Articles | Volume 23, issue 17
https://doi.org/10.5194/acp-23-10035-2023
https://doi.org/10.5194/acp-23-10035-2023
Research article
 | 
08 Sep 2023
Research article |  | 08 Sep 2023

Constraining the budget of atmospheric carbonyl sulfide using a 3-D chemical transport model

Michael P. Cartwright, Richard J. Pope, Jeremy J. Harrison, Martyn P. Chipperfield, Chris Wilson, Wuhu Feng, David P. Moore, and Parvadha Suntharalingam

Related authors

The Impact of the Stratospheric Quasi-Biennial Oscillation on Arctic Polar Stratospheric Cloud Occurrence
Douwang Li, Zhe Wang, Siyi Zhao, Jiankai Zhang, Wuhu Feng, and Martyn P. Chipperfield
EGUsphere, https://doi.org/10.5194/egusphere-2025-955,https://doi.org/10.5194/egusphere-2025-955, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Digitization and calibration of historical solar absorption infrared spectra from the Jungfraujoch site
Jamal Makkor, Mathias Palm, Matthias Buschmann, Emmanuel Mahieu, Martyn P. Chipperfield, and Justus Notholt
Atmos. Meas. Tech., 18, 1105–1114, https://doi.org/10.5194/amt-18-1105-2025,https://doi.org/10.5194/amt-18-1105-2025, 2025
Short summary
Performance evaluation of Atmotube PRO sensors for air quality measurements in an urban location
Aishah I. Shittu, Kirsty J. Pringle, Stephen R. Arnold, Richard J. Pope, Ailish M. Graham, Carly Reddington, Richard Rigby, and James B. McQuaid
Atmos. Meas. Tech., 18, 817–828, https://doi.org/10.5194/amt-18-817-2025,https://doi.org/10.5194/amt-18-817-2025, 2025
Short summary
Biosphere-atmosphere related processes influence trace-gas and aerosol satellite-model biases
Emma Sands, Ruth M. Doherty, Fiona M. O'Connor, Richard J. Pope, James Weber, and Daniel P. Grosvenor
EGUsphere, https://doi.org/10.5194/egusphere-2024-4014,https://doi.org/10.5194/egusphere-2024-4014, 2025
Short summary
Impact of host climate model on contrail cirrus effective radiative forcing estimates
Weiyu Zhang, Kwinten Van Weverberg, Cyril J. Morcrette, Wuhu Feng, Kalli Furtado, Paul R. Field, Chih-Chieh Chen, Andrew Gettelman, Piers M. Forster, Daniel R. Marsh, and Alexandru Rap
Atmos. Chem. Phys., 25, 473–489, https://doi.org/10.5194/acp-25-473-2025,https://doi.org/10.5194/acp-25-473-2025, 2025
Short summary

Related subject area

Subject: Gases | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Estimating the variability in NOx emissions from Wuhan with TROPOMI NO2 data during 2018 to 2023
Qianqian Zhang, K. Folkert Boersma, Chiel van der Laan, Alba Mols, Bin Zhao, Shengyue Li, and Yuepeng Pan
Atmos. Chem. Phys., 25, 3313–3326, https://doi.org/10.5194/acp-25-3313-2025,https://doi.org/10.5194/acp-25-3313-2025, 2025
Short summary
Enhanced understanding of atmospheric blocking modulation on ozone dynamics within a high-resolution Earth system model
Wenbin Kou, Yang Gao, Dan Tong, Xiaojie Guo, Xiadong An, Wenyu Liu, Mengshi Cui, Xiuwen Guo, Shaoqing Zhang, Huiwang Gao, and Lixin Wu
Atmos. Chem. Phys., 25, 3029–3048, https://doi.org/10.5194/acp-25-3029-2025,https://doi.org/10.5194/acp-25-3029-2025, 2025
Short summary
Natural emissions of VOC and NOx over Africa constrained by TROPOMI HCHO and NO2 data using the MAGRITTEv1.1 model
Beata Opacka, Trissevgeni Stavrakou, Jean-François Müller, Isabelle De Smedt, Jos van Geffen, Eloise A. Marais, Rebekah P. Horner, Dylan B. Millet, Kelly C. Wells, and Alex B. Guenther
Atmos. Chem. Phys., 25, 2863–2894, https://doi.org/10.5194/acp-25-2863-2025,https://doi.org/10.5194/acp-25-2863-2025, 2025
Short summary
Anthropogenic emission controls reduce summertime ozone–temperature sensitivity in the United States
Shuai Li, Haolin Wang, and Xiao Lu
Atmos. Chem. Phys., 25, 2725–2743, https://doi.org/10.5194/acp-25-2725-2025,https://doi.org/10.5194/acp-25-2725-2025, 2025
Short summary
Investigating the response of China's surface ozone concentration to the future changes of multiple factors
Jinya Yang, Yutong Wang, Lei Zhang, and Yu Zhao
Atmos. Chem. Phys., 25, 2649–2666, https://doi.org/10.5194/acp-25-2649-2025,https://doi.org/10.5194/acp-25-2649-2025, 2025
Short summary

Cited articles

ACE-FTS: ACE-FTS Data, University of Waterloo [data set], http://www.ace.uwaterloo.ca/data.php, last access: 14 March 2022. 
Asaf, D., Rotenberg, E., Tatarinov, F., Dicken, U., Montzka, S. A., and Yakir, D.: Ecosystem photosynthesis inferred from measurements of carbonyl sulphide flux, Nat. Geosci., 6, 186–190, https://doi.org/10.1038/ngeo1730, 2013. 
Aydin, M., Britten, G. L., Montzka, S. A., Buizert, C., Primeau, F., Petrenko, V., Battle, M. B., Nicewonger, M. R., Patterson, J., Hmiel, B., and Saltzman, E. S.: Anthropogenic Impacts on Atmospheric Carbonyl Sulfide Since the 19th Century Inferred From Polar Firn Air and Ice Core Measurements, J. Geophys. Res.-Atmos., 125, e2020JD033074, https://doi.org/10.1029/2020JD033074, 2020. 
Barkley, M. P., Palmer, P. I., Boone, C. D., Bernath, P. F., and Suntharalingam, P.: Global distributions of carbonyl sulfide in the upper troposphere and stratosphere, Geophys. Res. Lett., 35, L14810, https://doi.org/10.1029/2008GL034270, 2008. 
Download
Short summary
A 3-D chemical transport model, TOMCAT, is used to simulate global atmospheric carbonyl sulfide (OCS) distribution. Modelled OCS compares well with satellite observations of OCS from limb-sounding satellite observations. Model simulations also compare adequately with surface and atmospheric observations and suitably capture the seasonality of OCS and background concentrations.
Share
Altmetrics
Final-revised paper
Preprint