Articles | Volume 20, issue 4
https://doi.org/10.5194/acp-20-2201-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-2201-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
26 Feb 2020
Research article |
| 26 Feb 2020
| 26 Feb 2020
Comparing the impact of environmental conditions and microphysics on the forecast uncertainty of deep convective clouds and hail
Constanze Wellmann
CORRESPONDING AUTHOR
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Andrew I. Barrett
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Jill S. Johnson
Institute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, UK
Michael Kunz
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Bernhard Vogel
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
Ken S. Carslaw
Institute for Climate and Atmospheric Science, School of Earth and Environment, University of Leeds, Leeds, UK
Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Karlsruhe, Germany
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Lina Lucas, Christian Barthlott, Corinna Hoose, and Peter Knippertz
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We studied how climate change and cleaner air could affect severe storms in Central Europe. Using high-resolution weather simulations of past supercell storms under warmer and less polluted conditions, we found that storms may become more intense, with heavier rainfall and larger hailstones. These changes suggest an increased risk of damage in the future. Our findings help improve understanding of how extreme storms may evolve in a changing climate.
Rachel W. N. Sansom, Jill S. Johnson, Leighton A. Regayre, Lindsay A. Lee, and Ken S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2025-3104, https://doi.org/10.5194/egusphere-2025-3104, 2025
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Atmos. Chem. Phys., 25, 6607–6631, https://doi.org/10.5194/acp-25-6607-2025, https://doi.org/10.5194/acp-25-6607-2025, 2025
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Xinyue Shao, Yaman Liu, Xinyi Dong, Minghuai Wang, Ruochong Xu, Joel A. Thornton, Duseong S. Jo, Man Yue, Wenxiang Shen, Manish Shrivastava, Stephen R. Arnold, and Ken S. Carslaw
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Barbara Ervens, Ken S. Carslaw, Thomas Koop, and Ulrich Pöschl
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Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen R. Arnold, Leighton A. Regayre, Meinrat O. Andreae, Mira L. Pöhlker, Duseong S. Jo, Man Yue, and Ken S. Carslaw
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Barbara Dietel, Odran Sourdeval, and Corinna Hoose
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Behrooz Keshtgar, Aiko Voigt, Bernhard Mayer, and Corinna Hoose
Atmos. Chem. Phys., 24, 4751–4769, https://doi.org/10.5194/acp-24-4751-2024, https://doi.org/10.5194/acp-24-4751-2024, 2024
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Cloud-radiative heating (CRH) affects extratropical cyclones but is uncertain in weather and climate models. We provide a framework to quantify uncertainties in CRH within an extratropical cyclone due to four factors and show that the parameterization of ice optical properties contributes significantly to uncertainty in CRH. We also argue that ice optical properties, by affecting CRH on spatial scales of 100 km, are relevant for the large-scale dynamics of extratropical cyclones.
Rolf Müller, Ulrich Pöschl, Thomas Koop, Thomas Peter, and Ken Carslaw
Atmos. Chem. Phys., 23, 15445–15453, https://doi.org/10.5194/acp-23-15445-2023, https://doi.org/10.5194/acp-23-15445-2023, 2023
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Paul J. Crutzen was a pioneer in atmospheric sciences and a kind-hearted, humorous person with empathy for the private lives of his colleagues and students. He made fundamental scientific contributions to a wide range of scientific topics in all parts of the atmosphere. Paul was among the founders of the journal Atmospheric Chemistry and Physics. His work will continue to be a guide for generations of scientists and environmental policymakers to come.
Hyunju Jung, Peter Knippertz, Yvonne Ruckstuhl, Robert Redl, Tijana Janjic, and Corinna Hoose
Weather Clim. Dynam., 4, 1111–1134, https://doi.org/10.5194/wcd-4-1111-2023, https://doi.org/10.5194/wcd-4-1111-2023, 2023
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A narrow rainfall belt in the tropics is an important feature for large-scale circulations and the global water cycle. The accurate simulation of this rainfall feature has been a long-standing problem, with the reasons behind that unclear. We present a novel diagnostic tool that allows us to disentangle processes important for rainfall, which changes due to modifications in model. Using our diagnostic tool, one can potentially identify sources of uncertainty in weather and climate models.
Hamza Ahsan, Hailong Wang, Jingbo Wu, Mingxuan Wu, Steven J. Smith, Susanne Bauer, Harrison Suchyta, Dirk Olivié, Gunnar Myhre, Hitoshi Matsui, Huisheng Bian, Jean-François Lamarque, Ken Carslaw, Larry Horowitz, Leighton Regayre, Mian Chin, Michael Schulz, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Vaishali Naik
Atmos. Chem. Phys., 23, 14779–14799, https://doi.org/10.5194/acp-23-14779-2023, https://doi.org/10.5194/acp-23-14779-2023, 2023
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We examine the impact of the assumed effective height of SO2 injection, SO2 and BC emission seasonality, and the assumed fraction of SO2 emissions injected as SO4 on climate and chemistry model results. We find that the SO2 injection height has a large impact on surface SO2 concentrations and, in some models, radiative flux. These assumptions are a
hiddensource of inter-model variability and may be leading to bias in some climate model results.
Cunbo Han, Corinna Hoose, Martin Stengel, Quentin Coopman, and Andrew Barrett
Atmos. Chem. Phys., 23, 14077–14095, https://doi.org/10.5194/acp-23-14077-2023, https://doi.org/10.5194/acp-23-14077-2023, 2023
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Cloud phase has been found to significantly impact cloud thermodynamics and Earth’s radiation budget, and various factors influence it. This study investigates the sensitivity of the cloud-phase distribution to the ice-nucleating particle concentration and thermodynamics. Multiple simulation experiments were performed using the ICON model at the convection-permitting resolution of 1.2 km. Simulation results were compared to two different retrieval products based on SEVIRI measurements.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David M. H. Sexton, Christopher Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John W. Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 8749–8768, https://doi.org/10.5194/acp-23-8749-2023, https://doi.org/10.5194/acp-23-8749-2023, 2023
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Aerosol forcing of Earth’s energy balance has persisted as a major cause of uncertainty in climate simulations over generations of climate model development. We show that structural deficiencies in a climate model are exposed by comprehensively exploring parametric uncertainty and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. This provides a future pathway towards building models with greater physical realism and lower uncertainty.
