Articles | Volume 24, issue 20
https://doi.org/10.5194/acp-24-11849-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-11849-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
24 Oct 2024
Research article |
| 24 Oct 2024
| 24 Oct 2024
High ice water content in tropical mesoscale convective systems (a conceptual model)
Environment and Climate Change Canada, Toronto, ON, Canada
Zhipeng Qu
Environment and Climate Change Canada, Toronto, ON, Canada
Jason Milbrandt
Environment and Climate Change Canada, Toronto, ON, Canada
Ivan Heckman
Environment and Climate Change Canada, Toronto, ON, Canada
Mélissa Cholette
Environment and Climate Change Canada, Toronto, ON, Canada
Mengistu Wolde
National Research Council Canada, Ottawa, ON, Canada
Cuong Nguyen
National Research Council Canada, Ottawa, ON, Canada
Greg M. McFarquhar
Cooperative Institute for Severe and High Impact Weather Research and Operations and School of Meteorology, University of Oklahoma, Oklahoma City, OK, USA
Paul Lawson
Stratton Park Engineering Company, Boulder, CO, USA
Ann M. Fridlind
NASA Goddard Institute for Space Studies, New York, NY, USA
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Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
Atmos. Chem. Phys., 24, 7331–7345, https://doi.org/10.5194/acp-24-7331-2024, https://doi.org/10.5194/acp-24-7331-2024, 2024
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Michie Vianca De Vera, Larry Di Girolamo, Guangyu Zhao, Robert M. Rauber, Stephen W. Nesbitt, and Greg M. McFarquhar
Atmos. Chem. Phys., 24, 5603–5623, https://doi.org/10.5194/acp-24-5603-2024, https://doi.org/10.5194/acp-24-5603-2024, 2024
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Tropical oceanic low clouds remain a dominant source of uncertainty in cloud feedback in climate models due to their macrophysical properties (fraction, size, height, shape, distribution) being misrepresented. High-resolution satellite imagery over the Philippine oceans is used here to characterize cumulus macrophysical properties and their relationship to meteorological variables. Such information can act as a benchmark for cloud models and can improve low-cloud generation in climate models.
Lei Liu, Natalia Bliankinshtein, Yi Huang, John R. Gyakum, Philip M. Gabriel, Shiqi Xu, and Mengistu Wolde
Atmos. Meas. Tech., 17, 2219–2233, https://doi.org/10.5194/amt-17-2219-2024, https://doi.org/10.5194/amt-17-2219-2024, 2024
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Kamil Mroz, Alessandro Battaglia, and Ann M. Fridlind
Atmos. Meas. Tech., 17, 1577–1597, https://doi.org/10.5194/amt-17-1577-2024, https://doi.org/10.5194/amt-17-1577-2024, 2024
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Shannon L. Mason, Howard W. Barker, Jason N. S. Cole, Nicole Docter, David P. Donovan, Robin J. Hogan, Anja Hünerbein, Pavlos Kollias, Bernat Puigdomènech Treserras, Zhipeng Qu, Ulla Wandinger, and Gerd-Jan van Zadelhoff
Atmos. Meas. Tech., 17, 875–898, https://doi.org/10.5194/amt-17-875-2024, https://doi.org/10.5194/amt-17-875-2024, 2024
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Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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Zhipeng Qu, David P. Donovan, Howard W. Barker, Jason N. S. Cole, Mark W. Shephard, and Vincent Huijnen
Atmos. Meas. Tech., 16, 4927–4946, https://doi.org/10.5194/amt-16-4927-2023, https://doi.org/10.5194/amt-16-4927-2023, 2023
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The EarthCARE satellite mission Level 2 algorithm development requires realistic 3D cloud and aerosol scenes along the satellite orbits. One of the best ways to produce these scenes is to use a high-resolution numerical weather prediction model to simulate atmospheric conditions at 250 m horizontal resolution. This paper describes the production and validation of three EarthCARE test scenes.
Jason N. S. Cole, Howard W. Barker, Zhipeng Qu, Najda Villefranque, and Mark W. Shephard
Atmos. Meas. Tech., 16, 4271–4288, https://doi.org/10.5194/amt-16-4271-2023, https://doi.org/10.5194/amt-16-4271-2023, 2023
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Measurements from the EarthCARE satellite mission will be used to retrieve profiles of cloud and aerosol properties. These retrievals are combined with auxiliary information about surface properties and atmospheric state, e.g., temperature and water vapor. This information allows computation of 1D and 3D solar and thermal radiative transfer for small domains, which are compared with coincident radiometer observations to continually assess EarthCARE retrievals.
Qian Xiao, Jiaoshi Zhang, Yang Wang, Luke D. Ziemba, Ewan Crosbie, Edward L. Winstead, Claire E. Robinson, Joshua P. DiGangi, Glenn S. Diskin, Jeffrey S. Reid, K. Sebastian Schmidt, Armin Sorooshian, Miguel Ricardo A. Hilario, Sarah Woods, Paul Lawson, Snorre A. Stamnes, and Jian Wang
Atmos. Chem. Phys., 23, 9853–9871, https://doi.org/10.5194/acp-23-9853-2023, https://doi.org/10.5194/acp-23-9853-2023, 2023
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Using recent airborne measurements, we show that the influences of anthropogenic emissions, transport, convective clouds, and meteorology lead to new particle formation (NPF) under a variety of conditions and at different altitudes in tropical marine environments. NPF is enhanced by fresh urban emissions in convective outflow but is suppressed in air masses influenced by aged urban emissions where reactive precursors are mostly consumed while particle surface area remains relatively high.
McKenna W. Stanford, Ann M. Fridlind, Israel Silber, Andrew S. Ackerman, Greg Cesana, Johannes Mülmenstädt, Alain Protat, Simon Alexander, and Adrian McDonald
Atmos. Chem. Phys., 23, 9037–9069, https://doi.org/10.5194/acp-23-9037-2023, https://doi.org/10.5194/acp-23-9037-2023, 2023
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Clouds play an important role in the Earth’s climate system as they modulate the amount of radiation that either reaches the surface or is reflected back to space. This study demonstrates an approach to robustly evaluate surface-based observations against a large-scale model. We find that the large-scale model precipitates too infrequently relative to observations, contrary to literature documentation suggesting otherwise based on satellite measurements.
Rose Marie Miller, Robert M. Rauber, Larry Di Girolamo, Matthew Rilloraza, Dongwei Fu, Greg M. McFarquhar, Stephen W. Nesbitt, Luke D. Ziemba, Sarah Woods, and Kenneth Lee Thornhill
Atmos. Chem. Phys., 23, 8959–8977, https://doi.org/10.5194/acp-23-8959-2023, https://doi.org/10.5194/acp-23-8959-2023, 2023
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The influence of human-produced aerosols on clouds remains one of the uncertainties in radiative forcing of Earth’s climate. Measurements of aerosol chemistry from sources around the Philippines illustrate the linkage between aerosol chemical composition and cloud droplet characteristics. Differences in aerosol chemical composition in the marine layer from biomass burning, industrial, ship-produced, and marine aerosols are shown to impact cloud microphysical structure just above cloud base.
Zhipeng Qu, Howard W. Barker, Jason N. S. Cole, and Mark W. Shephard
Atmos. Meas. Tech., 16, 2319–2331, https://doi.org/10.5194/amt-16-2319-2023, https://doi.org/10.5194/amt-16-2319-2023, 2023
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This paper describes EarthCARE’s L2 product ACM-3D. It includes the scene construction algorithm (SCA) used to produce the indexes for reconstructing 3D atmospheric scene based on satellite nadir retrievals. It also provides the information about the buffer zone sizes of 3D assessment domains and the ranking scores for selecting the best 3D assessment domains. These output variables are needed to run 3D radiative transfer models for the radiative closure assessment of EarthCARE’s L2 retrievals.
