Articles | Volume 22, issue 23
https://doi.org/10.5194/acp-22-15207-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-15207-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Aerosol–cloud interaction in the atmospheric chemistry model GRAPES_Meso5.1/CUACE and its impacts on mesoscale numerical weather prediction under haze pollution conditions in Jing–Jin–Ji in China
Wenjie Zhang
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing, China
Department of Atmospheric and Oceanic Sciences & Institute of
Atmospheric Sciences, Fudan University, Shanghai, China
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing, China
Xiaoye Zhang
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing, China
Liping Huang
Earth System Modeling and Prediction Center, China Meteorological
Administration, Beijing, China
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing, China
Zhaodong Liu
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing, China
Xiao Zhang
Department of Atmospheric Sciences, Yunnan University, Kunming, China
Huizheng Che
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing, China
Related authors
Wenjie Zhang, Hong Wang, Xiaoye Zhang, Yue Peng, Zhaodong Liu, Deying Wang, Da Zhang, Chen Han, Yang Zhao, Junting Zhong, Wenxing Jia, Huiqiong Ning, and Huizheng Che
Atmos. Chem. Phys., 25, 9005–9030, https://doi.org/10.5194/acp-25-9005-2025, https://doi.org/10.5194/acp-25-9005-2025, 2025
Short summary
Short summary
This study achieves quantifiable subgrid-scale aerosol–cloud interaction in an atmospheric chemistry system, with better performance in terms of meteorology prediction, and further finds that subgrid-scale actual aerosol can somewhat improve overestimated cumulative precipitation during a typical heavy rainfall event, which helps us better understand the impact of subgrid-scale aerosol–cloud interaction on weather forecasts.
Wenxing Jia, Xiaoye Zhang, Hong Wang, Yaqiang Wang, Deying Wang, Junting Zhong, Wenjie Zhang, Lei Zhang, Lifeng Guo, Yadong Lei, Jizhi Wang, Yuanqin Yang, and Yi Lin
Geosci. Model Dev., 16, 6833–6856, https://doi.org/10.5194/gmd-16-6833-2023, https://doi.org/10.5194/gmd-16-6833-2023, 2023
Short summary
Short summary
In addition to the dominant role of the PBL scheme on the results of the meteorological field, many factors in the model are influenced by large uncertainties. This study focuses on the uncertainties that influence numerical simulation results (including horizontal resolution, vertical resolution, near-surface scheme, initial and boundary conditions, underlying surface update, and update of model version), hoping to provide a reference for scholars conducting research on the model.
Wenxing Jia, Xiaoye Zhang, Hong Wang, Yaqiang Wang, Deying Wang, Junting Zhong, Wenjie Zhang, Lei Zhang, Lifeng Guo, Yadong Lei, Jizhi Wang, Yuanqin Yang, and Yi Lin
Geosci. Model Dev., 16, 6635–6670, https://doi.org/10.5194/gmd-16-6635-2023, https://doi.org/10.5194/gmd-16-6635-2023, 2023
Short summary
Short summary
Most current studies on planetary boundary layer (PBL) parameterization schemes are relatively fragmented and lack systematic in-depth analysis and discussion. In this study, we comprehensively evaluate the performance capability of the PBL scheme in five typical regions of China in different seasons from the mechanism of the scheme and the effects of PBL schemes on the near-surface meteorological parameters, vertical structures of the PBL, PBL height, and turbulent diffusion.
Yue Peng, Hong Wang, Xiaoye Zhang, Zhaodong Liu, Wenjie Zhang, Siting Li, Chen Han, and Huizheng Che
Atmos. Chem. Phys., 23, 8325–8339, https://doi.org/10.5194/acp-23-8325-2023, https://doi.org/10.5194/acp-23-8325-2023, 2023
Short summary
Short summary
This study demonstrates a strong link between local circulation, aerosol–radiation interaction (ARI), and haze pollution. Under the weak weather-scale systems, the typical local circulation driven by mountainous topography is the main cause of pollutant distribution in the Beijing–Tianjin–Hebei region, and the ARI mechanism amplifies this influence of local circulation on pollutants, making haze pollution aggravated by the superposition of both.
Siting Li, Ping Wang, Hong Wang, Yue Peng, Zhaodong Liu, Wenjie Zhang, Hongli Liu, Yaqiang Wang, Huizheng Che, and Xiaoye Zhang
Geosci. Model Dev., 16, 4171–4191, https://doi.org/10.5194/gmd-16-4171-2023, https://doi.org/10.5194/gmd-16-4171-2023, 2023
Short summary
Short summary
Optimizing the initial state of atmospheric chemistry model input is one of the most essential methods to improve forecast accuracy. Considering the large computational load of the model, we introduce an ensemble optimal interpolation scheme (EnOI) for operational use and efficient updating of the initial fields of chemical components. The results suggest that EnOI provides a practical and cost-effective technique for improving the accuracy of chemical weather numerical forecasts.
Xinyao Hu, Aoyuan Yu, Xiaojing Shen, Jiayuan Lu, Yangmei Zhang, Quan Liu, Lei Liu, Linlin Liang, Hongfei Tong, Qianli Ma, Shuxian Zhang, Bing Qi, Rongguang Du, Huizheng Che, Xiaoye Zhang, and Junying Sun
EGUsphere, https://doi.org/10.5194/egusphere-2025-3796, https://doi.org/10.5194/egusphere-2025-3796, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Simultaneous measurements of aerosol hygroscopicity and volatility were performed using Volatility-Hygroscopicity Tandem Differential Mobility Analyzer in Beijing. The results reveal that hygroscopicity and volatility of accumulated mode particles are significantly influenced by dust. The size dependences of hygroscopicity and volatility during dust period were different from that before dust period. During dust period, the particles at 300 nm were hydrophobic and less volatile.
Wenjie Zhang, Hong Wang, Xiaoye Zhang, Yue Peng, Zhaodong Liu, Deying Wang, Da Zhang, Chen Han, Yang Zhao, Junting Zhong, Wenxing Jia, Huiqiong Ning, and Huizheng Che
Atmos. Chem. Phys., 25, 9005–9030, https://doi.org/10.5194/acp-25-9005-2025, https://doi.org/10.5194/acp-25-9005-2025, 2025
Short summary
Short summary
This study achieves quantifiable subgrid-scale aerosol–cloud interaction in an atmospheric chemistry system, with better performance in terms of meteorology prediction, and further finds that subgrid-scale actual aerosol can somewhat improve overestimated cumulative precipitation during a typical heavy rainfall event, which helps us better understand the impact of subgrid-scale aerosol–cloud interaction on weather forecasts.
