Articles | Volume 22, issue 9
https://doi.org/10.5194/acp-22-5743-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-5743-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
03 May 2022
Research article |
| 03 May 2022
| 03 May 2022
Stability-dependent increases in liquid water with droplet number in the Arctic
Rebecca J. Murray-Watson
CORRESPONDING AUTHOR
Space and Atmospheric Physics Group, Imperial College London, London, UK
Edward Gryspeerdt
Space and Atmospheric Physics Group, Imperial College London, London, UK
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Rebecca J. Murray-Watson and Edward Gryspeerdt
EGUsphere, https://doi.org/10.5194/egusphere-2024-129, https://doi.org/10.5194/egusphere-2024-129, 2024
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The formation of mixed-phase clouds during marine cold-air outbreaks is not well understood. Our study, using satellite data and Lagrangian trajectories, reveals that the occurrence of these clouds depends on both time and temperature, influenced partly by the presence of biological ice-nucleating particles. This highlights the importance of comprehending local aerosol dynamics for precise modeling of cloud phase transitions in the Arctic.
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Clouds formed in Arctic marine cold air outbreaks undergo a distinct evolution, but the factors controlling their transition from high-coverage to broken cloud fields are poorly understood. We use satellite and reanalysis data to study how these clouds develop in time and the different influences on their evolution. The aerosol concentration is correlated with cloud break-up; more aerosol is linked to prolonged coverage and a stronger cooling effect, with implications for a more polluted Arctic.
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The response of clouds to changes in aerosol remains a large uncertainty in our understanding of the climate. Studies typically look at aerosol and cloud processes in snapshot images, measuring all properties at the same time. Here we use multiple images to characterise how cloud temporal development responds to aerosol. We find a reduction in liquid water path with increasing aerosol, party due to feedbacks. This suggests the aerosol impact on cloud water may be weaker than in previous studies.
Harri Kokkola, Juha Tonttila, Silvia Calderón, Sami Romakkaniemi, Antti Lipponen, Aapo Peräkorpi, Tero Mielonen, Edward Gryspeerdt, Timo H. Virtanen, Pekka Kolmonen, and Antti Arola
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This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Rebecca J. Murray-Watson and Edward Gryspeerdt
EGUsphere, https://doi.org/10.5194/egusphere-2024-129, https://doi.org/10.5194/egusphere-2024-129, 2024
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The formation of mixed-phase clouds during marine cold-air outbreaks is not well understood. Our study, using satellite data and Lagrangian trajectories, reveals that the occurrence of these clouds depends on both time and temperature, influenced partly by the presence of biological ice-nucleating particles. This highlights the importance of comprehending local aerosol dynamics for precise modeling of cloud phase transitions in the Arctic.
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Atmos. Chem. Phys., 23, 14239–14253, https://doi.org/10.5194/acp-23-14239-2023, https://doi.org/10.5194/acp-23-14239-2023, 2023
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Tropical deep convective clouds, and the thin cirrus (ice) clouds that flow out from them, are important for modulating the energy budget of the tropical atmosphere. This work uses a new method to track the evolution of the properties of these clouds across their entire lifetimes. We find these clouds cool the atmosphere in the first 6 h before switching to a warming regime after the deep convective core has dissipated, which is sustained beyond 120 h from the initial convective event.
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Atmos. Chem. Phys., 23, 9365–9383, https://doi.org/10.5194/acp-23-9365-2023, https://doi.org/10.5194/acp-23-9365-2023, 2023
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The impact of aerosols on clouds is one of the largest uncertainties in the human forcing of the climate. Aerosol can increase the concentrations of droplets in clouds, but observational and model studies produce widely varying estimates of this effect. We show that these estimates can be reconciled if only polluted clouds are studied, but this is insufficient to constrain the climate impact of aerosol. The uncertainty in aerosol impact on clouds is currently driven by cases with little aerosol.
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Atmos. Chem. Phys., 22, 11727–11738, https://doi.org/10.5194/acp-22-11727-2022, https://doi.org/10.5194/acp-22-11727-2022, 2022
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Edward Gryspeerdt, Johannes Mülmenstädt, Andrew Gettelman, Florent F. Malavelle, Hugh Morrison, David Neubauer, Daniel G. Partridge, Philip Stier, Toshihiko Takemura, Hailong Wang, Minghuai Wang, and Kai Zhang
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The effect of aerosol–cloud interactions (ACIs) on Earth's energy budget continues to be highly uncertain. We decompose the effective radiative forcing by ACIs (ERFaci) into the instantaneous forcing due to anthropogenic increases in the number of cloud droplets and fast responses of cloud properties to the droplet number perturbation in the ECHAM–HAMMOZ aerosol–climate model. This decomposition maps onto the IPCC's Fifth Assessment Report analysis of ERFaci more directly than previous work.
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Atmos. Chem. Phys., 19, 5331–5347, https://doi.org/10.5194/acp-19-5331-2019, https://doi.org/10.5194/acp-19-5331-2019, 2019
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The liquid water path (LWP) is the strongest control on cloud albedo, such that a small change in LWP can have a large radiative impact. By changing the droplet number concentration (Nd) aerosols may be able to change the LWP, but the sign and magnitude of the effect is unclear. This work uses satellite data to investigate the relationship between Nd and LWP at a global scale and in response to large aerosol perturbations, suggesting that a strong decrease in LWP at high Nd may be overestimated.
Odran Sourdeval, Edward Gryspeerdt, Martina Krämer, Tom Goren, Julien Delanoë, Armin Afchine, Friederike Hemmer, and Johannes Quaas
Atmos. Chem. Phys., 18, 14327–14350, https://doi.org/10.5194/acp-18-14327-2018, https://doi.org/10.5194/acp-18-14327-2018, 2018
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The number concentration of ice crystals (Ni) is a key cloud property that remains very uncertain due to difficulties in determining it using satellites. This lack of global observational constraints limits our ability to constrain this property in models responsible for predicting future climate. This pair of papers fills this gap by showing and analyzing the first rigorously evaluated global climatology of Ni, leading to new information shedding light on the processes that control high clouds.
Edward Gryspeerdt, Odran Sourdeval, Johannes Quaas, Julien Delanoë, Martina Krämer, and Philipp Kühne
Atmos. Chem. Phys., 18, 14351–14370, https://doi.org/10.5194/acp-18-14351-2018, https://doi.org/10.5194/acp-18-14351-2018, 2018
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The concentration of ice crystals in a cloud affects both the properties and the life cycle of the cloud. This work uses a new satellite retrieval to investigate controls on the ice crystal concentration at a global scale. Both temperature and vertical wind speed in a cloud have a strong impact on the concentration of ice crystals. The ice crystal number is also related to the aerosol environment; defining this relation opens up new ways to investigate human impacts on clouds and the climate.
Edward Gryspeerdt, Johannes Quaas, Tom Goren, Daniel Klocke, and Matthias Brueck
Atmos. Chem. Phys., 18, 6157–6169, https://doi.org/10.5194/acp-18-6157-2018, https://doi.org/10.5194/acp-18-6157-2018, 2018
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Cirrus clouds can form by a variety of mechanisms, such as orographic uplift, through convective systems or through large-scale rising motions. In this work, an automated classification of cirrus clouds based on satellite and reanalysis data is presented to separate cirrus by these different formation mechanisms. The classification provides information on the ice origin and cloud-scale updraughts that could not be determined using satellite or reanalysis data alone.
Bethan White, Edward Gryspeerdt, Philip Stier, Hugh Morrison, Gregory Thompson, and Zak Kipling
Atmos. Chem. Phys., 17, 12145–12175, https://doi.org/10.5194/acp-17-12145-2017, https://doi.org/10.5194/acp-17-12145-2017, 2017
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Aerosols influence cloud and precipitation by modifying cloud droplet number concentrations (CDNCs). We simulate three different types of convective cloud using two different cloud microphysics parameterisations. The simulated cloud and precipitation depends much more strongly on the choice of microphysics scheme than on CDNC. The uncertainty differs between types of convection. Our results highlight a large uncertainty in cloud and precipitation responses to aerosol in current models.
Nick Schutgens, Svetlana Tsyro, Edward Gryspeerdt, Daisuke Goto, Natalie Weigum, Michael Schulz, and Philip Stier
Atmos. Chem. Phys., 17, 9761–9780, https://doi.org/10.5194/acp-17-9761-2017, https://doi.org/10.5194/acp-17-9761-2017, 2017
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We estimate representativeness errors in observations due to mismatching spatio-temporal sampling, on timescales of hours to a year and length scales of 50 to 200 km, for a variety of observing systems (in situ or remote sensing ground sites, satellites with imagers or lidar, etc.) and develop strategies to reduce them. This study is relevant to the use of observations in constructing satellite L3 products, observational intercomparison and model evaluation.
