Articles | Volume 13, issue 9
Atmos. Chem. Phys., 13, 4681–4695, 2013
https://doi.org/10.5194/acp-13-4681-2013
Atmos. Chem. Phys., 13, 4681–4695, 2013
https://doi.org/10.5194/acp-13-4681-2013

Research article 06 May 2013

Research article | 06 May 2013

Heterogeneous ice nucleation on phase-separated organic-sulfate particles: effect of liquid vs. glassy coatings

G. P. Schill and M. A. Tolbert

Related authors

Ambient aerosol properties in the remote atmosphere from global-scale in situ measurements
Charles A. Brock, Karl D. Froyd, Maximilian Dollner, Christina J. Williamson, Gregory Schill, Daniel M. Murphy, Nicholas J. Wagner, Agnieszka Kupc, Jose L. Jimenez, Pedro Campuzano-Jost, Benjamin A. Nault, Jason C. Schroder, Douglas A. Day, Derek J. Price, Bernadett Weinzierl, Joshua P. Schwarz, Joseph M. Katich, Siyuan Wang, Linghan Zeng, Rodney Weber, Jack Dibb, Eric Scheuer, Glenn S. Diskin, Joshua P. DiGangi, ThaoPaul​​​​​​​ Bui, Jonathan M. Dean-Day, Chelsea R. Thompson, Jeff Peischl, Thomas B. Ryerson, Ilann Bourgeois, Bruce C. Daube, Róisín Commane, and Steven C. Wofsy
Atmos. Chem. Phys., 21, 15023–15063, https://doi.org/10.5194/acp-21-15023-2021,https://doi.org/10.5194/acp-21-15023-2021, 2021
Short summary
Large hemispheric difference in nucleation mode aerosol concentrations in the lowermost stratosphere at mid- and high latitudes
Christina J. Williamson, Agnieszka Kupc, Andrew Rollins, Jan Kazil, Karl D. Froyd, Eric A. Ray, Daniel M. Murphy, Gregory P. Schill, Jeff Peischl, Chelsea Thompson, Ilann Bourgeois, Thomas B. Ryerson, Glenn S. Diskin, Joshua P. DiGangi, Donald R. Blake, Thao Paul V. Bui, Maximilian Dollner, Bernadett Weinzierl, and Charles A. Brock
Atmos. Chem. Phys., 21, 9065–9088, https://doi.org/10.5194/acp-21-9065-2021,https://doi.org/10.5194/acp-21-9065-2021, 2021
Short summary
Radiative and chemical implications of the size and composition of aerosol particles in the existing or modified global stratosphere
Daniel M. Murphy, Karl D. Froyd, Ilann Bourgeois, Charles A. Brock, Agnieszka Kupc, Jeff Peischl, Gregory P. Schill, Chelsea R. Thompson, Christina J. Williamson, and Pengfei Yu
Atmos. Chem. Phys., 21, 8915–8932, https://doi.org/10.5194/acp-21-8915-2021,https://doi.org/10.5194/acp-21-8915-2021, 2021
Short summary
The potential role of organics in new particle formation and initial growth in the remote tropical upper troposphere
Agnieszka Kupc, Christina J. Williamson, Anna L. Hodshire, Jan Kazil, Eric Ray, T. Paul Bui, Maximilian Dollner, Karl D. Froyd, Kathryn McKain, Andrew Rollins, Gregory P. Schill, Alexander Thames, Bernadett B. Weinzierl, Jeffrey R. Pierce, and Charles A. Brock
Atmos. Chem. Phys., 20, 15037–15060, https://doi.org/10.5194/acp-20-15037-2020,https://doi.org/10.5194/acp-20-15037-2020, 2020
Short summary
Characterization of organic aerosol across the global remote troposphere: a comparison of ATom measurements and global chemistry models
Alma Hodzic, Pedro Campuzano-Jost, Huisheng Bian, Mian Chin, Peter R. Colarco, Douglas A. Day, Karl D. Froyd, Bernd Heinold, Duseong S. Jo, Joseph M. Katich, John K. Kodros, Benjamin A. Nault, Jeffrey R. Pierce, Eric Ray, Jacob Schacht, Gregory P. Schill, Jason C. Schroder, Joshua P. Schwarz, Donna T. Sueper, Ina Tegen, Simone Tilmes, Kostas Tsigaridis, Pengfei Yu, and Jose L. Jimenez
Atmos. Chem. Phys., 20, 4607–4635, https://doi.org/10.5194/acp-20-4607-2020,https://doi.org/10.5194/acp-20-4607-2020, 2020
Short summary