Yongzhu Liu, Xiaoye Zhang, Wei Han, Chao Wang, Wenxing Jia, Deying Wang, Zhaorong Zhuang, and Xueshun Shen
Geosci. Model Dev., 18, 4855–4876, https://doi.org/10.5194/gmd-18-4855-2025, https://doi.org/10.5194/gmd-18-4855-2025, 2025
Short summary
Short summary
In order to investigate the feedbacks of chemical data assimilation on meteorological forecasts, we developed a strongly coupled aerosol–meteorology four-dimensional variational (4D-Var) assimilation system, CMA-GFS-AERO 4D-Var, based on the framework of the incremental analysis scheme of the China Meteorological Administration Global Forecasting System (CMA-GFS) operational global numerical weather model. The results show that assimilating BC (black carbon) observations can generate analysis increments not only for BC but also for atmospheric variables.
Xiaojing Shen, Quan Liu, Junying Sun, Wanlin Kong, Qianli Ma, Bing Qi, Lujie Han, Yangmei Zhang, Linlin Liang, Lei Liu, Shuo Liu, Xinyao Hu, Jiayuan Lu, Aoyuan Yu, Huizheng Che, and Xiaoye Zhang
Atmos. Chem. Phys., 25, 5711–5725, https://doi.org/10.5194/acp-25-5711-2025, https://doi.org/10.5194/acp-25-5711-2025, 2025
Short summary
Short summary
In this work, an automatic switched inlet system was developed and employed to investigate the aerosols and cloud droplets at a mountain site with frequent cloud processes. It showed different characteristics of cloud residual and interstitial particles. Stronger particle hygroscopicity reduced liquid water content and smaller cloud droplet diameters. This investigation contributes to understanding aerosol–cloud interactions by assessing the impact of aerosol particles on cloud microphysics.
Zhenyu Zhang, Jing Li, Huizheng Che, Yueming Dong, Oleg Dubovik, Thomas Eck, Pawan Gupta, Brent Holben, Jhoon Kim, Elena Lind, Trailokya Saud, Sachchida Nand Tripathi, and Tong Ying
Atmos. Chem. Phys., 25, 4617–4637, https://doi.org/10.5194/acp-25-4617-2025, https://doi.org/10.5194/acp-25-4617-2025, 2025
Short summary
Short summary
We used ground-based remote sensing data from the Aerosol Robotic Network to examine long-term trends in aerosol characteristics. We found aerosol loadings generally decreased globally, and aerosols became more scattering. These changes are closely related to variations in aerosol compositions, such as decreased anthropogenic emissions over East Asia, Europe, and North America; increased anthropogenic sources over northern India; and increased dust activity over the Arabian Peninsula.
Aoyuan Yu, Xiaojing Shen, Qianli Ma, Jiayuan Lu, Xinyao Hu, Yangmei Zhang, Quan Liu, Linlin Liang, Lei Liu, Shuo Liu, Hongfei Tong, Huizheng Che, Xiaoye Zhang, and Junying Sun
Atmos. Chem. Phys., 25, 3389–3412, https://doi.org/10.5194/acp-25-3389-2025, https://doi.org/10.5194/acp-25-3389-2025, 2025
Short summary
Short summary
In this work, we utilized a volatility hygroscopicity tandem differential mobility analyzer (VH-TDMA) to investigate, for the first time, the hygroscopicity and volatility of submicron aerosols, as well as their hygroscopicity after heating, in urban Beijing during the autumn of 2023. We analyzed the size-resolved characteristics of hygroscopicity and volatility, the relationship between hygroscopic and volatile properties, and the hygroscopicity of heated submicron aerosols.
Quan Liu, Xiaojing Shen, Junying Sun, Yangmei Zhang, Bing Qi, Qianli Ma, Lujie Han, Honghui Xu, Xinyao Hu, Jiayuan Lu, Shuo Liu, Aoyuan Yu, Linlin Liang, Qian Gao, Hong Wang, Huizheng Che, and Xiaoye Zhang
Atmos. Chem. Phys., 25, 3253–3267, https://doi.org/10.5194/acp-25-3253-2025, https://doi.org/10.5194/acp-25-3253-2025, 2025
Short summary
Short summary
Through simultaneous measurements of aerosol particles and fog droplets, the evolution of droplets size distribution during the eight observed fog events was investigated. The results showed that the concentration and size distribution of pre-fog aerosol had significant impacts on fog microphysical characteristics. The extinction of fog interstitial particles played an important role in visibility degradation for light fogs, especially in polluted regions.
Lijing Chen, Lei Zhang, Yong She, Zhaoliang Zeng, Yu Zheng, Biao Tian, Wenqian Zhang, Zhaohui Liu, Huizheng Che, and Minghu Ding
Atmos. Chem. Phys., 25, 727–739, https://doi.org/10.5194/acp-25-727-2025, https://doi.org/10.5194/acp-25-727-2025, 2025
Short summary
Short summary
Aerosol optical depth (AOD) at Zhongshan Station varies seasonally, with lower values in summer and higher values in winter. Winter and spring AOD increases due to reduced fine-mode particles, while summer and autumn increases are linked to particle growth. Diurnal AOD variation correlates positively with temperature but negatively with wind speed and humidity. Backward trajectories show that aerosols on high-AOD (low-AOD) days primarily originate from the ocean (interior Antarctica).
Xuan Wang, Lei Bi, Hong Wang, Yaqiang Wang, Wei Han, Xueshun Shen, and Xiaoye Zhang
Geosci. Model Dev., 18, 117–139, https://doi.org/10.5194/gmd-18-117-2025, https://doi.org/10.5194/gmd-18-117-2025, 2025
Short summary
Short summary
The Artificial-Intelligence-based Nonspherical Aerosol Optical Scheme (AI-NAOS) was developed to improve the estimation of the aerosol direct radiation effect and was coupled online with a chemical weather model. The AI-NAOS scheme considers black carbon as fractal aggregates and soil dust as super-spheroids, encapsulated with hygroscopic aerosols. Real-case simulations emphasize the necessity of accurately representing nonspherical and inhomogeneous aerosols in chemical weather models.
Wenxin Zhao, Yu Zhao, Yu Zheng, Dong Chen, Jinyuan Xin, Kaitao Li, Huizheng Che, Zhengqiang Li, Mingrui Ma, and Yun Hang
Atmos. Chem. Phys., 24, 6593–6612, https://doi.org/10.5194/acp-24-6593-2024, https://doi.org/10.5194/acp-24-6593-2024, 2024
Short summary
Short summary
We evaluate the long-term (2000–2020) variabilities of aerosol absorption optical depth, black carbon emissions, and associated health risks in China with an integrated framework that combines multiple observations and modeling techniques. We demonstrate the remarkable emission abatement resulting from the implementation of national pollution controls and show how human activities affected the emissions with a spatiotemporal heterogeneity, thus supporting differentiated policy-making by region.
