Articles | Volume 17, issue 15
https://doi.org/10.5194/acp-17-9365-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-9365-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
07 Aug 2017
Research article |
| 07 Aug 2017
Temporal characteristics of atmospheric ammonia and nitrogen dioxide over China based on emission data, satellite observations and atmospheric transport modeling since 1980
Lei Liu
Jiangsu Provincial Key Laboratory of Geographic Information Science
and Technology, International Institute for Earth System Science, Nanjing
University, Nanjing 210023, China
Xiuying Zhang
CORRESPONDING AUTHOR
Jiangsu Provincial Key Laboratory of Geographic Information Science
and Technology, International Institute for Earth System Science, Nanjing
University, Nanjing 210023, China
College of Resources and Environmental Sciences, Centre for
Resources, Environment and Food Security, Key Lab of Plant-Soil Interactions
of MOE, China Agricultural University, Beijing 100193, China
Xuejun Liu
College of Resources and Environmental Sciences, Centre for
Resources, Environment and Food Security, Key Lab of Plant-Soil Interactions
of MOE, China Agricultural University, Beijing 100193, China
Air Quality Division, Arizona Department of Environmental Quality,
Phoenix, AZ 85007, USA
Xuehe Lu
Jiangsu Provincial Key Laboratory of Geographic Information Science
and Technology, International Institute for Earth System Science, Nanjing
University, Nanjing 210023, China
Yuehan Zhang
School of Atmospheric Sciences, Nanjing University, Nanjing, China
Wuting Zhang
Jiangsu Provincial Key Laboratory of Geographic Information Science
and Technology, International Institute for Earth System Science, Nanjing
University, Nanjing 210023, China
Jiangsu Center for Collaborative Innovation in Geographical
Information Resource Development and Application, Nanjing 210023, China
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Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-770, https://doi.org/10.5194/acp-2017-770, 2017
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Atmos. Chem. Phys., 16, 1401–1416, https://doi.org/10.5194/acp-16-1401-2016, https://doi.org/10.5194/acp-16-1401-2016, 2016
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W. Xu, X. S. Luo, Y. P. Pan, L. Zhang, A. H. Tang, J. L. Shen, Y. Zhang, K. H. Li, Q. H. Wu, D. W. Yang, Y. Y. Zhang, J. Xue, W. Q. Li, Q. Q. Li, L. Tang, S. H. Lu, T. Liang, Y. A. Tong, P. Liu, Q. Zhang, Z. Q. Xiong, X. J. Shi, L. H. Wu, W. Q. Shi, K. Tian, X. H. Zhong, K. Shi, Q. Y. Tang, L. J. Zhang, J. L. Huang, C. E. He, F. H. Kuang, B. Zhu, H. Liu, X. Jin, Y. J. Xin, X. K. Shi, E. Z. Du, A. J. Dore, S. Tang, J. L. Collett Jr., K. Goulding, Y. X. Sun, J. Ren, F. S. Zhang, and X. J. Liu
Atmos. Chem. Phys., 15, 12345–12360, https://doi.org/10.5194/acp-15-12345-2015, https://doi.org/10.5194/acp-15-12345-2015, 2015
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M. Van Damme, L. Clarisse, E. Dammers, X. Liu, J. B. Nowak, C. Clerbaux, C. R. Flechard, C. Galy-Lacaux, W. Xu, J. A. Neuman, Y. S. Tang, M. A. Sutton, J. W. Erisman, and P. F. Coheur
Atmos. Meas. Tech., 8, 1575–1591, https://doi.org/10.5194/amt-8-1575-2015, https://doi.org/10.5194/amt-8-1575-2015, 2015
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Volcanic SO2 layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
Spaceborne tropospheric nitrogen dioxide (NO2) observations from 2005–2020 over the Yangtze River Delta (YRD), China: variabilities, implications, and drivers
Novel assessment of numerical forecasting model relative humidity with satellite probabilistic estimates
Influence of springtime atmospheric circulation types on the distribution of air pollutants in the Arctic
Technical note: Evaluation of profile retrievals of aerosols and trace gases for MAX-DOAS measurements under different aerosol scenarios based on radiative transfer simulations
Diurnal evolution of total column and surface atmospheric ammonia in the megacity of Paris, France, during an intense springtime pollution episode
The reduction in C2H6 from 2015 to 2020 over Hefei, eastern China, points to air quality improvement in China
Mapping the drivers of formaldehyde (HCHO) variability from 2015 to 2019 over eastern China: insights from Fourier transform infrared observation and GEOS-Chem model simulation
The impact of Los Angeles Basin pollution and stratospheric intrusions on the surrounding San Gabriel Mountains as seen by surface measurements, lidar, and numerical models
Sudden changes in nitrogen dioxide emissions over Greece due to lockdown after the outbreak of COVID-19
Monitoring CO emissions of the metropolis Mexico City using TROPOMI CO observations
Pollution trace gas distributions and their transport in the Asian monsoon upper troposphere and lowermost stratosphere during the StratoClim campaign 2017
Spatial distribution of enhanced BrO and its relation to meteorological parameters in Arctic and Antarctic sea ice regions
Trends of atmospheric water vapour in Switzerland from ground-based radiometry, FTIR and GNSS data
A Raman lidar tropospheric water vapour climatology and height-resolved trend analysis over Payerne, Switzerland
The potential of Orbiting Carbon Observatory-2 data to reduce the uncertainties in CO2 surface fluxes over Australia using a variational assimilation scheme
Observing carbon dioxide emissions over China's cities and industrial areas with the Orbiting Carbon Observatory-2
Observational evidence of moistening the lowermost stratosphere via isentropic mixing across the subtropical jet
Fourier transform infrared time series of tropospheric HCN in eastern China: seasonality, interannual variability, and source attribution
NH3 emissions from large point sources derived from CrIS and IASI satellite observations
Diurnal cycle of short-term fluctuations of integrated water vapour above Switzerland
Retrieval of total column and surface NO2 from Pandora zenith-sky measurements
MAX-DOAS measurements of tropospheric NO2 and HCHO in Nanjing and a comparison to ozone monitoring instrument observations
Consistency and representativeness of integrated water vapour from ground-based GPS observations and ERA-Interim reanalysis
Towards monitoring localized CO2 emissions from space: co-located regional CO2 and NO2 enhancements observed by the OCO-2 and S5P satellites
Variability of bulk water vapor content in the marine cloudy boundary layers from microwave and near-infrared imagery
Trends and trend reversal detection in 2 decades of tropospheric NO2 satellite observations
Satellite-derived sulfur dioxide (SO2) emissions from the 2014–2015 Holuhraun eruption (Iceland)
Emissions of methane in Europe inferred by total column measurements
On the interpretation of upper-tropospheric humidity based on a second-order retrieval from infrared radiances
Steffen Vanselow, Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Hartmut Boesch, and John P. Burrows
Atmos. Chem. Phys., 24, 10441–10473, https://doi.org/10.5194/acp-24-10441-2024, https://doi.org/10.5194/acp-24-10441-2024, 2024
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We developed an algorithm to automatically detect persistent methane source regions, to quantify their emissions and to determine their source types, by analyzing TROPOMI data from 2018–2021. The over 200 globally detected natural and anthropogenic source regions include small-scale point sources such as individual coal mines and larger-scale source regions such as wetlands and large oil and gas fields.
Debora Griffin, Jack Chen, Kerry Anderson, Paul Makar, Chris A. McLinden, Enrico Dammers, and Andre Fogal
Atmos. Chem. Phys., 24, 10159–10186, https://doi.org/10.5194/acp-24-10159-2024, https://doi.org/10.5194/acp-24-10159-2024, 2024
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Satellite-derived CO emissions provide new insights into the understanding of global CO emission rates from wildfires. We use TROPOMI satellite data to create a global inventory database of wildfire CO emissions. These satellite-derived wildfire emissions are used for the evaluation and improvement of existing fire emission inventories and to examine how the wildfire CO emissions have changed over the past 2 decades.
Matías Osorio, Alejandro Agesta, Tim Bösch, Nicolás Casaballe, Andreas Richter, Leonardo M. A. Alvarado, and Erna Frins
Atmos. Chem. Phys., 24, 7447–7465, https://doi.org/10.5194/acp-24-7447-2024, https://doi.org/10.5194/acp-24-7447-2024, 2024
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This study concerns the detection and quantification of long-transport emissions of a biomass burning event, which represents a major source of air pollutants, due to the release of large amounts of aerosols and chemical species into the atmosphere. The quantification was done using ground-based observations (which play an important role in assessing the abundance of trace gases and aerosols) over Montevideo (Uruguay) and using satellite observations.
