Articles | Volume 24, issue 14
https://doi.org/10.5194/acp-24-8489-2024
https://doi.org/10.5194/acp-24-8489-2024
Research article
 | 
29 Jul 2024
Research article |  | 29 Jul 2024

A model study investigating the sensitivity of aerosol forcing to the volatilities of semi-volatile organic compounds

Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola

Related authors

New particle formation dynamics in the central Andes: contrasting urban and mountaintop environments
Diego Aliaga, Victoria A. Sinclair, Radovan Krejci, Marcos Andrade, Paulo Artaxo, Luis Blacutt, Runlong Cai, Samara Carbone, Yvette Gramlich, Liine Heikkinen, Dominic Heslin-Rees, Wei Huang, Veli-Matti Kerminen, Alkuin Maximilian Koenig, Markku Kulmala, Paolo Laj, Valeria Mardoñez-Balderrama, Claudia Mohr, Isabel Moreno, Pauli Paasonen, Wiebke Scholz, Karine Sellegri, Laura Ticona, Gaëlle Uzu, Fernando Velarde, Alfred Wiedensohler, Doug Worsnop, Cheng Wu, Chen Xuemeng, Qiaozhi Zha, and Federico Bianchi
Aerosol Research, 3, 15–44, https://doi.org/10.5194/ar-3-15-2025,https://doi.org/10.5194/ar-3-15-2025, 2025
Short summary
Molecular and seasonal characteristics of organic vapors in urban Beijing: insights from Vocus-PTR measurements
Zhaojin An, Rujing Yin, Xinyan Zhao, Xiaoxiao Li, Yuyang Li, Yi Yuan, Junchen Guo, Yiqi Zhao, Xue Li, Dandan Li, Yaowei Li, Dongbin Wang, Chao Yan, Kebin He, Douglas R. Worsnop, Frank N. Keutsch, and Jingkun Jiang
Atmos. Chem. Phys., 24, 13793–13810, https://doi.org/10.5194/acp-24-13793-2024,https://doi.org/10.5194/acp-24-13793-2024, 2024
Short summary
An Algorithm for Automatic Fitting and Formula Assignment in Atmospheric Mass Spectra
Valter Mickwitz, Otso Peräkylä, Frans Graeffe, Douglas Worsnop, and Mikael Ehn
EGUsphere, https://doi.org/10.5194/egusphere-2024-3047,https://doi.org/10.5194/egusphere-2024-3047, 2024
Short summary
A comprehensive evaluation of enhanced temperature influence on gas and aerosol chemistry in the lamp-enclosed oxidation flow reactor (OFR) system
Tianle Pan, Andrew T. Lambe, Weiwei Hu, Yicong He, Minghao Hu, Huaishan Zhou, Xinming Wang, Qingqing Hu, Hui Chen, Yue Zhao, Yuanlong Huang, Doug R. Worsnop, Zhe Peng, Melissa A. Morris, Douglas A. Day, Pedro Campuzano-Jost, Jose-Luis Jimenez, and Shantanu H. Jathar
Atmos. Meas. Tech., 17, 4915–4939, https://doi.org/10.5194/amt-17-4915-2024,https://doi.org/10.5194/amt-17-4915-2024, 2024
Short summary
Measurement report: Impact of cloud processes on secondary organic aerosols at a forested mountain site in southeastern China
Zijun Zhang, Weiqi Xu, Yi Zhang, Wei Zhou, Xiangyu Xu, Aodong Du, Yinzhou Zhang, Hongqin Qiao, Ye Kuang, Xiaole Pan, Zifa Wang, Xueling Cheng, Lanzhong Liu, Qingyan Fu, Douglas R. Worsnop, Jie Li, and Yele Sun
Atmos. Chem. Phys., 24, 8473–8488, https://doi.org/10.5194/acp-24-8473-2024,https://doi.org/10.5194/acp-24-8473-2024, 2024
Short summary

Related subject area

Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Gaps in our understanding of ice-nucleating particle sources exposed by global simulation of the UK Earth System Model
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
Atmos. Chem. Phys., 25, 291–325, https://doi.org/10.5194/acp-25-291-2025,https://doi.org/10.5194/acp-25-291-2025, 2025
Short summary
The role of interfacial tension in the size-dependent phase separation of atmospheric aerosol particles
Ryan Schmedding and Andreas Zuend
Atmos. Chem. Phys., 25, 327–346, https://doi.org/10.5194/acp-25-327-2025,https://doi.org/10.5194/acp-25-327-2025, 2025
Short summary
Warming effects of reduced sulfur emissions from shipping
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 13681–13692, https://doi.org/10.5194/acp-24-13681-2024,https://doi.org/10.5194/acp-24-13681-2024, 2024
Short summary
The key role of atmospheric absorption in the Asian summer monsoon response to dust emissions in CMIP6 models
Alcide Zhao, Laura J. Wilcox, and Claire L. Ryder
Atmos. Chem. Phys., 24, 13385–13402, https://doi.org/10.5194/acp-24-13385-2024,https://doi.org/10.5194/acp-24-13385-2024, 2024
Short summary
Multi-model effective radiative forcing of the 2020 sulfur cap for shipping
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
Atmos. Chem. Phys., 24, 13361–13370, https://doi.org/10.5194/acp-24-13361-2024,https://doi.org/10.5194/acp-24-13361-2024, 2024
Short summary

Cited articles

Abdul-Razzak, H. and Ghan, S. J.: A parameterization of aerosol activation 3. Sectional representation, J. Geophys. Res.-Atmos., 107, 4026, https://doi.org/10.1029/2001JD000483, 2002. a
Andersson, C., Bergström, R., Bennet, C., Robertson, L., Thomas, M., Korhonen, H., Lehtinen, K. E. J., and Kokkola, H.: MATCH-SALSA – Multi-scale Atmospheric Transport and CHemistry model coupled to the SALSA aerosol microphysics model – Part 1: Model description and evaluation, Geosci. Model Dev., 8, 171–189, https://doi.org/10.5194/gmd-8-171-2015, 2015. a
Bergman, T., Kerminen, V.-M., Korhonen, H., Lehtinen, K. J., Makkonen, R., Arola, A., Mielonen, T., Romakkaniemi, S., Kulmala, M., and Kokkola, H.: Evaluation of the sectional aerosol microphysics module SALSA implementation in ECHAM5-HAM aerosol-climate model, Geosci. Model Dev., 5, 845–868, https://doi.org/10.5194/gmd-5-845-2012, 2012. a
Clarke, A. and Kapustin, V.: Hemispheric aerosol vertical profiles: Anthropogenic impacts on optical depth and cloud nuclei, Science, 329, 1488–1492, 2010. a
Collins, W. D., Ramaswamy, V., Schwarzkopf, M. D., Sun, Y., Portmann, R. W., Fu, Q., Casanova, S. E. B., Dufresne, J.-L., Fillmore, D. W., Forster, P. M. D., Galin, V. Y., Gohar, L. K., Ingram, W. J., Kratz, D. P., Lefebvre, M.-P., Li, J., Marquet, P., Oinas, V., Tsushima, Y., Uchiyama, T., and Zhong, W. Y: Radiative forcing by well-mixed greenhouse gases: Estimates from climate models in the Intergovernmental Panel on Climate Change (IPCC) Fourth Assessment Report (AR4), J. Geophys. Res.-Atmos., 111, D14317, https://doi.org/10.1029/2005JD006713, 2006. a
Download
Short summary
The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Altmetrics
Final-revised paper
Preprint