Jensen, Leendert Vergeynst, Lorenz Meire, Thomas Juul-Pedersen, Kai Finster, and Tina Šantl-Temkiv
Atmos. Chem. Phys., 25, 3327–3346, https://doi.org/10.5194/acp-25-3327-2025, https://doi.org/10.5194/acp-25-3327-2025, 2025
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The Arctic region is subject to profound changes due to a warming climate. Ice-nucleating particles (INPs) in the seawater can get transported to the atmosphere and impact cloud formation. However, the sources of characteristics of INPs in the marine areas are poorly understood. We investigated the INPs in seawater from Greenlandic fjords and identified a seasonal variability, with highly active INPs originating from terrestrial sources such as glacial and soil runoff.
Silke Groß, Volker Freudenthaler, Moritz Haarig, Albert Ansmann, Carlos Toledano, David Mateos, Petra Seibert, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Josef Gasteiger, Maximilian Dollner, Anne Tipka, Manuel Schöberl, Marilena Teri, and Bernadett Weinzierl
Atmos. Chem. Phys., 25, 3191–3211, https://doi.org/10.5194/acp-25-3191-2025, https://doi.org/10.5194/acp-25-3191-2025, 2025
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Aerosols contribute to the largest uncertainties in climate change predictions. The eastern Mediterranean is a hotspot for aerosols with natural and anthropogenic contributions. We present lidar measurements performed during A-LIFE (Absorbing aerosol layers in a changing climate: aging, lifetime and dynamics) to characterize aerosols and aerosol mixtures. We extend current lidar classification and separation schemes and compare them to classification schemes using different methods.
Ludovico Di Antonio, Claudia Di Biagio, Paola Formenti, Aline Gratien, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Patrice Coll, Barbara D'Anna, Joel F. de Brito, David O. De Haan, Juliette R. Dignum, Shravan Deshmukh, Olivier Favez, Pierre-Marie Flaud, Cecile Gaimoz, Lelia N. Hawkins, Julien Kammer, Brigitte Language, Franck Maisonneuve, Griša Močnik, Emilie Perraudin, Jean-Eudes Petit, Prodip Acharja, Laurent Poulain, Pauline Pouyes, Eva Drew Pronovost, Véronique Riffault, Kanuri I. Roundtree, Marwa Shahin, Guillaume Siour, Eric Villenave, Pascal Zapf, Gilles Foret, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 25, 3161–3189, https://doi.org/10.5194/acp-25-3161-2025, https://doi.org/10.5194/acp-25-3161-2025, 2025
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The spectral complex refractive index (CRI) and single scattering albedo were retrieved from submicron aerosol measurements at three sites within the greater Paris area during the ACROSS field campaign (June–July 2022). Measurements revealed urban emission impact on surrounding areas. CRI full period averages at 520 nm were 1.41 – 0.037i (urban), 1.52 – 0.038i (peri-urban), and 1.50 – 0.025i (rural). Organic aerosols dominated the aerosol mass and contributed up to 22 % of absorption at 370 nm.
Leah D. Gibson, Ezra J. T. Levin, Ethan Emerson, Nick Good, Anna Hodshire, Gavin McMeeking, Kate Patterson, Bryan Rainwater, Tom Ramin, and Ben Swanson
Atmos. Chem. Phys., 25, 2745–2762, https://doi.org/10.5194/acp-25-2745-2025, https://doi.org/10.5194/acp-25-2745-2025, 2025
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From fall 2021 to summer 2023, SAIL-Net, a network of six aerosol measurement nodes, was deployed in the East River watershed (Colorado, USA) to study aerosol variability across space and time in mountainous terrain. We found that aerosol variability is influenced by elevation differences, with the most representative site in the region changing seasonally, suggesting aerosol spatial variability also varies seasonally. This work offers a blueprint for future studies in other mountainous regions.
Tahereh Alinejadtabrizi, Yi Huang, Francisco Lang, Steven Siems, Michael Manton, Luis Ackermann, Melita Keywood, Ruhi Humphries, Paul Krummel, Alastair Williams, and Greg Ayers
Atmos. Chem. Phys., 25, 2631–2648, https://doi.org/10.5194/acp-25-2631-2025, https://doi.org/10.5194/acp-25-2631-2025, 2025
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Clouds over the Southern Ocean are crucial to Earth's energy balance, but understanding the factors that control them is complex. Our research examines how weather patterns affect tiny particles called cloud condensation nuclei (CCN), which influence cloud properties. Using data from Kennaook / Cape Grim, we found that winter air from Antarctica brings cleaner conditions with lower CCN, while summer patterns from Australia transport more particles. Precipitation also helps reduce CCN in winter.
