Articles | Volume 12, issue 23
https://doi.org/10.5194/acp-12-11723-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-12-11723-2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Experimental and modeled UV erythemal irradiance under overcast conditions: the role of cloud optical depth
M. Antón
Geophysics Centre of Evora, University of Evora, Evora, Portugal
Departamento de Física, Universidad de Extremadura, Badajoz, Spain
L. Alados-Arboledas
Centro Andaluz de Medio Ambiente (CEAMA), Universidad de Granada, Granada, Spain
Departamento de Física Aplicada, Universidad de Granada, Granada, Spain
J. L. Guerrero-Rascado
Centro Andaluz de Medio Ambiente (CEAMA), Universidad de Granada, Granada, Spain
Departamento de Física Aplicada, Universidad de Granada, Granada, Spain
Geophysics Centre of Evora, University of Evora, Evora, Portugal
M. J. Costa
Geophysics Centre of Evora, University of Evora, Evora, Portugal
J. C Chiu
Department of Meteorology, University of Reading, Reading, UK
F. J. Olmo
Centro Andaluz de Medio Ambiente (CEAMA), Universidad de Granada, Granada, Spain
Departamento de Física Aplicada, Universidad de Granada, Granada, Spain
Related authors
Francisco Javier Acero, Manuel Antón, Alejandro Jesús Pérez Aparicio, Nieves Bravo-Paredes, Víctor Manuel Sánchez Carrasco, María Cruz Gallego, José Agustín García, Marcelino Núñez, Irene Tovar, Javier Vaquero-Martínez, and José Manuel Vaquero
Nat. Hazards Earth Syst. Sci., 25, 305–320, https://doi.org/10.5194/nhess-25-305-2025, https://doi.org/10.5194/nhess-25-305-2025, 2025
Short summary
Short summary
The month of June 1925 was found to be exceptional in the southwest interior of the Iberian Peninsula due to the large number of thunderstorms and their significant impacts, with serious losses of human lives and material resources. We analyzed this event from different, complementary perspectives: reconstruction of the history of the events from newspapers, study of monthly meteorological variables of the longest series available, and the analysis of the meteorological synoptic situation.
María Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Michaël Sicard, Jesús Abril-Gago, Vanda Salgueiro, Adolfo Comerón, María José Granados-Muñoz, Maria João Costa, Constantino Muñoz-Porcar, Juan Antonio Bravo-Aranda, Daniele Bortoli, Alejandro Rodríguez-Gómez, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
EGUsphere, https://doi.org/10.5194/egusphere-2025-4905, https://doi.org/10.5194/egusphere-2025-4905, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Due to the major radiative role of dust in Climate Change, a vertical assessment of the long-wave (and net) dust direct radiative effect of both fine and coarse dust, separately, is introduced. The study relies on an intense Saharan dust outbreak across the Iberian Peninsula, observed by five lidar stations with SW-centre-NE coverage. A comparative evaluation of the differences by considering the total dust (no separation) is also examined. It complements a similar study in the short-wave range.
Ana del Águila, Pablo Ortiz-Amezcua, Siham Tabik, Juan Antonio Bravo-Aranda, Sol Fernández-Carvelo, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 25, 12549–12567, https://doi.org/10.5194/acp-25-12549-2025, https://doi.org/10.5194/acp-25-12549-2025, 2025
Short summary
Short summary
This study applies machine learning (ML) techniques to classify aerosols using high-resolution multiwavelength lidar data from EARLINET network. We developed a reference dataset and evaluated six ML models, with LightGBM achieving over 90 % accuracy. Depolarization data proved critical for improving dust classification. Validated against independent datasets, our approach improves aerosol classification and may help refine lidar-based processing strategies.
Jesús Yus-Díez, Luka Drinovec, Lucas Alados-Arboledas, Gloria Titos, Elena Bazo, Andrea Casans, Diego Patrón, Xavier Querol, Adolfo Gonzalez-Romero, Carlos Perez García-Pando, and Griša Močnik
Atmos. Meas. Tech., 18, 3073–3093, https://doi.org/10.5194/amt-18-3073-2025, https://doi.org/10.5194/amt-18-3073-2025, 2025
Short summary
Short summary
We have used absorption from a photothermal interferometer and scattering measurements to evaluate the most deployed filter photometers used to measure absorption for monitoring networks. We used soot- and dust-dominated aerosol samples in both laboratory and ambient settings. Our results indicated that one of these filter photometers, the MAAP (Multiangle Absorption Photometer), usually used as a pseudo-reference instrument, had 47 % higher absorption values than our reference measurements.
Elena Bazo, Daniel Pérez-Ramírez, Antonio Valenzuela, J. Vanderlei Martins, Gloria Titos, Alberto Cazorla, Fernando Rejano, Diego Patrón, Arlett Díaz-Zurita, Francisco José García-Izquierdo, David Fuertes, Lucas Alados-Arboledas, and Francisco José Olmo
Atmos. Chem. Phys., 25, 6325–6352, https://doi.org/10.5194/acp-25-6325-2025, https://doi.org/10.5194/acp-25-6325-2025, 2025
Short summary
Short summary
This works analyzes the aerosol scattering phase function for transported Saharan dust to the city of Granada – located in southwestern Europe. We use the novel technique polar imaging nephelometry that helps to determine the phase functions using a CMOS camera. The capability of measuring with polarized light helps to infer new properties about the mixture of Saharan dust particles with those of anthropogenic origin.