Annika Oertel, Annette K. Miltenberger, Christian M. Grams, and Corinna Hoose
Atmos. Chem. Phys., 23, 8553–8581, https://doi.org/10.5194/acp-23-8553-2023, https://doi.org/10.5194/acp-23-8553-2023, 2023
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Warm conveyor belts (WCBs) are cloud- and precipitation-producing airstreams in extratropical cyclones that are important for the large-scale flow and cloud radiative forcing. We analyze cloud formation processes during WCB ascent in a two-moment microphysics scheme. Quantification of individual diabatic heating rates shows the importance of condensation, vapor deposition, rain evaporation, melting, and cloud-top radiative cooling for total heating and WCB-related potential vorticity structure.
Daniel P. Grosvenor and Kenneth S. Carslaw
Atmos. Chem. Phys., 23, 6743–6773, https://doi.org/10.5194/acp-23-6743-2023, https://doi.org/10.5194/acp-23-6743-2023, 2023
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We determine what causes long-term trends in short-wave (SW) radiative fluxes in two climate models. A positive trend occurs between 1850 and 1970 (increasing SW reflection) and a negative trend between 1970 and 2014; the pre-1970 positive trend is mainly driven by an increase in cloud droplet number concentrations due to increases in aerosol, and the 1970–2014 trend is driven by a decrease in cloud fraction, which we attribute to changes in clouds caused by greenhouse gas-induced warming.
Axel Seifert, Vanessa Bachmann, Florian Filipitsch, Jochen Förstner, Christian M. Grams, Gholam Ali Hoshyaripour, Julian Quinting, Anika Rohde, Heike Vogel, Annette Wagner, and Bernhard Vogel
Atmos. Chem. Phys., 23, 6409–6430, https://doi.org/10.5194/acp-23-6409-2023, https://doi.org/10.5194/acp-23-6409-2023, 2023
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We investigate how mineral dust can lead to the formation of cirrus clouds. Dusty cirrus clouds lead to a reduction in solar radiation at the surface and, hence, a reduced photovoltaic power generation. Current weather prediction systems are not able to predict this interaction between mineral dust and cirrus clouds. We have developed a new physical description of the formation of dusty cirrus clouds. Overall we can show a considerable improvement in the forecast quality of clouds and radiation.
Ernesto Reyes-Villegas, Douglas Lowe, Jill S. Johnson, Kenneth S. Carslaw, Eoghan Darbyshire, Michael Flynn, James D. Allan, Hugh Coe, Ying Chen, Oliver Wild, Scott Archer-Nicholls, Alex Archibald, Siddhartha Singh, Manish Shrivastava, Rahul A. Zaveri, Vikas Singh, Gufran Beig, Ranjeet Sokhi, and Gordon McFiggans
Atmos. Chem. Phys., 23, 5763–5782, https://doi.org/10.5194/acp-23-5763-2023, https://doi.org/10.5194/acp-23-5763-2023, 2023
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Organic aerosols (OAs), their sources and their processes remain poorly understood. The volatility basis set (VBS) approach, implemented in air quality models such as WRF-Chem, can be a useful tool to describe primary OA (POA) production and aging. However, the main disadvantage is its complexity. We used a Gaussian process simulator to reproduce model results and to estimate the sources of model uncertainty. We do this by comparing the outputs with OA observations made at Delhi, India, in 2018.
Heinz Jürgen Punge, Kristopher M. Bedka, Michael Kunz, Sarah D. Bang, and Kyle F. Itterly
Nat. Hazards Earth Syst. Sci., 23, 1549–1576, https://doi.org/10.5194/nhess-23-1549-2023, https://doi.org/10.5194/nhess-23-1549-2023, 2023
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We have estimated the probability of hail events in South Africa using a combination of satellite observations, reanalysis, and insurance claims data. It is found that hail is mainly concentrated in the southeast. Multivariate stochastic modeling of event characteristics, such as multiple events per day or track dimensions, provides an event catalogue for 25 000 years. This can be used to estimate hail risk for return periods of 200 years, as required by insurance companies.
Xuemei Wang, Hamish Gordon, Daniel P. Grosvenor, Meinrat O. Andreae, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 4431–4461, https://doi.org/10.5194/acp-23-4431-2023, https://doi.org/10.5194/acp-23-4431-2023, 2023
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New particle formation in the upper troposphere is important for the global boundary layer aerosol population, and they can be transported downward in Amazonia. We use a global and a regional model to quantify the number of aerosols that are formed at high altitude and transported downward in a 1000 km region. We find that the majority of the aerosols are from outside the region. This suggests that the 1000 km region is unlikely to be a
closed loopfor aerosol formation, transport and growth.
Ruth Price, Andrea Baccarini, Julia Schmale, Paul Zieger, Ian M. Brooks, Paul Field, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 2927–2961, https://doi.org/10.5194/acp-23-2927-2023, https://doi.org/10.5194/acp-23-2927-2023, 2023
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Arctic clouds can control how much energy is absorbed by the surface or reflected back to space. Using a computer model of the atmosphere we investigated the formation of atmospheric particles that allow cloud droplets to form. We found that particles formed aloft are transported to the lowest part of the Arctic atmosphere and that this is a key source of particles. Our results have implications for the way Arctic clouds will behave in the future as climate change continues to impact the region.
Julia Thomas, Andrew Barrett, and Corinna Hoose
Atmos. Chem. Phys., 23, 1987–2002, https://doi.org/10.5194/acp-23-1987-2023, https://doi.org/10.5194/acp-23-1987-2023, 2023
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We study the sensitivity of rain formation processes during a heavy-rainfall event over mountains to changes in temperature and pollution. Total rainfall increases by 2 % K−1, and a 6 % K−1 increase is found at the highest altitudes, caused by a mixed-phase seeder–feeder mechanism (frozen cloud particles melt and grow further as they fall through a liquid cloud layer). In a cleaner atmosphere this process is enhanced. Thus the risk of severe rainfall in mountains may increase in the future.
Susanna Mohr, Uwe Ehret, Michael Kunz, Patrick Ludwig, Alberto Caldas-Alvarez, James E. Daniell, Florian Ehmele, Hendrik Feldmann, Mário J. Franca, Christian Gattke, Marie Hundhausen, Peter Knippertz, Katharina Küpfer, Bernhard Mühr, Joaquim G. Pinto, Julian Quinting, Andreas M. Schäfer, Marc Scheibel, Frank Seidel, and Christina Wisotzky
Nat. Hazards Earth Syst. Sci., 23, 525–551, https://doi.org/10.5194/nhess-23-525-2023, https://doi.org/10.5194/nhess-23-525-2023, 2023
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The flood event in July 2021 was one of the most severe disasters in Europe in the last half century. The objective of this two-part study is a multi-disciplinary assessment that examines the complex process interactions in different compartments, from meteorology to hydrological conditions to hydro-morphological processes to impacts on assets and environment. In addition, we address the question of what measures are possible to generate added value to early response management.
