Articles | Volume 16, issue 14
https://doi.org/10.5194/acp-16-9003-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-9003-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
22 Jul 2016
Research article |
| 22 Jul 2016
Linking variations in sea spray aerosol particle hygroscopicity to composition during two microcosm experiments
Sara D. Forestieri
Department of Civil and Environmental Engineering, University of
California, Davis, CA 95616, USA
Gavin C. Cornwell
Department of Chemistry and Biochemistry, University of California,
San Diego, La Jolla, CA 92093, USA
Taylor M. Helgestad
Department of Civil and Environmental Engineering, University of
California, Davis, CA 95616, USA
Kathryn A. Moore
Department of Chemistry and Biochemistry, University of California,
San Diego, La Jolla, CA 92093, USA
Christopher Lee
Department of Chemistry and Biochemistry, University of California,
San Diego, La Jolla, CA 92093, USA
Gordon A. Novak
Department of Chemistry, University of Wisconsin, Madison, WI 53706, USA
Camille M. Sultana
Department of Chemistry and Biochemistry, University of California,
San Diego, La Jolla, CA 92093, USA
Xiaofei Wang
Department of Chemistry and Biochemistry, University of California,
San Diego, La Jolla, CA 92093, USA
Timothy H. Bertram
Department of Chemistry and Biochemistry, University of California,
San Diego, La Jolla, CA 92093, USA
Department of Chemistry, University of Wisconsin, Madison, WI 53706, USA
Kimberly A. Prather
Department of Chemistry and Biochemistry, University of California,
San Diego, La Jolla, CA 92093, USA
Scripps Institution of Oceanography, 9500 Gilman Drive, La Jolla, CA
92093, USA
Department of Civil and Environmental Engineering, University of
California, Davis, CA 95616, USA
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Cited
29 citations as recorded by crossref.
- Summertime Primary and Secondary Contributions to Southern Ocean Cloud Condensation Nuclei K. Fossum et al. 10.1038/s41598-018-32047-4
- Sodium–carboxylate contact ion pair formation induces stabilization of palmitic acid monolayers at high pH E. Adams et al. 10.1039/C7CP00167C
- Discerning Poly- and Monosaccharide Enrichment Mechanisms: Alginate and Glucuronate Adsorption to a Stearic Acid Sea Surface Microlayer M. Vazquez de Vasquez et al. 10.1021/acsearthspacechem.2c00066
- Biological Influence on δ13C and Organic Composition of Nascent Sea Spray Aerosol D. Crocker et al. 10.1021/acsearthspacechem.0c00072
- Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry J. Schiffer et al. 10.1021/acscentsci.8b00674
- A Dynamic Link between Ice Nucleating Particles Released in Nascent Sea Spray Aerosol and Oceanic Biological Activity during Two Mesocosm Experiments C. McCluskey et al. 10.1175/JAS-D-16-0087.1
- Halide Ion Microhydration: Structure, Energetics, and Spectroscopy of Small Halide–Water Clusters P. Bajaj et al. 10.1021/acs.jpca.9b00816
- Biological Impacts on Carbon Speciation and Morphology of Sea Spray Aerosol D. Pham et al. 10.1021/acsearthspacechem.7b00069
- Effects of Wind Speed on Size-Dependent Morphology and Composition of Sea Spray Aerosols C. Madawala et al. 10.1021/acsearthspacechem.4c00119
- Number‐Size Distribution and CCN Activity of Atmospheric Aerosols in the Western North Pacific During Spring Pre‐Bloom Period: Influences of Terrestrial and Marine Sources K. Kawana et al. 10.1029/2022JD036690
- Impacts of marine organic emissions on low-level stratiform clouds – a large eddy simulator study M. Prank et al. 10.5194/acp-22-10971-2022
- Physicochemical Mixing State of Sea Spray Aerosols: Morphologies Exhibit Size Dependence H. Lee et al. 10.1021/acsearthspacechem.0c00153
- Expanding Single Particle Mass Spectrometer Analyses for the Identification of Microbe Signatures in Sea Spray Aerosol C. Sultana et al. 10.1021/acs.analchem.7b00933
