Articles | Volume 21, issue 5
https://doi.org/10.5194/acp-21-4219-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-4219-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Interhemispheric transport of metallic ions within ionospheric sporadic E layers by the lower thermospheric meridional circulation
Bingkun Yu
CAS Key Laboratory of Geospace Environment, Department of Geophysics and Planetary Sciences, University of Science and Technology of China, Hefei, China
Department of Meteorology, University of Reading, Berkshire, UK
CAS Key Laboratory of Geospace Environment, Department of Geophysics and Planetary Sciences, University of Science and Technology of China, Hefei, China
CAS Center for Excellence in Comparative Planetology, Hefei, China
Anhui Mengcheng Geophysics National Observation and Research Station, University of Science and Technology of China, Hefei, China
Hefei National Laboratory for the Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, China
Christopher J. Scott
CORRESPONDING AUTHOR
Department of Meteorology, University of Reading, Berkshire, UK
Jianfei Wu
CAS Key Laboratory of Geospace Environment, Department of Geophysics and Planetary Sciences, University of Science and Technology of China, Hefei, China
CAS Center for Excellence in Comparative Planetology, Hefei, China
Anhui Mengcheng Geophysics National Observation and Research Station, University of Science and Technology of China, Hefei, China
Xinan Yue
Key Laboratory of Earth and Planetary Physics, Institute of Geology and Geophysics, Chinese Academy of Sciences, Beijing, China
Wuhu Feng
School of Chemistry, University of Leeds, Leeds, UK
National Center for Atmospheric Science, University of Leeds, Leeds, UK
Yutian Chi
CAS Key Laboratory of Geospace Environment, Department of Geophysics and Planetary Sciences, University of Science and Technology of China, Hefei, China
Department of Meteorology, University of Reading, Berkshire, UK
Daniel R. Marsh
School of Chemistry, University of Leeds, Leeds, UK
National Center for Atmospheric Research, Boulder, CO, USA
Hanli Liu
High Altitude Observatory, National Center for Atmospheric Research, Boulder, CO, USA
Xiankang Dou
CAS Key Laboratory of Geospace Environment, Department of Geophysics and Planetary Sciences, University of Science and Technology of China, Hefei, China
Hefei National Laboratory for the Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, China
Electronic Information School, Wuhan University, Wuhan, China
John M. C. Plane
School of Chemistry, University of Leeds, Leeds, UK
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Long-term change in the ionosphere are expected due to increases in greenhouse gases in the lower atmosphere. Empirical formulae are used to estimate height. Through comparison with independent data we show that there are seasonal and long-term biases introduced by the empirical model. We conclude that estimates of long-term changes in ionospheric height need to account for these biases.
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Atmos. Chem. Phys., 25, 4391–4401, https://doi.org/10.5194/acp-25-4391-2025, https://doi.org/10.5194/acp-25-4391-2025, 2025
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Gregory Cooke, Dan Marsh, Catherine Walsh, Felix Sainsbury-Martinez, and Marrick Braam
EGUsphere, https://doi.org/10.5194/egusphere-2025-1133, https://doi.org/10.5194/egusphere-2025-1133, 2025
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During the Archean eon (4–2.4 Gyr ago), Earth's atmosphere lacked oxygen (O2) but contained nitrogen, carbon dioxide, and methane. As cyanobacteria evolved, they produced O2, while hydrogen (H) escaped, making Earth more oxidized. Around 2.4 billion years ago, oxygen levels rose, limiting hydrogen loss. Using 3D computer simulations, we found that oxygen concentrations affect the upward diffusion of water vapor (H2O). We therefore quantify the rate of hydrogen escape as O2 changes.
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Atmos. Chem. Phys., 24, 10639–10653, https://doi.org/10.5194/acp-24-10639-2024, https://doi.org/10.5194/acp-24-10639-2024, 2024
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Long-term change in the ionosphere are expected due to increases in greenhouse gases in the lower atmosphere. Empirical formulae are used to estimate height. Through comparison with independent data we show that there are seasonal and long-term biases introduced by the empirical model. We conclude that estimates of long-term changes in ionospheric height need to account for these biases.
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Ozone is a potent air pollutant in the lower troposphere, with adverse impacts on human health. Satellite records of tropospheric ozone currently show large-scale inconsistencies in long-term trends. Our detailed study of the potential factors (e.g. satellite errors, where the satellite can observe ozone) potentially driving these inconsistencies found that, in North America, Europe, and East Asia, the underlying trends are typically small with large uncertainties.
Miriam Sinnhuber, Christina Arras, Stefan Bender, Bernd Funke, Hanli Liu, Daniel R. Marsh, Thomas Reddmann, Eugene Rozanov, Timofei Sukhodolov, Monika E. Szelag, and Jan Maik Wissing
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Formation of nitric oxide NO in the upper atmosphere varies with solar activity. Observations show that it starts a chain of processes in the entire atmosphere affecting the ozone layer and climate system. This is often underestimated in models. We compare five models which show large differences in simulated NO. Analysis of results point out problems related to the oxygen balance, and to the impact of atmospheric waves on dynamics. Both must be modeled well to reproduce the downward coupling.
Qinzeng Li, Jiyao Xu, Aditya Riadi Gusman, Hanli Liu, Wei Yuan, Weijun Liu, Yajun Zhu, and Xiao Liu
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The 2022 Hunga Tonga–Hunga Ha’apai (HTHH) volcanic eruption not only triggered broad-spectrum atmospheric waves but also generated unusual tsunamis which can generate atmospheric gravity waves (AGWs). Multiple strong atmospheric waves were observed in the far-field area of the 2022 HTHH volcano eruption in the upper atmosphere by a ground-based airglow imager network. AGWs caused by tsunamis can propagate to the mesopause region; there is a good match between atmospheric waves and tsunamis.
