Articles | Volume 22, issue 17
https://doi.org/10.5194/acp-22-11305-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-11305-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
02 Sep 2022
Research article |
| 02 Sep 2022
| 02 Sep 2022
Experimental study on the evolution of droplet size distribution during the fog life cycle
CNRM, Université de Toulouse, Météo-France, CNRS, Toulouse, France
Frédéric Burnet
CNRM, Université de Toulouse, Météo-France, CNRS, Toulouse, France
Cyrielle Denjean
CNRM, Université de Toulouse, Météo-France, CNRS, Toulouse, France
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Marie Mazoyer, Frédéric Burnet, Cyrielle Denjean, Gregory C. Roberts, Martial Haeffelin, Jean-Charles Dupont, and Thierry Elias
Atmos. Chem. Phys., 19, 4323–4344, https://doi.org/10.5194/acp-19-4323-2019, https://doi.org/10.5194/acp-19-4323-2019, 2019
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In situ microphysical measurements collected during 23 fog events at SIRTA (south of Paris) are examined here. An original iterative method based on the κ-Köhler theory has been used to compute statistics of their activation properties. Useful information is provided to constrain and validate numerical simulations. The paper demonstrates that supersaturation encountered in these fogs is too low to observe a correlation between concentrations of aerosols > 200 nm and droplet concentrations.
Marie Mazoyer, Christine Lac, Odile Thouron, Thierry Bergot, Valery Masson, and Luc Musson-Genon
Atmos. Chem. Phys., 17, 13017–13035, https://doi.org/10.5194/acp-17-13017-2017, https://doi.org/10.5194/acp-17-13017-2017, 2017
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Large eddy simulations of a radiation fog event occurring during the ParisFog experiment have been studied to analyze the impact of the dynamics on the fog life cycle. They included a sophisticated microphysical scheme, the drag effect of a trees barrier and deposition on vegetation. The blocking effect of the trees induces elevated fog formation and limits cooling and cloud water production. The deposition process was found to exert the most significant impact on the fog prediction.
M. Mazoyer, F. Burnet, G. C. Roberts, M. Haeffelin, J.-C Dupont, and T. Elias
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-103, https://doi.org/10.5194/acp-2016-103, 2016
Preprint withdrawn
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Comprehensive field campaigns dedicated to fog life cycle observation were conducted during the winters of 2010–2013 at the SIRTA observatory in the suburb of Paris. The objective of this paper is to evaluate the impact of aerosol particles on the fog microphysics
through an original method. We conclude that the actual supersaturations reached during these fog episodes are too low and no simultaneous increase of aerosols (D > 200 nm) and droplet concentrations can be observed.
Maud Leriche, Pierre Tulet, Laurent Deguillaume, Frédéric Burnet, Aurélie Colomb, Agnès Borbon, Corinne Jambert, Valentin Duflot, Stéphan Houdier, Jean-Luc Jaffrezo, Mickaël Vaïtilingom, Pamela Dominutti, Manon Rocco, Camille Mouchel-Vallon, Samira El Gdachi, Maxence Brissy, Maroua Fathalli, Nicolas Maury, Bert Verreyken, Crist Amelynck, Niels Schoon, Valérie Gros, Jean-Marc Pichon, Mickael Ribeiro, Eric Pique, Emmanuel Leclerc, Thierry Bourrianne, Axel Roy, Eric Moulin, Joël Barrie, Jean-Marc Metzger, Guillaume Péris, Christian Guadagno, Chatrapatty Bhugwant, Jean-Mathieu Tibere, Arnaud Tournigand, Evelyn Freney, Karine Sellegri, Anne-Marie Delort, Pierre Amato, Muriel Joly, Jean-Luc Baray, Pascal Renard, Angelica Bianco, Anne Réchou, and Guillaume Payen
Atmos. Chem. Phys., 24, 4129–4155, https://doi.org/10.5194/acp-24-4129-2024, https://doi.org/10.5194/acp-24-4129-2024, 2024
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Aerosol particles in the atmosphere play a key role in climate change and air pollution. A large number of aerosol particles are formed from the oxidation of volatile organic compounds (VOCs and secondary organic aerosols – SOA). An important field campaign was organized on Réunion in March–April 2019 to understand the formation of SOA in a tropical atmosphere mostly influenced by VOCs emitted by forest and in the presence of clouds. This work synthesizes the results of this campaign.
Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Thierry Bourrianne, Véronique Pont, François Gheusi, and Emmanuel Leclerc
Atmos. Chem. Phys., 24, 1801–1824, https://doi.org/10.5194/acp-24-1801-2024, https://doi.org/10.5194/acp-24-1801-2024, 2024
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At a French high-altitude site, where many complex interactions between black carbon (BC), radiation, clouds and snow impact climate, 2 years of refractive BC (rBC) and aerosol optical and microphysical measurements have been made. We observed strong seasonal rBC properties variations, with an enhanced absorption in summer compared to winter. The combination of rBC emission sources, transport pathways, atmospheric dynamics and chemical processes explains the rBC light absorption seasonality.
Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Véronique Pont, Mathilde Arnaud, Thierry Bourrianne, Maria Dias Alves, and Eric Gardrat
EGUsphere, https://doi.org/10.5194/egusphere-2024-47, https://doi.org/10.5194/egusphere-2024-47, 2024
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The three most widely used techniques for measuring black carbon (BC) has been deployed continuously for two years at a french high-altitude measurement station. Despite a similar temporal variation in the BC load, we found significant biases by up to a factor 8 between the three instruments. This study raises questions about the relevance of using these instruments for specific background sites, as well as the processing of their data, which can vary according to atmospheric conditions.
Simone T. Andersen, Max R. McGillen, Chaoyang Xue, Tobias Seubert, Patrick Dewald, Gunther N. T. E. Türk, Jan Schuladen, Cyrielle Denjean, Jean-Claude Etienne, Olivier Garrouste, Marina Jamar, Sergio Harb, Manuela Cirtog, Vincent Michoud, Mathieu Cazaunau, Antonin Bergé, Christopher Cantrell, Sebastien Dusanter, Bénédicte Picquet-Varrault, Alexandre Kukui, Abdelwahid Mellouki, Lucy J. Carpenter, Jos Lelieveld, and John N. Crowley
EGUsphere, https://doi.org/10.5194/egusphere-2023-2848, https://doi.org/10.5194/egusphere-2023-2848, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Through measurements of various trace gases in a sub-urban forest near Paris in the summer of 2022 we were able to gain insight into the sources and sinks of NOx (NO+NO2) with a special focus on their nighttime chemical/physical loss processes. NO was observed as a result of nighttime soil emissions when ozone levels were strongly depleted by deposition. NO oxidation products were not observed at night indicating that soil and/or foliar surfaces are an efficient sink of reactive nitrogen.
Cheikh Dione, Martial Haeffelin, Frédéric Burnet, Christine Lac, Guylaine Canut, Julien Delanoë, Jean-Charles Dupont, Susana Jorquera, Pauline Martinet, Jean-François Ribaud, and Felipe Toledo
Atmos. Chem. Phys., 23, 15711–15731, https://doi.org/10.5194/acp-23-15711-2023, https://doi.org/10.5194/acp-23-15711-2023, 2023
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This paper documents the role of thermodynamics and turbulence in the fog life cycle over southwestern France. It is based on a unique dataset collected during the SOFOG3D field campaign in autumn and winter 2019–2020. The paper gives a threshold for turbulence driving the different phases of the fog life cycle and the role of advection in the night-time dissipation of fog. The results can be operationalised to nowcast fog and improve short-range forecasts in numerical weather prediction models.
Lucas Pailler, Laurent Deguillaume, Hélène Lavanant, Isabelle Schmitz, Marie Hubert, Edith Nicol, Micakël Ribeiro, Jean-Marc Pichon, Mickaël Vaïtilingom, Pamela Dominutti, Frédéric Burnet, Pierre Tulet, Maud Leriche, and Angelica Bianco
EGUsphere, https://doi.org/10.5194/egusphere-2023-2706, https://doi.org/10.5194/egusphere-2023-2706, 2023
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The composition of cloud water dissolved organic matter has been investigated through non-targeted high resolution mass spectrometry only on few samples, collected in the Northern hemisphere (NH). In this work, the chemical composition of samples collected at Reunion Island (SH) is investigated and compared to samples collected at the puy de Dôme (NH). Sampling, analysis and data treatment with the same methodology produced a unique dataset for investigating the molecular composition of clouds.
Lambert Delbeke, Chien Wang, Pierre Tulet, Cyrielle Denjean, Maurin Zouzoua, Nicolas Maury, and Adrien Deroubaix
Atmos. Chem. Phys., 23, 13329–13354, https://doi.org/10.5194/acp-23-13329-2023, https://doi.org/10.5194/acp-23-13329-2023, 2023
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Low-level stratiform clouds (LLSCs) appear frequently over southern West Africa during the West African monsoon. Local and remote aerosol sources (biomass burning aerosols from central Africa) play a significant role in the LLSC life cycle. Based on measurements by the DACCIWA campaign, large-eddy simulation (LES) was conducted using different aerosol scenarios. The results show that both indirect and semi-direct effects can act individually or jointly to influence the life cycles of LLSCs.
Pragya Vishwakarma, Julien Delanoë, Susana Jorquera, Pauline Martinet, Frederic Burnet, Alistair Bell, and Jean-Charles Dupont
Atmos. Meas. Tech., 16, 1211–1237, https://doi.org/10.5194/amt-16-1211-2023, https://doi.org/10.5194/amt-16-1211-2023, 2023
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Cloud observations are necessary to characterize the cloud properties at local and global scales. The observations must be translated to cloud geophysical parameters. This paper presents the estimation of liquid water content (LWC) using radar and microwave radiometer (MWR) measurements. Liquid water path from MWR scales LWC and retrieves the scaling factor (ln a). The retrievals are compared with in situ observations. A climatology of ln a is built to estimate LWC using only radar information.
