Articles | Volume 15, issue 23
https://doi.org/10.5194/acp-15-13787-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-15-13787-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
15 Dec 2015
Research article |
| 15 Dec 2015
Polarimetric radar and in situ observations of riming and snowfall microphysics during CLACE 2014
J. Grazioli
Environmental Remote Sensing Laboratory (LTE), École Polytechnique Fédérale de Lausanne (EPFL), Lausanne, Switzerland
G. Lloyd
Centre for Atmospheric Science, University of Manchester, Manchester, UK
L. Panziera
Environmental Remote Sensing Laboratory (LTE), École Polytechnique Fédérale de Lausanne (EPFL), Lausanne, Switzerland
C. R. Hoyle
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), Villigen, Switzerland
WSL Institute for Snow and Avalanche Research SLF, Davos, Switzerland
P. J. Connolly
Centre for Atmospheric Science, University of Manchester, Manchester, UK
J. Henneberger
Institute for Atmospheric and Climate Science, ETH, Zurich, Switzerland
Environmental Remote Sensing Laboratory (LTE), École Polytechnique Fédérale de Lausanne (EPFL), Lausanne, Switzerland
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The near-surface atmosphere over the Antarctic Plateau is cold and pristine and resembles to a certain extent the high troposphere where cirrus clouds form. In this study, we use innovative humidity measurements at Concordia Station to study the formation of ice fogs at temperatures <−40°C. We provide observational evidence that ice fogs can form through the homogeneous freezing of solution aerosols, a common nucleation pathway for cirrus clouds.
Jörg Wieder, Nikola Ihn, Claudia Mignani, Moritz Haarig, Johannes Bühl, Patric Seifert, Ronny Engelmann, Fabiola Ramelli, Zamin A. Kanji, Ulrike Lohmann, and Jan Henneberger
Atmos. Chem. Phys., 22, 9767–9797, https://doi.org/10.5194/acp-22-9767-2022, https://doi.org/10.5194/acp-22-9767-2022, 2022
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Ice formation and its evolution in mixed-phase clouds are still uncertain. We evaluate the lidar retrieval of ice-nucleating particle concentration in dust-dominated and continental air masses over the Swiss Alps with in situ observations. A calibration factor to improve the retrieval from continental air masses is proposed. Ice multiplication factors are obtained with a new method utilizing remote sensing. Our results indicate that secondary ice production occurs at temperatures down to −30 °C.
Alfonso Ferrone, Anne-Claire Billault-Roux, and Alexis Berne
Atmos. Meas. Tech., 15, 3569–3592, https://doi.org/10.5194/amt-15-3569-2022, https://doi.org/10.5194/amt-15-3569-2022, 2022
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The Micro Rain Radar PRO (MRR-PRO) is a meteorological radar, with a relevant set of features for deployment in remote locations. We developed an algorithm, named ERUO, for the processing of its measurements of snowfall. The algorithm addresses typical issues of the raw spectral data, such as interference lines, but also improves the quality and sensitivity of the radar variables. ERUO has been evaluated over four different datasets collected in Antarctica and in the Swiss Jura.
Jeong-Su Ko, Kyo-Sun Sunny Lim, Kwonil Kim, Gyuwon Lee, Gregory Thompson, and Alexis Berne
Geosci. Model Dev., 15, 4529–4553, https://doi.org/10.5194/gmd-15-4529-2022, https://doi.org/10.5194/gmd-15-4529-2022, 2022
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This study evaluates the performance of the four microphysics parameterizations, the WDM6, WDM7, Thompson, and Morrison schemes, in simulating snowfall events during the ICE-POP 2018 field campaign. Eight snowfall events are selected and classified into three categories (cold-low, warm-low, and air–sea interaction cases). The evaluation focuses on the simulated hydrometeors, microphysics budgets, wind fields, and precipitation using the measurement data.
Jörg Wieder, Claudia Mignani, Mario Schär, Lucie Roth, Michael Sprenger, Jan Henneberger, Ulrike Lohmann, Cyril Brunner, and Zamin A. Kanji
Atmos. Chem. Phys., 22, 3111–3130, https://doi.org/10.5194/acp-22-3111-2022, https://doi.org/10.5194/acp-22-3111-2022, 2022
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We investigate the variation in ice-nucleating particles (INPs) relevant for primary ice formation in mixed-phased clouds over the Alps based on simultaneous in situ observations at a mountaintop and a nearby high valley (1060 m height difference). In most cases, advection from the surrounding lower regions was responsible for changes in INP concentration, causing a diurnal cycle at the mountaintop. Our study underlines the importance of the planetary boundary layer as an INP reserve.
Graciela B. Raga, Darrel Baumgardner, Blanca Rios, Yanet Díaz-Esteban, Alejandro Jaramillo, Martin Gallagher, Bastien Sauvage, Pawel Wolff, and Gary Lloyd
Atmos. Chem. Phys., 22, 2269–2292, https://doi.org/10.5194/acp-22-2269-2022, https://doi.org/10.5194/acp-22-2269-2022, 2022
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The In-Service Aircraft for a Global Observing System (IAGOS) is a small fleet of commercial aircraft that carry a suite of meteorological, gas, aerosol, and cloud sensors and have been measuring worldwide for almost 9 years, since late 2011. Extreme ice events (EIEs) have been identified from the IAGOS cloud measurements and linked to surface emissions for biomass and fossil fuel consumption. The results reported here are highly relevant for climate change and flight operations forecasting.
Paraskevi Georgakaki, Georgia Sotiropoulou, Étienne Vignon, Anne-Claire Billault-Roux, Alexis Berne, and Athanasios Nenes
Atmos. Chem. Phys., 22, 1965–1988, https://doi.org/10.5194/acp-22-1965-2022, https://doi.org/10.5194/acp-22-1965-2022, 2022
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The modelling study focuses on the importance of ice multiplication processes in orographic mixed-phase clouds, which is one of the least understood cloud types in the climate system. We show that the consideration of ice seeding and secondary ice production through ice–ice collisional breakup is essential for correct predictions of precipitation in mountainous terrain, with important implications for radiation processes.
Waldemar Schledewitch, Gary Lloyd, Keith Bower, Thomas Choularton, Michael Flynn, and Martin Gallagher
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-69, https://doi.org/10.5194/acp-2022-69, 2022
Publication in ACP not foreseen
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Ice crystals on the surface of ice and snow covered terrain are thought to be transported into clouds that cover the surface. This has important implications for the properties of clouds in these regions. This research measured the potential transport of surface based ice crystals into the surrounding clouds at a mountain top site.
Zhiqiang Cui, Alan Blyth, Yahui Huang, Gary Lloyd, Thomas Choularton, Keith Bower, Paul Field, Rachel Hawker, and Lindsay Bennett
Atmos. Chem. Phys., 22, 1649–1667, https://doi.org/10.5194/acp-22-1649-2022, https://doi.org/10.5194/acp-22-1649-2022, 2022
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High concentrations of ice particles were observed at temperatures greater than about –8 C. The default scheme of the secondary ice production cannot explain the high concentrations. Relaxing the conditions for secondary ice production or considering dust aerosol alone is insufficient to produce the observed amount of ice particles. It is likely that multi-thermals play an important role in producing very high concentrations of secondary ice particles in some tropical clouds.
Dalrin Ampritta Amaladhasan, Claudia Heyn, Christopher R. Hoyle, Imad El Haddad, Miriam Elser, Simone M. Pieber, Jay G. Slowik, Antonio Amorim, Jonathan Duplissy, Sebastian Ehrhart, Vladimir Makhmutov, Ugo Molteni, Matti Rissanen, Yuri Stozhkov, Robert Wagner, Armin Hansel, Jasper Kirkby, Neil M. Donahue, Rainer Volkamer, Urs Baltensperger, Martin Gysel-Beer, and Andreas Zuend
Atmos. Chem. Phys., 22, 215–244, https://doi.org/10.5194/acp-22-215-2022, https://doi.org/10.5194/acp-22-215-2022, 2022
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We use a combination of models for gas-phase chemical reactions and equilibrium gas–particle partitioning of isoprene-derived secondary organic aerosols (SOAs) informed by dark ozonolysis experiments conducted in the CLOUD chamber. Our predictions cover high to low relative humidities (RHs) and quantify how SOA mass yields are enhanced at high RH as well as the impact of inorganic seeds of distinct hygroscopicities and acidities on the coupled partitioning of water and semi-volatile organics.
Rachel L. James, Vaughan T. J. Phillips, and Paul J. Connolly
Atmos. Chem. Phys., 21, 18519–18530, https://doi.org/10.5194/acp-21-18519-2021, https://doi.org/10.5194/acp-21-18519-2021, 2021
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Secondary ice production (SIP) plays an important role in ice formation within mixed-phase clouds. We present a laboratory investigation of a potentially new SIP mechanism involving the collisions of supercooled water drops with ice particles. At impact, the supercooled water drop fragments form smaller secondary drops. Approximately 30 % of the secondary drops formed during the retraction phase of the supercooled water drop impact freeze over a temperature range of −4 °C to −12 °C.
Monika Feldmann, Urs Germann, Marco Gabella, and Alexis Berne
Weather Clim. Dynam., 2, 1225–1244, https://doi.org/10.5194/wcd-2-1225-2021, https://doi.org/10.5194/wcd-2-1225-2021, 2021
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Mesocyclones are the rotating updraught of supercell thunderstorms that present a particularly hazardous subset of thunderstorms. A first-time characterisation of the spatiotemporal occurrence of mesocyclones in the Alpine region is presented, using 5 years of Swiss operational radar data. We investigate parallels to hailstorms, particularly the influence of large-scale flow, daily cycles and terrain. Improving understanding of mesocyclones is valuable for risk assessment and warning purposes.
Jussi Leinonen, Jacopo Grazioli, and Alexis Berne
Atmos. Meas. Tech., 14, 6851–6866, https://doi.org/10.5194/amt-14-6851-2021, https://doi.org/10.5194/amt-14-6851-2021, 2021
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Measuring the shape, size and mass of a large number of snowflakes is a challenging task; it is hard to achieve in an automatic and instrumented manner. We present a method to retrieve these properties of individual snowflakes using as input a triplet of images/pictures automatically collected by a multi-angle snowflake camera (MASC) instrument. Our method, based on machine learning, is trained on artificially generated snowflakes and evaluated on 3D-printed snowflake replicas.
Marc Schwaerzel, Dominik Brunner, Fabian Jakub, Claudia Emde, Brigitte Buchmann, Alexis Berne, and Gerrit Kuhlmann
Atmos. Meas. Tech., 14, 6469–6482, https://doi.org/10.5194/amt-14-6469-2021, https://doi.org/10.5194/amt-14-6469-2021, 2021
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NO2 maps from airborne imaging remote sensing often appear much smoother than one would expect from high-resolution model simulations of NO2 over cities, despite the small ground-pixel size of the sensors. Our case study over Zurich, using the newly implemented building module of the MYSTIC radiative transfer solver, shows that the 3D effect can explain part of the smearing and that building shadows cause a noticeable underestimation and noise in the measured NO2 columns.
Anna Špačková, Vojtěch Bareš, Martin Fencl, Marc Schleiss, Joël Jaffrain, Alexis Berne, and Jörg Rieckermann
Earth Syst. Sci. Data, 13, 4219–4240, https://doi.org/10.5194/essd-13-4219-2021, https://doi.org/10.5194/essd-13-4219-2021, 2021
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An original dataset of microwave signal attenuation and rainfall variables was collected during 1-year-long field campaign. The monitored 38 GHz dual-polarized commercial microwave link with a short sampling resolution (4 s) was accompanied by five disdrometers and three rain gauges along its path. Antenna radomes were temporarily shielded for approximately half of the campaign period to investigate antenna wetting impacts.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Paraskevi Georgakaki, Aikaterini Bougiatioti, Jörg Wieder, Claudia Mignani, Fabiola Ramelli, Zamin A. Kanji, Jan Henneberger, Maxime Hervo, Alexis Berne, Ulrike Lohmann, and Athanasios Nenes
Atmos. Chem. Phys., 21, 10993–11012, https://doi.org/10.5194/acp-21-10993-2021, https://doi.org/10.5194/acp-21-10993-2021, 2021
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Aerosol and cloud observations coupled with a droplet activation parameterization was used to investigate the aerosol–cloud droplet link in alpine mixed-phase clouds. Predicted droplet number, Nd, agrees with observations and never exceeds a characteristic “limiting droplet number”, Ndlim, which depends solely on σw. Nd becomes velocity limited when it is within 50 % of Ndlim. Identifying when dynamical changes control Nd variability is central for understanding aerosol–cloud interactions.
Noémie Planat, Josué Gehring, Étienne Vignon, and Alexis Berne
Atmos. Meas. Tech., 14, 4543–4564, https://doi.org/10.5194/amt-14-4543-2021, https://doi.org/10.5194/amt-14-4543-2021, 2021
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We implement a new method to identify microphysical processes during cold precipitation events based on the sign of the vertical gradient of polarimetric radar variables. We analytically asses the meteorological conditions for this vertical analysis to hold, apply it on two study cases and successfully compare it with other methods informing about the microphysics. Finally, we are able to obtain the main vertical structure and characteristics of the different processes during these study cases.
Martin Lainer, Jordi Figueras i Ventura, Zaira Schauwecker, Marco Gabella, Montserrat F.-Bolaños, Reto Pauli, and Jacopo Grazioli
Atmos. Meas. Tech., 14, 3541–3560, https://doi.org/10.5194/amt-14-3541-2021, https://doi.org/10.5194/amt-14-3541-2021, 2021
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We show results from two unique measurement campaigns aimed at better understanding effects of large wind turbines on radar returns by deploying a mobile X-band weather radar system in the proximity of a small wind park. Measurements were taken in 24/7 operation with dedicated scan strategies to retrieve the variability and most extreme values of reflectivity and radar cross-section of the wind turbines. The findings are useful for wind turbine interference mitigation measures in radar systems.
Fabiola Ramelli, Jan Henneberger, Robert O. David, Johannes Bühl, Martin Radenz, Patric Seifert, Jörg Wieder, Annika Lauber, Julie T. Pasquier, Ronny Engelmann, Claudia Mignani, Maxime Hervo, and Ulrike Lohmann
Atmos. Chem. Phys., 21, 6681–6706, https://doi.org/10.5194/acp-21-6681-2021, https://doi.org/10.5194/acp-21-6681-2021, 2021
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Orographic mixed-phase clouds are an important source of precipitation, but the ice formation processes within them remain uncertain. Here we investigate the origin of ice crystals in a mixed-phase cloud in the Swiss Alps using aerosol and cloud data from in situ and remote sensing observations. We found that ice formation primarily occurs in cloud top generating cells. Our results indicate that secondary ice processes are active in the feeder region, which can enhance orographic precipitation.
Daniel Wolfensberger, Marco Gabella, Marco Boscacci, Urs Germann, and Alexis Berne
Atmos. Meas. Tech., 14, 3169–3193, https://doi.org/10.5194/amt-14-3169-2021, https://doi.org/10.5194/amt-14-3169-2021, 2021
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In this work, we present a novel quantitative precipitation estimation method for Switzerland that uses random forests, an ensemble-based machine learning technique. The estimator has been trained with a database of 4 years of ground and radar observations. The results of an in-depth evaluation indicate that, compared with the more classical method in use at MeteoSwiss, this novel estimator is able to reduce both the average error and bias of the predictions.