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Atmos. Chem. Phys., 24, 8277–8293, https://doi.org/10.5194/acp-24-8277-2024, https://doi.org/10.5194/acp-24-8277-2024, 2024
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The Tibetan Plateau (TP), the highest and largest plateau, experiences strong surface solar UV radiation, whose excess can cause harmful influences on local biota. Hence, it is critical to study TP ozone. We find ENSO, the strongest interannual phenomenon, tends to induce tropospheric temperature change and thus modulate tropopause variability, which in turn favours ozone change over the TP. Our results have implications for a better understanding of the interannual variability of TP ozone.
Yanlin Li, Tai-Yin Huang, Julio Urbina, Fabio Vargas, and Wuhu Feng
Ann. Geophys., 42, 285–299, https://doi.org/10.5194/angeo-42-285-2024, https://doi.org/10.5194/angeo-42-285-2024, 2024
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This work combines lidar observation data and a new numerical sodium (Na) chemistry model, using data assimilation to study the relation between the mesospheric Na layer and the meteoric input function. Simulation captures the seasonal variability in the Na number density compared with lidar observations over the Colorado State University (CSU) lidar. The estimated global ablated meteoroid material inputs from Andes Lidar Observatory and CSU observations are 83 t d-1 and 53 t d-1, respectively.
Tinna L. Gunnarsdottir, Ingrid Mann, Wuhu Feng, Devin R. Huyghebaert, Ingemar Haeggstroem, Yasunobu Ogawa, Norihito Saito, Satonori Nozawa, and Takuya D. Kawahara
Ann. Geophys., 42, 213–228, https://doi.org/10.5194/angeo-42-213-2024, https://doi.org/10.5194/angeo-42-213-2024, 2024
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Several tons of meteoric particles burn up in our atmosphere each day. This deposits a great deal of material that binds with other atmospheric particles and forms so-called meteoric smoke particles. These particles are assumed to influence radar measurements. Here, we have compared radar measurements with simulations of a radar spectrum with and without dust particles and found that dust influences the radar spectrum in the altitude range of 75–85 km.
Manuel López-Puertas, Federico Fabiano, Victor Fomichev, Bernd Funke, and Daniel R. Marsh
Geosci. Model Dev., 17, 4401–4432, https://doi.org/10.5194/gmd-17-4401-2024, https://doi.org/10.5194/gmd-17-4401-2024, 2024
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The radiative infrared cooling of CO2 in the middle atmosphere is crucial for computing its thermal structure. It requires one however to include non-local thermodynamic equilibrium processes which are computationally very expensive, which cannot be afforded by climate models. In this work, we present an updated, efficient, accurate and very fast (~50 µs) parameterization of that cooling able to cope with CO2 abundances from half the pre-industrial values to 10 times the current abundance.
Richard J. Pope, Alexandru Rap, Matilda A. Pimlott, Brice Barret, Eric Le Flochmoen, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Anne Boynard, Christian Retscher, Wuhu Feng, Richard Rigby, Sandip S. Dhomse, Catherine Wespes, and Martyn P. Chipperfield
Atmos. Chem. Phys., 24, 3613–3626, https://doi.org/10.5194/acp-24-3613-2024, https://doi.org/10.5194/acp-24-3613-2024, 2024
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Tropospheric ozone is an important short-lived climate forcer which influences the incoming solar short-wave radiation and the outgoing long-wave radiation in the atmosphere (8–15 km) where the balance between the two yields a net positive (i.e. warming) effect at the surface. Overall, we find that the tropospheric ozone radiative effect ranges between 1.21 and 1.26 W m−2 with a negligible trend (2008–2017), suggesting that tropospheric ozone influences on climate have remained stable with time.
Bernd Funke, Thierry Dudok de Wit, Ilaria Ermolli, Margit Haberreiter, Doug Kinnison, Daniel Marsh, Hilde Nesse, Annika Seppälä, Miriam Sinnhuber, and Ilya Usoskin
Geosci. Model Dev., 17, 1217–1227, https://doi.org/10.5194/gmd-17-1217-2024, https://doi.org/10.5194/gmd-17-1217-2024, 2024
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We outline a road map for the preparation of a solar forcing dataset for the upcoming Phase 7 of the Coupled Model Intercomparison Project (CMIP7), considering the latest scientific advances made in the reconstruction of solar forcing and in the understanding of climate response while also addressing the issues that were raised during CMIP6.
Stefan Noll, John M. C. Plane, Wuhu Feng, Konstantinos S. Kalogerakis, Wolfgang Kausch, Carsten Schmidt, Michael Bittner, and Stefan Kimeswenger
Atmos. Chem. Phys., 24, 1143–1176, https://doi.org/10.5194/acp-24-1143-2024, https://doi.org/10.5194/acp-24-1143-2024, 2024
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The Earth's nighttime radiation in the range from the near-UV to the near-IR mainly originates between 75 and 105 km and consists of lines of different species, which are important indicators of the chemistry and dynamics at these altitudes. Based on astronomical spectra, we have characterised the structure and variability of a pseudo-continuum of a high number of faint lines and discovered a new emission process in the near-IR. By means of simulations, we identified HO2 as the likely emitter.