Alistair Bell, Pauline Martinet, Olivier Caumont, Frédéric Burnet, Julien Delanoë, Susana Jorquera, Yann Seity, and Vinciane Unger
Atmos. Meas. Tech., 15, 5415–5438, https://doi.org/10.5194/amt-15-5415-2022, https://doi.org/10.5194/amt-15-5415-2022, 2022
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Cloud radars and microwave radiometers offer the potential to improve fog forecasts when assimilated into a high-resolution model. As this process can be complex, a retrieval of model variables is sometimes made as a first step. In this work, results from a 1D-Var algorithm for the retrieval of temperature, humidity and cloud liquid water content are presented. The algorithm is applied first to a synthetic dataset and then to a dataset of real measurements from a recent field campaign.
Michael John Weston, Stuart John Piketh, Frédéric Burnet, Stephen Broccardo, Cyrielle Denjean, Thierry Bourrianne, and Paola Formenti
Atmos. Chem. Phys., 22, 10221–10245, https://doi.org/10.5194/acp-22-10221-2022, https://doi.org/10.5194/acp-22-10221-2022, 2022
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An aerosol-aware microphysics scheme is evaluated for fog cases in Namibia. AEROCLO-sA campaign observations are used to access and parameterise the model. The model cloud condensation nuclei activation is lower than the observations. The scheme is designed for clouds with updrafts, while fog typically forms in stable conditions. A pseudo updraft speed assigned to the lowest model levels helps achieve more realistic cloud droplet number concentration and size distribution in the model.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Peter Knippertz, Andreas H. Fink, Anneke Batenburg, Joel Brito, Cyrielle Denjean, Cheikh Dione, Régis Dupuy, Valerian Hahn, Norbert Kalthoff, Fabienne Lohou, Alfons Schwarzenboeck, Guillaume Siour, Paolo Tuccella, and Christiane Voigt
Atmos. Chem. Phys., 22, 3251–3273, https://doi.org/10.5194/acp-22-3251-2022, https://doi.org/10.5194/acp-22-3251-2022, 2022
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During the summer monsoon in West Africa, pollutants emitted in urbanized areas modify cloud cover and precipitation patterns. We analyze these patterns with the WRF-CHIMERE model, integrating the effects of aerosols on meteorology, based on the numerous observations provided by the Dynamics-Aerosol-Climate-Interactions campaign. This study adds evidence to recent findings that increased pollution levels in West Africa delay the breakup time of low-level clouds and reduce precipitation.
Pamela A. Dominutti, Pascal Renard, Mickaël Vaïtilingom, Angelica Bianco, Jean-Luc Baray, Agnès Borbon, Thierry Bourianne, Frédéric Burnet, Aurélie Colomb, Anne-Marie Delort, Valentin Duflot, Stephan Houdier, Jean-Luc Jaffrezo, Muriel Joly, Martin Leremboure, Jean-Marc Metzger, Jean-Marc Pichon, Mickaël Ribeiro, Manon Rocco, Pierre Tulet, Anthony Vella, Maud Leriche, and Laurent Deguillaume
Atmos. Chem. Phys., 22, 505–533, https://doi.org/10.5194/acp-22-505-2022, https://doi.org/10.5194/acp-22-505-2022, 2022
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We present here the results obtained during an intensive field campaign conducted in March to April 2019 in Reunion. Our study integrates a comprehensive chemical and microphysical characterization of cloud water. Our investigations reveal that air mass history and cloud microphysical properties do not fully explain the variability observed in their chemical composition. This highlights the complexity of emission sources, multiphasic exchanges, and transformations in clouds.
Sebastian Düsing, Albert Ansmann, Holger Baars, Joel C. Corbin, Cyrielle Denjean, Martin Gysel-Beer, Thomas Müller, Laurent Poulain, Holger Siebert, Gerald Spindler, Thomas Tuch, Birgit Wehner, and Alfred Wiedensohler
Atmos. Chem. Phys., 21, 16745–16773, https://doi.org/10.5194/acp-21-16745-2021, https://doi.org/10.5194/acp-21-16745-2021, 2021
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The work deals with optical properties of aerosol particles in dried and atmospheric states. Based on two measurement campaigns in the rural background of central Europe, different measurement approaches were compared with each other, such as modeling based on Mie theory and direct in situ or remote sensing measurements. Among others, it was shown that the aerosol extinction-to-backscatter ratio is relative humidity dependent, and refinement with respect to the model input parameters is needed.
Pauline Martinet, Domenico Cimini, Frédéric Burnet, Benjamin Ménétrier, Yann Michel, and Vinciane Unger
Atmos. Meas. Tech., 13, 6593–6611, https://doi.org/10.5194/amt-13-6593-2020, https://doi.org/10.5194/amt-13-6593-2020, 2020
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Each year large human and economical losses are due to fog episodes. However, fog forecasts remain quite inaccurate, partly due to a lack of observations in the atmospheric boundary layer. The benefit of ground-based microwave radiometers has been investigated and has demonstrated their capability of significantly improving the initial state of temperature and liquid water content profiles in current numerical weather prediction models, paving the way for improved fog forecasts in the future.
Cyrielle Denjean, Thierry Bourrianne, Frederic Burnet, Marc Mallet, Nicolas Maury, Aurélie Colomb, Pamela Dominutti, Joel Brito, Régis Dupuy, Karine Sellegri, Alfons Schwarzenboeck, Cyrille Flamant, and Peter Knippertz
Atmos. Chem. Phys., 20, 4735–4756, https://doi.org/10.5194/acp-20-4735-2020, https://doi.org/10.5194/acp-20-4735-2020, 2020
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This paper presents aircraft measurements of aerosol optical properties over southern West Africa. We show that aerosol optical properties in the boundary layer were dominated by a persistent biomass burning loading from the Southern Hemisphere. Biomass burning aerosols were more light absorbing that those previously measured in other areas (Amazonia, North America). Our study suggests that lens-coated black carbon particles were the dominant absorber for these biomass burning aerosols.
Sophie L. Haslett, Jonathan W. Taylor, Mathew Evans, Eleanor Morris, Bernhard Vogel, Alima Dajuma, Joel Brito, Anneke M. Batenburg, Stephan Borrmann, Johannes Schneider, Christiane Schulz, Cyrielle Denjean, Thierry Bourrianne, Peter Knippertz, Régis Dupuy, Alfons Schwarzenböck, Daniel Sauer, Cyrille Flamant, James Dorsey, Ian Crawford, and Hugh Coe
Atmos. Chem. Phys., 19, 15217–15234, https://doi.org/10.5194/acp-19-15217-2019, https://doi.org/10.5194/acp-19-15217-2019, 2019
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Three aircraft datasets from the DACCIWA campaign in summer 2016 are used here to show there is a background mass of pollution present in the lower atmosphere in southern West Africa. We suggest that this likely comes from biomass burning in central and southern Africa, which has been carried into the region over the Atlantic Ocean. This would have a negative health impact on populations living near the coast and may alter the impact of growing city emissions on cloud formation and the monsoon.
Valentin Duflot, Pierre Tulet, Olivier Flores, Christelle Barthe, Aurélie Colomb, Laurent Deguillaume, Mickael Vaïtilingom, Anne Perring, Alex Huffman, Mark T. Hernandez, Karine Sellegri, Ellis Robinson, David J. O'Connor, Odessa M. Gomez, Frédéric Burnet, Thierry Bourrianne, Dominique Strasberg, Manon Rocco, Allan K. Bertram, Patrick Chazette, Julien Totems, Jacques Fournel, Pierre Stamenoff, Jean-Marc Metzger, Mathilde Chabasset, Clothilde Rousseau, Eric Bourrianne, Martine Sancelme, Anne-Marie Delort, Rachel E. Wegener, Cedric Chou, and Pablo Elizondo
Atmos. Chem. Phys., 19, 10591–10618, https://doi.org/10.5194/acp-19-10591-2019, https://doi.org/10.5194/acp-19-10591-2019, 2019
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The Forests gAses aeRosols Clouds Exploratory (FARCE) campaign was conducted in March–April 2015 on the tropical island of La Réunion. For the first time, several scientific teams from different disciplines collaborated to provide reference measurements and characterization of La Réunion vegetation, volatile organic compounds (VOCs), biogenic VOCs (BVOCs), (bio)aerosols and composition of clouds, with a strong focus on the Maïdo mount slope area.
Jonathan W. Taylor, Sophie L. Haslett, Keith Bower, Michael Flynn, Ian Crawford, James Dorsey, Tom Choularton, Paul J. Connolly, Valerian Hahn, Christiane Voigt, Daniel Sauer, Régis Dupuy, Joel Brito, Alfons Schwarzenboeck, Thierry Bourriane, Cyrielle Denjean, Phil Rosenberg, Cyrille Flamant, James D. Lee, Adam R. Vaughan, Peter G. Hill, Barbara Brooks, Valéry Catoire, Peter Knippertz, and Hugh Coe
Atmos. Chem. Phys., 19, 8503–8522, https://doi.org/10.5194/acp-19-8503-2019, https://doi.org/10.5194/acp-19-8503-2019, 2019
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Low-level clouds cover a wide area of southern West Africa (SWA) and play an important role in the region's climate, reflecting sunlight away from the surface. We performed aircraft measurements of aerosols and clouds over SWA during the 2016 summer monsoon and found pollution, and polluted clouds, across the whole region. Smoke from biomass burning in Central Africa is transported to West Africa, causing a polluted background which limits the effect of local pollution on cloud properties.