Kaiden Sookdar, Scott Edward Giangrande, John Rausch, Lihong Ma, Meng Wang, Dié Wang, Michael Jensen, Ching-Shu Hung, and J. Christine Chiu
EGUsphere, https://doi.org/10.5194/egusphere-2025-694, https://doi.org/10.5194/egusphere-2025-694, 2025
Short summary
Short summary
Photometer observations of stratocumulus cloud properties are evaluated for a multiyear archive. Retrievals for cloud optical depth, cloud droplet effective radius, and liquid water path show solid agreement with collocated references. Continental stratocumulus clouds sorted by cloud thickness indicate double the cloud optical depth and liquid water path of their marine counterparts, while exhibiting similar bulk cloud droplet effective radius.
María-Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Michaël Sicard, Jesús Abril-Gago, Vanda Salgueiro, Adolfo Comerón, María José Granados-Muñoz, Maria João Costa, Constantino Muñoz-Porcar, Juan Antonio Bravo-Aranda, Daniele Bortoli, Alejandro Rodríguez-Gómez, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 25, 3213–3231, https://doi.org/10.5194/acp-25-3213-2025, https://doi.org/10.5194/acp-25-3213-2025, 2025
Short summary
Short summary
Due to the significant radiative role of dust in climate change, vertical assessments of the short-wave dust direct radiative effect of both fine and coarse dust particles are performed separately. The study is focused on an intense Saharan dust outbreak crossing the Iberian Peninsula in springtime monitored by five Iberian lidar stations with southwest–northeast coverage. A comparative study to evaluate the differences found by considering the total dust (no separation) is also examined.
Francisco Javier Acero, Manuel Antón, Alejandro Jesús Pérez Aparicio, Nieves Bravo-Paredes, Víctor Manuel Sánchez Carrasco, María Cruz Gallego, José Agustín García, Marcelino Núñez, Irene Tovar, Javier Vaquero-Martínez, and José Manuel Vaquero
Nat. Hazards Earth Syst. Sci., 25, 305–320, https://doi.org/10.5194/nhess-25-305-2025, https://doi.org/10.5194/nhess-25-305-2025, 2025
Short summary
Short summary
The month of June 1925 was found to be exceptional in the southwest interior of the Iberian Peninsula due to the large number of thunderstorms and their significant impacts, with serious losses of human lives and material resources. We analyzed this event from different, complementary perspectives: reconstruction of the history of the events from newspapers, study of monthly meteorological variables of the longest series available, and the analysis of the meteorological synoptic situation.
Fernando Rejano, Andrea Casans, Marta Via, Juan Andrés Casquero-Vera, Sonia Castillo, Hassan Lyamani, Alberto Cazorla, Elisabeth Andrews, Daniel Pérez-Ramírez, Andrés Alastuey, Francisco Javier Gómez-Moreno, Lucas Alados-Arboledas, Francisco José Olmo, and Gloria Titos
Atmos. Chem. Phys., 24, 13865–13888, https://doi.org/10.5194/acp-24-13865-2024, https://doi.org/10.5194/acp-24-13865-2024, 2024
Short summary
Short summary
This study provides valuable insights to improve cloud condensation nuclei (CCN) estimations at a high-altitude remote site which is influenced by nearby urban pollution. Understanding the factors that affect CCN estimations is essential to improve the CCN data coverage worldwide and assess aerosol–cloud interactions on a global scale. This is crucial for improving climate models, since aerosol–cloud interactions are the most important source of uncertainty in climate projections.
Wenyue Wang, Klemens Hocke, Leonardo Nania, Alberto Cazorla, Gloria Titos, Renaud Matthey, Lucas Alados-Arboledas, Agustín Millares, and Francisco Navas-Guzmán
Atmos. Chem. Phys., 24, 1571–1585, https://doi.org/10.5194/acp-24-1571-2024, https://doi.org/10.5194/acp-24-1571-2024, 2024
Short summary
Short summary
The south-central interior of Andalusia experiences complex precipitation patterns as a result of the semi-arid Mediterranean climate and the influence of Saharan dust. This study monitored the inter-relations between aerosols, clouds, meteorological variables, and precipitation systems using ground-based remote sensing and in situ instruments.
Juan Andrés Casquero-Vera, Daniel Pérez-Ramírez, Hassan Lyamani, Fernando Rejano, Andrea Casans, Gloria Titos, Francisco José Olmo, Lubna Dada, Simo Hakala, Tareq Hussein, Katrianne Lehtipalo, Pauli Paasonen, Antti Hyvärinen, Noemí Pérez, Xavier Querol, Sergio Rodríguez, Nikos Kalivitis, Yenny González, Mansour A. Alghamdi, Veli-Matti Kerminen, Andrés Alastuey, Tuukka Petäjä, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 23, 15795–15814, https://doi.org/10.5194/acp-23-15795-2023, https://doi.org/10.5194/acp-23-15795-2023, 2023
Short summary
Short summary
Here we present the first study of the effect of mineral dust on the inhibition/promotion of new particle formation (NPF) events in different dust-influenced areas. Unexpectedly, we show that the occurrence of NPF events is highly frequent during mineral dust outbreaks, occurring even during extreme dust outbreaks. We also show that the occurrence of NPF events during mineral dust outbreaks significantly affects the potential cloud condensation nuclei budget.
