Articles | Volume 17, issue 10
https://doi.org/10.5194/acp-17-6423-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-6423-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Particulate emissions from large North American wildfires estimated using a new top-down method
Tadas Nikonovas
CORRESPONDING AUTHOR
Geography Department, College of Science, Swansea University, Singleton
Park, Swansea, SA2 8PP, UK
Peter R. J. North
Geography Department, College of Science, Swansea University, Singleton
Park, Swansea, SA2 8PP, UK
Stefan H. Doerr
Geography Department, College of Science, Swansea University, Singleton
Park, Swansea, SA2 8PP, UK
Related authors
Tadas Nikonovas, Allan Spessa, Stefan H. Doerr, Gareth D. Clay, and Symon Mezbahuddin
Nat. Hazards Earth Syst. Sci., 22, 303–322, https://doi.org/10.5194/nhess-22-303-2022, https://doi.org/10.5194/nhess-22-303-2022, 2022
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Extreme fire episodes in Indonesia emit large amounts of greenhouse gasses and have negative effects on human health in the region. In this study we show that such burning events can be predicted several months in advance in large parts of Indonesia using existing seasonal climate forecasts and forest cover change datasets. A reliable early fire warning system would enable local agencies to prepare and mitigate the worst of the effects.
T. Nikonovas, P. R. J. North, and S. H. Doerr
Atmos. Chem. Phys., 15, 7929–7943, https://doi.org/10.5194/acp-15-7929-2015, https://doi.org/10.5194/acp-15-7929-2015, 2015
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The study found significant differences in smoke plumes attributed to different vegetation type fires in northern temperate and boreal regions. Plume particle sizes and optical properties varied not only when comparing grass and forest emissions, but also plumes from different forest types. Particles were found to increase in size in ageing plumes. Determined growth rates were significant and consistent between the emissions of different origin.
Matthew W. Jones, Douglas I. Kelley, Chantelle A. Burton, Francesca Di Giuseppe, Maria Lucia F. Barbosa, Esther Brambleby, Andrew J. Hartley, Anna Lombardi, Guilherme Mataveli, Joe R. McNorton, Fiona R. Spuler, Jakob B. Wessel, John T. Abatzoglou, Liana O. Anderson, Niels Andela, Sally Archibald, Dolors Armenteras, Eleanor Burke, Rachel Carmenta, Emilio Chuvieco, Hamish Clarke, Stefan H. Doerr, Paulo M. Fernandes, Louis Giglio, Douglas S. Hamilton, Stijn Hantson, Sarah Harris, Piyush Jain, Crystal A. Kolden, Tiina Kurvits, Seppe Lampe, Sarah Meier, Stacey New, Mark Parrington, Morgane M. G. Perron, Yuquan Qu, Natasha S. Ribeiro, Bambang H. Saharjo, Jesus San-Miguel-Ayanz, Jacquelyn K. Shuman, Veerachai Tanpipat, Guido R. van der Werf, Sander Veraverbeke, and Gavriil Xanthopoulos
Earth Syst. Sci. Data, 16, 3601–3685, https://doi.org/10.5194/essd-16-3601-2024, https://doi.org/10.5194/essd-16-3601-2024, 2024
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This inaugural State of Wildfires report catalogues extreme fires of the 2023–2024 fire season. For key events, we analyse their predictability and drivers and attribute them to climate change and land use. We provide a seasonal outlook and decadal projections. Key anomalies occurred in Canada, Greece, and western Amazonia, with other high-impact events catalogued worldwide. Climate change significantly increased the likelihood of extreme fires, and mitigation is required to lessen future risk.
Julia Kelly, Stefan H. Doerr, Johan Ekroos, Theresa S. Ibáñez, Md. Rafikul Islam, Cristina Santín, Margarida Soares, and Natascha Kljun
EGUsphere, https://doi.org/10.5194/egusphere-2024-2016, https://doi.org/10.5194/egusphere-2024-2016, 2024
Preprint archived
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We measured soil carbon fluxes during the first four years after a wildfire in the Swedish boreal forest. Soil CO2 emissions decreased substantially only when trees were killed by fire or by post-fire logging, but not when trees survived the fire and were left standing. Soil methane flux was not affected by fire. Logging trees already killed by fire had no additional impact on soil carbon fluxes. Post-fire forest management strategy impacted vegetation regrowth and carbon dynamics.
Tadas Nikonovas, Allan Spessa, Stefan H. Doerr, Gareth D. Clay, and Symon Mezbahuddin
Nat. Hazards Earth Syst. Sci., 22, 303–322, https://doi.org/10.5194/nhess-22-303-2022, https://doi.org/10.5194/nhess-22-303-2022, 2022
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Extreme fire episodes in Indonesia emit large amounts of greenhouse gasses and have negative effects on human health in the region. In this study we show that such burning events can be predicted several months in advance in large parts of Indonesia using existing seasonal climate forecasts and forest cover change datasets. A reliable early fire warning system would enable local agencies to prepare and mitigate the worst of the effects.
James M. Roberts, Chelsea E. Stockwell, Robert J. Yokelson, Joost de Gouw, Yong Liu, Vanessa Selimovic, Abigail R. Koss, Kanako Sekimoto, Matthew M. Coggon, Bin Yuan, Kyle J. Zarzana, Steven S. Brown, Cristina Santin, Stefan H. Doerr, and Carsten Warneke
Atmos. Chem. Phys., 20, 8807–8826, https://doi.org/10.5194/acp-20-8807-2020, https://doi.org/10.5194/acp-20-8807-2020, 2020
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We measured total reactive nitrogen, Nr, in lab fires from western North American fuels, along with measurements of individual nitrogen compounds. We measured the amount of N that gets converted to inactive compounds (avg. 70 %), and the amount that is accounted for by individual species (85 % of remaining N). We provide guidelines for how the reactive nitrogen is distributed among individual compounds such as NOx and ammonia. This will help estimates and predictions of wildfire emissions.
Christoph Brühl, Jennifer Schallock, Klaus Klingmüller, Charles Robert, Christine Bingen, Lieven Clarisse, Andreas Heckel, Peter North, and Landon Rieger
Atmos. Chem. Phys., 18, 12845–12857, https://doi.org/10.5194/acp-18-12845-2018, https://doi.org/10.5194/acp-18-12845-2018, 2018
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Use of multi-instrument satellite data is important to get consistent simulations of aerosol radiative forcing by a complex chemistry climate model, here with a main focus on the lower stratosphere. The satellite data at different wavelengths together with the patterns in the simulated size distribution point to a significant contribution from moist mineral dust lifted to the tropopause region by the Asian summer monsoon.
Emilia Urbanek and Stefan H. Doerr
Biogeosciences, 14, 4781–4794, https://doi.org/10.5194/bg-14-4781-2017, https://doi.org/10.5194/bg-14-4781-2017, 2017
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We studied CO2 emissions from soils that are seasonally water-epellent, and the wetting and water movement is restricted. When CO2 emissions are low soil is consistently water-repellent after a long dry spells, but when water repellency and thus soil moisture are patchy CO2 emission rates are high. The presence of water repellency may therefore increase rather than reduce soil CO2 emissions, which may result in higher soil carbon losses than it was previously anticipated.
T. Nikonovas, P. R. J. North, and S. H. Doerr
Atmos. Chem. Phys., 15, 7929–7943, https://doi.org/10.5194/acp-15-7929-2015, https://doi.org/10.5194/acp-15-7929-2015, 2015
Short summary
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The study found significant differences in smoke plumes attributed to different vegetation type fires in northern temperate and boreal regions. Plume particle sizes and optical properties varied not only when comparing grass and forest emissions, but also plumes from different forest types. Particles were found to increase in size in ageing plumes. Determined growth rates were significant and consistent between the emissions of different origin.