Ailish M. Graham, Richard J. Pope, Martyn P. Chipperfield, Sandip S. Dhomse, Matilda Pimlott, Wuhu Feng, Vikas Singh, Ying Chen, Oliver Wild, Ranjeet Sokhi, and Gufran Beig
Atmos. Chem. Phys., 24, 789–806, https://doi.org/10.5194/acp-24-789-2024, https://doi.org/10.5194/acp-24-789-2024, 2024
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Our paper uses novel satellite datasets and high-resolution emissions datasets alongside a back-trajectory model to investigate the balance of local and external sources influencing NOx air pollution changes in Delhi. We find in the post-monsoon season that NOx from local and non-local transport emissions contributes most to poor air quality in Delhi. Therefore, air quality mitigation strategies in Delhi and surrounding regions are used to control this issue.
Andrea Pazmiño, Florence Goutail, Sophie Godin-Beekmann, Alain Hauchecorne, Jean-Pierre Pommereau, Martyn P. Chipperfield, Wuhu Feng, Franck Lefèvre, Audrey Lecouffe, Michel Van Roozendael, Nis Jepsen, Georg Hansen, Rigel Kivi, Kimberly Strong, and Kaley A. Walker
Atmos. Chem. Phys., 23, 15655–15670, https://doi.org/10.5194/acp-23-15655-2023, https://doi.org/10.5194/acp-23-15655-2023, 2023
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The vortex-averaged ozone loss over the last 3 decades is evaluated for both polar regions using the passive ozone tracer of the chemical transport model TOMCAT/SLIMCAT and total ozone observations from the SAOZ network and MSR2 reanalysis. Three metrics were developed to compute ozone trends since 2000. The study confirms the ozone recovery in the Antarctic and shows a potential sign of quantitative detection of ozone recovery in the Arctic that needs to be robustly confirmed in the future.
Richard J. Pope, Brian J. Kerridge, Richard Siddans, Barry G. Latter, Martyn P. Chipperfield, Wuhu Feng, Matilda A. Pimlott, Sandip S. Dhomse, Christian Retscher, and Richard Rigby
Atmos. Chem. Phys., 23, 14933–14947, https://doi.org/10.5194/acp-23-14933-2023, https://doi.org/10.5194/acp-23-14933-2023, 2023
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Ozone is a potent air pollutant, and we present the first study to investigate long-term changes in lower tropospheric column ozone (LTCO3) from space. We have constructed a merged LTCO3 dataset from GOME-1, SCIAMACHY and OMI between 1996 and 2017. Comparing LTCO3 between the 1996–2000 and 2013–2017 5-year averages, we find significant positive increases in the tropics/sub-tropics, while in the northern mid-latitudes, we find small-scale differences.
Penghao Tian, Bingkun Yu, Hailun Ye, Xianghui Xue, Jianfei Wu, and Tingdi Chen
Atmos. Chem. Phys., 23, 13413–13431, https://doi.org/10.5194/acp-23-13413-2023, https://doi.org/10.5194/acp-23-13413-2023, 2023
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Modeling and prediction of ionospheric irregularities is an important topic in upper-atmospheric and upper-ionospheric physics. We proposed an artificial intelligence model to reconstruct the E-region ionospheric irregularities and first developed an open-source application for the community. The model reveals complex relationships between ionospheric irregularities and external driving factors. The findings suggest that spatiotemporal information plays an important role in the reconstruction.
John M. C. Plane, Jörg Gumbel, Konstantinos S. Kalogerakis, Daniel R. Marsh, and Christian von Savigny
Atmos. Chem. Phys., 23, 13255–13282, https://doi.org/10.5194/acp-23-13255-2023, https://doi.org/10.5194/acp-23-13255-2023, 2023
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The mesosphere or lower thermosphere region of the atmosphere borders the edge of space. It is subject to extreme ultraviolet photons and charged particles from the Sun and atmospheric gravity waves from below, which tend to break in this region. The pressure is very low, which facilitates chemistry involving species in excited states, and this is also the region where cosmic dust ablates and injects various metals. The result is a unique and exotic chemistry.
Richard J. Pope, Brian J. Kerridge, Martyn P. Chipperfield, Richard Siddans, Barry G. Latter, Lucy J. Ventress, Matilda A. Pimlott, Wuhu Feng, Edward Comyn-Platt, Garry D. Hayman, Stephen R. Arnold, and Ailish M. Graham
Atmos. Chem. Phys., 23, 13235–13253, https://doi.org/10.5194/acp-23-13235-2023, https://doi.org/10.5194/acp-23-13235-2023, 2023
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In the summer of 2018, Europe experienced several persistent large-scale ozone (O3) pollution episodes. Satellite tropospheric O3 and surface O3 data recorded substantial enhancements in 2018 relative to other years. Targeted model simulations showed that meteorological processes and emissions controlled the elevated surface O3, while mid-tropospheric O3 enhancements were dominated by stratospheric O3 intrusion and advection of North Atlantic O3-rich air masses into Europe.
Yajuan Li, Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Jianchun Bian, Yuan Xia, and Dong Guo
Atmos. Chem. Phys., 23, 13029–13047, https://doi.org/10.5194/acp-23-13029-2023, https://doi.org/10.5194/acp-23-13029-2023, 2023
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For the first time a regularized multivariate regression model is used to estimate stratospheric ozone trends. Regularized regression avoids the over-fitting issue due to correlation among explanatory variables. We demonstrate that there are considerable differences in satellite-based and chemical-model-based ozone trends, highlighting large uncertainties in our understanding about ozone variability. We argue that caution is needed when interpreting results with different methods and datasets.