Hengjia Ou, Mingfu Cai, Yongyun Zhang, Xue Ni, Baoling Liang, Qibin Sun, Shixin Mai, Cuizhi Sun, Shengzhen Zhou, Haichao Wang, Jiaren Sun, and Jun Zhao
Atmos. Chem. Phys., 25, 2495–2513, https://doi.org/10.5194/acp-25-2495-2025, https://doi.org/10.5194/acp-25-2495-2025, 2025
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Two shipborne observations in the South China Sea (SCS) in summer and winter 2021 were conducted. Our study found aerosol hygroscopicity is higher in the SCS in summer than winter, with significant influences from various terrestrial air masses. Aerosol size distribution had a stronger effect on activation ratio than aerosol hygroscopicity in summer and vice versa in winter. Our study provides valuable information to enhance our understanding of cloud condensation nuclei activities in the SCS.
Bighnaraj Sarangi, Darrel Baumgardner, Ana Isabel Calvo, Benjamin Bolaños-Rosero, Roberto Fraile, Alberto Rodríguez-Fernández, Delia Fernández-González, Carlos Blanco-Alegre, Cátia Gonçalves, Estela D. Vicente, and Olga L. Mayol-Bracero
Atmos. Chem. Phys., 25, 843–865, https://doi.org/10.5194/acp-25-843-2025, https://doi.org/10.5194/acp-25-843-2025, 2025
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Measurements of fluorescing aerosol particle properties have been made during two major African dust events, one over the island of Puerto Rico and the other over the city of León, Spain. The measurements were made with two wideband integrated bioaerosol spectrometers. A significant change in the background aerosol properties, at both locations, is observed when the dust is in the respective regions.
Lijing Chen, Lei Zhang, Yong She, Zhaoliang Zeng, Yu Zheng, Biao Tian, Wenqian Zhang, Zhaohui Liu, Huizheng Che, and Minghu Ding
Atmos. Chem. Phys., 25, 727–739, https://doi.org/10.5194/acp-25-727-2025, https://doi.org/10.5194/acp-25-727-2025, 2025
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Aerosol optical depth (AOD) at Zhongshan Station varies seasonally, with lower values in summer and higher values in winter. Winter and spring AOD increases due to reduced fine-mode particles, while summer and autumn increases are linked to particle growth. Diurnal AOD variation correlates positively with temperature but negatively with wind speed and humidity. Backward trajectories show that aerosols on high-AOD (low-AOD) days primarily originate from the ocean (interior Antarctica).
Shravan Deshmukh, Laurent Poulain, Birgit Wehner, Silvia Henning, Jean-Eudes Petit, Pauline Fombelle, Olivier Favez, Hartmut Herrmann, and Mira Pöhlker
Atmos. Chem. Phys., 25, 741–758, https://doi.org/10.5194/acp-25-741-2025, https://doi.org/10.5194/acp-25-741-2025, 2025
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Aerosol hygroscopicity has been investigated at a sub-urban site in Paris; analysis shows the sub-saturated regime's measured hygroscopicity and the chemically derived hygroscopic growth, shedding light on the large effect of external particle mixing and its influence on predicting hygroscopicity.
Takeshi Kinase, Fumikazu Taketani, Masayuki Takigawa, Chunmao Zhu, Yongwon Kim, Petr Mordovskoi, and Yugo Kanaya
Atmos. Chem. Phys., 25, 143–156, https://doi.org/10.5194/acp-25-143-2025, https://doi.org/10.5194/acp-25-143-2025, 2025
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Boreal forest wildfires in interior Alaska represent an important black carbon (BC) source for the Arctic and surrounding regions. We observed BC and carbon monoxide (CO) concentrations in the Poker Flat Research Range since 2016 and found a positive correlation between the observed BC / ∆CO ratio and fire radiative power (FRP) observed in Alaska and Canada. Our finding suggests the BC emission factor and/or inventory could be potentially improved by using FRP.
Erin N. Raif, Sarah L. Barr, Mark D. Tarn, James B. McQuaid, Martin I. Daily, Steven J. Abel, Paul A. Barrett, Keith N. Bower, Paul R. Field, Kenneth S. Carslaw, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 14045–14072, https://doi.org/10.5194/acp-24-14045-2024, https://doi.org/10.5194/acp-24-14045-2024, 2024
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Ice-nucleating particles (INPs) allow ice to form in clouds at temperatures warmer than −35°C. We measured INP concentrations over the Norwegian and Barents seas in weather events where cold air is ejected from the Arctic. These concentrations were among the highest measured in the Arctic. It is likely that the INPs were transported to the Arctic from distant regions. These results show it is important to consider hemispheric-scale INP processes to understand INP concentrations in the Arctic.