Related subject area
Subject: Aerosols | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The role of refractive indices in measuring mineral dust with high-spectral-resolution infrared satellite sounders: application to the Gobi Desert
Influence of covariance of aerosol and meteorology on co-located precipitating and non-precipitating clouds over the Indo-Gangetic Plain
Light-absorbing black carbon and brown carbon components of smoke aerosol from DSCOVR EPIC measurements over North America and central Africa
Fluorescence properties of long-range transported smoke: Insights from five-channel lidar observations over Moscow during the 2023 wildfire season
Distinct effects of Fine and Coarse Aerosols on Microphysical Processes of Shallow Precipitation Systems in Summer over Southern China
The emission, transport, and impacts of the extreme Saharan dust storm of 2015
Increased number concentrations of small particles explains perceived stagnation in air quality over Korea
California wildfire smoke contributes to a positive atmospheric temperature anomaly over the western United States
Remote Sensing detectability of airborne Arctic dust
Dust storms from the Taklamakan Desert significantly darken snow surface on surrounding mountains
Opposite effects of aerosols and meteorological parameters on warm clouds in two contrasting regions over eastern China
Effect of wind speed on marine aerosol optical properties over remote oceans with use of spaceborne lidar observations
Assessment of smoke plume height products derived from multisource satellite observations using lidar-derived height metrics for wildfires in the western US
A remote sensing algorithm for vertically resolved cloud condensation nuclei number concentrations from airborne and spaceborne lidar observations
Opinion: Aerosol remote sensing over the next 20 years
Monitoring biomass burning aerosol transport using CALIOP observations and reanalysis models: a Canadian wildfire event in 2019
Thermal infrared observations of a western United States biomass burning aerosol plume
A new look into the impacts of dust radiative effects on the energetics of tropical easterly waves
Wind-driven emissions of coarse-mode particles in an urban environment
Measurement report: Dust and anthropogenic aerosols' vertical distributions over northern China dense aerosols gathered at the top of the mixing layer
Climatological assessment of the vertically resolved optical and microphysical aerosol properties by lidar measurements, sun photometer, and in situ observations over 17 years at Universitat Politècnica de Catalunya (UPC) Barcelona
Aerosol optical depth climatology from the high-resolution MAIAC product over Europe: differences between major European cities and their surrounding environments
Impact of assimilating NOAA VIIRS aerosol optical depth (AOD) observations on global AOD analysis from the Copernicus Atmosphere Monitoring Service (CAMS)
Spectral dependence of birch and pine pollen optical properties using a synergy of lidar instruments
Validation activities of Aeolus wind products on the southeastern Iberian Peninsula
Thermal infrared dust optical depth and coarse-mode effective diameter over oceans retrieved from collocated MODIS and CALIOP observations
A comprehensive reappraisal of long-term aerosol characteristics, trends, and variability in Asia
Satellite (GOSAT-2 CAI-2) retrieval and surface (ARFINET) observations of aerosol black carbon over India
Spatiotemporal variation characteristics of global fires and their emissions
The (mis)identification of high-latitude dust events using remote sensing methods in the Yukon, Canada: a sub-daily variability analysis
Comparison of dust optical depth from multi-sensor products and MONARCH (Multiscale Online Non-hydrostatic AtmospheRe CHemistry) dust reanalysis over North Africa, the Middle East, and Europe
Understanding day–night differences in dust aerosols over the dust belt of North Africa, the Middle East, and Asia
Satellite observations of smoke–cloud–radiation interactions over the Amazon rainforest
Single-scattering properties of ellipsoidal dust aerosols constrained by measured dust shape distributions
Validation of the TROPOMI/S5P aerosol layer height using EARLINET lidars
Vertical characterization of fine and coarse dust particles during an intense Saharan dust outbreak over the Iberian Peninsula in springtime 2021
Aerosol optical depth regime over megacities of the world
South American 2020 regional smoke plume: intercomparison with previous years, impact on solar radiation, and the role of Pantanal biomass burning season
Circular polarization in atmospheric aerosols
Spatiotemporal continuous estimates of daily 1 km PM2.5 from 2000 to present under the Tracking Air Pollution in China (TAP) framework
Robust evidence for reversal of the trend in aerosol effective climate forcing
Simultaneous retrievals of biomass burning aerosols and trace gases from the ultraviolet to near-infrared over northern Thailand during the 2019 pre-monsoon season
A decadal assessment of the climatology of aerosol and cloud properties over South Africa
Aerosol characterisation in the subtropical eastern North Atlantic region using long-term AERONET measurements
Long-range transport of Asian dust to the Arctic: identification of transport pathways, evolution of aerosol optical properties, and impact assessment on surface albedo changes
Canadian and Alaskan wildfire smoke particle properties, their evolution, and controlling factors, from satellite observations
Evaluation of aerosol optical depths and clear-sky radiative fluxes of the CERES Edition 4.1 SYN1deg data product
Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 1: Climatology and trend
Vertical structure of biomass burning aerosol transported over the southeast Atlantic Ocean
Arctic spring and summertime aerosol optical depth baseline from long-term observations and model reanalyses – Part 2: Statistics of extreme AOD events, and implications for the impact of regional biomass burning processes
Perla Alalam, Fabrice Ducos, and Hervé Herbin
Atmos. Chem. Phys., 24, 12277–12294, https://doi.org/10.5194/acp-24-12277-2024, https://doi.org/10.5194/acp-24-12277-2024, 2024
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This study dives into the impact of mineral dust laboratory complex refractive indices (CRIs) on quantifying the dust microphysical properties using satellite infrared remote sensing. Results show that using CRIs obtained by advanced realistic techniques can improve the accuracy of these measurements, emphasizing the importance of choosing the suitable CRI in atmospheric models. This improvement is crucial for better predicting the dust radiative effect and impact on the climate.
Nabia Gulistan, Khan Alam, and Yangang Liu
Atmos. Chem. Phys., 24, 11333–11349, https://doi.org/10.5194/acp-24-11333-2024, https://doi.org/10.5194/acp-24-11333-2024, 2024
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This study looks at the influence of aerosol and meteorology on precipitating and non-precipitating clouds over the Indo-Gangetic Plain (IGP). A major finding of this study was that the high loading of aerosols led to a high occurrence of precipitating clouds under unstable conditions in summer. The study has the potential to open a new avenue for the scientific community to further explore and understand the complications of aerosol–cloud–precipitation over the complex topography of the IGP.
Myungje Choi, Alexei Lyapustin, Gregory L. Schuster, Sujung Go, Yujie Wang, Sergey Korkin, Ralph Kahn, Jeffrey S. Reid, Edward J. Hyer, Thomas F. Eck, Mian Chin, David J. Diner, Olga Kalashnikova, Oleg Dubovik, Jhoon Kim, and Hans Moosmüller
Atmos. Chem. Phys., 24, 10543–10565, https://doi.org/10.5194/acp-24-10543-2024, https://doi.org/10.5194/acp-24-10543-2024, 2024
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This paper introduces a retrieval algorithm to estimate two key absorbing components in smoke (black carbon and brown carbon) using DSCOVR EPIC measurements. Our analysis reveals distinct smoke properties, including spectral absorption, layer height, and black carbon and brown carbon, over North America and central Africa. The retrieved smoke properties offer valuable observational constraints for modeling radiative forcing and informing health-related studies.
Igor Veselovskii, Mikhail Korenskiy, Nikita Kasianik, Boris Barchunov, Qiaoyun Hu, Philippe Goloub, and Thierry Podvin
EGUsphere, https://doi.org/10.5194/egusphere-2024-2874, https://doi.org/10.5194/egusphere-2024-2874, 2024
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A fluorescence lidar was utilized to study transported smoke during the wildfire season from May to September 2023. The lidar performs fluorescence measurements at 5 wavelengths. Observations reveal that the fluorescence capacity increases with altitude, suggesting higher concentration of organic compounds in the UTLS compared to the lower troposphere. And urban aerosol fluorescence tends to decrease with wavelength, while the peak of smoke fluorescence is observed at 513 or 560 nm channels.
Fengjiao Chen, Yuanjian Yang, Lu Yu, Yang Li, Weiguang Liu, Yan Liu, and Simone Lolli
EGUsphere, https://doi.org/10.5194/egusphere-2024-2206, https://doi.org/10.5194/egusphere-2024-2206, 2024
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The precipitation microphysical mechanisms responsible for the varied impacts of aerosols on shallow precipitation remain unclear. This study reveals that coarse aerosols invigorate shallow rainfall through enhanced coalescence processes, whereas fine aerosols suppress shallow rainfall via intensified breakup microphysical processes. These impacts are independent of thermodynamic environments but are more significant in low-humidity conditions.
Brian Harr, Bing Pu, and Qinjian Jin
Atmos. Chem. Phys., 24, 8625–8651, https://doi.org/10.5194/acp-24-8625-2024, https://doi.org/10.5194/acp-24-8625-2024, 2024
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We found that the formation of the extreme trans-Atlantic African dust event in June 2015 was associated with a brief surge in dust emissions over western North Africa and extreme circulation patterns, including intensified easterly jets, which facilitated the westward transport of dust. The dust plume modified radiative flux along its transport pathway but had minor impacts on air quality in the US due to the record-high Caribbean low-level jet advecting part of the plume to the Pacific.
Sohee Joo, Juseon Shin, Matthias Tesche, Dehkhoda Naghmeh, Taegyeong Kim, and Youngmin Noh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1208, https://doi.org/10.5194/egusphere-2024-1208, 2024
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In our study, we investigated why, in Northeast Asia, visibility has not improved even though air pollution levels have decreased. By examining trends in Seoul and Ulsan, we found that the particles in the air are getting smaller, which scatters light more effectively and reduces how far we can see. Our findings suggest that changes in particle properties adversely affected public perception of air quality improvement even though the PM2.5 mass concentration is continuously decreasing.