Qiansi Tu, Frank Hase, Kai Qin, Jason Blake Cohen, Farahnaz Khosrawi, Xinrui Zou, Matthias Schneider, and Fan Lu
Atmos. Chem. Phys., 24, 4875–4894, https://doi.org/10.5194/acp-24-4875-2024, https://doi.org/10.5194/acp-24-4875-2024, 2024
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Four-year satellite observations of XCH4 are used to derive CH4 emissions in three regions of China’s coal-rich Shanxi province. The wind-assigned anomalies for two opposite wind directions are calculated, and the estimated emission rates are comparable to the current bottom-up inventory but lower than the CAMS and EDGAR inventories. This research enhances the understanding of emissions in Shanxi and supports climate mitigation strategies by validating emission inventories.
Paul S. Jeffery, James R. Drummond, Jiansheng Zou, and Kaley A. Walker
Atmos. Chem. Phys., 24, 4253–4263, https://doi.org/10.5194/acp-24-4253-2024, https://doi.org/10.5194/acp-24-4253-2024, 2024
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The MOPITT instrument has been monitoring carbon monoxide (CO) since March 2000. This dataset has been used for many applications; however, episodic emission events, which release large amounts of CO into the atmosphere, are a major source of uncertainty. This study presents a method for identifying these events by determining measurements that are unlikely to have typically arisen. The distribution and frequency of these flagged measurements in the MOPITT dataset are presented and discussed.
Ailish M. Graham, Richard J. Pope, Martyn P. Chipperfield, Sandip S. Dhomse, Matilda Pimlott, Wuhu Feng, Vikas Singh, Ying Chen, Oliver Wild, Ranjeet Sokhi, and Gufran Beig
Atmos. Chem. Phys., 24, 789–806, https://doi.org/10.5194/acp-24-789-2024, https://doi.org/10.5194/acp-24-789-2024, 2024
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Our paper uses novel satellite datasets and high-resolution emissions datasets alongside a back-trajectory model to investigate the balance of local and external sources influencing NOx air pollution changes in Delhi. We find in the post-monsoon season that NOx from local and non-local transport emissions contributes most to poor air quality in Delhi. Therefore, air quality mitigation strategies in Delhi and surrounding regions are used to control this issue.
Camille Viatte, Nadir Guendouz, Clarisse Dufaux, Arjan Hensen, Daan Swart, Martin Van Damme, Lieven Clarisse, Pierre Coheur, and Cathy Clerbaux
Atmos. Chem. Phys., 23, 15253–15267, https://doi.org/10.5194/acp-23-15253-2023, https://doi.org/10.5194/acp-23-15253-2023, 2023
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Ammonia (NH3) is an important air pollutant which, as a precursor of fine particulate matter, raises public health concerns. Models have difficulty predicting events of pollution associated with NH3 since ground-based observations of this gas are still relatively sparse and difficult to implement. We present the first relatively long (2.5 years) and continuous record of hourly NH3 concentrations in Paris to determine its temporal variabilities at different scales to unravel emission sources.
Hirofumi Ohyama, Matthias M. Frey, Isamu Morino, Kei Shiomi, Masahide Nishihashi, Tatsuya Miyauchi, Hiroko Yamada, Makoto Saito, Masanobu Wakasa, Thomas Blumenstock, and Frank Hase
Atmos. Chem. Phys., 23, 15097–15119, https://doi.org/10.5194/acp-23-15097-2023, https://doi.org/10.5194/acp-23-15097-2023, 2023
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We conducted a field campaign for CO2 column measurements in the Tokyo metropolitan area with three ground-based Fourier transform spectrometers. The model simulations using prior CO2 fluxes were generally in good agreement with the observations. We developed an urban-scale inversion system in which spatially resolved CO2 fluxes and a scaling factor of large point source emissions were estimated. The posterior total CO2 emissions agreed with emission inventories within the posterior uncertainty.
Chris Wilson, Brian J. Kerridge, Richard Siddans, David P. Moore, Lucy J. Ventress, Emily Dowd, Wuhu Feng, Martyn P. Chipperfield, and John J. Remedios
EGUsphere, https://doi.org/10.5194/egusphere-2023-1652, https://doi.org/10.5194/egusphere-2023-1652, 2023
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The leaks from the Nord Stream gas pipelines in September 2022 released a large amount of methane (CH4) to the atmosphere. We provide observational data from a satellite instrument, IASI, that shows a large CH4 plume over the North Sea off the coast of Scandinavia. We use this, together with atmospheric models, to quantify the CH4 leaked into the atmosphere from the pipelines. We find that 215–390 Gg CH4 was emitted, making this the largest individual fossil fuel-related CH4 leak on record.
Xi Shao, Shu-Peng Ho, Xin Jing, Xinjia Zhou, Yong Chen, Tung-Chang Liu, Bin Zhang, and Jun Dong
Atmos. Chem. Phys., 23, 14187–14218, https://doi.org/10.5194/acp-23-14187-2023, https://doi.org/10.5194/acp-23-14187-2023, 2023
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Atmospheric water vapor plays an essential role in the global energy balance, hydrological cycle, and climate system. This paper characterizes and compares the global, latitudinal, and regional variabilities of COSMIC and ERA5 water vapor distribution, as well as the seasonality and long-term trends at selected pressure levels from 2007 to 2018. Evaluation of spatiotemporal variabilities of atmospheric water vapor ensures the qualities of COSMIC and reanalysis water vapor for climate studies.
Anthony Rey-Pommier, Frédéric Chevallier, Philippe Ciais, Jonilda Kushta, Theodoros Christoudias, I. Safak Bayram, and Jean Sciare
Atmos. Chem. Phys., 23, 13565–13583, https://doi.org/10.5194/acp-23-13565-2023, https://doi.org/10.5194/acp-23-13565-2023, 2023
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We use four years (2019–2022) of TROPOMI NO2 data to map NOx emissions in Qatar. We estimate average monthly emissions for the country and industrial facilities and derive an emission factor for the power sector. Monthly emissions have a weekly cycle reflecting the social norms in Qatar and an annual cycle consistent with the electricity production by gas-fired power plants. Their mean value is lower than the NOx emissions in global inventories but similar to the emissions reported for 2007.
Daniel A. Potts, Roger Timmis, Emma J. S. Ferranti, and Joshua D. Vande Hey
Atmos. Chem. Phys., 23, 4577–4593, https://doi.org/10.5194/acp-23-4577-2023, https://doi.org/10.5194/acp-23-4577-2023, 2023
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With the launch of the TROPOspheric Monitoring Instrument (TROPOMI) in 2017, it is now possible to observe pollutants emitted from individual industrial facilities on a daily basis around the globe. By using observations of nitrogen dioxide (NO2) from 16 different industrial sites, we show how the Coriolis effect influences the trajectory of these emission plumes as well as how the additional curvature can lead to a substantial underestimation of the calculated emissions.
Peng Yuan, Roeland Van Malderen, Xungang Yin, Hannes Vogelmann, Weiping Jiang, Joseph Awange, Bernhard Heck, and Hansjörg Kutterer
Atmos. Chem. Phys., 23, 3517–3541, https://doi.org/10.5194/acp-23-3517-2023, https://doi.org/10.5194/acp-23-3517-2023, 2023
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Water vapour plays an important role in various weather and climate processes. However, due to its large spatiotemporal variability, its high-accuracy quantification remains a challenge. In this study, 20+ years of GPS-derived integrated water vapour (IWV) retrievals in Europe were obtained. They were then used to characterise the temporal features of Europe's IWV and assess six atmospheric reanalyses. Results show that ERA5 outperforms the other reanalyses at most temporal scales.
Jing Wei, Zhanqing Li, Jun Wang, Can Li, Pawan Gupta, and Maureen Cribb
Atmos. Chem. Phys., 23, 1511–1532, https://doi.org/10.5194/acp-23-1511-2023, https://doi.org/10.5194/acp-23-1511-2023, 2023
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This study estimated the daily seamless 10 km ambient gaseous pollutants (NO2, SO2, and CO) across China using machine learning with extensive input variables measured on monitors, satellites, and models. Our dataset yields a high data quality via cross-validation at varying spatiotemporal scales and outperforms most previous related studies, making it most helpful to future (especially short-term) air pollution and environmental health-related studies.
Camille Viatte, Rimal Abeed, Shoma Yamanouchi, William C. Porter, Sarah Safieddine, Martin Van Damme, Lieven Clarisse, Beatriz Herrera, Michel Grutter, Pierre-Francois Coheur, Kimberly Strong, and Cathy Clerbaux
Atmos. Chem. Phys., 22, 12907–12922, https://doi.org/10.5194/acp-22-12907-2022, https://doi.org/10.5194/acp-22-12907-2022, 2022
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Large cities can experience high levels of fine particulate matter (PM2.5) pollution linked to ammonia (NH3) mainly emitted from agricultural activities. Using a combination of PM2.5 and NH3 measurements from in situ instruments, satellite infrared spectrometers, and atmospheric model simulations, we have demonstrated the role of NH3 and meteorological conditions on pollution events occurring over Paris, Toronto, and Mexico City.