Fernando Rejano, Andrea Casans, Marta Via, Juan Andrés Casquero-Vera, Sonia Castillo, Hassan Lyamani, Alberto Cazorla, Elisabeth Andrews, Daniel Pérez-Ramírez, Andrés Alastuey, Francisco Javier Gómez-Moreno, Lucas Alados-Arboledas, Francisco José Olmo, and Gloria Titos
Atmos. Chem. Phys., 24, 13865–13888, https://doi.org/10.5194/acp-24-13865-2024, https://doi.org/10.5194/acp-24-13865-2024, 2024
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This study provides valuable insights to improve cloud condensation nuclei (CCN) estimations at a high-altitude remote site which is influenced by nearby urban pollution. Understanding the factors that affect CCN estimations is essential to improve the CCN data coverage worldwide and assess aerosol–cloud interactions on a global scale. This is crucial for improving climate models, since aerosol–cloud interactions are the most important source of uncertainty in climate projections.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Junying Sun, Ye Kuang, Paola Formenti, and Steven G. Howell
Atmos. Chem. Phys., 24, 13849–13864, https://doi.org/10.5194/acp-24-13849-2024, https://doi.org/10.5194/acp-24-13849-2024, 2024
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Using airborne measurements over the southeast Atlantic Ocean, we examined how much moisture aerosols take up during Africa’s biomass burning season. Our study revealed the important role of organic aerosols and introduced a predictive model for moisture uptake, accounting for organics, sulfate, and black carbon, summarizing results from various campaigns. These findings improve our understanding of aerosol–moisture interactions and their radiative effects in this climatically critical region.
Mary C. Robinson, Kaitlin Schueth, and Karin Ardon-Dryer
Atmos. Chem. Phys., 24, 13733–13750, https://doi.org/10.5194/acp-24-13733-2024, https://doi.org/10.5194/acp-24-13733-2024, 2024
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On 26 February 2023, New Mexico and West Texas were impacted by a severe dust storm. To analyze this storm, 28 meteorological stations and 19 PM2.5 and PM10 stations were used. Dust particles were in the air for 16 h, and dust storm conditions lasted for up to 120 min. Hourly PM2.5 and PM10 concentrations were up to 518 and 9983 µg m−3, respectively. For Lubbock, Texas, the maximum PM2.5 concentrations were the highest ever recorded.
Jerome D. Fast, Adam C. Varble, Fan Mei, Mikhail Pekour, Jason Tomlinson, Alla Zelenyuk, Art J. Sedlacek III, Maria Zawadowicz, and Louisa Emmons
Atmos. Chem. Phys., 24, 13477–13502, https://doi.org/10.5194/acp-24-13477-2024, https://doi.org/10.5194/acp-24-13477-2024, 2024
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Aerosol property measurements recently collected on the ground and by a research aircraft in central Argentina during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) campaign exhibit large spatial and temporal variability. These measurements coupled with coincident meteorological information provide a valuable data set needed to evaluate and improve model predictions of aerosols in a traditionally data-sparse region of South America.
Julika Zinke, Gabriel Pereira Freitas, Rachel Ann Foster, Paul Zieger, Ernst Douglas Nilsson, Piotr Markuszewski, and Matthew Edward Salter
Atmos. Chem. Phys., 24, 13413–13428, https://doi.org/10.5194/acp-24-13413-2024, https://doi.org/10.5194/acp-24-13413-2024, 2024
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Bioaerosols, which can influence climate and human health, were studied in the Baltic Sea. In May and August 2021, we used a sea spray simulation chamber during two ship-based campaigns to collect and measure these aerosols. We found that microbes were enriched in air compared to seawater. Bacterial diversity was analysed using DNA sequencing. Our methods provided consistent estimates of microbial emission fluxes, aligning with previous studies.
Chimurkar Navinya, Taveen Singh Kapoor, Gupta Anurag, Chandra Venkataraman, Harish C. Phuleria, and Rajan K. Chakrabarty
Atmos. Chem. Phys., 24, 13285–13297, https://doi.org/10.5194/acp-24-13285-2024, https://doi.org/10.5194/acp-24-13285-2024, 2024
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Brown carbon (BrC) aerosols show an order-of-magnitude variation in their light absorption strength. Our understanding of BrC from real-world biomass burning remains limited, complicating the determination of its radiative impact. Our study reports absorption properties of BrC emitted from four major biomass burning sources using field measurements in India. It develops an absorption parameterization for BrC and examines the spatial variability in BrC's absorption strength across India.
