Articles | Volume 17, issue 24
https://doi.org/10.5194/acp-17-14871-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-14871-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
14 Dec 2017
Research article |
| 14 Dec 2017
Changing transport processes in the stratosphere by radiative heating of sulfate aerosols
Ulrike Niemeier
CORRESPONDING AUTHOR
Max Planck Institute for Meteorology, Bundesstr. 53, 20146 Hamburg, Germany
Hauke Schmidt
Max Planck Institute for Meteorology, Bundesstr. 53, 20146 Hamburg, Germany
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Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
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Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.
Felix Wrana, Ulrike Niemeier, Larry W. Thomason, Sandra Wallis, and Christian von Savigny
EGUsphere, https://doi.org/10.5194/egusphere-2023-837, https://doi.org/10.5194/egusphere-2023-837, 2023
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
The stratospheric aerosol layer is a naturally occuring and permanent layer of aerosol, in this case very small droplets of mostly sulfuric acid and water, that has a cooling effect on our climate. To quantify this effect and for our general understanding of stratospheric microphysical processes, knowledge of the size of those aerosol particles is needed. Using satellite measurements and atmospheric models we show, that some volcanic eruptions can lead to on average smaller aerosol sizes.
Yangxin Chen, Duoying Ji, Qian Zhang, John C. Moore, Olivier Boucher, Andy Jones, Thibaut Lurton, Michael J. Mills, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Earth Syst. Dynam., 14, 55–79, https://doi.org/10.5194/esd-14-55-2023, https://doi.org/10.5194/esd-14-55-2023, 2023
Short summary
Short summary
Solar geoengineering has been proposed as a way of counteracting the warming effects of increasing greenhouse gases by reflecting solar radiation. This work shows that solar geoengineering can slow down the northern-high-latitude permafrost degradation but cannot preserve the permafrost ecosystem as that under a climate of the same warming level without solar geoengineering.
Ilaria Quaglia, Claudia Timmreck, Ulrike Niemeier, Daniele Visioni, Giovanni Pitari, Christina Brodowsky, Christoph Brühl, Sandip S. Dhomse, Henning Franke, Anton Laakso, Graham W. Mann, Eugene Rozanov, and Timofei Sukhodolov
Atmos. Chem. Phys., 23, 921–948, https://doi.org/10.5194/acp-23-921-2023, https://doi.org/10.5194/acp-23-921-2023, 2023
Short summary
Short summary
The last very large explosive volcanic eruption we have measurements for is the eruption of Mt. Pinatubo in 1991. It is therefore often used as a benchmark for climate models' ability to reproduce these kinds of events. Here, we compare available measurements with the results from multiple experiments conducted with climate models interactively simulating the aerosol cloud formation.
Simone Tilmes, Daniele Visioni, Andy Jones, James Haywood, Roland Séférian, Pierre Nabat, Olivier Boucher, Ewa Monica Bednarz, and Ulrike Niemeier
Atmos. Chem. Phys., 22, 4557–4579, https://doi.org/10.5194/acp-22-4557-2022, https://doi.org/10.5194/acp-22-4557-2022, 2022
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Short summary
This study assesses the impacts of climate interventions, using stratospheric sulfate aerosol and solar dimming on stratospheric ozone, based on three Earth system models with interactive stratospheric chemistry. The climate interventions have been applied to a high emission (baseline) scenario in order to reach global surface temperatures of a medium emission scenario. We find significant increases and decreases in total column ozone, depending on regions and seasons.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Debra K. Weisenstein, Daniele Visioni, Henning Franke, Ulrike Niemeier, Sandro Vattioni, Gabriel Chiodo, Thomas Peter, and David W. Keith
Atmos. Chem. Phys., 22, 2955–2973, https://doi.org/10.5194/acp-22-2955-2022, https://doi.org/10.5194/acp-22-2955-2022, 2022
Short summary
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This paper explores a potential method of geoengineering that could be used to slow the rate of change of climate over decadal scales. We use three climate models to explore how injections of accumulation-mode sulfuric acid aerosol change the large-scale stratospheric particle size distribution and radiative forcing response for the chosen scenarios. Radiative forcing per unit sulfur injected and relative to the change in aerosol burden is larger with particulate than with SO2 injections.
Anton Laakso, Ulrike Niemeier, Daniele Visioni, Simone Tilmes, and Harri Kokkola
Atmos. Chem. Phys., 22, 93–118, https://doi.org/10.5194/acp-22-93-2022, https://doi.org/10.5194/acp-22-93-2022, 2022
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The use of different spatio-temporal sulfur injection strategies with different magnitudes to create an artificial reflective aerosol layer to cool the climate is studied using sectional and modal aerosol schemes in a climate model. There are significant differences in the results depending on the aerosol microphysical module used. Different spatio-temporal injection strategies have a significant impact on the magnitude and zonal distribution of radiative forcing and atmospheric dynamics.
Elizaveta Malinina, Alexei Rozanov, Ulrike Niemeier, Sandra Wallis, Carlo Arosio, Felix Wrana, Claudia Timmreck, Christian von Savigny, and John P. Burrows
Atmos. Chem. Phys., 21, 14871–14891, https://doi.org/10.5194/acp-21-14871-2021, https://doi.org/10.5194/acp-21-14871-2021, 2021
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In the paper, changes in the stratospheric aerosol loading after the 2018 Ambae eruption were analyzed using OMPS-LP observations. The eruption was also simulated with the MAECHAM5-HAM global climate model. Generally, the model and observations agree very well. We attribute the good consistency of the results to a precisely determined altitude and mass of the volcanic injection, as well as nudging of the meteorological data. The radiative forcing from the eruption was estimated to be −0.13 W m−2.
Daniele Visioni, Douglas G. MacMartin, Ben Kravitz, Olivier Boucher, Andy Jones, Thibaut Lurton, Michou Martine, Michael J. Mills, Pierre Nabat, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 10039–10063, https://doi.org/10.5194/acp-21-10039-2021, https://doi.org/10.5194/acp-21-10039-2021, 2021
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A new set of simulations is used to investigate commonalities, differences and sources of uncertainty when simulating the injection of SO2 in the stratosphere in order to mitigate the effects of climate change (solar geoengineering). The models differ in how they simulate the aerosols and how they spread around the stratosphere, resulting in differences in projected regional impacts. Overall, however, the models agree that aerosols have the potential to mitigate the warming produced by GHGs.
Henning Franke, Ulrike Niemeier, and Daniele Visioni
Atmos. Chem. Phys., 21, 8615–8635, https://doi.org/10.5194/acp-21-8615-2021, https://doi.org/10.5194/acp-21-8615-2021, 2021
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Stratospheric aerosol modification (SAM) can alter the quasi-biennial oscillation (QBO). Our simulations with two different models show that the characteristics of the QBO response are primarily determined by the meridional structure of the aerosol-induced heating. Therefore, the QBO response to SAM depends primarily on the location of injection, while injection type and rate act to scale the specific response. Our results have important implications for evaluating adverse side effects of SAM.
Ben Kravitz, Douglas G. MacMartin, Daniele Visioni, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Andy Jones, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Alan Robock, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 4231–4247, https://doi.org/10.5194/acp-21-4231-2021, https://doi.org/10.5194/acp-21-4231-2021, 2021
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This study investigates multi-model response to idealized geoengineering (high CO2 with solar reduction) across two different generations of climate models. We find that, with the exception of a few cases, the results are unchanged between the different generations. This gives us confidence that broad conclusions about the response to idealized geoengineering are robust.
Ulrike Niemeier, Felix Riede, and Claudia Timmreck
Clim. Past, 17, 633–652, https://doi.org/10.5194/cp-17-633-2021, https://doi.org/10.5194/cp-17-633-2021, 2021
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The 13 kyr BP Laacher See eruption impacted local environments, human communities and climate. We have simulated the evolution of its fine ash and sulfur cloud such that it reflects the empirically known ash distribution. In our models, the heating of the ash causes a mesocyclone which changes the dispersion of the cloud itself, resulting in enhanced transport to low latitudes. This may partially explain why no Laacher See ash has yet been found in Greenlandic ice cores.
Margot Clyne, Jean-Francois Lamarque, Michael J. Mills, Myriam Khodri, William Ball, Slimane Bekki, Sandip S. Dhomse, Nicolas Lebas, Graham Mann, Lauren Marshall, Ulrike Niemeier, Virginie Poulain, Alan Robock, Eugene Rozanov, Anja Schmidt, Andrea Stenke, Timofei Sukhodolov, Claudia Timmreck, Matthew Toohey, Fiona Tummon, Davide Zanchettin, Yunqian Zhu, and Owen B. Toon
Atmos. Chem. Phys., 21, 3317–3343, https://doi.org/10.5194/acp-21-3317-2021, https://doi.org/10.5194/acp-21-3317-2021, 2021
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This study finds how and why five state-of-the-art global climate models with interactive stratospheric aerosols differ when simulating the aftermath of large volcanic injections as part of the Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP). We identify and explain the consequences of significant disparities in the underlying physics and chemistry currently in some of the models, which are problems likely not unique to the models participating in this study.
Ulrike Niemeier, Jadwiga H. Richter, and Simone Tilmes
Atmos. Chem. Phys., 20, 8975–8987, https://doi.org/10.5194/acp-20-8975-2020, https://doi.org/10.5194/acp-20-8975-2020, 2020
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Artificial injections of SO2 into the tropical stratosphere show an impact on the quasi-biennial oscillation (QBO). Different numerical models show only qualitatively but not quantitatively consistent impacts. We show for two models that the response of the QBO is similar when a similar stratospheric heating rate is induced by SO2 injections of different amounts. The reason is very different vertical advection in the two models resulting in different aerosol burden and heating of the aerosols.
Ulrike Niemeier, Claudia Timmreck, and Kirstin Krüger
Atmos. Chem. Phys., 19, 10379–10390, https://doi.org/10.5194/acp-19-10379-2019, https://doi.org/10.5194/acp-19-10379-2019, 2019
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In 1963 Mt. Agung, Indonesia, showed unrest for several months. During this period,
two medium-sized eruptions injected SO2 into the stratosphere. Recent volcanic emission datasets include only one large eruption phase. Therefore, we compared model experiments, with (a) one larger eruption and (b) two eruptions as observed. The evolution of the volcanic cloud differs significantly between the two experiments. Both climatic eruptions should be taken into account.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Lauren Marshall, Anja Schmidt, Matthew Toohey, Ken S. Carslaw, Graham W. Mann, Michael Sigl, Myriam Khodri, Claudia Timmreck, Davide Zanchettin, William T. Ball, Slimane Bekki, James S. A. Brooke, Sandip Dhomse, Colin Johnson, Jean-Francois Lamarque, Allegra N. LeGrande, Michael J. Mills, Ulrike Niemeier, James O. Pope, Virginie Poulain, Alan Robock, Eugene Rozanov, Andrea Stenke, Timofei Sukhodolov, Simone Tilmes, Kostas Tsigaridis, and Fiona Tummon
Atmos. Chem. Phys., 18, 2307–2328, https://doi.org/10.5194/acp-18-2307-2018, https://doi.org/10.5194/acp-18-2307-2018, 2018
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We use four global aerosol models to compare the simulated sulfate deposition from the 1815 Mt. Tambora eruption to ice core records. Inter-model volcanic sulfate deposition differs considerably. Volcanic sulfate deposited on polar ice sheets is used to estimate the atmospheric sulfate burden and subsequently radiative forcing of historic eruptions. Our results suggest that deriving such relationships from model simulations may be associated with greater uncertainties than previously thought.