Duncan Watson-Parris, Nick Schutgens, Nicholas Cook, Zak Kipling, Philip Kershaw, Edward Gryspeerdt, Bryan Lawrence, and Philip Stier
Geosci. Model Dev., 9, 3093–3110, https://doi.org/10.5194/gmd-9-3093-2016, https://doi.org/10.5194/gmd-9-3093-2016, 2016
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In this paper we describe CIS, a new command line tool for the easy visualization, analysis and comparison of a wide variety of gridded and ungridded data sets used in Earth sciences. Users can now use a single tool to not only view plots of satellite, aircraft, station or model data, but also bring them onto the same spatio-temporal sampling. This allows robust, quantitative comparisons to be made easily. CIS is an open-source project and welcomes input from the community.
Nick A. J. Schutgens, Edward Gryspeerdt, Natalie Weigum, Svetlana Tsyro, Daisuke Goto, Michael Schulz, and Philip Stier
Atmos. Chem. Phys., 16, 6335–6353, https://doi.org/10.5194/acp-16-6335-2016, https://doi.org/10.5194/acp-16-6335-2016, 2016
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We show that evaluating global aerosol model data with observations of very different spatial scales (200 vs. 10 km) can lead to large discrepancies, solely due to different spatial sampling. Strategies for reducing these sampling errors are developed and tested using a set of high-resolution model simulations.
E. Gryspeerdt, P. Stier, B. A. White, and Z. Kipling
Atmos. Chem. Phys., 15, 7557–7570, https://doi.org/10.5194/acp-15-7557-2015, https://doi.org/10.5194/acp-15-7557-2015, 2015
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Wet scavenging generates differences between the aerosol properties in clear-sky scenes (observed by satellites) and cloudy scenes, leading to different
aerosol-precipitation relationships in satellite data and global models. Convective systems usually draw in air from clear-sky regions, but global models have difficulty separating this aerosol from the aerosol in cloudy scenes within a model gridbox. This may prevent models from reproducing the observed aerosol-precipitation relationships.
E. Gryspeerdt, P. Stier, and D. G. Partridge
Atmos. Chem. Phys., 14, 9677–9694, https://doi.org/10.5194/acp-14-9677-2014, https://doi.org/10.5194/acp-14-9677-2014, 2014
E. Gryspeerdt, P. Stier, and D. G. Partridge
Atmos. Chem. Phys., 14, 1141–1158, https://doi.org/10.5194/acp-14-1141-2014, https://doi.org/10.5194/acp-14-1141-2014, 2014
Related subject area
Subject: Clouds and Precipitation | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
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Investigating the development of clouds within marine cold-air outbreaks
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Grégory V. Cesana, Olivia Pierpaoli, Matteo Ottaviani, Linh Vu, Zhonghai Jin, and Israel Silber
Atmos. Chem. Phys., 24, 7899–7909, https://doi.org/10.5194/acp-24-7899-2024, https://doi.org/10.5194/acp-24-7899-2024, 2024
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Better characterizing the relationship between sea ice and clouds is key to understanding Arctic climate because clouds and sea ice affect surface radiation and modulate Arctic surface warming. Our results indicate that Arctic liquid clouds robustly increase in response to sea ice decrease. This increase has a cooling effect on the surface because more solar radiation is reflected back to space, and it should contribute to dampening future Arctic surface warming.
Ziming Wang, Husi Letu, Huazhe Shang, and Luca Bugliaro
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The supercooled liquid fraction (SLF) in mixed-phase clouds is retrieved for the first time using passive geostationary satellite observations based on differences in liquid droplet and ice particle radiative properties. The retrieved results are comparable to global distributions observed by active instruments, and the feasibility of the retrieval method to analyze the observed trends of the SLF has been validated.
Barbara Dietel, Odran Sourdeval, and Corinna Hoose
Atmos. Chem. Phys., 24, 7359–7383, https://doi.org/10.5194/acp-24-7359-2024, https://doi.org/10.5194/acp-24-7359-2024, 2024
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Uncertainty with respect to cloud phases over the Southern Ocean and Arctic marine regions leads to large uncertainties in the radiation budget of weather and climate models. This study investigates the phases of low-base and mid-base clouds using satellite-based remote sensing data. A comprehensive analysis of the correlation of cloud phase with various parameters, such as temperature, aerosols, sea ice, vertical and horizontal cloud extent, and cloud radiative effect, is presented.
Ryan Eastman, Isabel L. McCoy, Hauke Schulz, and Robert Wood
Atmos. Chem. Phys., 24, 6613–6634, https://doi.org/10.5194/acp-24-6613-2024, https://doi.org/10.5194/acp-24-6613-2024, 2024
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Cloud types are determined using machine learning image classifiers applied to satellite imagery for 1 year in the North Atlantic. This survey of these cloud types shows that the climate impact of a cloud scene is, in part, a function of cloud type. Each type displays a different mix of thick and thin cloud cover, with the fraction of thin cloud cover having the strongest impact on the clouds' radiative effect. Future studies must account for differing properties and processes among cloud types.
Thomas Lesigne, François Ravetta, Aurélien Podglajen, Vincent Mariage, and Jacques Pelon
Atmos. Chem. Phys., 24, 5935–5952, https://doi.org/10.5194/acp-24-5935-2024, https://doi.org/10.5194/acp-24-5935-2024, 2024
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Upper tropical clouds have a strong impact on Earth's climate but are challenging to observe. We report the first long-duration observations of tropical clouds from lidars flying on board stratospheric balloons. Comparisons with spaceborne observations reveal the enhanced sensitivity of balloon-borne lidar to optically thin cirrus. These clouds, which have a significant coverage and lie in the uppermost troposphere, are linked with the dehydration of air masses on their way to the stratosphere.
Georgios Dekoutsidis, Martin Wirth, and Silke Groß
Atmos. Chem. Phys., 24, 5971–5987, https://doi.org/10.5194/acp-24-5971-2024, https://doi.org/10.5194/acp-24-5971-2024, 2024
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For decades the earth's temperature has been rising. The Arctic regions are warming faster. Cirrus clouds can contribute to this phenomenon. During warm-air intrusions, air masses are transported into the Arctic from the mid-latitudes. The HALO-(AC)3 campaign took place to measure cirrus during intrusion events and under normal conditions. We study the two cloud types based on these measurements and find differences in their geometry, relative humidity distribution and vertical structure.
Huige Di and Yun Yuan
Atmos. Chem. Phys., 24, 5783–5801, https://doi.org/10.5194/acp-24-5783-2024, https://doi.org/10.5194/acp-24-5783-2024, 2024
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We observed the seeder–feeder process among double-layer clouds using a cloud radar and microwave radiometer. By defining the parameters of the seeding depth and seeding time of the upper cloud affecting the lower cloud, we find that the cloud particle terminal velocity is significantly enhanced during the seeder–feeder period, and the lower the height and thinner the thickness of the height difference between double-layer clouds, the lower the height and thicker the thickness of seeding depth.
Kristofer S. Tuftedal, Bernat Puigdomènech Treserras, Mariko Oue, and Pavlos Kollias
Atmos. Chem. Phys., 24, 5637–5657, https://doi.org/10.5194/acp-24-5637-2024, https://doi.org/10.5194/acp-24-5637-2024, 2024
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This study analyzed coastal convective cells from June through September 2018–2021. The cells were classified and their lifecycles were analyzed to better understand their characteristics. Features such as convective-core growth, for example, are shown. The study found differences in the initiation location of shallow convection and in the aerosol loading in deep convective environments. This work provides a foundation for future analyses of convection or other tracked events elsewhere.
Michie Vianca De Vera, Larry Di Girolamo, Guangyu Zhao, Robert M. Rauber, Stephen W. Nesbitt, and Greg M. McFarquhar
Atmos. Chem. Phys., 24, 5603–5623, https://doi.org/10.5194/acp-24-5603-2024, https://doi.org/10.5194/acp-24-5603-2024, 2024
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Tropical oceanic low clouds remain a dominant source of uncertainty in cloud feedback in climate models due to their macrophysical properties (fraction, size, height, shape, distribution) being misrepresented. High-resolution satellite imagery over the Philippine oceans is used here to characterize cumulus macrophysical properties and their relationship to meteorological variables. Such information can act as a benchmark for cloud models and can improve low-cloud generation in climate models.