Wenxing Jia, Xiaoye Zhang, Hong Wang, Yaqiang Wang, Deying Wang, Junting Zhong, Wenjie Zhang, Lei Zhang, Lifeng Guo, Yadong Lei, Jizhi Wang, Yuanqin Yang, and Yi Lin
Geosci. Model Dev., 16, 6833–6856, https://doi.org/10.5194/gmd-16-6833-2023, https://doi.org/10.5194/gmd-16-6833-2023, 2023
Short summary
Short summary
In addition to the dominant role of the PBL scheme on the results of the meteorological field, many factors in the model are influenced by large uncertainties. This study focuses on the uncertainties that influence numerical simulation results (including horizontal resolution, vertical resolution, near-surface scheme, initial and boundary conditions, underlying surface update, and update of model version), hoping to provide a reference for scholars conducting research on the model.
Wenxing Jia, Xiaoye Zhang, Hong Wang, Yaqiang Wang, Deying Wang, Junting Zhong, Wenjie Zhang, Lei Zhang, Lifeng Guo, Yadong Lei, Jizhi Wang, Yuanqin Yang, and Yi Lin
Geosci. Model Dev., 16, 6635–6670, https://doi.org/10.5194/gmd-16-6635-2023, https://doi.org/10.5194/gmd-16-6635-2023, 2023
Short summary
Short summary
Most current studies on planetary boundary layer (PBL) parameterization schemes are relatively fragmented and lack systematic in-depth analysis and discussion. In this study, we comprehensively evaluate the performance capability of the PBL scheme in five typical regions of China in different seasons from the mechanism of the scheme and the effects of PBL schemes on the near-surface meteorological parameters, vertical structures of the PBL, PBL height, and turbulent diffusion.
Yue Peng, Hong Wang, Xiaoye Zhang, Zhaodong Liu, Wenjie Zhang, Siting Li, Chen Han, and Huizheng Che
Atmos. Chem. Phys., 23, 8325–8339, https://doi.org/10.5194/acp-23-8325-2023, https://doi.org/10.5194/acp-23-8325-2023, 2023
Short summary
Short summary
This study demonstrates a strong link between local circulation, aerosol–radiation interaction (ARI), and haze pollution. Under the weak weather-scale systems, the typical local circulation driven by mountainous topography is the main cause of pollutant distribution in the Beijing–Tianjin–Hebei region, and the ARI mechanism amplifies this influence of local circulation on pollutants, making haze pollution aggravated by the superposition of both.
Siting Li, Ping Wang, Hong Wang, Yue Peng, Zhaodong Liu, Wenjie Zhang, Hongli Liu, Yaqiang Wang, Huizheng Che, and Xiaoye Zhang
Geosci. Model Dev., 16, 4171–4191, https://doi.org/10.5194/gmd-16-4171-2023, https://doi.org/10.5194/gmd-16-4171-2023, 2023
Short summary
Short summary
Optimizing the initial state of atmospheric chemistry model input is one of the most essential methods to improve forecast accuracy. Considering the large computational load of the model, we introduce an ensemble optimal interpolation scheme (EnOI) for operational use and efficient updating of the initial fields of chemical components. The results suggest that EnOI provides a practical and cost-effective technique for improving the accuracy of chemical weather numerical forecasts.
Xiaojing Shen, Junying Sun, Huizheng Che, Yangmei Zhang, Chunhong Zhou, Ke Gui, Wanyun Xu, Quan Liu, Junting Zhong, Can Xia, Xinyao Hu, Sinan Zhang, Jialing Wang, Shuo Liu, Jiayuan Lu, Aoyuan Yu, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 8241–8257, https://doi.org/10.5194/acp-23-8241-2023, https://doi.org/10.5194/acp-23-8241-2023, 2023
Short summary
Short summary
New particle formation (NPF) events occur when the dust episodes' fade is analysed based on long-term measurement of particle number size distribution. Analysis shows that the observed formation and growth rates are approximately 50 % of and 30 % lower than those of other NPF events. As a consequence of the uptake of precursor gases on mineral dust, the physical and chemical properties of submicron particles, as well as the ability to be cloud condensation nuclei, can be changed.
Xinyao Hu, Junying Sun, Can Xia, Xiaojing Shen, Yangmei Zhang, Quan Liu, Zhaodong Liu, Sinan Zhang, Jialing Wang, Aoyuan Yu, Jiayuan Lu, Shuo Liu, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 5517–5531, https://doi.org/10.5194/acp-23-5517-2023, https://doi.org/10.5194/acp-23-5517-2023, 2023
Short summary
Short summary
The simultaneous measurements under dry conditions of aerosol optical properties were conducted at three wavelengths for PM1 and PM10 in urban Beijing from 2018 to 2021. Considerable reductions in aerosol absorption coefficient and increased single scattering albedo demonstrated that absorbing aerosols were more effectively controlled than scattering aerosols due to pollution control measures. The aerosol radiative effect and the transport's impact on aerosol optical properties were analysed.
Yingfang Li, Zhili Wang, Yadong Lei, Huizheng Che, and Xiaoye Zhang
Atmos. Chem. Phys., 23, 2499–2523, https://doi.org/10.5194/acp-23-2499-2023, https://doi.org/10.5194/acp-23-2499-2023, 2023
Short summary
Short summary
Since few studies have assessed the impacts of future combined reductions in aerosols, ozone, and their precursors on future climate change, we use models with an interactive representation of tropospheric aerosols and atmospheric chemistry schemes to quantify the impact of their reductions on the Asian climate. Our results suggest that their reductions will exacerbate the warming effect caused by greenhouse gases, increasing future climate extremes and associated population exposure risk.
Mengying Li, Shaocai Yu, Xue Chen, Zhen Li, Yibo Zhang, Zhe Song, Weiping Liu, Pengfei Li, Xiaoye Zhang, Meigen Zhang, Yele Sun, Zirui Liu, Caiping Sun, Jingkun Jiang, Shuxiao Wang, Benjamin N. Murphy, Kiran Alapaty, Rohit Mathur, Daniel Rosenfeld, and John H. Seinfeld
Atmos. Chem. Phys., 22, 11845–11866, https://doi.org/10.5194/acp-22-11845-2022, https://doi.org/10.5194/acp-22-11845-2022, 2022
Short summary
Short summary
This study constructed an emission inventory of condensable particulate matter (CPM) in China with a focus on organic aerosols (OAs), based on collected CPM emission information. The results show that OA emissions are enhanced twofold for the years 2014 and 2017 after the inclusion of CPM in the new inventory. Sensitivity cases demonstrated the significant contributions of CPM emissions from stationary combustion and mobile sources to primary, secondary, and total OA concentrations.
Lei Li, Yevgeny Derimian, Cheng Chen, Xindan Zhang, Huizheng Che, Gregory L. Schuster, David Fuertes, Pavel Litvinov, Tatyana Lapyonok, Anton Lopatin, Christian Matar, Fabrice Ducos, Yana Karol, Benjamin Torres, Ke Gui, Yu Zheng, Yuanxin Liang, Yadong Lei, Jibiao Zhu, Lei Zhang, Junting Zhong, Xiaoye Zhang, and Oleg Dubovik
Earth Syst. Sci. Data, 14, 3439–3469, https://doi.org/10.5194/essd-14-3439-2022, https://doi.org/10.5194/essd-14-3439-2022, 2022
Short summary
Short summary
A climatology of aerosol composition concentration derived from POLDER-3 observations using GRASP/Component is presented. The conceptual specifics of the GRASP/Component approach are in the direct retrieval of aerosol speciation without intermediate retrievals of aerosol optical characteristics. The dataset of satellite-derived components represents scarce but imperative information for validation and potential adjustment of chemical transport models.