Related subject area

Subject: Aerosols | Research Activity: Laboratory Studies | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The effect of (NH4)2SO4 on the freezing properties of non-mineral dust ice-nucleating substances of atmospheric relevance
Soleil E. Worthy, Anand Kumar, Yu Xi, Jingwei Yun, Jessie Chen, Cuishan Xu, Victoria E. Irish, Pierre Amato, and Allan K. Bertram
Atmos. Chem. Phys., 21, 14631–14648, https://doi.org/10.5194/acp-21-14631-2021,https://doi.org/10.5194/acp-21-14631-2021, 2021
Short summary
Heterogeneous ice nucleation ability of aerosol particles generated from Arctic sea surface microlayer and surface seawater samples at cirrus temperatures
Robert Wagner, Luisa Ickes, Allan K. Bertram, Nora Els, Elena Gorokhova, Ottmar Möhler, Benjamin J. Murray, Nsikanabasi Silas Umo, and Matthew E. Salter
Atmos. Chem. Phys., 21, 13903–13930, https://doi.org/10.5194/acp-21-13903-2021,https://doi.org/10.5194/acp-21-13903-2021, 2021
Short summary
Aerosol formation and growth rates from chamber experiments using Kalman smoothing
Matthew Ozon, Dominik Stolzenburg, Lubna Dada, Aku Seppänen, and Kari E. J. Lehtinen
Atmos. Chem. Phys., 21, 12595–12611, https://doi.org/10.5194/acp-21-12595-2021,https://doi.org/10.5194/acp-21-12595-2021, 2021
Short summary
Phase state of secondary organic aerosol in chamber photo-oxidation of mixed precursors
Yu Wang, Aristeidis Voliotis, Yunqi Shao, Taomou Zong, Xiangxinyue Meng, Mao Du, Dawei Hu, Ying Chen, Zhijun Wu, M. Rami Alfarra, and Gordon McFiggans
Atmos. Chem. Phys., 21, 11303–11316, https://doi.org/10.5194/acp-21-11303-2021,https://doi.org/10.5194/acp-21-11303-2021, 2021
Short summary
Ice nucleation on surrogates of boreal forest SOA particles: effect of water content and oxidative age
Ana A. Piedehierro, André Welti, Angela Buchholz, Kimmo Korhonen, Iida Pullinen, Ilkka Summanen, Annele Virtanen, and Ari Laaksonen
Atmos. Chem. Phys., 21, 11069–11078, https://doi.org/10.5194/acp-21-11069-2021,https://doi.org/10.5194/acp-21-11069-2021, 2021
Short summary

Cited articles

Abbatt, J. P. D., Benz, S., Cziczo, D. J., Kanji, Z., Lohmann, U., and Möhler, O.: Solid ammonium sulfate aerosols as ice nuclei: A pathway for cirrus cloud formation, Science, 313, 1770–1773, https://doi.org/10.1126/science.1129726, 2006.
Baustian, K. J., Wise, M. E., and Tolbert, M. A.: Depositional ice nucleation on solid ammonium sulfate and glutaric acid particles, Atmos. Chem. Phys., 10, 2307–2317, https://doi.org/10.5194/acp-10-2307-2010, 2010.
Baustian, K. J., Cziczo, D. J., Wise, M. E., Pratt, K. A., Kulkarni, G., Hallar, A. G., and Tolbert, M. A.: Importance of aerosol composition, mixing state, and morphology for heterogeneous ice nucleation: A combined field and laboratory approach, J. Geophys. Res., 117, D06217, https://doi.org/10.1029/2011jd016784, 2012a.
Baustian, K. J., Wise, M. E., Jensen, E. J., Schill, G. P., Freedman, M. A., and Tolbert, M. A.: State transformations and ice nucleation in glassy or (semi-)solid amorphous organic aerosol, Atmos. Chem. Phys. Discuss., 12, 27333-27366, https://doi.org/10.5194/acpd-12-27333-2012, 2012b.
Download
Altmetrics
Final-revised paper
Preprint