Ruhi S. Humphries, Melita D. Keywood, Jason P. Ward, James Harnwell, Simon P. Alexander, Andrew R. Klekociuk, Keiichiro Hara, Ian M. McRobert, Alain Protat, Joel Alroe, Luke T. Cravigan, Branka Miljevic, Zoran D. Ristovski, Robyn Schofield, Stephen R. Wilson, Connor J. Flynn, Gourihar R. Kulkarni, Gerald G. Mace, Greg M. McFarquhar, Scott D. Chambers, Alastair G. Williams, and Alan D. Griffiths
Atmos. Chem. Phys., 23, 3749–3777, https://doi.org/10.5194/acp-23-3749-2023, https://doi.org/10.5194/acp-23-3749-2023, 2023
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Observations of aerosols in pristine regions are rare but are vital to constraining the natural baseline from which climate simulations are calculated. Here we present recent seasonal observations of aerosols from the Southern Ocean and contrast them with measurements from Antarctica, Australia and regionally relevant voyages. Strong seasonal cycles persist, but striking differences occur at different latitudes. This study highlights the need for more long-term observations in remote regions.
Sergey Y. Matrosov, Alexei Korolev, Mengistu Wolde, and Cuong Nguyen
Atmos. Meas. Tech., 15, 6373–6386, https://doi.org/10.5194/amt-15-6373-2022, https://doi.org/10.5194/amt-15-6373-2022, 2022
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A remote sensing method to retrieve sizes of particles in ice clouds and precipitation from radar measurements at two wavelengths is described. This method is based on relating the particle size information to the ratio of radar signals at these two wavelengths. It is demonstrated that this ratio is informative about different characteristic particle sizes. Knowing atmospheric ice particle sizes is important for many applications such as precipitation estimation and climate modeling.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Alexei Korolev, Paul J. DeMott, Ivan Heckman, Mengistu Wolde, Earle Williams, David J. Smalley, and Michael F. Donovan
Atmos. Chem. Phys., 22, 13103–13113, https://doi.org/10.5194/acp-22-13103-2022, https://doi.org/10.5194/acp-22-13103-2022, 2022
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The present study provides the first explicit in situ observation of secondary ice production at temperatures as low as −27 °C, which is well outside the range of the Hallett–Mossop process (−3 to −8 °C). This observation expands our knowledge of the temperature range of initiation of secondary ice in clouds. The obtained results are intended to stimulate laboratory and theoretical studies to develop physically based parameterizations for weather prediction and climate models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Ian Chang, Lan Gao, Feng Xu, and Jens Redemann
Atmos. Chem. Phys., 22, 12923–12943, https://doi.org/10.5194/acp-22-12923-2022, https://doi.org/10.5194/acp-22-12923-2022, 2022
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The ability of NASA’s Terra and Aqua satellites to retrieve cloud properties and estimate the changes in cloud properties due to aerosol–cloud interactions (ACI) was examined. There was good agreement between satellite retrievals and in situ measurements over the southeast Atlantic Ocean. This suggests that, combined with information on aerosol properties, satellite retrievals of cloud properties can be used to study ACI over larger domains and longer timescales in the absence of in situ data.
Frederic Tridon, Israel Silber, Alessandro Battaglia, Stefan Kneifel, Ann Fridlind, Petros Kalogeras, and Ranvir Dhillon
Atmos. Chem. Phys., 22, 12467–12491, https://doi.org/10.5194/acp-22-12467-2022, https://doi.org/10.5194/acp-22-12467-2022, 2022
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The role of ice precipitation in the Earth water budget is not well known because ice particles are complex, and their formation involves intricate processes. Riming of ice crystals by supercooled water droplets is an efficient process, but little is known about its importance at high latitudes. In this work, by exploiting the deployment of an unprecedented number of remote sensing systems in Antarctica, we find that riming occurs at much lower temperatures compared with the mid-latitudes.
Katherine L. Hayden, Shao-Meng Li, John Liggio, Michael J. Wheeler, Jeremy J. B. Wentzell, Amy Leithead, Peter Brickell, Richard L. Mittermeier, Zachary Oldham, Cristian M. Mihele, Ralf M. Staebler, Samar G. Moussa, Andrea Darlington, Mengistu Wolde, Daniel Thompson, Jack Chen, Debora Griffin, Ellen Eckert, Jenna C. Ditto, Megan He, and Drew R. Gentner
Atmos. Chem. Phys., 22, 12493–12523, https://doi.org/10.5194/acp-22-12493-2022, https://doi.org/10.5194/acp-22-12493-2022, 2022
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In this study, airborne measurements provided the most detailed characterization, to date, of boreal forest wildfire emissions. Measurements showed a large diversity of air pollutants expanding the volatility range typically reported. A large portion of organic species was unidentified, likely comprised of complex organic compounds. Aircraft-derived emissions improve wildfire chemical speciation and can support reliable model predictions of pollution from boreal forest wildfires.
Zhipeng Qu, Alexei Korolev, Jason A. Milbrandt, Ivan Heckman, Yongjie Huang, Greg M. McFarquhar, Hugh Morrison, Mengistu Wolde, and Cuong Nguyen
Atmos. Chem. Phys., 22, 12287–12310, https://doi.org/10.5194/acp-22-12287-2022, https://doi.org/10.5194/acp-22-12287-2022, 2022
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Secondary ice production (SIP) is an important physical phenomenon that results in an increase in the cloud ice particle concentration and can have a significant impact on the evolution of clouds. Here, idealized simulations of a tropical convective system were conducted. Agreement between the simulations and observations highlights the impacts of SIP on the maintenance of tropical convection in nature and the importance of including the modelling of SIP in numerical weather prediction models.
Michael S. Diamond, Pablo E. Saide, Paquita Zuidema, Andrew S. Ackerman, Sarah J. Doherty, Ann M. Fridlind, Hamish Gordon, Calvin Howes, Jan Kazil, Takanobu Yamaguchi, Jianhao Zhang, Graham Feingold, and Robert Wood
Atmos. Chem. Phys., 22, 12113–12151, https://doi.org/10.5194/acp-22-12113-2022, https://doi.org/10.5194/acp-22-12113-2022, 2022
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Smoke from southern Africa blankets the southeast Atlantic from June-October, overlying a major transition region between overcast and scattered clouds. The smoke affects Earth's radiation budget by absorbing sunlight and changing cloud properties. We investigate these effects in regional climate and large eddy simulation models based on international field campaigns. We find that large-scale circulation changes more strongly affect cloud transitions than smoke microphysical effects in our case.
Dongwei Fu, Larry Di Girolamo, Robert M. Rauber, Greg M. McFarquhar, Stephen W. Nesbitt, Jesse Loveridge, Yulan Hong, Bastiaan van Diedenhoven, Brian Cairns, Mikhail D. Alexandrov, Paul Lawson, Sarah Woods, Simone Tanelli, Sebastian Schmidt, Chris Hostetler, and Amy Jo Scarino
Atmos. Chem. Phys., 22, 8259–8285, https://doi.org/10.5194/acp-22-8259-2022, https://doi.org/10.5194/acp-22-8259-2022, 2022
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Satellite-retrieved cloud microphysics are widely used in climate research because of their central role in water and energy cycles. Here, we provide the first detailed investigation of retrieved cloud drop sizes from in situ and various satellite and airborne remote sensing techniques applied to real cumulus cloud fields. We conclude that the most widely used passive remote sensing method employed in climate research produces high biases of 6–8 µm (60 %–80 %) caused by 3-D radiative effects.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Rose M. Miller, and Jennifer D. Small Griswold
Atmos. Chem. Phys., 22, 2769–2793, https://doi.org/10.5194/acp-22-2769-2022, https://doi.org/10.5194/acp-22-2769-2022, 2022
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This study evaluates the impact of biomass burning aerosols on precipitation in marine stratocumulus clouds using observations from the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign over the Southeast Atlantic. Instances of contact and separation between aerosol and cloud layers show polluted clouds have a lower precipitation rate and a lower precipitation susceptibility. This information will help improve cloud representation in Earth system models.
