Articles | Volume 17, issue 12
Atmos. Chem. Phys., 17, 7581–7591, 2017
https://doi.org/10.5194/acp-17-7581-2017
Atmos. Chem. Phys., 17, 7581–7591, 2017
https://doi.org/10.5194/acp-17-7581-2017

Research article 22 Jun 2017

Research article | 22 Jun 2017

Nucleation modeling of the Antarctic stratospheric CN layer and derivation of sulfuric acid profiles

Steffen Münch and Joachim Curtius

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Cited articles

Arnold, F., Fabian, R., and Joos, W.: Measurements of the height variation of sulfuric acid vapor concentrations in the stratosphere. Geophys. Res. Lett., 8, 293–296, 1981.
Arnold, F., Curtius, J., Spreng, S., and Deshler, T.: Stratospheric aerosol sulfuric acid: First direct in situ measurements using a novel balloon-based mass spectrometer apparatus, J. Atmos. Chem., 30, 3–10, 1998.
Borrmann, S., Kunkel, D., Weigel, R., Minikin, A., Deshler, T., Wilson, J. C., Curtius, J., Volk, C. M., Homan, C. D., Ulanovsky, A., Ravegnani, F., Viciani, S., Shur, G. N., Belyaev, G. V., Law, K. S., and Cairo, F.: Aerosols in the tropical and subtropical UT/LS: in-situ measurements of submicron particle abundance and volatility, Atmos. Chem. Phys., 10, 5573–5592, https://doi.org/10.5194/acp-10-5573-2010, 2010.
Brock, C. A., Hamill, P., Wilson, J. C., Jonsson, H. H., and Chan, K. R.: Particle formation in the upper tropical troposphere: A source of nuclei for the stratospheric aerosol, Science, 270, p. 1650, 1995.
Campbell, P. and Deshler, T.: Condensation nuclei measurements in the midlatitude (1982–2012) and Antarctic (1986–2010) stratosphere between 20 and 35 km, J. Geophys. Res.-Atmos., 119, 137–152, 2014.
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Recent research has analyzed the formation of a particle (CN) layer in the stratosphere above Antarctica after sunrise. We investigate the CN layer formation processes with our particle formation model and derive sulfuric acid profiles (no measurements exist). Our study confirms existing explanations and gives more insights into the formation process, leading to higher derived concentrations. Therefore, this paper improves our understanding of the processes in the high atmosphere.
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