James L. Gomez, Robert J. Allen, and King-Fai Li
Atmos. Chem. Phys., 24, 6937–6963, https://doi.org/10.5194/acp-24-6937-2024, https://doi.org/10.5194/acp-24-6937-2024, 2024
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Wildfires in California (CA) have grown very large during the past 20 years. These fires emit sunlight-absorbing aerosols. Analyzing observational data, our study finds that aerosols emitted from large fires in northern CA spread throughout CA and Nevada and heat the atmosphere. This heating is consistent with larger-than-normal temperatures and dry conditions. Further study is needed to determine how much the aerosols heat the atmosphere and whether they are drying the atmosphere as well.
Norman T. O’Neill, Keyvan Ranjbar, Liviu Ivănescu, Yann Blanchard, Seyed Ali Sayedain, and Yasmin AboEl-Fetouh
EGUsphere, https://doi.org/10.5194/egusphere-2024-1057, https://doi.org/10.5194/egusphere-2024-1057, 2024
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Dust from mid-latitude deserts or from local drainage basins is a weak component of atmospheric aerosols in the Arctic. Satellite-based dust estimates are often overestimated because dust and cloud measurements can be confused. Illustrations are given with an emphasis on the flawed claim that a classic indicator of dust (negative brightness temperature differences) is proof of the presence of airborne Arctic dust. Low altitude “warm” water plumes are the likely source of such negative values.
Yuxuan Xing, Yang Chen, Shirui Yan, Xiaoyi Cao, Yong Zhou, Xueying Zhang, Tenglong Shi, Xiaoying Niu, Dongyou Wu, Jiecan Cui, Yue Zhou, Xin Wang, and Wei Pu
Atmos. Chem. Phys., 24, 5199–5219, https://doi.org/10.5194/acp-24-5199-2024, https://doi.org/10.5194/acp-24-5199-2024, 2024
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This study investigated the impact of dust storms from the Taklamakan Desert on surrounding high mountains and regional radiation balance. Using satellite data and simulations, researchers found that dust storms significantly darken the snow surface in the Tien Shan, Kunlun, and Qilian mountains, reaching mountains up to 1000 km away. This darkening occurs not only in spring but also during summer and autumn, leading to increased absorption of solar radiation.
Yuqin Liu, Tao Lin, Jiahua Zhang, Fu Wang, Yiyi Huang, Xian Wu, Hong Ye, Guoqin Zhang, Xin Cao, and Gerrit de Leeuw
Atmos. Chem. Phys., 24, 4651–4673, https://doi.org/10.5194/acp-24-4651-2024, https://doi.org/10.5194/acp-24-4651-2024, 2024
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A new method, the geographical detector method (GDM), has been applied to satellite data, in addition to commonly used statistical methods, to study the sensitivity of cloud properties to aerosol over China. Different constraints for aerosol and cloud liquid water path apply over polluted and clean areas. The GDM shows that cloud parameters are more sensitive to combinations of parameters than to individual parameters, but confounding effects due to co-variation of parameters cannot be excluded.
Kangwen Sun, Guangyao Dai, Songhua Wu, Oliver Reitebuch, Holger Baars, Jiqiao Liu, and Suping Zhang
Atmos. Chem. Phys., 24, 4389–4409, https://doi.org/10.5194/acp-24-4389-2024, https://doi.org/10.5194/acp-24-4389-2024, 2024
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This paper investigates the correlation between marine aerosol optical properties and wind speeds over remote oceans using the spaceborne lidars ALADIN and CALIOP. Three remote ocean areas are selected. Pure marine aerosol optical properties at 355 nm are derived from ALADIN. The relationships between marine aerosol optical properties and wind speeds are analyzed within and above the marine atmospheric boundary layer, revealing the effect of wind speed on marine aerosols over remote oceans.
Jingting Huang, S. Marcela Loría-Salazar, Min Deng, Jaehwa Lee, and Heather A. Holmes
Atmos. Chem. Phys., 24, 3673–3698, https://doi.org/10.5194/acp-24-3673-2024, https://doi.org/10.5194/acp-24-3673-2024, 2024
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Increased wildfire intensity has resulted in taller wildfire smoke plumes. We investigate the vertical structure of wildfire smoke plumes using aircraft lidar data and establish two effective smoke plume height metrics. Four novel satellite-based plume height products are evaluated for wildfires in the western US. Our results provide guidance on the strengths and limitations of these satellite products and set the stage for improved plume rise estimates by leveraging satellite products.
Piyushkumar N. Patel, Jonathan H. Jiang, Ritesh Gautam, Harish Gadhavi, Olga Kalashnikova, Michael J. Garay, Lan Gao, Feng Xu, and Ali Omar
Atmos. Chem. Phys., 24, 2861–2883, https://doi.org/10.5194/acp-24-2861-2024, https://doi.org/10.5194/acp-24-2861-2024, 2024
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Global measurements of cloud condensation nuclei (CCN) are essential for understanding aerosol–cloud interactions and predicting climate change. To address this gap, we introduced a remote sensing algorithm that retrieves vertically resolved CCN number concentrations from airborne and spaceborne lidar systems. This innovation offers a global distribution of CCN concentrations from space, facilitating model evaluation and precise quantification of aerosol climate forcing.
Lorraine A. Remer, Robert C. Levy, and J. Vanderlei Martins
Atmos. Chem. Phys., 24, 2113–2127, https://doi.org/10.5194/acp-24-2113-2024, https://doi.org/10.5194/acp-24-2113-2024, 2024
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Aerosols are small liquid or solid particles suspended in the atmosphere, including smoke, particulate pollution, dust, and sea salt. Today, we rely on satellites viewing Earth's atmosphere to learn about these particles. Here, we speculate on the future to imagine how satellite viewing of aerosols will change. We expect more public and private satellites with greater capabilities, better ways to infer information from satellites, and merging of data with models.
Xiaoxia Shang, Antti Lipponen, Maria Filioglou, Anu-Maija Sundström, Mark Parrington, Virginie Buchard, Anton S. Darmenov, Ellsworth J. Welton, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Alejandro Rodríguez-Gómez, Mika Komppula, and Tero Mielonen
Atmos. Chem. Phys., 24, 1329–1344, https://doi.org/10.5194/acp-24-1329-2024, https://doi.org/10.5194/acp-24-1329-2024, 2024
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In June 2019, smoke particles from a Canadian wildfire event were transported to Europe. The long-range-transported smoke plumes were monitored with a spaceborne lidar and reanalysis models. Based on the aerosol mass concentrations estimated from the observations, the reanalysis models had difficulties in reproducing the amount and location of the smoke aerosols during the transport event. Consequently, more spaceborne lidar missions are needed for reliable monitoring of aerosol plumes.
Blake T. Sorenson, Jeffrey S. Reid, Jianglong Zhang, Robert E. Holz, William L. Smith Sr., and Amanda Gumber
Atmos. Chem. Phys., 24, 1231–1248, https://doi.org/10.5194/acp-24-1231-2024, https://doi.org/10.5194/acp-24-1231-2024, 2024
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Smoke particles are typically submicron in size and assumed to have negligible impacts at the thermal infrared spectrum. However, we show that infrared signatures can be observed over dense smoke plumes from satellites. We found that giant particles are unlikely to be the dominant cause. Rather, co-transported water vapor injected to the middle to upper troposphere and surface cooling beneath the plume due to shadowing are significant, with the surface cooling effect being the most dominant.
Farnaz Hosseinpour and Eric M. Wilcox
Atmos. Chem. Phys., 24, 707–724, https://doi.org/10.5194/acp-24-707-2024, https://doi.org/10.5194/acp-24-707-2024, 2024
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This study shows mechanistic relationships between the radiative effect of dust aerosols in the Saharan air layer and the kinetic energy of the African easterly waves across the tropical Atlantic Ocean using 22 years of daily satellite observations and reanalysis data based on satellite assimilation. Our findings suggest that dust aerosols not merely are transported by these waves but also contribute to the growth of waves through the enhancement of diabatic heating induced by dust.
Markus D. Petters, Tyas Pujiastuti, Ajmal Rasheeda Satheesh, Sabin Kasparoglu, Bethany Sutherland, and Nicholas Meskhidze
Atmos. Chem. Phys., 24, 745–762, https://doi.org/10.5194/acp-24-745-2024, https://doi.org/10.5194/acp-24-745-2024, 2024
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This work introduces a new method that uses remote sensing techniques to obtain surface number emissions of particles with a diameter greater than 500 nm. The technique was applied to study particle emissions at an urban site near Houston, TX, USA. The emissions followed a diurnal pattern and peaked near noon local time. The daily averaged emissions correlated with wind speed. The source is likely due to wind-driven erosion of material situated on asphalted and other hard surfaces.
Zhuang Wang, Chune Shi, Hao Zhang, Yujia Chen, Xiyuan Chi, Congzi Xia, Suyao Wang, Yizhi Zhu, Kaidi Zhang, Xintong Chen, Chengzhi Xing, and Cheng Liu
Atmos. Chem. Phys., 23, 14271–14292, https://doi.org/10.5194/acp-23-14271-2023, https://doi.org/10.5194/acp-23-14271-2023, 2023
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The annual cycle of dust and anthropogenic aerosols' vertical distributions was revealed by polarization Raman lidar in Beijing. Anthropogenic aerosols typically accumulate at the top of the mixing layer (ML) due to the hygroscopic growth of atmospheric particles, and this is most significant in summer. There is no significant relationship between bottom dust mass concentration and ML height, while the dust in the upper air tends to be distributed near the mixing layer.