Marie Mazoyer, Frédéric Burnet, Cyrielle Denjean, Gregory C. Roberts, Martial Haeffelin, Jean-Charles Dupont, and Thierry Elias
Atmos. Chem. Phys., 19, 4323–4344, https://doi.org/10.5194/acp-19-4323-2019, https://doi.org/10.5194/acp-19-4323-2019, 2019
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In situ microphysical measurements collected during 23 fog events at SIRTA (south of Paris) are examined here. An original iterative method based on the κ-Köhler theory has been used to compute statistics of their activation properties. Useful information is provided to constrain and validate numerical simulations. The paper demonstrates that supersaturation encountered in these fogs is too low to observe a correlation between concentrations of aerosols > 200 nm and droplet concentrations.
María José Granados-Muñoz, Michael Sicard, Roberto Román, Jose Antonio Benavent-Oltra, Rubén Barragán, Gerard Brogniez, Cyrielle Denjean, Marc Mallet, Paola Formenti, Benjamín Torres, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 19, 523–542, https://doi.org/10.5194/acp-19-523-2019, https://doi.org/10.5194/acp-19-523-2019, 2019
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The influence of mineral dust in the direct radiative effect is affected by a large uncertainty. This study investigates mineral dust radiative properties during an episode affecting southern Spain in June 2013 by using remote sensors and data collected on board an aircraft to feed a radiative transfer model. The study reveals the complexity of parameterizing these models, as characterizing mineral dust is still quite challenging, and the need for accurate mineral dust measurements.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Joel Brito, Cyrielle Denjean, Volker Dreiling, Andreas Fink, Corinne Jambert, Norbert Kalthoff, Peter Knippertz, Russ Ladkin, Sylvain Mailler, Marlon Maranan, Federica Pacifico, Bruno Piguet, Guillaume Siour, and Solène Turquety
Atmos. Chem. Phys., 19, 473–497, https://doi.org/10.5194/acp-19-473-2019, https://doi.org/10.5194/acp-19-473-2019, 2019
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This article presents a detailed analysis of anthropogenic and biomass burning pollutants over the Gulf of Guinea coastal region, using observations from the DACCIWA field campaign and modeling. The novelty is that we focus on how these two pollution sources are mixed and transported further inland. We show that during the day pollutants are accumulated along the coastline and transported northward as soon as the daytime convection in the atmospheric boundary layer ceases (16:00 UTC).
Cyrille Flamant, Adrien Deroubaix, Patrick Chazette, Joel Brito, Marco Gaetani, Peter Knippertz, Andreas H. Fink, Gaëlle de Coetlogon, Laurent Menut, Aurélie Colomb, Cyrielle Denjean, Rémi Meynadier, Philip Rosenberg, Regis Dupuy, Pamela Dominutti, Jonathan Duplissy, Thierry Bourrianne, Alfons Schwarzenboeck, Michel Ramonet, and Julien Totems
Atmos. Chem. Phys., 18, 12363–12389, https://doi.org/10.5194/acp-18-12363-2018, https://doi.org/10.5194/acp-18-12363-2018, 2018
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This work sheds light on the complex mechanisms by which coastal shallow circulations distribute atmospheric pollutants over the densely populated southern West African region. Pollutants of concern are anthropogenic emissions from coastal cities, as well as biomass burning aerosol and dust associated with long-range transport. The complex vertical distribution of aerosols over coastal southern West Africa is investigated using airborne observations and numerical simulations.
Daniela Meloni, Alcide di Sarra, Gérard Brogniez, Cyrielle Denjean, Lorenzo De Silvestri, Tatiana Di Iorio, Paola Formenti, José L. Gómez-Amo, Julian Gröbner, Natalia Kouremeti, Giuliano Liuzzi, Marc Mallet, Giandomenico Pace, and Damiano M. Sferlazzo
Atmos. Chem. Phys., 18, 4377–4401, https://doi.org/10.5194/acp-18-4377-2018, https://doi.org/10.5194/acp-18-4377-2018, 2018
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This study examines how different aerosol optical properties determine the dust longwave radiative effects at the surface, in the atmosphere and at the top of the atmosphere, based on the combination of remote sensing and in situ observations from the ground, from airborne sensors, and from space, by means of radiative transfer modelling. The closure experiment is based on longwave irradiances and spectral brightness temperatures measured during the 2013 ChArMEx–ADRIMED campaign at Lampedusa.
Jean-Baptiste Renard, François Dulac, Pierre Durand, Quentin Bourgeois, Cyrielle Denjean, Damien Vignelles, Benoit Couté, Matthieu Jeannot, Nicolas Verdier, and Marc Mallet
Atmos. Chem. Phys., 18, 3677–3699, https://doi.org/10.5194/acp-18-3677-2018, https://doi.org/10.5194/acp-18-3677-2018, 2018
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A campaign was performed in the summer of 2013 above the Mediterranean basin, including in situ counting balloon-borne aerosol measurements (LOAC), for the detection of mineral dust. Three modes in the dust particle volume size distributions were detected, at roughly 0.2, 4, and 30 mm. Particles larger than 40 mm were often observed. They were lifted several days before and their persistence after transport over long distances is in conflict with dust sedimentation calculations.
Joel Brito, Evelyn Freney, Pamela Dominutti, Agnes Borbon, Sophie L. Haslett, Anneke M. Batenburg, Aurelie Colomb, Regis Dupuy, Cyrielle Denjean, Frederic Burnet, Thierry Bourriane, Adrien Deroubaix, Karine Sellegri, Stephan Borrmann, Hugh Coe, Cyrille Flamant, Peter Knippertz, and Alfons Schwarzenboeck
Atmos. Chem. Phys., 18, 757–772, https://doi.org/10.5194/acp-18-757-2018, https://doi.org/10.5194/acp-18-757-2018, 2018
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This work focuses on sources of submicron aerosol particles over southern West Africa (SWA). Results have shown that isoprene, a gas-phase compound of biogenic origin, is responsible for roughly 25 % of the organic aerosol (OA) loading, under most background or urban plumes alike. This fraction represents a lower estimate from the biogenic contribution in this fairly polluted region. This work sheds light upon the role of anthropogenic and biogenic emissions on the pollution burden over SWA.
Jose A. Benavent-Oltra, Roberto Román, María J. Granados-Muñoz, Daniel Pérez-Ramírez, Pablo Ortiz-Amezcua, Cyrielle Denjean, Anton Lopatin, Hassan Lyamani, Benjamin Torres, Juan L. Guerrero-Rascado, David Fuertes, Oleg Dubovik, Anatoli Chaikovsky, Francisco J. Olmo, Marc Mallet, and Lucas Alados-Arboledas
Atmos. Meas. Tech., 10, 4439–4457, https://doi.org/10.5194/amt-10-4439-2017, https://doi.org/10.5194/amt-10-4439-2017, 2017
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In this study, vertical profiles and column integrated aerosol properties retrieved by GRASP (Generalized Retrieval of Atmosphere and Surface Properties) algorithm are evaluated with in situ airborne measurements made during the ChArMEx-ADRIMED field campaign in summer 2013. Differences between GRASP retrievals and airborne extinction profiles are in the range of 15 to 30 %. Also, the total volume concentration differences between in situ data and GRASP retrieval ranges from 15 to 36 %.
Marie Mazoyer, Christine Lac, Odile Thouron, Thierry Bergot, Valery Masson, and Luc Musson-Genon
Atmos. Chem. Phys., 17, 13017–13035, https://doi.org/10.5194/acp-17-13017-2017, https://doi.org/10.5194/acp-17-13017-2017, 2017
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Large eddy simulations of a radiation fog event occurring during the ParisFog experiment have been studied to analyze the impact of the dynamics on the fog life cycle. They included a sophisticated microphysical scheme, the drag effect of a trees barrier and deposition on vegetation. The blocking effect of the trees induces elevated fog formation and limits cooling and cloud water production. The deposition process was found to exert the most significant impact on the fog prediction.
Pierre Tulet, Andréa Di Muro, Aurélie Colomb, Cyrielle Denjean, Valentin Duflot, Santiago Arellano, Brice Foucart, Jérome Brioude, Karine Sellegri, Aline Peltier, Alessandro Aiuppa, Christelle Barthe, Chatrapatty Bhugwant, Soline Bielli, Patrice Boissier, Guillaume Boudoire, Thierry Bourrianne, Christophe Brunet, Fréderic Burnet, Jean-Pierre Cammas, Franck Gabarrot, Bo Galle, Gaetano Giudice, Christian Guadagno, Fréderic Jeamblu, Philippe Kowalski, Jimmy Leclair de Bellevue, Nicolas Marquestaut, Dominique Mékies, Jean-Marc Metzger, Joris Pianezze, Thierry Portafaix, Jean Sciare, Arnaud Tournigand, and Nicolas Villeneuve
Atmos. Chem. Phys., 17, 5355–5378, https://doi.org/10.5194/acp-17-5355-2017, https://doi.org/10.5194/acp-17-5355-2017, 2017
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The STRAP campaign was conducted in 2015 to investigate the volcanic plumes of Piton de La Fournaise (La Réunion, France). For the first time, measurements were conducted at the local (near the vent) and regional scales around the island. The STRAP 2015 campaign gave a unique set of multi-disciplinary data that can now be used by modellers to improve the numerical parameterisations of the physical and chemical evolution of the volcanic plumes.
M. Mazoyer, F. Burnet, G. C. Roberts, M. Haeffelin, J.-C Dupont, and T. Elias
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-103, https://doi.org/10.5194/acp-2016-103, 2016
Preprint withdrawn
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Comprehensive field campaigns dedicated to fog life cycle observation were conducted during the winters of 2010–2013 at the SIRTA observatory in the suburb of Paris. The objective of this paper is to evaluate the impact of aerosol particles on the fog microphysics
through an original method. We conclude that the actual supersaturations reached during these fog episodes are too low and no simultaneous increase of aerosols (D > 200 nm) and droplet concentrations can be observed.