Junting Zhong, Xiaoye Zhang, Ke Gui, Jie Liao, Ye Fei, Lipeng Jiang, Lifeng Guo, Liangke Liu, Huizheng Che, Yaqiang Wang, Deying Wang, and Zijiang Zhou
Earth Syst. Sci. Data, 14, 3197–3211, https://doi.org/10.5194/essd-14-3197-2022, https://doi.org/10.5194/essd-14-3197-2022, 2022
Short summary
Short summary
Historical long-term PM2.5 records with high temporal resolution are essential but lacking for research and environmental management. Here, we reconstruct site-based and gridded PM2.5 datasets at 6-hour intervals from 1960 to 2020 that combine visibility, meteorological data, and emissions based on a machine learning model with extracted spatial features. These two PM2.5 datasets will lay the foundation of research studies associated with air pollution, climate change, and aerosol reanalysis.
Haochi Che, Michal Segal-Rozenhaimer, Lu Zhang, Caroline Dang, Paquita Zuidema, Arthur J. Sedlacek III, Xiaoye Zhang, and Connor Flynn
Atmos. Chem. Phys., 22, 8767–8785, https://doi.org/10.5194/acp-22-8767-2022, https://doi.org/10.5194/acp-22-8767-2022, 2022
Short summary
Short summary
A 17-month in situ study on Ascension Island found low single-scattering albedo and strong absorption enhancement of the marine boundary layer aerosols during biomass burnings on the African continent, along with apparent patterns of regular monthly variability. We further discuss the characteristics and drivers behind these changes and find that biomass burning conditions in Africa may be the main factor influencing the optical properties of marine boundary aerosols.
Ke Gui, Wenrui Yao, Huizheng Che, Linchang An, Yu Zheng, Lei Li, Hujia Zhao, Lei Zhang, Junting Zhong, Yaqiang Wang, and Xiaoye Zhang
Atmos. Chem. Phys., 22, 7905–7932, https://doi.org/10.5194/acp-22-7905-2022, https://doi.org/10.5194/acp-22-7905-2022, 2022
Short summary
Short summary
This study investigates the aerosol optical and radiative properties and meteorological drivers during two mega SDS events over Northern China in March 2021. The MODIS-retrieved DOD data registered these two events as the most intense episode in the same period in history over the past 20 years. These two extreme SDS events were associated with both atmospheric circulation extremes and local meteorological anomalies that favor enhanced dust emissions in the Gobi Desert.
Yu Zheng, Huizheng Che, Yupeng Wang, Xiangao Xia, Xiuqing Hu, Xiaochun Zhang, Jun Zhu, Jibiao Zhu, Hujia Zhao, Lei Li, Ke Gui, and Xiaoye Zhang
Atmos. Meas. Tech., 15, 2139–2158, https://doi.org/10.5194/amt-15-2139-2022, https://doi.org/10.5194/amt-15-2139-2022, 2022
Short summary
Short summary
Ground-based observations of aerosols and aerosol data verification is important for satellite and climate model modification. Here we present an evaluation of aerosol microphysical, optical and radiative properties measured using a multiwavelength photometer with a highly integrated design and smart control performance. The validation of this product is discussed in detail using AERONET as a reference. This work contributes to reducing AOD uncertainties in China and combating climate change.
Wenxing Jia and Xiaoye Zhang
Atmos. Chem. Phys., 21, 16827–16841, https://doi.org/10.5194/acp-21-16827-2021, https://doi.org/10.5194/acp-21-16827-2021, 2021
Short summary
Short summary
Heavy aerosol pollution incidents have attracted much attention since 2013, but the temporal and spatial limitations of observations and the inaccuracy of simulation are a stumbling block to assessing pollution mechanisms. The correct simulation of boundary layer mixing process of pollutant is a challenge for mesoscale numerical models. We add the turbulent diffusion term of aerosol to the WRF-Chem model to prove the impact of turbulent diffusion on pollutant concentration.
Ke Gui, Huizheng Che, Yu Zheng, Hujia Zhao, Wenrui Yao, Lei Li, Lei Zhang, Hong Wang, Yaqiang Wang, and Xiaoye Zhang
Atmos. Chem. Phys., 21, 15309–15336, https://doi.org/10.5194/acp-21-15309-2021, https://doi.org/10.5194/acp-21-15309-2021, 2021
Short summary
Short summary
This study utilized the globally gridded aerosol extinction data from CALIOP during 2007–2019 to investigate the 3D climatology, trends, and meteorological drivers of tropospheric type-dependent aerosols. Results revealed that the planetary boundary layer (PBL) and the free troposphere contribute 62.08 % and 37.92 %, respectively, of the global tropospheric TAOD. Trends in
CALIOP-derived aerosol loading, in particular those partitioned in the PBL, can be explained to a large extent by meteorology.
Qingyang Xiao, Yixuan Zheng, Guannan Geng, Cuihong Chen, Xiaomeng Huang, Huizheng Che, Xiaoye Zhang, Kebin He, and Qiang Zhang
Atmos. Chem. Phys., 21, 9475–9496, https://doi.org/10.5194/acp-21-9475-2021, https://doi.org/10.5194/acp-21-9475-2021, 2021
Short summary
Short summary
We used both statistical methods and a chemical transport model to assess the contribution of meteorology and emissions to PM2.5 during 2000–2018. Both methods revealed that emissions dominated the long-term PM2.5 trend with notable meteorological effects ranged up to 37.9 % of regional annual average PM2.5. The meteorological contribution became more beneficial to PM2.5 control in southern China but more unfavorable in northern China during the studied period.
Xiaojing Shen, Junying Sun, Fangqun Yu, Ying Wang, Junting Zhong, Yangmei Zhang, Xinyao Hu, Can Xia, Sinan Zhang, and Xiaoye Zhang
Atmos. Chem. Phys., 21, 7039–7052, https://doi.org/10.5194/acp-21-7039-2021, https://doi.org/10.5194/acp-21-7039-2021, 2021
Short summary
Short summary
In this work, we revealed the changes of PNSD and NPF events during the COVID-19 lockdown period in Beijing, China, to illustrate the impact of reduced primary emission and elavated atmospheric oxidized capicity on the nucleation and growth processes. The subsequent growth of nucleated particles and their contribution to the aerosol pollution formation were also explored, to highlight the necessity of controlling the nanoparticles in the future air quality management.