Camilla W. Stjern, Helene Muri, Lars Ahlm, Olivier Boucher, Jason N. S. Cole, Duoying Ji, Andy Jones, Jim Haywood, Ben Kravitz, Andrew Lenton, John C. Moore, Ulrike Niemeier, Steven J. Phipps, Hauke Schmidt, Shingo Watanabe, and Jón Egill Kristjánsson
Atmos. Chem. Phys., 18, 621–634, https://doi.org/10.5194/acp-18-621-2018, https://doi.org/10.5194/acp-18-621-2018, 2018
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Marine cloud brightening (MCB) has been proposed to help limit global warming. We present here the first multi-model assessment of idealized MCB simulations from the Geoengineering Model Intercomparison Project. While all models predict a global cooling as intended, there is considerable spread between the models both in terms of radiative forcing and the climate response, largely linked to the substantial differences in the models' representation of clouds.
Davide Zanchettin, Myriam Khodri, Claudia Timmreck, Matthew Toohey, Anja Schmidt, Edwin P. Gerber, Gabriele Hegerl, Alan Robock, Francesco S. R. Pausata, William T. Ball, Susanne E. Bauer, Slimane Bekki, Sandip S. Dhomse, Allegra N. LeGrande, Graham W. Mann, Lauren Marshall, Michael Mills, Marion Marchand, Ulrike Niemeier, Virginie Poulain, Eugene Rozanov, Angelo Rubino, Andrea Stenke, Kostas Tsigaridis, and Fiona Tummon
Geosci. Model Dev., 9, 2701–2719, https://doi.org/10.5194/gmd-9-2701-2016, https://doi.org/10.5194/gmd-9-2701-2016, 2016
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Simulating volcanically-forced climate variability is a challenging task for climate models. The Model Intercomparison Project on the climatic response to volcanic forcing (VolMIP) – an endorsed contribution to CMIP6 – defines a protocol for idealized volcanic-perturbation experiments to improve comparability of results across different climate models. This paper illustrates the design of VolMIP's experiments and describes the aerosol forcing input datasets to be used.
A. Laakso, H. Kokkola, A.-I. Partanen, U. Niemeier, C. Timmreck, K. E. J. Lehtinen, H. Hakkarainen, and H. Korhonen
Atmos. Chem. Phys., 16, 305–323, https://doi.org/10.5194/acp-16-305-2016, https://doi.org/10.5194/acp-16-305-2016, 2016
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We have studied the impacts of a volcanic eruption during solar radiation management (SRM) using an aerosol-climate model ECHAM5-HAM-SALSA and an Earth system model MPI-ESM. A volcanic eruption during stratospheric sulfur geoengineering would lead to larger particles and smaller amount of new particles than if an volcano erupts in normal atmospheric conditions. Thus, volcanic eruption during SRM would lead to only a small additional cooling which would last for a significantly shorter period.
B. Kravitz, A. Robock, S. Tilmes, O. Boucher, J. M. English, P. J. Irvine, A. Jones, M. G. Lawrence, M. MacCracken, H. Muri, J. C. Moore, U. Niemeier, S. J. Phipps, J. Sillmann, T. Storelvmo, H. Wang, and S. Watanabe
Geosci. Model Dev., 8, 3379–3392, https://doi.org/10.5194/gmd-8-3379-2015, https://doi.org/10.5194/gmd-8-3379-2015, 2015
V. N. Aswathy, O. Boucher, M. Quaas, U. Niemeier, H. Muri, J. Mülmenstädt, and J. Quaas
Atmos. Chem. Phys., 15, 9593–9610, https://doi.org/10.5194/acp-15-9593-2015, https://doi.org/10.5194/acp-15-9593-2015, 2015
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Simulations conducted in the GeoMIP and IMPLICC model intercomparison studies for climate engineering by stratospheric sulfate injection and marine cloud brightening via sea salt are analysed and compared to the reference scenario RCP4.5. The focus is on extremes in surface temperature and precipitation. It is found that the extreme changes mostly follow the mean changes and that extremes are also in general well mitigated, except for in polar regions.
U. Niemeier and C. Timmreck
Atmos. Chem. Phys., 15, 9129–9141, https://doi.org/10.5194/acp-15-9129-2015, https://doi.org/10.5194/acp-15-9129-2015, 2015
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The injection of sulfur dioxide is considered as an option for solar radiation management. We have calculated the effects of SO2 injections up to 100 Tg(S)/y. Our calculations show that the forcing efficiency of the injection decays exponentially. This result implies that SO2 injections in the order of 6 times Mt. Pinatubo eruptions per year are required to keep temperatures constant at that anticipated for 2020, whilst maintaining business as usual emission conditions.
S. Tilmes, M. J. Mills, U. Niemeier, H. Schmidt, A. Robock, B. Kravitz, J.-F. Lamarque, G. Pitari, and J. M. English
Geosci. Model Dev., 8, 43–49, https://doi.org/10.5194/gmd-8-43-2015, https://doi.org/10.5194/gmd-8-43-2015, 2015
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A new Geoengineering Model Intercomparison Project (GeoMIP) experiment “G4 specified stratospheric aerosols” (G4SSA) is proposed to investigate the impact of stratospheric aerosol geoengineering on atmosphere, chemistry, dynamics, climate, and the environment. In contrast to the earlier G4 GeoMIP experiment, which requires an emission of sulfur dioxide (SO2) into the model, a prescribed aerosol forcing file is provided to the community, to be consistently applied to future model experiments.
Daniele Visioni, Ben Kravitz, Alan Robock, Simone Tilmes, Jim Haywood, Olivier Boucher, Mark Lawrence, Peter Irvine, Ulrike Niemeier, Lili Xia, Gabriel Chiodo, Chris Lennard, Shingo Watanabe, John C. Moore, and Helene Muri
Atmos. Chem. Phys., 23, 5149–5176, https://doi.org/10.5194/acp-23-5149-2023, https://doi.org/10.5194/acp-23-5149-2023, 2023
Short summary
Short summary
Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.
Felix Wrana, Ulrike Niemeier, Larry W. Thomason, Sandra Wallis, and Christian von Savigny
EGUsphere, https://doi.org/10.5194/egusphere-2023-837, https://doi.org/10.5194/egusphere-2023-837, 2023
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
The stratospheric aerosol layer is a naturally occuring and permanent layer of aerosol, in this case very small droplets of mostly sulfuric acid and water, that has a cooling effect on our climate. To quantify this effect and for our general understanding of stratospheric microphysical processes, knowledge of the size of those aerosol particles is needed. Using satellite measurements and atmospheric models we show, that some volcanic eruptions can lead to on average smaller aerosol sizes.
Cathy Hohenegger, Peter Korn, Leonidas Linardakis, René Redler, Reiner Schnur, Panagiotis Adamidis, Jiawei Bao, Swantje Bastin, Milad Behravesh, Martin Bergemann, Joachim Biercamp, Hendryk Bockelmann, Renate Brokopf, Nils Brüggemann, Lucas Casaroli, Fatemeh Chegini, George Datseris, Monika Esch, Geet George, Marco Giorgetta, Oliver Gutjahr, Helmuth Haak, Moritz Hanke, Tatiana Ilyina, Thomas Jahns, Johann Jungclaus, Marcel Kern, Daniel Klocke, Lukas Kluft, Tobias Kölling, Luis Kornblueh, Sergey Kosukhin, Clarissa Kroll, Junhong Lee, Thorsten Mauritsen, Carolin Mehlmann, Theresa Mieslinger, Ann Kristin Naumann, Laura Paccini, Angel Peinado, Divya Sri Praturi, Dian Putrasahan, Sebastian Rast, Thomas Riddick, Niklas Roeber, Hauke Schmidt, Uwe Schulzweida, Florian Schütte, Hans Segura, Radomyra Shevchenko, Vikram Singh, Mia Specht, Claudia Christine Stephan, Jin-Song von Storch, Raphaela Vogel, Christian Wengel, Marius Winkler, Florian Ziemen, Jochem Marotzke, and Bjorn Stevens
Geosci. Model Dev., 16, 779–811, https://doi.org/10.5194/gmd-16-779-2023, https://doi.org/10.5194/gmd-16-779-2023, 2023
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Models of the Earth system used to understand climate and predict its change typically employ a grid spacing of about 100 km. Yet, many atmospheric and oceanic processes occur on much smaller scales. In this study, we present a new model configuration designed for the simulation of the components of the Earth system and their interactions at kilometer and smaller scales, allowing an explicit representation of the main drivers of the flow of energy and matter by solving the underlying equations.
Yangxin Chen, Duoying Ji, Qian Zhang, John C. Moore, Olivier Boucher, Andy Jones, Thibaut Lurton, Michael J. Mills, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Earth Syst. Dynam., 14, 55–79, https://doi.org/10.5194/esd-14-55-2023, https://doi.org/10.5194/esd-14-55-2023, 2023
Short summary
Short summary
Solar geoengineering has been proposed as a way of counteracting the warming effects of increasing greenhouse gases by reflecting solar radiation. This work shows that solar geoengineering can slow down the northern-high-latitude permafrost degradation but cannot preserve the permafrost ecosystem as that under a climate of the same warming level without solar geoengineering.
Ilaria Quaglia, Claudia Timmreck, Ulrike Niemeier, Daniele Visioni, Giovanni Pitari, Christina Brodowsky, Christoph Brühl, Sandip S. Dhomse, Henning Franke, Anton Laakso, Graham W. Mann, Eugene Rozanov, and Timofei Sukhodolov
Atmos. Chem. Phys., 23, 921–948, https://doi.org/10.5194/acp-23-921-2023, https://doi.org/10.5194/acp-23-921-2023, 2023
Short summary
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The last very large explosive volcanic eruption we have measurements for is the eruption of Mt. Pinatubo in 1991. It is therefore often used as a benchmark for climate models' ability to reproduce these kinds of events. Here, we compare available measurements with the results from multiple experiments conducted with climate models interactively simulating the aerosol cloud formation.