Michael P. Cartwright, Richard J. Pope, Jeremy J. Harrison, Martyn P. Chipperfield, Chris Wilson, Wuhu Feng, David P. Moore, and Parvadha Suntharalingam
Atmos. Chem. Phys., 23, 10035–10056, https://doi.org/10.5194/acp-23-10035-2023, https://doi.org/10.5194/acp-23-10035-2023, 2023
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A 3-D chemical transport model, TOMCAT, is used to simulate global atmospheric carbonyl sulfide (OCS) distribution. Modelled OCS compares well with satellite observations of OCS from limb-sounding satellite observations. Model simulations also compare adequately with surface and atmospheric observations and suitably capture the seasonality of OCS and background concentrations.
Robert Wagner, Alexander D. James, Victoria L. Frankland, Ottmar Möhler, Benjamin J. Murray, John M. C. Plane, Harald Saathoff, Ralf Weigel, and Martin Schnaiter
Atmos. Chem. Phys., 23, 6789–6811, https://doi.org/10.5194/acp-23-6789-2023, https://doi.org/10.5194/acp-23-6789-2023, 2023
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Polar stratospheric clouds (PSCs) play an important role in the depletion of stratospheric ozone. They can consist of different chemical species, including crystalline nitric acid hydrates. We found that mineral dust or meteoric ablation material can efficiently catalyse the formation of a specific phase of nitric acid dihydrate crystals. We determined predominant particle shapes and infrared optical properties of these crystals, which are important inputs for remote sensing detection of PSCs.
Xu Zhou, Xinan Yue, Yihui Cai, Zhipeng Ren, Yong Wei, and Yongxin Pan
Atmos. Chem. Phys., 23, 6383–6393, https://doi.org/10.5194/acp-23-6383-2023, https://doi.org/10.5194/acp-23-6383-2023, 2023
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Secular variations in CO2 concentration and geomagnetic field can affect the dynamics of the upper atmosphere. We examine how these two factors influence the dynamics of the upper atmosphere during the Holocene, using two sets of ~ 12 000-year control runs by the coupled thermosphere–ionosphere model. The main results show that (a) increased CO2 enhances the thermospheric circulation, but non-linearly; and (b) geomagnetic variation induced a significant hemispheric asymmetrical effect.
Yihui Cai, Xinan Yue, Xu Zhou, Zhipeng Ren, Yong Wei, and Yongxin Pan
Atmos. Chem. Phys., 23, 5009–5021, https://doi.org/10.5194/acp-23-5009-2023, https://doi.org/10.5194/acp-23-5009-2023, 2023
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On timescales longer than the solar cycle, secular changes in CO2 concentration and geomagnetic field play a key role in influencing the thermosphere. We performed four sets of ~12000-year control runs with the coupled thermosphere–ionosphere model to examine the effects of the geomagnetic field, CO2, and solar activity on thermospheric density and temperature, deepening our understanding of long-term changes in the thermosphere and making projections for future thermospheric changes.
Alexander D. James, Finn Pace, Sebastien N. F. Sikora, Graham W. Mann, John M. C. Plane, and Benjamin J. Murray
Atmos. Chem. Phys., 23, 2215–2233, https://doi.org/10.5194/acp-23-2215-2023, https://doi.org/10.5194/acp-23-2215-2023, 2023
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Here, we examine whether several materials of meteoric origin can nucleate crystallisation in stratospheric cloud droplets which would affect ozone depletion. We find that material which could fragment on atmospheric entry without melting is unlikely to be present in high enough concentration in the stratosphere to contribute to observed crystalline clouds. Material which ablates completely then forms a new solid known as meteoric smoke can provide enough nucleation to explain observed clouds.
Cornelius Csar Jude H. Salinas, Dong L. Wu, Jae N. Lee, Loren C. Chang, Liying Qian, and Hanli Liu
Atmos. Chem. Phys., 23, 1705–1730, https://doi.org/10.5194/acp-23-1705-2023, https://doi.org/10.5194/acp-23-1705-2023, 2023
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Upper mesospheric carbon monoxide's (CO) photochemical lifetime is longer than dynamical timescales. This work uses satellite observations and model simulations to establish that the migrating diurnal tide and its seasonal and interannual variabilities drive CO primarily through vertical advection. Vertical advection is a transport process that is currently difficult to observe. This work thus shows that we can use CO as a tracer for vertical advection across seasonal and interannual timescales.
Wen Yi, Jie Zeng, Xianghui Xue, Iain Reid, Wei Zhong, Jianfei Wu, Tingdi Chen, and Xiankang Dou
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2022-254, https://doi.org/10.5194/amt-2022-254, 2022
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In recent years, the concept of multistatic meteor radar systems has attracted the attention of the atmospheric radar community, focusing on the MLT region. In this study, we apply a multistatic meteor radar system consisting of a monostatic meteor radar in Mengcheng (33.36° N, 116.49° E) and a remote receiver in Changfeng (31.98° N, 117.22° E) to estimate the two-dimensional horizontal wind field, and the horizontal divergence and relative vorticity of the wind field.
Qinzeng Li, Jiyao Xu, Hanli Liu, Xiao Liu, and Wei Yuan
Atmos. Chem. Phys., 22, 12077–12091, https://doi.org/10.5194/acp-22-12077-2022, https://doi.org/10.5194/acp-22-12077-2022, 2022
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We use ground-based airglow network observations, reanalysis data, and satellite observations to explore the propagation process of concentric gravity waves (CGWs) excited by a typhoon between the troposphere, stratosphere, mesosphere, and thermosphere. We find that CGWs in the mesosphere are generated directly by the typhoon but the CGW observed in the thermosphere may be excited by CGW dissipation in the mesosphere, rather than directly excited by a typhoon and propagated to the thermosphere.