Linlin Liang, Guenter Engling, Chang Liu, Wanyun Xu, Xuyan Liu, Yuan Cheng, Zhenyu Du, Gen Zhang, Junying Sun, and Xiaoye Zhang
Atmos. Chem. Phys., 21, 3181–3192, https://doi.org/10.5194/acp-21-3181-2021, https://doi.org/10.5194/acp-21-3181-2021, 2021
Short summary
Short summary
A unique episode with extreme biomass burning (BB) impact, with daily concentration of levoglucosan as high as 4.37 µg m-3, was captured at an area upwind of Beijing. How this extreme BB pollution event was generated and what were the chemical properties of PM2.5 under this kind severe BB pollution level in the real atmospheric environment were both presented in this measurement report. Moreover, the variation of the ratios of BB tracers during different BB pollution periods was also exhibited.
Lei Zhang, Sunling Gong, Tianliang Zhao, Chunhong Zhou, Yuesi Wang, Jiawei Li, Dongsheng Ji, Jianjun He, Hongli Liu, Ke Gui, Xiaomei Guo, Jinhui Gao, Yunpeng Shan, Hong Wang, Yaqiang Wang, Huizheng Che, and Xiaoye Zhang
Geosci. Model Dev., 14, 703–718, https://doi.org/10.5194/gmd-14-703-2021, https://doi.org/10.5194/gmd-14-703-2021, 2021
Short summary
Short summary
Development of chemical transport models with advanced physics and chemical schemes is important for improving air-quality forecasts. This study develops the chemical module CUACE by updating with a new particle dry deposition scheme and adding heterogenous chemical reactions and couples it with the WRF model. The coupled model (WRF/CUACE) was able to capture well the variations of PM2.5, O3, NO2, and secondary inorganic aerosols in eastern China.
Xiaoning Xie, Anmin Duan, Zhengguo Shi, Xinzhou Li, Hui Sun, Xiaodong Liu, Xugeng Cheng, Tianliang Zhao, Huizheng Che, and Yangang Liu
Atmos. Chem. Phys., 20, 11143–11159, https://doi.org/10.5194/acp-20-11143-2020, https://doi.org/10.5194/acp-20-11143-2020, 2020
Short summary
Short summary
Observational and modeling results both show that the surface dust concentrations over the East Asian (EA) dust source region and over the northwestern Pacific (NP) in MAM are significantly positively correlated with TPSH. These atmospheric circulation anomalies induced by the increased TPSH result in increasing westerly winds over both EA and NP, which in turn increases dust emissions over the dust source and dust transport over these two regions, as well as the regional dust cycles.
Cited articles
Albrecht, B.: Aerosols, Cloud Microphysics, and Fractional Cloudiness,
Science, 245, 1227–1230,
https://doi.org/10.1126/science.245.4923.1227, 1989.
Andreae, M. O. and Rosenfeld, D.: Aerosol–cloud–precipitation
interactions. Part 1. The nature and sources of cloud-active aerosols,
Earth-Sci. Rev., 89, 13–41,
https://doi.org/10.1016/j.earscirev.2008.03.001, 2008.
Bennartz, R.: Global assessment of marine boundary layer cloud droplet
number concentration from satellite, J. Geophys. Res.-Atmos., 112, D02201,
https://doi.org/10.1029/2006JD007547, 2007.
Borys, R. D., Lowenthal, D. H., and Mitchell, D. L.: The relationships among
cloud microphysics, chemistry, and precipitation rate in cold mountain
clouds, Atmos. Environ., 34, 2593–2602,
https://doi.org/10.1016/S1352-2310(99)00492-6, 2000.
Chang, D. Y., Lelieveld, J., Steil, B., Yoon, J., Yum, S. S., and Kim, A.
H.: Variability of aerosol-cloud interactions induced by different cloud
droplet nucleation schemes, Atmos. Res., 250, 105367,
https://doi.org/10.1016/j.atmosres.2020.105367, 2021.
Che, H., Zhang, X.-Y., Xia, X., Goloub, P., Holben, B., Zhao, H., Wang, Y., Zhang, X.-C., Wang, H., Blarel, L., Damiri, B., Zhang, R., Deng, X., Ma, Y., Wang, T., Geng, F., Qi, B., Zhu, J., Yu, J., Chen, Q., and Shi, G.: Ground-based aerosol climatology of China: aerosol optical depths from the China Aerosol Remote Sensing Network (CARSNET) 2002–2013, Atmos. Chem. Phys., 15, 7619–7652, https://doi.org/10.5194/acp-15-7619-2015, 2015.
Che, H. C., Zhang, X. Y., Zhang, L., Wang, Y. Q., Zhang, Y. M., Shen, X. J.,
Ma, Q. L., Sun, J. Y., and Zhong, J. T.: Prediction of size-resolved number
concentration of cloud condensation nuclei and long-term measurements of
their activation characteristics, Sci. Rep.-UK, 7, 5819,
https://doi.org/10.1038/s41598-017-05998-3, 2017.
Chen, D. and Shen, X.: Recent Progress on GRAPES Research and
Application, J. Appl. Meteorol. Sci., 17, 773–777, 2006.
Chen, D. H., Xue, J., Yang, X., Zhang, H., Shen, X., Hu, J., Wang, Y., Ji,
L., and Chen, J.: New generation of multi-scale NWP system (GRAPES): general
scientific design, Chinese Sci. Bull., 53, 3433–3445, 2008.
Chen, F. and Dudhia, J.: Coupling an advanced land surface–hydrology model
with the Penn State–NCAR MM5 modeling system. Part I: Model implementation
and sensitivity, Mon. Weather Rev., 129, 569–585, 2001.
Chou, M.-D., Suarez, M., Ho, C.-H., Yan, M., and Lee, K.-T.:
Parameterizations for Cloud Overlapping and Shortwave Single-Scattering
Properties for Use in General Circulation and Cloud Ensemble Models, J. Climate, 11, 202–214,
https://doi.org/10.1175/1520-0442(1998)011<0202:PFCOAS>2.0.CO;2, 1998.
DeMott, P. J., Prenni, A. J., Liu, X., Kreidenweis, S. M., Petters, M. D.,
Twohy, C. H., Richardson, M. S., Eidhammer, T., and Rogers, D. C.:
Predicting global atmospheric ice nuclei distributions and their impacts on
climate, P. Natl. Acad. Sci. USA, 107, 11217–11222,
https://doi.org/10.1073/pnas.0910818107, 2010.
Ding, S., Zhao, C., Shi G., and Wu, C.: Analysis of global total cloud
amount variation over the past 20 years, Journal of Applied Meteorological
Science, 16, 670–677, 2005.
Ekman, A. M. L., Engström, A., and Söderberg, A.: Impact of Two-Way
Aerosol–Cloud Interaction and Changes in Aerosol Size Distribution on
Simulated Aerosol-Induced Deep Convective Cloud Sensitivity, J.
Atmos. Sci., 68, 685–698, https://doi.org/10.1175/2010JAS3651.1,
2011.