Sandra Wallis, Hauke Schmidt, and Christian von Savigny
EGUsphere, https://doi.org/10.5194/egusphere-2023-20, https://doi.org/10.5194/egusphere-2023-20, 2023
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Strong volcanic eruptions are able to alter the temperature and the circulation of the middle atmosphere. This study simulates the atmospheric response to an idealized strong tropical eruption and focuses on the impact on the mesosphere. The simulations show a warming of the polar summer mesopause in the first November after the eruption. Our study indicate that this is mainly due to dynamical coupling in the summer hemisphere with a potential contribution from interhemispheric coupling.
Shih-Wei Fang, Claudia Timmreck, Johann Jungclaus, Kirstin Krüger, and Hauke Schmidt
Earth Syst. Dynam., 13, 1535–1555, https://doi.org/10.5194/esd-13-1535-2022, https://doi.org/10.5194/esd-13-1535-2022, 2022
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The early 19th century was the coldest period over the past 500 years, when strong tropical volcanic events and a solar minimum coincided. This study quantifies potential surface cooling from the solar and volcanic forcing in the early 19th century with large ensemble simulations, and identifies the regions that their impacts cannot be simply additive. The cooling perspective of Arctic amplification exists in both solar and post-volcano period with the albedo feedback as the main contribution.
Simone Tilmes, Daniele Visioni, Andy Jones, James Haywood, Roland Séférian, Pierre Nabat, Olivier Boucher, Ewa Monica Bednarz, and Ulrike Niemeier
Atmos. Chem. Phys., 22, 4557–4579, https://doi.org/10.5194/acp-22-4557-2022, https://doi.org/10.5194/acp-22-4557-2022, 2022
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This study assesses the impacts of climate interventions, using stratospheric sulfate aerosol and solar dimming on stratospheric ozone, based on three Earth system models with interactive stratospheric chemistry. The climate interventions have been applied to a high emission (baseline) scenario in order to reach global surface temperatures of a medium emission scenario. We find significant increases and decreases in total column ozone, depending on regions and seasons.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
Short summary
Short summary
Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Debra K. Weisenstein, Daniele Visioni, Henning Franke, Ulrike Niemeier, Sandro Vattioni, Gabriel Chiodo, Thomas Peter, and David W. Keith
Atmos. Chem. Phys., 22, 2955–2973, https://doi.org/10.5194/acp-22-2955-2022, https://doi.org/10.5194/acp-22-2955-2022, 2022
Short summary
Short summary
This paper explores a potential method of geoengineering that could be used to slow the rate of change of climate over decadal scales. We use three climate models to explore how injections of accumulation-mode sulfuric acid aerosol change the large-scale stratospheric particle size distribution and radiative forcing response for the chosen scenarios. Radiative forcing per unit sulfur injected and relative to the change in aerosol burden is larger with particulate than with SO2 injections.
Anton Laakso, Ulrike Niemeier, Daniele Visioni, Simone Tilmes, and Harri Kokkola
Atmos. Chem. Phys., 22, 93–118, https://doi.org/10.5194/acp-22-93-2022, https://doi.org/10.5194/acp-22-93-2022, 2022
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The use of different spatio-temporal sulfur injection strategies with different magnitudes to create an artificial reflective aerosol layer to cool the climate is studied using sectional and modal aerosol schemes in a climate model. There are significant differences in the results depending on the aerosol microphysical module used. Different spatio-temporal injection strategies have a significant impact on the magnitude and zonal distribution of radiative forcing and atmospheric dynamics.
Mohammad M. Khabbazan, Marius Stankoweit, Elnaz Roshan, Hauke Schmidt, and Hermann Held
Earth Syst. Dynam., 12, 1529–1542, https://doi.org/10.5194/esd-12-1529-2021, https://doi.org/10.5194/esd-12-1529-2021, 2021
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We ask for an optimal amount of solar radiation management (SRM) in conjunction with mitigation if global warming is limited to 2 °C and regional precipitation anomalies are confined to an amount ethically compatible with the 2 °C target. Then, compared to a scenario without regional targets, most of the SRM usage is eliminated from the portfolio even if transgressing regional targets are tolerated in terms of 1/10 of the standard deviation of natural variability.
Elizaveta Malinina, Alexei Rozanov, Ulrike Niemeier, Sandra Wallis, Carlo Arosio, Felix Wrana, Claudia Timmreck, Christian von Savigny, and John P. Burrows
Atmos. Chem. Phys., 21, 14871–14891, https://doi.org/10.5194/acp-21-14871-2021, https://doi.org/10.5194/acp-21-14871-2021, 2021
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In the paper, changes in the stratospheric aerosol loading after the 2018 Ambae eruption were analyzed using OMPS-LP observations. The eruption was also simulated with the MAECHAM5-HAM global climate model. Generally, the model and observations agree very well. We attribute the good consistency of the results to a precisely determined altitude and mass of the volcanic injection, as well as nudging of the meteorological data. The radiative forcing from the eruption was estimated to be −0.13 W m−2.
Gunter Stober, Ales Kuchar, Dimitry Pokhotelov, Huixin Liu, Han-Li Liu, Hauke Schmidt, Christoph Jacobi, Kathrin Baumgarten, Peter Brown, Diego Janches, Damian Murphy, Alexander Kozlovsky, Mark Lester, Evgenia Belova, Johan Kero, and Nicholas Mitchell
Atmos. Chem. Phys., 21, 13855–13902, https://doi.org/10.5194/acp-21-13855-2021, https://doi.org/10.5194/acp-21-13855-2021, 2021
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Little is known about the climate change of wind systems in the mesosphere and lower thermosphere at the edge of space at altitudes from 70–110 km. Meteor radars represent a well-accepted remote sensing technique to measure winds at these altitudes. Here we present a state-of-the-art climatological interhemispheric comparison using continuous and long-lasting observations from worldwide distributed meteor radars from the Arctic to the Antarctic and sophisticated general circulation models.
Daniele Visioni, Douglas G. MacMartin, Ben Kravitz, Olivier Boucher, Andy Jones, Thibaut Lurton, Michou Martine, Michael J. Mills, Pierre Nabat, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 10039–10063, https://doi.org/10.5194/acp-21-10039-2021, https://doi.org/10.5194/acp-21-10039-2021, 2021
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A new set of simulations is used to investigate commonalities, differences and sources of uncertainty when simulating the injection of SO2 in the stratosphere in order to mitigate the effects of climate change (solar geoengineering). The models differ in how they simulate the aerosols and how they spread around the stratosphere, resulting in differences in projected regional impacts. Overall, however, the models agree that aerosols have the potential to mitigate the warming produced by GHGs.
Henning Franke, Ulrike Niemeier, and Daniele Visioni
Atmos. Chem. Phys., 21, 8615–8635, https://doi.org/10.5194/acp-21-8615-2021, https://doi.org/10.5194/acp-21-8615-2021, 2021
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Stratospheric aerosol modification (SAM) can alter the quasi-biennial oscillation (QBO). Our simulations with two different models show that the characteristics of the QBO response are primarily determined by the meridional structure of the aerosol-induced heating. Therefore, the QBO response to SAM depends primarily on the location of injection, while injection type and rate act to scale the specific response. Our results have important implications for evaluating adverse side effects of SAM.
Clarissa Alicia Kroll, Sally Dacie, Alon Azoulay, Hauke Schmidt, and Claudia Timmreck
Atmos. Chem. Phys., 21, 6565–6591, https://doi.org/10.5194/acp-21-6565-2021, https://doi.org/10.5194/acp-21-6565-2021, 2021
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Volcanic forcing is counteracted by stratospheric water vapor (SWV) entering the stratosphere as a consequence of aerosol-induced cold-point warming. We find that depending on the emission strength, aerosol profile height and season of the eruption, up to 4 % of the tropical aerosol forcing can be counterbalanced. A power function relationship between cold-point warming/SWV forcing and AOD in the yearly average is found, allowing us to estimate the SWV forcing for comparable eruptions.
Ben Kravitz, Douglas G. MacMartin, Daniele Visioni, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Andy Jones, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Alan Robock, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 4231–4247, https://doi.org/10.5194/acp-21-4231-2021, https://doi.org/10.5194/acp-21-4231-2021, 2021
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This study investigates multi-model response to idealized geoengineering (high CO2 with solar reduction) across two different generations of climate models. We find that, with the exception of a few cases, the results are unchanged between the different generations. This gives us confidence that broad conclusions about the response to idealized geoengineering are robust.
Ulrike Niemeier, Felix Riede, and Claudia Timmreck
Clim. Past, 17, 633–652, https://doi.org/10.5194/cp-17-633-2021, https://doi.org/10.5194/cp-17-633-2021, 2021
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The 13 kyr BP Laacher See eruption impacted local environments, human communities and climate. We have simulated the evolution of its fine ash and sulfur cloud such that it reflects the empirically known ash distribution. In our models, the heating of the ash causes a mesocyclone which changes the dispersion of the cloud itself, resulting in enhanced transport to low latitudes. This may partially explain why no Laacher See ash has yet been found in Greenlandic ice cores.
Margot Clyne, Jean-Francois Lamarque, Michael J. Mills, Myriam Khodri, William Ball, Slimane Bekki, Sandip S. Dhomse, Nicolas Lebas, Graham Mann, Lauren Marshall, Ulrike Niemeier, Virginie Poulain, Alan Robock, Eugene Rozanov, Anja Schmidt, Andrea Stenke, Timofei Sukhodolov, Claudia Timmreck, Matthew Toohey, Fiona Tummon, Davide Zanchettin, Yunqian Zhu, and Owen B. Toon
Atmos. Chem. Phys., 21, 3317–3343, https://doi.org/10.5194/acp-21-3317-2021, https://doi.org/10.5194/acp-21-3317-2021, 2021
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This study finds how and why five state-of-the-art global climate models with interactive stratospheric aerosols differ when simulating the aftermath of large volcanic injections as part of the Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP). We identify and explain the consequences of significant disparities in the underlying physics and chemistry currently in some of the models, which are problems likely not unique to the models participating in this study.
Cathy W. Y. Li, Guy P. Brasseur, Hauke Schmidt, and Juan Pedro Mellado
Atmos. Chem. Phys., 21, 483–503, https://doi.org/10.5194/acp-21-483-2021, https://doi.org/10.5194/acp-21-483-2021, 2021
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Intense and localised emissions of pollutants are common in urban environments, in which turbulence cannot mix these segregated pollutants efficiently in the atmosphere. Despite their relatively high resolution, regional models cannot resolve such segregation and assume instantaneous mixing of these pollutants in their model grids, which potentially induces significant error in the subsequent chemical calculation, based on our calculation with a model that explicitly resolves turbulent motions.