Yongjie Huang, Wei Wu, Greg M. McFarquhar, Ming Xue, Hugh Morrison, Jason Milbrandt, Alexei V. Korolev, Yachao Hu, Zhipeng Qu, Mengistu Wolde, Cuong Nguyen, Alfons Schwarzenboeck, and Ivan Heckman
Atmos. Chem. Phys., 22, 2365–2384, https://doi.org/10.5194/acp-22-2365-2022, https://doi.org/10.5194/acp-22-2365-2022, 2022
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Numerous small ice crystals in tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. Previous numerical simulations failed to reproduce this phenomenon and hypothesized that key microphysical processes are still lacking in current models to realistically simulate the phenomenon. This study uses numerical experiments to confirm the dominant role of secondary ice production in the formation of these large numbers of small ice crystals.
Cuong M. Nguyen, Mengistu Wolde, Alessandro Battaglia, Leonid Nichman, Natalia Bliankinshtein, Samuel Haimov, Kenny Bala, and Dirk Schuettemeyer
Atmos. Meas. Tech., 15, 775–795, https://doi.org/10.5194/amt-15-775-2022, https://doi.org/10.5194/amt-15-775-2022, 2022
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An analysis of airborne triple-frequency radar and almost perfectly co-located coincident in situ data from an Arctic storm confirms the main findings of modeling work with radar dual-frequency ratios (DFRs) at different zones of the DFR plane associated with different ice habits. High-resolution CPI images provide accurate identification of rimed particles within the DFR plane. The relationships between the triple-frequency signals and cloud microphysical properties are also presented.
Israel Silber, Robert C. Jackson, Ann M. Fridlind, Andrew S. Ackerman, Scott Collis, Johannes Verlinde, and Jiachen Ding
Geosci. Model Dev., 15, 901–927, https://doi.org/10.5194/gmd-15-901-2022, https://doi.org/10.5194/gmd-15-901-2022, 2022
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The Earth Model Column Collaboratory (EMC2) is an open-source ground-based (and air- or space-borne) lidar and radar simulator and subcolumn generator designed for large-scale models, in particular climate models, applicable also for high-resolution models. EMC2 emulates measurements while remaining faithful to large-scale models' physical assumptions implemented in their cloud or radiation schemes. We demonstrate the use of EMC2 to compare AWARE measurements with the NASA GISS ModelE3 and LES.
Daniel Hernandez-Deckers, Toshihisa Matsui, and Ann M. Fridlind
Atmos. Chem. Phys., 22, 711–724, https://doi.org/10.5194/acp-22-711-2022, https://doi.org/10.5194/acp-22-711-2022, 2022
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We investigate how the concentration of aerosols (small particles that serve as seeds for cloud droplets) affect the dynamics of simulated clouds using two different frameworks, i.e., the traditional selection of cloudy rising grid points and tracking small-scale coherent rising features (cumulus thermals). By doing so, we find that these cumulus thermals reveal useful information about the coupling between internal cloud circulations and cloud droplet and raindrop formation.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Kamil Mroz, Alessandro Battaglia, Cuong Nguyen, Andrew Heymsfield, Alain Protat, and Mengistu Wolde
Atmos. Meas. Tech., 14, 7243–7254, https://doi.org/10.5194/amt-14-7243-2021, https://doi.org/10.5194/amt-14-7243-2021, 2021
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A method for estimating microphysical properties of ice clouds based on radar measurements is presented. The algorithm exploits the information provided by differences in the radar response at different frequency bands in relation to changes in the snow morphology. The inversion scheme is based on a statistical relation between the radar simulations and the properties of snow calculated from in-cloud sampling.
Rose M. Miller, Greg M. McFarquhar, Robert M. Rauber, Joseph R. O'Brien, Siddhant Gupta, Michal Segal-Rozenhaimer, Amie N. Dobracki, Arthur J. Sedlacek, Sharon P. Burton, Steven G. Howell, Steffen Freitag, and Caroline Dang
Atmos. Chem. Phys., 21, 14815–14831, https://doi.org/10.5194/acp-21-14815-2021, https://doi.org/10.5194/acp-21-14815-2021, 2021
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A large stratocumulus cloud deck resides off the west coast of central Africa. Biomass burning in Africa produces a large plume of aerosol that is carried by the wind over this stratocumulus cloud deck. This paper shows that particles with sizes from 0.01 to 1 mm reside within this plume. Past studies have shown that biomass burning produces such particles, but this is the first study to show that they can be transported westward, over long distances, to the Atlantic stratocumulus cloud deck.
Haoran Li, Alexei Korolev, and Dmitri Moisseev
Atmos. Chem. Phys., 21, 13593–13608, https://doi.org/10.5194/acp-21-13593-2021, https://doi.org/10.5194/acp-21-13593-2021, 2021
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Kelvin–Helmholtz (K–H) clouds embedded in a stratiform precipitation event were uncovered via radar Doppler spectral analysis. Given the unprecedented detail of the observations, we show that multiple populations of secondary ice columns were generated in the pockets where larger cloud droplets are formed and not at some constant level within the cloud. Our results highlight that the K–H instability is favorable for liquid droplet growth and secondary ice formation.
Ruhi S. Humphries, Melita D. Keywood, Sean Gribben, Ian M. McRobert, Jason P. Ward, Paul Selleck, Sally Taylor, James Harnwell, Connor Flynn, Gourihar R. Kulkarni, Gerald G. Mace, Alain Protat, Simon P. Alexander, and Greg McFarquhar
Atmos. Chem. Phys., 21, 12757–12782, https://doi.org/10.5194/acp-21-12757-2021, https://doi.org/10.5194/acp-21-12757-2021, 2021
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The Southern Ocean region is one of the most pristine in the world and serves as an important proxy for the pre-industrial atmosphere. Improving our understanding of the natural processes in this region is likely to result in the largest reductions in the uncertainty of climate and earth system models. In this paper we present a statistical summary of the latitudinal gradient of aerosol and cloud condensation nuclei concentrations obtained from five voyages spanning the Southern Ocean.
Youssef Wehbe, Sarah A. Tessendorf, Courtney Weeks, Roelof Bruintjes, Lulin Xue, Roy Rasmussen, Paul Lawson, Sarah Woods, and Marouane Temimi
Atmos. Chem. Phys., 21, 12543–12560, https://doi.org/10.5194/acp-21-12543-2021, https://doi.org/10.5194/acp-21-12543-2021, 2021
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The role of dust aerosols as ice-nucleating particles is well established in the literature, whereas their role as cloud condensation nuclei is less understood, particularly in polluted desert environments. We analyze coincident aerosol size distributions and cloud particle imagery collected over the UAE with a research aircraft. Despite the presence of ultra-giant aerosol sizes associated with dust, an active collision–coalescence process is not observed within the limited depths of warm cloud.
Jing Feng, Yi Huang, and Zhipeng Qu
Atmos. Meas. Tech., 14, 5717–5734, https://doi.org/10.5194/amt-14-5717-2021, https://doi.org/10.5194/amt-14-5717-2021, 2021
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It is challenging to measure the atmospheric conditions above convective storms. In this study, a method of retrieving thermodynamic variables above convective storms using a combination of satellite-based observations from a hyperspectral infrared sounder and active sensors is developed. We find that this method captures the spatial distributions of thermodynamic anomalies above convective clouds well. This method is potentially applicable to observations from current and future satellites.