Simone Lolli, Michaël Sicard, Francesco Amato, Adolfo Comeron, Cristina Gíl-Diaz, Tony C. Landi, Constantino Munoz-Porcar, Daniel Oliveira, Federico Dios Otin, Francesc Rocadenbosch, Alejandro Rodriguez-Gomez, Andrés Alastuey, Xavier Querol, and Cristina Reche
Atmos. Chem. Phys., 23, 12887–12906, https://doi.org/10.5194/acp-23-12887-2023, https://doi.org/10.5194/acp-23-12887-2023, 2023
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We evaluated the long-term trends and seasonal variability of the vertically resolved aerosol properties over the past 17 years in Barcelona. Results shows that air quality is improved, with a consistent drop in PM concentrations at the surface, as well as the column aerosol optical depth. The results also show that natural dust outbreaks are more likely in summer, with aerosols reaching an altitude of 5 km, while in winter, aerosols decay as an exponential with a scale height of 600 m.
Ludovico Di Antonio, Claudia Di Biagio, Gilles Foret, Paola Formenti, Guillaume Siour, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 23, 12455–12475, https://doi.org/10.5194/acp-23-12455-2023, https://doi.org/10.5194/acp-23-12455-2023, 2023
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Long-term (2000–2021) 1 km resolution satellite data have been used to investigate the climatological aerosol optical depth (AOD) variability and trends at different scales in Europe. Average enhancements of the local-to-regional AOD ratio at 550 nm of 57 %, 55 %, 39 % and 32 % are found for large metropolitan areas such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions.
Sebastien Garrigues, Melanie Ades, Samuel Remy, Johannes Flemming, Zak Kipling, Istvan Laszlo, Mark Parrington, Antje Inness, Roberto Ribas, Luke Jones, Richard Engelen, and Vincent-Henri Peuch
Atmos. Chem. Phys., 23, 10473–10487, https://doi.org/10.5194/acp-23-10473-2023, https://doi.org/10.5194/acp-23-10473-2023, 2023
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The Copernicus Atmosphere Monitoring Service (CAMS) provides global monitoring of aerosols using the ECMWF forecast model constrained by the assimilation of satellite aerosol optical depth (AOD). This work aims at evaluating the assimilation of the NOAA VIIRS AOD product in the ECMWF model. It shows that the introduction of VIIRS in the CAMS data assimilation system enhances the accuracy of the aerosol analysis, particularly over Europe and desert and maritime sites.
Maria Filioglou, Ari Leskinen, Ville Vakkari, Ewan O'Connor, Minttu Tuononen, Pekko Tuominen, Samuli Laukkanen, Linnea Toiviainen, Annika Saarto, Xiaoxia Shang, Petri Tiitta, and Mika Komppula
Atmos. Chem. Phys., 23, 9009–9021, https://doi.org/10.5194/acp-23-9009-2023, https://doi.org/10.5194/acp-23-9009-2023, 2023
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Pollen impacts climate and public health, and it can be detected in the atmosphere by lidars which measure the linear particle depolarization ratio (PDR), a shape-relevant optical parameter. As aerosols also cause depolarization, surface aerosol and pollen observations were combined with measurements from ground-based lidars operating at different wavelengths to determine the optical properties of birch and pine pollen and quantify their relative contribution to the PDR.
Jesús Abril-Gago, Pablo Ortiz-Amezcua, Diego Bermejo-Pantaleón, Juana Andújar-Maqueda, Juan Antonio Bravo-Aranda, María José Granados-Muñoz, Francisco Navas-Guzmán, Lucas Alados-Arboledas, Inmaculada Foyo-Moreno, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 8453–8471, https://doi.org/10.5194/acp-23-8453-2023, https://doi.org/10.5194/acp-23-8453-2023, 2023
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Validation activities of Aeolus wind products were performed in Granada with different upward-probing instrumentation (Doppler lidar system and radiosondes) and spatiotemporal collocation criteria. Specific advantages and disadvantages of each instrument were identified, and an optimal comparison criterion is proposed. Aeolus was proven to provide reliable wind products, and the upward-probing instruments were proven to be useful for Aeolus wind product validation activities.
Jianyu Zheng, Zhibo Zhang, Hongbin Yu, Anne Garnier, Qianqian Song, Chenxi Wang, Claudia Di Biagio, Jasper F. Kok, Yevgeny Derimian, and Claire Ryder
Atmos. Chem. Phys., 23, 8271–8304, https://doi.org/10.5194/acp-23-8271-2023, https://doi.org/10.5194/acp-23-8271-2023, 2023
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We developed a multi-year satellite-based retrieval of dust optical depth at 10 µm and the coarse-mode dust effective diameter over global oceans. It reveals climatological coarse-mode dust transport patterns and regional differences over the North Atlantic, the Indian Ocean and the North Pacific.
Shikuan Jin, Yingying Ma, Zhongwei Huang, Jianping Huang, Wei Gong, Boming Liu, Weiyan Wang, Ruonan Fan, and Hui Li
Atmos. Chem. Phys., 23, 8187–8210, https://doi.org/10.5194/acp-23-8187-2023, https://doi.org/10.5194/acp-23-8187-2023, 2023
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To better understand the Asian aerosol environment, we studied distributions and trends of aerosol with different sizes and types. Over the past 2 decades, dust, sulfate, and sea salt aerosol decreased by 5.51 %, 3.07 %, and 9.80 %, whereas organic carbon and black carbon aerosol increased by 17.09 % and 6.23 %, respectively. The increase in carbonaceous aerosols was a feature of Asia. An exception is found in East Asia, where the carbonaceous aerosols reduced, owing largely to China's efforts.
Mukunda M. Gogoi, S. Suresh Babu, Ryoichi Imasu, and Makiko Hashimoto
Atmos. Chem. Phys., 23, 8059–8079, https://doi.org/10.5194/acp-23-8059-2023, https://doi.org/10.5194/acp-23-8059-2023, 2023
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Considering the climate warming potential of atmospheric black carbon (BC), satellite-based retrieval is a novel idea. This study highlights the regional distribution of BC based on observations by the Cloud and Aerosol Imager-2 on board the GOSAT-2 satellite and near-surface measurements of BC in ARFINET. The satellite retrieval fairly depicts the regional and seasonal features of BC over the Indian region, which are similar to those recorded by surface observations.
Hao Fan, Xingchuan Yang, Chuanfeng Zhao, Yikun Yang, and Zhenyao Shen
Atmos. Chem. Phys., 23, 7781–7798, https://doi.org/10.5194/acp-23-7781-2023, https://doi.org/10.5194/acp-23-7781-2023, 2023
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Using 20-year multi-source data, this study shows pronounced regional and seasonal variations in fire activities and emissions. Seasonal variability of fires is larger with increasing latitude. The increase in temperature in the Northern Hemisphere's middle- and high-latitude forest regions was primarily responsible for the increase in fires and emissions, while the changes in fire occurrence in tropical regions were more influenced by the decrease in precipitation and relative humidity.
Rosemary Huck, Robert G. Bryant, and James King
Atmos. Chem. Phys., 23, 6299–6318, https://doi.org/10.5194/acp-23-6299-2023, https://doi.org/10.5194/acp-23-6299-2023, 2023
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This study shows that mineral aerosol (dust) emission events in high-latitude areas are under-represented in both ground- and space-based detecting methods. This is done through a suite of ground-based data to prove that dust emissions from the proglacial area, Lhù’ààn Mân, occur almost daily but are not always recorded at different timescales. Dust has multiple effects on atmospheric processes; therefore, accurate quantification is important in the calibration and validation of climate models.
Michail Mytilinaios, Sara Basart, Sergio Ciamprone, Juan Cuesta, Claudio Dema, Enza Di Tomaso, Paola Formenti, Antonis Gkikas, Oriol Jorba, Ralph Kahn, Carlos Pérez García-Pando, Serena Trippetta, and Lucia Mona
Atmos. Chem. Phys., 23, 5487–5516, https://doi.org/10.5194/acp-23-5487-2023, https://doi.org/10.5194/acp-23-5487-2023, 2023
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Multiscale Online Non-hydrostatic AtmospheRe CHemistry model (MONARCH) dust reanalysis provides a high-resolution 3D reconstruction of past dust conditions, allowing better quantification of climate and socioeconomic dust impacts. We assess the performance of the reanalysis needed to reproduce dust optical depth using dust-related products retrieved from satellite and ground-based observations and show that it reproduces the spatial distribution and seasonal variability of atmospheric dust well.