Bingkun Yu, Xianghui Xue, Christopher J. Scott, Mingjiao Jia, Wuhu Feng, John M. C. Plane, Daniel R. Marsh, Jonas Hedin, Jörg Gumbel, and Xiankang Dou
Atmos. Chem. Phys., 22, 11485–11504, https://doi.org/10.5194/acp-22-11485-2022, https://doi.org/10.5194/acp-22-11485-2022, 2022
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We present a study on the climatology of the metal sodium layer in the upper atmosphere from the ground-based measurements obtained from a lidar network, the Odin satellite measurements, and a global model of meteoric sodium in the atmosphere. Comprehensively, comparisons show good agreement and some discrepancies between ground-based observations, satellite measurements, and global model simulations.
Shican Qiu, Mengzhen Yuan, Willie Soon, Victor Manuel Velasco Herrera, Zhanming Zhang, and Xiankang Dou
Ann. Geophys. Discuss., https://doi.org/10.5194/angeo-2022-22, https://doi.org/10.5194/angeo-2022-22, 2022
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In this paper, the solar radiation index Y10 acts as an indicator of the solar activity, and the vertical column of ice water content (IWC) characterizes the nature of the polar mesosphere cloud (PMC). Superposed epoch analysis is used to determine the time lag days of temperature and IWC anomalies in responding to Y10 for the PMC seasons from 2007–2015. The results show that the IWC can respond quickly to temperature within time lag of one day.
Yajuan Li, Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Andreas Chrysanthou, Yuan Xia, and Dong Guo
Atmos. Chem. Phys., 22, 10635–10656, https://doi.org/10.5194/acp-22-10635-2022, https://doi.org/10.5194/acp-22-10635-2022, 2022
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Chemical transport models forced with (re)analysis meteorological fields are ideally suited for interpreting the influence of important physical processes on the ozone variability. We use TOMCAT forced by ECMWF ERA-Interim and ERA5 reanalysis data sets to investigate the effects of reanalysis forcing fields on ozone changes. Our results show that models forced by ERA5 reanalyses may not yet be capable of reproducing observed changes in stratospheric ozone, particularly in the lower stratosphere.
Matilda A. Pimlott, Richard J. Pope, Brian J. Kerridge, Barry G. Latter, Diane S. Knappett, Dwayne E. Heard, Lucy J. Ventress, Richard Siddans, Wuhu Feng, and Martyn P. Chipperfield
Atmos. Chem. Phys., 22, 10467–10488, https://doi.org/10.5194/acp-22-10467-2022, https://doi.org/10.5194/acp-22-10467-2022, 2022
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We present a new method to derive global information of the hydroxyl radical (OH), an important atmospheric oxidant. OH controls the lifetime of trace gases important to air quality and climate. We use satellite observations of ozone, carbon monoxide, methane and water vapour in a simple expression to derive OH around 3–4 km altitude. The derived OH compares well to model and aircraft OH data. We then apply the method to 10 years of satellite data to study the inter-annual variability of OH.
Yetao Cen, Chengyun Yang, Tao Li, James M. Russell III, and Xiankang Dou
Atmos. Chem. Phys., 22, 7861–7874, https://doi.org/10.5194/acp-22-7861-2022, https://doi.org/10.5194/acp-22-7861-2022, 2022
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The MLT DW1 amplitude is suppressed during El Niño winters in both satellite observation and SD-WACCM simulations. The suppressed Hough mode (1, 1) in the tropopause region propagates vertically to the MLT region, leading to decreased DW1 amplitude. The latitudinal zonal wind shear anomalies during El Niño winters would narrow the waveguide and prevent the vertical propagation of DW1. The gravity wave drag excited by ENSO-induced anomalous convection could also modulate the MLT DW1 amplitude.
Dawei Tang, Tianwen Wei, Jinlong Yuan, Haiyun Xia, and Xiankang Dou
Atmos. Meas. Tech., 15, 2819–2838, https://doi.org/10.5194/amt-15-2819-2022, https://doi.org/10.5194/amt-15-2819-2022, 2022
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During 11–20 March 2020, three aerosol transport events were investigated by a lidar system and an online bioaerosol detection system in Hefei, China.
Observation results reveal that the events not only contributed to high particulate matter pollution but also to the transport of external bioaerosols, resulting in changes in the fraction of fluorescent biological aerosol particles.
This detection method improved the time resolution and provided more parameters for aerosol detection.
Shican Qiu, Mengxi Shi, Willie Soon, Mingjiao Jia, Xianghui Xue, Tao Li, Peng Ju, and Xiankang Dou
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-1085, https://doi.org/10.5194/acp-2021-1085, 2022
Revised manuscript not accepted
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The solitary wave theory is applied for the first time to study the sporadic sodium layers (NaS). We perform soliton fitting processes on the observed data from the Andes Lidar Observatory, and find out that 24/27 NaS events exhibit similar features to a soliton. Time series of the net anomaly reveal the same variation process to the solution of a five-order KdV equation. Our results suggest the NaS phenomenon would be an appropriate tracer for nonlinear wave studies in the atmosphere.