- Linking hygroscopicity and the surface microstructure of model inorganic salts, simple and complex carbohydrates, and authentic sea spray aerosol particles A. Estillore et al. 10.1039/C7CP04051B
- Effect of Structural Heterogeneity in Chemical Composition on Online Single-Particle Mass Spectrometry Analysis of Sea Spray Aerosol Particles C. Sultana et al. 10.1021/acs.est.6b06399
- Size-Dependent Morphology, Composition, Phase State, and Water Uptake of Nascent Submicrometer Sea Spray Aerosols during a Phytoplankton Bloom C. Kaluarachchi et al. 10.1021/acsearthspacechem.1c00306
- Mass Spectrometry Analysis in Atmospheric Chemistry J. Laskin et al. 10.1021/acs.analchem.7b04249
- Aerosol Emissions from Great Lakes Harmful Algal Blooms N. May et al. 10.1021/acs.est.7b03609
- Impacts of Lipase Enzyme on the Surface Properties of Marine Aerosols J. Schiffer et al. 10.1021/acs.jpclett.8b01363
- Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea R. Kirpes et al. 10.1039/C9EM00495E
- Classification of aerosol population type and cloud condensation nuclei properties in a coastal California littoral environment using an unsupervised cluster model S. Atwood et al. 10.5194/acp-19-6931-2019
- The Impact of Divalent Cations on the Enrichment of Soluble Saccharides in Primary Sea Spray Aerosol S. Schill et al. 10.3390/atmos9120476
- Probing Individual Particles Generated at the Freshwater–Seawater Interface through Combined Raman, Photothermal Infrared, and X-ray Spectroscopic Characterization J. Mirrielees et al. 10.1021/acsmeasuresciau.2c00041
- Size-resolved aerosol and cloud condensation nuclei (CCN) properties in the remote marine South China Sea – Part 1: Observations and source classification S. Atwood et al. 10.5194/acp-17-1105-2017
- Sea Spray Aerosol: The Chemical Link between the Oceans, Atmosphere, and Climate R. Cochran et al. 10.1021/acs.accounts.6b00603
- Sea spray aerosol chemical composition: elemental and molecular mimics for laboratory studies of heterogeneous and multiphase reactions T. Bertram et al. 10.1039/C7CS00008A
- Chemical composition-dependent hygroscopic behavior of individual ambient aerosol particles collected at a coastal site L. Wu et al. 10.5194/acp-23-12571-2023
- Organic Enrichment, Physical Phase State, and Surface Tension Depression of Nascent Core–Shell Sea Spray Aerosols during Two Phytoplankton Blooms H. Lee et al. 10.1021/acsearthspacechem.0c00032
- Effects of Atmospheric Aging Processes on Nascent Sea Spray Aerosol Physicochemical Properties C. Kaluarachchi et al. 10.1021/acsearthspacechem.2c00258
29 citations as recorded by crossref.
- Summertime Primary and Secondary Contributions to Southern Ocean Cloud Condensation Nuclei K. Fossum et al. 10.1038/s41598-018-32047-4
- Sodium–carboxylate contact ion pair formation induces stabilization of palmitic acid monolayers at high pH E. Adams et al. 10.1039/C7CP00167C
- Discerning Poly- and Monosaccharide Enrichment Mechanisms: Alginate and Glucuronate Adsorption to a Stearic Acid Sea Surface Microlayer M. Vazquez de Vasquez et al. 10.1021/acsearthspacechem.2c00066
- Biological Influence on δ13C and Organic Composition of Nascent Sea Spray Aerosol D. Crocker et al. 10.1021/acsearthspacechem.0c00072
- Sea Spray Aerosol: Where Marine Biology Meets Atmospheric Chemistry J. Schiffer et al. 10.1021/acscentsci.8b00674
- A Dynamic Link between Ice Nucleating Particles Released in Nascent Sea Spray Aerosol and Oceanic Biological Activity during Two Mesocosm Experiments C. McCluskey et al. 10.1175/JAS-D-16-0087.1
- Halide Ion Microhydration: Structure, Energetics, and Spectroscopy of Small Halide–Water Clusters P. Bajaj et al. 10.1021/acs.jpca.9b00816
- Biological Impacts on Carbon Speciation and Morphology of Sea Spray Aerosol D. Pham et al. 10.1021/acsearthspacechem.7b00069
- Effects of Wind Speed on Size-Dependent Morphology and Composition of Sea Spray Aerosols C. Madawala et al. 10.1021/acsearthspacechem.4c00119