Anne-Claire Billault-Roux and Alexis Berne
Atmos. Meas. Tech., 14, 2749–2769, https://doi.org/10.5194/amt-14-2749-2021, https://doi.org/10.5194/amt-14-2749-2021, 2021
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In the context of climate studies, understanding the role of clouds on a global and local scale is of paramount importance. One aspect is the quantification of cloud liquid water, which impacts the Earth’s radiative balance. This is routinely achieved with radiometers operating at different frequencies. In this study, we propose an approach that uses a single-frequency radiometer and that can be applied at any location to retrieve vertically integrated quantities of liquid water and water vapor.
Fabiola Ramelli, Jan Henneberger, Robert O. David, Annika Lauber, Julie T. Pasquier, Jörg Wieder, Johannes Bühl, Patric Seifert, Ronny Engelmann, Maxime Hervo, and Ulrike Lohmann
Atmos. Chem. Phys., 21, 5151–5172, https://doi.org/10.5194/acp-21-5151-2021, https://doi.org/10.5194/acp-21-5151-2021, 2021
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Interactions between dynamics, microphysics and orography can enhance precipitation. Yet the exact role of these interactions is still uncertain. Here we investigate the role of low-level blocking and turbulence for precipitation by combining remote sensing and in situ observations. The observations show that blocked flow can induce the formation of feeder clouds and that turbulence can enhance hydrometeor growth, demonstrating the importance of local flow effects for orographic precipitation.
Annika Lauber, Jan Henneberger, Claudia Mignani, Fabiola Ramelli, Julie T. Pasquier, Jörg Wieder, Maxime Hervo, and Ulrike Lohmann
Atmos. Chem. Phys., 21, 3855–3870, https://doi.org/10.5194/acp-21-3855-2021, https://doi.org/10.5194/acp-21-3855-2021, 2021
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An accurate prediction of the ice crystal number concentration (ICNC) is important to determine the radiation budget, lifetime, and precipitation formation of clouds. Even though secondary-ice processes can increase the ICNC by several orders of magnitude, they are poorly constrained and lack a well-founded quantification. During measurements on a mountain slope, a high ICNC of small ice crystals was observed just below 0 °C, attributed to a secondary-ice process and parametrized in this study.
Josué Gehring, Alfonso Ferrone, Anne-Claire Billault-Roux, Nikola Besic, Kwang Deuk Ahn, GyuWon Lee, and Alexis Berne
Earth Syst. Sci. Data, 13, 417–433, https://doi.org/10.5194/essd-13-417-2021, https://doi.org/10.5194/essd-13-417-2021, 2021
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This article describes a dataset of precipitation and cloud measurements collected from November 2017 to March 2018 in Pyeongchang, South Korea. The dataset includes weather radar data and images of snowflakes. It allows for studying the snowfall intensity; wind conditions; and shape, size and fall speed of snowflakes. Classifications of the types of snowflakes show that aggregates of ice crystals were dominant. This dataset represents a unique opportunity to study snowfall in this region.
Georgia Sotiropoulou, Étienne Vignon, Gillian Young, Hugh Morrison, Sebastian J. O'Shea, Thomas Lachlan-Cope, Alexis Berne, and Athanasios Nenes
Atmos. Chem. Phys., 21, 755–771, https://doi.org/10.5194/acp-21-755-2021, https://doi.org/10.5194/acp-21-755-2021, 2021
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Summer clouds have a significant impact on the radiation budget of the Antarctic surface and thus on ice-shelf melting. However, these are poorly represented in climate models due to errors in their microphysical structure, including the number of ice crystals that they contain. We show that breakup from ice particle collisions can substantially magnify the ice crystal number concentration with significant implications for surface radiation. This process is currently missing in climate models.
Claudia Mignani, Jörg Wieder, Michael A. Sprenger, Zamin A. Kanji, Jan Henneberger, Christine Alewell, and Franz Conen
Atmos. Chem. Phys., 21, 657–664, https://doi.org/10.5194/acp-21-657-2021, https://doi.org/10.5194/acp-21-657-2021, 2021
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Most precipitation above land starts with ice in clouds. It is promoted by extremely rare particles. Some ice-nucleating particles (INPs) cause cloud droplets to already freeze above −15°C, a temperature at which many clouds begin to snow. We found that the abundance of such INPs among other particles of similar size is highest in precipitating air masses and lowest when air carries desert dust. This brings us closer to understanding the interactions between land, clouds, and precipitation.
Jessica Slater, Juha Tonttila, Gordon McFiggans, Paul Connolly, Sami Romakkaniemi, Thomas Kühn, and Hugh Coe
Atmos. Chem. Phys., 20, 11893–11906, https://doi.org/10.5194/acp-20-11893-2020, https://doi.org/10.5194/acp-20-11893-2020, 2020
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The feedback effect between aerosol particles, radiation and meteorology reduces turbulent motion and results in increased surface aerosol concentrations during Beijing haze. Observational analysis and regional modelling studies have examined the feedback effect but these studies are limited. In this work, we set up a high-resolution model for the Beijing environment to examine the sensitivity of the aerosol feedback effect to initial meteorological conditions and aerosol loading.
Martin Heinritzi, Lubna Dada, Mario Simon, Dominik Stolzenburg, Andrea C. Wagner, Lukas Fischer, Lauri R. Ahonen, Stavros Amanatidis, Rima Baalbaki, Andrea Baccarini, Paulus S. Bauer, Bernhard Baumgartner, Federico Bianchi, Sophia Brilke, Dexian Chen, Randall Chiu, Antonio Dias, Josef Dommen, Jonathan Duplissy, Henning Finkenzeller, Carla Frege, Claudia Fuchs, Olga Garmash, Hamish Gordon, Manuel Granzin, Imad El Haddad, Xucheng He, Johanna Helm, Victoria Hofbauer, Christopher R. Hoyle, Juha Kangasluoma, Timo Keber, Changhyuk Kim, Andreas Kürten, Houssni Lamkaddam, Tiia M. Laurila, Janne Lampilahti, Chuan Ping Lee, Katrianne Lehtipalo, Markus Leiminger, Huajun Mai, Vladimir Makhmutov, Hanna Elina Manninen, Ruby Marten, Serge Mathot, Roy Lee Mauldin, Bernhard Mentler, Ugo Molteni, Tatjana Müller, Wei Nie, Tuomo Nieminen, Antti Onnela, Eva Partoll, Monica Passananti, Tuukka Petäjä, Joschka Pfeifer, Veronika Pospisilova, Lauriane L. J. Quéléver, Matti P. Rissanen, Clémence Rose, Siegfried Schobesberger, Wiebke Scholz, Kay Scholze, Mikko Sipilä, Gerhard Steiner, Yuri Stozhkov, Christian Tauber, Yee Jun Tham, Miguel Vazquez-Pufleau, Annele Virtanen, Alexander L. Vogel, Rainer Volkamer, Robert Wagner, Mingyi Wang, Lena Weitz, Daniela Wimmer, Mao Xiao, Chao Yan, Penglin Ye, Qiaozhi Zha, Xueqin Zhou, Antonio Amorim, Urs Baltensperger, Armin Hansel, Markku Kulmala, António Tomé, Paul M. Winkler, Douglas R. Worsnop, Neil M. Donahue, Jasper Kirkby, and Joachim Curtius
Atmos. Chem. Phys., 20, 11809–11821, https://doi.org/10.5194/acp-20-11809-2020, https://doi.org/10.5194/acp-20-11809-2020, 2020
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With experiments performed at CLOUD, we show how isoprene interferes in monoterpene oxidation via RO2 termination at atmospherically relevant concentrations. This interference shifts the distribution of highly oxygenated organic molecules (HOMs) away from C20 class dimers towards C15 class dimers, which subsequently reduces both biogenic nucleation and early growth rates. Our results may help to understand the absence of new-particle formation in isoprene-rich environments.
Marc Schwaerzel, Claudia Emde, Dominik Brunner, Randulph Morales, Thomas Wagner, Alexis Berne, Brigitte Buchmann, and Gerrit Kuhlmann
Atmos. Meas. Tech., 13, 4277–4293, https://doi.org/10.5194/amt-13-4277-2020, https://doi.org/10.5194/amt-13-4277-2020, 2020
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Horizontal homogeneity is often assumed for trace gases remote sensing, although it is not valid where trace gas concentrations have high spatial variability, e.g., in cities. We show the importance of 3D effects for MAX-DOAS and airborne imaging spectrometers using 3D-box air mass factors implemented in the MYSTIC radiative transfer solver. In both cases, 3D information is invaluable for interpreting the measurements, as not considering 3D effects can lead to misinterpretation of measurements.
Mario Simon, Lubna Dada, Martin Heinritzi, Wiebke Scholz, Dominik Stolzenburg, Lukas Fischer, Andrea C. Wagner, Andreas Kürten, Birte Rörup, Xu-Cheng He, João Almeida, Rima Baalbaki, Andrea Baccarini, Paulus S. Bauer, Lisa Beck, Anton Bergen, Federico Bianchi, Steffen Bräkling, Sophia Brilke, Lucia Caudillo, Dexian Chen, Biwu Chu, António Dias, Danielle C. Draper, Jonathan Duplissy, Imad El-Haddad, Henning Finkenzeller, Carla Frege, Loic Gonzalez-Carracedo, Hamish Gordon, Manuel Granzin, Jani Hakala, Victoria Hofbauer, Christopher R. Hoyle, Changhyuk Kim, Weimeng Kong, Houssni Lamkaddam, Chuan P. Lee, Katrianne Lehtipalo, Markus Leiminger, Huajun Mai, Hanna E. Manninen, Guillaume Marie, Ruby Marten, Bernhard Mentler, Ugo Molteni, Leonid Nichman, Wei Nie, Andrea Ojdanic, Antti Onnela, Eva Partoll, Tuukka Petäjä, Joschka Pfeifer, Maxim Philippov, Lauriane L. J. Quéléver, Ananth Ranjithkumar, Matti P. Rissanen, Simon Schallhart, Siegfried Schobesberger, Simone Schuchmann, Jiali Shen, Mikko Sipilä, Gerhard Steiner, Yuri Stozhkov, Christian Tauber, Yee J. Tham, António R. Tomé, Miguel Vazquez-Pufleau, Alexander L. Vogel, Robert Wagner, Mingyi Wang, Dongyu S. Wang, Yonghong Wang, Stefan K. Weber, Yusheng Wu, Mao Xiao, Chao Yan, Penglin Ye, Qing Ye, Marcel Zauner-Wieczorek, Xueqin Zhou, Urs Baltensperger, Josef Dommen, Richard C. Flagan, Armin Hansel, Markku Kulmala, Rainer Volkamer, Paul M. Winkler, Douglas R. Worsnop, Neil M. Donahue, Jasper Kirkby, and Joachim Curtius
Atmos. Chem. Phys., 20, 9183–9207, https://doi.org/10.5194/acp-20-9183-2020, https://doi.org/10.5194/acp-20-9183-2020, 2020
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Highly oxygenated organic compounds (HOMs) have been identified as key vapors involved in atmospheric new-particle formation (NPF). The molecular distribution, HOM yield, and NPF from α-pinene oxidation experiments were measured at the CLOUD chamber over a wide tropospheric-temperature range. This study shows on a molecular scale that despite the sharp reduction in HOM yield at lower temperatures, the reduced volatility counteracts this effect and leads to an overall increase in the NPF rate.
Josué Gehring, Annika Oertel, Étienne Vignon, Nicolas Jullien, Nikola Besic, and Alexis Berne
Atmos. Chem. Phys., 20, 7373–7392, https://doi.org/10.5194/acp-20-7373-2020, https://doi.org/10.5194/acp-20-7373-2020, 2020
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In this study, we analyse how large-scale meteorological conditions influenced the local enhancement of snowfall during an intense precipitation event in Korea. We used atmospheric models, weather radars and snowflake images. We found out that a rising airstream in the warm sector of the low pressure system associated to this event influenced the evolution of snowfall. This study highlights the importance of interactions between large and local scales in this intense precipitation event.
Jussi Leinonen and Alexis Berne
Atmos. Meas. Tech., 13, 2949–2964, https://doi.org/10.5194/amt-13-2949-2020, https://doi.org/10.5194/amt-13-2949-2020, 2020
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The appearance of snowflakes provides a signature of the atmospheric processes that created them. To get this information from large numbers of snowflake images, automated analysis using computer image recognition is needed. In this work, we use a neural network that learns the structure of the snowflake images to divide a snowflake dataset into classes corresponding to different sizes and structures. Unlike with most comparable methods, only minimal input from a human expert is needed.
Nicolas Jullien, Étienne Vignon, Michael Sprenger, Franziska Aemisegger, and Alexis Berne
The Cryosphere, 14, 1685–1702, https://doi.org/10.5194/tc-14-1685-2020, https://doi.org/10.5194/tc-14-1685-2020, 2020
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Although snowfall is the main input of water to the Antarctic ice sheet, snowflakes are often evaporated by dry and fierce winds near the surface of the continent. The amount of snow that actually reaches the ground is therefore considerably reduced. By analyzing the position of cyclones and fronts as well as by back-tracing the atmospheric moisture pathway towards Antarctica, this study explains in which meteorological conditions snowfall is either completely evaporated or reaches the ground.
Floor van den Heuvel, Loris Foresti, Marco Gabella, Urs Germann, and Alexis Berne
Atmos. Meas. Tech., 13, 2481–2500, https://doi.org/10.5194/amt-13-2481-2020, https://doi.org/10.5194/amt-13-2481-2020, 2020
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In areas with reduced visibility at the ground level, radar precipitation measurements higher up in the atmosphere need to be extrapolated to the ground and be corrected for the vertical change (i.e. growth and transformation) of precipitation. This study proposes a method based on hydrometeor proportions and machine learning (ML) to apply these corrections at smaller spatiotemporal scales. In comparison with existing techniques, the ML methods can make predictions from higher altitudes.
Georgios Touloupas, Annika Lauber, Jan Henneberger, Alexander Beck, and Aurélien Lucchi
Atmos. Meas. Tech., 13, 2219–2239, https://doi.org/10.5194/amt-13-2219-2020, https://doi.org/10.5194/amt-13-2219-2020, 2020
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Images of cloud particles give important information for improving our understanding of microphysical cloud processes. For phase-resolved measurements, a large number of water droplets and ice crystals need to be classified by an automated approach. In this study, a convolutional neural network was designed, which exceeds the classification ability of traditional methods and therefore shortens the analysis procedure of cloud particle images.
Gary Lloyd, Thomas Choularton, Keith Bower, Jonathan Crosier, Martin Gallagher, Michael Flynn, James Dorsey, Dantong Liu, Jonathan W. Taylor, Oliver Schlenczek, Jacob Fugal, Stephan Borrmann, Richard Cotton, Paul Field, and Alan Blyth
Atmos. Chem. Phys., 20, 3895–3904, https://doi.org/10.5194/acp-20-3895-2020, https://doi.org/10.5194/acp-20-3895-2020, 2020
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Measurements of liquid and ice cloud particles were made using an aircraft to penetrate fresh growing convective clouds in the tropical Atlantic. We found small ice particles at surprisingly high temperatures just below freezing. At colder temperatures secondary ice processes rapidly generated high concentrations of ice crystals.
Fabiola Ramelli, Alexander Beck, Jan Henneberger, and Ulrike Lohmann
Atmos. Meas. Tech., 13, 925–939, https://doi.org/10.5194/amt-13-925-2020, https://doi.org/10.5194/amt-13-925-2020, 2020
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Boundary layer clouds are influenced by many physical and dynamical processes, making accurate forecasting difficult. Here we present a new measurement platform on a tethered balloon to measure cloud microphysical and meteorological profiles. The unique combination of holography and balloon-borne observations allows high-resolution measurements in a well-defined volume. Field measurements in stratus clouds over the Swiss Plateau revealed unique microphysical signatures in the cloud structure.