Hossain Mohammed Syedul Hoque, Kengo Sudo, Hitoshi Irie, Alessandro Damiani, Manish Naja, and Al Mashroor Fatmi
Atmos. Chem. Phys., 22, 12559–12589, https://doi.org/10.5194/acp-22-12559-2022, https://doi.org/10.5194/acp-22-12559-2022, 2022
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Nitrogen dioxide (NO2) and formaldehyde (HCHO) are essential trace graces regulating tropospheric ozone chemistry. These trace constituents are measured using an optical passive remote sensing technique. In addition, NO2 and HCHO are simulated with a computer model and evaluated against the observations. Such evaluations are essential to assess model uncertainties and improve their predictability. The results yielded good agreement between the two datasets with some discrepancies.
Qiansi Tu, Matthias Schneider, Frank Hase, Farahnaz Khosrawi, Benjamin Ertl, Jaroslaw Necki, Darko Dubravica, Christopher J. Diekmann, Thomas Blumenstock, and Dianjun Fang
Atmos. Chem. Phys., 22, 9747–9765, https://doi.org/10.5194/acp-22-9747-2022, https://doi.org/10.5194/acp-22-9747-2022, 2022
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Three-year satellite observations and high-resolution model forecast of XCH4 are used to derive CH4 emissions in the USCB region, Poland – a region of intense coal mining activities. The wind-assigned anomalies for two opposite wind directions are calculated and the estimated emission rates are very close to the inventories and in reasonable agreement with the previous studies. Our method is quite robust and can serve as a simple method to estimate CH4 or CO2 emissions for other regions.
Pu Liu, Jia Ding, Lei Liu, Wen Xu, and Xuejun Liu
Atmos. Chem. Phys., 22, 9099–9110, https://doi.org/10.5194/acp-22-9099-2022, https://doi.org/10.5194/acp-22-9099-2022, 2022
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Ammonia (NH3) is the important alkaline gas and the key component of fine particulate matter. We used satellite-based observations to analyze the changes in hourly NH3 concentrations and estimated surface NH3 concentrations and NH3 emissions in China. This study shows enormous potential for using satellite data to estimate surface NH3 concentrations and NH3 emissions and provides an important reference for understanding NH3 variation in China.
Yohanna Villalobos, Peter J. Rayner, Jeremy D. Silver, Steven Thomas, Vanessa Haverd, Jürgen Knauer, Zoë M. Loh, Nicholas M. Deutscher, David W. T. Griffith, and David F. Pollard
Atmos. Chem. Phys., 22, 8897–8934, https://doi.org/10.5194/acp-22-8897-2022, https://doi.org/10.5194/acp-22-8897-2022, 2022
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We study the interannual variability in Australian carbon fluxes for 2015–2019 derived from OCO-2 satellite data. Our results suggest that Australia's semi-arid ecosystems are highly responsive to variations in climate drivers such as rainfall and temperature. We found that high rainfall and low temperatures recorded in 2016 led to an anomalous carbon sink over savanna and sparsely vegetated regions, while unprecedented dry and hot weather in 2019 led to anomalous carbon release.
Tianlang Zhao, Jingqiu Mao, William R. Simpson, Isabelle De Smedt, Lei Zhu, Thomas F. Hanisco, Glenn M. Wolfe, Jason M. St. Clair, Gonzalo González Abad, Caroline R. Nowlan, Barbara Barletta, Simone Meinardi, Donald R. Blake, Eric C. Apel, and Rebecca S. Hornbrook
Atmos. Chem. Phys., 22, 7163–7178, https://doi.org/10.5194/acp-22-7163-2022, https://doi.org/10.5194/acp-22-7163-2022, 2022
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Monitoring formaldehyde (HCHO) can help us understand Arctic vegetation change. Here, we compare satellite data and model and show that Alaska summertime HCHO is largely dominated by a background from methane oxidation during mild wildfire years and is dominated by wildfire (largely from direct emission of fire) during strong fire years. Consequently, it is challenging to use satellite HCHO to study vegetation change in the Arctic region.
Maria-Elissavet Koukouli, Konstantinos Michailidis, Pascal Hedelt, Isabelle A. Taylor, Antje Inness, Lieven Clarisse, Dimitris Balis, Dmitry Efremenko, Diego Loyola, Roy G. Grainger, and Christian Retscher
Atmos. Chem. Phys., 22, 5665–5683, https://doi.org/10.5194/acp-22-5665-2022, https://doi.org/10.5194/acp-22-5665-2022, 2022
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Volcanic eruptions eject large amounts of ash and trace gases into the atmosphere. The use of space-borne instruments enables the global monitoring of volcanic SO2 emissions in an economical and risk-free manner. The main aim of this paper is to present its extensive verification, accomplished within the ESA S5P+I: SO2LH project, over major recent volcanic eruptions, against collocated space-borne measurements, as well as assess its impact on the forecasts provided by CAMS.
Hao Yin, Youwen Sun, Justus Notholt, Mathias Palm, and Cheng Liu
Atmos. Chem. Phys., 22, 4167–4185, https://doi.org/10.5194/acp-22-4167-2022, https://doi.org/10.5194/acp-22-4167-2022, 2022
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In this study, we quantity the long-term variabilities and the underlying drivers of NO2 from 2005 to 2020 over the Yangtze River Delta (YRD), one of the most densely populated and highly industrialized city clusters in China. We reveal the significant effect of the Action Plan on the Prevention and Control of Air Pollution since 2013 adopted by the Chinese government to reduce NOx pollution. Our study can improve the understanding of pollution control measures on a regional scale.
Chloé Radice, Hélène Brogniez, Pierre-Emmanuel Kirstetter, and Philippe Chambon
Atmos. Chem. Phys., 22, 3811–3825, https://doi.org/10.5194/acp-22-3811-2022, https://doi.org/10.5194/acp-22-3811-2022, 2022
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A novel probabilistic approach is proposed to evaluate relative humidity (RH) profiles simulated by an atmospheric model with respect to satellite-based RH defined from probability distributions. It improves upon deterministic comparisons by enhancing the information content to enable a finer assessment of each model–observation discrepancy, highlighting significant departures within a deterministic confidence range. Geographical and vertical distributions of the model biases are discussed.
Manu Anna Thomas, Abhay Devasthale, and Tiina Nygård
Atmos. Chem. Phys., 21, 16593–16608, https://doi.org/10.5194/acp-21-16593-2021, https://doi.org/10.5194/acp-21-16593-2021, 2021
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The impact of transported pollutants and their spatial distribution in the Arctic are governed by the local atmospheric circulation or weather states. Therefore, we investigated eight different atmospheric circulation types observed during the spring season in the Arctic. Using satellite and reanalysis datasets, this study provides a comprehensive assessment of the typical circulation patterns that can lead to enhanced or reduced pollution concentrations in the different sectors of the Arctic.
Xin Tian, Yang Wang, Steffen Beirle, Pinhua Xie, Thomas Wagner, Jin Xu, Ang Li, Steffen Dörner, Bo Ren, and Xiaomei Li
Atmos. Chem. Phys., 21, 12867–12894, https://doi.org/10.5194/acp-21-12867-2021, https://doi.org/10.5194/acp-21-12867-2021, 2021
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The performances of two MAX-DOAS inversion algorithms were evaluated for various aerosol pollution scenarios. One inversion algorithm is based on optimal estimation; the other uses a parameterized approach. In this analysis, three types of profile shapes for aerosols and NO2 were considered: exponential, Boltzmann, and Gaussian. The evaluation results can effectively guide the application of the two inversion algorithms in the actual atmosphere and improve the accuracy of the actual inversion.
Rebecca D. Kutzner, Juan Cuesta, Pascale Chelin, Jean-Eudes Petit, Mokhtar Ray, Xavier Landsheere, Benoît Tournadre, Jean-Charles Dupont, Amandine Rosso, Frank Hase, Johannes Orphal, and Matthias Beekmann
Atmos. Chem. Phys., 21, 12091–12111, https://doi.org/10.5194/acp-21-12091-2021, https://doi.org/10.5194/acp-21-12091-2021, 2021
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Our work investigates the diurnal evolution of atmospheric ammonia concentrations during a major pollution event. It analyses it in regard of both chemical (gas–particle conversion) and physical (vertical mixing, meteorology) processes in the atmosphere. These mechanisms are key for understanding the evolution of the physicochemical state of the atmosphere; therefore, it clearly fits into the scope of Atmospheric Chemistry and Physics.
