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Volume 16, issue 14
Atmos. Chem. Phys., 16, 9003–9018, 2016
https://doi.org/10.5194/acp-16-9003-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 16, 9003–9018, 2016
https://doi.org/10.5194/acp-16-9003-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 22 Jul 2016

Research article | 22 Jul 2016

Linking variations in sea spray aerosol particle hygroscopicity to composition during two microcosm experiments

Sara D. Forestieri et al.

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Ault, A. P., Guasco, T. L., Ryder, O. S., Baltrusaitis, J., Cuadra-Rodriguez, L. A., Collins, D. B., Ruppel, M. J., Bertram, T. H., Prather, K. A., and Grassian, V. H.: Inside versus outside: Ion redistribution in nitric acid reacted sea spray aerosol particles as determined by single particle analysis, J. Am. Chem. Soc., 135, 14528–14531, https://doi.org/10.1021/ja407117x, 2013.
Bates, T., Quinn, P., Frossard, A., Russell, L., Hakala, J., Petäjä, T., Kulmala, M., Covert, D., Cappa, C., and Li, S. M.: Measurements of ocean derived aerosol off the coast of california, J. Geophys. Res.-Atmos., 117, D00V15, https://doi.org/10.1029/2012JD017588, 2012.
Biskos, G., Malinowski, A., Russell, L., Buseck, P., and Martin, S.: Nanosize effect on the deliquescence and the efflorescence of sodium chloride particles, Aerosol Sci. Tech., 40, 97–106, https://doi.org/10.1080/02786820500484396, 2006.
Bouvet, M., Hoepffner, N., and Dowell, M. D.: Parameterization of a spectral solar irradiance model for the global ocean using multiple satellite sensors, J. Geophys. Res.-Oceans, 107, 8-1–8-18, https://doi.org/10.1029/2001JC001126, 2002.
Canagaratna, M. R., Jayne, J. T., Jimenez, J. L., Allan, J. D., Alfarra, M. R., Zhang, Q., Onasch, T. B., Drewnick, F., Coe, H., Middlebrook, A., Delia, A., Williams, L. R., Trimborn, A. M., Northway, M. J., DeCarlo, P. F., Kolb, C. E., Davidovits, P., and Worsnop, D. R.: Chemical and microphysical characterization of ambient aerosols with the aerodyne aerosol mass spectrometer, Mass Spectrom. Rev., 26, 185–222, https://doi.org/10.1002/mas.20115, 2007.
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Hygroscopic growth factors at 85 % relative humidity (GF(85 %)) were quantified along with particle composition for primary sea spray aerosol (SSA) particles generated in marine aerosol reference tanks (MARTs) from seawater in which two independent phytoplankton blooms were induced. The observed 5 to 15 % depression in the GF(85 %) values (relative to pure sea salt) is consistent with the large observed volume fractions of non-refractory organic matter (NR-OM) comprising the SSA.
Hygroscopic growth factors at 85 % relative humidity (GF(85 %)) were quantified along with...
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