Yao Song, Jing Wei, Wenlong Zhao, Jinmei Ding, Xiangyu Pei, Fei Zhang, Zhengning Xu, Ruifang Shi, Ya Wei, Lu Zhang, Lingling Jin, and Zhibin Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-3298, https://doi.org/10.5194/egusphere-2024-3298, 2024
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This study investigates the size-resolved effective density (ρeff) of aerosol particles in Hangzhou using an AAC-SMPS. The ρeff values ranged from 1.47 to 1.63 g/cm3, increasing with particle diameter. Smaller particles showed significant diurnal density variations. The relationship between ρeff and particle diameter varies due to differences in the chemical composition of the particles. A new method to derive size-resolved chemical composition of particles from ρeff was proposed.
Sami D. Harni, Minna Aurela, Sanna Saarikoski, Jarkko V. Niemi, Harri Portin, Hanna Manninen, Ville Leinonen, Pasi Aalto, Phil K. Hopke, Tuukka Petäjä, Topi Rönkkö, and Hilkka Timonen
Atmos. Chem. Phys., 24, 12143–12160, https://doi.org/10.5194/acp-24-12143-2024, https://doi.org/10.5194/acp-24-12143-2024, 2024
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In this study, particle number size distribution data were used in a novel way in positive matrix factorization analysis to find aerosol source profiles in the area. Measurements were made in Helsinki at a street canyon and urban background sites between February 2015 and June 2019. Five different aerosol sources were identified. These sources underline the significance of traffic-related emissions in urban environments despite recent improvements in emission reduction technologies.
Natalie G. Ratcliffe, Claire L. Ryder, Nicolas Bellouin, Stephanie Woodward, Anthony Jones, Ben Johnson, Lisa-Maria Wieland, Maximilian Dollner, Josef Gasteiger, and Bernadett Weinzierl
Atmos. Chem. Phys., 24, 12161–12181, https://doi.org/10.5194/acp-24-12161-2024, https://doi.org/10.5194/acp-24-12161-2024, 2024
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Large mineral dust particles are more abundant in the atmosphere than expected and have different impacts on the environment than small particles, which are better represented in climate models. We use aircraft measurements to assess a climate model representation of large-dust transport. We find that the model underestimates the amount of large dust at all stages of transport and that fast removal of the large particles increases this underestimation with distance from the Sahara.
Sergio Rodríguez and Jessica López-Darias
Atmos. Chem. Phys., 24, 12031–12053, https://doi.org/10.5194/acp-24-12031-2024, https://doi.org/10.5194/acp-24-12031-2024, 2024
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Extreme Saharan dust events expanded northward to the Atlantic and Europe, prompting record-breaking PM10 and PM2.5 events. These episodes are caused by low-to-high dipole meteorology during hemispheric anomalies characterized by subtropical anticyclones shifting to higher latitudes, anomalous low pressures beyond the tropics and amplified Rossby waves. Extreme dust events occur in a paradoxical context of a multidecadal decrease in dust emissions, a topic that requires further investigation.
Valeria Mardoñez-Balderrama, Griša Močnik, Marco Pandolfi, Robin L. Modini, Fernando Velarde, Laura Renzi, Angela Marinoni, Jean-Luc Jaffrezo, Isabel Moreno R., Diego Aliaga, Federico Bianchi, Claudia Mohr, Martin Gysel-Beer, Patrick Ginot, Radovan Krejci, Alfred Wiedensohler, Gaëlle Uzu, Marcos Andrade, and Paolo Laj
Atmos. Chem. Phys., 24, 12055–12077, https://doi.org/10.5194/acp-24-12055-2024, https://doi.org/10.5194/acp-24-12055-2024, 2024
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Levels of black carbon (BC) are scarcely reported in the Southern Hemisphere, especially in high-altitude conditions. This study provides insight into the concentration level, variability, and optical properties of BC in La Paz and El Alto and at the Chacaltaya Global Atmosphere Watch Station. Two methods of source apportionment of absorption were tested and compared showing traffic as the main contributor to absorption in the urban area, in addition to biomass and open waste burning.
Krishnakant Budhavant, Mohanan Remani Manoj, Hari Ram Chandrika Rajendran Nair, Samuel Mwaniki Gaita, Henry Holmstrand, Abdus Salam, Ahmed Muslim, Sreedharan Krishnakumari Satheesh, and Örjan Gustafsson
Atmos. Chem. Phys., 24, 11911–11925, https://doi.org/10.5194/acp-24-11911-2024, https://doi.org/10.5194/acp-24-11911-2024, 2024
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The South Asian Pollution Experiment 2018 used access to three strategically located receptor observatories. Observational constraints revealed opposing trends in the mass absorption cross sections of black carbon (BC MAC) and brown carbon (BrC MAC) during long-range transport. Models estimating the climate effects of BC aerosols may have underestimated the ambient BC MAC over distant receptor areas, leading to discrepancies in aerosol absorption predicted by observation-constrained models.