William K. Jones, Martin Stengel, and Philip Stier
Atmos. Chem. Phys., 24, 5165–5180, https://doi.org/10.5194/acp-24-5165-2024, https://doi.org/10.5194/acp-24-5165-2024, 2024
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Storm clouds cover large areas of the tropics. These clouds both reflect incoming sunlight and trap heat from the atmosphere below, regulating the temperature of the tropics. Over land, storm clouds occur in the late afternoon and evening and so exist both during the daytime and at night. Changes in this timing could upset the balance of the respective cooling and heating effects of these clouds. We find that isolated storms have a larger effect on this balance than their small size suggests.
Shaoyue Qiu, Xue Zheng, David Painemal, Christopher R. Terai, and Xiaoli Zhou
Atmos. Chem. Phys., 24, 2913–2935, https://doi.org/10.5194/acp-24-2913-2024, https://doi.org/10.5194/acp-24-2913-2024, 2024
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The aerosol indirect effect (AIE) depends on cloud states, which exhibit significant diurnal variations in the northeastern Atlantic. Yet the AIE diurnal cycle remains poorly understood. Using satellite retrievals, we find a pronounced “U-shaped” diurnal variation in the AIE, which is contributed to by the transition of cloud states combined with the lagged cloud responses. This suggests that polar-orbiting satellites with overpass times at noon underestimate daytime mean values of the AIE.
Yuxin Zhao, Jiming Li, Deyu Wen, Yarong Li, Yuan Wang, and Jianping Huang
EGUsphere, https://doi.org/10.5194/egusphere-2024-480, https://doi.org/10.5194/egusphere-2024-480, 2024
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This study identifies deep convection systems (DCSs), including deep convection core and anvils over Tibetan Plateau and Tropical Oceans. The results show that the DCSs over TP are less frequent, exhibiting narrower and thinner cores and anvils compared to those over TO. The TP DCSs show stronger longwave cloud radiative effect on the surface and low-level atmosphere. Unique aerosol-cloud-precipitation interaction is found in TP DCSs, due to the cold cloud bases.
Irene Bartolomé García, Odran Sourdeval, Reinhold Spang, and Martina Krämer
Atmos. Chem. Phys., 24, 1699–1716, https://doi.org/10.5194/acp-24-1699-2024, https://doi.org/10.5194/acp-24-1699-2024, 2024
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How many ice crystals of each size are in a cloud is a key parameter for the retrieval of cloud properties. The distribution of ice crystals is obtained from in situ measurements and used to create parameterizations that can be used when analyzing the remote-sensing data. Current parameterizations are based on data sets that do not include reliable measurements of small crystals, but in our study we use a data set that includes very small ice crystals to improve these parameterizations.
Wenyue Wang, Klemens Hocke, Leonardo Nania, Alberto Cazorla, Gloria Titos, Renaud Matthey, Lucas Alados-Arboledas, Agustín Millares, and Francisco Navas-Guzmán
Atmos. Chem. Phys., 24, 1571–1585, https://doi.org/10.5194/acp-24-1571-2024, https://doi.org/10.5194/acp-24-1571-2024, 2024
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The south-central interior of Andalusia experiences complex precipitation patterns as a result of the semi-arid Mediterranean climate and the influence of Saharan dust. This study monitored the inter-relations between aerosols, clouds, meteorological variables, and precipitation systems using ground-based remote sensing and in situ instruments.
Francisco Lang, Steven T. Siems, Yi Huang, Tahereh Alinejadtabrizi, and Luis Ackermann
Atmos. Chem. Phys., 24, 1451–1466, https://doi.org/10.5194/acp-24-1451-2024, https://doi.org/10.5194/acp-24-1451-2024, 2024
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Marine low-level clouds play a crucial role in the Earth's energy balance, trapping heat from the surface and reflecting sunlight back into space. These clouds are distinguishable by their large-scale spatial structures, primarily characterized as hexagonal patterns with either filled (closed) or empty (open) cells. Utilizing satellite observations, these two cloud type patterns have been categorized over the Southern Ocean and North Pacific Ocean through a pattern recognition program.
Julian Hofer, Patric Seifert, J. Ben Liley, Martin Radenz, Osamu Uchino, Isamu Morino, Tetsu Sakai, Tomohiro Nagai, and Albert Ansmann
Atmos. Chem. Phys., 24, 1265–1280, https://doi.org/10.5194/acp-24-1265-2024, https://doi.org/10.5194/acp-24-1265-2024, 2024
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An 11-year dataset of polarization lidar observations from Lauder, New Zealand / Aotearoa, was used to distinguish the thermodynamic phase of natural clouds. The cloud dataset was separated to assess the impact of air mass origin on the frequency of heterogeneous ice formation. Ice formation efficiency in clouds above Lauder was found to be lower than in the polluted Northern Hemisphere midlatitudes but higher than in very clean and pristine environments, such as Punta Arenas in southern Chile.
Hannes Jascha Griesche, Carola Barrientos-Velasco, Hartwig Deneke, Anja Hünerbein, Patric Seifert, and Andreas Macke
Atmos. Chem. Phys., 24, 597–612, https://doi.org/10.5194/acp-24-597-2024, https://doi.org/10.5194/acp-24-597-2024, 2024
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The Arctic is strongly affected by climate change and the role of clouds therein is not yet completely understood. Measurements from the Arctic expedition PS106 were used to simulate radiative fluxes with and without clouds at very low altitudes (below 165 m), and their radiative effect was calculated to be 54 Wm-2. The low heights of these clouds make them hard to observe. This study shows the importance of accurate measurements and simulations of clouds and gives suggestions for improvements.
Thomas D. DeWitt, Timothy J. Garrett, Karlie N. Rees, Corey Bois, Steven K. Krueger, and Nicolas Ferlay
Atmos. Chem. Phys., 24, 109–122, https://doi.org/10.5194/acp-24-109-2024, https://doi.org/10.5194/acp-24-109-2024, 2024
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Viewed from space, a defining feature of Earth's atmosphere is the wide spectrum of cloud sizes. A recent study predicted the distribution of cloud sizes, and this paper compares the prediction to observations. Although there is nuance in viewing perspective, we find robust agreement with theory across different climatological conditions, including land–ocean contrasts, time of year, or latitude, suggesting a minor role for Coriolis forces, aerosol loading, or surface temperature.
Marcus Klingebiel, André Ehrlich, Elena Ruiz-Donoso, Nils Risse, Imke Schirmacher, Evelyn Jäkel, Michael Schäfer, Kevin Wolf, Mario Mech, Manuel Moser, Christiane Voigt, and Manfred Wendisch
Atmos. Chem. Phys., 23, 15289–15304, https://doi.org/10.5194/acp-23-15289-2023, https://doi.org/10.5194/acp-23-15289-2023, 2023
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In this study we explain how we use aircraft measurements from two Arctic research campaigns to identify cloud properties (like droplet size) over sea-ice and ice-free ocean. To make sure that our measurements make sense, we compare them with other observations. Our results show, e.g., larger cloud droplets in early summer than in spring. Moreover, the cloud droplets are also larger over ice-free ocean than compared to sea ice. In the future, our data can be used to improve climate models.
Pablo Saavedra Garfias, Heike Kalesse-Los, Luisa von Albedyll, Hannes Griesche, and Gunnar Spreen
Atmos. Chem. Phys., 23, 14521–14546, https://doi.org/10.5194/acp-23-14521-2023, https://doi.org/10.5194/acp-23-14521-2023, 2023
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An important Arctic climate process is the release of heat fluxes from sea ice openings to the atmosphere that influence the clouds. The characterization of this process is the objective of this study. Using synergistic observations from the MOSAiC expedition, we found that single-layer cloud properties show significant differences when clouds are coupled or decoupled to the water vapour transport which is used as physical link between the upwind sea ice openings and the cloud under observation.
Matthew D. Lebsock and Mikael Witte
Atmos. Chem. Phys., 23, 14293–14305, https://doi.org/10.5194/acp-23-14293-2023, https://doi.org/10.5194/acp-23-14293-2023, 2023
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This paper evaluates measurements of cloud drop size distributions made from airplanes. We find that as the number of cloud drops increases the distribution of the cloud drop sizes narrows. The data are used to develop a simple equation that relates the drop number to the width of the drop sizes. We then use this equation to demonstrate that existing approaches to observe the drop number from satellites contain errors that can be corrected by including the new relationship.