Ulrike Niemeier, Jadwiga H. Richter, and Simone Tilmes
Atmos. Chem. Phys., 20, 8975–8987, https://doi.org/10.5194/acp-20-8975-2020, https://doi.org/10.5194/acp-20-8975-2020, 2020
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Artificial injections of SO2 into the tropical stratosphere show an impact on the quasi-biennial oscillation (QBO). Different numerical models show only qualitatively but not quantitatively consistent impacts. We show for two models that the response of the QBO is similar when a similar stratospheric heating rate is induced by SO2 injections of different amounts. The reason is very different vertical advection in the two models resulting in different aerosol burden and heating of the aerosols.
Katja Matthes, Arne Biastoch, Sebastian Wahl, Jan Harlaß, Torge Martin, Tim Brücher, Annika Drews, Dana Ehlert, Klaus Getzlaff, Fritz Krüger, Willi Rath, Markus Scheinert, Franziska U. Schwarzkopf, Tobias Bayr, Hauke Schmidt, and Wonsun Park
Geosci. Model Dev., 13, 2533–2568, https://doi.org/10.5194/gmd-13-2533-2020, https://doi.org/10.5194/gmd-13-2533-2020, 2020
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A new Earth system model, the Flexible Ocean and Climate Infrastructure (FOCI), is introduced, consisting of a high-top atmosphere, an ocean model, sea-ice and land surface model components. A unique feature of FOCI is the ability to explicitly resolve small-scale oceanic features, for example, the Agulhas Current and the Gulf Stream. It allows to study the evolution of the climate system on regional and seasonal to (multi)decadal scales and bridges the gap to coarse-resolution climate models.
Ulrike Niemeier, Claudia Timmreck, and Kirstin Krüger
Atmos. Chem. Phys., 19, 10379–10390, https://doi.org/10.5194/acp-19-10379-2019, https://doi.org/10.5194/acp-19-10379-2019, 2019
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In 1963 Mt. Agung, Indonesia, showed unrest for several months. During this period,
two medium-sized eruptions injected SO2 into the stratosphere. Recent volcanic emission datasets include only one large eruption phase. Therefore, we compared model experiments, with (a) one larger eruption and (b) two eruptions as observed. The evolution of the volcanic cloud differs significantly between the two experiments. Both climatic eruptions should be taken into account.
Sebastian Borchert, Guidi Zhou, Michael Baldauf, Hauke Schmidt, Günther Zängl, and Daniel Reinert
Geosci. Model Dev., 12, 3541–3569, https://doi.org/10.5194/gmd-12-3541-2019, https://doi.org/10.5194/gmd-12-3541-2019, 2019
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We present an upper-atmosphere extension of the ICOsahedral Non-hydrostatic (ICON) model.
This includes an extension of the model dynamics from a shallow to a deep atmosphere
and the implementation of upper-atmosphere physics parameterizations.
Idealized test cases and climate simulations are performed in order to evaluate this new configuration, named UA-ICON.
Ina Tegen, David Neubauer, Sylvaine Ferrachat, Colombe Siegenthaler-Le Drian, Isabelle Bey, Nick Schutgens, Philip Stier, Duncan Watson-Parris, Tanja Stanelle, Hauke Schmidt, Sebastian Rast, Harri Kokkola, Martin Schultz, Sabine Schroeder, Nikos Daskalakis, Stefan Barthel, Bernd Heinold, and Ulrike Lohmann
Geosci. Model Dev., 12, 1643–1677, https://doi.org/10.5194/gmd-12-1643-2019, https://doi.org/10.5194/gmd-12-1643-2019, 2019
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We describe a new version of the aerosol–climate model ECHAM–HAM and show tests of the model performance by comparing different aspects of the aerosol distribution with different datasets. The updated version of HAM contains improved descriptions of aerosol processes, including updated emission fields and cloud processes. While there are regional deviations between the model and observations, the model performs well overall.
Uwe Mikolajewicz, Florian Ziemen, Guido Cioni, Martin Claussen, Klaus Fraedrich, Marvin Heidkamp, Cathy Hohenegger, Diego Jimenez de la Cuesta, Marie-Luise Kapsch, Alexander Lemburg, Thorsten Mauritsen, Katharina Meraner, Niklas Röber, Hauke Schmidt, Katharina D. Six, Irene Stemmler, Talia Tamarin-Brodsky, Alexander Winkler, Xiuhua Zhu, and Bjorn Stevens
Earth Syst. Dynam., 9, 1191–1215, https://doi.org/10.5194/esd-9-1191-2018, https://doi.org/10.5194/esd-9-1191-2018, 2018
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Model experiments show that changing the sense of Earth's rotation has relatively little impact on the globally and zonally averaged energy budgets but leads to large shifts in continental climates and patterns of precipitation. The retrograde world is greener as the desert area shrinks. Deep water formation shifts from the North Atlantic to the North Pacific with subsequent changes in ocean overturning. Over large areas of the Indian Ocean, cyanobacteria dominate over bulk phytoplankton.
Ben Kravitz, Philip J. Rasch, Hailong Wang, Alan Robock, Corey Gabriel, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Duoying Ji, Andy Jones, Andrew Lenton, John C. Moore, Helene Muri, Ulrike Niemeier, Steven Phipps, Hauke Schmidt, Shingo Watanabe, Shuting Yang, and Jin-Ho Yoon
Atmos. Chem. Phys., 18, 13097–13113, https://doi.org/10.5194/acp-18-13097-2018, https://doi.org/10.5194/acp-18-13097-2018, 2018
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Marine cloud brightening has been proposed as a means of geoengineering/climate intervention, or deliberately altering the climate system to offset anthropogenic climate change. In idealized simulations that highlight contrasts between land and ocean, we find that the globe warms, including the ocean due to transport of heat from land. This study reinforces that no net energy input into the Earth system does not mean that temperature will necessarily remain unchanged.
Amanda C. Maycock, Katja Matthes, Susann Tegtmeier, Hauke Schmidt, Rémi Thiéblemont, Lon Hood, Hideharu Akiyoshi, Slimane Bekki, Makoto Deushi, Patrick Jöckel, Oliver Kirner, Markus Kunze, Marion Marchand, Daniel R. Marsh, Martine Michou, David Plummer, Laura E. Revell, Eugene Rozanov, Andrea Stenke, Yousuke Yamashita, and Kohei Yoshida
Atmos. Chem. Phys., 18, 11323–11343, https://doi.org/10.5194/acp-18-11323-2018, https://doi.org/10.5194/acp-18-11323-2018, 2018
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The 11-year solar cycle is an important driver of climate variability. Changes in incoming solar ultraviolet radiation affect atmospheric ozone, which in turn influences atmospheric temperatures. Constraining the impact of the solar cycle on ozone is therefore important for understanding climate variability. This study examines the representation of the solar influence on ozone in numerical models used to simulate past and future climate. We highlight important differences among model datasets.
J. Federico Conte, Jorge L. Chau, Fazlul I. Laskar, Gunter Stober, Hauke Schmidt, and Peter Brown
Ann. Geophys., 36, 999–1008, https://doi.org/10.5194/angeo-36-999-2018, https://doi.org/10.5194/angeo-36-999-2018, 2018
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Based on comparisons of meteor radar measurements with HAMMONIA model simulations, we show that the differences exhibited by the semidiurnal solar tide (S2) observed at middle and high latitudes of the Northern Hemisphere between equinox times are mainly due to distinct behaviors of the migrating semidiurnal (SW2) and the non-migrating westward-propagating wave number 1 semidiurnal (SW1) tidal components.
Martin G. Schultz, Scarlet Stadtler, Sabine Schröder, Domenico Taraborrelli, Bruno Franco, Jonathan Krefting, Alexandra Henrot, Sylvaine Ferrachat, Ulrike Lohmann, David Neubauer, Colombe Siegenthaler-Le Drian, Sebastian Wahl, Harri Kokkola, Thomas Kühn, Sebastian Rast, Hauke Schmidt, Philip Stier, Doug Kinnison, Geoffrey S. Tyndall, John J. Orlando, and Catherine Wespes
Geosci. Model Dev., 11, 1695–1723, https://doi.org/10.5194/gmd-11-1695-2018, https://doi.org/10.5194/gmd-11-1695-2018, 2018
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The chemistry–climate model ECHAM-HAMMOZ contains a detailed representation of tropospheric and stratospheric reactive chemistry and state-of-the-art parameterizations of aerosols. It thus allows for detailed investigations of chemical processes in the climate system. Evaluation of the model with various observational data yields good results, but the model has a tendency to produce too much OH in the tropics. This highlights the important interplay between atmospheric chemistry and dynamics.
Lauren Marshall, Anja Schmidt, Matthew Toohey, Ken S. Carslaw, Graham W. Mann, Michael Sigl, Myriam Khodri, Claudia Timmreck, Davide Zanchettin, William T. Ball, Slimane Bekki, James S. A. Brooke, Sandip Dhomse, Colin Johnson, Jean-Francois Lamarque, Allegra N. LeGrande, Michael J. Mills, Ulrike Niemeier, James O. Pope, Virginie Poulain, Alan Robock, Eugene Rozanov, Andrea Stenke, Timofei Sukhodolov, Simone Tilmes, Kostas Tsigaridis, and Fiona Tummon
Atmos. Chem. Phys., 18, 2307–2328, https://doi.org/10.5194/acp-18-2307-2018, https://doi.org/10.5194/acp-18-2307-2018, 2018
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We use four global aerosol models to compare the simulated sulfate deposition from the 1815 Mt. Tambora eruption to ice core records. Inter-model volcanic sulfate deposition differs considerably. Volcanic sulfate deposited on polar ice sheets is used to estimate the atmospheric sulfate burden and subsequently radiative forcing of historic eruptions. Our results suggest that deriving such relationships from model simulations may be associated with greater uncertainties than previously thought.
Katharina Meraner and Hauke Schmidt
Atmos. Chem. Phys., 18, 1079–1089, https://doi.org/10.5194/acp-18-1079-2018, https://doi.org/10.5194/acp-18-1079-2018, 2018
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Using a coupled Earth system model and radiative transfer modeling we show that the radiative forcing of a winter polar mesospheric ozone loss due to energetic particle precipitation is negligible. A climate impact of a mesospheric ozone loss as suggested by Andersson et al. (2014, Nature Communications) seems unlikely. A winter polar stratospheric ozone loss due to energetic particle precipitation leads to a small warming of the stratosphere, but only a few statistically significant changes.