Georgia Sotiropoulou, Sylvia Sullivan, Julien Savre, Gary Lloyd, Thomas Lachlan-Cope, Annica M. L. Ekman, and Athanasios Nenes
Atmos. Chem. Phys., 20, 1301–1316, https://doi.org/10.5194/acp-20-1301-2020, https://doi.org/10.5194/acp-20-1301-2020, 2020
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Arctic clouds constitute a large source of uncertainty in predictions of future climate. Observations indicate that the number concentration of cloud ice crystals exceeds the concentration of aerosols that can act as ice-nucleating particles (INPs). We show that ice multiplication due to mechanical break-up upon collisions between the few primary ice crystals (formed from INPs) can explain the discrepancy. Including a description of the process in climate models can improve cloud representation.
Mathieu Schaer, Christophe Praz, and Alexis Berne
The Cryosphere, 14, 367–384, https://doi.org/10.5194/tc-14-367-2020, https://doi.org/10.5194/tc-14-367-2020, 2020
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Wind and precipitation often occur together, making the distinction between particles coming from the atmosphere and those blown by the wind difficult. This is however a crucial task to accurately close the surface mass balance. We propose an algorithm based on Gaussian mixture models to separate blowing snow and precipitation in images collected by a Multi-Angle Snowflake Camera (MASC). The algorithm is trained and (positively) evaluated using data collected in the Swiss Alps and in Antarctica.
Kathryn Fowler, Paul Connolly, and David Topping
Atmos. Chem. Phys., 20, 683–698, https://doi.org/10.5194/acp-20-683-2020, https://doi.org/10.5194/acp-20-683-2020, 2020
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Observations of low–temperature cirrus clouds have found unexpectedly low ice crystal numbers and high supersaturations, suggesting an incomplete understanding of the freezing mechanisms under these conditions. The existence of viscous organic aerosol has offered alternative ice nucleation pathways, which have been observed in laboratory studies. We have developed the first cloud parcel model to investigate the effect of viscosity on ice nucleation.
Jordi Figueras i Ventura, Nicolau Pineda, Nikola Besic, Jacopo Grazioli, Alessandro Hering, Oscar A. van der Velde, David Romero, Antonio Sunjerga, Amirhossein Mostajabi, Mohammad Azadifar, Marcos Rubinstein, Joan Montanyà, Urs Germann, and Farhad Rachidi
Atmos. Meas. Tech., 12, 5573–5591, https://doi.org/10.5194/amt-12-5573-2019, https://doi.org/10.5194/amt-12-5573-2019, 2019
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This paper presents an analysis of the lightning production of convective cells. Polarimetric weather radar data were used to identify and characterize the convective cells while lightning was detected using the EUCLID network and a lightning mapping array deployed during the summer of 2017 in the northeastern part of Switzerland. In it we show that there is a good correlation between the height of the rimed-particle column and the intensity of the lightning activity in the convective cell.
Jonathan W. Taylor, Sophie L. Haslett, Keith Bower, Michael Flynn, Ian Crawford, James Dorsey, Tom Choularton, Paul J. Connolly, Valerian Hahn, Christiane Voigt, Daniel Sauer, Régis Dupuy, Joel Brito, Alfons Schwarzenboeck, Thierry Bourriane, Cyrielle Denjean, Phil Rosenberg, Cyrille Flamant, James D. Lee, Adam R. Vaughan, Peter G. Hill, Barbara Brooks, Valéry Catoire, Peter Knippertz, and Hugh Coe
Atmos. Chem. Phys., 19, 8503–8522, https://doi.org/10.5194/acp-19-8503-2019, https://doi.org/10.5194/acp-19-8503-2019, 2019
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Low-level clouds cover a wide area of southern West Africa (SWA) and play an important role in the region's climate, reflecting sunlight away from the surface. We performed aircraft measurements of aerosols and clouds over SWA during the 2016 summer monsoon and found pollution, and polluted clouds, across the whole region. Smoke from biomass burning in Central Africa is transported to West Africa, causing a polluted background which limits the effect of local pollution on cloud properties.
Jordi Figueras i Ventura, Nicolau Pineda, Nikola Besic, Jacopo Grazioli, Alessandro Hering, Oscar A. van der Velde, David Romero, Antonio Sunjerga, Amirhossein Mostajabi, Mohammad Azadifar, Marcos Rubinstein, Joan Montanyà, Urs Germann, and Farhad Rachidi
Atmos. Meas. Tech., 12, 2881–2911, https://doi.org/10.5194/amt-12-2881-2019, https://doi.org/10.5194/amt-12-2881-2019, 2019
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This paper presents an analysis of a large dataset of lightning and polarimetric weather radar data collected over the course of a lightning measurement campaign that took place in the summer of 2017 in the area surrounding Säntis in northeastern Switzerland. We show that polarimetric weather radar data can be helpful in determining regions where lightning is more likely to occur, which is a first step towards a lightning nowcasting system.
Étienne Vignon, Olivier Traullé, and Alexis Berne
Atmos. Chem. Phys., 19, 4659–4683, https://doi.org/10.5194/acp-19-4659-2019, https://doi.org/10.5194/acp-19-4659-2019, 2019
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The future sea-level rise will depend on how much the Antarctic ice sheet gain – via precipitation – or loose mass. The simulation of precipitation by numerical models used for projections depends on the representation of the atmospheric circulation over and around Antarctica. Using daily measurements from balloon soundings at nine Antarctic stations, this study characterizes the structure of the atmosphere over the Antarctic coast and its representation in atmospheric simulations.
Florentin Lemonnier, Jean-Baptiste Madeleine, Chantal Claud, Christophe Genthon, Claudio Durán-Alarcón, Cyril Palerme, Alexis Berne, Niels Souverijns, Nicole van Lipzig, Irina V. Gorodetskaya, Tristan L'Ecuyer, and Norman Wood
The Cryosphere, 13, 943–954, https://doi.org/10.5194/tc-13-943-2019, https://doi.org/10.5194/tc-13-943-2019, 2019
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Evaluation of the vertical precipitation rate profiles of CloudSat radar by comparison with two surface-based micro-rain radars (MRR) located at two antarctic stations gives a near-perfect correlation between both datasets, even though climatic and geographic conditions are different for the stations. A better understanding and reassessment of CloudSat uncertainties ranging from −13 % up to +22 % confirms the robustness of the CloudSat retrievals of snowfall over Antarctica.
Claudio Durán-Alarcón, Brice Boudevillain, Christophe Genthon, Jacopo Grazioli, Niels Souverijns, Nicole P. M. van Lipzig, Irina V. Gorodetskaya, and Alexis Berne
The Cryosphere, 13, 247–264, https://doi.org/10.5194/tc-13-247-2019, https://doi.org/10.5194/tc-13-247-2019, 2019
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Precipitation is the main input in the surface mass balance of the Antarctic ice sheet, but it is still poorly understood due to a lack of observations in this region. We analyzed the vertical structure of the precipitation using multiyear observation of vertically pointing micro rain radars (MRRs) at two stations located in East Antarctica. The use of MRRs showed the potential to study the effect of climatology and hydrometeor microphysics on the vertical structure of Antarctic precipitation.
Franco Marenco, Claire Ryder, Victor Estellés, Debbie O'Sullivan, Jennifer Brooke, Luke Orgill, Gary Lloyd, and Martin Gallagher
Atmos. Chem. Phys., 18, 17655–17668, https://doi.org/10.5194/acp-18-17655-2018, https://doi.org/10.5194/acp-18-17655-2018, 2018
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The AER-D airborne campaign characterised Saharan dust in the eastern Atlantic. We report an instance of unusual vertical structure of the Saharan Air Layer during an intense event, showing a large radiative impact and correlated with anomalous lightning activity. Moreover, we report a significant presence of giant dust particles. This is important because most models would miss the giant particles. Our findings may change the way we represent dust transport and deposition in the Atlantic.
Claire L. Ryder, Franco Marenco, Jennifer K. Brooke, Victor Estelles, Richard Cotton, Paola Formenti, James B. McQuaid, Hannah C. Price, Dantong Liu, Patrick Ausset, Phil D. Rosenberg, Jonathan W. Taylor, Tom Choularton, Keith Bower, Hugh Coe, Martin Gallagher, Jonathan Crosier, Gary Lloyd, Eleanor J. Highwood, and Benjamin J. Murray
Atmos. Chem. Phys., 18, 17225–17257, https://doi.org/10.5194/acp-18-17225-2018, https://doi.org/10.5194/acp-18-17225-2018, 2018
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Every year, millions of tons of Saharan dust particles are carried across the Atlantic by the wind, where they can affect weather patterns and climate. Their sizes span orders of magnitude, but the largest (over 10 microns – around the width of a human hair) are difficult to measure and few observations exist. Here we show new aircraft observations of large dust particles, finding more than we would expect, and we quantify their properties which allow them to interact with atmospheric radiation.
Gary Lloyd, Thomas W. Choularton, Keith N. Bower, Martin W. Gallagher, Jonathan Crosier, Sebastian O'Shea, Steven J. Abel, Stuart Fox, Richard Cotton, and Ian A. Boutle
Atmos. Chem. Phys., 18, 17191–17206, https://doi.org/10.5194/acp-18-17191-2018, https://doi.org/10.5194/acp-18-17191-2018, 2018
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The work deals with cold weather outbreaks at high latitudes that often bring severe weather such as heavy snow, lightning and high winds but are poorly forecast by weather models. Here we made measurements of these events and the clouds associated with them using a research aircraft. We found that the properties of these clouds were often very different to what the models predicted, and these results can potentially be used to bring significant improvement to the forecasting of these events.
Niels Souverijns, Alexandra Gossart, Stef Lhermitte, Irina V. Gorodetskaya, Jacopo Grazioli, Alexis Berne, Claudio Duran-Alarcon, Brice Boudevillain, Christophe Genthon, Claudio Scarchilli, and Nicole P. M. van Lipzig
The Cryosphere, 12, 3775–3789, https://doi.org/10.5194/tc-12-3775-2018, https://doi.org/10.5194/tc-12-3775-2018, 2018
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Snowfall observations over Antarctica are scarce and currently limited to information from the CloudSat satellite. Here, a first evaluation of the CloudSat snowfall record is performed using observations of ground-based precipitation radars. Results indicate an accurate representation of the snowfall climatology over Antarctica, despite the low overpass frequency of the satellite, outperforming state-of-the-art model estimates. Individual snowfall events are however not well represented.
Franziska Gerber, Nikola Besic, Varun Sharma, Rebecca Mott, Megan Daniels, Marco Gabella, Alexis Berne, Urs Germann, and Michael Lehning
The Cryosphere, 12, 3137–3160, https://doi.org/10.5194/tc-12-3137-2018, https://doi.org/10.5194/tc-12-3137-2018, 2018
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A comparison of winter precipitation variability in operational radar measurements and high-resolution simulations reveals that large-scale variability is well captured by the model, depending on the event. Precipitation variability is driven by topography and wind. A good portion of small-scale variability is captured at the highest resolution. This is essential to address small-scale precipitation processes forming the alpine snow seasonal snow cover – an important source of water.
Floor van den Heuvel, Marco Gabella, Urs Germann, and Alexis Berne
Atmos. Meas. Tech., 11, 5181–5198, https://doi.org/10.5194/amt-11-5181-2018, https://doi.org/10.5194/amt-11-5181-2018, 2018
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The paper aims at characterising and quantifying the spatio-temporal variability of the melting layer (ML; transition zone from solid to liquid precipitation). A method based on the Fourier transform is found to accurately describe different ML signatures. Hence, it is applied to characterise the ML variability in a relatively flat area and in an inner Alpine valley in Switzerland, where the variability at smaller spatial scales is found to be relatively more important.
Christophe Genthon, Alexis Berne, Jacopo Grazioli, Claudio Durán Alarcón, Christophe Praz, and Brice Boudevillain
Earth Syst. Sci. Data, 10, 1605–1612, https://doi.org/10.5194/essd-10-1605-2018, https://doi.org/10.5194/essd-10-1605-2018, 2018
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Antarctica suffers from a severe shortage of in situ observations of precipitation. The APRES3 program contributes to improving observation from both the surface and from space. A field campaign with various instruments was deployed at the coast of Adélie Land, with an intensive observing period in austral summer 2015–16, then continuous radar monitoring through 2016 and beyond. This paper provides a compact presentation of the APRES3 dataset, which is now made open to the scientific community.
Nikola Besic, Josué Gehring, Christophe Praz, Jordi Figueras i Ventura, Jacopo Grazioli, Marco Gabella, Urs Germann, and Alexis Berne
Atmos. Meas. Tech., 11, 4847–4866, https://doi.org/10.5194/amt-11-4847-2018, https://doi.org/10.5194/amt-11-4847-2018, 2018
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In this paper we propose an innovative approach for hydrometeor de-mixing, i.e., to identify and quantify the presence of mixtures of different hydrometeor types in a radar sampling volume. It is a bin-based approach, inspired by conventional decomposition methods and evaluated using C- and X-band radar measurements compared with synchronous ground observations. The paper also investigates the potential influence of incoherency in the backscattering from hydrometeor mixtures in a radar volume.
Matthew Crooks, Paul Connolly, and Gordon McFiggans
Geosci. Model Dev., 11, 3261–3278, https://doi.org/10.5194/gmd-11-3261-2018, https://doi.org/10.5194/gmd-11-3261-2018, 2018
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Clouds form when water condenses onto particles in the atmosphere and the size and chemical composition of these particles can have a large influence over how much water condenses and the subsequent formation of cloud. Additional gases exist in the atmosphere that can condense onto the aerosol particles and change their composition. We present a fast and efficient method of calculating the effect of atmospheric gases on the formation of cloud that can be used in climate and weather models.
Robin G. Stevens, Katharina Loewe, Christopher Dearden, Antonios Dimitrelos, Anna Possner, Gesa K. Eirund, Tomi Raatikainen, Adrian A. Hill, Benjamin J. Shipway, Jonathan Wilkinson, Sami Romakkaniemi, Juha Tonttila, Ari Laaksonen, Hannele Korhonen, Paul Connolly, Ulrike Lohmann, Corinna Hoose, Annica M. L. Ekman, Ken S. Carslaw, and Paul R. Field
Atmos. Chem. Phys., 18, 11041–11071, https://doi.org/10.5194/acp-18-11041-2018, https://doi.org/10.5194/acp-18-11041-2018, 2018
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We perform a model intercomparison of summertime high Arctic clouds. Observed concentrations of aerosol particles necessary for cloud formation fell to extremely low values, coincident with a transition from cloudy to nearly cloud-free conditions. Previous analyses have suggested that at these low concentrations, the radiative properties of the clouds are determined primarily by these particle concentrations. The model results strongly support this hypothesis.
Fanny Jeanneret, Giovanni Martucci, Simon Pinnock, and Alexis Berne
Atmos. Meas. Tech., 11, 4153–4170, https://doi.org/10.5194/amt-11-4153-2018, https://doi.org/10.5194/amt-11-4153-2018, 2018
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Above mountainous regions, satellites may have difficulty in discriminating snow from clouds: this study proposes a new method that combines different ground-based measurements to assess the sky cloudiness with high temporal resolution. The method's output is used as input to a model capable of identifying false satellite cloud detections. Results show that 62 ± 13 % of these false detections can be identified by the model when applied to the AVHRR-PM and MODIS Aqua data sets of the Cloud_cci.