George Horner and Edward Gryspeerdt
Atmos. Chem. Phys., 23, 14239–14253, https://doi.org/10.5194/acp-23-14239-2023, https://doi.org/10.5194/acp-23-14239-2023, 2023
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Tropical deep convective clouds, and the thin cirrus (ice) clouds that flow out from them, are important for modulating the energy budget of the tropical atmosphere. This work uses a new method to track the evolution of the properties of these clouds across their entire lifetimes. We find these clouds cool the atmosphere in the first 6 h before switching to a warming regime after the deep convective core has dissipated, which is sustained beyond 120 h from the initial convective event.
Rodanthi-Elisavet Mamouri, Albert Ansmann, Kevin Ohneiser, Daniel A. Knopf, Argyro Nisantzi, Johannes Bühl, Ronny Engelmann, Annett Skupin, Patric Seifert, Holger Baars, Dragos Ene, Ulla Wandinger, and Diofantos Hadjimitsis
Atmos. Chem. Phys., 23, 14097–14114, https://doi.org/10.5194/acp-23-14097-2023, https://doi.org/10.5194/acp-23-14097-2023, 2023
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For the first time, rather clear evidence is found that wildfire smoke particles can trigger strong cirrus formation. This finding is of importance because intensive and large wildfires may occur increasingly often in the future as climate change proceeds. Based on lidar observations in Cyprus in autumn 2020, we provide detailed insight into the cirrus formation at the tropopause in the presence of aged wildfire smoke (here, 8–9 day old Californian wildfire smoke).
Peter Manshausen, Duncan Watson-Parris, Matthew W. Christensen, Jukka-Pekka Jalkanen, and Philip Stier
Atmos. Chem. Phys., 23, 12545–12555, https://doi.org/10.5194/acp-23-12545-2023, https://doi.org/10.5194/acp-23-12545-2023, 2023
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Aerosol from burning fuel changes cloud properties, e.g., the number of droplets and the content of water. Here, we study how clouds respond to different amounts of shipping aerosol. Droplet numbers increase linearly with increasing aerosol over a broad range until they stop increasing, while the amount of liquid water always increases, independently of emission amount. These changes in cloud properties can make them reflect more or less sunlight, which is important for the earth's climate.
Hendrik Andersen, Jan Cermak, Alyson Douglas, Timothy A. Myers, Peer Nowack, Philip Stier, Casey J. Wall, and Sarah Wilson Kemsley
Atmos. Chem. Phys., 23, 10775–10794, https://doi.org/10.5194/acp-23-10775-2023, https://doi.org/10.5194/acp-23-10775-2023, 2023
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This study uses an observation-based cloud-controlling factor framework to study near-global sensitivities of cloud radiative effects to a large number of meteorological and aerosol controls. We present near-global sensitivity patterns to selected thermodynamic, dynamic, and aerosol factors and discuss the physical mechanisms underlying the derived sensitivities. Our study hopes to guide future analyses aimed at constraining cloud feedbacks and aerosol–cloud interactions.
Anne-Claire Billault-Roux, Paraskevi Georgakaki, Josué Gehring, Louis Jaffeux, Alfons Schwarzenboeck, Pierre Coutris, Athanasios Nenes, and Alexis Berne
Atmos. Chem. Phys., 23, 10207–10234, https://doi.org/10.5194/acp-23-10207-2023, https://doi.org/10.5194/acp-23-10207-2023, 2023
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Secondary ice production plays a key role in clouds and precipitation. In this study, we analyze radar measurements from a snowfall event in the Jura Mountains. Complex signatures are observed, which reveal that ice crystals were formed through various processes. An analysis of multi-sensor data suggests that distinct ice multiplication processes were taking place. Both the methods used and the insights gained through this case study contribute to a better understanding of snowfall microphysics.
Rebecca J. Murray-Watson, Edward Gryspeerdt, and Tom Goren
Atmos. Chem. Phys., 23, 9365–9383, https://doi.org/10.5194/acp-23-9365-2023, https://doi.org/10.5194/acp-23-9365-2023, 2023
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Clouds formed in Arctic marine cold air outbreaks undergo a distinct evolution, but the factors controlling their transition from high-coverage to broken cloud fields are poorly understood. We use satellite and reanalysis data to study how these clouds develop in time and the different influences on their evolution. The aerosol concentration is correlated with cloud break-up; more aerosol is linked to prolonged coverage and a stronger cooling effect, with implications for a more polluted Arctic.
Michael S. Diamond
Atmos. Chem. Phys., 23, 8259–8269, https://doi.org/10.5194/acp-23-8259-2023, https://doi.org/10.5194/acp-23-8259-2023, 2023
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Fuel sulfur regulations were implemented for ships in 2020 to improve air quality but may also accelerate global warming. We use spatial statistics and satellite retrievals to detect changes in the size of cloud droplets and find evidence for a resulting decrease in cloud brightness within a major shipping corridor after the sulfur limits went into effect. Our results confirm both that the regulations are being followed and that they are having a warming influence via their effect on clouds.
Hao Luo, Johannes Quaas, and Yong Han
Atmos. Chem. Phys., 23, 8169–8186, https://doi.org/10.5194/acp-23-8169-2023, https://doi.org/10.5194/acp-23-8169-2023, 2023
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Clouds exhibit a wide range of vertical structures with varying microphysical and radiative properties. We show a global survey of spatial distribution, vertical extent and radiative effect of various classified cloud vertical structures using joint satellite observations from the new CCCM datasets during 2007–2010. Moreover, the long-term trends in CVSs are investigated based on different CMIP6 future scenarios to capture the cloud variations with different, increasing anthropogenic forcings.
Gregor Köcher, Tobias Zinner, and Christoph Knote
Atmos. Chem. Phys., 23, 6255–6269, https://doi.org/10.5194/acp-23-6255-2023, https://doi.org/10.5194/acp-23-6255-2023, 2023
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Polarimetric radar observations of 30 d of convective precipitation events are used to statistically analyze 5 state-of-the-art microphysics schemes of varying complexity. The frequency and area of simulated heavy-precipitation events are in some cases significantly different from those observed, depending on the microphysics scheme. Analysis of simulated particle size distributions and reflectivities shows that some schemes have problems reproducing the correct particle size distributions.
Claudia J. Stubenrauch, Giulio Mandorli, and Elisabeth Lemaitre
Atmos. Chem. Phys., 23, 5867–5884, https://doi.org/10.5194/acp-23-5867-2023, https://doi.org/10.5194/acp-23-5867-2023, 2023
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Organized convection leads to large convective cloud systems and intense rain and may change with a warming climate. Their complete 3D description, attained by machine learning techniques in combination with various satellite observations, together with a cloud system concept, link convection to anvil properties, while convective organization can be identified by the horizontal structure of intense rain.
Scott E. Giangrande, Thiago S. Biscaro, and John M. Peters
Atmos. Chem. Phys., 23, 5297–5316, https://doi.org/10.5194/acp-23-5297-2023, https://doi.org/10.5194/acp-23-5297-2023, 2023
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Our study tracks thunderstorms observed during the wet and dry seasons of the Amazon Basin using weather radar. We couple this precipitation tracking with opportunistic overpasses of a wind profiler and other ground observations to add unique insights into the upwards and downwards air motions within these clouds at various stages in the storm life cycle. The results of a simple updraft model are provided to give physical explanations for observed seasonal differences.
Edward Gryspeerdt, Adam C. Povey, Roy G. Grainger, Otto Hasekamp, N. Christina Hsu, Jane P. Mulcahy, Andrew M. Sayer, and Armin Sorooshian
Atmos. Chem. Phys., 23, 4115–4122, https://doi.org/10.5194/acp-23-4115-2023, https://doi.org/10.5194/acp-23-4115-2023, 2023
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The impact of aerosols on clouds is one of the largest uncertainties in the human forcing of the climate. Aerosol can increase the concentrations of droplets in clouds, but observational and model studies produce widely varying estimates of this effect. We show that these estimates can be reconciled if only polluted clouds are studied, but this is insufficient to constrain the climate impact of aerosol. The uncertainty in aerosol impact on clouds is currently driven by cases with little aerosol.
Zackary Mages, Pavlos Kollias, Zeen Zhu, and Edward P. Luke
Atmos. Chem. Phys., 23, 3561–3574, https://doi.org/10.5194/acp-23-3561-2023, https://doi.org/10.5194/acp-23-3561-2023, 2023
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Cold-air outbreaks (when cold air is advected over warm water and creates low-level convection) are a dominant cloud regime in the Arctic, and we capitalized on ground-based observations, which did not previously exist, from the COMBLE field campaign to study them. We characterized the extent and strength of the convection and turbulence and found evidence of secondary ice production. This information is useful for model intercomparison studies that will represent cold-air outbreak processes.