Behrooz Keshtgar, Aiko Voigt, Corinna Hoose, Michael Riemer, and Bernhard Mayer
Weather Clim. Dynam., 4, 115–132, https://doi.org/10.5194/wcd-4-115-2023, https://doi.org/10.5194/wcd-4-115-2023, 2023
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Forecasting extratropical cyclones is challenging due to many physical factors influencing their behavior. One such factor is the impact of heating and cooling of the atmosphere by the interaction between clouds and radiation. In this study, we show that cloud-radiative heating (CRH) increases the intensity of an idealized cyclone and affects its predictability. We find that CRH affects the cyclone mostly via increasing latent heat release and subsequent changes in the synoptic circulation.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David Sexton, Christopher C. Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
EGUsphere, https://doi.org/10.5194/egusphere-2022-1330, https://doi.org/10.5194/egusphere-2022-1330, 2022
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We show that potential structural deficiencies in a climate model can be exposed by comprehensively exploring its parametric uncertainty, and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. Combined consideration of parametric and structural uncertainties provides a future pathway towards building models that have greater physical realism and lower uncertainty.
Ville Leinonen, Harri Kokkola, Taina Yli-Juuti, Tero Mielonen, Thomas Kühn, Tuomo Nieminen, Simo Heikkinen, Tuuli Miinalainen, Tommi Bergman, Ken Carslaw, Stefano Decesari, Markus Fiebig, Tareq Hussein, Niku Kivekäs, Radovan Krejci, Markku Kulmala, Ari Leskinen, Andreas Massling, Nikos Mihalopoulos, Jane P. Mulcahy, Steffen M. Noe, Twan van Noije, Fiona M. O'Connor, Colin O'Dowd, Dirk Olivie, Jakob B. Pernov, Tuukka Petäjä, Øyvind Seland, Michael Schulz, Catherine E. Scott, Henrik Skov, Erik Swietlicki, Thomas Tuch, Alfred Wiedensohler, Annele Virtanen, and Santtu Mikkonen
Atmos. Chem. Phys., 22, 12873–12905, https://doi.org/10.5194/acp-22-12873-2022, https://doi.org/10.5194/acp-22-12873-2022, 2022
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We provide the first extensive comparison of detailed aerosol size distribution trends between in situ observations from Europe and five different earth system models. We investigated aerosol modes (nucleation, Aitken, and accumulation) separately and were able to show the differences between measured and modeled trends and especially their seasonal patterns. The differences in model results are likely due to complex effects of several processes instead of certain specific model features.
Amy H. Peace, Ben B. B. Booth, Leighton A. Regayre, Ken S. Carslaw, David M. H. Sexton, Céline J. W. Bonfils, and John W. Rostron
Earth Syst. Dynam., 13, 1215–1232, https://doi.org/10.5194/esd-13-1215-2022, https://doi.org/10.5194/esd-13-1215-2022, 2022
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Anthropogenic aerosol emissions have been linked to driving climate responses such as shifts in the location of tropical rainfall. However, the interaction of aerosols with climate remains one of the most uncertain aspects of climate modelling and limits our ability to predict future climate change. We use an ensemble of climate model simulations to investigate what impact the large uncertainty in how aerosols interact with climate has on predicting future tropical rainfall shifts.
Natalia E. Chubarova, Heike Vogel, Elizaveta E. Androsova, Alexander A. Kirsanov, Olga B. Popovicheva, Bernhard Vogel, and Gdaliy S. Rivin
Atmos. Chem. Phys., 22, 10443–10466, https://doi.org/10.5194/acp-22-10443-2022, https://doi.org/10.5194/acp-22-10443-2022, 2022
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Effects of urban aerosol pollution in Moscow were analyzed using the COSMO-ART chemical transport model and intensive measurement campaigns. We show that urban aerosol comprises about 15–20% of columnar aerosol content, consisting mainly of fine aerosol mode. The black carbon (BC) fraction is about 5 %, depending on particle dispersion intensity (IPD). The BC fraction low value explains weak absorbing properties of the Moscow atmosphere. IPD also defines the daily cycle of urban aerosol species.
Alexander D. Harrison, Daniel O'Sullivan, Michael P. Adams, Grace C. E. Porter, Edmund Blades, Cherise Brathwaite, Rebecca Chewitt-Lucas, Cassandra Gaston, Rachel Hawker, Ovid O. Krüger, Leslie Neve, Mira L. Pöhlker, Christopher Pöhlker, Ulrich Pöschl, Alberto Sanchez-Marroquin, Andrea Sealy, Peter Sealy, Mark D. Tarn, Shanice Whitehall, James B. McQuaid, Kenneth S. Carslaw, Joseph M. Prospero, and Benjamin J. Murray
Atmos. Chem. Phys., 22, 9663–9680, https://doi.org/10.5194/acp-22-9663-2022, https://doi.org/10.5194/acp-22-9663-2022, 2022
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The formation of ice in clouds fundamentally alters cloud properties; hence it is important we understand the special aerosol particles that can nucleate ice when immersed in supercooled cloud droplets. In this paper we show that African desert dust that has travelled across the Atlantic to the Caribbean nucleates ice much less well than we might have expected.
Julia Bruckert, Gholam Ali Hoshyaripour, Ákos Horváth, Lukas O. Muser, Fred J. Prata, Corinna Hoose, and Bernhard Vogel
Atmos. Chem. Phys., 22, 3535–3552, https://doi.org/10.5194/acp-22-3535-2022, https://doi.org/10.5194/acp-22-3535-2022, 2022
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Volcanic emissions endanger aviation and public health and also influence weather and climate. Forecasting the volcanic-plume dispersion is therefore a critical yet sophisticated task. Here, we show that explicit treatment of volcanic-plume dynamics and eruption source parameters significantly improves volcanic-plume dispersion forecasts. We further demonstrate the lofting of the SO2 due to a heating of volcanic particles by sunlight with major implications for volcanic aerosol research.
Rachel E. Hawker, Annette K. Miltenberger, Jill S. Johnson, Jonathan M. Wilkinson, Adrian A. Hill, Ben J. Shipway, Paul R. Field, Benjamin J. Murray, and Ken S. Carslaw
Atmos. Chem. Phys., 21, 17315–17343, https://doi.org/10.5194/acp-21-17315-2021, https://doi.org/10.5194/acp-21-17315-2021, 2021
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We find that ice-nucleating particles (INPs), aerosols that can initiate the freezing of cloud droplets, cause substantial changes to the properties of radiatively important convectively generated anvil cirrus. The number concentration of INPs had a large effect on ice crystal number concentration while the INP temperature dependence controlled ice crystal size and cloud fraction. The results indicate information on INP number and source is necessary for the representation of cloud glaciation.