Stefanie Augustin-Bauditz, Heike Wex, Cyrielle Denjean, Susan Hartmann, Johannes Schneider, Susann Schmidt, Martin Ebert, and Frank Stratmann
Atmos. Chem. Phys., 16, 5531–5543, https://doi.org/10.5194/acp-16-5531-2016, https://doi.org/10.5194/acp-16-5531-2016, 2016
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In this study, we mixed a pure mineral dust sample with ice active biological material and quantified the immersion freezing behavior of the resulting particles utilizing the Leipzig Aerosol Cloud Interaction Simulator (LACIS). Furthermore, we used different methods to investigate the mixing state of our generated aerosol.
We found that internally mixed particles, containing ice active biological material, follow the ice nucleation behavior observed for the pure biological particles.
C. Denjean, F. Cassola, A. Mazzino, S. Triquet, S. Chevaillier, N. Grand, T. Bourrianne, G. Momboisse, K. Sellegri, A. Schwarzenbock, E. Freney, M. Mallet, and P. Formenti
Atmos. Chem. Phys., 16, 1081–1104, https://doi.org/10.5194/acp-16-1081-2016, https://doi.org/10.5194/acp-16-1081-2016, 2016
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This study investigates the size distribution, chemical composition, and optical properties of Saharan mineral dust transported over the western Mediterranean using in situ measurements collected from aircraft. Their variability due to altitude, time of transport, and mixing rate with pollution particles are discussed. We found moderate light absorption of the dust plumes even in the presence of pollution particles and the persistence of large dust particles after transport in the Mediterranean.
M. Mallet, F. Dulac, P. Formenti, P. Nabat, J. Sciare, G. Roberts, J. Pelon, G. Ancellet, D. Tanré, F. Parol, C. Denjean, G. Brogniez, A. di Sarra, L. Alados-Arboledas, J. Arndt, F. Auriol, L. Blarel, T. Bourrianne, P. Chazette, S. Chevaillier, M. Claeys, B. D'Anna, Y. Derimian, K. Desboeufs, T. Di Iorio, J.-F. Doussin, P. Durand, A. Féron, E. Freney, C. Gaimoz, P. Goloub, J. L. Gómez-Amo, M. J. Granados-Muñoz, N. Grand, E. Hamonou, I. Jankowiak, M. Jeannot, J.-F. Léon, M. Maillé, S. Mailler, D. Meloni, L. Menut, G. Momboisse, J. Nicolas, T. Podvin, V. Pont, G. Rea, J.-B. Renard, L. Roblou, K. Schepanski, A. Schwarzenboeck, K. Sellegri, M. Sicard, F. Solmon, S. Somot, B Torres, J. Totems, S. Triquet, N. Verdier, C. Verwaerde, F. Waquet, J. Wenger, and P. Zapf
Atmos. Chem. Phys., 16, 455–504, https://doi.org/10.5194/acp-16-455-2016, https://doi.org/10.5194/acp-16-455-2016, 2016
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The aim of this article is to present an experimental campaign over the Mediterranean focused on aerosol-radiation measurements and modeling. Results indicate an important atmospheric loading associated with a moderate absorbing ability of mineral dust. Observations suggest a complex vertical structure and size distributions characterized by large aerosols within dust plumes. The radiative effect is highly variable, with negative forcing over the Mediterranean and positive over northern Africa.
G. Guyot, C. Gourbeyre, G. Febvre, V. Shcherbakov, F. Burnet, J.-C. Dupont, K. Sellegri, and O. Jourdan
Atmos. Meas. Tech., 8, 4347–4367, https://doi.org/10.5194/amt-8-4347-2015, https://doi.org/10.5194/amt-8-4347-2015, 2015
C. Rose, K. Sellegri, E. Freney, R. Dupuy, A. Colomb, J.-M. Pichon, M. Ribeiro, T. Bourianne, F. Burnet, and A. Schwarzenboeck
Atmos. Chem. Phys., 15, 10203–10218, https://doi.org/10.5194/acp-15-10203-2015, https://doi.org/10.5194/acp-15-10203-2015, 2015
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In the present paper we report airborne measurements of new particle formation (NPF) above the Mediterranean Sea (HYMEX campaign). We show that NPF occurs over large areas above the sea, but the process is clearly promoted at high altitude, above 1000m, i.e. frequently in the free troposphere. NPF also seems to be mainly influenced by local processes occurring above the sea. After their formation, particles slowly grow at high altitude while not being greatly depleted or affected by coagulation.
T. Elias, J.-C. Dupont, E. Hammer, C. R. Hoyle, M. Haeffelin, F. Burnet, and D. Jolivet
Atmos. Chem. Phys., 15, 6605–6623, https://doi.org/10.5194/acp-15-6605-2015, https://doi.org/10.5194/acp-15-6605-2015, 2015
C. Denjean, P. Formenti, B. Picquet-Varrault, M. Camredon, E. Pangui, P. Zapf, Y. Katrib, C. Giorio, A. Tapparo, B. Temime-Roussel, A. Monod, B. Aumont, and J. F. Doussin
Atmos. Chem. Phys., 15, 883–897, https://doi.org/10.5194/acp-15-883-2015, https://doi.org/10.5194/acp-15-883-2015, 2015
O. Geoffroy, A. P. Siebesma, and F. Burnet
Atmos. Chem. Phys., 14, 10897–10909, https://doi.org/10.5194/acp-14-10897-2014, https://doi.org/10.5194/acp-14-10897-2014, 2014
E. Hammer, M. Gysel, G. C. Roberts, T. Elias, J. Hofer, C. R. Hoyle, N. Bukowiecki, J.-C. Dupont, F. Burnet, U. Baltensperger, and E. Weingartner
Atmos. Chem. Phys., 14, 10517–10533, https://doi.org/10.5194/acp-14-10517-2014, https://doi.org/10.5194/acp-14-10517-2014, 2014
Related subject area
Subject: Clouds and Precipitation | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Thermodynamic and cloud evolution in a cold-air outbreak during HALO-(AC)3: quasi-Lagrangian observations compared to the ERA5 and CARRA reanalyses
Powering aircraft with 100 % sustainable aviation fuel reduces ice crystals in contrails
Supercooled liquid water clouds observed over Dome C, Antarctica: temperature sensitivity and cloud radiative forcing
Role of thermodynamic and turbulence processes on the fog life cycle during SOFOG3D experiment
Characterizing the near-global cloud vertical structures over land using high-resolution radiosonde measurements
Lifecycle of Updrafts and Mass Flux in Isolated Deep Convection over the Amazon Rainforest: Insights from Cell Tracking
Differences in microphysical properties of cirrus at high and mid-latitudes
Sub-cloud rain evaporation in the North Atlantic winter trade winds derived by pairing isotopic data with a bin-resolved microphysical model
Overview and statistical analysis of boundary layer clouds and precipitation over the western North Atlantic Ocean
A set of methods to evaluate the below-cloud evaporation effect on local precipitation isotopic composition: a case study for Xi'an, China
Earth-system-model evaluation of cloud and precipitation occurrence for supercooled and warm clouds over the Southern Ocean's Macquarie Island
Pollution slightly enhances atmospheric cooling by low-level clouds in tropical West Africa
Investigating an indirect aviation effect on mid-latitude cirrus clouds – linking lidar-derived optical properties to in situ measurements
Investigating the vertical extent and short-wave radiative effects of the ice phase in Arctic summertime low-level clouds
Microphysical and thermodynamic phase analyses of Arctic low-level clouds measured above the sea ice and the open ocean in spring and summer
Aircraft observations of gravity wave activity and turbulence in the tropical tropopause layer: prevalence, influence on cirrus clouds, and comparison with global storm-resolving models
Influence of air mass origin on microphysical properties of low-level clouds in a subarctic environment
Sensitivity of convectively driven tropical tropopause cirrus properties to ice habits in high-resolution simulations
Upper-tropospheric slightly ice-subsaturated regions: frequency of occurrence and statistical evidence for the appearance of contrail cirrus
Examination of aerosol indirect effects during cirrus cloud evolution
In situ microphysics observations of intense pyroconvection from a large wildfire
Conditions favorable for secondary ice production in Arctic mixed-phase clouds
Interaction between cloud–radiation, atmospheric dynamics and thermodynamics based on observational data from GoAmazon 2014/15 and a cloud-resolving model
Snowfall in Northern Finland derives mostly from ice clouds
Observation of secondary ice production in clouds at low temperatures
In situ and satellite-based estimates of cloud properties and aerosol–cloud interactions over the southeast Atlantic Ocean
Ice fog observed at cirrus temperatures at Dome C, Antarctic Plateau
Life cycle of stratocumulus clouds over 1 year at the coast of the Atacama Desert
Significant continental source of ice-nucleating particles at the tip of Chile's southernmost Patagonia region
Retrieving ice-nucleating particle concentration and ice multiplication factors using active remote sensing validated by in situ observations
Temporal and vertical distributions of the occurrence of cirrus clouds over a coastal station in the Indian monsoon region
Continental thunderstorm ground enhancement observed at an exceptionally low altitude
Ice-nucleating particles from multiple aerosol sources in the urban environment of Beijing under mixed-phase cloud conditions
In situ observation of riming in mixed-phase clouds using the PHIPS probe
Measurement report: Introduction to the HyICE-2018 campaign for measurements of ice-nucleating particles and instrument inter-comparison in the Hyytiälä boreal forest
North Atlantic Ocean SST-gradient-driven variations in aerosol and cloud evolution along Lagrangian cold-air outbreak trajectories
Factors affecting precipitation formation and precipitation susceptibility of marine stratocumulus with variable above- and below-cloud aerosol concentrations over the Southeast Atlantic
An assessment of macrophysical and microphysical cloud properties driving radiative forcing of shallow trade-wind clouds
High concentrations of ice crystals in upper-tropospheric tropical clouds: is there a link to biomass and fossil fuel combustion?