Camilla W. Stjern, Helene Muri, Lars Ahlm, Olivier Boucher, Jason N. S. Cole, Duoying Ji, Andy Jones, Jim Haywood, Ben Kravitz, Andrew Lenton, John C. Moore, Ulrike Niemeier, Steven J. Phipps, Hauke Schmidt, Shingo Watanabe, and Jón Egill Kristjánsson
Atmos. Chem. Phys., 18, 621–634, https://doi.org/10.5194/acp-18-621-2018, https://doi.org/10.5194/acp-18-621-2018, 2018
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Marine cloud brightening (MCB) has been proposed to help limit global warming. We present here the first multi-model assessment of idealized MCB simulations from the Geoengineering Model Intercomparison Project. While all models predict a global cooling as intended, there is considerable spread between the models both in terms of radiative forcing and the climate response, largely linked to the substantial differences in the models' representation of clouds.
Johann H. Jungclaus, Edouard Bard, Mélanie Baroni, Pascale Braconnot, Jian Cao, Louise P. Chini, Tania Egorova, Michael Evans, J. Fidel González-Rouco, Hugues Goosse, George C. Hurtt, Fortunat Joos, Jed O. Kaplan, Myriam Khodri, Kees Klein Goldewijk, Natalie Krivova, Allegra N. LeGrande, Stephan J. Lorenz, Jürg Luterbacher, Wenmin Man, Amanda C. Maycock, Malte Meinshausen, Anders Moberg, Raimund Muscheler, Christoph Nehrbass-Ahles, Bette I. Otto-Bliesner, Steven J. Phipps, Julia Pongratz, Eugene Rozanov, Gavin A. Schmidt, Hauke Schmidt, Werner Schmutz, Andrew Schurer, Alexander I. Shapiro, Michael Sigl, Jason E. Smerdon, Sami K. Solanki, Claudia Timmreck, Matthew Toohey, Ilya G. Usoskin, Sebastian Wagner, Chi-Ju Wu, Kok Leng Yeo, Davide Zanchettin, Qiong Zhang, and Eduardo Zorita
Geosci. Model Dev., 10, 4005–4033, https://doi.org/10.5194/gmd-10-4005-2017, https://doi.org/10.5194/gmd-10-4005-2017, 2017
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Climate model simulations covering the last millennium provide context for the evolution of the modern climate and for the expected changes during the coming centuries. They can help identify plausible mechanisms underlying palaeoclimatic reconstructions. Here, we describe the forcing boundary conditions and the experimental protocol for simulations covering the pre-industrial millennium. We describe the PMIP4 past1000 simulations as contributions to CMIP6 and additional sensitivity experiments.
Bernd Funke, William Ball, Stefan Bender, Angela Gardini, V. Lynn Harvey, Alyn Lambert, Manuel López-Puertas, Daniel R. Marsh, Katharina Meraner, Holger Nieder, Sanna-Mari Päivärinta, Kristell Pérot, Cora E. Randall, Thomas Reddmann, Eugene Rozanov, Hauke Schmidt, Annika Seppälä, Miriam Sinnhuber, Timofei Sukhodolov, Gabriele P. Stiller, Natalia D. Tsvetkova, Pekka T. Verronen, Stefan Versick, Thomas von Clarmann, Kaley A. Walker, and Vladimir Yushkov
Atmos. Chem. Phys., 17, 3573–3604, https://doi.org/10.5194/acp-17-3573-2017, https://doi.org/10.5194/acp-17-3573-2017, 2017
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Simulations from eight atmospheric models have been compared to tracer and temperature observations from seven satellite instruments in order to evaluate the energetic particle indirect effect (EPP IE) during the perturbed northern hemispheric (NH) winter 2008/2009. Models are capable to reproduce the EPP IE in dynamically and geomagnetically quiescent NH winter conditions. The results emphasize the need for model improvements in the dynamical representation of elevated stratopause events.
Davide Zanchettin, Myriam Khodri, Claudia Timmreck, Matthew Toohey, Anja Schmidt, Edwin P. Gerber, Gabriele Hegerl, Alan Robock, Francesco S. R. Pausata, William T. Ball, Susanne E. Bauer, Slimane Bekki, Sandip S. Dhomse, Allegra N. LeGrande, Graham W. Mann, Lauren Marshall, Michael Mills, Marion Marchand, Ulrike Niemeier, Virginie Poulain, Eugene Rozanov, Angelo Rubino, Andrea Stenke, Kostas Tsigaridis, and Fiona Tummon
Geosci. Model Dev., 9, 2701–2719, https://doi.org/10.5194/gmd-9-2701-2016, https://doi.org/10.5194/gmd-9-2701-2016, 2016
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Simulating volcanically-forced climate variability is a challenging task for climate models. The Model Intercomparison Project on the climatic response to volcanic forcing (VolMIP) – an endorsed contribution to CMIP6 – defines a protocol for idealized volcanic-perturbation experiments to improve comparability of results across different climate models. This paper illustrates the design of VolMIP's experiments and describes the aerosol forcing input datasets to be used.
A. Laakso, H. Kokkola, A.-I. Partanen, U. Niemeier, C. Timmreck, K. E. J. Lehtinen, H. Hakkarainen, and H. Korhonen
Atmos. Chem. Phys., 16, 305–323, https://doi.org/10.5194/acp-16-305-2016, https://doi.org/10.5194/acp-16-305-2016, 2016
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We have studied the impacts of a volcanic eruption during solar radiation management (SRM) using an aerosol-climate model ECHAM5-HAM-SALSA and an Earth system model MPI-ESM. A volcanic eruption during stratospheric sulfur geoengineering would lead to larger particles and smaller amount of new particles than if an volcano erupts in normal atmospheric conditions. Thus, volcanic eruption during SRM would lead to only a small additional cooling which would last for a significantly shorter period.
B. Kravitz, A. Robock, S. Tilmes, O. Boucher, J. M. English, P. J. Irvine, A. Jones, M. G. Lawrence, M. MacCracken, H. Muri, J. C. Moore, U. Niemeier, S. J. Phipps, J. Sillmann, T. Storelvmo, H. Wang, and S. Watanabe
Geosci. Model Dev., 8, 3379–3392, https://doi.org/10.5194/gmd-8-3379-2015, https://doi.org/10.5194/gmd-8-3379-2015, 2015
V. N. Aswathy, O. Boucher, M. Quaas, U. Niemeier, H. Muri, J. Mülmenstädt, and J. Quaas
Atmos. Chem. Phys., 15, 9593–9610, https://doi.org/10.5194/acp-15-9593-2015, https://doi.org/10.5194/acp-15-9593-2015, 2015
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Simulations conducted in the GeoMIP and IMPLICC model intercomparison studies for climate engineering by stratospheric sulfate injection and marine cloud brightening via sea salt are analysed and compared to the reference scenario RCP4.5. The focus is on extremes in surface temperature and precipitation. It is found that the extreme changes mostly follow the mean changes and that extremes are also in general well mitigated, except for in polar regions.
U. Niemeier and C. Timmreck
Atmos. Chem. Phys., 15, 9129–9141, https://doi.org/10.5194/acp-15-9129-2015, https://doi.org/10.5194/acp-15-9129-2015, 2015
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The injection of sulfur dioxide is considered as an option for solar radiation management. We have calculated the effects of SO2 injections up to 100 Tg(S)/y. Our calculations show that the forcing efficiency of the injection decays exponentially. This result implies that SO2 injections in the order of 6 times Mt. Pinatubo eruptions per year are required to keep temperatures constant at that anticipated for 2020, whilst maintaining business as usual emission conditions.
S. Tilmes, M. J. Mills, U. Niemeier, H. Schmidt, A. Robock, B. Kravitz, J.-F. Lamarque, G. Pitari, and J. M. English
Geosci. Model Dev., 8, 43–49, https://doi.org/10.5194/gmd-8-43-2015, https://doi.org/10.5194/gmd-8-43-2015, 2015
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A new Geoengineering Model Intercomparison Project (GeoMIP) experiment “G4 specified stratospheric aerosols” (G4SSA) is proposed to investigate the impact of stratospheric aerosol geoengineering on atmosphere, chemistry, dynamics, climate, and the environment. In contrast to the earlier G4 GeoMIP experiment, which requires an emission of sulfur dioxide (SO2) into the model, a prescribed aerosol forcing file is provided to the community, to be consistently applied to future model experiments.