Maria P. Cadeddu, Virendra P. Ghate, David D. Turner, and Thomas E. Surleta
Atmos. Chem. Phys., 23, 3453–3470, https://doi.org/10.5194/acp-23-3453-2023, https://doi.org/10.5194/acp-23-3453-2023, 2023
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We analyze the variability in marine boundary layer moisture at the Eastern North Atlantic site on a monthly and daily temporal scale and examine its fundamental role in the control of boundary layer cloudiness and precipitation. The study also highlights the complex interaction between large-scale and local processes controlling the boundary layer moisture and the importance of the mesoscale spatial distribution of vapor to support convection and precipitation.
Zhenquan Wang, Jian Yuan, Robert Wood, Yifan Chen, and Tiancheng Tong
Atmos. Chem. Phys., 23, 3247–3266, https://doi.org/10.5194/acp-23-3247-2023, https://doi.org/10.5194/acp-23-3247-2023, 2023
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This study develops a novel profile-based algorithm based on the ERA5 to estimate the inversion strength in the planetary boundary layer better than the previous inversion index, which is a key low-cloud-controlling factor. This improved measure is more effective at representing the meteorological influence on low-cloud variations. It can better constrain the meteorological influence on low clouds to better isolate cloud responses to aerosols or to estimate low cloud feedbacks in climate models.
Georgios Dekoutsidis, Silke Groß, Martin Wirth, Martina Krämer, and Christian Rolf
Atmos. Chem. Phys., 23, 3103–3117, https://doi.org/10.5194/acp-23-3103-2023, https://doi.org/10.5194/acp-23-3103-2023, 2023
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Cirrus clouds affect Earth's atmosphere, deeming our study important. Here we use water vapor measurements by lidar and study the relative humidity (RHi) within and around midlatitude cirrus clouds. We find high supersaturations in the cloud-free air and within the clouds, especially near the cloud top. We study two cloud types with different formation processes. Finally, we conclude that the shape of the distribution of RHi can be used as an indicator of different cloud evolutionary stages.
Huazhe Shang, Souichiro Hioki, Guillaume Penide, Céline Cornet, Husi Letu, and Jérôme Riedi
Atmos. Chem. Phys., 23, 2729–2746, https://doi.org/10.5194/acp-23-2729-2023, https://doi.org/10.5194/acp-23-2729-2023, 2023
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We find that cloud profiles can be divided into four prominent patterns, and the frequency of these four patterns is related to intensities of cloud-top entrainment and precipitation. Based on these analyses, we further propose a cloud profile parameterization scheme allowing us to represent these patterns. Our results shed light on how to facilitate the representation of cloud profiles and how to link them to cloud entrainment or precipitating status in future remote-sensing applications.
Luca Lelli, Marco Vountas, Narges Khosravi, and John Philipp Burrows
Atmos. Chem. Phys., 23, 2579–2611, https://doi.org/10.5194/acp-23-2579-2023, https://doi.org/10.5194/acp-23-2579-2023, 2023
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Arctic amplification describes the recent period in which temperatures have been rising twice as fast as or more than the global average and sea ice and the Greenland ice shelf are approaching a tipping point. Hence, the Arctic ability to reflect solar energy decreases and absorption by the surface increases. Using 2 decades of complementary satellite data, we discover that clouds unexpectedly increase the pan-Arctic reflectance by increasing their liquid water content, thus cooling the Arctic.
Yabin Gou, Haonan Chen, Hong Zhu, and Lulin Xue
Atmos. Chem. Phys., 23, 2439–2463, https://doi.org/10.5194/acp-23-2439-2023, https://doi.org/10.5194/acp-23-2439-2023, 2023
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This article investigates the complex precipitation microphysics associated with super typhoon Lekima using a host of in situ and remote sensing observations, including rain gauge and disdrometer data, as well as polarimetric radar observations. The impacts of precipitation microphysics on multi-source data consistency and radar precipitation estimation are quantified. It is concluded that the dynamical precipitation microphysical processes must be considered in radar precipitation estimation.
Hongxia Zhu, Rui Li, Shuping Yang, Chun Zhao, Zhe Jiang, and Chen Huang
Atmos. Chem. Phys., 23, 2421–2437, https://doi.org/10.5194/acp-23-2421-2023, https://doi.org/10.5194/acp-23-2421-2023, 2023
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The impacts of atmospheric dust aerosols and cloud dynamic conditions on precipitation vertical development in southeastern China were studied using multiple satellite observations. It was found that the precipitating drops under dusty conditions grow faster in the middle layer but slower in the upper and lower layers compared with their pristine counterparts. Quantitative estimation of the sensitivity of the precipitation top temperature to the dust aerosol optical depth is also provided.
Zane Dedekind, Jacopo Grazioli, Philip H. Austin, and Ulrike Lohmann
Atmos. Chem. Phys., 23, 2345–2364, https://doi.org/10.5194/acp-23-2345-2023, https://doi.org/10.5194/acp-23-2345-2023, 2023
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Simulations allowing ice particles to collide with one another producing more ice particles represented surface observations of ice particles accurately. An increase in ice particles formed through collisions was related to sharp changes in the wind direction and speed with height. Changes in wind speed and direction can therefore cause more enhanced collisions between ice particles and alter how fast and how much precipitation forms. Simulations were conducted with the atmospheric model COSMO.
Ramon Padullés, Estel Cardellach, and F. Joseph Turk
Atmos. Chem. Phys., 23, 2199–2214, https://doi.org/10.5194/acp-23-2199-2023, https://doi.org/10.5194/acp-23-2199-2023, 2023
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The results of comparing the polarimetric radio occultation observables and the ice water content retrieved from the CloudSat radar in a global and statistical way show a strong correlation between the geographical patterns of both quantities for a wide range of heights. This implies that horizontally oriented hydrometeors are systematically present through the whole globe and through all vertical levels, which could provide insights on the physical processes leading to precipitation.
Ziming Wang, Luca Bugliaro, Tina Jurkat-Witschas, Romy Heller, Ulrike Burkhardt, Helmut Ziereis, Georgios Dekoutsidis, Martin Wirth, Silke Groß, Simon Kirschler, Stefan Kaufmann, and Christiane Voigt
Atmos. Chem. Phys., 23, 1941–1961, https://doi.org/10.5194/acp-23-1941-2023, https://doi.org/10.5194/acp-23-1941-2023, 2023
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Differences in the microphysical properties of contrail cirrus and natural cirrus in a contrail outbreak situation during the ML-CIRRUS campaign over the North Atlantic flight corridor can be observed from in situ measurements. The cirrus radiative effect in the area of the outbreak, derived from satellite observation-based radiative transfer modeling, is warming in the early morning and cooling during the day.
Gerald G. Mace, Sally Benson, Ruhi Humphries, Peter M. Gombert, and Elizabeth Sterner
Atmos. Chem. Phys., 23, 1677–1685, https://doi.org/10.5194/acp-23-1677-2023, https://doi.org/10.5194/acp-23-1677-2023, 2023
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The number of cloud droplets per unit volume is a significantly important property of clouds that controls their reflective properties. Computer models of the Earth's atmosphere and climate have low skill at predicting the reflective properties of Southern Ocean clouds. Here we investigate the properties of those clouds using satellite data and find that the cloud droplet number and cloud albedo in the Southern Ocean are related to the oceanic phytoplankton abundance near Antarctica.
Jianhao Zhang and Graham Feingold
Atmos. Chem. Phys., 23, 1073–1090, https://doi.org/10.5194/acp-23-1073-2023, https://doi.org/10.5194/acp-23-1073-2023, 2023
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Using observations from space, we show maps of potential brightness changes in marine warm clouds in response to increases in cloud droplet concentrations. The environmental and aerosol conditions in which these clouds reside covary differently in each ocean basin, leading to distinct evolutions of cloud brightness changes. This work stresses the central importance of the covariability between meteorology and aerosol for scaling up the radiative response of cloud brightness changes.
Yuxin Zhao, Jiming Li, Lijie Zhang, Cong Deng, Yarong Li, Bida Jian, and Jianping Huang
Atmos. Chem. Phys., 23, 743–769, https://doi.org/10.5194/acp-23-743-2023, https://doi.org/10.5194/acp-23-743-2023, 2023
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Diurnal variations of clouds play an important role in the radiative budget and precipitation. Based on satellite observations, reanalysis, and CMIP6 outputs, the diurnal variations in total cloud cover and cloud vertical distribution over the Tibetan Plateau are explored. The diurnal cycle of cirrus is a key focus and found to have different characteristics from those found in the tropics. The relationship between the diurnal cycle of cirrus and meteorological factors is also discussed.