Heather Guy, Ian M. Brooks, Ken S. Carslaw, Benjamin J. Murray, Von P. Walden, Matthew D. Shupe, Claire Pettersen, David D. Turner, Christopher J. Cox, William D. Neff, Ralf Bennartz, and Ryan R. Neely III
Atmos. Chem. Phys., 21, 15351–15374, https://doi.org/10.5194/acp-21-15351-2021, https://doi.org/10.5194/acp-21-15351-2021, 2021
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We present the first full year of surface aerosol number concentration measurements from the central Greenland Ice Sheet. Aerosol concentrations here have a distinct seasonal cycle from those at lower-altitude Arctic sites, which is driven by large-scale atmospheric circulation. Our results can be used to help understand the role aerosols might play in Greenland surface melt through the modification of cloud properties. This is crucial in a rapidly changing region where observations are sparse.
Mao Xiao, Christopher R. Hoyle, Lubna Dada, Dominik Stolzenburg, Andreas Kürten, Mingyi Wang, Houssni Lamkaddam, Olga Garmash, Bernhard Mentler, Ugo Molteni, Andrea Baccarini, Mario Simon, Xu-Cheng He, Katrianne Lehtipalo, Lauri R. Ahonen, Rima Baalbaki, Paulus S. Bauer, Lisa Beck, David Bell, Federico Bianchi, Sophia Brilke, Dexian Chen, Randall Chiu, António Dias, Jonathan Duplissy, Henning Finkenzeller, Hamish Gordon, Victoria Hofbauer, Changhyuk Kim, Theodore K. Koenig, Janne Lampilahti, Chuan Ping Lee, Zijun Li, Huajun Mai, Vladimir Makhmutov, Hanna E. Manninen, Ruby Marten, Serge Mathot, Roy L. Mauldin, Wei Nie, Antti Onnela, Eva Partoll, Tuukka Petäjä, Joschka Pfeifer, Veronika Pospisilova, Lauriane L. J. Quéléver, Matti Rissanen, Siegfried Schobesberger, Simone Schuchmann, Yuri Stozhkov, Christian Tauber, Yee Jun Tham, António Tomé, Miguel Vazquez-Pufleau, Andrea C. Wagner, Robert Wagner, Yonghong Wang, Lena Weitz, Daniela Wimmer, Yusheng Wu, Chao Yan, Penglin Ye, Qing Ye, Qiaozhi Zha, Xueqin Zhou, Antonio Amorim, Ken Carslaw, Joachim Curtius, Armin Hansel, Rainer Volkamer, Paul M. Winkler, Richard C. Flagan, Markku Kulmala, Douglas R. Worsnop, Jasper Kirkby, Neil M. Donahue, Urs Baltensperger, Imad El Haddad, and Josef Dommen
Atmos. Chem. Phys., 21, 14275–14291, https://doi.org/10.5194/acp-21-14275-2021, https://doi.org/10.5194/acp-21-14275-2021, 2021
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Experiments at CLOUD show that in polluted environments new particle formation (NPF) is largely driven by the formation of sulfuric acid–base clusters, stabilized by amines, high ammonia concentrations or lower temperatures. While oxidation products of aromatics can nucleate, they play a minor role in urban NPF. Our experiments span 4 orders of magnitude variation of observed NPF rates in ambient conditions. We provide a framework based on NPF and growth rates to interpret ambient observations.
Ramiro Checa-Garcia, Yves Balkanski, Samuel Albani, Tommi Bergman, Ken Carslaw, Anne Cozic, Chris Dearden, Beatrice Marticorena, Martine Michou, Twan van Noije, Pierre Nabat, Fiona M. O'Connor, Dirk Olivié, Joseph M. Prospero, Philippe Le Sager, Michael Schulz, and Catherine Scott
Atmos. Chem. Phys., 21, 10295–10335, https://doi.org/10.5194/acp-21-10295-2021, https://doi.org/10.5194/acp-21-10295-2021, 2021
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Thousands of tons of dust are emitted into the atmosphere every year, producing important impacts on the Earth system. However, current global climate models are not yet able to reproduce dust emissions, transport and depositions with the desirable accuracy. Our study analyses five different Earth system models to report aspects to be improved to reproduce better available observations, increase the consistency between models and therefore decrease the current uncertainties.
Rachel E. Hawker, Annette K. Miltenberger, Jonathan M. Wilkinson, Adrian A. Hill, Ben J. Shipway, Zhiqiang Cui, Richard J. Cotton, Ken S. Carslaw, Paul R. Field, and Benjamin J. Murray
Atmos. Chem. Phys., 21, 5439–5461, https://doi.org/10.5194/acp-21-5439-2021, https://doi.org/10.5194/acp-21-5439-2021, 2021
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The impact of aerosols on clouds is a large source of uncertainty for future climate projections. Our results show that the radiative properties of a complex convective cloud field in the Saharan outflow region are sensitive to the temperature dependence of ice-nucleating particle concentrations. This means that differences in the aerosol source or composition, for the same aerosol size distribution, can cause differences in the outgoing radiation from regions dominated by tropical convection.
Ananth Ranjithkumar, Hamish Gordon, Christina Williamson, Andrew Rollins, Kirsty Pringle, Agnieszka Kupc, Nathan Luke Abraham, Charles Brock, and Ken Carslaw
Atmos. Chem. Phys., 21, 4979–5014, https://doi.org/10.5194/acp-21-4979-2021, https://doi.org/10.5194/acp-21-4979-2021, 2021
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The effect aerosols have on climate can be better understood by studying their vertical and spatial distribution throughout the atmosphere. We use observation data from the ATom campaign and evaluate the vertical profile of aerosol number concentration, sulfur dioxide and condensation sink using the UKESM (UK Earth System Model). We identify uncertainties in key atmospheric processes that help improve their theoretical representation in global climate models.