Atmospheric rivers and associated precipitation patterns during the ACLOUD and PASCAL campaigns near Svalbard (May–June 2017): case studies using observations, reanalyses, and a regional climate model
Mass of different snow crystal shapes derived from fall speed measurements
Measurement report: Impact of African aerosol particles on cloud evolution in a tropical montane cloud forest in the Caribbean
Annual exposure to polycyclic aromatic hydrocarbons in urban environments linked to wintertime wood-burning episodes
Reduced ice number concentrations in contrails from low-aromatic biofuel blends
Distinct impacts on precipitation by aerosol radiative effect over three different megacity regions of eastern China
Estimation of the terms acting on local 1 h surface temperature variations in Paris region: the specific contribution of clouds
Contrasting characteristics of open- and closed-cellular stratocumulus cloud in the eastern North Atlantic
Mass and density of individual frozen hydrometeors
Linear relationship between effective radius and precipitation water content near the top of convective clouds: measurement results from ACRIDICON–CHUVA campaign
Supercooled liquid water and secondary ice production in Kelvin–Helmholtz instability as revealed by radar Doppler spectra observations
Benjamin Kirbus, Imke Schirmacher, Marcus Klingebiel, Michael Schäfer, André Ehrlich, Nils Slättberg, Johannes Lucke, Manuel Moser, Hanno Müller, and Manfred Wendisch
Atmos. Chem. Phys., 24, 3883–3904, https://doi.org/10.5194/acp-24-3883-2024, https://doi.org/10.5194/acp-24-3883-2024, 2024
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A research aircraft is used to track the changes in air temperature, moisture, and cloud properties for air that moves from cold Arctic sea ice onto warmer oceanic waters. The measurements are compared to two reanalysis models named ERA5 and CARRA. The biggest differences are found for air temperature over the sea ice and moisture over the ocean. CARRA data are more accurate than ERA5 because they better simulate the sea ice, the transition from sea ice to open ocean, and the forming clouds.
Raphael Satoru Märkl, Christiane Voigt, Daniel Sauer, Rebecca Katharina Dischl, Stefan Kaufmann, Theresa Harlaß, Valerian Hahn, Anke Roiger, Cornelius Weiß-Rehm, Ulrike Burkhardt, Ulrich Schumann, Andreas Marsing, Monika Scheibe, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Reetu Sallinen, Tobias Schripp, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 3813–3837, https://doi.org/10.5194/acp-24-3813-2024, https://doi.org/10.5194/acp-24-3813-2024, 2024
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In situ measurements of contrails from a large passenger aircraft burning 100 % sustainable aviation fuel (SAF) show a 56 % reduction in contrail ice crystal numbers compared to conventional Jet A-1. Results from a climate model initialized with the observations suggest a significant decrease in radiative forcing from contrails. Our study confirms that future increased use of low aromatic SAF can reduce the climate impact from aviation.
Philippe Ricaud, Massimo Del Guasta, Angelo Lupi, Romain Roehrig, Eric Bazile, Pierre Durand, Jean-Luc Attié, Alessia Nicosia, and Paolo Grigioni
Atmos. Chem. Phys., 24, 613–630, https://doi.org/10.5194/acp-24-613-2024, https://doi.org/10.5194/acp-24-613-2024, 2024
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Clouds affect the Earth's climate in ways that depend on the type of cloud (solid/liquid water). From observations at Concordia (Antarctica), we show that in supercooled liquid water (liquid water for temperatures below 0°C) clouds (SLWCs), temperature and SLWC radiative forcing increase with liquid water (up to 70 W m−2). We extrapolated that the maximum SLWC radiative forcing can reach 40 W m−2 over the Antarctic Peninsula, highlighting the importance of SLWCs for global climate prediction.
Cheikh Dione, Martial Haeffelin, Frédéric Burnet, Christine Lac, Guylaine Canut, Julien Delanoë, Jean-Charles Dupont, Susana Jorquera, Pauline Martinet, Jean-François Ribaud, and Felipe Toledo
Atmos. Chem. Phys., 23, 15711–15731, https://doi.org/10.5194/acp-23-15711-2023, https://doi.org/10.5194/acp-23-15711-2023, 2023
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This paper documents the role of thermodynamics and turbulence in the fog life cycle over southwestern France. It is based on a unique dataset collected during the SOFOG3D field campaign in autumn and winter 2019–2020. The paper gives a threshold for turbulence driving the different phases of the fog life cycle and the role of advection in the night-time dissipation of fog. The results can be operationalised to nowcast fog and improve short-range forecasts in numerical weather prediction models.
Hui Xu, Jianping Guo, Bing Tong, Jinqiang Zhang, Tianmeng Chen, Xiaoran Guo, Jian Zhang, and Wenqing Chen
Atmos. Chem. Phys., 23, 15011–15038, https://doi.org/10.5194/acp-23-15011-2023, https://doi.org/10.5194/acp-23-15011-2023, 2023
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The radiative effect of cloud remains one of the largest uncertain factors in climate change, largely due to the lack of cloud vertical structure (CVS) observations. The study presents the first near-global CVS climatology using high-vertical-resolution soundings. Single-layer cloud mainly occurs over arid regions. As the number of cloud layers increases, clouds tend to have lower bases and thinner layer thicknesses. The occurrence frequency of cloud exhibits a pronounced seasonal diurnal cycle.
Siddhant Gupta, Die Wang, Scott E. Giangrande, Thiago S. Biscaro, and Michael P. Jensen
EGUsphere, https://doi.org/10.5194/egusphere-2023-2410, https://doi.org/10.5194/egusphere-2023-2410, 2023
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We examine the lifecycle of isolated deep convective clouds (DCCs) in the Amazon rainforest. Weather radar echoes from the DCCs are tracked to evaluate their lifecycle. The DCC size and intensity increase, reach a peak, and then decrease over the DCC lifetime. Vertical profiles of air motion and mass transport from different seasons are examined to understand the transport of energy and momentum within DCC cores and to address the deficiencies in simulating DCCs using weather and climate models.
Elena De La Torre Castro, Tina Jurkat-Witschas, Armin Afchine, Volker Grewe, Valerian Hahn, Simon Kirschler, Martina Krämer, Johannes Lucke, Nicole Spelten, Heini Wernli, Martin Zöger, and Christiane Voigt
Atmos. Chem. Phys., 23, 13167–13189, https://doi.org/10.5194/acp-23-13167-2023, https://doi.org/10.5194/acp-23-13167-2023, 2023
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In this study, we show the differences in the microphysical properties between high-latitude (HL) cirrus and mid-latitude (ML) cirrus over the Arctic, North Atlantic, and central Europe during summer. The in situ measurements are combined with backward trajectories to investigate the influence of the region on cloud formation. We show that HL cirrus are characterized by a lower concentration of larger ice crystals when compared to ML cirrus.
Mampi Sarkar, Adriana Bailey, Peter Blossey, Simon P. de Szoeke, David Noone, Estefanía Quiñones Meléndez, Mason D. Leandro, and Patrick Y. Chuang
Atmos. Chem. Phys., 23, 12671–12690, https://doi.org/10.5194/acp-23-12671-2023, https://doi.org/10.5194/acp-23-12671-2023, 2023
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We study rain evaporation characteristics below shallow cumulus clouds over the North Atlantic Ocean by pairing isotope observations with a microphysical model. The modeled fraction of rain mass that evaporates below the cloud strongly depends on the raindrop size and distribution width. Moreover, the higher the rain mass fraction evaporated, the greater the change in deuterium excess. In this way, rain evaporation could be studied independently using only isotope and microphysical observations.
Simon Kirschler, Christiane Voigt, Bruce E. Anderson, Gao Chen, Ewan C. Crosbie, Richard A. Ferrare, Valerian Hahn, Johnathan W. Hair, Stefan Kaufmann, Richard H. Moore, David Painemal, Claire E. Robinson, Kevin J. Sanchez, Amy J. Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 23, 10731–10750, https://doi.org/10.5194/acp-23-10731-2023, https://doi.org/10.5194/acp-23-10731-2023, 2023
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In this study we present an overview of liquid and mixed-phase clouds and precipitation in the marine boundary layer over the western North Atlantic Ocean. We compare microphysical properties of pure liquid clouds to mixed-phase clouds and show that the initiation of the ice phase in mixed-phase clouds promotes precipitation. The observational data presented in this study are well suited for investigating the processes that give rise to liquid and mixed-phase clouds, ice, and precipitation.
Meng Xing, Weiguo Liu, Jing Hu, and Zheng Wang
Atmos. Chem. Phys., 23, 9123–9136, https://doi.org/10.5194/acp-23-9123-2023, https://doi.org/10.5194/acp-23-9123-2023, 2023
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The below-cloud evaporation effect (BCE) on precipitation largely impacts the final isotopic composition. However, determining the BCE effect remains poorly constrained. Our work used a ΔdΔδ diagram to differentiate the below-cloud processes. Moreover, by comparing two different computing methods, we considered that both methods are suitable for evaluation the BCE, except for snowfall events. Overall, our work compiled a set of effective methods to evaluate the BCE effect.