Jacob Z. Tindan, Qinjian Jin, and Bing Pu
Atmos. Chem. Phys., 23, 5435–5466, https://doi.org/10.5194/acp-23-5435-2023, https://doi.org/10.5194/acp-23-5435-2023, 2023
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We use the Infrared Atmospheric Sounder Interferometer (IASI) retrievals of dust variables (dust optical depth and dust layer height) and surface observations to understand the day- and nighttime variations in dust aerosols over the dust belt. Our results show that daytime dust aerosols are significantly different from nighttime, and such day–night variations are influenced by meteorological factors such as wind speed, precipitation, and turbulent motions within the atmospheric boundary layer.
Ross Herbert and Philip Stier
Atmos. Chem. Phys., 23, 4595–4616, https://doi.org/10.5194/acp-23-4595-2023, https://doi.org/10.5194/acp-23-4595-2023, 2023
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We provide robust evidence from multiple sources showing that smoke from fires in the Amazon rainforest significantly modifies the diurnal cycle of convection and cools the climate. Low to moderate amounts of smoke increase deep convective clouds and rain, whilst beyond a threshold amount, the smoke starts to suppress the convection and rain. We are currently at this threshold, suggesting increases in fires from agricultural practices or droughts will reduce cloudiness and rain over the region.
Yue Huang, Jasper F. Kok, Masanori Saito, and Olga Muñoz
Atmos. Chem. Phys., 23, 2557–2577, https://doi.org/10.5194/acp-23-2557-2023, https://doi.org/10.5194/acp-23-2557-2023, 2023
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Global aerosol models and remote sensing retrievals use dust optical models with inconsistent and inaccurate dust shape approximations. Here, we present a new dust optical model constrained by measured dust shape distributions. This new dust optical model is an improvement on the current dust optical models used in models and retrieval algorithms, as quantified by comparisons against laboratory and field observations of dust optics.
Konstantinos Michailidis, Maria-Elissavet Koukouli, Dimitris Balis, J. Pepijn Veefkind, Martin de Graaf, Lucia Mona, Nikolaos Papagianopoulos, Gesolmina Pappalardo, Ioanna Tsikoudi, Vassilis Amiridis, Eleni Marinou, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Daniele Bortoli, Maria João Costa, Vanda Salgueiro, Alexandros Papayannis, Maria Mylonaki, Lucas Alados-Arboledas, Salvatore Romano, Maria Rita Perrone, and Holger Baars
Atmos. Chem. Phys., 23, 1919–1940, https://doi.org/10.5194/acp-23-1919-2023, https://doi.org/10.5194/acp-23-1919-2023, 2023
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Comparisons with ground-based correlative lidar measurements constitute a key component in the validation of satellite aerosol products. This paper presents the validation of the TROPOMI aerosol layer height (ALH) product, using archived quality assured ground-based data from lidar stations that belong to the EARLINET network. Comparisons between the TROPOMI ALH and co-located EARLINET measurements show good agreement over the ocean.
María Ángeles López-Cayuela, Carmen Córdoba-Jabonero, Diego Bermejo-Pantaleón, Michaël Sicard, Vanda Salgueiro, Francisco Molero, Clara Violeta Carvajal-Pérez, María José Granados-Muñoz, Adolfo Comerón, Flavio T. Couto, Rubén Barragán, María-Paz Zorzano, Juan Antonio Bravo-Aranda, Constantino Muñoz-Porcar, María João Costa, Begoña Artíñano, Alejandro Rodríguez-Gómez, Daniele Bortoli, Manuel Pujadas, Jesús Abril-Gago, Lucas Alados-Arboledas, and Juan Luis Guerrero-Rascado
Atmos. Chem. Phys., 23, 143–161, https://doi.org/10.5194/acp-23-143-2023, https://doi.org/10.5194/acp-23-143-2023, 2023
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An intense Saharan dust outbreak crossing the Iberian Peninsula in springtime was monitored to determinine the specific contribution of fine and coarse dust particles at five lidar stations, strategically covering its SW–central–NE pathway. Expected dust ageing along the transport started unappreciated. A different fine-dust impact on optical (~30 %) and mass (~10 %) properties was found. Use of polarized lidar measurements (mainly in elastic systems) for fine/coarse dust separation is crucial.
Kyriakoula Papachristopoulou, Ioannis-Panagiotis Raptis, Antonis Gkikas, Ilias Fountoulakis, Akriti Masoom, and Stelios Kazadzis
Atmos. Chem. Phys., 22, 15703–15727, https://doi.org/10.5194/acp-22-15703-2022, https://doi.org/10.5194/acp-22-15703-2022, 2022
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Megacities' air quality is determined by atmospheric aerosols. We focus on changes over the last two decades in the 81 largest cities, using satellite data. European and American cities have lower aerosol compared to African and Asian cities. For European, North American and East Asian cities, aerosols are decreasing over time, especially in China and the US. In the remaining cities, aerosol loads are increasing, particularly in India.
Nilton Évora do Rosário, Elisa Thomé Sena, and Marcia Akemi Yamasoe
Atmos. Chem. Phys., 22, 15021–15033, https://doi.org/10.5194/acp-22-15021-2022, https://doi.org/10.5194/acp-22-15021-2022, 2022
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The 2020 burning season in Brazil was marked by an atypically high number of fire spots across Pantanal, leading to high amounts of smoke within the biome. This study shows that smoke over Pantanal, usually a fraction of that over Amazonia, was higher and resulted mainly from fires in conservation and indigenous areas. It also contributes to highlighting Pantanal's 2020 burning season as the worst combination of a climate extreme scenario and inadequately enforced environmental regulations.
Santiago Gassó and Kirk D. Knobelspiesse
Atmos. Chem. Phys., 22, 13581–13605, https://doi.org/10.5194/acp-22-13581-2022, https://doi.org/10.5194/acp-22-13581-2022, 2022
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Atmospheric particles interact with light resulting in observable optical polarization. Thus, we can learn about their composition from space. New satellite sensor technology measures full polarization of reflected sunlight. This paper considers circular polarization, an overlooked category of polarization with distinctive features that could bring new insights. We review existing literature and make novel computations to consider this previously underappreciated category of polarization.
Qingyang Xiao, Guannan Geng, Shigan Liu, Jiajun Liu, Xia Meng, and Qiang Zhang
Atmos. Chem. Phys., 22, 13229–13242, https://doi.org/10.5194/acp-22-13229-2022, https://doi.org/10.5194/acp-22-13229-2022, 2022
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We provided complete coverage PM2.5 concentrations at a 1-km resolution from 2000 to the present, carefully considering the significant changes in land use characteristics in China. This high-resolution PM2.5 data successfully revealed the local-scale PM2.5 variations. We noticed changes in PM2.5 spatial patterns in association with the clean air policies, with the pollution hotspots having transferred from urban centers to rural regions with limited air quality monitoring.
Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas, Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M. Forster, Daniel Grosvenor, Stuart Jenkins, Zbigniew Klimont, Norman G. Loeb, Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar Myhre, and Michael Schulz
Atmos. Chem. Phys., 22, 12221–12239, https://doi.org/10.5194/acp-22-12221-2022, https://doi.org/10.5194/acp-22-12221-2022, 2022
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Pollution particles cool climate and offset part of the global warming. However, they are washed out by rain and thus their effect responds quickly to changes in emissions. We show multiple datasets to demonstrate that aerosol emissions and their concentrations declined in many regions influenced by human emissions, as did the effects on clouds. Consequently, the cooling impact on the Earth energy budget became smaller. This change in trend implies a relative warming.
Ukkyo Jeong, Si-Chee Tsay, N. Christina Hsu, David M. Giles, John W. Cooper, Jaehwa Lee, Robert J. Swap, Brent N. Holben, James J. Butler, Sheng-Hsiang Wang, Somporn Chantara, Hyunkee Hong, Donghee Kim, and Jhoon Kim
Atmos. Chem. Phys., 22, 11957–11986, https://doi.org/10.5194/acp-22-11957-2022, https://doi.org/10.5194/acp-22-11957-2022, 2022
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Ultraviolet (UV) measurements from satellite and ground are important for deriving information on several atmospheric trace and aerosol characteristics. Simultaneous retrievals of aerosol and trace gases in this study suggest that water uptake by aerosols is one of the important phenomena affecting aerosol properties over northern Thailand, which is important for regional air quality and climate. Obtained aerosol properties covering the UV are also important for various satellite algorithms.
Abdulaziz Tunde Yakubu and Naven Chetty
Atmos. Chem. Phys., 22, 11065–11087, https://doi.org/10.5194/acp-22-11065-2022, https://doi.org/10.5194/acp-22-11065-2022, 2022
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This study examined the source of atmospheric aerosols and their role in forming clouds and rainfall over South Africa. The research provided answers to the cause of low precipitation, mainly linked to drought and water shortages experienced over the region. Further insight into the cause of occasional flooding that occurs in other parts of the area is provided. Finally, the study described the relationship between aerosol–cloud precipitation based on observation over the region.