Alexandra Tsekeri, Anna Gialitaki, Marco Di Paolantonio, Davide Dionisi, Gian Luigi Liberti, Alnilam Fernandes, Artur Szkop, Aleksander Pietruczuk, Daniel Pérez-Ramírez, Maria J. Granados Muñoz, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Diego Bermejo Pantaleón, Juan Antonio Bravo-Aranda, Anna Kampouri, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Salvatore Romano, Maria Rita Perrone, Xiaoxia Shang, Mika Komppula, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Diofantos Hadjimitsis, Francisco Navas-Guzmán, Alexander Haefele, Dominika Szczepanik, Artur Tomczak, Iwona S. Stachlewska, Livio Belegante, Doina Nicolae, Kalliopi Artemis Voudouri, Dimitris Balis, Athena A. Floutsi, Holger Baars, Linda Miladi, Nicolas Pascal, Oleg Dubovik, and Anton Lopatin
Atmos. Meas. Tech., 16, 6025–6050, https://doi.org/10.5194/amt-16-6025-2023, https://doi.org/10.5194/amt-16-6025-2023, 2023
Short summary
Short summary
EARLINET/ACTRIS organized an intensive observational campaign in May 2020, with the objective of monitoring the atmospheric state over Europe during the COVID-19 lockdown and relaxation period. The work presented herein focuses on deriving a common methodology for applying a synergistic retrieval that utilizes the network's ground-based passive and active remote sensing measurements and deriving the aerosols from anthropogenic activities over Europe.
Jesús Abril-Gago, Pablo Ortiz-Amezcua, Diego Bermejo-Pantaleón, Juana Andújar-Maqueda, Juan Antonio Bravo-Aranda, María José Granados-Muñoz, Francisco Navas-Guzmán, Lucas Alados-Arboledas, Inmaculada Foyo-Moreno, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 8453–8471, https://doi.org/10.5194/acp-23-8453-2023, https://doi.org/10.5194/acp-23-8453-2023, 2023
Short summary
Short summary
Validation activities of Aeolus wind products were performed in Granada with different upward-probing instrumentation (Doppler lidar system and radiosondes) and spatiotemporal collocation criteria. Specific advantages and disadvantages of each instrument were identified, and an optimal comparison criterion is proposed. Aeolus was proven to provide reliable wind products, and the upward-probing instruments were proven to be useful for Aeolus wind product validation activities.
Konstantinos Michailidis, Maria-Elissavet Koukouli, Dimitris Balis, J. Pepijn Veefkind, Martin de Graaf, Lucia Mona, Nikolaos Papagianopoulos, Gesolmina Pappalardo, Ioanna Tsikoudi, Vassilis Amiridis, Eleni Marinou, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Daniele Bortoli, Maria João Costa, Vanda Salgueiro, Alexandros Papayannis, Maria Mylonaki, Lucas Alados-Arboledas, Salvatore Romano, Maria Rita Perrone, and Holger Baars
Atmos. Chem. Phys., 23, 1919–1940, https://doi.org/10.5194/acp-23-1919-2023, https://doi.org/10.5194/acp-23-1919-2023, 2023
Short summary
Short summary
Comparisons with ground-based correlative lidar measurements constitute a key component in the validation of satellite aerosol products. This paper presents the validation of the TROPOMI aerosol layer height (ALH) product, using archived quality assured ground-based data from lidar stations that belong to the EARLINET network. Comparisons between the TROPOMI ALH and co-located EARLINET measurements show good agreement over the ocean.
Simone Kotthaus, Juan Antonio Bravo-Aranda, Martine Collaud Coen, Juan Luis Guerrero-Rascado, Maria João Costa, Domenico Cimini, Ewan J. O'Connor, Maxime Hervo, Lucas Alados-Arboledas, María Jiménez-Portaz, Lucia Mona, Dominique Ruffieux, Anthony Illingworth, and Martial Haeffelin
Atmos. Meas. Tech., 16, 433–479, https://doi.org/10.5194/amt-16-433-2023, https://doi.org/10.5194/amt-16-433-2023, 2023
Short summary
Short summary
Profile observations of the atmospheric boundary layer now allow for layer heights and characteristics to be derived at high temporal and vertical resolution. With novel high-density ground-based remote-sensing measurement networks emerging, horizontal information content is also increasing. This review summarises the capabilities and limitations of various sensors and retrieval algorithms which need to be considered during the harmonisation of data products for high-impact applications.
María Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Diego Bermejo-Pantaleón, Michaël Sicard, Vanda Salgueiro, Francisco Molero, Clara Violeta Carvajal-Pérez, María José Granados-Muñoz, Adolfo Comerón, Flavio T. Couto, Rubén Barragán, María-Paz Zorzano, Juan Antonio Bravo-Aranda, Constantino Muñoz-Porcar, María João Costa, Begoña Artíñano, Alejandro Rodríguez-Gómez, Daniele Bortoli, Manuel Pujadas, Jesús Abril-Gago, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 143–161, https://doi.org/10.5194/acp-23-143-2023, https://doi.org/10.5194/acp-23-143-2023, 2023
Short summary
Short summary
An intense Saharan dust outbreak crossing the Iberian Peninsula in springtime was monitored to determinine the specific contribution of fine and coarse dust particles at five lidar stations, strategically covering its SW–central–NE pathway. Expected dust ageing along the transport started unappreciated. A different fine-dust impact on optical (~30 %) and mass (~10 %) properties was found. Use of polarized lidar measurements (mainly in elastic systems) for fine/coarse dust separation is crucial.