S. Studer, K. Hocke, A. Schanz, H. Schmidt, and N. Kämpfer
Atmos. Chem. Phys., 14, 5905–5919, https://doi.org/10.5194/acp-14-5905-2014, https://doi.org/10.5194/acp-14-5905-2014, 2014
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Stratosphere | Science Focus: Physics (physical properties and processes)
Including ash in UKESM1 model simulations of the Raikoke volcanic eruption reveals improved agreement with observations
Particle number concentrations and size distributions in the stratosphere: implications of nucleation mechanisms and particle microphysics
Interactive stratospheric aerosol models' response to different amounts and altitudes of SO2 injection during the 1991 Pinatubo eruption
Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 2: Stratospheric and free-tropospheric response
The effect of ash, water vapor, and heterogeneous chemistry on the evolution of a Pinatubo-size volcanic cloud
Opinion: How Nuclear Winter has Saved the World, So Far
Dynamical perturbation of the stratosphere by a pyrocumulonimbus injection of carbonaceous aerosols
Important role of stratospheric injection height for the distribution and radiative forcing of smoke aerosol from the 2019–2020 Australian wildfires
Volcanic stratospheric injections up to 160 Tg(S) yield a Eurasian winter warming indistinguishable from internal variability
Assessing the consequences of including aerosol absorption in potential stratospheric aerosol injection climate intervention strategies
An approach to sulfate geoengineering with surface emissions of carbonyl sulfide
Online treatment of eruption dynamics improves the volcanic ash and SO2 dispersion forecast: case of the 2019 Raikoke eruption
The impact of stratospheric aerosol intervention on the North Atlantic and Quasi-Biennial Oscillations in the Geoengineering Model Intercomparison Project (GeoMIP) G6sulfur experiment
An interactive stratospheric aerosol model intercomparison of solar geoengineering by stratospheric injection of SO2 or accumulation-mode sulfuric acid aerosols
Limitations of assuming internal mixing between different aerosol species: a case study with sulfate geoengineering simulations
Dependency of the impacts of geoengineering on the stratospheric sulfur injection strategy – Part 1: Intercomparison of modal and sectional aerosol modules
The long-term transport and radiative impacts of the 2017 British Columbia pyrocumulonimbus smoke aerosols in the stratosphere
Identifying the sources of uncertainty in climate model simulations of solar radiation modification with the G6sulfur and G6solar Geoengineering Model Intercomparison Project (GeoMIP) simulations
Harnessing stratospheric diffusion barriers for enhanced climate geoengineering
Comparing different generations of idealized solar geoengineering simulations in the Geoengineering Model Intercomparison Project (GeoMIP)
Model physics and chemistry causing intermodel disagreement within the VolMIP-Tambora Interactive Stratospheric Aerosol ensemble
North Atlantic Oscillation response in GeoMIP experiments G6solar and G6sulfur: why detailed modelling is needed for understanding regional implications of solar radiation management
Scant evidence for a volcanically forced winter warming over Eurasia following the Krakatau eruption of August 1883
Differing responses of the quasi-biennial oscillation to artificial SO2 injections in two global models
Revisiting the Agung 1963 volcanic forcing – impact of one or two eruptions
Northern Hemisphere continental winter warming following the 1991 Mt. Pinatubo eruption: reconciling models and observations
Upper tropospheric ice sensitivity to sulfate geoengineering
Stratospheric aerosol radiative forcing simulated by the chemistry climate model EMAC using Aerosol CCI satellite data
Dynamical response of Mediterranean precipitation to greenhouse gases and aerosols
Global radiative effects of solid fuel cookstove aerosol emissions
Model simulations of the chemical and aerosol microphysical evolution of the Sarychev Peak 2009 eruption cloud compared to in situ and satellite observations
Sensitivity of the radiative forcing by stratospheric sulfur geoengineering to the amount and strategy of the SO2injection studied with the LMDZ-S3A model
Sulfur deposition changes under sulfate geoengineering conditions: quasi-biennial oscillation effects on the transport and lifetime of stratospheric aerosols
Equatorward dispersion of a high-latitude volcanic plume and its relation to the Asian summer monsoon: a case study of the Sarychev eruption in 2009
Sulfate geoengineering impact on methane transport and lifetime: results from the Geoengineering Model Intercomparison Project (GeoMIP)
Nucleation modeling of the Antarctic stratospheric CN layer and derivation of sulfuric acid profiles
Radiative and climate effects of stratospheric sulfur geoengineering using seasonally varying injection areas
Volcanic ash modeling with the online NMMB-MONARCH-ASH v1.0 model: model description, case simulation, and evaluation
Sulfate geoengineering: a review of the factors controlling the needed injection of sulfur dioxide
Climatic impacts of stratospheric geoengineering with sulfate, black carbon and titania injection
Radiative and climate impacts of a large volcanic eruption during stratospheric sulfur geoengineering
Climate extremes in multi-model simulations of stratospheric aerosol and marine cloud brightening climate engineering
What is the limit of climate engineering by stratospheric injection of SO2?
Quasi-biennial oscillation of the tropical stratospheric aerosol layer
The impact of volcanic aerosol on the Northern Hemisphere stratospheric polar vortex: mechanisms and sensitivity to forcing structure
Modeling the stratospheric warming following the Mt. Pinatubo eruption: uncertainties in aerosol extinctions
Transport of aerosols into the UTLS and their impact on the Asian monsoon region as seen in a global model simulation
Could aerosol emissions be used for regional heat wave mitigation?
The influence of eruption season on the global aerosol evolution and radiative impact of tropical volcanic eruptions
Microphysical simulations of new particle formation in the upper troposphere and lower stratosphere
Alice F. Wells, Andy Jones, Martin Osborne, Lilly Damany-Pearce, Daniel G. Partridge, and James M. Haywood
Atmos. Chem. Phys., 23, 3985–4007, https://doi.org/10.5194/acp-23-3985-2023, https://doi.org/10.5194/acp-23-3985-2023, 2023
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In 2019 the Raikoke volcano erupted explosively, emitting the largest injection of SO2 into the stratosphere since 2011. Observations indicated that a large amount of volcanic ash was also injected. Previous studies have identified that volcanic ash can prolong the lifetime of stratospheric aerosol optical depth, which we explore in UKESM1. Comparisons to observations suggest that including ash in model emission schemes can improve the representation of volcanic plumes in global climate models.
Fangqun Yu, Gan Luo, Arshad Arjunan Nair, Sebastian Eastham, Christina J. Williamson, Agnieszka Kupc, and Charles A. Brock
Atmos. Chem. Phys., 23, 1863–1877, https://doi.org/10.5194/acp-23-1863-2023, https://doi.org/10.5194/acp-23-1863-2023, 2023
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Particle number concentrations and size distributions in the stratosphere are studied through model simulations and comparisons with measurements. The nucleation scheme used in most of the solar geoengineering modeling studies overpredicts the nucleation rates and particle number concentrations in the stratosphere. The model based on updated nucleation schemes captures reasonably well some aspects of particle size distributions but misses some features. The possible reasons are discussed.
Ilaria Quaglia, Claudia Timmreck, Ulrike Niemeier, Daniele Visioni, Giovanni Pitari, Christina Brodowsky, Christoph Brühl, Sandip S. Dhomse, Henning Franke, Anton Laakso, Graham W. Mann, Eugene Rozanov, and Timofei Sukhodolov
Atmos. Chem. Phys., 23, 921–948, https://doi.org/10.5194/acp-23-921-2023, https://doi.org/10.5194/acp-23-921-2023, 2023
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The last very large explosive volcanic eruption we have measurements for is the eruption of Mt. Pinatubo in 1991. It is therefore often used as a benchmark for climate models' ability to reproduce these kinds of events. Here, we compare available measurements with the results from multiple experiments conducted with climate models interactively simulating the aerosol cloud formation.
Ewa M. Bednarz, Daniele Visioni, Ben Kravitz, Andy Jones, James M. Haywood, Jadwiga Richter, Douglas G. MacMartin, and Peter Braesicke
Atmos. Chem. Phys., 23, 687–709, https://doi.org/10.5194/acp-23-687-2023, https://doi.org/10.5194/acp-23-687-2023, 2023
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Building on Part 1 of this two-part study, we demonstrate the role of biases in climatological circulation and specific aspects of model microphysics in driving the differences in simulated sulfate distributions amongst three Earth system models. We then characterize the simulated changes in stratospheric and free-tropospheric temperatures, ozone, water vapor, and large-scale circulation, elucidating the role of the above aspects in the surface responses discussed in Part 1.
Mohamed Abdelkader, Georgiy Stenchikov, Andrea Pozzer, Holger Tost, and Jos Lelieveld
Atmos. Chem. Phys., 23, 471–500, https://doi.org/10.5194/acp-23-471-2023, https://doi.org/10.5194/acp-23-471-2023, 2023
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We study the effect of injected volcanic ash, water vapor, and SO2 on the development of the volcanic cloud and the stratospheric aerosol optical depth (AOD). Both are sensitive to the initial injection height and to the aging of the volcanic ash shaped by heterogeneous chemistry coupled with the ozone cycle. The paper explains the large differences in AOD for different injection scenarios, which could improve the estimate of the radiative forcing of volcanic eruptions.
Alan Robock, Lili Xia, Cheryl S. Harrison, Joshua Coupe, Owen B. Toon, and Charles G. Bardeen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-852, https://doi.org/10.5194/acp-2022-852, 2023
Revised manuscript accepted for ACP
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A nuclear war could produce a nuclear winter, with catastrophic consequences for global food supplies. Smoke from city fires ignited by nuclear weapons would block out sunlight, causing dark, cold, and dry surface conditions for years. Nuclear winter theory helped to end the nuclear arms race in the 1980s, to produce the Treaty on the Prohibition of Nuclear Weapons in 2017, which led to the 2017 Nobel Peace Prize, and so far to prevent additional use of nuclear weapons. They must be eliminated.
Giorgio Doglioni, Valentina Aquila, Sampa Das, Peter R. Colarco, and Dino Zardi
Atmos. Chem. Phys., 22, 11049–11064, https://doi.org/10.5194/acp-22-11049-2022, https://doi.org/10.5194/acp-22-11049-2022, 2022
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We use a global chemistry climate model to analyze the perturbations to the stratospheric dynamics caused by an injection of carbonaceous aerosol comparable to the one caused by a series of pyrocumulonimbi that formed over British Columbia, Canada on 13 August 2017. The injection of light-absorbing aerosol in an otherwise clean lower stratosphere causes the formation of long-lasting stratospheric anticyclones at the synoptic scale.
Bernd Heinold, Holger Baars, Boris Barja, Matthew Christensen, Anne Kubin, Kevin Ohneiser, Kerstin Schepanski, Nick Schutgens, Fabian Senf, Roland Schrödner, Diego Villanueva, and Ina Tegen
Atmos. Chem. Phys., 22, 9969–9985, https://doi.org/10.5194/acp-22-9969-2022, https://doi.org/10.5194/acp-22-9969-2022, 2022
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The extreme 2019–2020 Australian wildfires produced massive smoke plumes lofted into the lower stratosphere by pyrocumulonimbus convection. Most climate models do not adequately simulate the injection height of such intense fires. By combining aerosol-climate modeling with prescribed pyroconvective smoke injection and lidar observations, this study shows the importance of the representation of the most extreme wildfire events for estimating the atmospheric energy budget.
Kevin DallaSanta and Lorenzo M. Polvani
Atmos. Chem. Phys., 22, 8843–8862, https://doi.org/10.5194/acp-22-8843-2022, https://doi.org/10.5194/acp-22-8843-2022, 2022
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Volcanic eruptions cool the earth by reducing the amount of sunlight reaching the surface. Paradoxically, it has been suggested that they may also warm the surface, but the evidence for this is scant. Here, we show that a small warming can be seen in a climate model for large-enough eruptions. However, even for eruptions much larger than those that have occurred in the past two millennia, post-eruption winters over Eurasia are indistinguishable from those occurring without a prior eruption.
Jim M. Haywood, Andy Jones, Ben T. Johnson, and William McFarlane Smith
Atmos. Chem. Phys., 22, 6135–6150, https://doi.org/10.5194/acp-22-6135-2022, https://doi.org/10.5194/acp-22-6135-2022, 2022
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Simulations are presented investigating the influence of moderately absorbing aerosol in the stratosphere to combat the impacts of climate change. A number of detrimental impacts are noted compared to sulfate aerosol, including (i) reduced cooling efficiency, (ii) increased deficits in global precipitation, (iii) delays in the recovery of the stratospheric ozone hole, and (iv) disruption of the stratospheric circulation and the wintertime storm tracks that impact European precipitation.
Ilaria Quaglia, Daniele Visioni, Giovanni Pitari, and Ben Kravitz
Atmos. Chem. Phys., 22, 5757–5773, https://doi.org/10.5194/acp-22-5757-2022, https://doi.org/10.5194/acp-22-5757-2022, 2022
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Carbonyl sulfide is a gas that mixes very well in the atmosphere and can reach the stratosphere, where it reacts with sunlight and produces aerosol. Here we propose that, by increasing surface fluxes by an order of magnitude, the number of stratospheric aerosols produced may be enough to partially offset the warming produced by greenhouse gases. We explore what effect this would have on the atmospheric composition.