África Barreto, Rosa D. García, Carmen Guirado-Fuentes, Emilio Cuevas, A. Fernando Almansa, Celia Milford, Carlos Toledano, Francisco J. Expósito, Juan P. Díaz, and Sergio F. León-Luis
Atmos. Chem. Phys., 22, 11105–11124, https://doi.org/10.5194/acp-22-11105-2022, https://doi.org/10.5194/acp-22-11105-2022, 2022
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A comprehensive characterization of atmospheric aerosols in the subtropical eastern North Atlantic has been carried out in this paper using long-term ground AERONET photometric observations over the period 2005–2020 from a unique network made up of four stations strategically located from sea level to 3555 m height on the island of Tenerife. This is a region that can be considered a key location to study the seasonal dependence of dust transport from the Sahel-Sahara.
Xiaoxi Zhao, Kan Huang, Joshua S. Fu, and Sabur F. Abdullaev
Atmos. Chem. Phys., 22, 10389–10407, https://doi.org/10.5194/acp-22-10389-2022, https://doi.org/10.5194/acp-22-10389-2022, 2022
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Long-range transport of Asian dust to the Arctic was considered an important source of Arctic air pollution. Different transport routes to the Arctic had divergent effects on the evolution of aerosol properties. Depositions of long-range-transported dust particles can reduce the Arctic surface albedo considerably. This study implied that the ubiquitous long-transport dust from China exerted considerable aerosol indirect effects on the Arctic and may have potential biogeochemical significance.
Katherine T. Junghenn Noyes, Ralph A. Kahn, James A. Limbacher, and Zhanqing Li
Atmos. Chem. Phys., 22, 10267–10290, https://doi.org/10.5194/acp-22-10267-2022, https://doi.org/10.5194/acp-22-10267-2022, 2022
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We compare retrievals of wildfire smoke particle size, shape, and light absorption from the MISR satellite instrument to modeling and other satellite data on land cover type, drought conditions, meteorology, and estimates of fire intensity (fire radiative power – FRP). We find statistically significant differences in the particle properties based on burning conditions and land cover type, and we interpret how changes in these properties point to specific aerosol aging mechanisms.
David W. Fillmore, David A. Rutan, Seiji Kato, Fred G. Rose, and Thomas E. Caldwell
Atmos. Chem. Phys., 22, 10115–10137, https://doi.org/10.5194/acp-22-10115-2022, https://doi.org/10.5194/acp-22-10115-2022, 2022
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This paper presents an evaluation of the aerosol analysis incorporated into the Clouds and the Earth's Radiant Energy System (CERES) data products as well as the aerosols' impact on solar radiation reaching the surface. CERES is a NASA Earth observation mission with instruments flying on various polar-orbiting satellites. Its primary objective is the study of the radiative energy balance of the climate system as well as examination of the influence of clouds and aerosols on this balance.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Travis D. Toth, Blake Sorenson, Peter R. Colarco, Zak Kipling, Edward J. Hyer, James R. Campbell, Jeffrey S. Reid, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9915–9947, https://doi.org/10.5194/acp-22-9915-2022, https://doi.org/10.5194/acp-22-9915-2022, 2022
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The study provides baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Harshvardhan Harshvardhan, Richard Ferrare, Sharon Burton, Johnathan Hair, Chris Hostetler, David Harper, Anthony Cook, Marta Fenn, Amy Jo Scarino, Eduard Chemyakin, and Detlef Müller
Atmos. Chem. Phys., 22, 9859–9876, https://doi.org/10.5194/acp-22-9859-2022, https://doi.org/10.5194/acp-22-9859-2022, 2022
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The evolution of aerosol in biomass burning smoke plumes that travel over marine clouds off the Atlantic coast of central Africa was studied using measurements made by a lidar deployed on a high-altitude aircraft. The main finding was that the physical properties of aerosol do not change appreciably once the plume has left land and travels over the ocean over a timescale of 1 to 2 d. Almost all particles in the plume are of radius less than 1 micrometer and spherical in shape.
Peng Xian, Jianglong Zhang, Norm T. O'Neill, Jeffrey S. Reid, Travis D. Toth, Blake Sorenson, Edward J. Hyer, James R. Campbell, and Keyvan Ranjbar
Atmos. Chem. Phys., 22, 9949–9967, https://doi.org/10.5194/acp-22-9949-2022, https://doi.org/10.5194/acp-22-9949-2022, 2022
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The study provides a baseline Arctic spring and summertime aerosol optical depth climatology, trend, and extreme event statistics from 2003 to 2019 using a combination of aerosol reanalyses, remote sensing, and ground observations. Biomass burning smoke has an overwhelming contribution to black carbon (an efficient climate forcer) compared to anthropogenic sources. Burning's large interannual variability and increasing summer trend have important implications for the Arctic climate.
Cited articles
Akagi, S. K., Yokelson, R. J., Wiedinmyer, C., Alvarado, M. J., Reid, J. S., Karl, T., Crounse, J. D., and Wennberg, P. O.: Emission factors for open and domestic biomass burning for use in atmospheric models, Atmos. Chem. Phys., 11, 4039–4072, https://doi.org/10.5194/acp-11-4039-2011, 2011.
Andreae, M. O. and Merlet, P.: Emission of trace gases and aerosols from biomass burning, Global Biogeochem. Cy., 15, 955–966, https://doi.org/10.1029/2000GB001382, 2001.
Arola, A., Schuster, G., Myhre, G., Kazadzis, S., Dey, S., and Tripathi, S. N.: Inferring absorbing organic carbon content from AERONET data, Atmos. Chem. Phys., 11, 215–225, https://doi.org/10.5194/acp-11-215-2011, 2011.
Bohren, C. F. and Huffman, D. R.: Absorption and scattering of light by small particles, John Wiley & Sons, New York, 1983.
Bond, T. C. and Bergstrom, R. W.: Light absorption by carbonaceous particles: an investigative review, Aerosol Sci. Tech., 40, 27–67, 2006.
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., DeAngelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., Kinne, S., Kondo, Y., Quinn, P. K., Sarofim, M. C., Schultz, M. G., Schulz, M., Venkataraman, C., Zhang, H., Zhang, S., Bellouin, N., Guttikunda, S. K., Hopke, P. K., Jacobson, M. Z., Kaiser, J. W., Klimont, Z., Lohmann, U., Schwarz, J. P., Shindell, D., Storelvmo, T., Warren, S. G., and Zender, C. S.: Bounding the role of black carbon in the climate system: a scientific assessment, J. Geophys. Res.-Atmos., 118, 5380–5552, https://doi.org/10.1002/jgrd.50171, 2013.
Brock, C. A., Cozic, J., Bahreini, R., Froyd, K. D., Middlebrook, A. M., McComiskey, A., Brioude, J., Cooper, O. R., Stohl, A., Aikin, K. C., de Gouw, J. A., Fahey, D. W., Ferrare, R. A., Gao, R.-S., Gore, W., Holloway, J. S., Hübler, G., Jefferson, A., Lack, D. A., Lance, S., Moore, R. H., Murphy, D. M., Nenes, A., Novelli, P. C., Nowak, J. B., Ogren, J. A., Peischl, J., Pierce, R. B., Pilewskie, P., Quinn, P. K., Ryerson, T. B., Schmidt, K. S., Schwarz, J. P., Sodemann, H., Spackman, J. R., Stark, H., Thomson, D. S., Thornberry, T., Veres, P., Watts, L. A., Warneke, C., and Wollny, A. G.: Characteristics, sources, and transport of aerosols measured in spring 2008 during the aerosol, radiation, and cloud processes affecting Arctic Climate (ARCPAC) Project, Atmos. Chem. Phys., 11, 2423–2453, https://doi.org/10.5194/acp-11-2423-2011, 2011.
Chand, D., Guyon, P., Artaxo, P., Schmid, O., Frank, G. P., Rizzo, L. V., Mayol-Bracero, O. L., Gatti, L. V., and Andreae, M. O.: Optical and physical properties of aerosols in the boundary layer and free troposphere over the Amazon Basin during the biomass burning season, Atmos. Chem. Phys., 6, 2911–2925, https://doi.org/10.5194/acp-6-2911-2006, 2006.
Colarco, P., Schoeberl, M., Doddridge, B., Marufu, L., Torres, O., and Welton, E.: Transport of smoke from Canadian forest fires to the surface near Washington, DC: injection height, entrainment, and optical properties, J. Geophys. Res.-Atmos., 109, D06203, https://doi.org/10.1029/2003JD004248, 2004.
Dahlkötter, F., Gysel, M., Sauer, D., Minikin, A., Baumann, R., Seifert, P., Ansmann, A., Fromm, M., Voigt, C., and Weinzierl, B.: The Pagami Creek smoke plume after long-range transport to the upper troposphere over Europe – aerosol properties and black carbon mixing state, Atmos. Chem. Phys., 14, 6111–6137, https://doi.org/10.5194/acp-14-6111-2014, 2014.