Jesús Abril-Gago, Juan Luis Guerrero-Rascado, Maria João Costa, Juan Antonio Bravo-Aranda, Michaël Sicard, Diego Bermejo-Pantaleón, Daniele Bortoli, María José Granados-Muñoz, Alejandro Rodríguez-Gómez, Constantino Muñoz-Porcar, Adolfo Comerón, Pablo Ortiz-Amezcua, Vanda Salgueiro, Marta María Jiménez-Martín, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 22, 1425–1451, https://doi.org/10.5194/acp-22-1425-2022, https://doi.org/10.5194/acp-22-1425-2022, 2022
Short summary
Short summary
A validation of Aeolus reprocessed optical products is carried out via an intercomparison with ground-based measurements taken at several ACTRIS/EARLINET stations in western Europe. Case studies and a statistical analysis are presented. The stations are located in a hot spot between Africa and the rest of Europe, which guarantees a variety of aerosol types, from mineral dust layers to continental/anthropogenic aerosol, and allows us to test Aeolus performance under different scenarios.
Nicholas J. Kedzuf, J. Christine Chiu, V. Chandrasekar, Sounak Biswas, Shashank S. Joshil, Yinghui Lu, Peter Jan van Leeuwen, Christopher Westbrook, Yann Blanchard, and Sebastian O'Shea
Atmos. Meas. Tech., 14, 6885–6904, https://doi.org/10.5194/amt-14-6885-2021, https://doi.org/10.5194/amt-14-6885-2021, 2021
Short summary
Short summary
Ice clouds play a key role in our climate system due to their strong controls on precipitation and the radiation budget. However, it is difficult to characterize co-existing ice species using radar observations. We present a new method that separates the radar signals of pristine ice embedded in snow aggregates and retrieves their respective abundances and sizes for the first time. The ability to provide their quantitative microphysical properties will open up many research opportunities.
Mariana Adam, Iwona S. Stachlewska, Lucia Mona, Nikolaos Papagiannopoulos, Juan Antonio Bravo-Aranda, Michaël Sicard, Doina N. Nicolae, Livio Belegante, Lucja Janicka, Dominika Szczepanik, Maria Mylonaki, Christina-Anna Papanikolaou, Nikolaos Siomos, Kalliopi Artemis Voudouri, Luca Alados-Arboledas, Arnoud Apituley, Ina Mattis, Anatoli Chaikovsky, Constantino Muñoz-Porcar, Aleksander Pietruczuk, Daniele Bortoli, Holger Baars, Ivan Grigorov, and Zahary Peshev
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-759, https://doi.org/10.5194/acp-2021-759, 2021
Revised manuscript not accepted
Short summary
Short summary
Results over 10 years of biomass burning events measured by EARLINET are analysed by means of the intensive parameters, based on the methodology described in Part I. Smoke type is characterized for each of the four geographical regions based on continental smoke origin. Relationships between intensive parameters or colour ratios are shown. The smoke is labelled in average as aged smoke.
Gloria Titos, María A. Burgos, Paul Zieger, Lucas Alados-Arboledas, Urs Baltensperger, Anne Jefferson, James Sherman, Ernest Weingartner, Bas Henzing, Krista Luoma, Colin O'Dowd, Alfred Wiedensohler, and Elisabeth Andrews
Atmos. Chem. Phys., 21, 13031–13050, https://doi.org/10.5194/acp-21-13031-2021, https://doi.org/10.5194/acp-21-13031-2021, 2021
Short summary
Short summary
This paper investigates the impact of water uptake on aerosol optical properties, in particular the aerosol light-scattering coefficient. Although in situ measurements are performed at low relative humidity (typically at
RH < 40 %), to address the climatic impact of aerosol particles it is necessary to take into account the effect that water uptake may have on the aerosol optical properties.
Jose Antonio Benavent-Oltra, Juan Andrés Casquero-Vera, Roberto Román, Hassan Lyamani, Daniel Pérez-Ramírez, María José Granados-Muñoz, Milagros Herrera, Alberto Cazorla, Gloria Titos, Pablo Ortiz-Amezcua, Andrés Esteban Bedoya-Velásquez, Gregori de Arruda Moreira, Noemí Pérez, Andrés Alastuey, Oleg Dubovik, Juan Luis Guerrero-Rascado, Francisco José Olmo-Reyes, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 21, 9269–9287, https://doi.org/10.5194/acp-21-9269-2021, https://doi.org/10.5194/acp-21-9269-2021, 2021
Short summary
Short summary
In this paper, we use the GRASP algorithm combining different remote sensing measurements to obtain the aerosol vertical and column properties during the SLOPE I and II campaigns. We show an overview of aerosol properties retrieved by GRASP during these campaigns and evaluate the retrievals of aerosol properties using the in situ measurements performed at a high-altitude station and airborne flights. For the first time we present an evaluation of the absorption coefficient by GRASP.