Youwen Sun, Hao Yin, Cheng Liu, Emmanuel Mahieu, Justus Notholt, Yao Té, Xiao Lu, Mathias Palm, Wei Wang, Changgong Shan, Qihou Hu, Min Qin, Yuan Tian, and Bo Zheng
Atmos. Chem. Phys., 21, 11759–11779, https://doi.org/10.5194/acp-21-11759-2021, https://doi.org/10.5194/acp-21-11759-2021, 2021
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The variability, sources, and transport of ethane (C2H6) over eastern China from 2015 to 2020 were studied using ground-based Fourier transform infrared (FTIR) spectroscopy and GEOS-Chem simulations. C2H6 variability is driven by both meteorological and emission factors. The reduction in C2H6 in recent years over eastern China points to air quality improvement in China.
Youwen Sun, Hao Yin, Cheng Liu, Lin Zhang, Yuan Cheng, Mathias Palm, Justus Notholt, Xiao Lu, Corinne Vigouroux, Bo Zheng, Wei Wang, Nicholas Jones, Changong Shan, Min Qin, Yuan Tian, Qihou Hu, Fanhao Meng, and Jianguo Liu
Atmos. Chem. Phys., 21, 6365–6387, https://doi.org/10.5194/acp-21-6365-2021, https://doi.org/10.5194/acp-21-6365-2021, 2021
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This study mapped the drivers of HCHO variability from 2015 to 2019 over eastern China. Hydroxyl (OH) radical production rates from HCHO photolysis were evaluated. The relative contributions of emitted and photochemical sources to the observed HCHO abundance were analyzed. Contributions of various emission sources and geographical regions to the observed HCHO summertime enhancements were determined.
Fernando Chouza, Thierry Leblanc, Mark Brewer, Patrick Wang, Sabino Piazzolla, Gabriele Pfister, Rajesh Kumar, Carl Drews, Simone Tilmes, Louisa Emmons, and Matthew Johnson
Atmos. Chem. Phys., 21, 6129–6153, https://doi.org/10.5194/acp-21-6129-2021, https://doi.org/10.5194/acp-21-6129-2021, 2021
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The tropospheric ozone lidar at the JPL Table Mountain Facility (TMF) was used to investigate the impact of Los Angeles (LA) Basin pollution transport and stratospheric intrusions in the planetary boundary layer on the San Gabriel Mountains. The results of this study indicate a dominant role of the LA Basin pollution on days when high ozone levels were observed at TMF (March–October period).
Maria-Elissavet Koukouli, Ioanna Skoulidou, Andreas Karavias, Isaak Parcharidis, Dimitris Balis, Astrid Manders, Arjo Segers, Henk Eskes, and Jos van Geffen
Atmos. Chem. Phys., 21, 1759–1774, https://doi.org/10.5194/acp-21-1759-2021, https://doi.org/10.5194/acp-21-1759-2021, 2021
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In recent years, satellite observations have contributed to monitoring air quality. During the first COVID-19 lockdown, lower levels of nitrogen dioxide were observed over Greece by S5P/TROPOMI for March and April 2020 (than the preceding year) due to decreased transport emissions. Taking meteorology into account, using LOTOS-EUROS CTM simulations, the resulting decline due to the lockdown was estimated to range between 0 % and −37 % for the five largest Greek cities, with an average of ~ −10 %.
Tobias Borsdorff, Agustín García Reynoso, Gilberto Maldonado, Bertha Mar-Morales, Wolfgang Stremme, Michel Grutter, and Jochen Landgraf
Atmos. Chem. Phys., 20, 15761–15774, https://doi.org/10.5194/acp-20-15761-2020, https://doi.org/10.5194/acp-20-15761-2020, 2020
Sören Johansson, Michael Höpfner, Oliver Kirner, Ingo Wohltmann, Silvia Bucci, Bernard Legras, Felix Friedl-Vallon, Norbert Glatthor, Erik Kretschmer, Jörn Ungermann, and Gerald Wetzel
Atmos. Chem. Phys., 20, 14695–14715, https://doi.org/10.5194/acp-20-14695-2020, https://doi.org/10.5194/acp-20-14695-2020, 2020
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We present high-resolution measurements of pollutant trace gases (PAN, C2H2, and HCOOH) in the Asian monsoon UTLS from the airborne limb imager GLORIA during StratoClim 2017. Enhancements are observed up to 16 km altitude, and PAN and C2H2 even up to 18 km. Two atmospheric models, CAMS and EMAC, reproduce the pollutant's large-scale structures but not finer structures. Convection is investigated using backward trajectories of the models ATLAS and TRACZILLA with advanced detection of convection.
Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows
Atmos. Chem. Phys., 20, 12285–12312, https://doi.org/10.5194/acp-20-12285-2020, https://doi.org/10.5194/acp-20-12285-2020, 2020
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In this study, we present spatial distributions of occurrence frequency of enhanced total BrO column and various meteorological parameters affecting it in the Arctic and Antarctic sea ice regions by using 10 years of GOME-2 measurements and meteorological model data. Statistical analysis using the long-term dataset shows clear differences in the meteorological conditions between the mean field and the situation of enhanced total BrO columns in both polar sea ice regions.
Leonie Bernet, Elmar Brockmann, Thomas von Clarmann, Niklaus Kämpfer, Emmanuel Mahieu, Christian Mätzler, Gunter Stober, and Klemens Hocke
Atmos. Chem. Phys., 20, 11223–11244, https://doi.org/10.5194/acp-20-11223-2020, https://doi.org/10.5194/acp-20-11223-2020, 2020
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With global warming, water vapour increases in the atmosphere. Water vapour is an important gas because it is a natural greenhouse gas and affects the formation of clouds, rain and snow. How much water vapour increases can vary in different regions of the world. To verify if it increases as expected on a regional scale, we analysed water vapour measurements in Switzerland. We found that water vapour generally increases as expected from temperature changes, except in winter.
Shannon Hicks-Jalali, Robert J. Sica, Giovanni Martucci, Eliane Maillard Barras, Jordan Voirin, and Alexander Haefele
Atmos. Chem. Phys., 20, 9619–9640, https://doi.org/10.5194/acp-20-9619-2020, https://doi.org/10.5194/acp-20-9619-2020, 2020
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We have calculated an 11.5-year water vapour climatology using the Raman Lidar for Meteorological Observations (RALMO), located in Payerne, Switzerland. The climatology shows that the highest water vapour concentrations are in the summer months and the lowest in the winter months. We present for the first time height-resolved water vapour trends, which show that water vapour increases specific humidity by between 5 % and 15 % per decade depending on the altitude.
Yohanna Villalobos, Peter Rayner, Steven Thomas, and Jeremy Silver
Atmos. Chem. Phys., 20, 8473–8500, https://doi.org/10.5194/acp-20-8473-2020, https://doi.org/10.5194/acp-20-8473-2020, 2020
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Estimated carbon fluxes for Australia are subject to considerable uncertainty. We ran simulation experiments over Australia to determine how much these uncertainties can be constrained using satellite data. We found that the satellite data has the potential to reduce these uncertainties up to 80 % across the whole continent. For 1 month, this percentage corresponds to 0.51 Pg C y-1 for Australia. This method could lead to significantly more accurate estimates of Australia's carbon budget.
Bo Zheng, Frédéric Chevallier, Philippe Ciais, Grégoire Broquet, Yilong Wang, Jinghui Lian, and Yuanhong Zhao
Atmos. Chem. Phys., 20, 8501–8510, https://doi.org/10.5194/acp-20-8501-2020, https://doi.org/10.5194/acp-20-8501-2020, 2020
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The Paris Climate Agreement requires all parties to report CO2 emissions regularly. Given the self-reporting nature of this system, it is critical to evaluate the emission reports with independent observation systems. Here we present the direct observations of city CO2 plumes from space and the quantification of CO2 emissions from these observations over the largest emitter country China. The emissions from 46 hot-spot regions representing 13 % of China's total emissions can be well constrained.
Jeffery Langille, Adam Bourassa, Laura L. Pan, Daniel Letros, Brian Solheim, Daniel Zawada, and Doug Degenstein
Atmos. Chem. Phys., 20, 5477–5486, https://doi.org/10.5194/acp-20-5477-2020, https://doi.org/10.5194/acp-20-5477-2020, 2020
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Water vapour (WV) is a highly variable and extremely important trace gas in Earth’s atmosphere. Due to its radiative and chemical properties, it is coupled to the climate in an extremely complex manner. This is especially true in the lowermost stratosphere (LMS). Despite its importance, the physical processes that control mixing and the distribution of WV in the LMS are poorly understood. This study provides observational evidence of moistening the LMS via mixing across the subtropical jet.