Kamalika Sengupta, Kirsty Pringle, Jill S. Johnson, Carly Reddington, Jo Browse, Catherine E. Scott, and Ken Carslaw
Atmos. Chem. Phys., 21, 2693–2723, https://doi.org/10.5194/acp-21-2693-2021, https://doi.org/10.5194/acp-21-2693-2021, 2021
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Global models consistently underestimate atmospheric secondary organic aerosol (SOA), which has significant climatic implications. We use a perturbed parameter model ensemble and ground-based observations to reduce the uncertainty in modelling SOA formation from oxidation of volatile organic compounds. We identify plausible parameter spaces for the yields of extremely low-volatility, low-volatility, and semi-volatile organic compounds based on model–observation match for three key model outputs.
Elody Fluck, Michael Kunz, Peter Geissbuehler, and Stefan P. Ritz
Nat. Hazards Earth Syst. Sci., 21, 683–701, https://doi.org/10.5194/nhess-21-683-2021, https://doi.org/10.5194/nhess-21-683-2021, 2021
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Severe convective storms (SCSs) and the related hail events constitute major atmospheric hazards in parts of Europe. In our study, we identified the regions of France, Germany, Belgium and Luxembourg that were most affected by hail over a 10 year period (2005 to 2014). A cell-tracking algorithm was computed on remote-sensing data to enable the reconstruction of several thousand SCS tracks. The location of hail hotspots will help us understand hail formation and improve hail forecasting.
Jim M. Haywood, Steven J. Abel, Paul A. Barrett, Nicolas Bellouin, Alan Blyth, Keith N. Bower, Melissa Brooks, Ken Carslaw, Haochi Che, Hugh Coe, Michael I. Cotterell, Ian Crawford, Zhiqiang Cui, Nicholas Davies, Beth Dingley, Paul Field, Paola Formenti, Hamish Gordon, Martin de Graaf, Ross Herbert, Ben Johnson, Anthony C. Jones, Justin M. Langridge, Florent Malavelle, Daniel G. Partridge, Fanny Peers, Jens Redemann, Philip Stier, Kate Szpek, Jonathan W. Taylor, Duncan Watson-Parris, Robert Wood, Huihui Wu, and Paquita Zuidema
Atmos. Chem. Phys., 21, 1049–1084, https://doi.org/10.5194/acp-21-1049-2021, https://doi.org/10.5194/acp-21-1049-2021, 2021
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Every year, the seasonal cycle of biomass burning from agricultural practices in Africa creates a huge plume of smoke that travels many thousands of kilometres over the Atlantic Ocean. This study provides an overview of a measurement campaign called the cloud–aerosol–radiation interaction and forcing for year 2017 (CLARIFY-2017) and documents the rationale, deployment strategy, observations, and key results from the campaign which utilized the heavily equipped FAAM atmospheric research aircraft.
Benjamin J. Murray, Kenneth S. Carslaw, and Paul R. Field
Atmos. Chem. Phys., 21, 665–679, https://doi.org/10.5194/acp-21-665-2021, https://doi.org/10.5194/acp-21-665-2021, 2021
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The balance between the amounts of ice and supercooled water in clouds over the world's oceans strongly influences how much these clouds can dampen or amplify global warming. Aerosol particles which catalyse ice formation can dramatically reduce the amount of supercooled water in clouds; hence we argue that we need a concerted effort to improve our understanding of these ice-nucleating particles if we are to improve our predictions of climate change.
Jane P. Mulcahy, Colin Johnson, Colin G. Jones, Adam C. Povey, Catherine E. Scott, Alistair Sellar, Steven T. Turnock, Matthew T. Woodhouse, Nathan Luke Abraham, Martin B. Andrews, Nicolas Bellouin, Jo Browse, Ken S. Carslaw, Mohit Dalvi, Gerd A. Folberth, Matthew Glover, Daniel P. Grosvenor, Catherine Hardacre, Richard Hill, Ben Johnson, Andy Jones, Zak Kipling, Graham Mann, James Mollard, Fiona M. O'Connor, Julien Palmiéri, Carly Reddington, Steven T. Rumbold, Mark Richardson, Nick A. J. Schutgens, Philip Stier, Marc Stringer, Yongming Tang, Jeremy Walton, Stephanie Woodward, and Andrew Yool
Geosci. Model Dev., 13, 6383–6423, https://doi.org/10.5194/gmd-13-6383-2020, https://doi.org/10.5194/gmd-13-6383-2020, 2020
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Aerosols are an important component of the Earth system. Here, we comprehensively document and evaluate the aerosol schemes as implemented in the physical and Earth system models, HadGEM3-GC3.1 and UKESM1. This study provides a useful characterisation of the aerosol climatology in both models, facilitating the understanding of the numerous aerosol–climate interaction studies that will be conducted for CMIP6 and beyond.
Daniel P. Grosvenor and Kenneth S. Carslaw
Atmos. Chem. Phys., 20, 15681–15724, https://doi.org/10.5194/acp-20-15681-2020, https://doi.org/10.5194/acp-20-15681-2020, 2020
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Particles arising from human activity interact with clouds and affect how much of the Sun's energy is reflected away. Lack of understanding about how to represent this in models leads to large uncertainties in climate predictions. We quantify cloud responses to particles in the latest UK Met Office climate model over the North Atlantic Ocean, showing that, in contrast to suggestions elsewhere, increases in cloud coverage and thickness are important over large areas.
Lukas O. Muser, Gholam Ali Hoshyaripour, Julia Bruckert, Ákos Horváth, Elizaveta Malinina, Sandra Wallis, Fred J. Prata, Alexei Rozanov, Christian von Savigny, Heike Vogel, and Bernhard Vogel
Atmos. Chem. Phys., 20, 15015–15036, https://doi.org/10.5194/acp-20-15015-2020, https://doi.org/10.5194/acp-20-15015-2020, 2020
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Volcanic aerosols endanger aircraft and thus disrupt air travel globally. For aviation safety, it is vital to know the location and lifetime of such aerosols in the atmosphere. Here we show that the interaction of volcanic particles with each other eventually reduces their atmospheric lifetime. Moreover, we demonstrate that sunlight heats these particles, which lifts them several kilometers in the atmosphere. These findings support a more reliable forecast of volcanic aerosol dispersion.
Sandip S. Dhomse, Graham W. Mann, Juan Carlos Antuña Marrero, Sarah E. Shallcross, Martyn P. Chipperfield, Kenneth S. Carslaw, Lauren Marshall, N. Luke Abraham, and Colin E. Johnson
Atmos. Chem. Phys., 20, 13627–13654, https://doi.org/10.5194/acp-20-13627-2020, https://doi.org/10.5194/acp-20-13627-2020, 2020
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We confirm downward adjustment of SO2 emission to simulate the Pinatubo aerosol cloud with aerosol microphysics models. Similar adjustment is also needed to simulate the El Chichón and Agung volcanic cloud, indicating potential missing removal or vertical redistribution process in models. Important inhomogeneities in the CMIP6 forcing datasets after Agung and El Chichón eruptions are difficult to reconcile. Quasi-biennial oscillation plays an important role in modifying stratospheric warming.