Julia Bruckert, Gholam Ali Hoshyaripour, Ákos Horváth, Lukas O. Muser, Fred J. Prata, Corinna Hoose, and Bernhard Vogel
Atmos. Chem. Phys., 22, 3535–3552, https://doi.org/10.5194/acp-22-3535-2022, https://doi.org/10.5194/acp-22-3535-2022, 2022
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Volcanic emissions endanger aviation and public health and also influence weather and climate. Forecasting the volcanic-plume dispersion is therefore a critical yet sophisticated task. Here, we show that explicit treatment of volcanic-plume dynamics and eruption source parameters significantly improves volcanic-plume dispersion forecasts. We further demonstrate the lofting of the SO2 due to a heating of volcanic particles by sunlight with major implications for volcanic aerosol research.
Andy Jones, Jim M. Haywood, Adam A. Scaife, Olivier Boucher, Matthew Henry, Ben Kravitz, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Roland Séférian, Simone Tilmes, and Daniele Visioni
Atmos. Chem. Phys., 22, 2999–3016, https://doi.org/10.5194/acp-22-2999-2022, https://doi.org/10.5194/acp-22-2999-2022, 2022
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Simulations by six Earth-system models of geoengineering by introducing sulfuric acid aerosols into the tropical stratosphere are compared. A robust impact on the northern wintertime North Atlantic Oscillation is found, exacerbating precipitation reduction over parts of southern Europe. In contrast, the models show no consistency with regard to impacts on the Quasi-Biennial Oscillation, although results do indicate a risk that the oscillation could become locked into a permanent westerly phase.
Debra K. Weisenstein, Daniele Visioni, Henning Franke, Ulrike Niemeier, Sandro Vattioni, Gabriel Chiodo, Thomas Peter, and David W. Keith
Atmos. Chem. Phys., 22, 2955–2973, https://doi.org/10.5194/acp-22-2955-2022, https://doi.org/10.5194/acp-22-2955-2022, 2022
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This paper explores a potential method of geoengineering that could be used to slow the rate of change of climate over decadal scales. We use three climate models to explore how injections of accumulation-mode sulfuric acid aerosol change the large-scale stratospheric particle size distribution and radiative forcing response for the chosen scenarios. Radiative forcing per unit sulfur injected and relative to the change in aerosol burden is larger with particulate than with SO2 injections.
Daniele Visioni, Simone Tilmes, Charles Bardeen, Michael Mills, Douglas G. MacMartin, Ben Kravitz, and Jadwiga H. Richter
Atmos. Chem. Phys., 22, 1739–1756, https://doi.org/10.5194/acp-22-1739-2022, https://doi.org/10.5194/acp-22-1739-2022, 2022
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Aerosols are simulated in a simplified way in climate models: in the model analyzed here, they are represented in every grid as described by three simple logarithmic distributions, mixing all different species together. The size can evolve when new particles are formed, particles merge together to create a larger one or particles are deposited to the surface. This approximation normally works fairly well. Here we show however that when large amounts of sulfate are simulated, there are problems.
Anton Laakso, Ulrike Niemeier, Daniele Visioni, Simone Tilmes, and Harri Kokkola
Atmos. Chem. Phys., 22, 93–118, https://doi.org/10.5194/acp-22-93-2022, https://doi.org/10.5194/acp-22-93-2022, 2022
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The use of different spatio-temporal sulfur injection strategies with different magnitudes to create an artificial reflective aerosol layer to cool the climate is studied using sectional and modal aerosol schemes in a climate model. There are significant differences in the results depending on the aerosol microphysical module used. Different spatio-temporal injection strategies have a significant impact on the magnitude and zonal distribution of radiative forcing and atmospheric dynamics.
Sampa Das, Peter R. Colarco, Luke D. Oman, Ghassan Taha, and Omar Torres
Atmos. Chem. Phys., 21, 12069–12090, https://doi.org/10.5194/acp-21-12069-2021, https://doi.org/10.5194/acp-21-12069-2021, 2021
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Interactions of extreme fires with weather systems can produce towering smoke plumes that inject aerosols at very high altitudes (> 10 km). Three such major injections, largest at the time in terms of emitted aerosol mass, took place over British Columbia, Canada, in August 2017. We model the transport and impacts of injected aerosols on the radiation balance of the atmosphere. Our model results match the satellite-observed plume transport and residence time at these high altitudes very closely.
Daniele Visioni, Douglas G. MacMartin, Ben Kravitz, Olivier Boucher, Andy Jones, Thibaut Lurton, Michou Martine, Michael J. Mills, Pierre Nabat, Ulrike Niemeier, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 10039–10063, https://doi.org/10.5194/acp-21-10039-2021, https://doi.org/10.5194/acp-21-10039-2021, 2021
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A new set of simulations is used to investigate commonalities, differences and sources of uncertainty when simulating the injection of SO2 in the stratosphere in order to mitigate the effects of climate change (solar geoengineering). The models differ in how they simulate the aerosols and how they spread around the stratosphere, resulting in differences in projected regional impacts. Overall, however, the models agree that aerosols have the potential to mitigate the warming produced by GHGs.
Nikolas O. Aksamit, Ben Kravitz, Douglas G. MacMartin, and George Haller
Atmos. Chem. Phys., 21, 8845–8861, https://doi.org/10.5194/acp-21-8845-2021, https://doi.org/10.5194/acp-21-8845-2021, 2021
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There exist robust and influential material features evolving within turbulent fluids that behave as the skeleton for fluid transport pathways. Recent developments in applied mathematics have made the identification of these time-varying structures more rigorous and insightful than ever. Using short-range wind forecasts, we detail how and why these material features can be exploited in an effort to optimize the spread of aerosols in the stratosphere for climate geoengineering.
Ben Kravitz, Douglas G. MacMartin, Daniele Visioni, Olivier Boucher, Jason N. S. Cole, Jim Haywood, Andy Jones, Thibaut Lurton, Pierre Nabat, Ulrike Niemeier, Alan Robock, Roland Séférian, and Simone Tilmes
Atmos. Chem. Phys., 21, 4231–4247, https://doi.org/10.5194/acp-21-4231-2021, https://doi.org/10.5194/acp-21-4231-2021, 2021
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This study investigates multi-model response to idealized geoengineering (high CO2 with solar reduction) across two different generations of climate models. We find that, with the exception of a few cases, the results are unchanged between the different generations. This gives us confidence that broad conclusions about the response to idealized geoengineering are robust.
Margot Clyne, Jean-Francois Lamarque, Michael J. Mills, Myriam Khodri, William Ball, Slimane Bekki, Sandip S. Dhomse, Nicolas Lebas, Graham Mann, Lauren Marshall, Ulrike Niemeier, Virginie Poulain, Alan Robock, Eugene Rozanov, Anja Schmidt, Andrea Stenke, Timofei Sukhodolov, Claudia Timmreck, Matthew Toohey, Fiona Tummon, Davide Zanchettin, Yunqian Zhu, and Owen B. Toon
Atmos. Chem. Phys., 21, 3317–3343, https://doi.org/10.5194/acp-21-3317-2021, https://doi.org/10.5194/acp-21-3317-2021, 2021
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This study finds how and why five state-of-the-art global climate models with interactive stratospheric aerosols differ when simulating the aftermath of large volcanic injections as part of the Model Intercomparison Project on the climatic response to Volcanic forcing (VolMIP). We identify and explain the consequences of significant disparities in the underlying physics and chemistry currently in some of the models, which are problems likely not unique to the models participating in this study.
Andy Jones, Jim M. Haywood, Anthony C. Jones, Simone Tilmes, Ben Kravitz, and Alan Robock
Atmos. Chem. Phys., 21, 1287–1304, https://doi.org/10.5194/acp-21-1287-2021, https://doi.org/10.5194/acp-21-1287-2021, 2021
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Two different methods of simulating a geoengineering scenario are compared using data from two different Earth system models. One method is very idealised while the other includes details of a plausible mechanism. The results from both models agree that the idealised approach does not capture an impact found when detailed modelling is included, namely that geoengineering induces a positive phase of the North Atlantic Oscillation which leads to warmer, wetter winters in northern Europe.
Lorenzo M. Polvani and Suzana J. Camargo
Atmos. Chem. Phys., 20, 13687–13700, https://doi.org/10.5194/acp-20-13687-2020, https://doi.org/10.5194/acp-20-13687-2020, 2020
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On the basis of questionable early studies, it is widely believed that low-latitude volcanic eruptions cause winter warming over Eurasia. However, we here demonstrate that the winter warming over Eurasia following the 1883 Krakatau eruption was unremarkable and, in all likelihood, unrelated to that eruption. Confirming similar findings for the 1991 Pinatubo eruption, the new research demonstrates that no detectable Eurasian winter warming is to be expected after eruptions of similar magnitude.
Ulrike Niemeier, Jadwiga H. Richter, and Simone Tilmes
Atmos. Chem. Phys., 20, 8975–8987, https://doi.org/10.5194/acp-20-8975-2020, https://doi.org/10.5194/acp-20-8975-2020, 2020
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Artificial injections of SO2 into the tropical stratosphere show an impact on the quasi-biennial oscillation (QBO). Different numerical models show only qualitatively but not quantitatively consistent impacts. We show for two models that the response of the QBO is similar when a similar stratospheric heating rate is induced by SO2 injections of different amounts. The reason is very different vertical advection in the two models resulting in different aerosol burden and heating of the aerosols.
Ulrike Niemeier, Claudia Timmreck, and Kirstin Krüger
Atmos. Chem. Phys., 19, 10379–10390, https://doi.org/10.5194/acp-19-10379-2019, https://doi.org/10.5194/acp-19-10379-2019, 2019
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In 1963 Mt. Agung, Indonesia, showed unrest for several months. During this period,
two medium-sized eruptions injected SO2 into the stratosphere. Recent volcanic emission datasets include only one large eruption phase. Therefore, we compared model experiments, with (a) one larger eruption and (b) two eruptions as observed. The evolution of the volcanic cloud differs significantly between the two experiments. Both climatic eruptions should be taken into account.
Lorenzo M. Polvani, Antara Banerjee, and Anja Schmidt
Atmos. Chem. Phys., 19, 6351–6366, https://doi.org/10.5194/acp-19-6351-2019, https://doi.org/10.5194/acp-19-6351-2019, 2019
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This study provides compelling new evidence that the surface winter warming observed over the Northern Hemisphere continents following the 1991 eruption of Mt. Pinatubo was, very likely, completely unrelated to the eruption. This result has implications for earlier eruptions, as the evidence presented here demonstrates that the surface signal of even the very largest known eruptions may be swamped by the internal variability at high latitudes.