Davide Zanchettin, Claudia Timmreck, Myriam Khodri, Anja Schmidt, Matthew Toohey, Manabu Abe, Slimane Bekki, Jason Cole, Shih-Wei Fang, Wuhu Feng, Gabriele Hegerl, Ben Johnson, Nicolas Lebas, Allegra N. LeGrande, Graham W. Mann, Lauren Marshall, Landon Rieger, Alan Robock, Sara Rubinetti, Kostas Tsigaridis, and Helen Weierbach
Geosci. Model Dev., 15, 2265–2292, https://doi.org/10.5194/gmd-15-2265-2022, https://doi.org/10.5194/gmd-15-2265-2022, 2022
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This paper provides metadata and first analyses of the volc-pinatubo-full experiment of CMIP6-VolMIP. Results from six Earth system models reveal significant differences in radiative flux anomalies that trace back to different implementations of volcanic forcing. Surface responses are in contrast overall consistent across models, reflecting the large spread due to internal variability. A second phase of VolMIP shall consider both aspects toward improved protocol for volc-pinatubo-full.
Sandip S. Dhomse, Martyn P. Chipperfield, Wuhu Feng, Ryan Hossaini, Graham W. Mann, Michelle L. Santee, and Mark Weber
Atmos. Chem. Phys., 22, 903–916, https://doi.org/10.5194/acp-22-903-2022, https://doi.org/10.5194/acp-22-903-2022, 2022
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Solar flux variations associated with 11-year sunspot cycle is believed to exert important external climate forcing. As largest variations occur at shorter wavelengths such as ultra-violet part of the solar spectrum, associated changes in stratospheric ozone are thought to provide direct evidence for solar climate interaction. Until now, most of the studies reported double-peak structured solar cycle signal (SCS), but relatively new satellite data suggest only single-peak-structured SCS.
Ioannis A. Daglis, Loren C. Chang, Sergio Dasso, Nat Gopalswamy, Olga V. Khabarova, Emilia Kilpua, Ramon Lopez, Daniel Marsh, Katja Matthes, Dibyendu Nandy, Annika Seppälä, Kazuo Shiokawa, Rémi Thiéblemont, and Qiugang Zong
Ann. Geophys., 39, 1013–1035, https://doi.org/10.5194/angeo-39-1013-2021, https://doi.org/10.5194/angeo-39-1013-2021, 2021
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We present a detailed account of the science programme PRESTO (PREdictability of the variable Solar–Terrestrial cOupling), covering the period 2020 to 2024. PRESTO was defined by a dedicated committee established by SCOSTEP (Scientific Committee on Solar-Terrestrial Physics). We review the current state of the art and discuss future studies required for the most effective development of solar–terrestrial physics.
Sandip S. Dhomse, Carlo Arosio, Wuhu Feng, Alexei Rozanov, Mark Weber, and Martyn P. Chipperfield
Earth Syst. Sci. Data, 13, 5711–5729, https://doi.org/10.5194/essd-13-5711-2021, https://doi.org/10.5194/essd-13-5711-2021, 2021
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High-quality long-term ozone profile data sets are key to estimating short- and long-term ozone variability. Almost all the satellite (and chemical model) data sets show some kind of bias with respect to each other. This is because of differences in measurement methodologies as well as simplified processes in the models. We use satellite data sets and chemical model output to generate 42 years of ozone profile data sets using a random-forest machine-learning algorithm that is named ML-TOMCAT.
Liang Tang, Sheng-Yang Gu, and Xian-Kang Dou
Atmos. Chem. Phys., 21, 17495–17512, https://doi.org/10.5194/acp-21-17495-2021, https://doi.org/10.5194/acp-21-17495-2021, 2021
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Our study explores the variation in the occurrence date, peak amplitude and wave period for eastward waves and the role of instability, background wind structure and the critical layer in eastward wave propagation and amplification.
Jianfei Wu, Wuhu Feng, Han-Li Liu, Xianghui Xue, Daniel Robert Marsh, and John Maurice Campbell Plane
Atmos. Chem. Phys., 21, 15619–15630, https://doi.org/10.5194/acp-21-15619-2021, https://doi.org/10.5194/acp-21-15619-2021, 2021
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Metal layers occur in the MLT region (80–120 km) from the ablation of cosmic dust. The latest lidar observations show these metals can reach a height approaching 200 km, which is challenging to explain. We have developed the first global simulation incorporating the full life cycle of metal atoms and ions. The model results compare well with lidar and satellite observations of the seasonal and diurnal variation of the metals and demonstrate the importance of ion mass and ion-neutral coupling.
Jayanarayanan Kuttippurath, Wuhu Feng, Rolf Müller, Pankaj Kumar, Sarath Raj, Gopalakrishna Pillai Gopikrishnan, and Raina Roy
Atmos. Chem. Phys., 21, 14019–14037, https://doi.org/10.5194/acp-21-14019-2021, https://doi.org/10.5194/acp-21-14019-2021, 2021
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The Arctic winter/spring 2020 was one of the coldest with a strong and long-lasting vortex, high chlorine activation, severe denitrification, and unprecedented ozone loss. The loss was even equal to the levels of some of the warm Antarctic winters. Total column ozone values below 220 DU for several weeks and ozone loss saturation were observed during the period. These results show an unusual meteorology and warrant dedicated studies on the impact of climate change on ozone loss.