Fan, J., Wang, Y., Rosenfeld, D., and Liu, X.: Review of Aerosol–Cloud
Interactions: Mechanisms, Significance, and Challenges, J.
Atmos. Sci., 73, 4221–4252,
https://doi.org/10.1175/JAS-D-16-0037.1, 2016.
Gong, S. L. and Zhang, X. Y.: CUACE/Dust – an integrated system of observation and modeling systems for operational dust forecasting in Asia, Atmos. Chem. Phys., 8, 2333–2340, https://doi.org/10.5194/acp-8-2333-2008, 2008.
Hahn, C. J., Rossow, W. B., and Warren, S. G.: ISCCP cloud properties
associated with standard cloud types identified in individual surface
observations, J. Climate, 14, 11–28, 2001.
Hong, S.-Y. and Pan, H.-L.: Nonlocal Boundary Layer Vertical Diffusion in a
Medium-Range Forecast Model, Mon. Weather Rev., 124, 2322–2339,
https://doi.org/10.1175/1520-0493(1996)124<2322:NBLVDI>2.0.CO;2, 1996.
Hong, S. Y. and Lim, J. O.: The WRF single-moment 6-class microphysics
scheme (WSM6), J. Korean Meteor. Soc., 42, 129–151, 2006.
Huang, X. and Ding, A.: Aerosol as a critical factor causing forecast biases
of air temperature in global numerical weather prediction models, Sci.
Bull., 66, 1917–1924, https://doi.org/10.1016/j.scib.2021.05.009, 2021.
Hudson, J. G. and Noble, S.: CCN and Vertical Velocity Influences
on Droplet Concentrations and Supersaturations in Clean and Polluted Stratus
Clouds, J. Atmos. Sci., 71, 312–331,
https://doi.org/10.1175/JAS-D-13-086.1, 2014.
Kain, J. S. and Fritsch, J. M.: Convective Parameterization for Mesoscale
Models: The Kain-Fritsch Scheme, in: The Representation of Cumulus
Convection in Numerical Models, edited by: Emanuel, K. A. and Raymond, D.
J., American Meteorological Society, Boston, MA, 165–170,
https://doi.org/10.1007/978-1-935704-13-3_16, 1993.
Lawand, D., Bhakare, S., Fadnavis, S., Bhawar, R., Rahul, P., Pallath, P.,
and Lolli, S.: Variability of Aerosols and Clouds Over North Indian and
Myanmar During the COVID-19 Lockdown Period, Front. Environ.
Sci., 10, 838778, https://doi.org/10.3389/fenvs.2022.838778, 2022.
Li, M., Zhang, Q., Streets, D. G., He, K. B., Cheng, Y. F., Emmons, L. K., Huo, H., Kang, S. C., Lu, Z., Shao, M., Su, H., Yu, X., and Zhang, Y.: Mapping Asian anthropogenic emissions of non-methane volatile organic compounds to multiple chemical mechanisms, Atmos. Chem. Phys., 14, 5617–5638, https://doi.org/10.5194/acp-14-5617-2014, 2014.
Li, M., Liu, H., Geng, G., Hong, C., Liu, F., Song, Y., Tong, D., Zheng, B.,
Cui, H., Hanyang, M., Zhang, Q., and He, K.: Anthropogenic emission
inventories in China: A review, Nat. Sci. Rev., 4, 834–866,
https://doi.org/10.1093/nsr/nwx150, 2017.
Lim, K.-S. S. and Hong, S.-Y.: Development of an Effective Double-Moment
Cloud Microphysics Scheme with Prognostic Cloud Condensation Nuclei (CCN)
for Weather and Climate Models, Mon. Weather Rev., 138, 1587–1612,
https://doi.org/10.1175/2009MWR2968.1, 2010.
Listowski, C. and Lachlan-Cope, T.: The microphysics of clouds over the Antarctic Peninsula – Part 2: modelling aspects within Polar WRF, Atmos. Chem. Phys., 17, 10195–10221, https://doi.org/10.5194/acp-17-10195-2017, 2017.
Liu, S., Xing, J., Zhao, B., Wang, J., Wang, S., Zhang, X., and Ding, A.:
Understanding of Aerosol–Climate Interactions in China: Aerosol Impacts on
Solar Radiation, Temperature, Cloud, and Precipitation and Its Changes Under
Future Climate and Emission Scenarios, Current Pollution Reports, 5, 36–51,
https://doi.org/10.1007/s40726-019-00107-6, 2019.
Lohmann, U. and Feichter, J.: Global indirect aerosol effects: a review, Atmos. Chem. Phys., 5, 715–737, https://doi.org/10.5194/acp-5-715-2005, 2005.
Lu, C., Liu, Y., Niu, S., and Vogelmann, A. M.: Observed impacts of vertical
velocity on cloud microphysics and implications for aerosol indirect
effects, Geophys. Res. Lett., 39, L21808,
https://doi.org/10.1029/2012GL053599, 2012.
Makar, P. A., Gong, W., Milbrandt, J., Hogrefe, C., Zhang, Y., Curci, G.,
Žabkar, R., Im, U., Balzarini, A., Baró, R., Bianconi, R., Cheung,
P., Forkel, R., Gravel, S., Hirtl, M., Honzak, L., Hou, A.,
Jiménez-Guerrero, P., Langer, M., Moran, M. D., Pabla, B., Pérez, J.
L., Pirovano, G., San José, R., Tuccella, P., Werhahn, J., Zhang, J.,
and Galmarini, S.: Feedbacks between air pollution and weather, Part 1:
Effects on weather, Atmos. Environ., 115, 442–469,
https://doi.org/10.1016/j.atmosenv.2014.12.003, 2015.
Mao, K., Yuan, Z., Zuo, Z., Xu, T., Shen, X., and Gao, C.: Changes in Global
Cloud Cover Based on Remote Sensing Data from 2003 to 2012, Chinese
Geogr. Sci., 29, 306–315,
https://doi.org/10.1007/s11769-019-1030-6, 2019.
McCoy, D. T., Field, P. R., Schmidt, A., Grosvenor, D. P., Bender, F. A.-M., Shipway, B. J., Hill, A. A., Wilkinson, J. M., and Elsaesser, G. S.: Aerosol midlatitude cyclone indirect effects in observations and high-resolution simulations, Atmos. Chem. Phys., 18, 5821–5846, https://doi.org/10.5194/acp-18-5821-2018, 2018.
McFiggans, G., Artaxo, P., Baltensperger, U., Coe, H., Facchini, M. C., Feingold, G., Fuzzi, S., Gysel, M., Laaksonen, A., Lohmann, U., Mentel, T. F., Murphy, D. M., O'Dowd, C. D., Snider, J. R., and Weingartner, E.: The effect of physical and chemical aerosol properties on warm cloud droplet activation, Atmos. Chem. Phys., 6, 2593–2649, https://doi.org/10.5194/acp-6-2593-2006, 2006.
