Articles | Volume 21, issue 2
https://doi.org/10.5194/acp-21-1341-2021
https://doi.org/10.5194/acp-21-1341-2021
Measurement report
 | 
01 Feb 2021
Measurement report |  | 01 Feb 2021

Measurement report: Effects of photochemical aging on the formation and evolution of summertime secondary aerosol in Beijing

Tianzeng Chen, Jun Liu, Qingxin Ma, Biwu Chu, Peng Zhang, Jinzhu Ma, Yongchun Liu, Cheng Zhong, Pengfei Liu, Yafei Wang, Yujing Mu, and Hong He

Related authors

A study on the influence of inorganic ions, organic carbon and microstructure on the hygroscopic property of soot
Zhanyu Su, Lanxiadi Chen, Yuan Liu, Peng Zhang, Tianzeng Chen, Biwu Chu, Mingjin Tang, Qingxin Ma, and Hong He
Atmos. Chem. Phys., 24, 993–1003, https://doi.org/10.5194/acp-24-993-2024,https://doi.org/10.5194/acp-24-993-2024, 2024
Short summary
Evaluation of the first year of Pandora NO2 measurements over Beijing and application to satellite validation
Ouyang Liu, Zhengqiang Li, Yangyan Lin, Cheng Fan, Ying Zhang, Kaitao Li, Peng Zhang, Yuanyuan Wei, Tianzeng Chen, Jiantao Dong, and Gerrit de Leeuw
Atmos. Meas. Tech., 17, 377–395, https://doi.org/10.5194/amt-17-377-2024,https://doi.org/10.5194/amt-17-377-2024, 2024
Short summary
Increased primary and secondary H2SO4 showing the opposing roles in secondary organic aerosol formation from ethyl methacrylate ozonolysis
Peng Zhang, Tianzeng Chen, Jun Liu, Guangyan Xu, Qingxin Ma, Biwu Chu, Wanqi Sun, and Hong He
Atmos. Chem. Phys., 21, 7099–7112, https://doi.org/10.5194/acp-21-7099-2021,https://doi.org/10.5194/acp-21-7099-2021, 2021
Short summary
Significant source of secondary aerosol: formation from gasoline evaporative emissions in the presence of SO2 and NH3
Tianzeng Chen, Yongchun Liu, Qingxin Ma, Biwu Chu, Peng Zhang, Changgeng Liu, Jun Liu, and Hong He
Atmos. Chem. Phys., 19, 8063–8081, https://doi.org/10.5194/acp-19-8063-2019,https://doi.org/10.5194/acp-19-8063-2019, 2019
Short summary
Enhancement of secondary organic aerosol formation and its oxidation state by SO2 during photooxidation of 2-methoxyphenol
Changgeng Liu, Tianzeng Chen, Yongchun Liu, Jun Liu, Hong He, and Peng Zhang
Atmos. Chem. Phys., 19, 2687–2700, https://doi.org/10.5194/acp-19-2687-2019,https://doi.org/10.5194/acp-19-2687-2019, 2019
Short summary