Hamish Gordon, Paul R. Field, Steven J. Abel, Paul Barrett, Keith Bower, Ian Crawford, Zhiqiang Cui, Daniel P. Grosvenor, Adrian A. Hill, Jonathan Taylor, Jonathan Wilkinson, Huihui Wu, and Ken S. Carslaw
Atmos. Chem. Phys., 20, 10997–11024, https://doi.org/10.5194/acp-20-10997-2020, https://doi.org/10.5194/acp-20-10997-2020, 2020
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The Met Office's Unified Model is widely used both for weather forecasting and climate prediction. We present the first version of the model in which both aerosol and cloud particle mass and number concentrations are allowed to evolve separately and independently, which is important for studying how aerosols affect weather and climate. We test the model against aircraft observations near Ascension Island in the Atlantic, focusing on how aerosols can "activate" to become cloud droplets.
Cited articles
Adams-Selin, R. D., van den Heever, S. C., and Johnson, R. H.: Impact of Graupel Parameterization Schemes on Idealized Bow Echo Simulations, Mon. Weather Rev., 141, 1241–1262, https://doi.org/10.1175/MWR-D-12-00064.1, 2013. a
Baldauf, M., Seifert, A., Förstner, J., Majewski, D., Raschendorfer, M., and Reinhardt, T.: Operational Convective-Scale Numerical Weather Prediction with the COSMO Model: Description and Sensitivities, Mon. Weather Rev., 139, 3887–3905, https://doi.org/10.1175/MWR-D-10-05013.1, 2011. a
Barrett, A. I., Wellmann, C., Seifert, A., Hoose, C., Vogel, B., and Kunz, M.: One Step at a Time: How Model Time Step Significantly Affects Convection-Permitting Simulations, J. Adv. Model. Earth Sy., 11, 641–658, https://doi.org/10.1029/2018MS001418, 2019. a, b
Bastos, L. S. and O'Hagan, A.: Diagnostics for Gaussian Process Emulators, Technometrics, 51, 425–438, https://doi.org/10.1198/TECH.2009.08019, 2009. a
Bigg, E. K.: The formation of atmospheric ice crystals by the freezing of droplets, Q. J. Roy. Meteor. Soc., 79, 510–519, https://doi.org/10.1002/qj.49707934207, 1953. a
Brooks, H.: Operational implications of the sensitivity of modeled
thunderstorms to thermal perturbations, Fourth AES/CMOS Workshop on
Operational Meteorology, Whistler, B.C., Canada, 15–18 September 1992, 110, 398–407, 1992. a
Chen, Q., Fan, J., Hagos, S., Gustafson Jr., W. I., and Berg, L. K.: Roles of wind shear at different vertical levels: Cloud system organization and properties, J. Geophys. Res. Atmos., 120, 6551–6574, https://doi.org/10.1002/2015JD023253, 2015. a
Connolly, P. J., Choularton, T. W., Gallagher, M. W., Bower, K. N., Flynn, M. J., and Whiteway, J. A.: Cloud-resolving simulations of intense tropical Hector thunderstorms: Implications for aerosol–cloud interactions, Q. J. Roy. Meteor. Soc., 132, 3079–3106, https://doi.org/10.1256/qj.05.86, 2006. a
Davies-Jones, R.: A review of supercell and tornado dynamics, Atmos. Res., 158–159, 274–291, https://doi.org/10.1016/j.atmosres.2014.04.007, 2015. a
DeMott, P. J., Prenni, A. J., Liu, X., Kreidenweis, S. M., Petters, M. D., Twohy, C. H., Richardson, M. S., Eidhammer, T., and Rogers, D. C.: Predicting global atmospheric ice nuclei distributions and their impacts on climate, P. Natl. Acad. Sci. USA, 107, 11217–11222, https://doi.org/10.1073/pnas.0910818107, 2010. a
Fan, J., Tianle, Y., M., C. J., Steven, G., Alexander, K., Ruby, L. L., Zhanqing, L., J., M. V., and Mikhail, O.: Dominant role by vertical wind shear in regulating aerosol effects on deep convective clouds, J. Geophys. Res., 114, D22206, https://doi.org/10.1029/2009JD012352, 2009. a
Fan, J., Leung, L. R., Rosenfeld, D., Chen, Q., Li, Z., Zhang, J., and Yan, H.: Microphysical effects determine macrophysical response for aerosol impacts on deep convective clouds, P. Natl. Acad. Sci. USA, 110, E4581–E4590, https://doi.org/10.1073/pnas.1316830110, 2013. a, b, c, d
Gal-Chen, T. and Somerville, R. C.: On the use of a coordinate transformation for the solution of the Navier-Stokes equations, J. Comput. Phys., 17, 209–228, https://doi.org/10.1016/0021-9991(75)90037-6, 1975. a
Gilmore, M. S., Straka, J. M., and Rasmussen, E. N.: Precipitation Uncertainty Due to Variations in Precipitation Particle Parameters within a Simple Microphysics Scheme, Mon. Weather Rev., 132, 2610–2627, https://doi.org/10.1175/MWR2810.1, 2004. a
Glassmeier, F., Hoffmann, F., Johnson, J. S., Yamaguchi, T., Carslaw, K. S., and Feingold, G.: An emulator approach to stratocumulus susceptibility, Atmos. Chem. Phys., 19, 10191–10203, https://doi.org/10.5194/acp-19-10191-2019, 2019. a
Hallett, J. and Mossop, S. C.: Production of secondary ice particles during the riming process, Nature, 249, 26–28, https://doi.org/10.1038/249026a0, 1974. a, b, c
Heymsfield, A., Szakáll, M., Jost, A., Giammanco, I., and Wright, R.: A Comprehensive Observational Study of Graupel and Hail Terminal Velocity, Mass Flux, and Kinetic Energy, J. Atmos. Sci., 75, 3861–3885, https://doi.org/10.1175/JAS-D-18-0035.1, 2018. a
Huang, W., Bao, J.-W., Zhang, X., and Chen, B.: Comparison of the Vertical Distributions of Cloud Properties from Idealized Extratropical Deep Convection Simulations Using Various Horizontal Resolutions, Mon. Weather Rev., 146, 833–851, https://doi.org/10.1175/MWR-D-17-0162.1, 2018. a
Huffman, P. J. and Vali, G.: The Effect of Vapor Depletion on Ice Nucleus Measurements with Membrane Filters, J. Appl. Meteorol., 12, 1018–1024, https://doi.org/10.1175/1520-0450(1973)012<1018:TEOVDO>2.0.CO;2, 1973. a