Miltenberger, A. K., Field, P. R., Hill, A. A., Rosenberg, P., Shipway, B. J., Wilkinson, J. M., Scovell, R., and Blyth, A. M.: Aerosol–cloud interactions in mixed-phase convective clouds – Part 1: Aerosol perturbations, Atmos. Chem. Phys., 18, 3119–3145, https://doi.org/10.5194/acp-18-3119-2018, 2018.
Mlawer, E. J., Taubman, S. J., Brown, P. D., Iacono, M. J., and Clough, S.
A.: Radiative transfer for inhomogeneous atmospheres: RRTM, a validated
correlated-k model for the longwave, J. Geophys. Res.-Atmos., 102, 16663–16682, https://doi.org/10.1029/97JD00237, 1997.
Morrison, H., Thompson, G., and Tatarskii, V.: Impact of Cloud Microphysics
on the Development of Trailing Stratiform Precipitation in a Simulated
Squall Line: Comparison of One- and Two-Moment Schemes, Mon. Weather
Rev., 137, 991–1007, https://doi.org/10.1175/2008MWR2556.1, 2009.
Myhre, G., Samset, B. H., Schulz, M., Balkanski, Y., Bauer, S., Berntsen, T. K., Bian, H., Bellouin, N., Chin, M., Diehl, T., Easter, R. C., Feichter, J., Ghan, S. J., Hauglustaine, D., Iversen, T., Kinne, S., Kirkevåg, A., Lamarque, J.-F., Lin, G., Liu, X., Lund, M. T., Luo, G., Ma, X., van Noije, T., Penner, J. E., Rasch, P. J., Ruiz, A., Seland, Ø., Skeie, R. B., Stier, P., Takemura, T., Tsigaridis, K., Wang, P., Wang, Z., Xu, L., Yu, H., Yu, F., Yoon, J.-H., Zhang, K., Zhang, H., and Zhou, C.: Radiative forcing of the direct aerosol effect from AeroCom Phase II simulations, Atmos. Chem. Phys., 13, 1853–1877, https://doi.org/10.5194/acp-13-1853-2013, 2013.
National Centers for Environmental Prediction/National Weather Service/NOAA/U.S. Department of Commerce: NCEP GDAS/FNL 0.25 Degree Global Tropospheric Analyses and
Forecast Grids, Research Data Archive at the National Center for Atmospheric Research,
Computational and Information Systems Laboratory [data set], https://doi.org/10.5065/D65Q4T4Z,
2015.
NASA/LARC/SD/ASDC: CALIPSO Lidar Level 2 Vertical Feature Mask (VFM),
V4-20, NASA Langley Atmospheric Science Data Center [data set],
https://doi.org/10.5067/CALIOP/CALIPSO/LID_L2_VFM-STANDARD-V4-20, 2018.
Platnick, S., Meyer, K. G., Hubanks, P., Holz, R., Ackerman, S. A., and Heidinger, A.
K.: VIIRS Atmosphere L3 Cloud Properties Product, Version-1.1, NASA Level-1 and Atmosphere
Archive & Distribution System (LAADS) Distributed Active Archive Center (DAAC), Goddard
Space Flight Center, USA [data set],
https://doi.org/10.5067/VIIRS/CLDPROP_D3_VIIRS_SNPP.011, 2019.
Pawlowska, H. and Brenguier, J.-L.: Microphysical properties of
stratocumulus clouds during ACE-2, Tellus B, 52, 868–887,
https://doi.org/10.1034/j.1600-0889.2000.00076.x, 2000.
Pleim, J.: A Combined Local and Nonlocal Closure Model for the Atmospheric
Boundary Layer. Part II: Application and Evaluation in a Mesoscale
Meteorological Model, J. Appl. Meteorol. Clim., 46, 1396–1409,
https://doi.org/10.1175/JAM2534.1, 2007.
Pruppacher, H. R. and Klett, J. D.: Microphysics of Clouds and
Precipitation, Nature, 284, 88–88, https://doi.org/10.1038/284088b0, 1980.
Quaas, J.: Approaches to Observe Anthropogenic Aerosol-Cloud Interactions,
Current Climate Change Reports, 1, 297–304,
https://doi.org/10.1007/s40641-015-0028-0, 2015.
Ramanathan, V., Chung, C., Kim, D., Bettge, T., Buja, L., Kiehl, J. T.,
Washington, W. M., Fu, Q., Sikka, D. R., and Wild, M.: Atmospheric brown
clouds: Impacts on South Asian climate and hydrological cycle, P.
Natl. Acad. Sci. USA, 102, 5326–5333,
https://doi.org/10.1073/pnas.0500656102, 2005.
Rosenfeld, D., Andreae, M. O., Asmi, A., Chin, M., de Leeuw, G., Donovan, D.
P., Kahn, R., Kinne, S., Kivekäs, N., Kulmala, M., Lau, W., Schmidt, K.
S., Suni, T., Wagner, T., Wild, M., and Quaas, J.: Global observations of
aerosol-cloud-precipitation-climate interactions, Rev. Geophys., 52,
750–808, https://doi.org/10.1002/2013RG000441, 2014.
Rosenfeld, D., Zhu, Y., Wang, M., Zheng, Y., Goren, T., and Yu, S.:
Aerosol-driven droplet concentrations dominate coverage and water of oceanic
low-level clouds, Science, 363, eaav0566,
https://doi.org/10.1126/science.aav0566, 2019.
Rossow, W. B. and Schiffer, R. A.: ISCCP Cloud Data Products, B.
Am. Meteorol. Soc., 72, 2–20,
https://doi.org/10.1175/1520-0477(1991)072<0002:ICDP>2.0.CO;2, 1991.
Seifert, A., Köhler, C., and Beheng, K. D.: Aerosol-cloud-precipitation effects over Germany as simulated by a convective-scale numerical weather prediction model, Atmos. Chem. Phys., 12, 709–725, https://doi.org/10.5194/acp-12-709-2012, 2012.
Stockwell, W. R., Middleton, P., Chang, J. S., and Tang, X.: The second
generation regional acid deposition model chemical mechanism for regional
air quality modeling, J. Geophys. Res.-Atmos., 95,
16343–16367, https://doi.org/10.1029/JD095iD10p16343, 1990.
Su, L. and Fung, J. C. H.: Investigating the role of dust in ice nucleation within clouds and further effects on the regional weather system over East Asia – Part 1: model development and validation, Atmos. Chem. Phys., 18, 8707–8725, https://doi.org/10.5194/acp-18-8707-2018, 2018.
Sun, J. and Ariya, P. A.: Atmospheric organic and bio-aerosols as cloud
condensation nuclei (CCN): A review, Atmos. Environ., 40, 795–820,
https://doi.org/10.1016/j.atmosenv.2005.05.052, 2006.
Thompson, G. and Eidhammer, T.: A Study of Aerosol Impacts on Clouds and
Precipitation Development in a Large Winter Cyclone, J.