Florian Tornow, Andrew S. Ackerman, and Ann M. Fridlind
Atmos. Chem. Phys., 21, 12049–12067, https://doi.org/10.5194/acp-21-12049-2021, https://doi.org/10.5194/acp-21-12049-2021, 2021
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Cold air outbreaks affect the local energy budget by forming bright boundary layer clouds that, once it rains, evolve into dimmer, broken cloud fields that are depleted of condensation nuclei – an evolution consistent with closed-to-open cell transitions. We find that cloud ice accelerates this evolution, primarily via riming prior to rain onset, which (1) reduces liquid water, (2) reduces condensation nuclei, and (3) leads to early precipitation cooling and moistening below cloud.
Konstantin Baibakov, Samuel LeBlanc, Keyvan Ranjbar, Norman T. O'Neill, Mengistu Wolde, Jens Redemann, Kristina Pistone, Shao-Meng Li, John Liggio, Katherine Hayden, Tak W. Chan, Michael J. Wheeler, Leonid Nichman, Connor Flynn, and Roy Johnson
Atmos. Chem. Phys., 21, 10671–10687, https://doi.org/10.5194/acp-21-10671-2021, https://doi.org/10.5194/acp-21-10671-2021, 2021
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We find that the airborne measurements of the vertical extinction due to aerosols (aerosol optical depth, AOD) obtained in the Athabasca Oil Sands Region (AOSR) can significantly exceed ground-based values. This can have an effect on estimating the AOSR radiative impact and is relevant to satellite validation based on ground-based measurements. We also show that the AOD can marginally increase as the plumes are being transported away from the source and the new particles are being formed.
Katherine Hayden, Shao-Meng Li, Paul Makar, John Liggio, Samar G. Moussa, Ayodeji Akingunola, Robert McLaren, Ralf M. Staebler, Andrea Darlington, Jason O'Brien, Junhua Zhang, Mengistu Wolde, and Leiming Zhang
Atmos. Chem. Phys., 21, 8377–8392, https://doi.org/10.5194/acp-21-8377-2021, https://doi.org/10.5194/acp-21-8377-2021, 2021
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We developed a method using aircraft measurements to determine lifetimes with respect to dry deposition for oxidized sulfur and nitrogen compounds over the boreal forest in Alberta, Canada. Atmospheric lifetimes were significantly shorter than derived from chemical transport models with differences related to modelled dry deposition velocities. The shorter lifetimes suggest models need to reassess dry deposition treatment and predictions of sulfur and nitrogen in the atmosphere and ecosystems.
Yongjie Huang, Wei Wu, Greg M. McFarquhar, Xuguang Wang, Hugh Morrison, Alexander Ryzhkov, Yachao Hu, Mengistu Wolde, Cuong Nguyen, Alfons Schwarzenboeck, Jason Milbrandt, Alexei V. Korolev, and Ivan Heckman
Atmos. Chem. Phys., 21, 6919–6944, https://doi.org/10.5194/acp-21-6919-2021, https://doi.org/10.5194/acp-21-6919-2021, 2021
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Numerous small ice crystals in the tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. This study evaluated the numerical models against the airborne observations and investigated the potential cloud processes that could lead to the production of these large numbers of small ice crystals. It is found that key microphysical processes are still lacking or misrepresented in current numerical models to realistically simulate the phenomenon.
Andrew M. Dzambo, Tristan L'Ecuyer, Kenneth Sinclair, Bastiaan van Diedenhoven, Siddhant Gupta, Greg McFarquhar, Joseph R. O'Brien, Brian Cairns, Andrzej P. Wasilewski, and Mikhail Alexandrov
Atmos. Chem. Phys., 21, 5513–5532, https://doi.org/10.5194/acp-21-5513-2021, https://doi.org/10.5194/acp-21-5513-2021, 2021
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This work highlights a new algorithm using data collected from the 2016–2018 NASA ORACLES field campaign. This algorithm synthesizes cloud and rain measurements to attain estimates of cloud and precipitation properties over the southeast Atlantic Ocean. Estimates produced by this algorithm compare well against in situ estimates. Increased rain fractions and rain rates are found in regions of atmospheric instability. This dataset can be used to explore aerosol–cloud–precipitation interactions.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, David J. Delene, Michael R. Poellot, Amie Dobracki, James R. Podolske, Jens Redemann, Samuel E. LeBlanc, Michal Segal-Rozenhaimer, and Kristina Pistone
Atmos. Chem. Phys., 21, 4615–4635, https://doi.org/10.5194/acp-21-4615-2021, https://doi.org/10.5194/acp-21-4615-2021, 2021
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Observations from the 2016 NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign examine how biomass burning aerosols from southern Africa affect marine stratocumulus cloud decks over the Southeast Atlantic. Instances of contact and separation between aerosols and clouds are examined to quantify the impact of aerosol mixing into cloud top on cloud drop numbers and sizes. This information is needed for improving Earth system models and satellite retrievals.
Israel Silber, Ann M. Fridlind, Johannes Verlinde, Andrew S. Ackerman, Grégory V. Cesana, and Daniel A. Knopf
Atmos. Chem. Phys., 21, 3949–3971, https://doi.org/10.5194/acp-21-3949-2021, https://doi.org/10.5194/acp-21-3949-2021, 2021
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Long-term ground-based radar and sounding measurements over Alaska (Antarctica) indicate that more than 85 % (75 %) of supercooled clouds are precipitating at cloud base and that 75 % (50 %) are precipitating to the surface. Such high prevalence is reconciled with lesser spaceborne estimates by considering radar sensitivity. Results provide a strong observational constraint for polar cloud processes in large-scale models.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Martina Krämer, Christian Rolf, Nicole Spelten, Armin Afchine, David Fahey, Eric Jensen, Sergey Khaykin, Thomas Kuhn, Paul Lawson, Alexey Lykov, Laura L. Pan, Martin Riese, Andrew Rollins, Fred Stroh, Troy Thornberry, Veronika Wolf, Sarah Woods, Peter Spichtinger, Johannes Quaas, and Odran Sourdeval
Atmos. Chem. Phys., 20, 12569–12608, https://doi.org/10.5194/acp-20-12569-2020, https://doi.org/10.5194/acp-20-12569-2020, 2020
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To improve the representations of cirrus clouds in climate predictions, extended knowledge of their properties and geographical distribution is required. This study presents extensive airborne in situ and satellite remote sensing climatologies of cirrus and humidity, which serve as a guide to cirrus clouds. Further, exemplary radiative characteristics of cirrus types and also in situ observations of tropical tropopause layer cirrus and humidity in the Asian monsoon anticyclone are shown.
Alexei Korolev and Thomas Leisner
Atmos. Chem. Phys., 20, 11767–11797, https://doi.org/10.5194/acp-20-11767-2020, https://doi.org/10.5194/acp-20-11767-2020, 2020
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Secondary ice production (SIP) plays a key role in the formation of ice particles in tropospheric clouds. This work presents a critical review of the laboratory studies related to secondary ice production. It aims to identify gaps in our knowledge of SIP as well as to stimulate further laboratory studies focused on obtaining a quantitative description of efficiencies for each SIP mechanism.
Cited articles
Ackerman, A. S., Fridlind, A. M., Grandin, A., Dezitter, F., Weber, M., Strapp, J. W., and Korolev, A. V.: High ice water content at low radar reflectivity near deep convection – Part 2: Evaluation of microphysical pathways in updraft parcel simulations, Atmos. Chem. Phys., 15, 11729–11751, https://doi.org/10.5194/acp-15-11729-2015, 2015.
aufm Kampe, H. J., Weickmann, H. K., and Kelly, J. J.: The influence of temperature on the shape of ice crystals growing at water saturation, J. Atmos. Sci., 8, 168–174, https://doi.org/10.1175/1520-0469(1951)008<0168:TIOTOT>2.0.CO;2, 1951.