Damoah, R., Spichtinger, N., Forster, C., James, P., Mattis, I., Wandinger, U., Beirle, S., Wagner, T., and Stohl, A.: Around the world in 17 days – hemispheric-scale transport of forest fire smoke from Russia in May 2003, Atmos. Chem. Phys., 4, 1311–1321, https://doi.org/10.5194/acp-4-1311-2004, 2004.
Darmenov, A. and da Silva, A.: The Quick Fire Emissions Dataset (QFED): Documentation of versions 2.1, 2.2 and 2.4. NASA/TM-2015-104606, 38, available at: http://gmao.gsfc.nasa.gov/pubs/docs/Darmenov796.pdf, last access: 1 December 2015.
Dick, W. D., Ziemann, P. J., and McMurry, P. H.: Multiangle light-scattering measurements of refractive index of submicron atmospheric particles, Aerosol Sci. Tech., 41, 549–569, 2007.
Draxler, R. and Rolph, G.: HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) model access via NOAA ARL READY website, available at: http://www.arl.noaa.gov/ready/hysplit4.html (last access: 17 December 2014), NOAA Air Resources Laboratory, Silver Spring, 2003.
Dubovik, O. and King, M. D.: a flexible inversion algorithm for retrieval of aerosol optical properties from Sun and sky radiance measurements, J. Geophys. Res.-Atmos., 105, 20673–20696, 2000.
Dubovik, O., Smirnov, A., Holben, B., King, M., Kaufman, Y., Eck, T., and Slutsker, I.: Accuracy assessments of aerosol optical properties retrieved from Aerosol Robotic Network (AERONET) Sun and sky radiance measurements, J. Geophys. Res.-Atmos., 105, 9791–9806, 2000.
Dubovik, O., Holben, B., Eck, T. F., Smirnov, A., Kaufman, Y. J., King, M. D., Tanre, D., and Slutsker, I.: Variability of absorption and optical properties of key aerosol types observed in worldwide locations, J. Atmos. Sci., 59, 590–608, 2002.
Dubovik, O., Lapyonok, T., Kaufman, Y. J., Chin, M., Ginoux, P., Kahn, R. A., and Sinyuk, A.: Retrieving global aerosol sources from satellites using inverse modeling, Atmos. Chem. Phys., 8, 209–250, https://doi.org/10.5194/acp-8-209-2008, 2008.
French, N. H. F., Goovaerts, P., and Kasischke, E. S.: Uncertainty in estimating carbon emissions from boreal forest fires, J. Geophys. Res.-Atmos., 109, https://doi.org/10.1029/2003JD003635, 2004.
Giglio, L., Csiszar, I., and Justice, C. O.: Global distribution and seasonality of active fires as observed with the Terra and Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) sensors, J. Geophys. Res., 111, https://doi.org/10.1029/2005JG000142, 2006.
Giglio, L., Randerson, J. T., and Van der Werf, G. R.: Analysis of daily, monthly, and annual burned area using the fourth-generation global fire emissions database (GFED4), J. Geophys. Res., 118, 317–328, https://doi.org/10.1002/jgrg.20042, 2013.
Hobbs, P. V., Reid, J. S., Herring, J. A., Nance, J. D., and Weiss, R. E.: Particle and Trace-Gas Measurements in the Smoke from Prescribed Burns of Forest Products in the Pacific Northwest, in: Biomass Burning and Global Change, Vol. 1, edited by: Levine, J. S., MIT Press, New York, 1006, 697–715, 1996.
Hoffer, A., Gelencsér, A., Guyon, P., Kiss, G., Schmid, O., Frank, G. P., Artaxo, P., and Andreae, M. O.: Optical properties of humic-like substances (HULIS) in biomass-burning aerosols, Atmos. Chem. Phys., 6, 3563–3570, https://doi.org/10.5194/acp-6-3563-2006, 2006.
Holben, B., Eck, T., Slutsker, I., Tanre, D., Buis, J., Setzer, A., Vermote, E., Reagan, J., Kaufman, Y., Nakajima, T., Lavenu, F., Jankowiak, I., and Smirnov, A.: AERONET a federated instrument network and data archive for aerosol characterization, Remote Sens. Environ., 66, 1–16, 1998.
Hyer, E. J. and Reid, J. S.: Baseline uncertainties in biomass burning emission models resulting from spatial error in satellite active fire location data, J. Geophys. Res. Lett., 36, L05802, https://doi.org/10.1029/2008GL036767, 2009.
Hyer, E. J., Reid, J. S., and Zhang, J.: An over-land aerosol optical depth data set for data assimilation by filtering, correction, and aggregation of MODIS Collection 5 optical depth retrievals, Atmos. Meas. Tech., 4, 379–408, https://doi.org/10.5194/amt-4-379-2011, 2011.
Ichoku, C. and Ellison, L.: Global top-down smoke-aerosol emissions estimation using satellite fire radiative power measurements, Atmos. Chem. Phys., 14, 6643–6667, https://doi.org/10.5194/acp-14-6643-2014, 2014.
Ichoku, C. and Kaufman, Y. J.: a method to derive smoke emission rates from MODIS fire radiative energy measurements, IEEE T. Geosci. Remote, 43, 2636–2649, https://doi.org/10.1109/TGRS.2005.857328, 2005.
Janhäll, S., Andreae, M. O., and Pöschl, U.: Biomass burning aerosol emissions from vegetation fires: particle number and mass emission factors and size distributions, Atmos. Chem. Phys., 10, 1427–1439, https://doi.org/10.5194/acp-10-1427-2010, 2010.
Johnston, F. H., Henderson, S. B., Chen, Y., Randerson, J. T., Marlier, M., DeFries, R. S., Kinney, P., Bowman, D. M., and Brauer, M.: Estimated global mortality attributable to smoke from landscape fires, Environ. Health Persp., 120, 695–701, 2012.
Kaiser, J. W., Heil, A., Andreae, M. O., Benedetti, A., Chubarova, N., Jones, L., Morcrette, J.-J., Razinger, M., Schultz, M. G., Suttie, M., and van der Werf, G. R.: Biomass burning emissions estimated with a global fire assimilation system based on observed fire radiative power, Biogeosciences, 9, 527–554, https://doi.org/10.5194/bg-9-527-2012, 2012.
Kasischke, E. S., Williams, D., and Barry, D.: Analysis of the patterns of large fires in the boreal forest region of Alaska, Int. J. Wildland Fire, 11, 131–144, 2002.
Kaufman, Y. J. and Tanre, D.: Algorithm for remote sensing of tropospheric aerosol from MODIS, NASA MODIS Algorithm Theoretical Basis Document, Goddard Space Flight Center, Greenbelt, Md, 85 pp., 1998.
Kirchstetter, T. W., Novakov, T., and Hobbs, P. V.: Evidence that the spectral dependence of light absorption by aerosols is affected by organic carbon, J. Geophys. Res.-Atmos., 109, D21208, https://doi.org/10.1029/2004JD004999, 2004.
Kotchenmther, R. A. and Hobbs, P. V.: Humidification factors of aerosols from biomass burning, J. Geophys. Res.-Atmos., 104, 2239–2251, 1998.
Kreidenweis, S. M., Remer, L. A., Bruintjes, R., and Dubovik, O.: Smoke aerosol from biomass burning in Mexico: Hygroscopic smoke optical model, J. Geophys. Res.-Atmos., 106, 4831–4844, https://doi.org/10.1029/2000JD900488, 2001.
Langmann, B., Duncan, B., Textor, C., Trentmann, J., and van der Werf, G. R.: Vegetation fire emissions and their impact on air pollution and climate, Atmos. Environ., 43, 107–116, 2009.
Levy, R. C., Remer, L. A., Tanre, D., Mattoo, S., and Kaufman, Y. J.: Algorithm for Remote Sensing of Tropospheric Aerosol over Dark Targets from MODIS: Collections 005 and 051: Revision 2, February 2009, available at: http://modis-atmos.gsfc.nasa.gov/_docs/ATBD_MOD04_C005_rev2.pdf (last access: 24 February 2015), 2009.
Levy, R. C., Remer, L. A., Kleidman, R. G., Mattoo, S., Ichoku, C., Kahn, R., and Eck, T. F.: Global evaluation of the Collection 5 MODIS dark-target aerosol products over land, Atmos. Chem. Phys., 10, 10399–10420, https://doi.org/10.5194/acp-10-10399-2010, 2010.
Livingston, J. M., Redemann, J., Shinozuka, Y., Johnson, R., Russell, P. B., Zhang, Q., Mattoo, S., Remer, L., Levy, R., Munchak, L., and Ramachandran, S.: Comparison of MODIS 3 km and 10 km resolution aerosol optical depth retrievals over land with airborne sunphotometer measurements during ARCTAS summer 2008, Atmos. Chem. Phys., 14, 2015–2038, https://doi.org/10.5194/acp-14-2015-2014, 2014.