Wiebke Frey, Dawei Hu, James Dorsey, M. Rami Alfarra, Aki Pajunoja, Annele Virtanen, Paul Connolly, and Gordon McFiggans
Atmos. Chem. Phys., 18, 9393–9409, https://doi.org/10.5194/acp-18-9393-2018, https://doi.org/10.5194/acp-18-9393-2018, 2018
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The coupled system of the Manchester Aerosol Chamber and Manchester Ice Cloud Chamber was used to study the ice-forming abilities of secondary
organic aerosol particles under mixed-phase cloud conditions. Given the vast abundance of secondary organic particles in the atmosphere, they
might present an important contribution to ice-nucleating particles. However, we find that in the studied temperature range (20 to 28 °C)
the secondary organic particles do not nucleate ice particles.
Daniel Wolfensberger and Alexis Berne
Atmos. Meas. Tech., 11, 3883–3916, https://doi.org/10.5194/amt-11-3883-2018, https://doi.org/10.5194/amt-11-3883-2018, 2018
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This work presents a polarimetric forward operator for the COSMO weather prediction model. This tool is able to simulate radar observables from the state of the atmosphere simulated by the model, taking into account most physical aspects of radar beam propagation and backscattering. This operator was validated with a large dataset of radar observations from several instruments and it was shown that is able to simulate a realistic radar signature in liquid precipitation.
Alexander Beck, Jan Henneberger, Jacob P. Fugal, Robert O. David, Larissa Lacher, and Ulrike Lohmann
Atmos. Chem. Phys., 18, 8909–8927, https://doi.org/10.5194/acp-18-8909-2018, https://doi.org/10.5194/acp-18-8909-2018, 2018
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This study assesses the impact of surface processes (e.g. blowing snow) on in situ cloud observations at Sonnblick Observatory. Vertical profiles of ice crystal number concentrations (ICNCs) above a snow-covered surface were observed up to a height of 10 m. The ICNC near the ground is at least a factor of 2 larger than at 10 m. Therefore, in situ measurements of ICNCs at mountain-top research stations close to the surface are strongly influenced by surface processes and overestimate the ICNC.
Emma L. Simpson, Paul J. Connolly, and Gordon McFiggans
Atmos. Chem. Phys., 18, 7237–7250, https://doi.org/10.5194/acp-18-7237-2018, https://doi.org/10.5194/acp-18-7237-2018, 2018
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This study explores the process of ice formation in clouds by conducting computer model simulations and laboratory experiments in a cloud chamber. We show that the formation of ice in clouds can be limited by the presence of atmospheric aerosol particles and that further research is required to identify the requirements for freezing, e.g. minimum mass of water, in order to accurately calculate ice formation and thus improve climate and weather prediction.
Dantong Liu, Jonathan W. Taylor, Jonathan Crosier, Nicholas Marsden, Keith N. Bower, Gary Lloyd, Claire L. Ryder, Jennifer K. Brooke, Richard Cotton, Franco Marenco, Alan Blyth, Zhiqiang Cui, Victor Estelles, Martin Gallagher, Hugh Coe, and Tom W. Choularton
Atmos. Chem. Phys., 18, 3817–3838, https://doi.org/10.5194/acp-18-3817-2018, https://doi.org/10.5194/acp-18-3817-2018, 2018
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This article presents measurements of aerosol properties off the coast of west Africa during August 2015. For the first time, an airborne laser-induced incandescence instrument was deployed to measure the hematite content of dust. The single scattering albedo of dust was found to be influenced by the hematite content, but depended on the dust source and potential dust age. This highlights the importance of size-dependent composition in determining the optical properties of dust.
Kathryn Fowler, Paul J. Connolly, David O. Topping, and Simon O'Meara
Atmos. Chem. Phys., 18, 1629–1642, https://doi.org/10.5194/acp-18-1629-2018, https://doi.org/10.5194/acp-18-1629-2018, 2018
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This is the first time the Maxwell–Stefan framework has been applied to an atmospheric aerosol core–shell model and shows that there is a complex interplay between the viscous and solubility effects on aerosol composition. Understanding aerosol composition is essential to accurately model their interactions within atmospheric systems. We use simple binary systems to demonstrate how viscosity and solubility both play a role in affecting the rate of diffusion through aerosol particles.
Gillian Young, Paul J. Connolly, Christopher Dearden, and Thomas W. Choularton
Atmos. Chem. Phys., 18, 1475–1494, https://doi.org/10.5194/acp-18-1475-2018, https://doi.org/10.5194/acp-18-1475-2018, 2018
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Large-scale subsidence, associated with high-pressure systems, is often used in cloud-resolving models to maintain the height of boundary layer clouds; however, its influence on the small-scale interactions in mixed-phase clouds has not been previously investigated. Using large-eddy simulations, we have identified a relationship between subsidence and convection development in such clouds, with implications for mixed-phase boundary layer clouds forming in the ocean-exposed Arctic regions.
Olivia Goulden, Matthew Crooks, and Paul Connolly
Atmos. Chem. Phys., 18, 275–287, https://doi.org/10.5194/acp-18-275-2018, https://doi.org/10.5194/acp-18-275-2018, 2018
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The formation of cloud from the condensation of water vapour in the atmosphere on aerosol particles is highly dependent of the chemical properties of the particles. The chemistry is further complicated by the presence of condensible gases in the atmosphere other than water. We provide several methods of including the complicated chemical properties of the aerosol particles and condensing gases into single parameter descriptions, which are suitable for inclusion in large-scale models.
Carla Frege, Ismael K. Ortega, Matti P. Rissanen, Arnaud P. Praplan, Gerhard Steiner, Martin Heinritzi, Lauri Ahonen, António Amorim, Anne-Kathrin Bernhammer, Federico Bianchi, Sophia Brilke, Martin Breitenlechner, Lubna Dada, António Dias, Jonathan Duplissy, Sebastian Ehrhart, Imad El-Haddad, Lukas Fischer, Claudia Fuchs, Olga Garmash, Marc Gonin, Armin Hansel, Christopher R. Hoyle, Tuija Jokinen, Heikki Junninen, Jasper Kirkby, Andreas Kürten, Katrianne Lehtipalo, Markus Leiminger, Roy Lee Mauldin, Ugo Molteni, Leonid Nichman, Tuukka Petäjä, Nina Sarnela, Siegfried Schobesberger, Mario Simon, Mikko Sipilä, Dominik Stolzenburg, António Tomé, Alexander L. Vogel, Andrea C. Wagner, Robert Wagner, Mao Xiao, Chao Yan, Penglin Ye, Joachim Curtius, Neil M. Donahue, Richard C. Flagan, Markku Kulmala, Douglas R. Worsnop, Paul M. Winkler, Josef Dommen, and Urs Baltensperger
Atmos. Chem. Phys., 18, 65–79, https://doi.org/10.5194/acp-18-65-2018, https://doi.org/10.5194/acp-18-65-2018, 2018
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It was recently shown that biogenic highly oxygenated molecules (HOMs) form particles in the absence of sulfuric acid and ions enhance the nucleation rate. Here we compare the molecular composition of positive and negative HOM clusters at 25, 5 and −25 °C. At lower temperatures the HOM average oxygen-to-carbon ratio decreases indicating a reduction in the rate of autoxidation due to rather high activation energy. The experimental findings are supported by quantum chemical calculations.
Robert Wagner, Chao Yan, Katrianne Lehtipalo, Jonathan Duplissy, Tuomo Nieminen, Juha Kangasluoma, Lauri R. Ahonen, Lubna Dada, Jenni Kontkanen, Hanna E. Manninen, Antonio Dias, Antonio Amorim, Paulus S. Bauer, Anton Bergen, Anne-Kathrin Bernhammer, Federico Bianchi, Sophia Brilke, Stephany Buenrostro Mazon, Xuemeng Chen, Danielle C. Draper, Lukas Fischer, Carla Frege, Claudia Fuchs, Olga Garmash, Hamish Gordon, Jani Hakala, Liine Heikkinen, Martin Heinritzi, Victoria Hofbauer, Christopher R. Hoyle, Jasper Kirkby, Andreas Kürten, Alexander N. Kvashnin, Tiia Laurila, Michael J. Lawler, Huajun Mai, Vladimir Makhmutov, Roy L. Mauldin III, Ugo Molteni, Leonid Nichman, Wei Nie, Andrea Ojdanic, Antti Onnela, Felix Piel, Lauriane L. J. Quéléver, Matti P. Rissanen, Nina Sarnela, Simon Schallhart, Kamalika Sengupta, Mario Simon, Dominik Stolzenburg, Yuri Stozhkov, Jasmin Tröstl, Yrjö Viisanen, Alexander L. Vogel, Andrea C. Wagner, Mao Xiao, Penglin Ye, Urs Baltensperger, Joachim Curtius, Neil M. Donahue, Richard C. Flagan, Martin Gallagher, Armin Hansel, James N. Smith, António Tomé, Paul M. Winkler, Douglas Worsnop, Mikael Ehn, Mikko Sipilä, Veli-Matti Kerminen, Tuukka Petäjä, and Markku Kulmala
Atmos. Chem. Phys., 17, 15181–15197, https://doi.org/10.5194/acp-17-15181-2017, https://doi.org/10.5194/acp-17-15181-2017, 2017
Daniel Wolfensberger, Auguste Gires, Ioulia Tchiguirinskaia, Daniel Schertzer, and Alexis Berne
Atmos. Chem. Phys., 17, 14253–14273, https://doi.org/10.5194/acp-17-14253-2017, https://doi.org/10.5194/acp-17-14253-2017, 2017
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Precipitation intensities simulated by the COSMO weather prediction model are compared to radar observations over a range of spatial and temporal scales using the universal multifractal framework. Our results highlight the strong influence of meteorological and topographical features on the multifractal characteristics of precipitation. Moreover, the influence of the subgrid parameterizations of COSMO is clearly visible by a break in the scaling properties that is absent from the radar data.
Leonid Nichman, Emma Järvinen, James Dorsey, Paul Connolly, Jonathan Duplissy, Claudia Fuchs, Karoliina Ignatius, Kamalika Sengupta, Frank Stratmann, Ottmar Möhler, Martin Schnaiter, and Martin Gallagher
Atmos. Meas. Tech., 10, 3231–3248, https://doi.org/10.5194/amt-10-3231-2017, https://doi.org/10.5194/amt-10-3231-2017, 2017
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Optical probes are frequently used for the detection of cloud particles. The detected microphysical properties may affect particle growth and accretion mechanisms and the light scattering properties of cirrus clouds. In the CLOUD chamber study at CERN, we compared four optical measurement techniques. We show that shape derivation alone is not sufficient to determine the phase of the small cloud particles. None of the instruments were able to unambiguously determine the phase of small particles.
Jacopo Grazioli, Christophe Genthon, Brice Boudevillain, Claudio Duran-Alarcon, Massimo Del Guasta, Jean-Baptiste Madeleine, and Alexis Berne
The Cryosphere, 11, 1797–1811, https://doi.org/10.5194/tc-11-1797-2017, https://doi.org/10.5194/tc-11-1797-2017, 2017
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We present medium and long-term measurements of precipitation in a coastal region of Antarctica. These measurements are among the first of their kind on the Antarctic continent and combine remote sensing with in situ observations. The benefits of this synergy are demonstrated and the lessons learned from this measurements, which are still ongoing, are very important for the creation of similar observatories elsewhere on the continent.
Timothy H. Raupach and Alexis Berne
Atmos. Meas. Tech., 10, 2573–2594, https://doi.org/10.5194/amt-10-2573-2017, https://doi.org/10.5194/amt-10-2573-2017, 2017
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The raindrop size distribution (DSD) describes the microstructure of rain. It is required knowledge for weather radar applications and has broad applicability to studies of rainfall processes, including weather models and rain retrieval algorithms. We present a new technique for estimating the DSD from polarimetric radar data. The new method was tested in three different domains, and its performance was found to be similar to and often better than an an existing DSD retrieval method.
Christophe Praz, Yves-Alain Roulet, and Alexis Berne
Atmos. Meas. Tech., 10, 1335–1357, https://doi.org/10.5194/amt-10-1335-2017, https://doi.org/10.5194/amt-10-1335-2017, 2017
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The Multi-Angle Snowflake Camera (MASC) provides high-resolution pictures of individual falling snowflakes and ice crystals. A method is proposed to automatically classify these pictures into six classes of snowflakes as well to estimate the degree of riming and to detect whether or not the particles are melting. Multinomial logistic regression is used with a manually classified
reference set. The evaluation demonstrates the good and reliable performance of the proposed technique.
Gillian Young, Paul J. Connolly, Hazel M. Jones, and Thomas W. Choularton
Atmos. Chem. Phys., 17, 4209–4227, https://doi.org/10.5194/acp-17-4209-2017, https://doi.org/10.5194/acp-17-4209-2017, 2017
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Arctic mixed-phase clouds are poorly represented in numerical models, due in part to an overpredicted ice phase. Here, we examine the sensitivity of cloud structure, evolution, and lifetime to modelled primary ice number concentrations over three different surfaces – sea ice, marginal ice, and ocean – to investigate the dependency on both the ice phase and dynamics induced from surface fluxes.
Guillaume Nord, Brice Boudevillain, Alexis Berne, Flora Branger, Isabelle Braud, Guillaume Dramais, Simon Gérard, Jérôme Le Coz, Cédric Legoût, Gilles Molinié, Joel Van Baelen, Jean-Pierre Vandervaere, Julien Andrieu, Coralie Aubert, Martin Calianno, Guy Delrieu, Jacopo Grazioli, Sahar Hachani, Ivan Horner, Jessica Huza, Raphaël Le Boursicaud, Timothy H. Raupach, Adriaan J. Teuling, Magdalena Uber, Béatrice Vincendon, and Annette Wijbrans
Earth Syst. Sci. Data, 9, 221–249, https://doi.org/10.5194/essd-9-221-2017, https://doi.org/10.5194/essd-9-221-2017, 2017
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A high space–time resolution dataset linking hydrometeorological forcing and hydro-sedimentary response in a mesoscale catchment (Auzon, 116 km2) of the Ardèche region (France) is presented. This region is subject to precipitating systems of Mediterranean origin, which can result in significant rainfall amount. The data presented cover a period of 4 years (2011–2014) and aim at improving the understanding of processes triggering flash floods.
Carla Frege, Federico Bianchi, Ugo Molteni, Jasmin Tröstl, Heikki Junninen, Stephan Henne, Mikko Sipilä, Erik Herrmann, Michel J. Rossi, Markku Kulmala, Christopher R. Hoyle, Urs Baltensperger, and Josef Dommen
Atmos. Chem. Phys., 17, 2613–2629, https://doi.org/10.5194/acp-17-2613-2017, https://doi.org/10.5194/acp-17-2613-2017, 2017
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We present measurements of the chemical composition of atmospheric ions at high altitude (3450 m a.s.l.) during a 9-month campaign. We detected remarkably high correlation between methanesulfonic acid (MSA) and SO5−. Halogenated species were also detected frequently at this continental location. New-particle formation events occurred via the condensation of highly oxygenated molecules (HOMs) at very low sulfuric acid concentration or, less frequently, due to ammonia–sulfuric acid clusters.
Alexander Beck, Jan Henneberger, Sarah Schöpfer, Jacob Fugal, and Ulrike Lohmann
Atmos. Meas. Tech., 10, 459–476, https://doi.org/10.5194/amt-10-459-2017, https://doi.org/10.5194/amt-10-459-2017, 2017
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In situ observations of cloud properties in complex alpine terrain are commonly conducted at mountain-top research stations and limited to single-point measurements. The HoloGondel platform overcomes this limitation by using a cable car to obtain vertical profiles of the microphysical and meteorological cloud parameters. In this work example measurements of the vertical profiles observed in a liquid cloud and a mixed-phase cloud at the Eggishorn in the Swiss Alps are presented.