Bailey, M. and J. Hallett, H.: A comprehensive habit diagram for atmospheric ice crystals: Confirmation from the laboratory, AIRS II, and other field studies, J. Atmos. Sci., 66, 2888–2899, https://doi.org/10.1175/2009JAS2883.1, 2009.
Baumgardner, D., Jonsson, H. H., Dawson, W., O'Connor, D. P., and Newton, R.: The Cloud, Aerosol and Precipitation Spectrometer: A New Instrument for Cloud Investigations, Atmos. Res., 59–60, 251–264, https://doi.org/10.1016/S0169-8095(01)00119-3, 2001.
Baumgardner, D., Abel, S. J., Axisa, D., Cotton, R., Crosier, J., Field, P., Gurganus, C., Heymsfield, A., Korolev, A., Krämer, M., Lawson, P., McFarquhar, G., Ulanowski, Z., and Um, J.: Cloud Ice Properties: In Situ Measurement Challenges, Meteor. Mon., 58, 9.1–9.23, https://doi.org/10.1175/AMSMONOGRAPHS-D-16-0011.1, 2017.
Belair, S., Leroyer, S., Seino, N., Spacek, L., Souvanlassy, V., and Paquin, D.: Role and Impact of the urban environment in a numerical forecast of an intense summertime precipitation event over Tokyo, J. Meteor. Soc. Jpn., 96A, 77–94, https://doi.org/10.2151/jmsj.2018-011, 2018.
Beswick, K. M., Gallagher, M. W., Webb, A. R., Norton, E. G., and Perry, F.: Application of the Aventech AIMMS20AQ airborne probe for turbulence measurements during the Convective Storm Initiation Project, Atmos. Chem. Phys., 8, 5449–5463, https://doi.org/10.5194/acp-8-5449-2008, 2008.
Brechner, P., McFarquhar, G. M., Schwarzenboeck, A., Korolev, A. V.: Ice Crystal Size Distributions in Tropical Mesoscale Convective Systems in the Vicinity of Darwin, Australia: Results from the HAIC/HIWC Campaign, J. Atmos. Sci., 80, 2147–2164, https://doi.org/10.1175/JAS-D-22-0209.1, 2023.
Brown, P. R. A. and Francis, P. N.: Improved measurements of the ice water content in cirrus using a total-water probe, J. Atmos. Ocean. Tech., 12, 410–414, https://doi.org/10.1175/1520-0426(1995)012%3C0410:IMOTIW%3E2.0.CO;2, 1995.
Cai, Y., Montague, D. C., Mooiweer-Bryan, W., and Deshler, T.: Performance characteristics of the ultra high sensitivity aerosol spectrometer for particles between 55 and 800 nm: Laboratory and field studies, J. Aerosol Sci., 39, 759–769, https://doi.org/10.1016/j.jaerosci.2008.04.007, 2008.
Cholette, M., Milbrandt, J. A., Morrison, H., Paquin-Ricard, D., Jaques, D.: Combining triple-moment ice with prognostic liquid fraction in the P3 microphysics scheme: Impacts on a simulated squall line, J. Adv. Model. Earth Sy., 15, e2022MS003328, https://doi.org/10.1029/2022MS003328, 2023.
Connolly, P. J., Flynn, M. J., Ulanowski, Z., Choularton, T. W., Gallagher, M. W., and Bower, K. N.: Calibration of the cloud particle imager probes using calibration beads and ice crystal analogs: The depth of field, J. Atmos. Ocean. Tech., 24, 1860–1879, https://doi.org/10.1175/JTECH2096.1, 2007.
Côté, J., Gravel, S., Méthot, A., Patoine, A., Roch, M., and Staniforth, A.: The operational CMC–MRD global environmental multiscale (GEM) model. Part I: Design considerations and formulation, Mon. Weather Rev., 126, 1373–1395, https://doi.org/10.1175/1520-0493(1998)126,1373:TOCMGE.2.0.CO;2, 1998.
Davison, C., Ratvasky, T., and Lyle, L.: Naturally Aspirating Isokinetic Total Water Content Probe: Wind Tunnel Test Results and Design Modifications, in: SAE 2011 International Conference on Aircraft and Engine Icing and Ground Deicing, Chicago, Illinois, 13–17 June 2011, https://doi.org/10.4271/2011-38-0036, 2011.
Dezitter, F., Grandin, A., Brenguier, J.-L., Hervy, F. Hans Schlager, H., Villedieu, P., and, G.: HAIC—High Altitude Ice Cry–27 June 2013, San Diego, CA, American Institute of Aeronautics and Astronautics, http://arc.aiaa.org/doi/abs/10.2514/6.2013-2674 (last access: 20 October 2024), 2013.
Environment and Climate Change Canada: The Global Environmental Multiscale Model (GEM) (version 5.1.0-rc3), GitHub [code], https://github.com/ECCC-ASTD-MRD/gem/tree/5.1.0-rc3 (last access: 20 October 2024), 2020.
Environment and Climate Change Canada and National Center for Atmospheric Research: The Predicted Particle Properties (P3) bulk microphysics scheme, GitHub [code], https://github.com/P3-microphysics/P3-microphysics (last access: 20 October 2024), 2023.
Field, P. R., Lawson, P., Brown, P., Lloyd, G., Westbrook, C., Moisseev, D., Miltenberger, A., Nenes, A., Blyth, A., Choularton, T., Connolly, P., Bühl, J., Crosier, J., Cui, Z., Dearden, C., DeMott, P., Flossmann, A. I., Heymsfield, A. J., Huang, Y., and Sullivan, S.: Secondary Ice Production: Current State of the Science and Recommendations for the Future, Meteor. Mon., 58, 7.1–7.20, https://doi.org/10.1175/AMSMONOGRAPHS-D-16-0014.1, 2017.
Franklin, C. N., Protat, A., Leroy, D., and Fontaine, E.: Controls on phase composition and ice water content in a convection-permitting model simulation of a tropical mesoscale convective system, Atmos. Chem. Phys., 16, 8767–8789, https://doi.org/10.5194/acp-16-8767-2016, 2016.
Fridlind, A. M., Ackerman, A. S., Grandin, A., Dezitter, F., Weber, M., Strapp, J. W., Korolev, A. V., and Williams, C. R.: High ice water content at low radar reflectivity near deep convection – Part 1: Consistency of in situ and remote-sensing observations with stratiform rain column simulations, Atmos. Chem. Phys., 15, 11713–11728, https://doi.org/10.5194/acp-15-11713-2015, 2015.
Girard, C., Plante A., Desgagné, M., McTaggart-Cowan, R., Côté J., Charron, M., Gravel, S., Lee, V., Patoine, A., Qaddouri, A., Roch, M., Spacek, L., Tanguay, M., and Vaillancourt, P. A.: Staggered vertical discretization of the Canadian environmental multiscale (GEM) model using a coordinate of the loghydrostatic-pressure type, Mon. Weather Rev., 142, 1183–1196, https://doi.org/10.1175/MWR-D-13-00255.1, 2014.
Grzych, M. L. and Mason, J. G.: Weather conditions associated with jet engine power loss and damage due to ingestion of ice particles: What we've learned through 2009, 14th Conf. on Aviation, Range, and Aerospace Meteorology, 18–21 January 2010, Atlanta, GA, 6.8, Amer. Meteor. Soc., https://ams.confex.com/ams/pdfpapers/165923.pdf (last access: 20 October 2024), 2010.
Hallett, J. and Mason, B. J.: The influence of temperature and supersaturation on the habit of ice crystals grown from the vapour, P. Roy. Soc. A, 247, 440–453, https://doi.org/10.1098/rspa.1958.0199, 1958.