Qiang Li and Silke Groß
Atmos. Chem. Phys., 22, 15963–15980, https://doi.org/10.5194/acp-22-15963-2022, https://doi.org/10.5194/acp-22-15963-2022, 2022
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The IPCC report identified that cirrus clouds have a significant impact on the radiation balance comparable to the CO2 effects, which, however, is still hard to parameterize. The current study investigates the possible impact of aviation on cirrus properties based on the analysis of 10-year lidar measurements of CALIPSO. The results reveal that there is a significant positive trend in cirrus depolarization ratio in the last 10 years before COVID-19, which is strongly correlated with aviation.
Linda Forster and Bernhard Mayer
Atmos. Chem. Phys., 22, 15179–15205, https://doi.org/10.5194/acp-22-15179-2022, https://doi.org/10.5194/acp-22-15179-2022, 2022
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We present a novel retrieval using ground-based imaging observations of halo displays together with radiative transfer simulations to help improve our understanding of ice crystal properties representative of cirrus clouds. Analysis of 4400 calibrated HaloCam images featuring a 22° halo revealed aggregates of hexagonal columns of 20 µm effective radius with a mixture of about 37 % smooth and 63% severely roughened surfaces as the best match in general.
Yun He, Zhenping Yin, Fuchao Liu, and Fan Yi
Atmos. Chem. Phys., 22, 13067–13085, https://doi.org/10.5194/acp-22-13067-2022, https://doi.org/10.5194/acp-22-13067-2022, 2022
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A method is proposed to identify the sole presence of heterogeneous nucleation and competition between heterogeneous and homogeneous nucleation for dust-related cirrus clouds by characterizing the relationship between dust ice-nucleating particle concentration calculated from CALIOP using the POLIPHON method and in-cloud ice crystal number concentration from the DARDAR-Nice dataset. Two typical cirrus cases are shown as a demonstration, and the proposed method can be extended to a global scale.
Cited articles
Ackerman, A., Kirkpatrick, M., Stevens, D., and Toon, O.: The impact of
humidity above stratiform clouds on indirect aerosol climate forcing, Nature, 432,
1014–1017, https://doi.org/10.1038/nature03174, 2004. a, b
Albrecht, B. A.: Aerosols, Cloud Microphys. Fract. Cloud. Sci., 245, 1227–1230, https://doi.org/10.1126/science.245.4923.1227, 1989. a
Bennartz, R.: Global assessment of marine boundary layer cloud droplet number
concentration from satellite, J. Geophys. Res.-Atmos.,
112, https://doi.org/10.1029/2006JD007547, 2007. a
Bennartz, R., Shupe, M., Turner, D., Walden, V., Steffan, K., Cox, C., Kulie,
M., Miller, N., and Pettersen, C.: July 2012 Greenland melt extent enhanced
by low-level liquid clouds, Nature, 496, 83–86, https://doi.org/10.1038/nature12002,
2013. a
Boeke, R. C., Taylor, P. C., and Sejas, S. A.: On the Nature of the Arctic's
Positive Lapse-Rate Feedback, Geophys. Res. Lett., 48,
e2020GL091109, https://doi.org/10.1029/2020GL091109, 2021. a
Brenguier, J.-L., Pawlowska, H., Schüller, L., Preusker, R., Fischer, J., and
Fouquart, Y.: Radiative Properties of Boundary Layer Clouds: Droplet
Effective Radius versus Number Concentration, J. Atmos.
Sci., 57, 803–821,
https://doi.org/10.1175/1520-0469(2000)057<0803:RPOBLC>2.0.CO;2, 2000. a
Cavalieri, D. J., Parkinson, C. L., Gloersen, P., and Zwally, H. J.: Sea Ice
Concentrations from Nimbus-7 SMMR and DMSP SSM/I-SSMIS Passive Microwave
Data, Version 1, Boulder, Colorado USA, NASA National Snow and Ice Data
Center Distributed Active Archive Center, Updated yearly, [data set], https://doi.org/10.5067/8GQ8LZQVL0VL, 1996. a, b
Cesana, G., Kay, J. E., Chepfer, H., English, J. M., and de Boer, G.:
Ubiquitous low-level liquid-containing Arctic clouds: New observations and
climate model constraints from CALIPSO-GOCCP, Geophys. Res. Lett.,
39, L20804, https://doi.org/10.1029/2012GL053385, 2012. a
Chan, M. A. and Comiso, J. C.: Arctic Cloud Characteristics as Derived from
MODIS, CALIPSO, and CloudSat, J. Climate, 26, 3285–3306,
https://doi.org/10.1175/JCLI-D-12-00204.1, 2013. a
Choi, Y.-S., Kim, B.-M., Hur, S.-K., Kim, S.-J., Kim, J.-H., and Ho, C.-H.:
Connecting early summer cloud-controlled sunlight and late summer sea ice in
the Arctic, J. Geophys. Res.-Atmos., 119,
11087–11099, https://doi.org/10.1002/2014JD022013, 2014. a
Coopman, Q., Garrett, T. J., Riedi, J., Eckhardt, S., and Stohl, A.: Effects of long-range aerosol transport on the microphysical properties of low-level liquid clouds in the Arctic, Atmos. Chem. Phys., 16, 4661–4674, https://doi.org/10.5194/acp-16-4661-2016, 2016. a, b, c, d
Coopman, Q., Garrett, T. J., Finch, D. P., and Riedi, J.: High Sensitivity of
Arctic Liquid Clouds to Long-Range Anthropogenic Aerosol Transport,
Geophys. Res. Lett., 45, 372–381,
https://doi.org/10.1002/2017GL075795, 2018. a, b, c
Curry, J. A. and Ebert, E. E.: Annual Cycle of Radiation Fluxes over the Arctic
Ocean: Sensitivity to Cloud Optical Properties, J. Climate, 5, 1267–1280, https://doi.org/10.1175/1520-0442(1992)005<1267:ACORFO>2.0.CO;2, 1992. a
de Boer, G., Eloranta, E. W., and Shupe, M. D.: Arctic Mixed-Phase Stratiform
Cloud Properties from Multiple Years of Surface-Based Measurements at Two
High-Latitude Locations, J. Atmos. Sci., 66, 2874–2887, https://doi.org/10.1175/2009JAS3029.1, 2009. a
Dong, X., Xi, B., Qiu, S., Minnis, P., Sun-Mack, S., and Rose, F.: A radiation
closure study of Arctic stratus cloud microphysical properties using the
collocated satellite-surface data and Fu-Liou radiative transfer model,
J. Geophys. Res.-Atmos., 121, 10175–10198,
https://doi.org/10.1002/2016JD025255, 2016. a, b
Feingold, G., Remer, L. A., Ramaprasad, J., and Kaufman, Y. J.: Analysis of
smoke impact on clouds in Brazilian biomass burning regions: An extension of
Twomey's approach, J. Geophys. Res.-Atmos., 106,
22907–22922, https://doi.org/10.1029/2001JD000732, 2001. a
Fletcher, J. K., Mason, S., and Jakob, C.: A Climatology of Clouds in Marine
Cold Air Outbreaks in Both Hemispheres, J. Climate, 29, 6677–6692,
https://doi.org/10.1175/JCLI-D-15-0783.1, 2016. a
Garrett, T. J., Zhao, C., Dong, X., Mace, G. G., and Hobbs, P. V.: Effects of
varying aerosol regimes on low-level Arctic stratus, Geophys. Res. Lett., 31, L17105, https://doi.org/10.1029/2004GL019928, 2004. a, b, c
Graham, R. M., Hudson, S. R., and Maturilli, M.: Improved Performance of ERA5
in Arctic Gateway Relative to Four Global Atmospheric Reanalyses, Geophys. Res. Lett., 46, 6138–6147,
https://doi.org/10.1029/2019GL082781, 2019. a
Gryspeerdt, E., Quaas, J., and Bellouin, N.: Constraining the aerosol influence
on cloud fraction, J. Geophys. Res.-Atmos., 121,
3566–3583, https://doi.org/10.1002/2015JD023744, 2016. a, b
Gryspeerdt, E., Goren, T., Sourdeval, O., Quaas, J., Mülmenstädt, J., Dipu, S., Unglaub, C., Gettelman, A., and Christensen, M.: Constraining the aerosol influence on cloud liquid water path, Atmos. Chem. Phys., 19, 5331–5347, https://doi.org/10.5194/acp-19-5331-2019, 2019. a, b, c, d, e, f, g, h, i
Han, Q., Rossow, W. B., Zeng, J., and Welch, R.: Three Different Behaviors of
Liquid Water Path of Water Clouds in Aerosol–Cloud Interactions, J. Atmos. Sci., 59, 726–735,
https://doi.org/10.1175/1520-0469(2002)059<0726:TDBOLW>2.0.CO;2, 2002. a
Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A.,
Muñoz-Sabater, J., Nicolas, J., Peubey, C., Radu, R., Schepers, D., Simmons,
A., Soci, C., Abdalla, S., Abellan, X., Balsamo, G., Bechtold, P., Biavati,
G., Bidlot, J., Bonavita, M., De Chiara, G., Dahlgren, P., Dee, D.,
Diamantakis, M., Dragani, R., Flemming, J., Forbes, R., Fuentes, M., Geer,
A., Haimberger, L., Healy, S., Hogan, R. J., Hólm, E., Janisková, M.,
Keeley, S., Laloyaux, P., Lopez, P., Lupu, C., Radnoti, G., de Rosnay, P.,