Nikolaos Evangeliou, Stephen M. Platt, Sabine Eckhardt, Cathrine Lund Myhre, Paolo Laj, Lucas Alados-Arboledas, John Backman, Benjamin T. Brem, Markus Fiebig, Harald Flentje, Angela Marinoni, Marco Pandolfi, Jesus Yus-Dìez, Natalia Prats, Jean P. Putaud, Karine Sellegri, Mar Sorribas, Konstantinos Eleftheriadis, Stergios Vratolis, Alfred Wiedensohler, and Andreas Stohl
Atmos. Chem. Phys., 21, 2675–2692, https://doi.org/10.5194/acp-21-2675-2021, https://doi.org/10.5194/acp-21-2675-2021, 2021
Short summary
Short summary
Following the transmission of SARS-CoV-2 to Europe, social distancing rules were introduced to prevent further spread. We investigate the impacts of the European lockdowns on black carbon (BC) emissions by means of in situ observations and inverse modelling. BC emissions declined by 23 kt in Europe during the lockdowns as compared with previous years and by 11 % as compared to the period prior to lockdowns. Residential combustion prevailed in Eastern Europe, as confirmed by remote sensing data.
Ourania Soupiona, Alexandros Papayannis, Panagiotis Kokkalis, Romanos Foskinis, Guadalupe Sánchez Hernández, Pablo Ortiz-Amezcua, Maria Mylonaki, Christina-Anna Papanikolaou, Nikolaos Papagiannopoulos, Stefanos Samaras, Silke Groß, Rodanthi-Elisavet Mamouri, Lucas Alados-Arboledas, Aldo Amodeo, and Basil Psiloglou
Atmos. Chem. Phys., 20, 15147–15166, https://doi.org/10.5194/acp-20-15147-2020, https://doi.org/10.5194/acp-20-15147-2020, 2020
Short summary
Short summary
51 dust events over the Mediterranean from EARLINET were studied regarding the aerosol geometrical, optical and microphysical properties and radiative forcing. We found δp532 values of 0.24–0.28, LR532 values of 49–52 sr and AOT532 of 0.11–0.40. The aerosol mixing state was also examined. Depending on the dust properties, intensity and solar zenith angle, the estimated solar radiative forcing ranged from −59 to −22 W m−2 at the surface and from −24 to −1 W m−2 at the TOA (cooling effect).
Juan Andrés Casquero-Vera, Hassan Lyamani, Lubna Dada, Simo Hakala, Pauli Paasonen, Roberto Román, Roberto Fraile, Tuukka Petäjä, Francisco José Olmo-Reyes, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 20, 14253–14271, https://doi.org/10.5194/acp-20-14253-2020, https://doi.org/10.5194/acp-20-14253-2020, 2020
Short summary
Short summary
New particle formation was investigated at two stations located close to each other but at different altitudes: urban and high-altitude sites. Results show that sulfuric acid is able to explain a minimal fraction contribution to the observed growth rates and point to the availability of volatile organic compounds as the main factor controlling NPF events at both sites. A closer analysis of the NPF events that were observed at high-altitude sites during a Saharan dust episode was carried out.
Roberto Román, Ramiro González, Carlos Toledano, África Barreto, Daniel Pérez-Ramírez, Jose A. Benavent-Oltra, Francisco J. Olmo, Victoria E. Cachorro, Lucas Alados-Arboledas, and Ángel M. de Frutos
Atmos. Meas. Tech., 13, 6293–6310, https://doi.org/10.5194/amt-13-6293-2020, https://doi.org/10.5194/amt-13-6293-2020, 2020
Short summary
Short summary
Atmospheric-aerosol and gaseous properties can be derived at night-time if the lunar irradiance at the ground is measured. To this end, the knowledge of lunar irradiance at the top of the atmosphere is necessary. This extraterrestrial lunar irradiance is usually calculated by models since it varies with several geometric factors mainly depending on time and location. This paper proposes a correction to the most used lunar-irradiance model to be applied for atmospheric-aerosol characterization.
Cited articles
Alados-Arboledas, L., Alados, I., Foyo-Moreno, I., Olmo, F. J., and Alcántara, A.: The influence of clouds on surface UV erythemal irradiance, Atmos. Res., 66, 273–290, 2003.
Anderson, G., Clough, S., Kneizys, F., Chetwynd, J., and Shettle, E.: AFGL atmospheric constituent profiles (0–120 km), Tech. Rep. AFGL-TR-86-0110, Air Force Geophys. Lab., Hanscom Air Force Base, Bedford, Mass, 1986.
Antón, M., Gil, J. E., Cazorla, A., Fernández-Gálvez, J., Vilaplana, J. M., Olmo, F. J., and Alados-Arboledas, L.: Influence of the calibration on experimental UV index at a midlatitude site, Granada (Spain), Atmos. Meas. Tech., 4, 499–507, https://doi.org/10.5194/amt-4-499-2011, 2011a.
Antón, M., Gil, J. E., Fernández-Gálvez, J., Lyamani, H., Valenzuela, A., Foyo-Moreno, I., Olmo, F. J., and Alados-Arboledas, L.: Evaluation of the aerosol forcing efficiency in the UV erythemal range at Granada (Spain), J. Geophys. Res., 116, D20214, https://doi.org/10.1029/2011JD016112, 2011b.
Aun, M., Eerme, K., Ansko, I., Veismann, U., and Lätt, S.: Modification of spectral ultraviolet doses by different types of overcast cloudiness and atmospheric aerosol, Photochem. Photobiol., 87, 461–469, 2011.