Youwen Sun, Cheng Liu, Lin Zhang, Mathias Palm, Justus Notholt, Hao Yin, Corinne Vigouroux, Erik Lutsch, Wei Wang, Changong Shan, Thomas Blumenstock, Tomoo Nagahama, Isamu Morino, Emmanuel Mahieu, Kimberly Strong, Bavo Langerock, Martine De Mazière, Qihou Hu, Huifang Zhang, Christof Petri, and Jianguo Liu
Atmos. Chem. Phys., 20, 5437–5456, https://doi.org/10.5194/acp-20-5437-2020, https://doi.org/10.5194/acp-20-5437-2020, 2020
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We present multiyear time series of ground-based Fourier-transform infrared spectroscopy measurements of HCN in densely populated eastern China. The seasonality and interannual variability of tropospheric HCN columns were investigated. The potential sources that drive the observed HCN seasonality and interannual variability were determined using a GEOS-Chem tagged CO simulation, global fire maps, and potential source contribution function values calculated using HYSPLIT back trajectories.
Enrico Dammers, Chris A. McLinden, Debora Griffin, Mark W. Shephard, Shelley Van Der Graaf, Erik Lutsch, Martijn Schaap, Yonatan Gainairu-Matz, Vitali Fioletov, Martin Van Damme, Simon Whitburn, Lieven Clarisse, Karen Cady-Pereira, Cathy Clerbaux, Pierre Francois Coheur, and Jan Willem Erisman
Atmos. Chem. Phys., 19, 12261–12293, https://doi.org/10.5194/acp-19-12261-2019, https://doi.org/10.5194/acp-19-12261-2019, 2019
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Ammonia is an essential molecule in the environment, but at its current levels it is unsustainable. However, the emissions are highly uncertain. We explore the use of satellites to estimate the ammonia lifetime and emissions around point sources to help improve the budget. The same method applied to different satellite instruments shows consistent results. Comparison to the emission inventories shows that those are underestimating emissions of point sources by on average a factor of 2.5.
Klemens Hocke, Leonie Bernet, Jonas Hagen, Axel Murk, Matthias Renker, and Christian Mätzler
Atmos. Chem. Phys., 19, 12083–12090, https://doi.org/10.5194/acp-19-12083-2019, https://doi.org/10.5194/acp-19-12083-2019, 2019
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The Tropospheric Water Radiometer (TROWARA) observed an enhanced intensity of short-term integrated water vapour (IWV) fluctuations during daytime in summer. These IWV fluctuations are possibly related to latent heat flux and thermal convective activity in the lower troposphere. The observed climatology and spectra of IWV fluctuations might be useful for modelling studies of water vapour convection in the atmospheric boundary layer at mid latitudes.
Xiaoyi Zhao, Debora Griffin, Vitali Fioletov, Chris McLinden, Jonathan Davies, Akira Ogyu, Sum Chi Lee, Alexandru Lupu, Michael D. Moran, Alexander Cede, Martin Tiefengraber, and Moritz Müller
Atmos. Chem. Phys., 19, 10619–10642, https://doi.org/10.5194/acp-19-10619-2019, https://doi.org/10.5194/acp-19-10619-2019, 2019
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New nitrogen dioxide (NO2) retrieval algorithms are developed for Pandora zenith-sky measurements. A column-to-surface conversion look-up table was produced for the Pandora instruments; therefore, quick and practical Pandora-based surface NO2 concentration data can be obtained for air quality monitoring purposes. It is demonstrated that the surface NO2 concentration is controlled not only by the planetary boundary layer height but also by both boundary layer dynamics and photochemistry.
Ka Lok Chan, Zhuoru Wang, Aijun Ding, Klaus-Peter Heue, Yicheng Shen, Jing Wang, Feng Zhang, Yining Shi, Nan Hao, and Mark Wenig
Atmos. Chem. Phys., 19, 10051–10071, https://doi.org/10.5194/acp-19-10051-2019, https://doi.org/10.5194/acp-19-10051-2019, 2019
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The paper presents long-term observations of atmospheric nitrogen dioxide (NO2) and formaldehyde (HCHO) in Nanjing using a MAX-DOAS instrument. The measurements were performed from April 2013 to February 2017. The MAX-DOAS measurements of NO2 and HCHO are used to validate OMI satellite observations and to investigate the influences of region transport of air pollutants on the air quality in Nanjing.
Olivier Bock and Ana C. Parracho
Atmos. Chem. Phys., 19, 9453–9468, https://doi.org/10.5194/acp-19-9453-2019, https://doi.org/10.5194/acp-19-9453-2019, 2019
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We examine the consistency of global IWV data from ERA-Interim reanalysis and 16 years of GPS observations. Representativeness differences are found to be a dominant error source, with a strong dependence on geographic, topographic, and climatic features, which explain both average and extreme differences. A methodology for reducing the representativeness errors and detecting the extreme, outlying, cases is discussed.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Sven Krautwurst, Christopher W. O'Dell, Andreas Richter, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 19, 9371–9383, https://doi.org/10.5194/acp-19-9371-2019, https://doi.org/10.5194/acp-19-9371-2019, 2019
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The quantification of anthropogenic emissions with current CO2 satellite sensors is difficult, but NO2 is co-emitted, making it a suitable tracer of recently emitted CO2. We analyze enhancements of CO2 and NO2 observed by OCO-2 and S5P and estimate the CO2 plume cross-sectional fluxes that we compare with emission databases. Our results demonstrate the usefulness of simultaneous satellite observations of CO2 and NO2 as envisaged for the European Copernicus anthropogenic CO2 monitoring mission
Luis F. Millán, Matthew D. Lebsock, and Joao Teixeira
Atmos. Chem. Phys., 19, 8491–8502, https://doi.org/10.5194/acp-19-8491-2019, https://doi.org/10.5194/acp-19-8491-2019, 2019
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The synergy of the collocated Advanced Microwave Scanning Radiometer (AMSR) and the Moderate Resolution Imaging Spectroradiometer (MODIS) provides daily global estimates of marine boundary layer water vapor. AMSR provides the total column water vapor, while MODIS provides the water vapor above the cloud layers. The difference between the two gives the vapor between the surface and the cloud top, which may be interpreted as the boundary layer water vapor.
Aristeidis K. Georgoulias, Ronald J. van der A, Piet Stammes, K. Folkert Boersma, and Henk J. Eskes
Atmos. Chem. Phys., 19, 6269–6294, https://doi.org/10.5194/acp-19-6269-2019, https://doi.org/10.5194/acp-19-6269-2019, 2019
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In this paper, a ∼21-year self-consistent global dataset from four different satellite sensors is compiled for the first time to study the long-term tropospheric NO2 patterns and trends. A novel method capable of detecting the year when a reversal of trends happened shows that tropospheric NO2 concentrations switched from positive to negative trends and vice versa over several regions around the globe during the last 2 decades.
Elisa Carboni, Tamsin A. Mather, Anja Schmidt, Roy G. Grainger, Melissa A. Pfeffer, Iolanda Ialongo, and Nicolas Theys
Atmos. Chem. Phys., 19, 4851–4862, https://doi.org/10.5194/acp-19-4851-2019, https://doi.org/10.5194/acp-19-4851-2019, 2019
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The 2014–2015 Holuhraun eruption was the largest in Iceland for 200 years, emitting huge quantities of gas into the troposphere, at times overwhelming European anthropogenic emissions. Infrared Atmospheric sounding Interferometer data are used to derive the first time series of daily sulfur dioxide mass and vertical distribution over the eruption period. A scheme is used to estimate sulfur dioxide fluxes, the total erupted mass, and how long the sulfur dioxide remains in the atmosphere.
Debra Wunch, Dylan B. A. Jones, Geoffrey C. Toon, Nicholas M. Deutscher, Frank Hase, Justus Notholt, Ralf Sussmann, Thorsten Warneke, Jeroen Kuenen, Hugo Denier van der Gon, Jenny A. Fisher, and Joannes D. Maasakkers
Atmos. Chem. Phys., 19, 3963–3980, https://doi.org/10.5194/acp-19-3963-2019, https://doi.org/10.5194/acp-19-3963-2019, 2019
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We used five atmospheric observatories in Europe measuring total column dry-air mole fractions of methane and carbon monoxide to infer methane emissions in the area between the observatories. We find that the methane emissions are overestimated by the state-of-the-art inventories, and that this is likely due, at least in part, to the inventory disaggregation. We find that there is significant uncertainty in the carbon monoxide inventories that requires further investigation.
Klaus Gierens and Kostas Eleftheratos
Atmos. Chem. Phys., 19, 3733–3746, https://doi.org/10.5194/acp-19-3733-2019, https://doi.org/10.5194/acp-19-3733-2019, 2019
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We derive a new method to retrieve upper-tropospheric humidity (UTH) from High-resolution Infrared Radiation Sounder (HIRS) channel 12 brightness temperatures. With the new method we solve an old problem, namely that the wavelength change that occurred between HIRS 2 on NOAA 14 and HIRS 3 on NOAA 15 led to the retrieval of many more events with high UTH; that is, the time series shows strong jumps at high UTH values. This old problem is solved with the new retrieval.
