Articles | Volume 18, issue 20
https://doi.org/10.5194/acp-18-15291-2018
https://doi.org/10.5194/acp-18-15291-2018
Research article
 | 
24 Oct 2018
Research article |  | 24 Oct 2018

Eddy flux measurements of sulfur dioxide deposition to the sea surface

Jack G. Porter, Warren De Bruyn, and Eric S. Saltzman

Related authors

Methanethiol, dimethyl sulfide and acetone over biologically productive waters in the southwest Pacific Ocean
Sarah J. Lawson, Cliff S. Law, Mike J. Harvey, Thomas G. Bell, Carolyn F. Walker, Warren J. de Bruyn, and Eric S. Saltzman
Atmos. Chem. Phys., 20, 3061–3078, https://doi.org/10.5194/acp-20-3061-2020,https://doi.org/10.5194/acp-20-3061-2020, 2020
Short summary
Burning-derived vanillic acid in an Arctic ice core from Tunu, northeastern Greenland
Mackenzie M. Grieman, Murat Aydin, Joseph R. McConnell, and Eric S. Saltzman
Clim. Past, 14, 1625–1637, https://doi.org/10.5194/cp-14-1625-2018,https://doi.org/10.5194/cp-14-1625-2018, 2018
Short summary
Aromatic acids in an Arctic ice core from Svalbard: a proxy record of biomass burning
Mackenzie M. Grieman, Murat Aydin, Elisabeth Isaksson, Margit Schwikowski, and Eric S. Saltzman
Clim. Past, 14, 637–651, https://doi.org/10.5194/cp-14-637-2018,https://doi.org/10.5194/cp-14-637-2018, 2018
Short summary
Gradient flux measurements of sea–air DMS transfer during the Surface Ocean Aerosol Production (SOAP) experiment
Murray J. Smith, Carolyn F. Walker, Thomas G. Bell, Mike J. Harvey, Eric S. Saltzman, and Cliff S. Law
Atmos. Chem. Phys., 18, 5861–5877, https://doi.org/10.5194/acp-18-5861-2018,https://doi.org/10.5194/acp-18-5861-2018, 2018
Short summary
Estimation of bubble-mediated air–sea gas exchange from concurrent DMS and CO2 transfer velocities at intermediate–high wind speeds
Thomas G. Bell, Sebastian Landwehr, Scott D. Miller, Warren J. de Bruyn, Adrian H. Callaghan, Brian Scanlon, Brian Ward, Mingxi Yang, and Eric S. Saltzman
Atmos. Chem. Phys., 17, 9019–9033, https://doi.org/10.5194/acp-17-9019-2017,https://doi.org/10.5194/acp-17-9019-2017, 2017
Short summary

Related subject area

Subject: Gases | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Zugspitze ozone 1970–2020: the role of stratosphere–troposphere transport
Thomas Trickl, Cédric Couret, Ludwig Ries, and Hannes Vogelmann
Atmos. Chem. Phys., 23, 8403–8427, https://doi.org/10.5194/acp-23-8403-2023,https://doi.org/10.5194/acp-23-8403-2023, 2023
Short summary
High sulfur dioxide deposition velocities measured with the flux–gradient technique in a boreal forest in the Alberta Oil Sands Region
Mark Gordon, Dane Blanchard, Timothy Jiang, Paul A. Makar, Ralf M. Staebler, Julian Aherne, Cris Mihele, and Xuanyi Zhang
Atmos. Chem. Phys., 23, 7241–7255, https://doi.org/10.5194/acp-23-7241-2023,https://doi.org/10.5194/acp-23-7241-2023, 2023
Short summary
Quantification of methane emissions in Hamburg using a network of FTIR spectrometers and an inverse modeling approach
Andreas Forstmaier, Jia Chen, Florian Dietrich, Juan Bettinelli, Hossein Maazallahi, Carsten Schneider, Dominik Winkler, Xinxu Zhao, Taylor Jones, Carina van der Veen, Norman Wildmann, Moritz Makowski, Aydin Uzun, Friedrich Klappenbach, Hugo Denier van der Gon, Stefan Schwietzke, and Thomas Röckmann
Atmos. Chem. Phys., 23, 6897–6922, https://doi.org/10.5194/acp-23-6897-2023,https://doi.org/10.5194/acp-23-6897-2023, 2023
Short summary
Local-to-regional methane emissions from the Upper Silesian Coal Basin (USCB) quantified using UAV-based atmospheric measurements
Truls Andersen, Zhao Zhao, Marcel de Vries, Jaroslaw Necki, Justyna Swolkien, Malika Menoud, Thomas Röckmann, Anke Roiger, Andreas Fix, Wouter Peters, and Huilin Chen
Atmos. Chem. Phys., 23, 5191–5216, https://doi.org/10.5194/acp-23-5191-2023,https://doi.org/10.5194/acp-23-5191-2023, 2023
Short summary
Transport pathways of carbon monoxide from Indonesian fire pollution to a subtropical high-altitude mountain site in the western North Pacific
Saginela Ravindra Babu, Chang-Feng Ou-Yang, Stephen M. Griffith, Shantanu Kumar Pani, Steven Soon-Kai Kong, and Neng-Huei Lin
Atmos. Chem. Phys., 23, 4727–4740, https://doi.org/10.5194/acp-23-4727-2023,https://doi.org/10.5194/acp-23-4727-2023, 2023
Short summary

Cited articles

Bandy, A. R., Scott, D. L., Blomquist, B. W., Chen, S. M., and Thornton, D. C.: Low yields of SO2 from dimethyl sulfide oxidation in the marine boundary layer, Geophys. Res. Lett., 19, 1125–1127, https://doi.org/10.1029/92GL01041, 1992. a
Bandy, A. R., Thornton, D. C., Tu, F. H., Blomquist, B. W., Nadler, W., Mitchell, G. M., and Lenschow, D. H.: Determination of the vertical flux of dimethyl sulfide by eddy correlation and atmospheric pressure ionization mass spectrometry (APIMS), J. Geophys. Res.-Atmos., 107, ACH 3-1–ACH 3-9, https://doi.org/10.1029/2002JD002472, 2002. a
Bell, T. G., De Bruyn, W., Miller, S. D., Ward, B., Christensen, K. H., and Saltzman, E. S.: Air-sea dimethylsulfide (DMS) gas transfer in the North Atlantic: evidence for limited interfacial gas exchange at high wind speed, Atmos. Chem. Phys., 13, 11073–11087, https://doi.org/10.5194/acp-13-11073-2013, 2013. a, b
Bock, E. J. and Frew, N. M.: Static and dynamic response of natural multicomponent oceanic surface films to compression and dilation: Laboratory and field observations, J. Geophys. Res.-Oceans, 98, 14599–14617, https://doi.org/10.1029/93JC00428, 1993. a
Bowles, M. W., Mogollón, J. M., Kasten, S., Zabel, M., and Hinrichs, K.-U.: Global rates of marine sulfate reduction and implications for sub-sea-floor metabolic activities, Science, 344, 889–891, https://doi.org/10.1126/science.1249213, 2014. a
Download
Short summary
Deposition to the sea surface is a major loss pathway for highly soluble atmospheric trace gases. These fluxes are important to biogeochemical cycles, climate, and air quality. Here we report measurements of air–sea fluxes of sulfur dioxide, sensible heat, and momentum to coastal waters. Transfer velocities derived from the data show a dependence on molecular diffusivity, demonstrating the importance of diffusion in the interfacial layer on the atmospheric side of the air–sea interface.
Altmetrics
Final-revised paper
Preprint