Heymsfield, A. J., Bansemer, A. Field, P. R., Durden, S. L., Stith, J. L., Dye, J. E., Hall, W., and Grainger, C. A.: Observations and Parameterizations of Particle Size Distributions in Deep Tropical Cirrus and Stratiform Precipitating Clouds: Results from In Situ Observations in TRMM Field Campaigns, J. Atmos. Sci., 59, 3457–3491, https://doi.org/10.1175/1520-0469(2002)059%3C0003:AGAFDT%3E2.0.CO;2 2002.
Heymsfield, A. J., Bansemer, A., and Twohy, C. H.: Refinements to ice particle mass dimensional and terminal velocity relationships for ice clouds. Part I: Temperature dependence, J. Atmos. Sci., 64, 1047–1067, https://doi.org/10.1175/JAS3890.1, 2007.
Hu, Y., McFarquhar, G. M., Wu, W., Huang, Y., Schwarzenboeck, A., Protat, A., Korolev, A., Rauber, R. M., and Wang, H.: Dependence of Ice Microphysical Properties On Environmental Parameters: Results from HAIC-HIWC Cayenne Field Campaign, J. Atmos. Sci., 78, 2957–2981, https://doi.org/10.1175/JAS-D-21-0015.1, 2021.
Hu, Y., McFarquhar, G. M., Brechner, P., Wu, W., Huang, Y., Korolev, A., Protat, A., Nguyen, C., Wolde, M., Schwarzenboeck, A., Rauber, R. M., Wang, H.: Dependence of Ice Crystal Size Distributions in High Ice Water Content Conditions on Environmental Conditions: Results from the HAIC-HIWC Cayenne Campaign, J. Atmos. Sci., 80, 3103–3134, https://doi.org/10.1175/JAS-D-22-0008.1, 2022.
Huang, Y., Wu, W., McFarquhar, G. M., Wang, X., Morrison, H., Ryzhkov, A., Hu, Y., Wolde, M., Nguyen, C., Schwarzenboeck, A., Milbrandt, J., Korolev, A. V., and Heckman, I.: Microphysical processes producing high ice water contents (HIWCs) in tropical convective clouds during the HAIC-HIWC field campaign: evaluation of simulations using bulk microphysical schemes, Atmos. Chem. Phys., 21, 6919–6944, https://doi.org/10.5194/acp-21-6919-2021, 2021.
Huang, Y., Wu, W., McFarquhar, G. M., Xue, M., Morrison, H., Milbrandt, J., Korolev, A. V., Hu, Y., Qu, Z., Wolde, M., Nguyen, C., Schwarzenboeck, A., and Heckman, I.: Microphysical processes producing high ice water contents (HIWCs) in tropical convective clouds during the HAIC-HIWC field campaign: dominant role of secondary ice production, Atmos. Chem. Phys., 22, 2365–2384, https://doi.org/10.5194/acp-22-2365-2022, 2022.
James, R. L., Phillips, V. T. J., and Connolly, P. J.: Secondary ice production during the break-up of freezing water drops on impact with ice particles, Atmos. Chem. Phys., 21, 18519–18530, https://doi.org/10.5194/acp-21-18519-2021, 2021.
Keinert, A., Spannagel, D., Leisner, T., and Kiselev, A.: Secondary ice production upon freezing of freely falling drizzle droplets, J. Atmos. Sci., 77, 2959–2967, https://doi.org/10.1175/JAS-D-20-0081.1, 2020.
Knollenberg, R. G.: Techniques for probing cloud microstructure, in: Clouds their Formation, Optical Properties, and Effects, edited by: Hobbs, P. V. and Deepak, A., Academic Press, New York, 15–91, ISBN 0-12-350720-0, 1981.
Kobayashi, T.: Experimental researches on the snow crystal habit and growth by means of a diffusion cloud chamber, J. Meteor. Soc. Jpn., 35A, 38–47, https://doi.org/10.2151/jmsj1923.35A.0_38, 1957.
Kobayashi, T.: The growth of snow crystals at low supersaturation, Philos. Mag., 5, 1363–1370, https://doi.org/10.1080/14786436108241231, 1961.
Korolev, A. and Field, P. R.: Assessment of the performance of the inter-arrival time algorithm to identify ice shattering artifacts in cloud particle probe measurements, Atmos. Meas. Tech., 8, 761–777, https://doi.org/10.5194/amt-8-761-2015, 2015.
Korolev, A. and Heckman, I.: Cayenne NRC Convair 1D Data. Version 1.0. UCAR/NCAR – Earth Observing Laboratory [data set], https://doi.org/10.26023/PSC2-TTQS-390A, 2017.
Korolev, A. and Leisner, T.: Review of experimental studies of secondary ice production, Atmos. Chem. Phys., 20, 11767–11797, https://doi.org/10.5194/acp-20-11767-2020, 2020.
Korolev, A., Emery, E., and Creelman, K.: Modification and tests of particle probe tips to mitigate effects of ice shattering, J. Atmos. Ocean. Tech., 30, 690–708, https://doi.org/10.1175/JTECH-D-12-00142.1, 2013a.
Korolev, A., Emery, E., Strapp, J., Cober, S., and Isaac, G.: Quantification of the effects of shattering on airborne ice particle measurements, J. Atmos. Ocean. Tech., 30, 2527–2553, https://doi.org/10.1175/JTECH-D-13-00115.1, 2013b.
Korolev, A., Shashkov, A., and Barker, H.: Calibrations and Performance of the Airborne Cloud Extinction Probe, J. Atmos. Ocean. Tech., 31, 326–345, https://doi.org/10.1175/JTECH-D-13-00020.1, 2014.
Korolev, A., McFarquhar, G., Field, P. R., Franklin, C., Lawson, P., Wang, Z., Williams, E., Abel, S. J., Axisa, D., Borrmann, S., Crosier, J., Fugal, J., Krämer, M., Lohmann, U., Schlenczek, O., Schnaiter, M., and Wendisch, M.: Mixed-Phase Clouds: Progress and Challenges, Meteor. Mon., 58, 5.1–5.50, https://doi.org/10.1175/AMSMONOGRAPHS-D-17-0001.1, 2017.
Korolev, A., Heckman, I., and Wolde, M.: Observation of Phase Composition and Humidity, in: Oceanic Mesoscale Convective Systems, 15th AMS Cloud Physics Conference, Vancouver, BC, 9–13 July 2018, https://ams.confex.com/ams/15CLOUD15ATRAD/webprogram/Paper347111.html (last access: 30 April 2024), 2018.
Korolev, A., Heckman, I., Wolde, M., Ackerman, A. S., Fridlind, A. M., Ladino, L. A., Lawson, R. P., Milbrandt, J., and Williams, E.: A new look at the environmental conditions favorable to secondary ice production, Atmos. Chem. Phys., 20, 1391–1429, https://doi.org/10.5194/acp-20-1391-2020, 2020.
Korolev, A., Qu, Z., Milbrandt, J., Heckman, I., and Cholette, M.: Active Regions of Secondary Ice Production in a Modeled Tropical Mesoscale Convective System, Zenodo [video], https://doi.org/10.5281/zenodo.13952689, 2024.
Korolev, A. V. and Isaac, G. A.: Phase transformation of mixed phase clouds, Q. J. Roy. Meteor. Soc., 129, 19–38, https://doi.org/10.1256/qj.01.203, 2003.
Korolev, A. V. and Mazin, I. P.: Supersaturation of water vapor in clouds, J. Atmos. Sci., 60, 2957–2974, https://doi.org/10.1175/1520-0469(2003)060<2957:SOWVIC>2.0.CO;2, 2003.