Related subject area

Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Source apportionment and ecotoxicity of PM2.5 pollution events in a major Southern Hemisphere megacity: influence of a biofuel-impacted fleet and biomass burning
Guilherme Martins Pereira, Leonardo Yoshiaki Kamigauti, Rubens Fabio Pereira, Djacinto Monteiro dos Santos, Thayná da Silva Santos, José Vinicius Martins, Célia Alves, Cátia Gonçalves, Ismael Casotti Rienda, Nora Kováts, Thiago Nogueira, Luciana Rizzo, Paulo Artaxo, Regina Maura de Miranda, Marcia Akemi Yamasoe, Edmilson Dias de Freitas, Pérola de Castro Vasconcellos, and Maria de Fatima Andrade
Atmos. Chem. Phys., 25, 4587–4616, https://doi.org/10.5194/acp-25-4587-2025,https://doi.org/10.5194/acp-25-4587-2025, 2025
Short summary
Marine organic aerosol at Mace Head: effects from phytoplankton and source region variability
Emmanuel Chevassus, Kirsten N. Fossum, Darius Ceburnis, Lu Lei, Chunshui Lin, Wei Xu, Colin O'Dowd, and Jurgita Ovadnevaite
Atmos. Chem. Phys., 25, 4107–4129, https://doi.org/10.5194/acp-25-4107-2025,https://doi.org/10.5194/acp-25-4107-2025, 2025
Short summary
Measurement report: Sources and meteorology influencing highly time-resolved PM2.5 trace elements at three urban sites in the extremely polluted Indo-Gangetic Plain in India
Ashutosh K. Shukla, Sachchida N. Tripathi, Shamitaksha Talukdar, Vishnu Murari, Sreenivas Gaddamidi, Manousos-Ioannis Manousakas, Vipul Lalchandani, Kuldeep Dixit, Vinayak M. Ruge, Peeyush Khare, Mayank Kumar, Vikram Singh, Neeraj Rastogi, Suresh Tiwari, Atul K. Srivastava, Dilip Ganguly, Kaspar Rudolf Daellenbach, and André S. H. Prévôt
Atmos. Chem. Phys., 25, 3765–3784, https://doi.org/10.5194/acp-25-3765-2025,https://doi.org/10.5194/acp-25-3765-2025, 2025
Short summary
Formation of highly absorptive secondary brown carbon through nighttime multiphase chemistry of biomass burning emissions
Ye Kuang, Biao Luo, Shan Huang, Junwen Liu, Weiwei Hu, Yuwen Peng, Duohong Chen, Dingli Yue, Wanyun Xu, Bin Yuan, and Min Shao
Atmos. Chem. Phys., 25, 3737–3752, https://doi.org/10.5194/acp-25-3737-2025,https://doi.org/10.5194/acp-25-3737-2025, 2025
Short summary
Measurement report: Vertically resolved atmospheric properties observed over the Southern Great Plains with the ArcticShark uncrewed aerial system
Fan Mei, Qi Zhang, Damao Zhang, Jerome D. Fast, Gourihar Kulkarni, Mikhail S. Pekour, Christopher R. Niedek, Susanne Glienke, Israel Silber, Beat Schmid, Jason M. Tomlinson, Hardeep S. Mehta, Xena Mansoura, Zezhen Cheng, Gregory W. Vandergrift, Nurun Nahar Lata, Swarup China, and Zihua Zhu
Atmos. Chem. Phys., 25, 3425–3444, https://doi.org/10.5194/acp-25-3425-2025,https://doi.org/10.5194/acp-25-3425-2025, 2025
Short summary

Cited articles

An, Z., Huang, R.-J., Zhang, R., Tie, X., Li, G., Cao, J., Zhou, W., Shi, Z., Han, Y., Gu, Z., and Ji, Y.: Severe haze in northern China: A synergy of anthropogenic emissions and atmospheric processes, P. Natl. Acad. Sci. USA, 116, 8657–8666, https://doi.org/10.1073/pnas.1900125116, 2019. 
Atkinson, R. and Arey, J.: Atmospheric degradation of volatile organic compounds, Chem. Rev., 103, 4605–4638, https://doi.org/10.1021/cr0206420, 2003. 
Canagaratna, M. R., Jimenez, J. L., Kroll, J. H., Chen, Q., Kessler, S. H., Massoli, P., Hildebrandt Ruiz, L., Fortner, E., Williams, L. R., Wilson, K. R., Surratt, J. D., Donahue, N. M., Jayne, J. T., and Worsnop, D. R.: Elemental ratio measurements of organic compounds using aerosol mass spectrometry: characterization, improved calibration, and implications, Atmos. Chem. Phys., 15, 253–272, https://doi.org/10.5194/acp-15-253-2015, 2015. 
Chen, Q., Heald, C. L., Jimenez, J. L., Canagaratna, M. R., Zhang, Q., He, L.-Y., Huang, X.-F., Campuzano-Jost, P., Palm, B. B., Poulain, L., Kuwata, M., Martin, S. T., Abbatt, J. P. D., Lee, A. K. Y., and Liggio, J.: Elemental composition of organic aerosol: The gap between ambient and laboratory measurements, Geophys. Res. Lett., 42, 4182–4189, https://doi.org/10.1002/2015gl063693, 2015. 
Download
Short summary
Effects of photochemical aging on the formation and evolution of summertime secondary aerosol were systematically investigated in a suburb of Beijing. Higher PM1 concentration accompanied longer photochemical age (ta). Sulfate and more-oxidized OOA formation were significantly sensitive to the increase in ta, and their contributions were greatly enhanced at elevated ta levels. Our results suggested that photochemical aging process played a crucial role in PM1 and O3 pollution in summertime.
Share
Altmetrics
Final-revised paper
Preprint