Gunter Stober, Ales Kuchar, Dimitry Pokhotelov, Huixin Liu, Han-Li Liu, Hauke Schmidt, Christoph Jacobi, Kathrin Baumgarten, Peter Brown, Diego Janches, Damian Murphy, Alexander Kozlovsky, Mark Lester, Evgenia Belova, Johan Kero, and Nicholas Mitchell
Atmos. Chem. Phys., 21, 13855–13902, https://doi.org/10.5194/acp-21-13855-2021, https://doi.org/10.5194/acp-21-13855-2021, 2021
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Little is known about the climate change of wind systems in the mesosphere and lower thermosphere at the edge of space at altitudes from 70–110 km. Meteor radars represent a well-accepted remote sensing technique to measure winds at these altitudes. Here we present a state-of-the-art climatological interhemispheric comparison using continuous and long-lasting observations from worldwide distributed meteor radars from the Arctic to the Antarctic and sophisticated general circulation models.
Shican Qiu, Ning Wang, Willie Soon, Gaopeng Lu, Mingjiao Jia, Xingjin Wang, Xianghui Xue, Tao Li, and Xiankang Dou
Atmos. Chem. Phys., 21, 11927–11940, https://doi.org/10.5194/acp-21-11927-2021, https://doi.org/10.5194/acp-21-11927-2021, 2021
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Our results suggest that lightning strokes would probably influence the ionosphere and thus give rise to the occurrence of a sporadic sodium layer (NaS), with the overturning of the electric field playing an important role. Model simulation results show that the calculated first-order rate coefficient could explain the efficient recombination of Na+→Na in this NaS case study. A conjunction between the lower and upper atmospheres could be established by these inter-connected phenomena.
Ville Maliniemi, Hilde Nesse Tyssøy, Christine Smith-Johnsen, Pavle Arsenovic, and Daniel R. Marsh
Atmos. Chem. Phys., 21, 11041–11052, https://doi.org/10.5194/acp-21-11041-2021, https://doi.org/10.5194/acp-21-11041-2021, 2021
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We simulate ozone variability over the 21st century with different greenhouse gas scenarios. Our results highlight a novel mechanism of additional reactive nitrogen species descending to the Antarctic stratosphere from the thermosphere/upper mesosphere due to the accelerated residual circulation under climate change. This excess descending NOx can potentially prevent a super recovery of ozone in the Antarctic upper stratosphere.
Michael Kiefer, Thomas von Clarmann, Bernd Funke, Maya García-Comas, Norbert Glatthor, Udo Grabowski, Sylvia Kellmann, Anne Kleinert, Alexandra Laeng, Andrea Linden, Manuel López-Puertas, Daniel R. Marsh, and Gabriele P. Stiller
Atmos. Meas. Tech., 14, 4111–4138, https://doi.org/10.5194/amt-14-4111-2021, https://doi.org/10.5194/amt-14-4111-2021, 2021
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An improved dataset of vertical temperature profiles of the Earth's atmosphere in the altitude range 5–70 km is presented. These profiles are derived from measurements of the MIPAS instrument onboard ESA's Envisat satellite. The overall improvements are based on upgrades in the input data and several improvements in the data processing approach. Both of these are discussed, and an extensive error discussion is included. Enhancements of the new dataset are demonstrated by means of examples.
Wei Zhong, Xianghui Xue, Wen Yi, Iain M. Reid, Tingdi Chen, and Xiankang Dou
Atmos. Meas. Tech., 14, 3973–3988, https://doi.org/10.5194/amt-14-3973-2021, https://doi.org/10.5194/amt-14-3973-2021, 2021
Mingzhe Li and Xinan Yue
Atmos. Meas. Tech., 14, 3003–3013, https://doi.org/10.5194/amt-14-3003-2021, https://doi.org/10.5194/amt-14-3003-2021, 2021
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In this study, we statistically analyzed the correlation between the ionospheric irregularity and the quality of the GNSS atmospheric radio occultation (RO) products. The results show that the ionospheric irregularity could affect the GNSS atmospheric RO in terms of causing failed inverted RO events and the bending angle oscillation. Awareness of the ionospheric irregularity effect on RO could be beneficial to improve the RO data quality for weather and climate research.
Christopher J. Scott, Shannon Jones, and Luke A. Barnard
Ann. Geophys., 39, 309–319, https://doi.org/10.5194/angeo-39-309-2021, https://doi.org/10.5194/angeo-39-309-2021, 2021
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The composition of the upper atmosphere has been difficult to measure with localised observations relying on spacecraft, suborbital rockets or measurements of airglow from ground-based observatories. The height profile of ionisation within the neutral upper atmosphere is influenced by the composition of the neutral gas. We present a method for determining the neutral upper-atmosphere composition from measurements of the ionisation profile and compare these with spacecraft measurements.
Minna Palmroth, Maxime Grandin, Theodoros Sarris, Eelco Doornbos, Stelios Tourgaidis, Anita Aikio, Stephan Buchert, Mark A. Clilverd, Iannis Dandouras, Roderick Heelis, Alex Hoffmann, Nickolay Ivchenko, Guram Kervalishvili, David J. Knudsen, Anna Kotova, Han-Li Liu, David M. Malaspina, Günther March, Aurélie Marchaudon, Octav Marghitu, Tomoko Matsuo, Wojciech J. Miloch, Therese Moretto-Jørgensen, Dimitris Mpaloukidis, Nils Olsen, Konstantinos Papadakis, Robert Pfaff, Panagiotis Pirnaris, Christian Siemes, Claudia Stolle, Jonas Suni, Jose van den IJssel, Pekka T. Verronen, Pieter Visser, and Masatoshi Yamauchi
Ann. Geophys., 39, 189–237, https://doi.org/10.5194/angeo-39-189-2021, https://doi.org/10.5194/angeo-39-189-2021, 2021
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This is a review paper that summarises the current understanding of the lower thermosphere–ionosphere (LTI) in terms of measurements and modelling. The LTI is the transition region between space and the atmosphere and as such of tremendous importance to both the domains of space and atmosphere. The paper also serves as the background for European Space Agency Earth Explorer 10 candidate mission Daedalus.