Korolev, A. V., Strapp, J. W., Isaac, G. A., and Nevzorov, A. N.: The Nevzorov Airborne Hot-Wire LWC–TWC Probe: Principle of Operation and Performance Characteristics, J. Atmos. Ocean. Tech., 15, 1495–1510, https://doi.org/10.1175/1520-0426(1998)015<1495:TNAHWL>2.0.CO;2, 1998.
Korolev, A. V., Emery, E. F., Strapp, J. W., Cober, S. G., Isaac, G. A., Wasey, M., and Marcotte, D.: Small Ice Particles in Tropospheric Clouds: Fact or Artifact? Airborne Icing Instrumentation Evaluation Experiment, B. Am. Meteorol. Soc., 92, 967–973, https://doi.org/10.1175/2010BAMS3141.1, 2011.
Ladino, L. A., Korolev, A., Heckman, I., Wolde, M., Fridlind, A. M., and Ackerman, A. S.: On the role of ice-nucleating aerosol in the formation of ice particles in tropical mesoscale convective systems, Geophys. Res. Lett., 44, 1574–1582, https://doi.org/10.1002/2016GL072455, 2017.
Lance, S., Brock, C. A., Rogers, D., and Gordon, J. A.: Water droplet calibration of the Cloud Droplet Probe (CDP) and in-flight performance in liquid, ice and mixed-phase clouds during ARCPAC, Atmos. Meas. Tech., 3, 1683–1706, https://doi.org/10.5194/amt-3-1683-2010, 2010.
Lawson, R. P., Angus, L. J., and Heymsfield, A. J.: Cloud Particle Measurements in Thunderstorm Anvils and Possible Threat to Aviation, J. Aircraft, 35, 113–121, https://doi.org/10.2514/2.2268, 1998.
Lawson, R. P., Baker, B. A., Schmitt, C. G., and Jensen, T. L.: An overview of microphysical properties of Arctic clouds observed in May and July 1998 during FIRE ACE, J. Geophys. Res.-Atmos., 106, 14989–15014, https://doi.org/10.1029/2000JD900789, 2001.
Lawson, R. P., O'Connor, D., Zmarzly, P., Weaver, K., Baker, B., Mo, Q., and Jonsson, H.: The 2D-S (Stereo) Probe: Design and Preliminary Tests of a New Airborne, High-Speed, High-Resolution Particle Imaging Probe, J. Atmos. Ocean. Tech., 23, 1462–1477, https://doi.org/10.1175/JTECH1927.1, 2006.
Lawson, R. P., Woods, S., and Morrison, H.: The microphysics of ice and precipitation development in tropical cumulus clouds, J. Atmos. Sci., 72, 2429–2445, https://doi.org/10.1175/JAS-D-14-0274.1, 2015.
Lawson, R. P., Korolev, A. V., DeMott, P. J., Heymsfield, A. J., Bruintjes, R. T., Wolff, C. A., Woods, S., Patnaude, R. J., Jensen, J. B., Moore, K. A., Heckman, I., Rosky, E., Haggerty, J., Perkins, R. J., Fisher, T., and Hill, T. C. J.: The Secondary Production of Ice in Cumulus Experiment (SPICULE), B. Am. Meteorol. Soc., 104, E51–E76, https://doi.org/10.1175/BAMS-D-21-0209.1, 2023.
Leroy, D., Fontaine, E., Schwarzenboeck, A., and Strapp, J. W.: Ice Crystal Sizes in High Ice Water Content Clouds. Part I: On the Computation of Median Mass Diameters from In Situ Measurements, J. Atmos. Ocean. Tech. 33, 2461–2476, 2016, https://doi.org/10.1175/JTECH-D-15-0151.1, 2016.
Leroy, D., Fontaine, E., Schwarzenboeck, A., Strapp, J. W., Korolev, A., McFarquhar, G., Dupuy, R., Gourbeyre, C., Lilie, L., Protat, A., Delanoe, J., Dezitter F., and Grandin A.: Ice Crystal Sizes in High Ice Water Content Clouds. Part II: Statistics of Mass Diameter Percentiles in Tropical Convection Observed during the HAIC/HIWC Project, J. Atmos. Ocean. Tech., 34, 117–136, https://doi.org/10.1175/JTECH-D-15-0246.1, 2017.
Magono, C. and Lee, C.: Meteorological classification of natural snow crystals, Journal of the Faculty of Science, Hokkaido Univ. Ser. VII, 2, 321–335, http://hdl.handle.net/2115/8672, 1966.
Mason, J. and Grzych, M.: The Challenges Identifying Weather Associated with Jet Engine Ice Crystal Icing, SAE Technical Paper 2011-38-0094, SAE Mobilus, https://doi.org/10.4271/2011-38-0094, 2011.
Mason, J., Strapp, J. W., and Chow, P.: The Ice Particle Threat to Engines in Flight, in: 44th AIAA Aerospace Sciences Meeting and Exhibit, AIAA 2006-206, 9–12 January 2006, Reno, NV, https://doi.org/10.2514/6.2006-206, 2006.
Mazin, I. P., Korolev, A. V., Heymsfield, A., Isaac, G. A., and Cober, S. G.: Thermodynamics of Icing Cylinder for Measurements of Liquid Water Content in Supercooled Clouds, J. Atmos. Ocean. Tech., 18, 543–558, https://doi.org/10.1175/1520-0426(2001)018<0543:TOICFM>2.0.CO;2, 2001.
McFarquhar, G. M., Baumgardner, D., Bansemer, A., Abel, S. J., Crosier, J., French, J., Rosenberg, P., Korolev, A., Schwarzoenboeck, A., Leroy, D., Um, J., Wu, W., Heymsfield, A. J., Twohy, C., Detwiler, A., Field, P., Neumann, A., Cotton, R., Axisa, D., and Dong, J.: Processing of ice cloud in situ data collected by bulk water, scattering, and imaging probes: fundamentals, uncertainties, and efforts toward consistency, Meteor. Mon., 58, 11.1–11.33, https://doi.org/10.1175/AMSMONOGRAPHSD-16-0007.1, 2017.
Milbrandt, J. A. and Morrison, H.: Parameterization of cloud microphysics based on the prediction of bulk ice particle properties. Part III. Introduction of multiple free categories, J. Atmos. Sci., 73, 975–995, https://doi.org/10.1175/JAS-D-15-0204.1, 2016.
Morrison, H. and Milbrandt, J. A.: Parameterization of cloud microphysics based on the prediction of bulk ice particle properties. Part I: Scheme description and idealized tests, J. Atmos. Sci., 72, 287–311, https://doi.org/10.1175/JAS-D-14-0065.1, 2015.
Nakaya, U.: Snow Crystals, Natural and Artificial, Harvard University Press, 510 pp., 1954.
Naylor, J. and Gilmore, M. S.: Convective initiation in an idealized cloud model using an updraft nudging technique, Mon. Weather Rev., 140, 3699–3705, https://doi.org/10.1175/MWR-D-12-00163.1, 2012.
Nelson, J.: Growth mechanisms to explain the primary and secondary habits of snow crystals, Philos. Mag. A, 81, 2337–2373, https://doi.org/10.1080/01418610108217152, 2001.
Pinsky, M., Khain, A., and Korolev, A.: Analytical investigation of glaciation time in mixed-phase adiabatic cloud volumes, J. Atmos. Sci., 57, 4143–4157, https://doi.org/10.1175/JAS-D-13-0359.1, 2014.
Protat, A., Delanoë, J., Strapp, J., Fontaine, E., Leroy, D., Schwarzenboeck, A., Lilie, L., Davison, C., Dezitter, F., Grandin, A., and Weber, M.: The measured relationship between ice water content and cloud radar reflectivity in tropical convective clouds, J. Appl. Meteorol. Clim., 55, 1707–1729, https://doi.org/10.1175/JAMC-D-15-0248.1, 2016.