Bais, A. F., Zerefos, C. S., Meleti, C., Ziomas, I. C., and Tourpali, K.: Spectral measurements of solar UVB radiation and its relations to total ozone, SO2 and clouds, J. Geophys. Res., 98, 5199–5204, 1993.
Bernhard, G., Booth, C. R., and Ehramjian, J. C.: Version 2 data of the National Science Foundation's Ultraviolet Radiation Monitoring Network: South Pole, J. Geophys. Res., 109, D21207, https://doi.org/10.1029/2004JD004937, 2004.
Binyamin, J., Davies, J., and McArthur, B.: UV-B cloud optical properties for Canada, Int. J. Climatol., 30, 1246–1255, 2010.
Blumthaler, M., Ambach, W., and Salzberg, M.: Effects of cloudiness on global and diffuse UV irradiance in a high mountain area, Theor. Appl. Climatol., 50, 23–30, 1994.
Calbó, J., Pagés, D., and González, J.: Empirical studies of cloud effects on UV radiation: A review, Rev. Geophys., 43, RG2002, https://doi.org/10.1029/2004RG000155, 2005.
Cazorla, A., Olmo, F. J., and Alados-Arboledas, L.: Development of a sky imager for cloud cover assessment, J. Opt. Soc. Am. A., 25, 29–39, https://doi.org/10.1364/JOSAA.25.000029, 2008a.
Cazorla, A., Olmo, F. J., and Alados-Arboledas, L.: Using a sky imager for aerosol characterization, Atmos. Environ., 42, 2739–2745, https://doi.org/10.1016/j.atmosenv.2007.06.016, 2008b.
Cazorla, A., Shields, J. E., Karr, M. E., Olmo, F. J., Burden, A., and Alados-Arboledas, L.: Technical Note: Determination of aerosol optical properties by a calibrated sky imager, Atmos. Chem. Phys., 9, 6417–6427, https://doi.org/10.5194/acp-9-6417-2009, 2009.
Chiu, J. C., Marshak, A., Knyazikhin, Y., Wiscombe, W. J., Barker, H. W., Barnard, J. C., and Luo, Y.: Remote sensing of cloud properties using ground-based measurements of zenith radiance, J. Geophys. Res., 111, D16201, https://doi.org/10.1029/2005JD006843, 2006.
Chiu, J. C., Huang, C. H., Marshak, A., Slutsker, I., Giles, D. M., Holben, B.N., Knyazikhin, Y., and Wiscombe, W. J.: Cloud optical depth retrievals from the Aerosol Robotic Network (AERONET) cloud mode observations, J. Geophys. Res., 115, D14202, https://doi.org/10.1029/2009JD013121, 2010.
de Backer, H., Koepke, P., Bais, A., de Cabo, X., Frei, T., Gillotay, D., Haite, C., Heikkilä, A., Kazantzidis, A., Koskela, T., Kyrö, E., Lapeta, B., Lorente, J., Masson, K., Mayer, B., Plets, H., Redondas, A., Renaud, A., Schauberger, G., Schmalwieser, A., Schwander, H., and Vanicek, K.: Comparison of measured and modelled uv indices for the assessment of health risks, Meteorol. Appl., 8, 267–277, 2001.
Diffey, B.: Solar ultraviolet radiation effects on biological systems, Phys. Med. Biol., 36, 299–328, 1991.
Diffey, B.: Climate change, ozone depletion and the impact on ultraviolet exposure of human skin, Phys. Med. Biol., 49, R1–R11, 2004.
Dubovik, O. and King, M. D.: A flexible inversion algorithm for retrieval of aerosol optical properties from Sun and sky radiance measurements, J. Geophys. Res., 105, 20673–20696, https://doi.org/10.1029/2000JD900282, 2000.
Esteve, A. R., Marin, M. J., Tena, F., Utrillas, M. P., and Martínez-Lozano, J. A.: Influence of cloudiness over the values of erythemal radiation in Valencia, Spain, Int. J. Climatol., 30, 127–136, https://doi.org/10.1002/joc.1883, 2010.
Estupiñan, J. G., Raman, S., Grescenti, G. H., Streicher, J. J., and Barnard, W. F.: Effects of clouds and haze on UV-B radiation, J. Geophys. Res., 101, 16807–16816, 1996.
Forster, P. M. de F.: Modeling ultraviolet radiation at the Earth's surface. Part I: The sensitivity of ultraviolet irradiances to atmospheric changes, J. Appl. Meteorol., 34, 2412–2425, 1995.
Frederick, J. E. and Snell, H. E.: Tropospheric influence on solar ultraviolet radiation: The role of clouds, J. Climatol., 3, 373–381, 1990.
Frederick, J. E. and Steele, H. D.: The transmission of sunlight through cloudy skies: An analysis based on standard meteorological information, J. Appl. Meteorol., 34, 2755–2761, 1995.
Grant, R. H. and Heisler, G. M.: Estimation of ultraviolet-B irradiance under variable cloud conditions, J. Appl. Meteorol, 39, 904–916, 2000.
Holben, B. N., Eck, T. F., Slutsker, I., Tanre, D., Buis, J. P., Setzer, A., Vermote, E., Reagan, J. A., Kaufman, Y. J., Nakajima, T., Lavenu, F., Jankowiak, I., and Smirnov, A.: AERONET – A federated instrument network and data archive for aerosol characterization, Remote Sens. Environ., 66, 1–16, https://doi.org/10.1016/S0034-4257(98)00031-5, 1998.