Jieyao Liu, Fang Zhang, Jingye Ren, and Lu Chen
EGUsphere, https://doi.org/10.5194/egusphere-2024-2999, https://doi.org/10.5194/egusphere-2024-2999, 2024
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The particles mixing states and aging time scale are important for the evaluation of aerosols climate effects, but they are poorly parameterized in current models. We unravel the evolution of real-time mixing states and aging time scale of size-resolved particles based on field measurement in urban Beijing. This study provides observational basis for accurately parameterizing the aging time scale of aerosol particles in climate models.
Abigail S. Williams, Jeramy L. Dedrick, Lynn M. Russell, Florian Tornow, Israel Silber, Ann M. Fridlind, Benjamin Swanson, Paul J. DeMott, Paul Zieger, and Radovan Krejci
Atmos. Chem. Phys., 24, 11791–11805, https://doi.org/10.5194/acp-24-11791-2024, https://doi.org/10.5194/acp-24-11791-2024, 2024
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The measured aerosol size distribution modes reveal distinct properties characteristic of cold-air outbreaks in the Norwegian Arctic. We find higher sea spray number concentrations, smaller Hoppel minima, lower effective supersaturations, and accumulation-mode particle scavenging during cold-air outbreaks. These results advance our understanding of cold-air outbreak aerosol–cloud interactions in order to improve their accurate representation in models.
Franziska Vogel, Michael P. Adams, Larissa Lacher, Polly B. Foster, Grace C. E. Porter, Barbara Bertozzi, Kristina Höhler, Julia Schneider, Tobias Schorr, Nsikanabasi S. Umo, Jens Nadolny, Zoé Brasseur, Paavo Heikkilä, Erik S. Thomson, Nicole Büttner, Martin I. Daily, Romy Fösig, Alexander D. Harrison, Jorma Keskinen, Ulrike Proske, Jonathan Duplissy, Markku Kulmala, Tuukka Petäjä, Ottmar Möhler, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 11737–11757, https://doi.org/10.5194/acp-24-11737-2024, https://doi.org/10.5194/acp-24-11737-2024, 2024
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Primary ice formation in clouds strongly influences their properties; hence, it is important to understand the sources of ice-nucleating particles (INPs) and their variability. We present 2 months of INP measurements in a Finnish boreal forest using a new semi-autonomous INP counting device based on gas expansion. These results show strong variability in INP concentrations, and we present a case that the INPs we observe are, at least some of the time, of biological origin.
Xiaojing Shen, Quan Liu, Junying Sun, Wanlin Kong, Qianli Ma, Bing Qi, Lujie Han, Yangmei Zhang, Linlin Liang, Lei Liu, Shuo Liu, Xinyao Hu, Jiayuan Lu, Aoyuan Yu, Huizheng Che, and Xiaoye Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2850, https://doi.org/10.5194/egusphere-2024-2850, 2024
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In this work, an automatic switched inlet system was developed and employed to investigate the aerosols and cloud droplets at a mountain site with frequent cloud processes. It showed different characteristics of cloud residual and interstitial particles. Stronger particle hygroscopicity reduced liquid water content and smaller cloud droplet diameters. This investigation contributes to understanding aerosol-cloud interactions by assessing the impact of aerosol particles on cloud microphysics.
Rebecca Dischl, Daniel Sauer, Christiane Voigt, Theresa Harlaß, Felicitas Sakellariou, Raphael Märkl, Ulrich Schumann, Monika Scheibe, Stefan Kaufmann, Anke Roiger, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Mark Johnson, Denise Ahrens, Reetu Sallinen, Tobias Schripp, Georg Eckel, Uwe Bauder, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 11255–11273, https://doi.org/10.5194/acp-24-11255-2024, https://doi.org/10.5194/acp-24-11255-2024, 2024
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In-flight measurements of aircraft emissions burning 100 % sustainable aviation fuel (SAF) show reduced particle number concentrations up to 41 % compared to conventional jet fuel. Particle emissions are dependent on engine power setting, flight altitude, and fuel composition. Engine models show a good correlation with measurement results. Future increased prevalence of SAF can positively influence the climate impact of aviation.
Zoé Brasseur, Julia Schneider, Janne Lampilahti, Ville Vakkari, Victoria A. Sinclair, Christina J. Williamson, Carlton Xavier, Dmitri Moisseev, Markus Hartmann, Pyry Poutanen, Markus Lampimäki, Markku Kulmala, Tuukka Petäjä, Katrianne Lehtipalo, Erik S. Thomson, Kristina Höhler, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 24, 11305–11332, https://doi.org/10.5194/acp-24-11305-2024, https://doi.org/10.5194/acp-24-11305-2024, 2024
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Ice-nucleating particles (INPs) strongly influence the formation of clouds by initiating the formation of ice crystals. However, very little is known about the vertical distribution of INPs in the atmosphere. Here, we present aircraft measurements of INP concentrations above the Finnish boreal forest. Results show that near-surface INPs are efficiently transported and mixed within the boundary layer and occasionally reach the free troposphere.