McKenna W. Stanford, Ann M. Fridlind, Israel Silber, Andrew S. Ackerman, Greg Cesana, Johannes Mülmenstädt, Alain Protat, Simon Alexander, and Adrian McDonald
Atmos. Chem. Phys., 23, 9037–9069, https://doi.org/10.5194/acp-23-9037-2023, https://doi.org/10.5194/acp-23-9037-2023, 2023
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Clouds play an important role in the Earth’s climate system as they modulate the amount of radiation that either reaches the surface or is reflected back to space. This study demonstrates an approach to robustly evaluate surface-based observations against a large-scale model. We find that the large-scale model precipitates too infrequently relative to observations, contrary to literature documentation suggesting otherwise based on satellite measurements.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
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During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Silke Groß, Tina Jurkat-Witschas, Qiang Li, Martin Wirth, Benedikt Urbanek, Martina Krämer, Ralf Weigel, and Christiane Voigt
Atmos. Chem. Phys., 23, 8369–8381, https://doi.org/10.5194/acp-23-8369-2023, https://doi.org/10.5194/acp-23-8369-2023, 2023
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Aviation-emitted aerosol can have an impact on cirrus clouds. We present optical and microphysical properties of mid-latitude cirrus clouds which were formed under the influence of aviation-emitted aerosol or which were formed under rather pristine conditions. We find that cirrus clouds affected by aviation-emitted aerosol show larger values of the particle linear depolarization ratio, larger mean effective ice particle diameters and decreased ice particle number concentrations.
Emma Järvinen, Franziska Nehlert, Guanglang Xu, Fritz Waitz, Guillaume Mioche, Regis Dupuy, Olivier Jourdan, and Martin Schnaiter
Atmos. Chem. Phys., 23, 7611–7633, https://doi.org/10.5194/acp-23-7611-2023, https://doi.org/10.5194/acp-23-7611-2023, 2023
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The Arctic is warming faster than other regions. Arctic low-level mixed-phase clouds, where ice crystals and liquid droplets co-exist, are thought to have an important role in Arctic warming. Here we show airborne measurements of vertical distribution of liquid and ice particles and their relative abundance. Ice particles are found in relative warm clouds, which can be explained by multiplication of existing ice crystals. However, the role of ice particles in redistributing sun light is minimal.
Manuel Moser, Christiane Voigt, Tina Jurkat-Witschas, Valerian Hahn, Guillaume Mioche, Olivier Jourdan, Régis Dupuy, Christophe Gourbeyre, Alfons Schwarzenboeck, Johannes Lucke, Yvonne Boose, Mario Mech, Stephan Borrmann, André Ehrlich, Andreas Herber, Christof Lüpkes, and Manfred Wendisch
Atmos. Chem. Phys., 23, 7257–7280, https://doi.org/10.5194/acp-23-7257-2023, https://doi.org/10.5194/acp-23-7257-2023, 2023
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This study provides a comprehensive microphysical and thermodynamic phase analysis of low-level clouds in the northern Fram Strait, above the sea ice and the open ocean, during spring and summer. Using airborne in situ cloud data, we show that the properties of Arctic low-level clouds vary significantly with seasonal meteorological situations and surface conditions. The observations presented in this study can help one to assess the role of clouds in the Arctic climate system.
Rachel Atlas and Christopher S. Bretherton
Atmos. Chem. Phys., 23, 4009–4030, https://doi.org/10.5194/acp-23-4009-2023, https://doi.org/10.5194/acp-23-4009-2023, 2023
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The tropical tropopause layer exists between the troposphere and the stratosphere in the tropics. Very thin cirrus clouds cool Earth's surface by scrubbing water vapor (a greenhouse gas) out of air parcels as they ascend through the tropical tropopause layer on their way to the stratosphere. We show observational evidence from aircraft that small-scale (< 100 km) gravity waves and turbulence increase the amount of ice in these clouds and may allow them to remove more water vapor from the air.
Konstantinos Matthaios Doulgeris, Ville Vakkari, Ewan J. O'Connor, Veli-Matti Kerminen, Heikki Lihavainen, and David Brus
Atmos. Chem. Phys., 23, 2483–2498, https://doi.org/10.5194/acp-23-2483-2023, https://doi.org/10.5194/acp-23-2483-2023, 2023
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We investigated how different long-range-transported air masses can affect the microphysical properties of low-level clouds in a clean subarctic environment. A connection was revealed. Higher values of cloud droplet number concentrations were related to continental air masses, whereas the lowest values of number concentrations were related to marine air masses. These were characterized by larger cloud droplets. Clouds in all regions were sensitive to increases in cloud number concentration.
Fayçal Lamraoui, Martina Krämer, Armin Afchine, Adam B. Sokol, Sergey Khaykin, Apoorva Pandey, and Zhiming Kuang
Atmos. Chem. Phys., 23, 2393–2419, https://doi.org/10.5194/acp-23-2393-2023, https://doi.org/10.5194/acp-23-2393-2023, 2023
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Cirrus in the tropical tropopause layer (TTL) can play a key role in vertical transport. We investigate the role of different cloud regimes and the associated ice habits in regulating the properties of the TTL. We use high-resolution numerical experiments at the scales of large-eddy simulations (LESs) and aircraft measurements. We found that LES-scale parameterizations that predict ice shape are crucial for an accurate representation of TTL cirrus and thus the associated (de)hydration process.
Yun Li, Christoph Mahnke, Susanne Rohs, Ulrich Bundke, Nicole Spelten, Georgios Dekoutsidis, Silke Groß, Christiane Voigt, Ulrich Schumann, Andreas Petzold, and Martina Krämer
Atmos. Chem. Phys., 23, 2251–2271, https://doi.org/10.5194/acp-23-2251-2023, https://doi.org/10.5194/acp-23-2251-2023, 2023
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The radiative effect of aviation-induced cirrus is closely related to ambient conditions and its microphysical properties. Our study investigated the occurrence of contrail and natural cirrus measured above central Europe in spring 2014. It finds that contrail cirrus appears frequently in the pressure range 200 to 245 hPa and occurs more often in slightly ice-subsaturated environments than expected. Avoiding slightly ice-subsaturated regions by aviation might help mitigate contrail cirrus.
Flor Vanessa Maciel, Minghui Diao, and Ryan Patnaude
Atmos. Chem. Phys., 23, 1103–1129, https://doi.org/10.5194/acp-23-1103-2023, https://doi.org/10.5194/acp-23-1103-2023, 2023
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Aerosol indirect effects on cirrus clouds are investigated during cirrus evolution, using global-scale in situ observations and climate model simulations. As cirrus evolves, the mechanisms to form ice crystals also change with time. Both small and large aerosols are found to affect cirrus properties. Southern Hemisphere cirrus appears to be more sensitive to additional aerosols. The climate model underestimates ice crystal mass, likely due to biases of relative humidity and vertical velocity.
David E. Kingsmill, Jeffrey R. French, and Neil P. Lareau
Atmos. Chem. Phys., 23, 1–21, https://doi.org/10.5194/acp-23-1-2023, https://doi.org/10.5194/acp-23-1-2023, 2023
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This study uses in situ aircraft measurements to characterize the size and shape distributions of 10 µm to 6 mm diameter particles observed during six penetrations of wildfire-induced pyroconvection. Particles sampled in one penetration of a smoke plume are most likely pyrometeors composed of ash. The other penetrations are through pyrocumulus clouds where particle composition is most likely a combination of hydrometeors (ice particles) and pyrometeors (ash).
Julie Thérèse Pasquier, Jan Henneberger, Fabiola Ramelli, Annika Lauber, Robert Oscar David, Jörg Wieder, Tim Carlsen, Rosa Gierens, Marion Maturilli, and Ulrike Lohmann
Atmos. Chem. Phys., 22, 15579–15601, https://doi.org/10.5194/acp-22-15579-2022, https://doi.org/10.5194/acp-22-15579-2022, 2022
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It is important to understand how ice crystals and cloud droplets form in clouds, as their concentrations and sizes determine the exact radiative properties of the clouds. Normally, ice crystals form from aerosols, but we found evidence for the formation of additional ice crystals from the original ones over a large temperature range within Arctic clouds. In particular, additional ice crystals were formed during collisions of several ice crystals or during the freezing of large cloud droplets.
Layrson J. M. Gonçalves, Simone M. S. C. Coelho, Paulo Y. Kubota, and Dayana C. Souza
Atmos. Chem. Phys., 22, 15509–15526, https://doi.org/10.5194/acp-22-15509-2022, https://doi.org/10.5194/acp-22-15509-2022, 2022
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This research aims to study the environmental conditions that are favorable and not favorable to cloud formation, in this case specifically for the Amazon region. The results found in this research will be used to improve the representation of clouds in numerical models that are used in weather and climate prediction. In general, it is expected that with better knowledge regarding the cloud–radiation interaction, it is possible to make a better forecast of weather and climate.
Claudia Mignani, Lukas Zimmermann, Rigel Kivi, Alexis Berne, and Franz Conen
Atmos. Chem. Phys., 22, 13551–13568, https://doi.org/10.5194/acp-22-13551-2022, https://doi.org/10.5194/acp-22-13551-2022, 2022
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We determined over the course of 8 winter months the phase of clouds associated with snowfall in Northern Finland using radiosondes and observations of ice particle habits at ground level. We found that precipitating clouds were extending from near ground to at least 2.7 km altitude and approximately three-quarters of them were likely glaciated. Possible moisture sources and ice formation processes are discussed.
Alexei Korolev, Paul J. DeMott, Ivan Heckman, Mengistu Wolde, Earle Williams, David J. Smalley, and Michael F. Donovan
Atmos. Chem. Phys., 22, 13103–13113, https://doi.org/10.5194/acp-22-13103-2022, https://doi.org/10.5194/acp-22-13103-2022, 2022
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The present study provides the first explicit in situ observation of secondary ice production at temperatures as low as −27 °C, which is well outside the range of the Hallett–Mossop process (−3 to −8 °C). This observation expands our knowledge of the temperature range of initiation of secondary ice in clouds. The obtained results are intended to stimulate laboratory and theoretical studies to develop physically based parameterizations for weather prediction and climate models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Ian Chang, Lan Gao, Feng Xu, and Jens Redemann
Atmos. Chem. Phys., 22, 12923–12943, https://doi.org/10.5194/acp-22-12923-2022, https://doi.org/10.5194/acp-22-12923-2022, 2022
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The ability of NASA’s Terra and Aqua satellites to retrieve cloud properties and estimate the changes in cloud properties due to aerosol–cloud interactions (ACI) was examined. There was good agreement between satellite retrievals and in situ measurements over the southeast Atlantic Ocean. This suggests that, combined with information on aerosol properties, satellite retrievals of cloud properties can be used to study ACI over larger domains and longer timescales in the absence of in situ data.