Atmos. Sci., 71, 3636–3658,
https://doi.org/10.1175/JAS-D-13-0305.1, 2014.
Thompson, G., Rasmussen, R. M., and Manning, K.: Explicit forecasts of
winter precipitation using an improved bulk microphysics scheme. Part I:
Description and sensitivity analysis, Mon. Weather Rev., 132, 519–542, 2004.
Thompson, G., Field, P. R., Rasmussen, R. M., and Hall, W. D.: Explicit
forecasts of winter precipitation using an improved bulk microphysics
scheme. Part II: Implementation of a new snow parameterization, Mon. Weather
Rev., 136, 5095–5115, 2008.
Twomey, S.: The Influence of Pollution on the Shortwave Albedo of Clouds,
J. Atmos. Sci., 34, 1149–1154,
https://doi.org/10.1175/1520-0469(1977)034<1149:TIOPOT>2.0.CO;2, 1977.
Wang, H., Gong, S., Zhang, H., Chen, Y., Shen, X., Chen, D., Xue, J., Shen,
Y., Wu, X., and Jin, Z.: A new-generation sand and dust storm forecasting
system GRAPES_CUACE/Dust: Model development, verification and
numerical simulation, Chinese Sci. Bull., 55, 635–649,
https://doi.org/10.1007/s11434-009-0481-z, 2010.
Wang, K., Zhang, Y., Yu, S., Wong, D. C., Pleim, J., Mathur, R., Kelly, J. T., and Bell, M.: A comparative study of two-way and offline coupled WRF v3.4 and CMAQ v5.0.2 over the contiguous US: performance evaluation and impacts of chemistry–meteorology feedbacks on air quality, Geosci. Model Dev., 14, 7189–7221, https://doi.org/10.5194/gmd-14-7189-2021, 2021.
Wang, Z., Zhang, H., and Lu, P.: Improvement of cloud microphysics in the
aerosol-climate model BCC_AGCM2.0.1_CUACE/Aero, evaluation against observations, and updated aerosol indirect
effect, J. Geophys. Res.-Atmos., 119, 8400–8417,
https://doi.org/10.1002/2014JD021886, 2014.
White, B., Gryspeerdt, E., Stier, P., Morrison, H., Thompson, G., and Kipling, Z.: Uncertainty from the choice of microphysics scheme in convection-permitting models significantly exceeds aerosol effects, Atmos. Chem. Phys., 17, 12145–12175, https://doi.org/10.5194/acp-17-12145-2017, 2017.
Wong, D. C., Pleim, J., Mathur, R., Binkowski, F., Otte, T., Gilliam, R., Pouliot, G., Xiu, A., Young, J. O., and Kang, D.: WRF-CMAQ two-way coupled system with aerosol feedback: software development and preliminary results, Geosci. Model Dev., 5, 299–312, https://doi.org/10.5194/gmd-5-299-2012, 2012.
Xu, X., Lu, C., Liu, Y., Luo, S., Zhou, X., Endo, S., Zhu, L., and Wang, Y.: Influences of an entrainment–mixing parameterization on numerical simulations of cumulus and stratocumulus clouds, Atmos. Chem. Phys., 22, 5459–5475, https://doi.org/10.5194/acp-22-5459-2022, 2022.
Zhang, B., Wang, Y., and Hao, J.: Simulating aerosol–radiation–cloud feedbacks on meteorology and air quality over eastern China under severe haze conditionsin winter, Atmos. Chem. Phys., 15, 2387–2404, https://doi.org/10.5194/acp-15-2387-2015, 2015.
Zhang, R. H. and Shen, X.: On the development of the GRAPES – A new
generation of the national operational NWP system in China, Chinese Sci.
Bull., 53, 3429–3432, 2008.
Zhang, Y., Wen, X. Y., and Jang, C. J.: Simulating
chemistry–aerosol–cloud–radiation–climate feedbacks over the continental
U.S. using the online-coupled Weather Research Forecasting Model with
chemistry (WRF/Chem), Atmos. Environ., 44, 3568–3582,
https://doi.org/10.1016/j.atmosenv.2010.05.056, 2010.
Zhao, B., Liou, K.-N., Gu, Y., Li, Q., Jiang, J. H., Su, H., He, C., Tseng,
H.-L. R., Wang, S., Liu, R., Qi, L., Lee, W.-L., and Hao, J.: Enhanced
PM2.5 pollution in China due to aerosol-cloud interactions, Sci.
Rep.-UK, 7, 4453, https://doi.org/10.1038/s41598-017-04096-8, 2017.
Zheng, B., Tong, D., Li, M., Liu, F., Hong, C., Geng, G., Li, H., Li, X., Peng, L., Qi, J., Yan, L., Zhang, Y., Zhao, H., Zheng, Y., He, K., and Zhang, Q.: Trends in China's anthropogenic emissions since 2010 as the consequence of clean air actions, Atmos. Chem. Phys., 18, 14095–14111, https://doi.org/10.5194/acp-18-14095-2018, 2018.
Zheng, G., Wang, Y., Aiken, A. C., Gallo, F., Jensen, M. P., Kollias, P., Kuang, C., Luke, E., Springston, S., Uin, J., Wood, R., and Wang, J.: Marine boundary layer aerosol in the eastern North Atlantic: seasonal variations and key controlling processes, Atmos. Chem. Phys., 18, 17615–17635, https://doi.org/10.5194/acp-18-17615-2018, 2018.
Zhou, C.-H., Gong, S., Zhang, X.-Y., Liu, H.-L., Xue, M., Cao, G.-L., An,
X.-Q., Che, H.-Z., Zhang, Y.-M., and Niu, T.: Towards the improvements of
simulating the chemical and optical properties of Chinese aerosols using an
online coupled model – CUACE/Aero, Tellus B, 64, 18965, https://doi.org/10.3402/tellusb.v64i0.18965, 2012.
Zhou, C., Zhang, X., Gong, S., Wang, Y., and Xue, M.: Improving aerosol interaction with clouds and precipitation in a regional chemical weather modeling system, Atmos. Chem. Phys., 16, 145–160, https://doi.org/10.5194/acp-16-145-2016, 2016.
Zhou, S., Yang, J., Wang, W.-C., Zhao, C., Gong, D., and Shi, P.: An observational study of the effects of aerosols on diurnal variation of heavy rainfall and associated clouds over Beijing–Tianjin–Hebei, Atmos. Chem. Phys., 20, 5211–5229, https://doi.org/10.5194/acp-20-5211-2020, 2020.
Short summary
Aerosol–cloud interaction (ACI) is first implemented in the atmospheric chemistry system GRAPES_Meso5.1/CUACE. ACI can improve the simulated cloud, temperature, and precipitation under haze pollution conditions in Jing-Jin-Ji in China. This paper demonstrates the critical role of ACI in current numerical weather prediction over the severely polluted region.
Aerosol–cloud interaction (ACI) is first implemented in the atmospheric chemistry system...
Altmetrics
Final-revised paper
Preprint