Piotr Markuszewski, E. Douglas Nilsson, Julika Zinke, E. Monica Mårtensson, Matthew Salter, Przemysław Makuch, Małgorzata Kitowska, Iwona Niedźwiecka-Wróbel, Violetta Drozdowska, Dominik Lis, Tomasz Petelski, Luca Ferrero, and Jacek Piskozub
Atmos. Chem. Phys., 24, 11227–11253, https://doi.org/10.5194/acp-24-11227-2024, https://doi.org/10.5194/acp-24-11227-2024, 2024
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Our research provides new insights into the study of sea spray aerosol (SSA) emissions in the Baltic Sea and North Atlantic. We observed that SSA flux is suppressed during increased marine biological activity in the Baltic Sea. At the same time, the influence of wave age showed higher SSA emissions in the Baltic Sea for younger waves compared to the Atlantic Ocean. These insights underscore the complex interplay between biological activity and physical dynamics in regulating SSA emissions.
Heather Guy, Andrew S. Martin, Erik Olson, Ian M. Brooks, and Ryan R. Neely III
Atmos. Chem. Phys., 24, 11103–11114, https://doi.org/10.5194/acp-24-11103-2024, https://doi.org/10.5194/acp-24-11103-2024, 2024
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Aerosol particles impact cloud properties which influence Greenland Ice Sheet melt. Understanding the aerosol population that interacts with clouds is important for constraining future melt. Measurements of aerosols at cloud height over Greenland are rare, and surface measurements are often used to investigate cloud–aerosol interactions. We use a tethered balloon to measure aerosols up to cloud base and show that surface measurements are often not equivalent to those just below the cloud.
Kouji Adachi, Jack E. Dibb, Joseph M. Katich, Joshua P. Schwarz, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Jeff Peischl, Christopher D. Holmes, and James Crawford
Atmos. Chem. Phys., 24, 10985–11004, https://doi.org/10.5194/acp-24-10985-2024, https://doi.org/10.5194/acp-24-10985-2024, 2024
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We examined aerosol particles from wildfires and identified tarballs (TBs) from the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) campaign. This study reveals the compositions, abundance, sizes, and mixing states of TBs and shows that TBs formed as the smoke aged for up to 5 h. This study provides measurements of TBs from various biomass-burning events and ages, enhancing our knowledge of TB emissions and our understanding of their climate impact.
Sihan Liu, Honglei Wang, Delong Zhao, Wei Zhou, Yuanmou Du, Zhengguo Zhang, Peng Cheng, Tianliang Zhao, Yue Ke, Zihao Wu, and Mengyu Huang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2756, https://doi.org/10.5194/egusphere-2024-2756, 2024
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To understand the effect of aerosols on the vertical distribution of stratocumulus microphysical quantities in southwest China, the daily variation characteristics and formation mechanism of the vertical profiles of stratocumulus microphysical characteristics in this region were described by using the data of 9 cloud-crossing aircraft observations over Guangxi from October 10 to November 3, 2020.
Jia Sun, Markus Hermann, Kay Weinhold, Maik Merkel, Wolfram Birmili, Yifan Yang, Thomas Tuch, Harald Flentje, Björn Briel, Ludwig Ries, Cedric Couret, Michael Elsasser, Ralf Sohmer, Klaus Wirtz, Frank Meinhardt, Maik Schütze, Olaf Bath, Bryan Hellack, Veli-Matti Kerminen, Markku Kulmala, Nan Ma, and Alfred Wiedensohler
Atmos. Chem. Phys., 24, 10667–10687, https://doi.org/10.5194/acp-24-10667-2024, https://doi.org/10.5194/acp-24-10667-2024, 2024
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We investigated the characteristics of new particle formation (NPF) for various environments from urban background to high Alpine and the impacts of NPF on cloud condensation nuclei and aerosol radiative forcing. NPF features differ between site categories, implying the crucial role of local environmental factors such as the degree of emissions and meteorological conditions. The results also underscore the importance of local environments when assessing the impact of NPF on climate in models.
Baptiste Testa, Lukas Durdina, Jacinta Edebeli, Curdin Spirig, and Zamin A. Kanji
Atmos. Chem. Phys., 24, 10409–10424, https://doi.org/10.5194/acp-24-10409-2024, https://doi.org/10.5194/acp-24-10409-2024, 2024
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Aviation soot residuals released from contrails can become compacted upon sublimation of the ice crystals, generating new voids in the aggregates where ice nucleation can occur. Here we show that contrail-processed soot is highly compact but that it remains unable to form ice at a relative humidity different from that required for the formation of background cirrus from the more ubiquitous aqueous solution droplets, suggesting that it will not perturb cirrus cloud formation via ice nucleation.