Hülsen, G. and Gröbner, J.: Characterization and calibration of ultraviolet broadband radiometers measuring erythemally weighted irradiance, Appl. Optics, 46, 5877–5886, 2007.
Ilyas, M.: Effect of cloudiness on solar ultraviolet radiation reaching the surface, Atmos. Environ., 21, 1483–1484, 1987.
Iqbal, M.: Introduction to Solar Radiation, Acad. Press, Toronto, Canada, 1983.
Josefsson, W.: Solar ultraviolet radiation in Sweden, SMHI Rep. Meteorol. Climatol. 53, 71 pp., Swed. Meteorol. And Hydrol. Inst., Norrköping, Sweden, 1986.
Josefsson, W. and Landelius, T.: Effect of clouds on UV irradiance: As estimated from cloud amount, cloud type, precipitation, global radiation and sunshine duration, J. Geophys. Res., 105, 4927–4935, 2000.
Krzyscin, J. W., Jaroslawski, J., and Sobolewski, P. S.: Effects of clouds on the surface erythemal UV-B irradiance at northern midlatitudes: Estimation from the observations taken at Belsk, Poland (1999–2001), J. Atmos. Sol.-Terr. Phy., 65, 457–467, 2003.
Kuchinke, C. and Nunez, M.: Cloud transmission estimates of UV-B erythemal irradiance, Theor. Appl. Climatol., 63, 149–161, 1999.
Kylling, A., Bais, A. F., Blumthaler, M., Schreder, J., Zerefos, C. S., and Kosmidis, E.: Effect of aerosols on solar UV irradiances during the photochemical activity and solar ultraviolet radiation campaign, J. Geophys. Res., 103, 26051–26060, 1998.
Kylling, A., Webb, A. R., Kift, R., Gobbi, G. P., Ammannato, L., Barnaba, F., Bais, A., Kazadzis, S., Wendisch, M., Jäkel, E., Schmidt, S., Kniffka, A., Thiel, S., Junkermann, W., Blumthaler, M., Silbernagl, R., Schallhart, B., Schmitt, R., Kjeldstad, B., Thorseth, T. M., Scheirer, R., and Mayer, B.: Spectral actinic flux in the lower troposphere: measurement and 1-D simulations for cloudless, broken cloud and overcast situations, Atmos. Chem. Phys., 5, 1975–1997, https://doi.org/10.5194/acp-5-1975-2005, 2005.
Leontyeva, E. and Stammes, K.: Estimations of cloud optical thickness from ground-based measurements of incoming solar radiation in the Artic, J. Climatol., 7, 566–578, 1994.
Levelt, P. F., Hilsenrath, E., Leppelmeier, G. W., Van den Oord, G. H. J., Bhartia, P. K., Tamminen, J., De Haan, J. F., and Veefkind, J. P.: The ozone monitoring instrument, IEEE T. Geosci. Remote, 44, 1093–1101, 2006.
Li, Z., Wang, P., and Cihlar, J.: A simple and efficient method for retrieving surface UV radiation dose rate from satellite, J. Geohys. Res., 105, 5027–5036, 2000.
Litynska, Z., Koepke, P., De Backer, H., Gröbner, J., Schmalwieser, A., and Vuilleumier, L.: Long term changes and climatology of UV radiation over Europe. Final scientific report COST Action 726, available at: http://www-med-physik.vu-wien.ac.at/uv/COST726/COST726_Dateien/Results_Finalreport/COST726_fnal_report.pdf, 2010.
López, M. L., Palancar, G. G., and Toselli, B. M.: Effect of different types of clouds on surface UV-B and total solar irradiance at southern mid-latitudes: CMF determinations at Córdoba, Argentina, Atmos. Environ., 43, 3130–3136, 2009.
Lubin, D. and Frederick, J. E.: The ultraviolet radiation environment of the Antarctic Peninsula: The roles of ozone and cloud cover, J. Appl. Meteorol., 30, 478–493, 1991.
Lyamani, H., Olmo, F. J., and Alados-Arboledas, L.: Physical and optical properties of aerosols over an urban location in Spain: seasonal and diurnal variability, Atmos. Chem. Phys., 10, 239-254, https://doi.org/10.5194/acp-10-239-2010, 2010.
Madronich, S.: Analytic formula for the clear-sky UV index, Photochem. Photobiol., 83, 1537–1538, https://doi.org/10.1111/j.1751-1097.2010.00860.x, 2007.
Marshak, A., Knyazikhin, Y., Evans, K. D., and Wiscombe, W. J.: The "RED versus NIR" plane to retrieve broken-cloud optical depth from ground-based measurements, J. Atmos. Sci., 61, 1911–1925, 2004.
McKinlay, A. F. and Diffey, B. L.: A reference spectrum for ultraviolet induced erythema in human skin, CIE J., 6, 21–27, 1987.
Mayer, B. and Kylling, A.: Technical note: The libRadtran software package for radiative transfer calculations – description and examples of use, Atmos. Chem. Phys., 5, 1855–1877, https://doi.org/10.5194/acp-5-1855-2005, 2005.
Mayer, B., Seckmeyer, G., and Kylling, A.: Systematic long-term comparison of spectral UV measurements and UVSPEC modelling results, J. Geophys. Res., 102, 8755–8767, 1997.