Pruppacher, H. R. and Klett, J. D.: Microphysics of clouds and precipitation, Kluwer Academic Publishers, Dordrecht, 954 pp., ISBN 0-7923-4211-9, 1997.
Rottner, D. and Vali, G.: Snow crystal habit at small excesses of vapor density over ice saturation, J. Atmos. Sci., 31, 560–569, https://doi.org/10.1175/1520-0469(1974)031,0560:SCHASE.2.0.CO;2, 1974.
Rugg, A., A., Bernstein, B. C., Haggerty, J. A., Korolev, A., Nguyen, C., Wolde, M., Heckman, I., and DiVito, St.: High Ice Water Content Conditions Associated with Wintertime Elevated Convection in the Midwest, J. Appl. Meteorol. Clim., 61, 559–575, https://doi.org/10.1175/JAMC-D-21-0189.1, 2022.
Ryan, B. F., Wishart, E. R., and Shaw, D. E.: The Growth Rates and Densities of Ice Crystals between −3 °C and −21 °C, J. Atmos. Sci., 33, 842–850, https://doi.org/10.1175/1520-0469(1976)033<0842:TGRADO>2.0.CO;2, 1976.
Qu, Z., Barker, H. W., Korolev, A. V., Milbrandt, J. A., Heckman, I., Bélair, S., Leroyer, S., Vaillancourt, P. A., Wolde, M., Schwarzenboeck, A., Leroy, D., Strapp, J. W., Cole, J. N. S., Nguyen, L., and Heidinger, A.: Evaluation of a high-resolution NWP model's simulated clouds using observations from CloudSat and in situ aircraft, Q. J. Roy. Meteor. Soc., 144, 1681–1694, https://doi.org/10.1002/qj.3318, 2018.
Qu, Z., Korolev, A., Milbrandt, J. A., Heckman, I., Huang, Y., McFarquhar, G. M., Morrison, H., Wolde, M., and Nguyen, C.: The impacts of secondary ice production on microphysics and dynamics in tropical convection, Atmos. Chem. Phys., 22, 12287–12310, https://doi.org/10.5194/acp-22-12287-2022, 2022.
Stanford, M. W., Varble, A., Zipser, E., Strapp, J. W., Leroy, D., Schwarzenboeck, A., Potts, R., and Protat, A.: A ubiquitous ice size bias in simulations of tropical deep convection, Atmos. Chem. Phys., 17, 9599–9621, https://doi.org/10.5194/acp-17-9599-2017, 2017.
Strapp, J. W., Chow, P., Maltby, M., Bezer, A. D. Korolev A., Stromberg, I., Hallett, J.: Cloud Microphysical Measurements in Thunderstorm Outflow Regions during Allied/BAe 1997 Flight Trials, in: 37th AIAA Aerospace Sciences Meeting and Exhibit, AIAA 99-0498, 11–14 January 1999, Reno, NV, https://doi.org/10.2514/6.1999-498, 1999.
Strapp, J. W., Korolev, A., Ratvasky, T. P. Potts, R., Protat, A., May, P., Ackerman, A., Fridlind, A., Minnis, P., Haggerty, J., Riley, J. T., Lilie, L. E., and Isaac, G. A.: The High Ice Water Content (HIWC) Study of Deep Convective Clouds: Science and Technical Plan, FAA Rep. DOT/FAA/TC-14/31, 105 pp., https://rosap.ntl.bts.gov/pdfjs/web/viewer.html?file=https://rosap.ntl.bts.gov/view/dot/57622/dot_57622_DS1.pdf (last access: 20 October 2024), 2016.
Strapp, J. W., Schwarzenboeck, A., Bedka, K., Bond, T., Calmels, A., Delanoë, J., Dezitter, F., Grzych, M., Harrah, S., Korolev, A., Leroy, D., Lilie, L., Mason, J., Potts, R., Protat, A., Ratvasky, T., Riley, J., and Wolde, M.: An assessment of cloud total water content and particle size from flight test campaign measurements in high ice water content, mixed phase/ice crystal icing conditions: Primary in-situ measurements, project science and technical plan, FAA Rep. DOT/FAA/TC-18/1, 262 pp., https://rosap.ntl.bts.gov/view/dot/57746 (last access: 20 October 2024), 2020.
Strapp, J. W., Schwarzenboeck, A., Bedka, K., Bond, T., Camels, A., Delanoë, J., Dezitter, F., Grzych, M., Harrah, S., Korolev, A., Leroy, D., Lilie, L., Mason, J., Potts, R., Protat, A., Ratvasky, T., Riley, J., and Wolde, M.: Comparisons of Cloud In Situ Microphysical Properties of Deep Convective Clouds to Appendix D/P Using Data from the High-Altitude Ice Crystals-High Ice Water Content and High Ice Water Content-RADAR I Flight Campaigns, SAE Int. J. Aerosp., 14, 1946–3901, https://doi.org/10.4271/01-14-02-0007, 2021.
Sullivan, S. and Voigt, A.: Ice microphysical processes exert a strong control on the simulated radiative energy budget in the tropics, Communications Earth and Environment, 2, 1–8, https://doi.org/10.1038/s43247-021-00206-7, 2021.
Williams, A. and Marcotte, D.: Wind measurements on a maneuvering twin-engine turboprop aircraft accounting for flow distortion, J. Atmos. Ocean. Tech., 17, 795–810, https://doi.org/10.1175/1520-0426(2000)017%3C0795:WMOAMT%3E2.0.CO;2, 2000.
Wolde, M. and Pazmany, A.: NRC dual-frequency airborne radar for atmospheric research, in: 32nd Int. Conf. on Radar Meteorology, Albuquerque, NM, 22–29 October 2005, Amer. Meteor. Soc., P1R.9, https://ams.confex.com/ams/32Rad11Meso/techprogram/paper_96918.htm (last access: 25 April 2024), 2005.
Wolde, M., Nguyen, C., Korolev, A., and Bastian, M.: Characterization of the Pilot X-band radar responses to the HIWC environment during the Cayenne HAIC-HIWC 2015 Campaign, in: 8th Conf. on AIAA Atmospheric and Space Environments, 13–17 June 2016, Washington, DC, American Institute of Aeronautics and Astronautics, AIAA-2016-4201, https://doi.org/10.2514/6.2016-4201, 2016.
Wurtz, J., Bouniol, D., Vié, B., and Lac, C.: Evaluation of the AROME model's ability to represent ice crystal icing using in situ observations from the HAIC 2015 field campaign, Q. J. Roy. Meteor. Soc., 147, 2796–2817, https://doi.org/10.1002/qj.4100, 2021.
Wurtz, J., Bouniol, D., and Vié, B.: Improvements to the parametrization of snow in AROME in the context of ice crystal icing, Q. J. Roy. Meteor. Soc., 149, 878–893, https://doi.org/10.1002/qj.4437, 2023.
Yost, C. R., Bedka, K. M., Minnis, P., Nguyen, L., Strapp, J. W., Palikonda, R., Khlopenkov, K., Spangenberg, D., Smith Jr., W. L., Protat, A., and Delanoe, J.: A prototype method for diagnosing high ice water content probability using satellite imager data, Atmos. Meas. Tech., 11, 1615–1637, https://doi.org/10.5194/amt-11-1615-2018, 2018.
Short summary
The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCSs) when a large number of small ice particles with typical sizes of a few hundred micrometers is found at high altitudes. It was found that secondary ice production in the vicinity of the melting layer plays a key role in the formation and maintenance of HIWC. This study presents a conceptual model of the formation of HIWC in tropical MCSs based on in situ observations and numerical simulation.
The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCSs)...
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