Cited articles
Basto, S., Thompson, K., Phoenix, G., Sloan, V., Leake, J., and Rees, M.: Long-term nitrogen deposition depletes grassland seed banks, Nat. Commun., 6, 1–6, https://doi.org/10.1038/ncomms7185, 2015.
Beer, R., Shephard, M. W., Kulawik, S. S., Clough, S. A., Eldering, A., Bowman, K. W., Sander, S. P., Fisher, B. M., Payne, V. H., Luo, M., Osterman, G. B., and Worden, J. R.: First satellite observations of lower tropospheric ammonia and methanol, Geophys. Res. Lett., 35, L09801, https://doi.org/10.1029/2008GL033642, 2008.
Beig, G. and Singh, V.: Trends in tropical tropospheric column ozone from satellite data and MOZART model, Geophys. Res. Lett., 34, L17801, https://doi.org/10.1029/2007GL030460, 2007.
Boersma, K. F., Eskes, H. J., Veefkind, J. P., Brinksma, E. J., van der A, R. J., Sneep, M., van den Oord, G. H. J., Levelt, P. F., Stammes, P., Gleason, J. F., and Bucsela, E. J.: Near-real time retrieval of tropospheric NO2 from OMI, Atmos. Chem. Phys., 7, 2103–2118, https://doi.org/10.5194/acp-7-2103-2007, 2007.
Boersma, K. F., Eskes, H. J., Dirksen, R. J., van der A, R. J., Veefkind, J. P., Stammes, P., Huijnen, V., Kleipool, Q. L., Sneep, M., Claas, J., Leitão, J., Richter, A., Zhou, Y., and Brunner, D.: An improved tropospheric NO2 column retrieval algorithm for the Ozone Monitoring Instrument, Atmos. Meas. Tech., 4, 1905–1928, https://doi.org/10.5194/amt-4-1905-2011, 2011.
Boersma, K. F., Vinken, G. C. M., and Eskes, H. J.: Representativeness errors in comparing chemistry transport and chemistry climate models with satellite UV-Vis tropospheric column retrievals, Geosci. Model Dev., 9, 875–898, https://doi.org/10.5194/gmd-9-875-2016, 2016.
Brasseur, G., Hauglustaine, D., Walters, S., Rasch, P., Müller, J. F., Granier, C., and Tie, X.: MOZART, a global chemical transport model for ozone and related chemical tracers: 1. Model description, J. Geophys. Res.-Atmos., 103, 28265–28289, 1998.
Canfield, D. E., Glazer, A. N., and Falkowski, P. G.: The Evolution and Future of Earth's Nitrogen Cycle, Science, 330, 192–196, https://doi.org/10.1126/science.1186120, 2010.
Castellanos, P., Boersma, K. F., Torres, O., and de Haan, J. F.: OMI tropospheric NO2 air mass factors over South America: effects of biomass burning aerosols, Atmos. Meas. Tech., 8, 3831–3849, https://doi.org/10.5194/amt-8-3831-2015, 2015.
Clarisse, L., Clerbaux, C., Dentener, F., Hurtmans, D., and Coheur, P.-F.: Global ammonia distribution derived from infrared satellite observations, Nat. Geosci., 2, 479–483, 2009.
Cofala, J., Amann, M., Klimont, Z., Kupiainen, K., and Höglund-Isaksson, L.: Scenarios of global anthropogenic emissions of air pollutants and methane until 2030, Atmos. Environ., 41, 8486–8499, https://doi.org/10.1016/j.atmosenv.2007.07.010, 2007.
Coheur, P.-F., Clarisse, L., Turquety, S., Hurtmans, D., and Clerbaux, C.: IASI measurements of reactive trace species in biomass burning plumes, Atmos. Chem. Phys., 9, 5655–5667, https://doi.org/10.5194/acp-9-5655-2009, 2009.
Crippa, M., Janssens-Maenhout, G., Dentener, F., Guizzardi, D., Sindelarova, K., Muntean, M., Van Dingenen, R., and Granier, C.: Forty years of improvements in European air quality: regional policy-industry interactions with global impacts, Atmos. Chem. Phys., 16, 3825–3841, https://doi.org/10.5194/acp-16-3825-2016, 2016.
Dammers, E., Palm, M., Van Damme, M., Vigouroux, C., Smale, D., Conway, S., Toon, G. C., Jones, N., Nussbaumer, E., Warneke, T., Petri, C., Clarisse, L., Clerbaux, C., Hermans, C., Lutsch, E., Strong, K., Hannigan, J. W., Nakajima, H., Morino, I., Herrera, B., Stremme, W., Grutter, M., Schaap, M., Wichink Kruit, R. J., Notholt, J., Coheur, P.-F., and Erisman, J. W.: An evaluation of IASI-NH3 with ground-based Fourier transform infrared spectroscopy measurements, Atmos. Chem. Phys., 16, 10351–10368, https://doi.org/10.5194/acp-16-10351-2016, 2016.
De Smedt, I., Stavrakou, T., Hendrick, F., Danckaert, T., Vlemmix, T., Pinardi, G., Theys, N., Lerot, C., Gielen, C., Vigouroux, C., Hermans, C., Fayt, C., Veefkind, P., Müller, J.-F., and Van Roozendael, M.: Diurnal, seasonal and long-term variations of global formaldehyde columns inferred from combined OMI and GOME-2 observations, Atmos. Chem. Phys., 15, 12519–12545, https://doi.org/10.5194/acp-15-12519-2015, 2015.
Emmons, L. K., Walters, S., Hess, P. G., Lamarque, J.-F., Pfister, G. G., Fillmore, D., Granier, C., Guenther, A., Kinnison, D., Laepple, T., Orlando, J., Tie, X., Tyndall, G., Wiedinmyer, C., Baughcum, S. L., and Kloster, S.: Description and evaluation of the Model for Ozone and Related chemical Tracers, version 4 (MOZART-4), Geosci. Model Dev., 3, 43–67, https://doi.org/10.5194/gmd-3-43-2010, 2010.
Erisman, J. W., Sutton, M. A., Galloway, J., Klimont, Z., and Winiwarter, W.: How a century of ammonia synthesis changed the world, Nat. Geosci., 1, 636–639, 2008.
Foy, B. D., Lu, Z., and Streets, D. G.: Satellite NO2 retrievals suggest China has exceeded its NOxreduction goals from the twelfth Five-Year Plan, Scientific Reports, 6, 35912, 2016.
Fu, B., Li, S., Yu, X., Yang, P., Yu, G., Feng, R., and Zhuang, X.: Chinese ecosystem research network: Progress and perspectives, Ecological Complexity, 7, 225–233, https://doi.org/10.1016/j.ecocom.2010.02.007, 2010.
Galloway, J. N., Dentener, F. J., Capone, D. G., Boyer, E. W., Howarth, R. W., Seitzinger, S. P., Asner, G. P., Cleveland, C. C., Green, P. A., Holland, E. A., Karl, D. M., Michaels, A. F., Porter, J. H., Townsend, A. R., and Vöosmarty, C. J.: Nitrogen Cycles: Past, Present, and Future, Biogeochemistry, 70, 153–226, https://doi.org/10.1007/s10533-004-0370-0, 2004.
Galloway, J. N., Townsend, A. R., Erisman, J. W., Bekunda, M., Cai, Z., Freney, J. R., Martinelli, L. A., Seitzinger, S. P., and Sutton, M. A.: Transformation of the Nitrogen Cycle: Recent Trends, Questions, and Potential Solutions, Science, 320, 889–892, https://doi.org/10.1126/science.1136674, 2008.
Geddes, J. A. and Martin, R. V.: Global deposition of total reactive nitrogen oxides from 1996 to 2014 constrained with satellite observations of NO2 columns, Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-1100, in review, 2017.
Huang, X., Song, Y., Li, M., Li, J., Huo, Q., Cai, X., Zhu, T., Hu, M., and Zhang, H.: A high resolution ammonia emission inventory in China, Global Biogeochem. Cy., 26, 1–14, 2012.
Ialongo, I., Herman, J., Krotkov, N., Lamsal, L., Boersma, K. F., Hovila, J., and Tamminen, J.: Comparison of OMI NO2 observations and their seasonal and weekly cycles with ground-based measurements in Helsinki, Atmos. Meas. Tech., 9, 5203–5212, https://doi.org/10.5194/amt-9-5203-2016, 2016.
Jgj, O., Jjm, B., Jahw, P., Bakker, J., Ajh, V., and Jpj, B.: Applications of EDGAR Emission Database for Global Atmospheric Research, Rijksinstituut Voor Volksgezondheid En Milieu Rivm, 2002.