Étienne Vignon, Lea Raillard, Christophe Genthon, Massimo Del Guasta, Andrew J. Heymsfield, Jean-Baptiste Madeleine, and Alexis Berne
Atmos. Chem. Phys., 22, 12857–12872, https://doi.org/10.5194/acp-22-12857-2022, https://doi.org/10.5194/acp-22-12857-2022, 2022
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The near-surface atmosphere over the Antarctic Plateau is cold and pristine and resembles to a certain extent the high troposphere where cirrus clouds form. In this study, we use innovative humidity measurements at Concordia Station to study the formation of ice fogs at temperatures <−40°C. We provide observational evidence that ice fogs can form through the homogeneous freezing of solution aerosols, a common nucleation pathway for cirrus clouds.
Jan H. Schween, Camilo del Rio, Juan-Luis García, Pablo Osses, Sarah Westbrook, and Ulrich Löhnert
Atmos. Chem. Phys., 22, 12241–12267, https://doi.org/10.5194/acp-22-12241-2022, https://doi.org/10.5194/acp-22-12241-2022, 2022
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Marine stratocumulus clouds of the eastern Pacific play an essential role in the Earth's climate. These clouds form the major source of water to parts of the extreme dry Atacama Desert at the northern coast of Chile. For the first time these clouds are observed over a whole year with three remote sensing instruments. It is shown how these clouds are influenced by the land–sea wind system and the distribution of ocean temperatures.
Xianda Gong, Martin Radenz, Heike Wex, Patric Seifert, Farnoush Ataei, Silvia Henning, Holger Baars, Boris Barja, Albert Ansmann, and Frank Stratmann
Atmos. Chem. Phys., 22, 10505–10525, https://doi.org/10.5194/acp-22-10505-2022, https://doi.org/10.5194/acp-22-10505-2022, 2022
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The sources of ice-nucleating particles (INPs) are poorly understood in the Southern Hemisphere (SH). We studied INPs in the boundary layer in the southern Patagonia region. No seasonal cycle of INP concentrations was observed. The majority of INPs are biogenic particles, likely from local continental sources. The INP concentrations are higher when strong precipitation occurs. While previous studies focused on marine INP sources in SH, we point out the importance of continental sources of INPs.
Jörg Wieder, Nikola Ihn, Claudia Mignani, Moritz Haarig, Johannes Bühl, Patric Seifert, Ronny Engelmann, Fabiola Ramelli, Zamin A. Kanji, Ulrike Lohmann, and Jan Henneberger
Atmos. Chem. Phys., 22, 9767–9797, https://doi.org/10.5194/acp-22-9767-2022, https://doi.org/10.5194/acp-22-9767-2022, 2022
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Ice formation and its evolution in mixed-phase clouds are still uncertain. We evaluate the lidar retrieval of ice-nucleating particle concentration in dust-dominated and continental air masses over the Swiss Alps with in situ observations. A calibration factor to improve the retrieval from continental air masses is proposed. Ice multiplication factors are obtained with a new method utilizing remote sensing. Our results indicate that secondary ice production occurs at temperatures down to −30 °C.
Saleem Ali, Sanjay Kumar Mehta, Aravindhavel Ananthavel, and Tondapu Venkata Ramesh Reddy
Atmos. Chem. Phys., 22, 8321–8342, https://doi.org/10.5194/acp-22-8321-2022, https://doi.org/10.5194/acp-22-8321-2022, 2022
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Multiple cirrus clouds frequently occur over regions of deep convection in the tropics. Tropical convection has a strong diurnal pattern, with peaks in the afternoon to early evening, over the continents. Continuous micropulse lidar observations over a coastal station in the Indian monsoon region enable us, for the first time, to demonstrate a robust diurnal pattern of single and multiple cirrus occurrences, with peaks during the late afternoon and early morning hours, respectively.
Ivana Kolmašová, Ondřej Santolík, Jakub Šlegl, Jana Popová, Zbyněk Sokol, Petr Zacharov, Ondřej Ploc, Gerhard Diendorfer, Ronald Langer, Radek Lán, and Igor Strhárský
Atmos. Chem. Phys., 22, 7959–7973, https://doi.org/10.5194/acp-22-7959-2022, https://doi.org/10.5194/acp-22-7959-2022, 2022
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Gamma ray radiation related to thunderstorms was previously observed at the high-altitude mountain observatories or on the western coast of Japan, usually being terminated by lightning discharges. We show unusual observations of gamma rays at an altitude below 1000 m, coinciding with peculiar rapid variations in the vertical electric field, which are linked to inverted intracloud lightning discharges. This indicates that a strong, lower positive-charge region was present inside the thundercloud.
Cuiqi Zhang, Zhijun Wu, Jingchuan Chen, Jie Chen, Lizi Tang, Wenfei Zhu, Xiangyu Pei, Shiyi Chen, Ping Tian, Song Guo, Limin Zeng, Min Hu, and Zamin A. Kanji
Atmos. Chem. Phys., 22, 7539–7556, https://doi.org/10.5194/acp-22-7539-2022, https://doi.org/10.5194/acp-22-7539-2022, 2022
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The immersion ice nucleation effectiveness of aerosols from multiple sources in the urban environment remains elusive. In this study, we demonstrate that the immersion ice-nucleating particle (INP) concentration increased dramatically during a dust event in an urban atmosphere. Pollutant aerosols, including inorganic salts formed through secondary transformation (SIA) and black carbon (BC), might not act as effective INPs under mixed-phase cloud conditions.
Fritz Waitz, Martin Schnaiter, Thomas Leisner, and Emma Järvinen
Atmos. Chem. Phys., 22, 7087–7103, https://doi.org/10.5194/acp-22-7087-2022, https://doi.org/10.5194/acp-22-7087-2022, 2022
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Riming, i.e., the accretion of small droplets on the surface of ice particles via collision, is one of the major uncertainties in model prediction of mixed-phase clouds. We discuss the occurrence (up to 50% of particles) and aging of rimed ice particles and show correlations of the occurrence and the degree of riming with ambient meteorological parameters using data gathered by the Particle Habit Imaging and Polar Scattering (PHIPS) probe during three airborne in situ field campaigns.
Zoé Brasseur, Dimitri Castarède, Erik S. Thomson, Michael P. Adams, Saskia Drossaart van Dusseldorp, Paavo Heikkilä, Kimmo Korhonen, Janne Lampilahti, Mikhail Paramonov, Julia Schneider, Franziska Vogel, Yusheng Wu, Jonathan P. D. Abbatt, Nina S. Atanasova, Dennis H. Bamford, Barbara Bertozzi, Matthew Boyer, David Brus, Martin I. Daily, Romy Fösig, Ellen Gute, Alexander D. Harrison, Paula Hietala, Kristina Höhler, Zamin A. Kanji, Jorma Keskinen, Larissa Lacher, Markus Lampimäki, Janne Levula, Antti Manninen, Jens Nadolny, Maija Peltola, Grace C. E. Porter, Pyry Poutanen, Ulrike Proske, Tobias Schorr, Nsikanabasi Silas Umo, János Stenszky, Annele Virtanen, Dmitri Moisseev, Markku Kulmala, Benjamin J. Murray, Tuukka Petäjä, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 22, 5117–5145, https://doi.org/10.5194/acp-22-5117-2022, https://doi.org/10.5194/acp-22-5117-2022, 2022
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The present measurement report introduces the ice nucleation campaign organized in Hyytiälä, Finland, in 2018 (HyICE-2018). We provide an overview of the campaign settings, and we describe the measurement infrastructure and operating procedures used. In addition, we use results from ice nucleation instrument inter-comparison to show that the suite of these instruments deployed during the campaign reports consistent results.
Kevin J. Sanchez, Bo Zhang, Hongyu Liu, Matthew D. Brown, Ewan C. Crosbie, Francesca Gallo, Johnathan W. Hair, Chris A. Hostetler, Carolyn E. Jordan, Claire E. Robinson, Amy Jo Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Elizabeth B. Wiggins, Edward L. Winstead, Luke D. Ziemba, Georges Saliba, Savannah L. Lewis, Lynn M. Russell, Patricia K. Quinn, Timothy S. Bates, Jack Porter, Thomas G. Bell, Peter Gaube, Eric S. Saltzman, Michael J. Behrenfeld, and Richard H. Moore
Atmos. Chem. Phys., 22, 2795–2815, https://doi.org/10.5194/acp-22-2795-2022, https://doi.org/10.5194/acp-22-2795-2022, 2022
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Atmospheric particle concentrations impact clouds, which strongly impact the amount of sunlight reflected back into space and the overall climate. Measurements of particles over the ocean are rare and expensive to collect, so models are necessary to fill in the gaps by simulating both particle and clouds. However, some measurements are needed to test the accuracy of the models. Here, we measure changes in particles in different weather conditions, which are ideal for comparison with models.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Rose M. Miller, and Jennifer D. Small Griswold
Atmos. Chem. Phys., 22, 2769–2793, https://doi.org/10.5194/acp-22-2769-2022, https://doi.org/10.5194/acp-22-2769-2022, 2022
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This study evaluates the impact of biomass burning aerosols on precipitation in marine stratocumulus clouds using observations from the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign over the Southeast Atlantic. Instances of contact and separation between aerosol and cloud layers show polluted clouds have a lower precipitation rate and a lower precipitation susceptibility. This information will help improve cloud representation in Earth system models.