Kunfeng Gao, Franziska Vogel, Romanos Foskinis, Stergios Vratolis, Maria I. Gini, Konstantinos Granakis, Anne-Claire Billault-Roux, Paraskevi Georgakaki, Olga Zografou, Prodromos Fetfatzis, Alexis Berne, Alexandros Papayannis, Konstantinos Eleftheridadis, Ottmar Möhler, and Athanasios Nenes
Atmos. Chem. Phys., 24, 9939–9974, https://doi.org/10.5194/acp-24-9939-2024, https://doi.org/10.5194/acp-24-9939-2024, 2024
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Ice nucleating particle (INP) concentrations are required for correct predictions of clouds and precipitation in a changing climate, but they are poorly constrained in climate models. We unravel source contributions to INPs in the eastern Mediterranean and find that biological particles are important, regardless of their origin. The parameterizations developed exhibit superior performance and enable models to consider biological-particle effects on INPs.
Alexandra Kuwano, Amato T. Evan, Blake Walkowiak, and Robert Frouin
Atmos. Chem. Phys., 24, 9843–9868, https://doi.org/10.5194/acp-24-9843-2024, https://doi.org/10.5194/acp-24-9843-2024, 2024
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The dust direct radiative effect is highly uncertain. Here we used new measurements collected over 3 years and during dust storms at a field site in a desert region in the southwestern United States to estimate the regional dust direct radiative effect. We also used novel soil mineralogy retrieved from an airborne spectrometer to estimate this parameter with model output. We find that, in this region, dust has a minimal net cooling effect on this region's climate.
Denghui Ji, Mathias Palm, Matthias Buschmann, Kerstin Ebell, Marion Maturilli, Xiaoyu Sun, and Justus Notholt
EGUsphere, https://doi.org/10.5194/egusphere-2024-2241, https://doi.org/10.5194/egusphere-2024-2241, 2024
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Our study explores how certain aerosols, like sea salt, affect infrared heat radiation in the Arctic, potentially speeding up warming. We used advanced technology to measure aerosol composition and found that these particles grow with humidity, significantly increasing their heat-trapping effect in the infrared region, especially in winter. Our findings suggest these aerosols could be a key factor in Arctic warming, emphasizing the importance of understanding aerosols for climate prediction.
Jutta Kesti, Ewan J. O'Connor, Anne Hirsikko, John Backman, Maria Filioglou, Anu-Maija Sundström, Juha Tonttila, Heikki Lihavainen, Hannele Korhonen, and Eija Asmi
Atmos. Chem. Phys., 24, 9369–9386, https://doi.org/10.5194/acp-24-9369-2024, https://doi.org/10.5194/acp-24-9369-2024, 2024
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The study combines aerosol particle measurements at the surface and vertical profiling of the atmosphere with a scanning Doppler lidar to investigate how particle transportation together with boundary layer evolution can affect particle and SO2 concentrations at the surface in the Arabian Peninsula region. The instrumentation enabled us to see elevated nucleation mode particle and SO2 concentrations at the surface when air masses transported from polluted areas are mixed in the boundary layer.
Jiangchuan Tao, Biao Luo, Weiqi Xu, Gang Zhao, Hanbin Xu, Biao Xue, Miaomiao Zhai, Wanyun Xu, Huarong Zhao, Sanxue Ren, Guangsheng Zhou, Li Liu, Ye Kuang, and Yele Sun
Atmos. Chem. Phys., 24, 9131–9154, https://doi.org/10.5194/acp-24-9131-2024, https://doi.org/10.5194/acp-24-9131-2024, 2024
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Using simultaneous measurements of DMA–CCNC, H(/V)TDMA, and DMA–SP2, impacts of primary emissions and secondary aerosol formations on changes in aerosol physicochemical properties were comprehensively investigated. It was found that intercomparisons among aerosol mixing-state parameters derived from different techniques can help us gain more insight into aerosol physical properties which, in turn, will aid the investigation of emission characteristics and secondary aerosol formation pathways.
Elena Bazo, Daniel Perez-Ramirez, Antonio Valenzuela, Vanderlei Martins, Gloria Titos, Alberto Cazorla, Fernando Rejano, Diego Patrón, Arlett Diaz-Zurita, Francisco Jose Garcia-Izquierdo, David Fuertes, Lucas Alados-Arboledas, and Francisco Jose Olmo
EGUsphere, https://doi.org/10.5194/egusphere-2024-2080, https://doi.org/10.5194/egusphere-2024-2080, 2024
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This works analyses aerosol scattering phase function for transported Saharan dust to the city of Granada – located in southwestern Europe. We use the novel technique polar imaging nephelometry that helps to determine the phase functions using a CCD camara. The capability of measuring with polarized light helps to inferr new properties about the mixture of Saharan dust particles with other of anthropogenic origin.