- Number‐Size Distribution and CCN Activity of Atmospheric Aerosols in the Western North Pacific During Spring Pre‐Bloom Period: Influences of Terrestrial and Marine Sources K. Kawana et al. 10.1029/2022JD036690
- Impacts of marine organic emissions on low-level stratiform clouds – a large eddy simulator study M. Prank et al. 10.5194/acp-22-10971-2022
- Physicochemical Mixing State of Sea Spray Aerosols: Morphologies Exhibit Size Dependence H. Lee et al. 10.1021/acsearthspacechem.0c00153
- Expanding Single Particle Mass Spectrometer Analyses for the Identification of Microbe Signatures in Sea Spray Aerosol C. Sultana et al. 10.1021/acs.analchem.7b00933
- Linking hygroscopicity and the surface microstructure of model inorganic salts, simple and complex carbohydrates, and authentic sea spray aerosol particles A. Estillore et al. 10.1039/C7CP04051B
- Effect of Structural Heterogeneity in Chemical Composition on Online Single-Particle Mass Spectrometry Analysis of Sea Spray Aerosol Particles C. Sultana et al. 10.1021/acs.est.6b06399
- Size-Dependent Morphology, Composition, Phase State, and Water Uptake of Nascent Submicrometer Sea Spray Aerosols during a Phytoplankton Bloom C. Kaluarachchi et al. 10.1021/acsearthspacechem.1c00306
- Mass Spectrometry Analysis in Atmospheric Chemistry J. Laskin et al. 10.1021/acs.analchem.7b04249
- Aerosol Emissions from Great Lakes Harmful Algal Blooms N. May et al. 10.1021/acs.est.7b03609
- Impacts of Lipase Enzyme on the Surface Properties of Marine Aerosols J. Schiffer et al. 10.1021/acs.jpclett.8b01363
- Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea R. Kirpes et al. 10.1039/C9EM00495E
- Classification of aerosol population type and cloud condensation nuclei properties in a coastal California littoral environment using an unsupervised cluster model S. Atwood et al. 10.5194/acp-19-6931-2019
- The Impact of Divalent Cations on the Enrichment of Soluble Saccharides in Primary Sea Spray Aerosol S. Schill et al. 10.3390/atmos9120476
- Probing Individual Particles Generated at the Freshwater–Seawater Interface through Combined Raman, Photothermal Infrared, and X-ray Spectroscopic Characterization J. Mirrielees et al. 10.1021/acsmeasuresciau.2c00041
- Size-resolved aerosol and cloud condensation nuclei (CCN) properties in the remote marine South China Sea – Part 1: Observations and source classification S. Atwood et al. 10.5194/acp-17-1105-2017
- Sea Spray Aerosol: The Chemical Link between the Oceans, Atmosphere, and Climate R. Cochran et al. 10.1021/acs.accounts.6b00603
- Sea spray aerosol chemical composition: elemental and molecular mimics for laboratory studies of heterogeneous and multiphase reactions T. Bertram et al. 10.1039/C7CS00008A
- Chemical composition-dependent hygroscopic behavior of individual ambient aerosol particles collected at a coastal site L. Wu et al. 10.5194/acp-23-12571-2023
- Organic Enrichment, Physical Phase State, and Surface Tension Depression of Nascent Core–Shell Sea Spray Aerosols during Two Phytoplankton Blooms H. Lee et al. 10.1021/acsearthspacechem.0c00032
- Effects of Atmospheric Aging Processes on Nascent Sea Spray Aerosol Physicochemical Properties C. Kaluarachchi et al. 10.1021/acsearthspacechem.2c00258
Saved (preprint)
Latest update: 14 Dec 2024
Short summary
Hygroscopic growth factors at 85 % relative humidity (GF(85 %)) were quantified along with particle composition for primary sea spray aerosol (SSA) particles generated in marine aerosol reference tanks (MARTs) from seawater in which two independent phytoplankton blooms were induced. The observed 5 to 15 % depression in the GF(85 %) values (relative to pure sea salt) is consistent with the large observed volume fractions of non-refractory organic matter (NR-OM) comprising the SSA.
Hygroscopic growth factors at 85 % relative humidity (GF(85 %)) were quantified along with...
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