Rozum, I., Vamborg, F., Villaume, S., and Thépaut, J.-N.: The ERA5 global
reanalysis, [data set], Q. J. Roy. Meteor. Soc., 146,
1999–2049, https://doi.org/10.1002/qj.3803, 2020. a, b
Huang, Y., Dong, X., Xi, B., Dolinar, E. K., and Stanfield, R. E.: The
footprints of 16 year trends of Arctic springtime cloud and radiation
properties on September sea ice retreat, J. Geophys. Res.-Atmos., 122, 2179–2193, https://doi.org/10.1002/2016JD026020,
2017. a, b
Huang, Y., Dong, X., Bailey, D. A., Holland, M. M., Xi, B., DuVivier, A. K.,
Kay, J. E., Landrum, L. L., and Deng, Y.: Thicker Clouds and Accelerated
Arctic Sea Ice Decline: The Atmosphere-Sea Ice Interactions in Spring,
Geophys. Res. Lett., 46, 6980–6989,
https://doi.org/10.1029/2019GL082791, 2019. a, b, c
Intrieri, J. M., Fairall, C. W., Shupe, M. D., Persson, P. O. G., Andreas,
E. L., Guest, P. S., and Moritz, R. E.: An annual cycle of Arctic surface
cloud forcing at SHEBA, J. Geophys. Res.-Oceans, 107, 13–14, https://doi.org/10.1029/2000JC000439,
2002. a
Kay, J., L'Ecuyer, T., Chepfer, H., Loeb, N., Morrison, A., and Cesana, G.:
Recent Advances in Arctic Cloud and Climate Research, Curr. Clim. Change
Rep., 2, 159–169, https://doi.org/10.1007/s40641-016-0051-9, 2016. a
Kay, J. E. and Gettelman, A.: Cloud influence on and response to seasonal
Arctic sea ice loss, J. Geophys. Res.-Atmos., 114, D18204,
https://doi.org/10.1029/2009JD011773, 2009. a, b, c, d
Khanal, S. and Wang, Z.: Uncertainties in MODIS-Based Cloud Liquid Water Path
Retrievals at High Latitudes Due to Mixed-Phase Clouds and Cloud Top Height
Inhomogeneity, J. Geophys. Res.-Atmos., 123,
11154–11172, https://doi.org/10.1029/2018JD028558, 2018. a, b
Klein, S. A. and Hartmann, D. L.: The Seasonal Cycle of Low Stratiform Clouds,
J. Climate, 6, 1587–1606,
https://doi.org/10.1175/1520-0442(1993)006<1587:TSCOLS>2.0.CO;2, 1993. a
Kolstad, E. W. and Bracegirdle, T. J.: Marine cold-air outbreaks in the future:
an assessment of IPCC AR4 model results for the Northern Hemisphere, Clim.
Dynam., 30, 871–885, https://doi.org/10.1007/s00382-007-0331-0, 2008. a
L'Ecuyer, T. S., Hang, Y., Matus, A. V., and Wang, Z.: Reassessing the Effect
of Cloud Type on Earth's Energy Balance in the Age of Active Spaceborne
Observations, Part I: Top of Atmosphere and Surface, J. Climate, 32,
6197–6217, https://doi.org/10.1175/JCLI-D-18-0753.1, 2019. a
Lubin, D. and Vogelmann, A.: A climatologically significant aerosol longwave
indirect effect in the Arctic, Nature, 449, 453–456,
https://doi.org/10.1038/nature04449, 2006. a
Maahn, M., Goren, T., Shupe, M. D., and de Boer, G.: Liquid Containing Clouds
at the North Slope of Alaska Demonstrate Sensitivity to Local Industrial
Aerosol Emissions, Geophys. Res. Lett., 48, e2021GL094307,
https://doi.org/10.1029/2021GL094307, 2021. a
Malavelle, F. F., Haywood, J. M., Jones, A., Gettelman, A., Clarisse, L.,
Bauduin, S., Allan, R. P., Karset, I. H. H., Kristjánsson, J. E.,
Oreopoulos, L., Cho, N., Lee, D., Bellouin, N., Boucher, O., Grosvenor,
D. P., Carslaw, K. S., Dhomse, S., Mann, G. W., Schmidt, A., Coe, H.,
Hartley, M. E., Dalvi, M., Hill, A. A., Johnson, B. T., Johnson, C. E.,
Knight, J. R., O'Connor, F. M., Partridge, D. G., Stier, P., Myhre, G.,
Platnick, S., Stephens, G. L., Takahashi, H., and Thordarson, T.: Strong
constraints on aerosol–cloud interactions from volcanic eruptions, Nature,
546, 485–491, https://doi.org/10.1038/nature22974, 2017. a
Mann, H. B. and Whitney, D. R.: On a Test of Whether one of Two Random
Variables is Stochastically Larger than the Other, Ann.
Math. Stat., 18, 50–60, https://doi.org/10.1214/aoms/1177730491, 1947. a
McCoy, I. L., Wood, R., and Fletcher, J. K.: Identifying Meteorological
Controls on Open and Closed Mesoscale Cellular Convection Associated with
Marine Cold Air Outbreaks, J. Geophys. Res.-Atmos., 122,
11678–11702, https://doi.org/0.1002/2017JD027031, 2017. a
Merk, D., Deneke, H., Pospichal, B., and Seifert, P.: Investigation of the adiabatic assumption for estimating cloud micro- and macrophysical properties from satellite and ground observations, Atmos. Chem. Phys., 16, 933–952, https://doi.org/10.5194/acp-16-933-2016, 2016. a
Michibata, T., Suzuki, K., Sato, Y., and Takemura, T.: The source of discrepancies in aerosol–cloud–precipitation interactions between GCM and A-Train retrievals, Atmos. Chem. Phys., 16, 15413–15424, https://doi.org/10.5194/acp-16-15413-2016, 2016. a, b, c
Morrison, A. L., Kay, J. E., Chepfer, H., Guzman, R., and Yettella, V.:
Isolating the Liquid Cloud Response to Recent Arctic Sea Ice Variability
Using Spaceborne Lidar Observations, J. Geophys. Res.-Atmos., 123, 473–490, https://doi.org/10.1002/2017JD027248, 2018. a, b
Painemal, D. and Zuidema, P.: Assessment of MODIS cloud effective radius and
optical thickness retrievals over the Southeast Pacific with VOCALS-REx in
situ measurements, J. Geophys. Res.-Atmos., 116, D24206,
https://doi.org/10.1029/2011JD016155, 2011. a, b
Persson, P.: Onset and end of the summer melt season over sea ice: thermal
structure and surface energy perspective from SHEBA, Clim. Dynam., 39,
1349–1371, https://doi.org/10.1007/s00382-011-1196-9, 2012. a
Peters, G. P., Nilssen, T. B., Lindholt, L., Eide, M. S., Glomsrød, S., Eide, L. I., and Fuglestvedt, J. S.: Future emissions from shipping and petroleum activities in the Arctic, Atmos. Chem. Phys., 11, 5305–5320, https://doi.org/10.5194/acp-11-5305-2011, 2011. a
Pithan, F. and Mauritsen, T.: Arctic amplification dominated by temperature
feedbacks in contemporary climate models, Nat. Geosci., 7, 181–184,
https://doi.org/10.1038/ngeo2071, 2014. a
Pithan, F., Svensson, G., Caballero, R., Chechin, D., Cronin, T., Ekman, A.,
Neggers, R., Shupe, M., Solomon, A., Tjernström, M., and Wendisch, M.: Role
of air-mass transformations in exchange between the Arctic and mid-latitudes,
Nat. Geosci., 11, 805–812, https://doi.org/10.1038/s41561-018-0234-1, 2018. a
Platnick, S. and Twomey, S.: Remote sensing the susceptibility of cloud albedo
to changes in drop concentration, Atmos. Res., 34, 85–98,
https://doi.org/10.1016/0169-8095(94)90082-5, 1994. a
Platnick, S., Meyer, K. G., King, M. D., Wind, G., Amarasinghe, N., Marchant,
B., Arnold, G. T., Zhang, Z., Hubanks, P. A., Holz, R. E., Yang, P., Ridgway,
W. L., and Riedi, J.: The MODIS Cloud Optical and Microphysical Products:
Collection 6 Updates and Examples From Terra and Aqua, IEEE T. Geosci. Remote, [data set], 55, 502–525, https://doi.org/10.1109/TGRS.2016.2610522,
2017. a, b
Quaas, J., Boucher, O., and Lohmann, U.: Constraining the total aerosol indirect effect in the LMDZ and ECHAM4 GCMs using MODIS satellite data, Atmos. Chem. Phys., 6, 947–955, https://doi.org/10.5194/acp-6-947-2006, 2006. a, b
Quaas, J., Boucher, O., Bellouin, N., and Kinne, S.: Satellite-based estimate
of the direct and indirect aerosol climate forcing, J. Geophys. Res.-Atmos., 113, D05204,
https://doi.org/10.1029/2007JD008962, 2008. a
Quaas, J., Stevens, B., Stier, P., and Lohmann, U.: Interpreting the cloud cover – aerosol optical depth relationship found in satellite data using a general circulation model, Atmos. Chem. Phys., 10, 6129–6135, https://doi.org/10.5194/acp-10-6129-2010, 2010. a
Renfrew, I. A., Barrell, C., Elvidge, A. D., Brooke, J. K., Duscha, C., King,
J. C., Kristiansen, J., Cope, T. L., Moore, G. W. K., Pickart, R. S., Reuder,
J., Sandu, I., Sergeev, D., Terpstra, A., Våge, K., and Weiss, A.: An
evaluation of surface meteorology and fluxes over the Iceland and Greenland
Seas in ERA5 reanalysis: The impact of sea ice distribution, Q. J. Roy. Meteor. Soc., 147, 691–712,
https://doi.org/0.1002/qj.3941, 2021. a
Rosenfeld, D. and Gutman, G.: Retrieving microphysical properties near the tops
of potential rain clouds by multispectral analysis of AVHRR data, Atmos.