Gillian Young, Hazel M. Jones, Thomas W. Choularton, Jonathan Crosier, Keith N. Bower, Martin W. Gallagher, Rhiannon S. Davies, Ian A. Renfrew, Andrew D. Elvidge, Eoghan Darbyshire, Franco Marenco, Philip R. A. Brown, Hugo M. A. Ricketts, Paul J. Connolly, Gary Lloyd, Paul I. Williams, James D. Allan, Jonathan W. Taylor, Dantong Liu, and Michael J. Flynn
Atmos. Chem. Phys., 16, 13945–13967, https://doi.org/10.5194/acp-16-13945-2016, https://doi.org/10.5194/acp-16-13945-2016, 2016
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Clouds are intricately coupled to the Arctic sea ice. Our inability to accurately model cloud fractions causes large uncertainties in predicted radiative interactions in this region, therefore, affecting sea ice forecasts. Here, we present measurements of cloud microphysics, aerosol properties, and thermodynamic structure over the transition from sea ice to ocean to improve our understanding of the relationship between the Arctic atmosphere and clouds which develop in this region.
Matthew Crooks, Paul Connolly, David Topping, and Gordon McFiggans
Geosci. Model Dev., 9, 3617–3637, https://doi.org/10.5194/gmd-9-3617-2016, https://doi.org/10.5194/gmd-9-3617-2016, 2016
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Semi-volatile compounds, like water, can exist in both vapour phases and condensed phases within a system. This paper presents a method of calculating the condensed and vapour phases of semi-volatile compounds at equilibrium, in particular, when the condensed mass occurs within particles of different sizes and chemical composition. The applications of interest to the authors are those of atmospheric importance such as cloud droplet formation and reflection or absorption of solar radiation.
Lukas Kaufmann, Claudia Marcolli, Julian Hofer, Valeria Pinti, Christopher R. Hoyle, and Thomas Peter
Atmos. Chem. Phys., 16, 11177–11206, https://doi.org/10.5194/acp-16-11177-2016, https://doi.org/10.5194/acp-16-11177-2016, 2016
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We investigated dust samples from dust source regions all over the globe with respect to their ice nucleation activity and their mineralogical composition. Stones of reference minerals were milled and investigated the same way as the natural dust samples. We found that the mineralogical composition is a major determinant of ice nucleation ability. Natural samples consist of mixtures of minerals with remarkably similar ice nucleation ability.
Nikola Besic, Jordi Figueras i Ventura, Jacopo Grazioli, Marco Gabella, Urs Germann, and Alexis Berne
Atmos. Meas. Tech., 9, 4425–4445, https://doi.org/10.5194/amt-9-4425-2016, https://doi.org/10.5194/amt-9-4425-2016, 2016
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In this paper we propose a novel semi-supervised method for hydrometeor classification, which takes into account both the specificities of acquired polarimetric radar measurements and the presumed electromagnetic behavior of different hydrometeor types. The method has been applied on three datasets, each acquired by different C-band radar from the Swiss network, and on two X-band research radar datasets. The obtained classification is found to be of high quality.
Luca Panziera, Marco Gabella, Stefano Zanini, Alessandro Hering, Urs Germann, and Alexis Berne
Hydrol. Earth Syst. Sci., 20, 2317–2332, https://doi.org/10.5194/hess-20-2317-2016, https://doi.org/10.5194/hess-20-2317-2016, 2016
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This paper presents a novel system to issue heavy rainfall alerts for predefined geographical regions by evaluating the sum of precipitation fallen in the immediate past and expected in the near future. In order to objectively define the thresholds for the alerts, an extreme rainfall analysis for the 159 regions used for official warnings in Switzerland was developed. It is shown that the system has additional lead time with respect to thunderstorm tracking tools targeted for convective storms.
Karoliina Ignatius, Thomas B. Kristensen, Emma Järvinen, Leonid Nichman, Claudia Fuchs, Hamish Gordon, Paul Herenz, Christopher R. Hoyle, Jonathan Duplissy, Sarvesh Garimella, Antonio Dias, Carla Frege, Niko Höppel, Jasmin Tröstl, Robert Wagner, Chao Yan, Antonio Amorim, Urs Baltensperger, Joachim Curtius, Neil M. Donahue, Martin W. Gallagher, Jasper Kirkby, Markku Kulmala, Ottmar Möhler, Harald Saathoff, Martin Schnaiter, Antonio Tomé, Annele Virtanen, Douglas Worsnop, and Frank Stratmann
Atmos. Chem. Phys., 16, 6495–6509, https://doi.org/10.5194/acp-16-6495-2016, https://doi.org/10.5194/acp-16-6495-2016, 2016
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Viscous solid or semi-solid secondary organic aerosol (SOA) may influence cloud properties through ice nucleation in the atmosphere. Here, we observed heterogeneous ice nucleation of viscous α-pinene SOA at temperatures between −39 °C and −37.2 °C with ice saturation ratios significantly below the homogeneous freezing limit. Global modelling suggests that viscous biogenic SOA are present in regions where cirrus formation takes place and could contribute to the global ice nuclei budget.
Robert J. Farrington, Paul J. Connolly, Gary Lloyd, Keith N. Bower, Michael J. Flynn, Martin W. Gallagher, Paul R. Field, Chris Dearden, and Thomas W. Choularton
Atmos. Chem. Phys., 16, 4945–4966, https://doi.org/10.5194/acp-16-4945-2016, https://doi.org/10.5194/acp-16-4945-2016, 2016
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This paper assesses the reasons for high ice number concentrations observed in orographic clouds by comparing observations with model simulations over Jungfraujoch, Switzerland. The results suggest that ice nuclei do not significantly contribute to the high concentrations and that a surface source of ice crystals is responsible for the witnessed ice number concentrations.
Emma Järvinen, Karoliina Ignatius, Leonid Nichman, Thomas B. Kristensen, Claudia Fuchs, Christopher R. Hoyle, Niko Höppel, Joel C. Corbin, Jill Craven, Jonathan Duplissy, Sebastian Ehrhart, Imad El Haddad, Carla Frege, Hamish Gordon, Tuija Jokinen, Peter Kallinger, Jasper Kirkby, Alexei Kiselev, Karl-Heinz Naumann, Tuukka Petäjä, Tamara Pinterich, Andre S. H. Prevot, Harald Saathoff, Thea Schiebel, Kamalika Sengupta, Mario Simon, Jay G. Slowik, Jasmin Tröstl, Annele Virtanen, Paul Vochezer, Steffen Vogt, Andrea C. Wagner, Robert Wagner, Christina Williamson, Paul M. Winkler, Chao Yan, Urs Baltensperger, Neil M. Donahue, Rick C. Flagan, Martin Gallagher, Armin Hansel, Markku Kulmala, Frank Stratmann, Douglas R. Worsnop, Ottmar Möhler, Thomas Leisner, and Martin Schnaiter
Atmos. Chem. Phys., 16, 4423–4438, https://doi.org/10.5194/acp-16-4423-2016, https://doi.org/10.5194/acp-16-4423-2016, 2016
Christopher R. Hoyle, Clare S. Webster, Harald E. Rieder, Athanasios Nenes, Emanuel Hammer, Erik Herrmann, Martin Gysel, Nicolas Bukowiecki, Ernest Weingartner, Martin Steinbacher, and Urs Baltensperger
Atmos. Chem. Phys., 16, 4043–4061, https://doi.org/10.5194/acp-16-4043-2016, https://doi.org/10.5194/acp-16-4043-2016, 2016
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A simple statistical model to predict the number of aerosols which activate to form cloud droplets in warm clouds has been established, based on regression analysis of data from the high-altitude site Jungfraujoch. It is found that cloud droplet formation at the Jungfraujoch is predominantly controlled by the number concentration of aerosol particles. A statistical model based on only the number of particles larger than 80nm can explain 79 % of the observed variance in droplet numbers.
G. Young, H. M. Jones, E. Darbyshire, K. J. Baustian, J. B. McQuaid, K. N. Bower, P. J. Connolly, M. W. Gallagher, and T. W. Choularton
Atmos. Chem. Phys., 16, 4063–4079, https://doi.org/10.5194/acp-16-4063-2016, https://doi.org/10.5194/acp-16-4063-2016, 2016
Leonid Nichman, Claudia Fuchs, Emma Järvinen, Karoliina Ignatius, Niko Florian Höppel, Antonio Dias, Martin Heinritzi, Mario Simon, Jasmin Tröstl, Andrea Christine Wagner, Robert Wagner, Christina Williamson, Chao Yan, Paul James Connolly, James Robert Dorsey, Jonathan Duplissy, Sebastian Ehrhart, Carla Frege, Hamish Gordon, Christopher Robert Hoyle, Thomas Bjerring Kristensen, Gerhard Steiner, Neil McPherson Donahue, Richard Flagan, Martin William Gallagher, Jasper Kirkby, Ottmar Möhler, Harald Saathoff, Martin Schnaiter, Frank Stratmann, and António Tomé
Atmos. Chem. Phys., 16, 3651–3664, https://doi.org/10.5194/acp-16-3651-2016, https://doi.org/10.5194/acp-16-3651-2016, 2016
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Processes in the atmosphere are often governed by the physical and chemical properties of small cloud particles. Ice, water, and mixed clouds, as well as viscous aerosols, were formed under controlled conditions at the CLOUD-CERN facility. The experimental results show a link between cloud particle properties and their unique optical fingerprints. The classification map presented here allows easier discrimination between various particles such as viscous organic aerosol, salt, ice, and liquid.
I. Crawford, G. Lloyd, E. Herrmann, C. R. Hoyle, K. N. Bower, P. J. Connolly, M. J. Flynn, P. H. Kaye, T. W. Choularton, and M. W. Gallagher
Atmos. Chem. Phys., 16, 2273–2284, https://doi.org/10.5194/acp-16-2273-2016, https://doi.org/10.5194/acp-16-2273-2016, 2016
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In this manuscript we discuss observations of fluorescent aerosol and their interactions with cloud at a high-alpine site in the wintertime under background conditions. We find the majority of the fluorescent aerosol to be consistent in nature to mineral dust and no apparent trend was observed between the fluorescent aerosol fraction and meteorological or cloud microphysical parameters, suggesting that particle fluorescence does not impact cloud evolution or formation at the site.
C. R. Hoyle, C. Fuchs, E. Järvinen, H. Saathoff, A. Dias, I. El Haddad, M. Gysel, S. C. Coburn, J. Tröstl, A.-K. Bernhammer, F. Bianchi, M. Breitenlechner, J. C. Corbin, J. Craven, N. M. Donahue, J. Duplissy, S. Ehrhart, C. Frege, H. Gordon, N. Höppel, M. Heinritzi, T. B. Kristensen, U. Molteni, L. Nichman, T. Pinterich, A. S. H. Prévôt, M. Simon, J. G. Slowik, G. Steiner, A. Tomé, A. L. Vogel, R. Volkamer, A. C. Wagner, R. Wagner, A. S. Wexler, C. Williamson, P. M. Winkler, C. Yan, A. Amorim, J. Dommen, J. Curtius, M. W. Gallagher, R. C. Flagan, A. Hansel, J. Kirkby, M. Kulmala, O. Möhler, F. Stratmann, D. R. Worsnop, and U. Baltensperger
Atmos. Chem. Phys., 16, 1693–1712, https://doi.org/10.5194/acp-16-1693-2016, https://doi.org/10.5194/acp-16-1693-2016, 2016
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A significant portion of sulphate, an important constituent of atmospheric aerosols, is formed via the aqueous phase oxidation of sulphur dioxide by ozone. The rate of this reaction has previously only been measured over a relatively small temperature range. Here, we use the state of the art CLOUD chamber at CERN to perform the first measurements of this reaction rate in super-cooled droplets, confirming that the existing extrapolation of the reaction rate to sub-zero temperatures is accurate.
G. Lloyd, T. W. Choularton, K. N. Bower, M. W. Gallagher, P. J. Connolly, M. Flynn, R. Farrington, J. Crosier, O. Schlenczek, J. Fugal, and J. Henneberger
Atmos. Chem. Phys., 15, 12953–12969, https://doi.org/10.5194/acp-15-12953-2015, https://doi.org/10.5194/acp-15-12953-2015, 2015
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The paper explores the microphysical structure of clouds at the high-alpine measurement site Jungfraujoch, Switzerland. High concentrations of ice crystals were measured by a range of instruments. The presence of these high concentrations could not be explained through conventional understanding of ice formation processes in clouds and the possibility that the surface provides a significant source of ice crystals is investigated.
C. Emersic, P. J. Connolly, S. Boult, M. Campana, and Z. Li
Atmos. Chem. Phys., 15, 11311–11326, https://doi.org/10.5194/acp-15-11311-2015, https://doi.org/10.5194/acp-15-11311-2015, 2015
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E. Hammer, N. Bukowiecki, B. P. Luo, U. Lohmann, C. Marcolli, E. Weingartner, U. Baltensperger, and C. R. Hoyle
Atmos. Chem. Phys., 15, 10309–10323, https://doi.org/10.5194/acp-15-10309-2015, https://doi.org/10.5194/acp-15-10309-2015, 2015
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An important quantity which determines aerosol activation and cloud formation is the effective peak supersaturation. The box model ZOMM was used to simulate the effective peak supersaturation experienced by an air parcel approaching a high-alpine research station in Switzerland. With the box model the sensitivity of the effective peak supersaturation to key aerosol and dynamical parameters was investigated.
T. Elias, J.-C. Dupont, E. Hammer, C. R. Hoyle, M. Haeffelin, F. Burnet, and D. Jolivet
Atmos. Chem. Phys., 15, 6605–6623, https://doi.org/10.5194/acp-15-6605-2015, https://doi.org/10.5194/acp-15-6605-2015, 2015
M. Stähli, M. Sättele, C. Huggel, B. W. McArdell, P. Lehmann, A. Van Herwijnen, A. Berne, M. Schleiss, A. Ferrari, A. Kos, D. Or, and S. M. Springman
Nat. Hazards Earth Syst. Sci., 15, 905–917, https://doi.org/10.5194/nhess-15-905-2015, https://doi.org/10.5194/nhess-15-905-2015, 2015
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This review paper describes the state of the art in monitoring and predicting rapid mass movements for early warning. It further presents recent innovations in observation technologies and modelling to be used in future early warning systems (EWS). Finally, the paper proposes avenues towards successful implementation of next-generation EWS.
I. Steinke, C. Hoose, O. Möhler, P. Connolly, and T. Leisner
Atmos. Chem. Phys., 15, 3703–3717, https://doi.org/10.5194/acp-15-3703-2015, https://doi.org/10.5194/acp-15-3703-2015, 2015
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Ice nucleation in clouds has a significant influence on the global radiative budget and the hydrological cycle. Several studies have investigated the ice formation in droplets and parameterizations have been developed in order to include immersion freezing in climate models. In contrast, there are fewer studies regarding the conversion of water vapor into ice (so-called deposition nucleation) which is the topic of this paper which investigates deposition nucleation by Arizona Test dust in detail
G. Lloyd, T. W. Choularton, K. N. Bower, J. Crosier, H. Jones, J. R. Dorsey, M. W. Gallagher, P. Connolly, A. C. R. Kirchgaessner, and T. Lachlan-Cope
Atmos. Chem. Phys., 15, 3719–3737, https://doi.org/10.5194/acp-15-3719-2015, https://doi.org/10.5194/acp-15-3719-2015, 2015
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Measurements of cloud microphysics are reported from the Aerosol-Cloud Coupling And Climate Interactions (ACCACIA) campaign. Concentrations of ice particles from two spring and two summer cases are compared with particular attention to the role of secondary ice in these clouds. In addition aerosol measurements were used as input to a primary ice nucleation parameterisation which was compared with observed values of primary ice in these clouds. We found higher concentrations of ice during summer.