Kang, Y., Liu, M., Song, Y., Huang, X., Yao, H., Cai, X., Zhang, H., Kang, L., Liu, X., Yan, X., He, H., Zhang, Q., Shao, M., and Zhu, T.: High-resolution ammonia emissions inventories in China from 1980 to 2012, Atmos. Chem. Phys., 16, 2043–2058, https://doi.org/10.5194/acp-16-2043-2016, 2016.
Klimont, Z., Cofala, J., Schöpp, W., Amann, M., Streets, D. G., Ichikawa, Y., and Fujita, S.: Projections of SO2, NOx, NH3 and VOC Emissions in East Asia Up to 2030, Water Air Soil Poll., 130, 193–198, 2001.
Kurokawa, J., Ohara, T., Morikawa, T., Hanayama, S., Janssens-Maenhout, G., Fukui, T., Kawashima, K., and Akimoto, H.: Emissions of air pollutants and greenhouse gases over Asian regions during 2000–2008: Regional Emission inventory in ASia (REAS) version 2, Atmos. Chem. Phys., 13, 11019–11058, https://doi.org/10.5194/acp-13-11019-2013, 2013.
Lamsal, L. N., Duncan, B. N., Yoshida, Y., Krotkov, N. A., Pickering, K. E., Streets, D. G., and Lu, Z.: U.S. NO2 trends (2005–2013): EPA Air Quality System (AQS) data versus improved observations from the Ozone Monitoring Instrument (OMI), Atmos. Environ., 110, 130–143, https://doi.org/10.1016/j.atmosenv.2015.03.055, 2015.
Lan, Z., Jenerette, G. D., Zhan, S., Li, W., Zheng, S., and Bai, Y.: Testing the scaling effects and mechanisms of N-induced biodiversity loss: evidence from a decade-long grassland experiment, J. Ecol., 103, 750–760, https://doi.org/10.1111/1365-2745.12395, 2015.
Li, Y., Schwandner, F. M., Sewell, H. J., Zivkovich, A., Tigges, M., Raja, S., Holcomb, S., Molenar, J. V., Sherman, L., and Archuleta, C.: Observations of ammonia, nitric acid, and fine particles in a rural gas production region, Atmos. Environ., 83, 80–89, 2014.
Li, Y., Schichtel, B. A., Walker, J. T., Schwede, D. B., Chen, X., Lehmann, C. M., Puchalski, M. A., Gay, D. A., and Collett, J. L.: Increasing importance of deposition of reduced nitrogen in the United States, P. Natl. Acad. Sci. USA, 113, 5874–5879, 2016.
Li, Y., Thompson, T. M., Van Damme, M., Chen, X., Benedict, K. B., Shao, Y., Day, D., Boris, A., Sullivan, A. P., Ham, J., Whitburn, S., Clarisse, L., Coheur, P.-F., and Collett Jr., J. L.: Temporal and spatial variability of ammonia in urban and agricultural regions of northern Colorado, United States, Atmos. Chem. Phys., 17, 6197-6213, https://doi.org/10.5194/acp-17-6197-2017, 2017.
Liu, F., Zhang, Q., Ronald, J. v. d. A., Zheng, B., Tong, D., Yan, L., Zheng, Y., and He, K.: Recent reduction in NO x emissions over China: synthesis of satellite observations and emission inventories, Environ. Res. Lett., 11, 114002, https://doi.org/10.1088/1748-9326/11/11/114002, 2016.
Liu, L., Zhang, X., Wang, S., Lu, X., and Ouyang, X.: A Review of Spatial Variation of Inorganic Nitrogen (N) Wet Deposition in China, PloS one, 11, e0146051, https://doi.org/10.1371/journal.pone.0146051, 2016.
Liu, L., Zhang, X., Xu, W., Liu, X., Lu, X., Wang, S., Zhang, W., and Zhao, L.: Ground Ammonia Concentrations over China Derived from Satellite and Atmospheric Transport Modeling, Remote Sensing, 9, 467, https://doi.org/10.3390/rs9050467, 2017a.
Liu, L., Zhang, X., Zhang, Y., Xu, W., Liu, X., Zhang, X., Feng, J., Chen, X., Zhang, Y., Lu, X., Wang, S., Zhang, W., and Zhao, L.: Dry Particulate Nitrate Deposition in China, Environ. Sci. Technol., 51, 5572, https://doi.org/10.1021/acs.est.7b00898, 2017b.
Liu, X., Duan, L., Mo, J., Du, E., Shen, J., Lu, X., Zhang, Y., Zhou, X., He, C., and Zhang, F.: Nitrogen deposition and its ecological impact in China: An overview, Environ. Pollut., 159, 2251–2264, https://doi.org/10.1016/j.envpol.2010.08.002, 2011.
Liu, X., Zhang, Y., Han, W., Tang, A., Shen, J., Cui, Z., Vitousek, P., Erisman, J. W., Goulding, K., and Christie, P.: Enhanced nitrogen deposition over China, Nature, 494, 459–462, 2013.
Liu, X., Vitousek, P., Chang, Y., Zhang, W., Matson, P., and Zhang, F.: Evidence for a Historic Change Occurring in China, Environ. Sci. Technol., 50, 505–506, 2015.
Liu, X., Xu, W., Duan, L., Du, E., Pan, Y., Lu, X., Zhang, L., Wu, Z., Wang, X., and Zhang, Y.: Erratum to: Atmospheric Nitrogen Emission, Deposition, and Air Quality Impacts in China: an Overview, Current Pollution Reports, 1–1, 2017.
Lu, X., Jiang, H., Liu, J., Zhang, X., Jin, J., Zhu, Q., Zhang, Z., and Peng, C.: Simulated effects of nitrogen saturation on the global carbon budget using the IBIS model, Scientific Reports, 6, 39173, https://doi.org/10.1038/srep39173, 2016.
Ma, J. Z., Beirle, S., Jin, J. L., Shaiganfar, R., Yan, P., and Wagner, T.: Tropospheric NO2 vertical column densities over Beijing: results of the first three years of ground-based MAX-DOAS measurements (2008–2011) and satellite validation, Atmos. Chem. Phys., 13, 1547–1567, https://doi.org/10.5194/acp-13-1547-2013, 2013.
Meng, Z.-Y., Xu, X.-B., Wang, T., Zhang, X.-Y., Yu, X.-L., Wang, S.-F., Lin, W.-L., Chen, Y.-Z., Jiang, Y.-A., and An, X.-Q.: Ambient sulfur dioxide, nitrogen dioxide, and ammonia at ten background and rural sites in China during 2007–2008, Atmos. Environ., 44, 2625–2631, https://doi.org/10.1016/j.atmosenv.2010.04.008, 2010.
Meng, Z. Y., Lin, W. L., Jiang, X. M., Yan, P., Wang, Y., Zhang, Y. M., Jia, X. F., and Yu, X. L.: Characteristics of atmospheric ammonia over Beijing, China, Atmos. Chem. Phys., 11, 6139–6151, https://doi.org/10.5194/acp-11-6139-2011, 2011.
Nowlan, C., Martin, R., Philip, S., Lamsal, L., Krotkov, N., Marais, E., Wang, S., and Zhang, Q.: Global dry deposition of nitrogen dioxide and sulfur dioxide inferred from space-based measurements, Global Biogeochem. Cy., 28, 1025–1043, 2014.
Ohara, T., Akimoto, H., Kurokawa, J., Horii, N., Yamaji, K., Yan, X., and Hayasaka, T.: An Asian emission inventory of anthropogenic emission sources for the period 1980–2020, Atmos. Chem. Phys., 7, 4419–4444, https://doi.org/10.5194/acp-7-4419-2007, 2007.
Olivier, J. G. J., Bouwman, A. F., Hoek, K. W. V. D., and Berdowski, J. J. M.: Global air emission inventories for anthropogenic sources of NOx , NH3 and N2O in 1990, Environ. Pollut., 102, 135–148, 1998.
Pan, Y. P., Wang, Y. S., Tang, G. Q., and Wu, D.: Wet and dry deposition of atmospheric nitrogen at ten sites in Northern China, Atmos. Chem. Phys., 12, 6515–6535, https://doi.org/10.5194/acp-12-6515-2012, 2012.
Pfister, G., Emmons, L., Hess, P., Lamarque, J. F., Orlando, J., Walters, S., Guenther, A., Palmer, P., and Lawrence, P.: Contribution of isoprene to chemical budgets: A model tracer study with the NCAR CTM MOZART-4, J. Geophys. Res.-Atmos., 113, D05308, https://doi.org/10.1029/2007JD008948, 2008.