Igel, A. L. and van den Heever, S. C.: The Importance of the Shape of Cloud Droplet Size Distributions in Shallow Cumulus Clouds. Part I: Bin Microphysics Simulations, J. Atmos. Sci., 74, 249–258, https://doi.org/10.1175/JAS-D-15-0382.1, 2017a. a
Igel, A. L. and van den Heever, S. C.: The Importance of the Shape of Cloud Droplet Size Distributions in Shallow Cumulus Clouds. Part II: Bulk Microphysics Simulations, J. Atmos. Sci., 74, 259–273, https://doi.org/10.1175/JAS-D-15-0383.1, 2017b. a, b, c
Igel, A. L., van den Heever, S. C., and Johnson, J. S.: Meteorological and Land Surface Properties Impacting Sea Breeze Extent and Aerosol Distribution in a Dry Environment, J. Geophys. Res.-Atmos., 123, 22–37, https://doi.org/10.1002/2017JD027339, 2018. a
Joos, H. and Wernli, H.: Influence of microphysical processes on the potential vorticity development in a warm conveyor belt: a case-study with the limited-area model COSMO, Q. J. Roy. Meteor. Soc., 138, 407–418, https://doi.org/10.1002/qj.934, 2011. a, b
Khain, A., Rosenfeld, D., Pokrovsky, A., Blahak, U., and Ryzhkov, A.: The role of CCN in precipitation and hail in a mid-latitude storm as seen in simulations using a spectral (bin) microphysics model in a 2D dynamic frame, Atmos. Res., 99, 129–146, https://doi.org/10.1016/j.atmosres.2010.09.015, 2011. a
Knight, N. C. and Heymsfield, A. J.: Measurement and Interpretation of Hailstone Density and Terminal Velocity, J. Atmos. Sci., 40, 1510–1516, https://doi.org/10.1175/1520-0469(1983)040<1510:MAIOHD>2.0.CO;2, 1983. a, b, c
Lebo, Z. J., Morrison, H., and Seinfeld, J. H.: Are simulated aerosol-induced effects on deep convective clouds strongly dependent on saturation adjustment?, Atmos. Chem. Phys., 12, 9941–9964, https://doi.org/10.5194/acp-12-9941-2012, 2012. a
Lee, L. A., Carslaw, K. S., Pringle, K. J., Mann, G. W., and Spracklen, D. V.: Emulation of a complex global aerosol model to quantify sensitivity to uncertain parameters, Atmos. Chem. Phys., 11, 12253–12273, https://doi.org/10.5194/acp-11-12253-2011, 2011. a
Lee, L. A., Pringle, K. J., Reddington, C. L., Mann, G. W., Stier, P., Spracklen, D. V., Pierce, J. R., and Carslaw, K. S.: The magnitude and causes of uncertainty in global model simulations of cloud condensation nuclei, Atmos. Chem. Phys., 13, 8879–8914, https://doi.org/10.5194/acp-13-8879-2013, 2013. a
Lee, S. S., Donner, L. J., Phillips, V. T. J., and Ming, Y.: The dependence of aerosol effects on clouds and precipitation on cloud-system organization, shear and stability, J. Geophys. Res., 113, D16202, https://doi.org/10.1029/2007JD009224, 2008. a, b, c, d
Locatelli, J. D. and Hobbs, P. V.: Fall speeds and masses of solid precipitation particles, J. Geophys. Res., 79, 2185–2197, https://doi.org/10.1029/JC079i015p02185, 1974. a
Loftus, A. and Cotton, W.: Examination of CCN impacts on hail in a simulated supercell storm with triple-moment hail bulk microphysics, Atmos. Res., 147–148, 183–204, https://doi.org/10.1016/j.atmosres.2014.04.017, 2014. a, b, c, d
Morris, M. D. and Mitchell, T. J.: Exploratory designs for computational experiments, J. Stat. Plan. Infer., 43, 381–402, https://doi.org/10.1016/0378-3758(94)00035-T, 1995. a
Morrison, H. and Milbrandt, J.: Comparison of Two-Moment Bulk Microphysics Schemes in Idealized Supercell Thunderstorm Simulations, Mon. Weather Rev., 139, 1103–1130, https://doi.org/10.1175/2010MWR3433.1, 2011. a
Morrison, H., Curry, J. A., Shupe, M. D., and Zuidema, P.: A New Double-Moment Microphysics Parameterization for Application in Cloud and Climate Models. Part II: Single-Column Modeling of Arctic Clouds, J. Atmos. Sci., 62, 1678–1693, https://doi.org/10.1175/JAS3447.1, 2005. a
Morrison, H., Thompson, G., and Tatarskii, V.: Impact of Cloud Microphysics on the Development of Trailing Stratiform Precipitation in a Simulated Squall Line: Comparison of One- and Two-Moment Schemes, Mon. Weather Rev., 137, 991–1007, https://doi.org/10.1175/2008MWR2556.1, 2009. a
Oakley, J. E. and O'Hagan, A.: Probabilistic sensitivity analysis of complex models: a Bayesian approach, J. Roy. Stat. Soc. B, 66, 751–769, https://doi.org/10.1111/j.1467-9868.2004.05304.x, 2004. a, b
O'Hagan, A.: Bayesian analysis of computer code outputs: A tutorial, Reliab. Eng. Syst. Safe., 91, 1290–1300, https://doi.org/10.1016/j.ress.2005.11.025, 2006. a, b, c
Posselt, D. J. and Vukicevic, T.: Robust Characterization of Model Physics Uncertainty for Simulations of Deep Moist Convection, Mon. Weather Rev., 138, 1513–1535, https://doi.org/10.1175/2009MWR3094.1, 2010. a
Potvin, C. K. and Flora, M. L.: Sensitivity of Idealized Supercell Simulations to Horizontal Grid Spacing: Implications for Warn-on-Forecast, Mon. Weather Rev., 143, 2998–3024, https://doi.org/10.1175/MWR-D-14-00416.1, 2015. a
Rasmussen, C. E.: Gaussian Processes in Machine Learning, in: Advanced Lectures on Machine Learning: ML Summer Schools 2003, Canberra, Australia, 2–14 February 2003, Tübingen, Germany, 4–16 August 2003, Revised Lectures, edited by: Bousquet, O., von Luxburg, U., and Rätsch, G., Springer Berlin Heidelberg, Berlin, Heidelberg, 63–71, https://doi.org/10.1007/978-3-540-28650-9_4, 2004. a
Rasmussen, C. E. and Williams, C. K. I.: Gaussian Processes for Machine Learning, MIT Press, London, 2006. a