S. Schmidt, J. Schneider, T. Klimach, S. Mertes, L. P. Schenk, J. Curtius, P. Kupiszewski, E. Hammer, P. Vochezer, G. Lloyd, M. Ebert, K. Kandler, S. Weinbruch, and S. Borrmann
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-15-4677-2015, https://doi.org/10.5194/acpd-15-4677-2015, 2015
Revised manuscript not accepted
T. H. Raupach and A. Berne
Atmos. Meas. Tech., 8, 343–365, https://doi.org/10.5194/amt-8-343-2015, https://doi.org/10.5194/amt-8-343-2015, 2015
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Using the 2-D video disdrometer (2DVD) as a reference, a technique to correct the spectra of drop size distribution (DSD) measured by Parsivel disdrometers (1st and 2nd generation) is proposed. The measured velocities and equivolume diameters are corrected to better match those from the 2DVD. The correction is evaluated using data from southern France and the Swiss Plateau. It appears to be similar for both climatologies, and to improve the consistency with colocated 2DVDs and rain gauges.
J. Grazioli, D. Tuia, and A. Berne
Atmos. Meas. Tech., 8, 149–170, https://doi.org/10.5194/amt-8-149-2015, https://doi.org/10.5194/amt-8-149-2015, 2015
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A new approach for hydrometeor classification from polarimetric radar measurements is proposed. It takes adavantage of clustering techniques to objectively determine the number of hydrometeor classes that can be reliably identified. The proposed method is tested using observations from an X-band polarimetric radar in different regions and evaluated by comparison with existing algorithms and with measurements from a ground-based 2D video disdrometer (providing 2-D views of falling hydrometeors).
E. Hammer, M. Gysel, G. C. Roberts, T. Elias, J. Hofer, C. R. Hoyle, N. Bukowiecki, J.-C. Dupont, F. Burnet, U. Baltensperger, and E. Weingartner
Atmos. Chem. Phys., 14, 10517–10533, https://doi.org/10.5194/acp-14-10517-2014, https://doi.org/10.5194/acp-14-10517-2014, 2014
J. Grazioli, D. Tuia, S. Monhart, M. Schneebeli, T. Raupach, and A. Berne
Atmos. Meas. Tech., 7, 2869–2882, https://doi.org/10.5194/amt-7-2869-2014, https://doi.org/10.5194/amt-7-2869-2014, 2014
E. Simpson, P. Connolly, and G. McFiggans
Geosci. Model Dev., 7, 1535–1542, https://doi.org/10.5194/gmd-7-1535-2014, https://doi.org/10.5194/gmd-7-1535-2014, 2014
I. Engel, B. P. Luo, S. M. Khaykin, F. G. Wienhold, H. Vömel, R. Kivi, C. R. Hoyle, J.-U. Grooß, M. C. Pitts, and T. Peter
Atmos. Chem. Phys., 14, 3231–3246, https://doi.org/10.5194/acp-14-3231-2014, https://doi.org/10.5194/acp-14-3231-2014, 2014
P. J. Connolly, D. O. Topping, F. Malavelle, and G. McFiggans
Atmos. Chem. Phys., 14, 2289–2302, https://doi.org/10.5194/acp-14-2289-2014, https://doi.org/10.5194/acp-14-2289-2014, 2014
E. Hammer, N. Bukowiecki, M. Gysel, Z. Jurányi, C. R. Hoyle, R. Vogt, U. Baltensperger, and E. Weingartner
Atmos. Chem. Phys., 14, 1123–1139, https://doi.org/10.5194/acp-14-1123-2014, https://doi.org/10.5194/acp-14-1123-2014, 2014
J.-U. Grooß, I. Engel, S. Borrmann, W. Frey, G. Günther, C. R. Hoyle, R. Kivi, B. P. Luo, S. Molleker, T. Peter, M. C. Pitts, H. Schlager, G. Stiller, H. Vömel, K. A. Walker, and R. Müller
Atmos. Chem. Phys., 14, 1055–1073, https://doi.org/10.5194/acp-14-1055-2014, https://doi.org/10.5194/acp-14-1055-2014, 2014
I. Engel, B. P. Luo, M. C. Pitts, L. R. Poole, C. R. Hoyle, J.-U. Grooß, A. Dörnbrack, and T. Peter
Atmos. Chem. Phys., 13, 10769–10785, https://doi.org/10.5194/acp-13-10769-2013, https://doi.org/10.5194/acp-13-10769-2013, 2013
J. Henneberger, J. P. Fugal, O. Stetzer, and U. Lohmann
Atmos. Meas. Tech., 6, 2975–2987, https://doi.org/10.5194/amt-6-2975-2013, https://doi.org/10.5194/amt-6-2975-2013, 2013
A. Stenke, C. R. Hoyle, B. Luo, E. Rozanov, J. Gröbner, L. Maag, S. Brönnimann, and T. Peter
Atmos. Chem. Phys., 13, 9713–9729, https://doi.org/10.5194/acp-13-9713-2013, https://doi.org/10.5194/acp-13-9713-2013, 2013
C. R. Hoyle, I. Engel, B. P. Luo, M. C. Pitts, L. R. Poole, J.-U. Grooß, and T. Peter
Atmos. Chem. Phys., 13, 9577–9595, https://doi.org/10.5194/acp-13-9577-2013, https://doi.org/10.5194/acp-13-9577-2013, 2013
M. von Hobe, S. Bekki, S. Borrmann, F. Cairo, F. D'Amato, G. Di Donfrancesco, A. Dörnbrack, A. Ebersoldt, M. Ebert, C. Emde, I. Engel, M. Ern, W. Frey, S. Genco, S. Griessbach, J.-U. Grooß, T. Gulde, G. Günther, E. Hösen, L. Hoffmann, V. Homonnai, C. R. Hoyle, I. S. A. Isaksen, D. R. Jackson, I. M. Jánosi, R. L. Jones, K. Kandler, C. Kalicinsky, A. Keil, S. M. Khaykin, F. Khosrawi, R. Kivi, J. Kuttippurath, J. C. Laube, F. Lefèvre, R. Lehmann, S. Ludmann, B. P. Luo, M. Marchand, J. Meyer, V. Mitev, S. Molleker, R. Müller, H. Oelhaf, F. Olschewski, Y. Orsolini, T. Peter, K. Pfeilsticker, C. Piesch, M. C. Pitts, L. R. Poole, F. D. Pope, F. Ravegnani, M. Rex, M. Riese, T. Röckmann, B. Rognerud, A. Roiger, C. Rolf, M. L. Santee, M. Scheibe, C. Schiller, H. Schlager, M. Siciliani de Cumis, N. Sitnikov, O. A. Søvde, R. Spang, N. Spelten, F. Stordal, O. Sumińska-Ebersoldt, A. Ulanovski, J. Ungermann, S. Viciani, C. M. Volk, M. vom Scheidt, P. von der Gathen, K. Walker, T. Wegner, R. Weigel, S. Weinbruch, G. Wetzel, F. G. Wienhold, I. Wohltmann, W. Woiwode, I. A. K. Young, V. Yushkov, B. Zobrist, and F. Stroh
Atmos. Chem. Phys., 13, 9233–9268, https://doi.org/10.5194/acp-13-9233-2013, https://doi.org/10.5194/acp-13-9233-2013, 2013
P. J. Connolly, G. Vaughan, P. Cook, G. Allen, H. Coe, T. W. Choularton, C. Dearden, and A. Hill
Atmos. Chem. Phys., 13, 7133–7152, https://doi.org/10.5194/acp-13-7133-2013, https://doi.org/10.5194/acp-13-7133-2013, 2013
J. Skrotzki, P. Connolly, M. Schnaiter, H. Saathoff, O. Möhler, R. Wagner, M. Niemand, V. Ebert, and T. Leisner
Atmos. Chem. Phys., 13, 4451–4466, https://doi.org/10.5194/acp-13-4451-2013, https://doi.org/10.5194/acp-13-4451-2013, 2013
Related subject area
Subject: Clouds and Precipitation | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Daytime variation in the aerosol indirect effect for warm marine boundary layer clouds in the eastern North Atlantic
Technical note: Bimodal parameterizations of in situ ice cloud particle size distributions
Inter-relations of precipitation, aerosols, and clouds over Andalusia, southern Spain, revealed by the Andalusian Global ObseRvatory of the Atmosphere (AGORA)
On the relationship between mesoscale cellular convection and meteorological forcing: comparing the Southern Ocean against the North Pacific
Aerosol-related effects on the occurrence of heterogeneous ice formation over Lauder, New Zealand ∕ Aotearoa
Low-level Arctic clouds: a blind zone in our knowledge of the radiation budget
Climatologically invariant scale invariance seen in distributions of cloud horizontal sizes
Variability and properties of liquid-dominated clouds over the ice-free and sea-ice-covered Arctic Ocean
The correlation between Arctic sea ice, cloud phase and radiation using A-train satellites
Observations of the macrophysical properties of cumulus cloud fields over the tropical western Pacific and their connection to meteorological variables
The effects of warm air intrusions in the high arctic on cirrus clouds
Asymmetries in cloud microphysical properties ascribed to sea ice leads via water vapour transport in the central Arctic
Observations of Tropical Tropopause Layer clouds from a balloon-borne lidar
Quantifying the dependence of drop spectrum width on cloud drop number concentration for cloud remote sensing
The evolution of deep convective systems and their associated cirrus outflows
The characteristics of cloud macro parameters caused by seeder-feeder inside clouds measured by millimeter-wave cloud radar in Xi'an
Wildfire smoke triggers cirrus formation: lidar observations over the eastern Mediterranean
Rapid saturation of cloud water adjustments to shipping emissions
A Lagrangian Perspective on the Lifecycle and Cloud Radiative Effect of Deep Convective Clouds Over Africa
Sensitivities of cloud radiative effects to large-scale meteorology and aerosols from global observations
A Survey of Radiative and Physical Properties of North Atlantic Mesoscale Cloud Morphologies from Multiple Identification Methodologies
Distinct secondary ice production processes observed in radar Doppler spectra: insights from a case study
Investigating the development of clouds within marine cold-air outbreaks
Detection of large-scale cloud microphysical changes within a major shipping corridor after implementation of the International Maritime Organization 2020 fuel sulfur regulations
Examining cloud vertical structure and radiative effects from satellite retrievals and evaluation of CMIP6 scenarios
Influence of cloud microphysics schemes on weather model predictions of heavy precipitation
Convective organization and 3D structure of tropical cloud systems deduced from synergistic A-Train observations and machine learning
Shallow and Deep Convection Characteristics in the Greater Houston, Texas Area Using Cell Tracking Methodology
Seasonal controls on isolated convective storm drafts, precipitation intensity, and life cycle as observed during GoAmazon2014/5
Uncertainty in aerosol–cloud radiative forcing is driven by clean conditions
Surface-based observations of cold-air outbreak clouds during the COMBLE field campaign
Boundary layer moisture variability at the Atmospheric Radiation Measurement (ARM) Eastern North Atlantic observatory during marine conditions
Profile-based estimated inversion strength
Characteristics of supersaturation in midlatitude cirrus clouds and their adjacent cloud-free air
Establishment of an analytical model for remote sensing of typical stratocumulus cloud profiles under various precipitation and entrainment conditions
Satellite remote sensing of regional and seasonal Arctic cooling showing a multi-decadal trend towards brighter and more liquid clouds
Microphysical processes of super typhoon Lekima (2019) and their impacts on polarimetric radar remote sensing of precipitation
The impacts of dust aerosol and convective available potential energy on precipitation vertical structure in southeastern China as seen from multisource observations
Heavy snowfall event over the Swiss Alps: did wind shear impact secondary ice production?
On the global relationship between polarimetric radio occultation differential phase shift and ice water content
Observations of microphysical properties and radiative effects of a contrail cirrus outbreak over the North Atlantic
Natural marine cloud brightening in the Southern Ocean
Distinct regional meteorological influences on low-cloud albedo susceptibility over global marine stratocumulus regions
Diurnal cycles of cloud cover and its vertical distribution over the Tibetan Plateau revealed by satellite observations, reanalysis datasets, and CMIP6 outputs
Satellite observations of seasonality and long-term trends in cirrus cloud properties over Europe: investigation of possible aviation impacts
Ice crystal characterization in cirrus clouds III: retrieval of ice crystal shape and roughness from observations of halo displays
Technical note: Identification of two ice-nucleating regimes for dust-related cirrus clouds based on the relationship between number concentrations of ice-nucleating particles and ice crystals
Highly supercooled riming and unusual triple-frequency radar signatures over McMurdo Station, Antarctica
Ice microphysical processes in the dendritic growth layer: a statistical analysis combining multi-frequency and polarimetric Doppler cloud radar observations
Observing short-timescale cloud development to constrain aerosol–cloud interactions
Shaoyue Qiu, Xue Zheng, David Painemal, Christopher R. Terai, and Xiaoli Zhou
Atmos. Chem. Phys., 24, 2913–2935, https://doi.org/10.5194/acp-24-2913-2024, https://doi.org/10.5194/acp-24-2913-2024, 2024
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The aerosol indirect effect (AIE) depends on cloud states, which exhibit significant diurnal variations in the northeastern Atlantic. Yet the AIE diurnal cycle remains poorly understood. Using satellite retrievals, we find a pronounced “U-shaped” diurnal variation in the AIE, which is contributed to by the transition of cloud states combined with the lagged cloud responses. This suggests that polar-orbiting satellites with overpass times at noon underestimate daytime mean values of the AIE.
Irene Bartolomé García, Odran Sourdeval, Reinhold Spang, and Martina Krämer
Atmos. Chem. Phys., 24, 1699–1716, https://doi.org/10.5194/acp-24-1699-2024, https://doi.org/10.5194/acp-24-1699-2024, 2024
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How many ice crystals of each size are in a cloud is a key parameter for the retrieval of cloud properties. The distribution of ice crystals is obtained from in situ measurements and used to create parameterizations that can be used when analyzing the remote-sensing data. Current parameterizations are based on data sets that do not include reliable measurements of small crystals, but in our study we use a data set that includes very small ice crystals to improve these parameterizations.
Wenyue Wang, Klemens Hocke, Leonardo Nania, Alberto Cazorla, Gloria Titos, Renaud Matthey, Lucas Alados-Arboledas, Agustín Millares, and Francisco Navas-Guzmán
Atmos. Chem. Phys., 24, 1571–1585, https://doi.org/10.5194/acp-24-1571-2024, https://doi.org/10.5194/acp-24-1571-2024, 2024
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The south-central interior of Andalusia experiences complex precipitation patterns as a result of the semi-arid Mediterranean climate and the influence of Saharan dust. This study monitored the inter-relations between aerosols, clouds, meteorological variables, and precipitation systems using ground-based remote sensing and in situ instruments.