Mayer, B., Kylling, A., Madronich, S., and Seckmeyer, G.: Enhanced absorption of UV radiation due to multiple scattering in clouds, Experimental evidence and theoretical explanation, J. Geophys. Res., 103, 31241–31254, 1998.
Mateos, D., de Miguel, A., Bilbao, J., and Pérez-Burgos, A.: Dependence of ultraviolet (erythemal and total) radiation and CMF values on total and low cloud covers in Central Spain, Atmos. Res., 98, 21–27, 2010.
Mateos, D., di Sarra, A., Meloni, D., Di Biagio, C., and Sferlazzo, D. M.: Experimental determination of cloud influence on the spectral UV irradiance and implications for biological effects, J. Atmos. Sol.-Terr. Phy., 73, 1739–1746, 2011.
Min, Q. and Harrison, L. C.: Cloud properties derived from surface MFRSR measurements and comparison with GOES results at the ARM SGP site, J. Geophys. Res., 23, 1641–1644, 1996.
Nichol, S. E., Pfister, G., Bodeker, G. E., Mckenzie, R. L., and Wood, S. W.: Moderation of cloud reduction of UV in the Antarctic due to high surface albedo, J. Appl. Meteorol., 42, 1174–1183, 2003.
Paltridge, G. W. and Barton, I. J.: Erythemal ultraviolet radiation distribution over Australia – The calculations, detailed results and input data, Tech. Pap. 33, 48 pp., Aust. Div. of Atmos. Phys., Commonw. Sci. and Indus. Res. Organ., Aspendale, Victoria, Australia, 1978.
Sabburg, J. and Calbó, J.: Five years of cloud enhanced surface UV radiation measurements at two sites (in the Northern and Southern Hemispheres), Atmos. Res., 93, 902–912, 2009.
Sabburg, J. and Wong, J.: Evaluation of sky/cloud formula for estimating UV-B irradiance under cloudy skies, J. Geophys. Res., 105, 29685–29691, 2000.
Schafer, J. S., Saxena, V. K., Wenny, B. N., Barnard, W., and DeLuisi, J. J.: Observed influences of clouds on ultraviolet-B radiation, Geophys. Res. Lett., 23, 2625–2628, 1996.
Schaaf, C. B., Gao, F., Strahler, A. H., Lucht, W., Li, X., Tsang, T., Strugnell, N. C., Zhang, X., Jin, Y., Muller, J. P., Lewis, P., Barnsley, M., Hobson, P., Disney, M., Roberts, G., Dunderdale, M., Doll, C., d'Entremont, R. P., Hug, B., Liang, S., Privette, J. L., and Roy, D.: First operational BRDF, albedo nadir reflectance products from MODIS, Remote Sens. Environ., 83, 135–148, 2002.
Schwander, H., Koepke, P., Kaifel, A., and Seckmeyer, G.: Modification of spectral UV irradiance by clouds, J. Geophys. Res., 107, 4296, https://doi.org/10.1029/2001JD001297, 2002.
Shettle, E. P.: Models of aerosols, clouds and precipitation for atmospheric propagation studies, in: AGARD Conference Proceedings No. 454, Atmospheric propagation in the uv, visible, ir and mm-region and related system aspects, Advisory Group for Aerospace Research and Development (AGARD), Brussels, Belgium, 1989.
Thiel, S., Steiner, K., and Seidlitz, H. K.: Modification of global erythemally effective irradiance by clouds, Photochem. Photobiol., 65, 969–973, 1997.
Trepte, S. and Winkler, P.: Reconstruction of erythemal UV irradiance and dose at Hohenpeissenberg (1968–2001) considering trends of total ozone, cloudiness and turbidity, Theor. Appl. Climatol., 77, 159–171, 2004.
Turner, D., Vogelmann, A. M., Austin, R. T., Barnard, J. C., Cady, K., Chiu, J. C., Clough, S. A., Flynn, C., Khaiyer, M. M., Lijegren, J., Johnson, K., Lin, B., Long, C., Marshak, A., Matrosov, S. Y., Mcfarlane, S. A., Miller, M., Min, Q., Minnis, P., O'Hirok, W., Wang, Z., and Wiscombe, W.,: Thin liquid water clouds: Their importance and our challenge, B. Am. Meteorol. Soc., 88, 177–190, 2007.
Vilaplana, J. M., Serrano, A., Antón, M., Cancillo, M. L., Parias, M., Gröbner, J., Hulsen, G., Zablocky, G., Díaz, A., and de la Morena, B.: Report of the El Arenosillo/INTA-COST calibration an intercomparison campaign of UVER broadband radiometers, in: "El Arenosillo", Huelva, Spain, August–September 2007, COST Office, ISBN:978-84-692-2640-7, p. 64, 2009.
Wang, P. and Lenoble, J.: Influence of clouds on UV irradiance at ground level and backscattered exittance, Adv. Atmos. Sci., 13, 217–228, 1996.
Webb, A. and Holick, M.: The role of sunlight in the cutaneous production of vitamin D3, Annu. Rev. Nutr., 8, 375–399, 1998.
World Meteorological Organization (WMO): Scientific assessment of ozone depletion: Global ozone research and monitoring project, Technical Report, 52, Geneva, Switzerland, 2010.