FRCGC (Frontier Research Center for Global Change): Regional Emission Inventory in Asia, available at: http://www.jamstec.go.jp/frsgc/research/d4/emission.htm (last access: 1 August 2017), 2007
Russell, A. R., Perring, A. E., Valin, L. C., Bucsela, E. J., Browne, E. C., Wooldridge, P. J., and Cohen, R. C.: A high spatial resolution retrieval of NO2 column densities from OMI: method and evaluation, Atmos. Chem. Phys., 11, 8543–8554, https://doi.org/10.5194/acp-11-8543-2011, 2011.
Russell, A. R., Valin, L. C., and Cohen, R. C.: Trends in OMI NO2 observations over the United States: effects of emission control technology and the economic recession, Atmos. Chem. Phys., 12, 12197–12209, https://doi.org/10.5194/acp-12-12197-2012, 2012.
Sahu, L., Sheel, V., Kajino, M., Gunthe, S. S., Thouret, V., Nedelec, P., and Smit, H. G.: Characteristics of tropospheric ozone variability over an urban site in Southeast Asia: A study based on MOZAIC and MOZART vertical profiles, J. Geophys. Res.-Atmos., 118, 8729–8747, 2013.
Shi, Y., Cui, S., Ju, X., Cai, Z., and Zhu, Y.-G.: Impacts of reactive nitrogen on climate change in China, Scientific Reports, 5, 8118, https://doi.org/10.1038/srep08118, 2015.
Streets, D. G., Bond, T. C., Carmichael, G. R., Fernandes, S. D., He, D., Klimont, Z., Nelson, S. M., Tsai, N. Y., and Wang, M. Q.: An inventory of gaseous and primary aerosol emissions in Asia in the year 2000, J. Geophys. Res.-Atmos., 108, 30–31, 2003.
Sun, Q. and Wang, M.: Ammonia Emission and Concentration in the Atmosphere over China, Scientia Atmospherica Sinica, 1997.
Van Damme, M., Clarisse, L., Heald, C. L., Hurtmans, D., Ngadi, Y., Clerbaux, C., Dolman, A. J., Erisman, J. W., and Coheur, P. F.: Global distributions, time series and error characterization of atmospheric ammonia (NH3) from IASI satellite observations, Atmos. Chem. Phys., 14, 2905–2922, https://doi.org/10.5194/acp-14-2905-2014, 2014a.
Van Damme, M., Wichink Kruit, R., Schaap, M., Clarisse, L., Clerbaux, C., Coheur, P. F., Dammers, E., Dolman, A., and Erisman, J.: Evaluating 4 years of atmospheric ammonia (NH3) over Europe using IASI satellite observations and LOTOS-EUROS model results, J. Geophys. Res.-Atmos., 119, 9549–9566, 2014b.
Van Damme, M., Clarisse, L., Dammers, E., Liu, X., Nowak, J. B., Clerbaux, C., Flechard, C. R., Galy-Lacaux, C., Xu, W., Neuman, J. A., Tang, Y. S., Sutton, M. A., Erisman, J. W., and Coheur, P. F.: Towards validation of ammonia (NH3) measurements from the IASI satellite, Atmos. Meas. Tech., 8, 1575–1591, https://doi.org/10.5194/amt-8-1575-2015, 2015.
Walker, J. C., Dudhia, A., and Carboni, E.: An effective method for the detection of trace species demonstrated using the MetOp Infrared Atmospheric Sounding Interferometer, Atmos. Meas. Tech., 4, 1567–1580, https://doi.org/10.5194/amt-4-1567-2011, 2011.
Wang, S. W., Liao, J. H., Yu-Ting, H. U., and Yan, X. Y.: A Preliminary Inventory of NH3-N Emission and Its Temporal and Spatial Distribution of China, Journal of Agro-Environment Science, 2009.
Wang, S. W., Zhang, Q., Streets, D. G., He, K. B., Martin, R. V., Lamsal, L. N., Chen, D., Lei, Y., and Lu, Z.: Growth in NOx emissions from power plants in China: bottom-up estimates and satellite observations, Atmos. Chem. Phys., 12, 4429–4447, https://doi.org/10.5194/acp-12-4429-2012, 2012.
Wang, W. X., Lu, X. F., Pang, Y. B., Tang, D. G., and Zhang, W. H.: Geographical distribution of NH3 emission intensities in China, Actaentiae Circumstantiae, 1997.
Warner, J. X., Dickerson, R. R., Wei, Z., Strow, L. L., Wang, Y., and Liang, Q.: Increased atmospheric ammonia over the world's major agricultural areas detected from space, Geophys. Res. Lett., 44, 2875–2884, https://doi.org/10.1002/2016GL072305, 2017.
Whitburn, S., Van Damme, M., Clarisse, L., Bauduin, S., Heald, C. L., Hadji-Lazaro, J., Hurtmans, D., Zondlo, M. A., Clerbaux, C., and Coheur, P. F.: A flexible and robust neural network IASI-NH3 retrieval algorithm, J. Geophys. Res.-Atmos., 121, 6581–6599, https://doi.org/10.1002/2016JD024828, 2016a.
Whitburn, S., Van Damme, M., Clarisse, L., Turquety, S., Clerbaux, C., and Coheur, P. F.: Doubling of annual ammonia emissions from the peat fires in Indonesia during the 2015 El Niño, Geophys. Res. Lett., 43, 11007–11014, https://doi.org/10.1002/2016GL070620, 2016b.
Wichink Kruit, R. J., Schaap, M., Sauter, F. J., van Zanten, M. C., and van Pul, W. A. J.: Modeling the distribution of ammonia across Europe including bi-directional surface–atmosphere exchange, Biogeosciences, 9, 5261–5277, https://doi.org/10.5194/bg-9-5261-2012, 2012.
Xia, Y., Zhao, Y., and Nielsen, C. P.: Benefits of China's efforts in gaseous pollutant control indicated by the bottom-up emissions and satellite observations 2000–2014, Atmos. Environ., 136, 43–53, https://doi.org/10.1016/j.atmosenv.2016.04.013, 2016.
Xie, Y., Zhao, B., Zhang, L., and Luo, R.: Spatiotemporal variations of PM2.5 and PM10 concentrations between 31 Chinese cities and their relationships with SO2, NO2, CO and O3, Particuology, 20, 141–149, https://doi.org/10.1016/j.partic.2015.01.003, 2015.
Xu, W., Luo, X. S., Pan, Y. P., Zhang, L., Tang, A. H., Shen, J. L., Zhang, Y., Li, K. H., Wu, Q. H., Yang, D. W., Zhang, Y. Y., Xue, J., Li, W. Q., Li, Q. Q., Tang, L., Lu, S. H., Liang, T., Tong, Y. A., Liu, P., Zhang, Q., Xiong, Z. Q., Shi, X. J., Wu, L. H., Shi, W. Q., Tian, K., Zhong, X. H., Shi, K., Tang, Q. Y., Zhang, L. J., Huang, J. L., He, C. E., Kuang, F. H., Zhu, B., Liu, H., Jin, X., Xin, Y. J., Shi, X. K., Du, E. Z., Dore, A. J., Tang, S., Collett Jr., J. L., Goulding, K., Sun, Y. X., Ren, J., Zhang, F. S., and Liu, X. J.: Quantifying atmospheric nitrogen deposition through a nationwide monitoring network across China, Atmos. Chem. Phys., 15, 12345–12360, https://doi.org/10.5194/acp-15-12345-2015, 2015.
Xu, W., Song, W., Zhang, Y., Liu, X., Zhang, L., Zhao, Y., Liu, D., Tang, A., Yang, D., Wang, D., Wen, Z., Pan, Y., Fowler, D., Collett Jr., J. L., Erisman, J. W., Goulding, K., Li, Y., and Zhang, F.: Air quality improvement in a megacity: implications from 2015 Beijing Parade Blue pollution control actions, Atmos. Chem. Phys., 17, 31–46, https://doi.org/10.5194/acp-17-31-2017, 2017.
Zhao, C. and Wang, Y.: Assimilated inversion of NOx emissions over east Asia using OMI NO2 column measurements, Geophys. Res. Lett., 36, 1–5, 2009.
Zhou, Y., Shuiyuan, C., Lang, J., Chen, D., Zhao, B., Liu, C., Xu, R., and Li, T.: A comprehensive ammonia emission inventory with high-resolution and its evaluation in the Beijing–Tianjin–Hebei (BTH) region, China, Atmos. Environ., 106, 305–317, https://doi.org/10.1016/j.atmosenv.2015.01.069, 2015.
Short summary
We conducted temporal trend analysis of atmospheric NH3 and NO2 in China since 1980 based on emission data (during 1980–2010), satellite observations (for NH3 since 2008 and for NO2 since 2005) and atmospheric chemistry transport modeling (during 2008–2015). Our findings provide an overall insight into the temporal trends in both NO2 and NH3 since 1980, and the multivariate data used in this study have implications for estimating long-term Nr deposition datasets.
We conducted temporal trend analysis of atmospheric NH3 and NO2 in China since 1980 based on...
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