Francisco Lang, Steven T. Siems, Yi Huang, Tahereh Alinejadtabrizi, and Luis Ackermann
Atmos. Chem. Phys., 24, 1451–1466, https://doi.org/10.5194/acp-24-1451-2024, https://doi.org/10.5194/acp-24-1451-2024, 2024
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Marine low-level clouds play a crucial role in the Earth's energy balance, trapping heat from the surface and reflecting sunlight back into space. These clouds are distinguishable by their large-scale spatial structures, primarily characterized as hexagonal patterns with either filled (closed) or empty (open) cells. Utilizing satellite observations, these two cloud type patterns have been categorized over the Southern Ocean and North Pacific Ocean through a pattern recognition program.
Julian Hofer, Patric Seifert, J. Ben Liley, Martin Radenz, Osamu Uchino, Isamu Morino, Tetsu Sakai, Tomohiro Nagai, and Albert Ansmann
Atmos. Chem. Phys., 24, 1265–1280, https://doi.org/10.5194/acp-24-1265-2024, https://doi.org/10.5194/acp-24-1265-2024, 2024
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An 11-year dataset of polarization lidar observations from Lauder, New Zealand / Aotearoa, was used to distinguish the thermodynamic phase of natural clouds. The cloud dataset was separated to assess the impact of air mass origin on the frequency of heterogeneous ice formation. Ice formation efficiency in clouds above Lauder was found to be lower than in the polluted Northern Hemisphere midlatitudes but higher than in very clean and pristine environments, such as Punta Arenas in southern Chile.
Hannes Jascha Griesche, Carola Barrientos-Velasco, Hartwig Deneke, Anja Hünerbein, Patric Seifert, and Andreas Macke
Atmos. Chem. Phys., 24, 597–612, https://doi.org/10.5194/acp-24-597-2024, https://doi.org/10.5194/acp-24-597-2024, 2024
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The Arctic is strongly affected by climate change and the role of clouds therein is not yet completely understood. Measurements from the Arctic expedition PS106 were used to simulate radiative fluxes with and without clouds at very low altitudes (below 165 m), and their radiative effect was calculated to be 54 Wm-2. The low heights of these clouds make them hard to observe. This study shows the importance of accurate measurements and simulations of clouds and gives suggestions for improvements.
Thomas D. DeWitt, Timothy J. Garrett, Karlie N. Rees, Corey Bois, Steven K. Krueger, and Nicolas Ferlay
Atmos. Chem. Phys., 24, 109–122, https://doi.org/10.5194/acp-24-109-2024, https://doi.org/10.5194/acp-24-109-2024, 2024
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Viewed from space, a defining feature of Earth's atmosphere is the wide spectrum of cloud sizes. A recent study predicted the distribution of cloud sizes, and this paper compares the prediction to observations. Although there is nuance in viewing perspective, we find robust agreement with theory across different climatological conditions, including land–ocean contrasts, time of year, or latitude, suggesting a minor role for Coriolis forces, aerosol loading, or surface temperature.
Marcus Klingebiel, André Ehrlich, Elena Ruiz-Donoso, Nils Risse, Imke Schirmacher, Evelyn Jäkel, Michael Schäfer, Kevin Wolf, Mario Mech, Manuel Moser, Christiane Voigt, and Manfred Wendisch
Atmos. Chem. Phys., 23, 15289–15304, https://doi.org/10.5194/acp-23-15289-2023, https://doi.org/10.5194/acp-23-15289-2023, 2023
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In this study we explain how we use aircraft measurements from two Arctic research campaigns to identify cloud properties (like droplet size) over sea-ice and ice-free ocean. To make sure that our measurements make sense, we compare them with other observations. Our results show, e.g., larger cloud droplets in early summer than in spring. Moreover, the cloud droplets are also larger over ice-free ocean than compared to sea ice. In the future, our data can be used to improve climate models.
Grégory V. Cesana, Olivia Pierpaoli, Matteo Ottaviani, Linh Vu, and Zhonghai Jin
EGUsphere, https://doi.org/10.5194/egusphere-2023-2940, https://doi.org/10.5194/egusphere-2023-2940, 2023
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Better characterizing the relationship between sea ice and clouds is key to understanding Arctic climate, because clouds and sea ice affect surface radiation and modulate Arctic surface warming. Our results indicate that Arctic liquid clouds robustly increase in response to sea-ice decrease. This increase has a cooling effect on the surface, because more solar radiation is reflected back to space, and it should contribute to dampening future Arctic surface warming.
Michie Vianca De Vera, Larry Di Girolamo, Guangyu Zhao, Robert Rauber, Stephen Nesbitt, and Greg McFarquhar
EGUsphere, https://doi.org/10.5194/egusphere-2023-2852, https://doi.org/10.5194/egusphere-2023-2852, 2023
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Tropical oceanic low clouds remain a dominant source of uncertainty in cloud feedback in climate models due to their macrophysical properties (fraction, size, height, shape, distribution) being misrepresented. High resolution satellite imagery over the Philippine oceans is used here to characterize cumuli macrophysical properties and their relationship to meteorological variables. Such information can act as a benchmark for cloud models and can improve low cloud generation in climate models.
Georgios Dekoutsidis, Martin Wirth, and Silke Groß
EGUsphere, https://doi.org/10.5194/egusphere-2023-2708, https://doi.org/10.5194/egusphere-2023-2708, 2023
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Since decades the earth’s temperature has been rising. The arctic regions are warming faster. Cirrus clouds can contribute to this phenomenon. During warm air intrusions, airmasses are transported into the arctic from the mid-latitudes. The HALO-(AC)3 campaign took place to measure cirrus during intrusion events and under normal conditions. We study the two cloud types based on these measurements and find differences in their geometry, relative humidity distribution and vertical structure.
Pablo Saavedra Garfias, Heike Kalesse-Los, Luisa von Albedyll, Hannes Griesche, and Gunnar Spreen
Atmos. Chem. Phys., 23, 14521–14546, https://doi.org/10.5194/acp-23-14521-2023, https://doi.org/10.5194/acp-23-14521-2023, 2023
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An important Arctic climate process is the release of heat fluxes from sea ice openings to the atmosphere that influence the clouds. The characterization of this process is the objective of this study. Using synergistic observations from the MOSAiC expedition, we found that single-layer cloud properties show significant differences when clouds are coupled or decoupled to the water vapour transport which is used as physical link between the upwind sea ice openings and the cloud under observation.
Thomas Lesigne, Francois Ravetta, Aurélien Podglajen, Vincent Mariage, and Jacques Pelon
EGUsphere, https://doi.org/10.5194/egusphere-2023-2763, https://doi.org/10.5194/egusphere-2023-2763, 2023
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Upper tropical clouds have a strong impact on Earth climate but are challenging to observe. We report the first long-duration observations of tropical clouds from lidars flying onboard stratospheric balloons. Comparisons with space-borne observations reveal the unique sensitivity of balloon-borne lidar to optically thin clouds. The thinnest ones have a significant coverage and lay in the uppermost troposphere, they are linked with the dehydration of air masses on their way to the stratosphere.
Matthew D. Lebsock and Mikael Witte
Atmos. Chem. Phys., 23, 14293–14305, https://doi.org/10.5194/acp-23-14293-2023, https://doi.org/10.5194/acp-23-14293-2023, 2023
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This paper evaluates measurements of cloud drop size distributions made from airplanes. We find that as the number of cloud drops increases the distribution of the cloud drop sizes narrows. The data are used to develop a simple equation that relates the drop number to the width of the drop sizes. We then use this equation to demonstrate that existing approaches to observe the drop number from satellites contain errors that can be corrected by including the new relationship.
George Horner and Edward Gryspeerdt
Atmos. Chem. Phys., 23, 14239–14253, https://doi.org/10.5194/acp-23-14239-2023, https://doi.org/10.5194/acp-23-14239-2023, 2023
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Tropical deep convective clouds, and the thin cirrus (ice) clouds that flow out from them, are important for modulating the energy budget of the tropical atmosphere. This work uses a new method to track the evolution of the properties of these clouds across their entire lifetimes. We find these clouds cool the atmosphere in the first 6 h before switching to a warming regime after the deep convective core has dissipated, which is sustained beyond 120 h from the initial convective event.
Huige Di and Yun Yuan
EGUsphere, https://doi.org/10.5194/egusphere-2023-2183, https://doi.org/10.5194/egusphere-2023-2183, 2023
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Based on the observation data of the ground-based Ka-band millimeter-wave cloud radar (MMCR) and microwave radiometer in spring and autumn from 2020 to 2022, the seeder-feeder phenomenon among double-layer clouds in China Xi'an was studied. Through the analysis on the reflectivity factor and the radial velocity of cloud particles detected by MMCR and on the retrieved cloud dynamics parameters, it is shown that the reflectivity factor in the cloud are significantly enhanced.
Rodanthi-Elisavet Mamouri, Albert Ansmann, Kevin Ohneiser, Daniel A. Knopf, Argyro Nisantzi, Johannes Bühl, Ronny Engelmann, Annett Skupin, Patric Seifert, Holger Baars, Dragos Ene, Ulla Wandinger, and Diofantos Hadjimitsis
Atmos. Chem. Phys., 23, 14097–14114, https://doi.org/10.5194/acp-23-14097-2023, https://doi.org/10.5194/acp-23-14097-2023, 2023
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For the first time, rather clear evidence is found that wildfire smoke particles can trigger strong cirrus formation. This finding is of importance because intensive and large wildfires may occur increasingly often in the future as climate change proceeds. Based on lidar observations in Cyprus in autumn 2020, we provide detailed insight into the cirrus formation at the tropopause in the presence of aged wildfire smoke (here, 8–9 day old Californian wildfire smoke).
Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier
Atmos. Chem. Phys., 23, 12545–12555, https://doi.org/10.5194/acp-23-12545-2023, https://doi.org/10.5194/acp-23-12545-2023, 2023
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Aerosol from burning fuel changes cloud properties, e.g., the number of droplets and the content of water. Here, we study how clouds respond to different amounts of shipping aerosol. Droplet numbers increase linearly with increasing aerosol over a broad range until they stop increasing, while the amount of liquid water always increases, independently of emission amount. These changes in cloud properties can make them reflect more or less sunlight, which is important for the earth's climate.
William K. Jones, Martin Stengel, and Philip Stier
EGUsphere, https://doi.org/10.5194/egusphere-2023-2059, https://doi.org/10.5194/egusphere-2023-2059, 2023
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Storm clouds cover large areas of the tropics. These clouds both reflect incoming sunlight and trap heat from the atmosphere below, regulating the temperature of the tropics. Over land, storm clouds occur in the late afternoon and evening, and so exist both during the daytime and at night. Changes in this timing could upset the balance of the respective cooling and heating effects of these clouds. We find that isolated storms have a larger effect on this balance than their small size suggests.
Hendrik Andersen, Jan Cermak, Alyson Douglas, Timothy A. Myers, Peer Nowack, Philip Stier, Casey J. Wall, and Sarah Wilson Kemsley
Atmos. Chem. Phys., 23, 10775–10794, https://doi.org/10.5194/acp-23-10775-2023, https://doi.org/10.5194/acp-23-10775-2023, 2023
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This study uses an observation-based cloud-controlling factor framework to study near-global sensitivities of cloud radiative effects to a large number of meteorological and aerosol controls. We present near-global sensitivity patterns to selected thermodynamic, dynamic, and aerosol factors and discuss the physical mechanisms underlying the derived sensitivities. Our study hopes to guide future analyses aimed at constraining cloud feedbacks and aerosol–cloud interactions.
Ryan Eastman, Isabel Louise McCoy, Hauke Schulz, and Robert Wood
EGUsphere, https://doi.org/10.5194/egusphere-2023-2118, https://doi.org/10.5194/egusphere-2023-2118, 2023
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Cloud types are determined using machine learning image classifiers applied to satellite imagery for one year in the North Atlantic. This survey of these cloud types shows that the climate impact of a cloud scene is in-part a function of cloud type. Each type displays a different mix of thick and thin cloud cover, with the fraction of thin cloud cover having the strongest impact on the clouds radiative effect. Future studies must account for differing properties and processes among types.
Anne-Claire Billault-Roux, Paraskevi Georgakaki, Josué Gehring, Louis Jaffeux, Alfons Schwarzenboeck, Pierre Coutris, Athanasios Nenes, and Alexis Berne
Atmos. Chem. Phys., 23, 10207–10234, https://doi.org/10.5194/acp-23-10207-2023, https://doi.org/10.5194/acp-23-10207-2023, 2023
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Secondary ice production plays a key role in clouds and precipitation. In this study, we analyze radar measurements from a snowfall event in the Jura Mountains. Complex signatures are observed, which reveal that ice crystals were formed through various processes. An analysis of multi-sensor data suggests that distinct ice multiplication processes were taking place. Both the methods used and the insights gained through this case study contribute to a better understanding of snowfall microphysics.
Rebecca J. Murray-Watson, Edward Gryspeerdt, and Tom Goren
Atmos. Chem. Phys., 23, 9365–9383, https://doi.org/10.5194/acp-23-9365-2023, https://doi.org/10.5194/acp-23-9365-2023, 2023
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Clouds formed in Arctic marine cold air outbreaks undergo a distinct evolution, but the factors controlling their transition from high-coverage to broken cloud fields are poorly understood. We use satellite and reanalysis data to study how these clouds develop in time and the different influences on their evolution. The aerosol concentration is correlated with cloud break-up; more aerosol is linked to prolonged coverage and a stronger cooling effect, with implications for a more polluted Arctic.
Michael S. Diamond
Atmos. Chem. Phys., 23, 8259–8269, https://doi.org/10.5194/acp-23-8259-2023, https://doi.org/10.5194/acp-23-8259-2023, 2023
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Fuel sulfur regulations were implemented for ships in 2020 to improve air quality but may also accelerate global warming. We use spatial statistics and satellite retrievals to detect changes in the size of cloud droplets and find evidence for a resulting decrease in cloud brightness within a major shipping corridor after the sulfur limits went into effect. Our results confirm both that the regulations are being followed and that they are having a warming influence via their effect on clouds.
Hao Luo, Johannes Quaas, and Yong Han
Atmos. Chem. Phys., 23, 8169–8186, https://doi.org/10.5194/acp-23-8169-2023, https://doi.org/10.5194/acp-23-8169-2023, 2023
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Clouds exhibit a wide range of vertical structures with varying microphysical and radiative properties. We show a global survey of spatial distribution, vertical extent and radiative effect of various classified cloud vertical structures using joint satellite observations from the new CCCM datasets during 2007–2010. Moreover, the long-term trends in CVSs are investigated based on different CMIP6 future scenarios to capture the cloud variations with different, increasing anthropogenic forcings.
Gregor Köcher, Tobias Zinner, and Christoph Knote
Atmos. Chem. Phys., 23, 6255–6269, https://doi.org/10.5194/acp-23-6255-2023, https://doi.org/10.5194/acp-23-6255-2023, 2023
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Polarimetric radar observations of 30 d of convective precipitation events are used to statistically analyze 5 state-of-the-art microphysics schemes of varying complexity. The frequency and area of simulated heavy-precipitation events are in some cases significantly different from those observed, depending on the microphysics scheme. Analysis of simulated particle size distributions and reflectivities shows that some schemes have problems reproducing the correct particle size distributions.
Claudia J. Stubenrauch, Giulio Mandorli, and Elisabeth Lemaitre
Atmos. Chem. Phys., 23, 5867–5884, https://doi.org/10.5194/acp-23-5867-2023, https://doi.org/10.5194/acp-23-5867-2023, 2023
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Organized convection leads to large convective cloud systems and intense rain and may change with a warming climate. Their complete 3D description, attained by machine learning techniques in combination with various satellite observations, together with a cloud system concept, link convection to anvil properties, while convective organization can be identified by the horizontal structure of intense rain.