Marco A. Franco, Rafael Valiati, Bruna A. Holanda, Bruno B. Meller, Leslie A. Kremper, Luciana V. Rizzo, Samara Carbone, Fernando G. Morais, Janaína P. Nascimento, Meinrat O. Andreae, Micael A. Cecchini, Luiz A. T. Machado, Milena Ponczek, Ulrich Pöschl, David Walter, Christopher Pöhlker, and Paulo Artaxo
Atmos. Chem. Phys., 24, 8751–8770, https://doi.org/10.5194/acp-24-8751-2024, https://doi.org/10.5194/acp-24-8751-2024, 2024
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The Amazon wet-season atmosphere was studied at the Amazon Tall Tower Observatory site, revealing vertical variations (between 60 and 325 m) in natural aerosols. Daytime mixing contrasted with nighttime stratification, with distinct rain-induced changes in aerosol populations. Notably, optical property recovery at higher levels was faster, while near-canopy aerosols showed higher scattering efficiency. These findings enhance our understanding of aerosol impacts on climate dynamics.
Kristina Pistone, Eric M. Wilcox, Paquita Zuidema, Marco Giordano, James Podolske, Samuel E. LeBlanc, Meloë Kacenelenbogen, Steven G. Howell, and Steffen Freitag
Atmos. Chem. Phys., 24, 7983–8005, https://doi.org/10.5194/acp-24-7983-2024, https://doi.org/10.5194/acp-24-7983-2024, 2024
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The springtime southeast Atlantic atmosphere contains lots of smoke from continental fires. This smoke travels with water vapor; more smoke means more humidity. We use aircraft observations and models to describe how the values change through the season and over the region. We sort the atmosphere into different types by vertical structure and amount of smoke and humidity. Since our work shows how frequently these components coincide, it helps to better quantify heating effects over this region.
Haifeng Yu, Yunhua Chang, Lin Cheng, Yusen Duan, and Jianlin Hu
EGUsphere, https://doi.org/10.5194/egusphere-2024-1488, https://doi.org/10.5194/egusphere-2024-1488, 2024
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This study presents long-term measurements and comprehensive analysis of carbonaceous aerosols in PM2.5 in Shanghai. We further estimated POC and SOC levels, examining their temporal variations on interannual, monthly, seasonal, and diurnal scales. Through rigorous statistical analysis and correlation studies with meteorological parameters and pollutant concentrations, the origins, formation mechanisms, and spatial distribution patterns of SOC were elucidated.
Yange Deng, Hiroshi Tanimoto, Kohei Ikeda, Sohiko Kameyama, Sachiko Okamoto, Jinyoung Jung, Young Jun Yoon, Eun Jin Yang, and Sung-Ho Kang
Atmos. Chem. Phys., 24, 6339–6357, https://doi.org/10.5194/acp-24-6339-2024, https://doi.org/10.5194/acp-24-6339-2024, 2024
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Black carbon (BC) aerosols play important roles in Arctic climate change, yet they are not well understood because of limited observational data. We observed BC mass concentrations (mBC) in the western Arctic Ocean during summer and early autumn 2016–2020. The mean mBC in 2019 was much higher than in other years. Biomass burning was likely the dominant BC source. Boreal fire BC transport occurring near the surface and/or in the mid-troposphere contributed to high-BC events in the Arctic Ocean.
Máté Vörösmarty, Philip K. Hopke, and Imre Salma
Atmos. Chem. Phys., 24, 5695–5712, https://doi.org/10.5194/acp-24-5695-2024, https://doi.org/10.5194/acp-24-5695-2024, 2024
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The World Health Organization identified ultrafine particles, which make up most of the particle number concentrations, as a potential risk factor for humans. The sources of particle numbers are very different from those of the particulate matter mass. We performed source apportionment of size-segregated particle number concentrations over the diameter range of 6–1000 nm in Budapest for 11 full years. Six source types were identified, characterized and quantified.
Cited articles
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Short summary
This paper describes aspects of the 2012 7 Southeast Asian Studies (7SEAS) operations period, the largest within the Maritime Continent. Included were an enhanced deployment of Aerosol Robotic Network (AERONET) sun photometers, multiple lidars, and a Singapore supersite. Simultaneously, a ship was dispatched to the Palawan Archipelago and Sulu Sea of the Philippines for September 2012 to observe transported smoke and pollution as it entered the southwest monsoon trough.
This paper describes aspects of the 2012 7 Southeast Asian Studies (7SEAS) operations period,...
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