Tong Dang, Binzheng Zhang, Jiuhou Lei, Wenbin Wang, Alan Burns, Han-li Liu, Kevin Pham, and Kareem A. Sorathia
Geosci. Model Dev., 14, 859–873, https://doi.org/10.5194/gmd-14-859-2021, https://doi.org/10.5194/gmd-14-859-2021, 2021
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This paper describes a numerical treatment (ring average) to relax the time step in finite-difference schemes when using spherical and cylindrical coordinates with axis singularities. The ring average is used to develop a high-resolution thermosphere–ionosphere coupled community model. The technique is a significant improvement in space weather modeling capability, and it can also be adapted to more general finite-difference solvers for hyperbolic equations in spherical and polar geometries.
Jianyuan Wang, Wen Yi, Jianfei Wu, Tingdi Chen, Xianghui Xue, Robert A. Vincent, Iain M. Reid, Paulo P. Batista, Ricardo A. Buriti, Toshitaka Tsuda, and Xiankang Dou
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-33, https://doi.org/10.5194/acp-2021-33, 2021
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In this study, we report the climatology of migrating and non-migrating tides in mesopause winds estimated using multiyear observations from three meteor radars in the southern equatorial region. The results reveal that the climatological patterns of tidal amplitudes by meteor radars is similar to the Climatological Tidal Model of the Thermosphere (CTMT) results and the differences are mainly due to the effect of the stratospheric sudden warming (SSW) event.
Arseniy Karagodin-Doyennel, Eugene Rozanov, Ales Kuchar, William Ball, Pavle Arsenovic, Ellis Remsberg, Patrick Jöckel, Markus Kunze, David A. Plummer, Andrea Stenke, Daniel Marsh, Doug Kinnison, and Thomas Peter
Atmos. Chem. Phys., 21, 201–216, https://doi.org/10.5194/acp-21-201-2021, https://doi.org/10.5194/acp-21-201-2021, 2021
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The solar signal in the mesospheric H2O and CO was extracted from the CCMI-1 model simulations and satellite observations using multiple linear regression (MLR) analysis. MLR analysis shows a pronounced and statistically robust solar signal in both H2O and CO. The model results show a general agreement with observations reproducing a negative/positive solar signal in H2O/CO. The pattern of the solar signal varies among the considered models, reflecting some differences in the model setup.
Xiao Liu, Jiyao Xu, Jia Yue, and Hanli Liu
Atmos. Chem. Phys., 20, 14437–14456, https://doi.org/10.5194/acp-20-14437-2020, https://doi.org/10.5194/acp-20-14437-2020, 2020
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Large wind shears in the mesosphere and lower thermosphere are recognized as a common phenomenon. Simulation and ground-based observations show that the main contributor of large wind shears is gravity waves. We present a method of deriving wind shears induced by gravity waves according to the linear theory and using the global temperature observations by SABER (Sounding of the Atmosphere using Broadband Emission Radiometry). Our results agree well with observations and model simulations.
Benjamin Birner, Martyn P. Chipperfield, Eric J. Morgan, Britton B. Stephens, Marianna Linz, Wuhu Feng, Chris Wilson, Jonathan D. Bent, Steven C. Wofsy, Jeffrey Severinghaus, and Ralph F. Keeling
Atmos. Chem. Phys., 20, 12391–12408, https://doi.org/10.5194/acp-20-12391-2020, https://doi.org/10.5194/acp-20-12391-2020, 2020
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With new high-precision observations from nine aircraft campaigns and 3-D chemical transport modeling, we show that the argon-to-nitrogen ratio (Ar / N2) in the lowermost stratosphere provides a useful constraint on the “age of air” (the time elapsed since entry of an air parcel into the stratosphere). Therefore, Ar / N2 in combination with traditional age-of-air indicators, such as CO2 and N2O, could provide new insights into atmospheric mixing and transport.
Thomas R. Lewis, Juan Carlos Gómez Martín, Mark A. Blitz, Carlos A. Cuevas, John M. C. Plane, and Alfonso Saiz-Lopez
Atmos. Chem. Phys., 20, 10865–10887, https://doi.org/10.5194/acp-20-10865-2020, https://doi.org/10.5194/acp-20-10865-2020, 2020
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Iodine-bearing gasses emitted from the sea surface are chemically processed in the atmosphere, leading to iodine accumulation in aerosol and transport to continental ecosystems. Such processing involves light-induced break-up of large, particle-forming iodine oxides into smaller, ozone-depleting molecules. We combine experiments and theory to report the photolysis efficiency of iodine oxides required to assess the impact of iodine on ozone depletion and particle formation.
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Short summary
A long-standing mystery of metal ions within Es layers in the Earth's upper atmosphere is the marked seasonal dependence, with a summer maximum and a winter minimum. We report a large-scale winter-to-summer transport of metal ions from 6-year multi-satellite observations and worldwide ground-based stations. A global atmospheric circulation is responsible for the phenomenon. Our results emphasise the effect of this atmospheric circulation on the transport of composition in the upper atmosphere.
A long-standing mystery of metal ions within Es layers in the Earth's upper atmosphere is the...
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