Anna E. Luebke, André Ehrlich, Michael Schäfer, Kevin Wolf, and Manfred Wendisch
Atmos. Chem. Phys., 22, 2727–2744, https://doi.org/10.5194/acp-22-2727-2022, https://doi.org/10.5194/acp-22-2727-2022, 2022
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A combination of aircraft and satellite observations is used to show how the characteristics of tropical shallow clouds interact with incoming and outgoing energy. A complete depiction of these clouds is challenging to obtain, but such data are useful for understanding how models can correctly represent them. The amount of cloud is found to be the most important factor, while other cloud characteristics become increasingly impactful when more cloud is present.
Graciela B. Raga, Darrel Baumgardner, Blanca Rios, Yanet Díaz-Esteban, Alejandro Jaramillo, Martin Gallagher, Bastien Sauvage, Pawel Wolff, and Gary Lloyd
Atmos. Chem. Phys., 22, 2269–2292, https://doi.org/10.5194/acp-22-2269-2022, https://doi.org/10.5194/acp-22-2269-2022, 2022
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The In-Service Aircraft for a Global Observing System (IAGOS) is a small fleet of commercial aircraft that carry a suite of meteorological, gas, aerosol, and cloud sensors and have been measuring worldwide for almost 9 years, since late 2011. Extreme ice events (EIEs) have been identified from the IAGOS cloud measurements and linked to surface emissions for biomass and fossil fuel consumption. The results reported here are highly relevant for climate change and flight operations forecasting.
Carolina Viceto, Irina V. Gorodetskaya, Annette Rinke, Marion Maturilli, Alfredo Rocha, and Susanne Crewell
Atmos. Chem. Phys., 22, 441–463, https://doi.org/10.5194/acp-22-441-2022, https://doi.org/10.5194/acp-22-441-2022, 2022
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We focus on anomalous moisture transport events known as atmospheric rivers (ARs). During ACLOUD and PASCAL, three AR events were identified: 30 May, 6 June, and 9 June 2017. We explore their spatio-temporal evolution and precipitation patterns using measurements, reanalyses, and a model. We show the importance of the following: Atlantic and Siberian pathways during spring–summer in the Arctic, AR-associated heat/moisture increase, precipitation phase transition, and high-resolution datasets.
Sandra Vázquez-Martín, Thomas Kuhn, and Salomon Eliasson
Atmos. Chem. Phys., 21, 18669–18688, https://doi.org/10.5194/acp-21-18669-2021, https://doi.org/10.5194/acp-21-18669-2021, 2021
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High-resolution top- and side-view images of snow ice particles taken by the D-ICI instrument are used to determine the shape; size; cross-sectional area; fall speed; and, based upon these properties, the mass of the individual snow particles. The study analyses the relationships between these fundamental properties as a function of particle shape and highlights that the choice of size parameter, maximum dimension or another characteristic length, is crucial when relating fall speed to mass.
Elvis Torres-Delgado, Darrel Baumgardner, and Olga L. Mayol-Bracero
Atmos. Chem. Phys., 21, 18011–18027, https://doi.org/10.5194/acp-21-18011-2021, https://doi.org/10.5194/acp-21-18011-2021, 2021
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African dust aerosols can travel thousands of kilometers and reach the Caribbean and other places, where they can serve as ice and cloud condensation nuclei and alter precipitation patterns. Cloud microphysical properties (droplet number and size) were measured in a Caribbean tropical montane cloud forest along with models and satellite products. The results of the study suggest that meteorology and air mass history are more important for cloud processes than aerosols transported from Africa.
Irini Tsiodra, Georgios Grivas, Kalliopi Tavernaraki, Aikaterini Bougiatioti, Maria Apostolaki, Despina Paraskevopoulou, Alexandra Gogou, Constantine Parinos, Konstantina Oikonomou, Maria Tsagkaraki, Pavlos Zarmpas, Athanasios Nenes, and Nikolaos Mihalopoulos
Atmos. Chem. Phys., 21, 17865–17883, https://doi.org/10.5194/acp-21-17865-2021, https://doi.org/10.5194/acp-21-17865-2021, 2021
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We analyze observations from year-long measurements at Athens, Greece. Nighttime wintertime PAH levels are 4 times higher than daytime, and wintertime values are 15 times higher than summertime. Biomass burning aerosol during wintertime pollution events is responsible for these significant wintertime enhancements and accounts for 43 % of the population exposure to PAH carcinogenic risk. Biomass burning poses additional health risks beyond those associated with the high PM levels that develop.
Tiziana Bräuer, Christiane Voigt, Daniel Sauer, Stefan Kaufmann, Valerian Hahn, Monika Scheibe, Hans Schlager, Felix Huber, Patrick Le Clercq, Richard H. Moore, and Bruce E. Anderson
Atmos. Chem. Phys., 21, 16817–16826, https://doi.org/10.5194/acp-21-16817-2021, https://doi.org/10.5194/acp-21-16817-2021, 2021
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Over half of aviation climate impact is caused by contrails. Biofuels can reduce the ice crystal numbers in contrails and mitigate the climate impact. The experiment ECLIF II/NDMAX in 2018 assessed the effects of biofuels on contrails and aviation emissions. The NASA DC-8 aircraft performed measurements inside the contrail of the DLR A320. One reference fuel and two blends of the biofuel HEFA and kerosene are analysed. We find a max reduction of contrail ice numbers through biofuel use of 40 %.
Yue Sun and Chuanfeng Zhao
Atmos. Chem. Phys., 21, 16555–16574, https://doi.org/10.5194/acp-21-16555-2021, https://doi.org/10.5194/acp-21-16555-2021, 2021
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Using high-resolution multi-year warm season data, the influence of aerosol on precipitation time over the North China Plain (NCP), Yangtze River Delta (YRD), and Pearl River Delta (PRD) is investigated. Aerosol amount and type have significant influence on precipitation time: precipitation start time is advanced by 3 h in the NCP, delayed 2 h in the PRD, and negligibly changed in the YRD. Aerosol impact on precipitation is also influenced by precipitation type and meteorological conditions.
Oscar Javier Rojas Muñoz, Marjolaine Chiriaco, Sophie Bastin, and Justine Ringard
Atmos. Chem. Phys., 21, 15699–15723, https://doi.org/10.5194/acp-21-15699-2021, https://doi.org/10.5194/acp-21-15699-2021, 2021
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A method is developed and evaluated to quantify each process that affects hourly 2 m temperature variations on a local scale, based almost exclusively on observations retrieved from an observatory near the Paris region. Each term involved in surface temperature variations is estimated, and its contribution and importance are also assessed. It is found that clouds are the main modulator on hourly temperature variations for most hours of the day, and thus their characterization is addressed.
Michael P. Jensen, Virendra P. Ghate, Dié Wang, Diana K. Apoznanski, Mary J. Bartholomew, Scott E. Giangrande, Karen L. Johnson, and Mandana M. Thieman
Atmos. Chem. Phys., 21, 14557–14571, https://doi.org/10.5194/acp-21-14557-2021, https://doi.org/10.5194/acp-21-14557-2021, 2021
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This work compares the large-scale meteorology, cloud, aerosol, precipitation, and thermodynamics of closed- and open-cell cloud organizations using long-term observations from the astern North Atlantic. Open-cell cases are associated with cold-air outbreaks and occur in deeper boundary layers, with stronger winds and higher rain rates compared to closed-cell cases. These results offer important benchmarks for model representation of boundary layer clouds in this climatically important region.
Karlie N. Rees, Dhiraj K. Singh, Eric R. Pardyjak, and Timothy J. Garrett
Atmos. Chem. Phys., 21, 14235–14250, https://doi.org/10.5194/acp-21-14235-2021, https://doi.org/10.5194/acp-21-14235-2021, 2021
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Accurate predictions of weather and climate require descriptions of the mass and density of snowflakes as a function of their size. Few measurements have been obtained to date because snowflakes are so small and fragile. This article describes results from a new instrument that automatically measures individual snowflake size, mass, and density. Key findings are that small snowflakes have much lower densities than is often assumed and that snowflake density increases with temperature.
Ramon Campos Braga, Daniel Rosenfeld, Ovid O. Krüger, Barbara Ervens, Bruna A. Holanda, Manfred Wendisch, Trismono Krisna, Ulrich Pöschl, Meinrat O. Andreae, Christiane Voigt, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 14079–14088, https://doi.org/10.5194/acp-21-14079-2021, https://doi.org/10.5194/acp-21-14079-2021, 2021
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Quantifying the precipitation within clouds is crucial for our understanding of the Earth's hydrological cycle. Using in situ measurements of cloud and rain properties over the Amazon Basin and Atlantic Ocean, we show here a linear relationship between the effective radius (re) and precipitation water content near the tops of convective clouds for different pollution states and temperature levels. Our results emphasize the role of re to determine both initiation and amount of precipitation.
Haoran Li, Alexei Korolev, and Dmitri Moisseev
Atmos. Chem. Phys., 21, 13593–13608, https://doi.org/10.5194/acp-21-13593-2021, https://doi.org/10.5194/acp-21-13593-2021, 2021
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Kelvin–Helmholtz (K–H) clouds embedded in a stratiform precipitation event were uncovered via radar Doppler spectral analysis. Given the unprecedented detail of the observations, we show that multiple populations of secondary ice columns were generated in the pockets where larger cloud droplets are formed and not at some constant level within the cloud. Our results highlight that the K–H instability is favorable for liquid droplet growth and secondary ice formation.
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Short summary
The evolution of the droplet size distribution during the fog life cycle remains poorly understood and progress is required to reduce the uncertainty of fog forecasts. To gain insights into the physical processes driving the microphysics, intensive field campaigns were conducted during three winters at the SIRTA site in the south of Paris. This study analyzed the variations in fog microphysical properties and their potential interactions at the different evolutionary stages of the fog events.
The evolution of the droplet size distribution during the fog life cycle remains poorly...
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