Res., 34, 259–283, https://doi.org/10.1016/0169-8095(94)90096-5, 1994. a
Schmale, J., Arnold, S. R., Law, K. S., Thorp, T., Anenberg, S., Simpson,
W. R., Mao, J., and Pratt, K. A.: Local Arctic Air Pollution: A Neglected but
Serious Problem, Earth's Future, 6, 1385–1412,
https://doi.org/10.1029/2018EF000952, 2018. a, b
Schmale, J., Zieger, P., and Ekman, A.: Aerosols in current and future Arctic
climate, Nat. Clim. Change, 11, 95–105,
https://doi.org/10.1038/s41558-020-00969-5, 2021. a
Serreze, M. C. and Barry, R. G.: Processes and impacts of Arctic amplification:
A research synthesis, Glob. Planet. Change, 77, 85–96,
https://doi.org/10.1016/j.gloplacha.2011.03.004, 2011. a
Shupe, M. D.: Clouds at Arctic Atmospheric Observatories, Part II:
Thermodynamic Phase Characteristics, J. Appl. Meteorol. Clim., 50, 64–661, https://doi.org/10.1175/2010JAMC2468.1, 2011. a
Shupe, M. D. and Intrieri, J. M.: Cloud Radiative Forcing of the Arctic
Surface: The Influence of Cloud Properties, Surface Albedo, and Solar Zenith
Angle, J. Climate, 17, 616–628,
https://doi.org/10.1175/1520-0442(2004)017<0616:CRFOTA>2.0.CO;2, 2004. a, b
Sourdeval, O., C.-Labonnote, L., Baran, A. J., Mülmenstädt, J., and Brogniez,
G.: A methodology for simultaneous retrieval of ice and liquid water cloud
properties, Part 2: Near-global retrievals and evaluation against A-Train
products, Q. J. Roy. Meteor. Soc., 142,
3063–3081, https://doi.org/10.1002/qj.2889, 2016. a
Stevens, B. and Feingold, G.: Untangling aerosol effects on clouds and
precipitation in a buffered system, Nature, 461, 607–613,
https://doi.org/10.1038/nature08281, 2009. a
Tietze, K., Riedi, J., Stohl, A., and Garrett, T. J.: Space-based evaluation of interactions between aerosols and low-level Arctic clouds during the Spring and Summer of 2008, Atmos. Chem. Phys., 11, 3359–3373, https://doi.org/10.5194/acp-11-3359-2011, 2011. a
Toll, V., Christensen, M., Gassó, S., and Bellouin, N.: Volcano and Ship
Tracks Indicate Excessive Aerosol-Induced Cloud Water Increases in a Climate
Model, Geophys. Res. Lett., 44, 12492–12500,
https://doi.org/10.1002/2017GL075280, 2017. a
Toll, V., Christensen, M., Quaas, J., and Bellouin, N.: Weak average
liquid-cloud-water response to anthropogenic aerosols, Nature, 572, 51–55,
https://doi.org/10.1038/s41586-019-1423-9, 2019. a, b, c
Twomey, S.: The Influence of Pollution on the Shortwave Albedo of Clouds,
J. Atmos. Sci., 34, 1149–1152,
https://doi.org/10.1175/1520-0469(1977)034<1149:TIOPOT>2.0.CO;2, 1977. a
Wentz, F. J. and Meissner, T.: AMSR-E/Aqua L2B Global Swath Ocean Products
derived from Wentz Algorithm, Version 2.7, Boulder, Colorado USA, NASA
National Snow and Ice Data Center Distributed Active Archive Center, [data set],
https://doi.org/10.5067/AMSR-E/AE_OCEAN.002, 2004. a, b
Williams, A. S. and Igel, A. L.: Cloud Top Radiative Cooling Rate Drives
Non-Precipitating Stratiform Cloud Responses to Aerosol Concentration,
Geophys. Res. Lett., 48, e2021GL094740,
https://doi.org/10.1029/2021GL094740, 2021. a
Wood, R. and Hartmann, D. L.: Spatial Variability of Liquid Water Path in
Marine Low Cloud: The Importance of Mesoscale Cellular Convection, J. Climate, 19, 1748–1764, https://doi.org/10.1175/JCLI3702.1, 2006. a
Xue, H. and Feingold, G.: Large-Eddy Simulations of Trade Wind Cumuli:
Investigation of Aerosol Indirect Effects, J. Atmos.
Sci., 63, 1605–1622, https://doi.org/10.1175/JAS3706.1, 2006.
a
Zamora, L. M., Kahn, R. A., Huebert, K. B., Stohl, A., and Eckhardt, S.: A satellite-based estimate of combustion aerosol cloud microphysical effects over the Arctic Ocean, Atmos. Chem. Phys., 18, 14949–14964, https://doi.org/10.5194/acp-18-14949-2018, 2018. a
Zhang, Z. and Platnick, S.: An assessment of differences between cloud
effective particle radius retrievals for marine water clouds from three MODIS
spectral bands, J. Geophys. Res.-Atmos., 116, D20215,
https://doi.org/10.1029/2011JD016216, 2011. a
Zhao, C. and Garrett, T. J.: Effects of Arctic haze on surface cloud radiative
forcing, Geophys. Res. Lett., 42, 557–564,
https://doi.org/10.1002/2014GL062015, 2015. a
Zuidema, P., Westwater, E. R., Fairall, C., and Hazen, D.: Ship-based liquid
water path estimates in marine stratocumulus, J. Geophys. Res.-Atmos., 110, D20206,
https://doi.org/10.1029/2005JD005833, 2005. a
Short summary
Clouds are important to the Arctic surface energy budget, but the impact of aerosols on their properties is largely uncertain. This work shows that the response of liquid water path to cloud droplet number increases is strongly dependent on lower tropospheric stability (LTS), with weaker cooling effects in polluted clouds and at high LTS. LTS is projected to decrease in a warmer Arctic, reducing the cooling effect of aerosols and producing a positive, aerosol-dependent cloud feedback.
Clouds are important to the Arctic surface energy budget, but the impact of aerosols on their...
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