Rosenfeld, D., Lohmann, U., Raga, G. B., O'Dowd, C. D., Kulmala, M., Fuzzi, S., Reissell, A., and Andreae, M. O.: Flood or Drought: How Do Aerosols Affect Precipitation?, Science, 321, 1309–1313, https://doi.org/10.1126/science.1160606, 2008. a, b
Saltelli, A., Tarantola, S., and Chan, K. P.-S.: A Quantitative Model-Independent Method for Global Sensitivity Analysis of Model Output, Technometrics, 41, 39–56, https://doi.org/10.1080/00401706.1999.10485594, 1999. a, b
Schättler, U., Doms, G., and Schraff, C.: A description of the nonhydrostatic regional COSMO-model, Part VII: User's Guide, available at: http://www.cosmo-model.org/content/model/documentation/core/default.htm (last access: 9 February 2020), 2016. a
Schneider, L., Barthlott, C., Hoose, C., and Barrett, A. I.: Relative impact of aerosol, soil moisture, and orography perturbations on deep convection, Atmos. Chem. Phys., 19, 12343–12359, https://doi.org/10.5194/acp-19-12343-2019, 2019. a
Segal, Y. and Khain, A.: Dependence of droplet concentration on aerosol conditions in different cloud types: Application to droplet concentration parameterization of aerosol conditions, J. Geophys. Res., 111, D15204, https://doi.org/10.1029/2005JD006561, 2006. a
Seifert, A. and Beheng, K. D.: A two-moment cloud microphysics parameterization for mixed-phase clouds. Part 1: Model description, Meteorol. Atmos. Phys., 92, 45–66, https://doi.org/10.1007/s00703-005-0112-4, 2006. a, b, c, d
Storer, R. L., van den Heever, S. C., and Stephens, G. L.: Modeling Aerosol Impacts on Convective Storms in Different Environments, J. Atmos. Sci., 67, 3904–3915, https://doi.org/10.1175/2010JAS3363.1, 2010. a, b, c
Tao, W., Chen, J., Li, Z., Wang, C., and Zhang, C.: Impact of aerosols on convective clouds and precipitation, Rev. Geophys., 50, RG2001, https://doi.org/10.1029/2011RG000369, 2012. a
Thompson, G., Rasmussen, R. M., and Manning, K.: Explicit Forecasts of Winter Precipitation Using an Improved Bulk Microphysics Scheme. Part I: Description and Sensitivity Analysis, Mon. Weather Rev., 132, 519–542, https://doi.org/10.1175/1520-0493(2004)132<0519:EFOWPU>2.0.CO;2, 2004. a
Thompson, G., Field, P. R., Rasmussen, R. M., and Hall, W. D.: Explicit Forecasts of Winter Precipitation Using an Improved Bulk Microphysics Scheme. Part II: Implementation of a New Snow Parameterization, Mon. Weather Rev., 136, 5095–5115, https://doi.org/10.1175/2008MWR2387.1, 2008. a
Wang, Y., Fan, J., Zhang, R., Leung, L. R., and Franklin, C.: Improving bulk microphysics parameterizations in simulations of aerosol effects, J. Geophys. Res.-Atmos., 118, 5361–5379, https://doi.org/10.1002/jgrd.50432, 2013.
a
Weisman, M. L. and Klemp, J. B.: The Structure and Classification of Numerically Simulated Convective Storms in Directionally Varying Wind Shears, Mon. Weather Rev., 112, 2479–2498, https://doi.org/10.1175/1520-0493(1984)112<2479:TSACON>2.0.CO;2, 1984. a
Weisman, M. L. and Rotunno, R.: The Use of Vertical Wind Shear versus Helicity in Interpreting Supercell Dynamics, J. Atmos. Sci., 57, 1452–1472, https://doi.org/10.1175/1520-0469(2000)057<1452:TUOVWS>2.0.CO;2, 2000. a, b
Wellmann, C., Barrett, A. I., Johnson, J. S., Kunz, M., Vogel, B., Carslaw, K. S., and Hoose, C.: Using Emulators to Understand the Sensitivity of Deep Convective Clouds and Hail to Environmental Conditions, J. Adv. Model. Earth Sy., 10, 3103–3122, https://doi.org/10.1029/2018MS001465, 2018. a, b, c, d, e, f, g, h, i, j, k, l
Wellmann, M.-C. M.: Using statistical emulation for sensitivity studies of deep convective clouds, PhD thesis, Karlsruhe Institute of Technology (KIT), Karlsruhe, https://doi.org/10.5445/IR/1000091102, 2019a. a
Wellmann, M.-C.: Training data and emulators for the analysis of sensitivity of deep convective clouds and hail to environmental conditions and microphysics, KITopen, https://doi.org/10.5445/IR/1000099232, 2019b. a
White, B., Gryspeerdt, E., Stier, P., Morrison, H., Thompson, G., and Kipling, Z.: Uncertainty from the choice of microphysics scheme in convection-permitting models significantly exceeds aerosol effects, Atmos. Chem. Phys., 17, 12145–12175, https://doi.org/10.5194/acp-17-12145-2017, 2017. a
Yang, H., Xiao, H., Guo, C., Wen, G., Tang, Q., and Sun, Y.: Comparison of aerosol effects on simulated spring and summer hailstorm clouds, Adv. Atmos. Sci., 34, 877–893, https://doi.org/10.1007/s00376-017-6138-y, 2017. a, b
Yuter, S. E., Kingsmill, D. E., Nance, L. B., and Löffler-Mang, M.: Observations of Precipitation Size and Fall Speed Characteristics within Coexisting Rain and Wet Snow, J. Appl. Meteorol. Climat., 45, 1450–1464, https://doi.org/10.1175/JAM2406.1, 2006. a, b
Short summary
Severe hailstorms may cause damage to buildings and crops. Thus, the forecast of numerical weather prediction (NWP) models should be as reliable as possible.
Using statistical emulation, we identify those model input parameters describing environmental conditions and cloud microphysics which lead to large uncertainties in the prediction of deep convection. We find that the impact of the input parameters on the uncertainty depends on the considered output variable.
Severe hailstorms may cause damage to buildings and crops. Thus, the forecast of numerical...
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