Preprints
https://doi.org/10.5194/acp-2022-199
https://doi.org/10.5194/acp-2022-199
 
11 Apr 2022
11 Apr 2022
Status: this preprint is currently under review for the journal ACP.

Insight into seasonal aerosol concentrations, meteorological influence, and transport over the Pan-Third Pole region using multi-sensors satellite and model simulation

Mukesh Rai1,2, Shichang Kang1,2, Junhua Yang1, Maheswar Rupakheti4, Dipesh Rupakheti3, Lekhendra Tripathee1, Yuling Hu1, and Xintong Chen1,2 Mukesh Rai et al.
  • 1State Key Laboratory of Cryospheric Science, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
  • 2University of Chinese Academy of Sciences, Beijing 100049, China
  • 3Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China
  • 4Institute for Advanced Sustainability Studies, Potsdam, Germany

Abstract. The Pan-Third Pole (PTP) owns complex geography and demographic features where aerosol roles and their impact cannot be neglected as it jeopardizes both the environment and human health. Therefore, we analyzed spatio-temporal aerosol concentration, the influence of meteorological conditions, and underlying aerosol transport mechanisms over the PTP by leveraging observation, satellite dataset, and model outputs. The observation and model simulation result showed that aerosol concentrations exceeded the world health organization (WHO) and China guideline values in most of the locations. This study revealed distinctive seasonality with the highest and lowest aerosol concentrations during the winter and summer seasons, respectively, which could be favored by meteorological conditions and emissions from biomass burning. In response to higher aerosol concentrations, the maximum aerosol optical depth (AOD) values were observed over the major hotspot regions however, interestingly summer high (AOD > 0.8) was observed over the Indo Gangetic Plain (IGP) in South Asia. The columnar aerosol profile indicated that the higher aerosol concentrations were limited within 1–2 km elevation over the densely populated regions over South Asia and Eastern China. However, the significant aerosols concentrations found to be extended as high as 10 km could potentially be driven by the deep convection process and summer monsoon activities. Regionally, the integrated aerosol transport (IAT) for black carbon (BC) and organic carbon (OC) was found to be maximum over SA. Noticeable OC IAT anomaly (~5 times > annual mean) found during spring that was linked with the biomass burning events. Yet, the dust transportation was found to be originated from the arid land and deserts that prolonged especially during summer followed by spring seasons. This study highlights the driver mechanism in aerosol seasonality, transport mechanism, and further motivates the additional assessment into potential dynamic relation between aerosol species, aerosol atmospheric river, and its societal impact.

Mukesh Rai et al.

Status: final response (author comments only)

Comment types: AC – author | RC – referee | CC – community | EC – editor | CEC – chief editor | : Report abuse
  • RC1: 'Comment on acp-2022-199', Anonymous Referee #1, 05 Jun 2022
  • RC2: 'Comment on acp-2022-199', Anonymous Referee #2, 12 Jun 2022

Mukesh Rai et al.

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Short summary
Our study revealed distinctive seasonality with the maximum and minimum aerosol concentrations during the winter and summer seasons respectively. However, interestingly summer high (AOD > 0.8) was observed over South Asia. The highest aerosols are laden over South Asia and East China within 1–2 km, however, aerosol overshooting found up to 10 km due to the deep convection process. Whereas, integrated aerosol transport for OC during spring was found to be 5 times higher than the annual mean.
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