Kristofer S. Tuftedal, Bernat Puigdomènech Treserras, Mariko Oue, and Pavlos Kollias
EGUsphere, https://doi.org/10.5194/egusphere-2023-821, https://doi.org/10.5194/egusphere-2023-821, 2023
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This study analyzed coastal convective cells from June through September 2018–2021. The cells were classified and their lifecycles were analyzed to better understand their characteristics and environments. The study found differences in initiation location of shallow convection, in mid-level moisture between shallow and deep convection, and in the aerosol loading in deep convective environments. This work provides a foundation for future analyses of convection or other tracked events elsewhere.
Scott E. Giangrande, Thiago S. Biscaro, and John M. Peters
Atmos. Chem. Phys., 23, 5297–5316, https://doi.org/10.5194/acp-23-5297-2023, https://doi.org/10.5194/acp-23-5297-2023, 2023
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Our study tracks thunderstorms observed during the wet and dry seasons of the Amazon Basin using weather radar. We couple this precipitation tracking with opportunistic overpasses of a wind profiler and other ground observations to add unique insights into the upwards and downwards air motions within these clouds at various stages in the storm life cycle. The results of a simple updraft model are provided to give physical explanations for observed seasonal differences.
Edward Gryspeerdt, Adam C. Povey, Roy G. Grainger, Otto Hasekamp, N. Christina Hsu, Jane P. Mulcahy, Andrew M. Sayer, and Armin Sorooshian
Atmos. Chem. Phys., 23, 4115–4122, https://doi.org/10.5194/acp-23-4115-2023, https://doi.org/10.5194/acp-23-4115-2023, 2023
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The impact of aerosols on clouds is one of the largest uncertainties in the human forcing of the climate. Aerosol can increase the concentrations of droplets in clouds, but observational and model studies produce widely varying estimates of this effect. We show that these estimates can be reconciled if only polluted clouds are studied, but this is insufficient to constrain the climate impact of aerosol. The uncertainty in aerosol impact on clouds is currently driven by cases with little aerosol.
Zackary Mages, Pavlos Kollias, Zeen Zhu, and Edward P. Luke
Atmos. Chem. Phys., 23, 3561–3574, https://doi.org/10.5194/acp-23-3561-2023, https://doi.org/10.5194/acp-23-3561-2023, 2023
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Cold-air outbreaks (when cold air is advected over warm water and creates low-level convection) are a dominant cloud regime in the Arctic, and we capitalized on ground-based observations, which did not previously exist, from the COMBLE field campaign to study them. We characterized the extent and strength of the convection and turbulence and found evidence of secondary ice production. This information is useful for model intercomparison studies that will represent cold-air outbreak processes.
Maria P. Cadeddu, Virendra P. Ghate, David D. Turner, and Thomas E. Surleta
Atmos. Chem. Phys., 23, 3453–3470, https://doi.org/10.5194/acp-23-3453-2023, https://doi.org/10.5194/acp-23-3453-2023, 2023
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We analyze the variability in marine boundary layer moisture at the Eastern North Atlantic site on a monthly and daily temporal scale and examine its fundamental role in the control of boundary layer cloudiness and precipitation. The study also highlights the complex interaction between large-scale and local processes controlling the boundary layer moisture and the importance of the mesoscale spatial distribution of vapor to support convection and precipitation.
Zhenquan Wang, Jian Yuan, Robert Wood, Yifan Chen, and Tiancheng Tong
Atmos. Chem. Phys., 23, 3247–3266, https://doi.org/10.5194/acp-23-3247-2023, https://doi.org/10.5194/acp-23-3247-2023, 2023
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This study develops a novel profile-based algorithm based on the ERA5 to estimate the inversion strength in the planetary boundary layer better than the previous inversion index, which is a key low-cloud-controlling factor. This improved measure is more effective at representing the meteorological influence on low-cloud variations. It can better constrain the meteorological influence on low clouds to better isolate cloud responses to aerosols or to estimate low cloud feedbacks in climate models.
Georgios Dekoutsidis, Silke Groß, Martin Wirth, Martina Krämer, and Christian Rolf
Atmos. Chem. Phys., 23, 3103–3117, https://doi.org/10.5194/acp-23-3103-2023, https://doi.org/10.5194/acp-23-3103-2023, 2023
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Cirrus clouds affect Earth's atmosphere, deeming our study important. Here we use water vapor measurements by lidar and study the relative humidity (RHi) within and around midlatitude cirrus clouds. We find high supersaturations in the cloud-free air and within the clouds, especially near the cloud top. We study two cloud types with different formation processes. Finally, we conclude that the shape of the distribution of RHi can be used as an indicator of different cloud evolutionary stages.
Huazhe Shang, Souichiro Hioki, Guillaume Penide, Céline Cornet, Husi Letu, and Jérôme Riedi
Atmos. Chem. Phys., 23, 2729–2746, https://doi.org/10.5194/acp-23-2729-2023, https://doi.org/10.5194/acp-23-2729-2023, 2023
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We find that cloud profiles can be divided into four prominent patterns, and the frequency of these four patterns is related to intensities of cloud-top entrainment and precipitation. Based on these analyses, we further propose a cloud profile parameterization scheme allowing us to represent these patterns. Our results shed light on how to facilitate the representation of cloud profiles and how to link them to cloud entrainment or precipitating status in future remote-sensing applications.
Luca Lelli, Marco Vountas, Narges Khosravi, and John Philipp Burrows
Atmos. Chem. Phys., 23, 2579–2611, https://doi.org/10.5194/acp-23-2579-2023, https://doi.org/10.5194/acp-23-2579-2023, 2023
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Arctic amplification describes the recent period in which temperatures have been rising twice as fast as or more than the global average and sea ice and the Greenland ice shelf are approaching a tipping point. Hence, the Arctic ability to reflect solar energy decreases and absorption by the surface increases. Using 2 decades of complementary satellite data, we discover that clouds unexpectedly increase the pan-Arctic reflectance by increasing their liquid water content, thus cooling the Arctic.
Yabin Gou, Haonan Chen, Hong Zhu, and Lulin Xue
Atmos. Chem. Phys., 23, 2439–2463, https://doi.org/10.5194/acp-23-2439-2023, https://doi.org/10.5194/acp-23-2439-2023, 2023
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This article investigates the complex precipitation microphysics associated with super typhoon Lekima using a host of in situ and remote sensing observations, including rain gauge and disdrometer data, as well as polarimetric radar observations. The impacts of precipitation microphysics on multi-source data consistency and radar precipitation estimation are quantified. It is concluded that the dynamical precipitation microphysical processes must be considered in radar precipitation estimation.
Hongxia Zhu, Rui Li, Shuping Yang, Chun Zhao, Zhe Jiang, and Chen Huang
Atmos. Chem. Phys., 23, 2421–2437, https://doi.org/10.5194/acp-23-2421-2023, https://doi.org/10.5194/acp-23-2421-2023, 2023
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The impacts of atmospheric dust aerosols and cloud dynamic conditions on precipitation vertical development in southeastern China were studied using multiple satellite observations. It was found that the precipitating drops under dusty conditions grow faster in the middle layer but slower in the upper and lower layers compared with their pristine counterparts. Quantitative estimation of the sensitivity of the precipitation top temperature to the dust aerosol optical depth is also provided.
Zane Dedekind, Jacopo Grazioli, Philip H. Austin, and Ulrike Lohmann
Atmos. Chem. Phys., 23, 2345–2364, https://doi.org/10.5194/acp-23-2345-2023, https://doi.org/10.5194/acp-23-2345-2023, 2023
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Simulations allowing ice particles to collide with one another producing more ice particles represented surface observations of ice particles accurately. An increase in ice particles formed through collisions was related to sharp changes in the wind direction and speed with height. Changes in wind speed and direction can therefore cause more enhanced collisions between ice particles and alter how fast and how much precipitation forms. Simulations were conducted with the atmospheric model COSMO.
Ramon Padullés, Estel Cardellach, and F. Joseph Turk
Atmos. Chem. Phys., 23, 2199–2214, https://doi.org/10.5194/acp-23-2199-2023, https://doi.org/10.5194/acp-23-2199-2023, 2023
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The results of comparing the polarimetric radio occultation observables and the ice water content retrieved from the CloudSat radar in a global and statistical way show a strong correlation between the geographical patterns of both quantities for a wide range of heights. This implies that horizontally oriented hydrometeors are systematically present through the whole globe and through all vertical levels, which could provide insights on the physical processes leading to precipitation.
Ziming Wang, Luca Bugliaro, Tina Jurkat-Witschas, Romy Heller, Ulrike Burkhardt, Helmut Ziereis, Georgios Dekoutsidis, Martin Wirth, Silke Groß, Simon Kirschler, Stefan Kaufmann, and Christiane Voigt
Atmos. Chem. Phys., 23, 1941–1961, https://doi.org/10.5194/acp-23-1941-2023, https://doi.org/10.5194/acp-23-1941-2023, 2023
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Differences in the microphysical properties of contrail cirrus and natural cirrus in a contrail outbreak situation during the ML-CIRRUS campaign over the North Atlantic flight corridor can be observed from in situ measurements. The cirrus radiative effect in the area of the outbreak, derived from satellite observation-based radiative transfer modeling, is warming in the early morning and cooling during the day.
Gerald G. Mace, Sally Benson, Ruhi Humphries, Peter M. Gombert, and Elizabeth Sterner
Atmos. Chem. Phys., 23, 1677–1685, https://doi.org/10.5194/acp-23-1677-2023, https://doi.org/10.5194/acp-23-1677-2023, 2023
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The number of cloud droplets per unit volume is a significantly important property of clouds that controls their reflective properties. Computer models of the Earth's atmosphere and climate have low skill at predicting the reflective properties of Southern Ocean clouds. Here we investigate the properties of those clouds using satellite data and find that the cloud droplet number and cloud albedo in the Southern Ocean are related to the oceanic phytoplankton abundance near Antarctica.
Jianhao Zhang and Graham Feingold
Atmos. Chem. Phys., 23, 1073–1090, https://doi.org/10.5194/acp-23-1073-2023, https://doi.org/10.5194/acp-23-1073-2023, 2023
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Using observations from space, we show maps of potential brightness changes in marine warm clouds in response to increases in cloud droplet concentrations. The environmental and aerosol conditions in which these clouds reside covary differently in each ocean basin, leading to distinct evolutions of cloud brightness changes. This work stresses the central importance of the covariability between meteorology and aerosol for scaling up the radiative response of cloud brightness changes.
Yuxin Zhao, Jiming Li, Lijie Zhang, Cong Deng, Yarong Li, Bida Jian, and Jianping Huang
Atmos. Chem. Phys., 23, 743–769, https://doi.org/10.5194/acp-23-743-2023, https://doi.org/10.5194/acp-23-743-2023, 2023
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Diurnal variations of clouds play an important role in the radiative budget and precipitation. Based on satellite observations, reanalysis, and CMIP6 outputs, the diurnal variations in total cloud cover and cloud vertical distribution over the Tibetan Plateau are explored. The diurnal cycle of cirrus is a key focus and found to have different characteristics from those found in the tropics. The relationship between the diurnal cycle of cirrus and meteorological factors is also discussed.
Qiang Li and Silke Groß
Atmos. Chem. Phys., 22, 15963–15980, https://doi.org/10.5194/acp-22-15963-2022, https://doi.org/10.5194/acp-22-15963-2022, 2022
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The IPCC report identified that cirrus clouds have a significant impact on the radiation balance comparable to the CO2 effects, which, however, is still hard to parameterize. The current study investigates the possible impact of aviation on cirrus properties based on the analysis of 10-year lidar measurements of CALIPSO. The results reveal that there is a significant positive trend in cirrus depolarization ratio in the last 10 years before COVID-19, which is strongly correlated with aviation.
Linda Forster and Bernhard Mayer
Atmos. Chem. Phys., 22, 15179–15205, https://doi.org/10.5194/acp-22-15179-2022, https://doi.org/10.5194/acp-22-15179-2022, 2022
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We present a novel retrieval using ground-based imaging observations of halo displays together with radiative transfer simulations to help improve our understanding of ice crystal properties representative of cirrus clouds. Analysis of 4400 calibrated HaloCam images featuring a 22° halo revealed aggregates of hexagonal columns of 20 µm effective radius with a mixture of about 37 % smooth and 63% severely roughened surfaces as the best match in general.
Yun He, Zhenping Yin, Fuchao Liu, and Fan Yi
Atmos. Chem. Phys., 22, 13067–13085, https://doi.org/10.5194/acp-22-13067-2022, https://doi.org/10.5194/acp-22-13067-2022, 2022
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A method is proposed to identify the sole presence of heterogeneous nucleation and competition between heterogeneous and homogeneous nucleation for dust-related cirrus clouds by characterizing the relationship between dust ice-nucleating particle concentration calculated from CALIOP using the POLIPHON method and in-cloud ice crystal number concentration from the DARDAR-Nice dataset. Two typical cirrus cases are shown as a demonstration, and the proposed method can be extended to a global scale.
Frederic Tridon, Israel Silber, Alessandro Battaglia, Stefan Kneifel, Ann Fridlind, Petros Kalogeras, and Ranvir Dhillon
Atmos. Chem. Phys., 22, 12467–12491, https://doi.org/10.5194/acp-22-12467-2022, https://doi.org/10.5194/acp-22-12467-2022, 2022
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The role of ice precipitation in the Earth water budget is not well known because ice particles are complex, and their formation involves intricate processes. Riming of ice crystals by supercooled water droplets is an efficient process, but little is known about its importance at high latitudes. In this work, by exploiting the deployment of an unprecedented number of remote sensing systems in Antarctica, we find that riming occurs at much lower temperatures compared with the mid-latitudes.
Leonie von Terzi, José Dias Neto, Davide Ori, Alexander Myagkov, and Stefan Kneifel
Atmos. Chem. Phys., 22, 11795–11821, https://doi.org/10.5194/acp-22-11795-2022, https://doi.org/10.5194/acp-22-11795-2022, 2022
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We present a statistical analysis of ice microphysical processes (IMP) in mid-latitude clouds. Combining various radar approaches, we find that the IMP active at −20 to −10 °C seems to be the main driver of ice particle size, shape and concentration. The strength of aggregation at −20 to −10 °C correlates with the increase in concentration and aspect ratio of locally formed ice particles. Despite ongoing aggregation, the concentration of ice particles stays enhanced until −4 °C.
Edward Gryspeerdt, Franziska Glassmeier, Graham Feingold, Fabian Hoffmann, and Rebecca J. Murray-Watson
Atmos. Chem. Phys., 22, 11727–11738, https://doi.org/10.5194/acp-22-11727-2022, https://doi.org/10.5194/acp-22-11727-2022, 2022
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The response of clouds to changes in aerosol remains a large uncertainty in our understanding of the climate. Studies typically look at aerosol and cloud processes in snapshot images, measuring all properties at the same time. Here we use multiple images to characterise how cloud temporal development responds to aerosol. We find a reduction in liquid water path with increasing aerosol, party due to feedbacks. This suggests the aerosol impact on cloud water may be weaker than in previous studies.
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Short summary
This study investigates the microphysics of winter alpine snowfall occurring in mixed-phase clouds in an inner-Alpine valley during CLACE2014. From polarimetric radar and in situ observations, riming is shown to be an important process leading to more intense snowfall. Riming is usually associated with more intense turbulence providing supercooled liquid water. Distinct features are identified in the vertical structure of polarimetric radar variables.
This study investigates the microphysics of winter alpine snowfall occurring in mixed-phase...
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