Articles | Volume 19, issue 1
https://doi.org/10.5194/acp-19-57-2019
https://doi.org/10.5194/acp-19-57-2019
Research article
 | 
03 Jan 2019
Research article |  | 03 Jan 2019

Aircraft-based measurements of High Arctic springtime aerosol show evidence for vertically varying sources, transport and composition

Megan D. Willis, Heiko Bozem, Daniel Kunkel, Alex K. Y. Lee, Hannes Schulz, Julia Burkart, Amir A. Aliabadi, Andreas B. Herber, W. Richard Leaitch, and Jonathan P. D. Abbatt

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Cited articles

Abbatt, J. P. D., Benz, S., Cziczo, D. J., Kanji, Z., Lohmann, U., and Moehler, O.: Solid ammonium sulfate aerosols as ice nuclei: A pathway for cirrus cloud formation, Science, 313, 1770–1773, https://doi.org/10.1126/science.1129726, 2006. a, b
Abbatt, J. P. D., Thomas, J. L., Abrahamsson, K., Boxe, C., Granfors, A., Jones, A. E., King, M. D., Saiz-Lopez, A., Shepson, P. B., Sodeau, J., Toohey, D. W., Toubin, C., von Glasow, R., Wren, S. N., and Yang, X.: Halogen activation via interactions with environmental ice and snow in the polar lower troposphere and other regions, Atmos. Chem. Phys., 12, 6237–6271, https://doi.org/10.5194/acp-12-6237-2012, 2012. a, b
Abbatt, J. P. D., Leaitch, W. R., Herber, A. B., Bertram, A. K., Blanchet, J. P., Korolev, A., Burkart, J., Bozem, H., Willis, M. D., Lee, A. K. Y., Schulz, H., Hanna, S., Aliabadi, A. A., and Staebler, R.: NETCARE 2015 POLAR6 aircraft campaign, available at: https://open.canada.ca/data/dataset/efe0e41c-890d-404d-bb1b-421456022d51, last access: 20 December 2018. a
Arnold, S. R., Law, K. S., Brock, C. A., Thomas, J. L., Starkweather, S. M., von Salzen, K., Stohl, A., Sharma, S., Lund, M. T., Flanner, M. G., Petäjä, T., Tanimoto, H., Gamble, J., Dibb, J. E., Melamed, M., Johnson, N., Fidel, M., Tynkkynen, V. P., Baklanov, A., Eckhardt, S., Monks, S. A., Browse, J., and Bozem, H.: Arctic air pollution: Challenges and opportunities for the next decade, Elementa, 4, 000104, https://doi.org/10.12952/journal.elementa.000104, 2016. a, b, c, d, e, f
Asmi, E., Kondratyev, V., Brus, D., Laurila, T., Lihavainen, H., Backman, J., Vakkari, V., Aurela, M., Hatakka, J., Viisanen, Y., Uttal, T., Ivakhov, V., and Makshtas, A.: Aerosol size distribution seasonal characteristics measured in Tiksi, Russian Arctic, Atmos. Chem. Phys., 16, 1271–1287, https://doi.org/10.5194/acp-16-1271-2016, 2016. a
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Short summary
The vertical distribution of Arctic aerosol is an important driver of its climate impacts. We present vertically resolved measurements of aerosol composition and properties made in the High Arctic during spring on an aircraft platform. We explore how aerosol properties are related to transport history and show evidence of vertical trends in aerosol sources, transport mechanisms and composition. These results will help us to better understand aerosol–climate interactions in the Arctic.
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