Liu, Y., Stanturf, J., and Scott, G.: Trends in global wildfire potential in a changing climate, Forest Ecol. Manag., 259, 685–697,2013.
Magi, B. I. and Hobbs, P. V.: Effects of humidity on aerosols in southern Africa during the biomass burning season, J. Geophys. Res.-Atmos., 108, 2156–2202, 2003
Nikonovas, T., North, P. R. J., and Doerr, S. H.: Smoke aerosol properties and ageing effects for northern temperate and boreal regions derived from AERONET source and age attribution, Atmos. Chem. Phys., 15, 7929–7943, https://doi.org/10.5194/acp-15-7929-2015, 2015.
O'Neill, N. T., Eck, T. F., Holben, B. N., Smirnov, A., Royer, A., and Li, Z.: Optical properties of boreal forest fire smoke derived from Sun photometry, J. Geophys. Res.-Atmos., 107, AAC 6-1–AAC 6-19, https://doi.org/10.1029/2001JD000877, 2002.
Peterson, D., Hyer, E., and Wang, J.: Quantifying the potential for high-altitude smoke injection in the North American boreal forest using the standard MODIS fire products and subpixel-based methods, J. Geophys. Res.-Atmos., 119, 3401–3419, https://doi.org/10.1002/2013JD021067, 2014.
Randerson, J. T., Chen, Y., Van der Werf, G. R., Rogers, B. M., and Morton, D. C.: Global burned area and biomass burning emissions from small fires, J. Geophys. Res., 117, G04012, https://doi.org/10.1029/2012JG002128, 2012.
Reid, J. S., Koppmann, R., Eck, T. F., and Eleuterio, D. P.: A review of biomass burning emissions part II: intensive physical properties of biomass burning particles, Atmos. Chem. Phys., 5, 799–825, https://doi.org/10.5194/acp-5-799-2005, 2005a.
Reid, J. S., Eck, T. F., Christopher, S. A., Koppmann, R., Dubovik, O., Eleuterio, D. P., Holben, B. N., Reid, E. A., and Zhang, J.: A review of biomass burning emissions part III: intensive optical properties of biomass burning particles, Atmos. Chem. Phys., 5, 827–849, https://doi.org/10.5194/acp-5-827-2005, 2005b.
Reid, J. S. and Hobbs, P. V.: Physical and optical properties of young smoke from individual biomass fires in Brazil, J. Geophys. Res.-Atmos., 103, 32013–32030, 1998.
Rudich, Y., Donahue, N. M., and Mentel, T. F.: Aging of organic aerosol: Bridging the gap between laboratory and field studies, Annu. Rev. Phys. Chem., 58, 321–352, 2007.
Saide, P. E., Peterson, D. A., da Silva, A., Anderson, B., Ziemba, L. D., Diskin, G., Sachse, G., Hair, J., Butler, C., Fenn, M., Jimenez, J. L., Campuzano-Jost, P., Perring, A. E., Schwarz, J. P., Markovic, M. Z., Russell, P., Redemann, J., Shinozuka, Y., Streets, D. G., Yan, F., Dibb, J., Yokelson, R., Toon, O. B., Hyer, E., and Carmichael, G. R.: Revealing important nocturnal and day-to-day variations in fire smoke emissions through a multiplatform inversion, Geophys. Res. Lett., 42, 3609–3618, https://doi.org/10.1002/2015GL063737, 2015.
Schuster, G. L., Dubovik, O., Holben, B. N., and Clothiaux, E. E.: Inferring black carbon content and specific absorption from Aerosol Robotic Network (AERONET) aerosol retrievals, J. Geoph. Res.-Atmos., 110, https://doi.org/10.1029/2004JD004548, 2005.
Schuster, G. L., Lin, B., and Dubovik, O.: Remote sensing of aerosol water uptake, Geophys. Res. Lett., 36, L03814, https://doi.org/10.1029/2008GL036576, 2009.
Schuster, G. L., Dubovik, O., and Arola, A.: Remote sensing of soot carbon – Part 1: Distinguishing different absorbing aerosol species, Atmos. Chem. Phys., 16, 1565–1585, https://doi.org/10.5194/acp-16-1565-2016, 2016.
Stocks, B. J., Mason, J. A., Todd, J. B., Bosch, E. M., Wotton, B. M., Amiro, B. D., Flannigan, M. D., Hirsch, K. G., Logan, K. A., Martell, D. L., and Skinner, W. R.: Large forest fires in Canada, 1959–1997, J. Geophys. Res.-Atmos., 107, 8149, https://doi.org/10.1029/2001JD000484, 2002.
Strauss, D., Bednar, L., and Mees, R.: Do one percent of the forest fires cause ninety-nine percent of the damage?, Forest Sci., 35, 319–328, 1989.
Swietlicki, E., Hansson, H.-C., Hämeri, K., Svenningsson, B., Massling, A., Mcfiggans, G., Mcmurry, P. H., Petäjä, T., Tunved, P., Gysel, M., Topping, D., Weingartner, E., Baltensperger, U., Rissler, J., Wiedensohler, A., and Kulmala, M.: Hygroscopic properties of submicrometer atmospheric aerosol particles measured with H-TDMA instruments in various environments – a review, Tellus B, 60, 432–469, https://doi.org/10.1111/j.1600-0889.2008.00350.x, 2008.
Toon, O. B., Pollack, J. B., and Khare, B. N.: The optical constants of several atmospheric aerosol species: Ammonium sulfate, aluminum oxide, and sodium chloride, J. Geophys. Res., 81, 5733–5748, https://doi.org/10.1029/JC081i033p05733, 1976.
Turetsky, M., R., Benscoter, B., Page, S., Rein, G., Van der Werf, G. R., and Watts, A.: Global vulnerability of peatlands to fire and carbon loss, Nat. Geosci., 8, 11–14, 2015.
Turpin, B. J. and Lim, H.: Species Contributions to PM2. 5 Mass Concentrations: Revisiting Common Assumptions for Estimating Organic Mass, Aerosol Sci. Tech., 35, 602–610, https://doi.org/10.1080/02786820119445, 2001.
Urbanski, S.: Wildland fire emissions, carbon, and climate: Emission factors, Forest Ecol. Manag., 317, 51–60, https://doi.org/10.1016/j.foreco.2013.05.045, 2014.
Val Martin, M., Logan, J. A., Kahn, R. A., Leung, F.-Y., Nelson, D. L., and Diner, D. J.: Smoke injection heights from fires in North America: analysis of 5 years of satellite observations, Atmos. Chem. Phys., 10, 1491–1510, https://doi.org/10.5194/acp-10-1491-2010, 2010.
van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Mu, M., Kasibhatla, P. S., Morton, D. C., DeFries, R. S., Jin, Y., and van Leeuwen, T. T.: Global fire emissions and the contribution of deforestation, savanna, forest, agricultural, and peat fires (1997–2009), Atmos. Chem. Phys., 10, 11707–11735, https://doi.org/10.5194/acp-10-11707-2010, 2010.
van Leeuwen, T. T. and van der Werf, G. R.: Spatial and temporal variability in the ratio of trace gases emitted from biomass burning, Atmos. Chem. Phys., 11, 3611–3629, https://doi.org/10.5194/acp-11-3611-2011, 2011.
van Leeuwen, T. T., van der Werf, G. R., Hoffmann, A. A., Detmers, R. G., Rücker, G., French, N. H. F., Archibald, S., Carvalho Jr., J. A., Cook, G. D., de Groot, W. J., Hély, C., Kasischke, E. S., Kloster, S., McCarty, J. L., Pettinari, M. L., Savadogo, P., Alvarado, E. C., Boschetti, L., Manuri, S., Meyer, C. P., Siegert, F., Trollope, L. A., and Trollope, W. S. W.: Biomass burning fuel consumption rates: a field measurement database, Biogeosciences, 11, 7305–7329, https://doi.org/10.5194/bg-11-7305-2014, 2014.
Wooster, M. J., Zhukov, B., and Oertel, D.: Fire radiative energy for quantitative study of biomass burning: derivation from the {BIRD} experimental satellite and comparison to {MODIS} fire products, Remote Sens. Environ., 86, 83–107, https://doi.org/10.1016/S0034-4257(03)00070-1, 2003.
Wooster, M. J., Roberts, G., Perry, G. L. W., and Kaufman, Y. J.: Retrieval of biomass combustion rates and totals from fire radiative power observations: FRP derivation and calibration relationships between biomass consumption and fire radiative energy release, J. Geophys. Res.-Atmos., 110, D24311, https://doi.org/10.1029/2005JD006318, 2005.
Short summary
The study presents a new method for estimating particulate matter emissions from large wildfires. The method relies solely on satellite observations of fire activity and particles suspended in the atmosphere. The results indicate that temperate and boreal forest fires in North America emit similar amounts of particles per unit of fire radiative power. The findings differ from estimates by modelling studies which suggest much larger emissions for boreal events compared to temperate fires.
The study presents a new method for estimating particulate matter emissions from large...
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