Articles | Volume 23, issue 17
https://doi.org/10.5194/acp-23-10137-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-23-10137-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Surface ozone over the Tibetan Plateau controlled by stratospheric intrusion
Xiufeng Yin
State Key Laboratory of Cryospheric Science, Northwest Institute of
Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000,
China
University of Chinese Academy of Sciences, Beijing 100049, China
Dipesh Rupakheti
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and
Pollution Control, Collaborative Innovation Center of Atmospheric
Environment and Equipment Technology, School of Environmental Science and
Engineering, Nanjing University of Information Science and Technology,
Nanjing 210044, China
Guoshuai Zhang
Chinese Academy of Environmental Planning, Beijing 100012, China
Jiali Luo
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou
730000, China
Shichang Kang
State Key Laboratory of Cryospheric Science, Northwest Institute of
Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000,
China
University of Chinese Academy of Sciences, Beijing 100049, China
Benjamin de Foy
Department of Earth and Atmospheric Sciences, Saint Louis
University, St. Louis, MO 63108, USA
Junhua Yang
State Key Laboratory of Cryospheric Science, Northwest Institute of
Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000,
China
Zhenming Ji
School of Atmospheric Sciences, Key Laboratory for Climate Change
and Natural Disaster Studies of and Guangdong Province, Sun Yat-sen
University, Guangzhou 510275, China
Zhiyuan Cong
State Key Laboratory of Tibetan Plateau Earth System, Environment
and Resources (TPESER), Institute of Tibetan Plateau Research, Chinese
Academy of Sciences, Beijing 100101, China
Maheswar Rupakheti
Research Institute for Sustainability – Helmholtz Centre Potsdam (RIFS), 14467 Potsdam, Germany
Ping Li
University of Chinese Academy of Sciences, Beijing 100049, China
Key Laboratory of Land Surface Process and Climate Change in Cold
and Arid Regions, Northwest Institute of Eco-Environment and Resources,
Chinese Academy of Sciences, Lanzhou 730000, China
Yuling Hu
CORRESPONDING AUTHOR
Key Laboratory of Land Surface Process and Climate Change in Cold
and Arid Regions, Northwest Institute of Eco-Environment and Resources,
Chinese Academy of Sciences, Lanzhou 730000, China
Qianggong Zhang
CORRESPONDING AUTHOR
State Key Laboratory of Tibetan Plateau Earth System, Environment
and Resources (TPESER), Institute of Tibetan Plateau Research, Chinese
Academy of Sciences, Beijing 100101, China
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Sulfate aerosols play an important climatic role and exert adverse effects on the ecological environment and human health. In this study, we present the triple oxygen isotopic composition of sulfate from the Mt. Everest region, southern Tibetan Plateau, and decipher the formation mechanisms of atmospheric sulfate in this pristine environment. The results indicate the important role of the S(IV) + O3 pathway in atmospheric sulfate formation promoted by conditions of high cloud water pH.
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The occurrence frequency of different aerosol types and aerosol optical depth over the Arctic, Antarctic and Tibetan Plateau (TP) show distinctive spatiotemporal differences. The aerosol extinction coefficient in the Arctic and TP has a broad vertical distribution, while that of the Antarctic has obvious seasonal differences. Compared with the Antarctic, the Arctic and TP are vulnerable to surrounding pollutants, and the source of air masses has obvious seasonal variations.
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Short summary
The monthly mean surface ozone concentrations peaked earlier in the south in April and May and later in the north in June and July over the Tibetan Plateau. The migration of monthly surface ozone peaks was coupled with the synchronous movement of tropopause folds and the westerly jet that created conditions conducive to stratospheric ozone intrusion. Stratospheric ozone intrusion significantly contributed to surface ozone across the Tibetan Plateau.
The monthly mean surface ozone concentrations peaked earlier in the south in April and May and...
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