Daniele Visioni, Giovanni Pitari, Glauco di Genova, Simone Tilmes, and Irene Cionni
Atmos. Chem. Phys., 18, 14867–14887, https://doi.org/10.5194/acp-18-14867-2018, https://doi.org/10.5194/acp-18-14867-2018, 2018
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Many side effects of sulfate geoengineering have to be analyzed before the world can even consider deploying this method of solar radiation management. In particular, we show that ice clouds in the upper troposphere are modified by a sulfate injection, producing a change that (by allowing for more planetary radiation to escape to space) would produce a further cooling. This might be important when considering the necessary amount of sulfate that needs to be injected to achieve a certain target.
Christoph Brühl, Jennifer Schallock, Klaus Klingmüller, Charles Robert, Christine Bingen, Lieven Clarisse, Andreas Heckel, Peter North, and Landon Rieger
Atmos. Chem. Phys., 18, 12845–12857, https://doi.org/10.5194/acp-18-12845-2018, https://doi.org/10.5194/acp-18-12845-2018, 2018
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Use of multi-instrument satellite data is important to get consistent simulations of aerosol radiative forcing by a complex chemistry climate model, here with a main focus on the lower stratosphere. The satellite data at different wavelengths together with the patterns in the simulated size distribution point to a significant contribution from moist mineral dust lifted to the tropopause region by the Asian summer monsoon.
Tao Tang, Drew Shindell, Bjørn H. Samset, Oliviér Boucher, Piers M. Forster, Øivind Hodnebrog, Gunnar Myhre, Jana Sillmann, Apostolos Voulgarakis, Timothy Andrews, Gregory Faluvegi, Dagmar Fläschner, Trond Iversen, Matthew Kasoar, Viatcheslav Kharin, Alf Kirkevåg, Jean-Francois Lamarque, Dirk Olivié, Thomas Richardson, Camilla W. Stjern, and Toshihiko Takemura
Atmos. Chem. Phys., 18, 8439–8452, https://doi.org/10.5194/acp-18-8439-2018, https://doi.org/10.5194/acp-18-8439-2018, 2018
Yaoxian Huang, Nadine Unger, Trude Storelvmo, Kandice Harper, Yiqi Zheng, and Chris Heyes
Atmos. Chem. Phys., 18, 5219–5233, https://doi.org/10.5194/acp-18-5219-2018, https://doi.org/10.5194/acp-18-5219-2018, 2018
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We apply a global 3-D climate model to quantify the climate impacts of carbonaceous aerosols from solid fuel cookstove emissions. Without black carbon (BC) serving as ice nuclei (IN), global and Indian solid fuel cookstove aerosol emissions have net global cooling impacts. However, when BC acts as IN, the net sign of radiative impacts of carbonaceous aerosols from solid fuel cookstove emissions varies with the choice of maximum freezing efficiency of BC during ice cloud formation.
Thibaut Lurton, Fabrice Jégou, Gwenaël Berthet, Jean-Baptiste Renard, Lieven Clarisse, Anja Schmidt, Colette Brogniez, and Tjarda J. Roberts
Atmos. Chem. Phys., 18, 3223–3247, https://doi.org/10.5194/acp-18-3223-2018, https://doi.org/10.5194/acp-18-3223-2018, 2018
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We quantify the chemical and microphysical effects of volcanic SO2 and HCl from the June 2009 Sarychev Peak eruption using a comprehensive aerosol–chemistry model combined with in situ measurements and satellite retrievals. Our results suggest that previous studies underestimated the eruption's atmospheric and climatic impact, mainly because previous model-to-satellite comparisons had to make assumptions about the aerosol size distribution and were based on biased satellite retrievals of AOD.
Christoph Kleinschmitt, Olivier Boucher, and Ulrich Platt
Atmos. Chem. Phys., 18, 2769–2786, https://doi.org/10.5194/acp-18-2769-2018, https://doi.org/10.5194/acp-18-2769-2018, 2018
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We use a state-of-the-art stratospheric aerosol model to study geoengineering through stratospheric sulfur injections. We find that the efficiency may decrease more drastically for larger injections than previously estimated and that injections at higher altitude are not more effective. This study may provide additional evidence that this proposed geoengineering technique is still more complicated, probably less effective, and may implicate stronger side effects than initially thought.
Daniele Visioni, Giovanni Pitari, Paolo Tuccella, and Gabriele Curci
Atmos. Chem. Phys., 18, 2787–2808, https://doi.org/10.5194/acp-18-2787-2018, https://doi.org/10.5194/acp-18-2787-2018, 2018
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Sulfate geoengineering is a proposed technique that would mimic explosive volcanic eruptions by injecting sulfur dioxide (SO2) into the stratosphere to counteract global warming produced by greenhouse gases by reflecting part of the incoming solar radiation. In this study we use two models to simulate how the injected aerosols would react to dynamical changes in the stratosphere (due to the quasi-biennial oscillation - QBO) and how this would affect the deposition of sulfate at the surface.
Xue Wu, Sabine Griessbach, and Lars Hoffmann
Atmos. Chem. Phys., 17, 13439–13455, https://doi.org/10.5194/acp-17-13439-2017, https://doi.org/10.5194/acp-17-13439-2017, 2017
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This study is focused on the Sarychev eruption in 2009. Based on Lagrangian model simulations and satellite data, the equatorward transport of the plume and aerosol from the Sarychev eruption is confirmed, and the transport is facilitated by the Asian summer monsoon anticyclonic circulations. The aerosol transported to the tropics remained for months and dispersed upward, which could make the Sarychev eruption have a similar global climate impact as a tropical volcanic eruption.
Daniele Visioni, Giovanni Pitari, Valentina Aquila, Simone Tilmes, Irene Cionni, Glauco Di Genova, and Eva Mancini
Atmos. Chem. Phys., 17, 11209–11226, https://doi.org/10.5194/acp-17-11209-2017, https://doi.org/10.5194/acp-17-11209-2017, 2017
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Sulfate geoengineering (SG), the sustained injection of SO2 in the lower stratosphere, is being discussed as a way to counterbalance surface warming, mimicking volcanic eruptions. In this paper, we analyse results from two models part of the GeoMIP project in order to understand the effect SG might have on the concentration and lifetime of methane, which acts in the atmosphere as a greenhouse gas. Understanding possible side effects of SG is a crucial step if its viability is to be assessed.
Steffen Münch and Joachim Curtius
Atmos. Chem. Phys., 17, 7581–7591, https://doi.org/10.5194/acp-17-7581-2017, https://doi.org/10.5194/acp-17-7581-2017, 2017
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Recent research has analyzed the formation of a particle (CN) layer in the stratosphere above Antarctica after sunrise. We investigate the CN layer formation processes with our particle formation model and derive sulfuric acid profiles (no measurements exist). Our study confirms existing explanations and gives more insights into the formation process, leading to higher derived concentrations. Therefore, this paper improves our understanding of the processes in the high atmosphere.
Anton Laakso, Hannele Korhonen, Sami Romakkaniemi, and Harri Kokkola
Atmos. Chem. Phys., 17, 6957–6974, https://doi.org/10.5194/acp-17-6957-2017, https://doi.org/10.5194/acp-17-6957-2017, 2017
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Based on simulations, equatorial stratospheric sulfur injections have shown to be an efficient strategy to counteract ongoing global warming. However, equatorial injections would result in relatively larger cooling in low latitudes than in high latitudes. This together with greenhouse-gas-induced warming would lead to cooling in the Equator and warming in the high latitudes. Results of this study show that a more optimal cooling effect is achieved by varying the injection area seasonally.
Alejandro Marti, Arnau Folch, Oriol Jorba, and Zavisa Janjic
Atmos. Chem. Phys., 17, 4005–4030, https://doi.org/10.5194/acp-17-4005-2017, https://doi.org/10.5194/acp-17-4005-2017, 2017
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We describe and evaluate NMMB-MONARCH-ASH, a novel online multi-scale meteorological and transport model developed at the BSC-CNS capable of forecasting the dispersal and deposition of volcanic ash. The forecast skills of the model have been validated and they improve on those from traditional operational offline (decoupled) models. The results support the use of online coupled models to aid civil aviation and emergency management during a crisis such as the 2010 eruption of Eyjafjallajökull.
Daniele Visioni, Giovanni Pitari, and Valentina Aquila
Atmos. Chem. Phys., 17, 3879–3889, https://doi.org/10.5194/acp-17-3879-2017, https://doi.org/10.5194/acp-17-3879-2017, 2017
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This review paper summarizes the state-of-the-art knowledge of the direct and indirect side effects of sulfate geoengineering, that is, the injection of sulfur dioxide into the stratosphere in order to offset the warming caused by the anthropic increase in greenhouse gasses. An overview of the various effects and their uncertainties, using results from published scientific articles, may help fine-tune the best amount of sulfate to be injected in an eventual realization of the experiment.
Anthony C. Jones, James M. Haywood, and Andy Jones
Atmos. Chem. Phys., 16, 2843–2862, https://doi.org/10.5194/acp-16-2843-2016, https://doi.org/10.5194/acp-16-2843-2016, 2016
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In this paper we assess the potential climatic impacts of geoengineering with sulfate, black carbon and titania injection strategies. We find that black carbon injection results in severe stratospheric warming and precipitation impacts, and therefore black carbon is unsuitable for geoengineering purposes. As the injection rates and climatic impacts for titania are close to those for sulfate, there appears little benefit of using titania when compared to injection of sulfur dioxide.
A. Laakso, H. Kokkola, A.-I. Partanen, U. Niemeier, C. Timmreck, K. E. J. Lehtinen, H. Hakkarainen, and H. Korhonen
Atmos. Chem. Phys., 16, 305–323, https://doi.org/10.5194/acp-16-305-2016, https://doi.org/10.5194/acp-16-305-2016, 2016
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We have studied the impacts of a volcanic eruption during solar radiation management (SRM) using an aerosol-climate model ECHAM5-HAM-SALSA and an Earth system model MPI-ESM. A volcanic eruption during stratospheric sulfur geoengineering would lead to larger particles and smaller amount of new particles than if an volcano erupts in normal atmospheric conditions. Thus, volcanic eruption during SRM would lead to only a small additional cooling which would last for a significantly shorter period.
V. N. Aswathy, O. Boucher, M. Quaas, U. Niemeier, H. Muri, J. Mülmenstädt, and J. Quaas
Atmos. Chem. Phys., 15, 9593–9610, https://doi.org/10.5194/acp-15-9593-2015, https://doi.org/10.5194/acp-15-9593-2015, 2015
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Simulations conducted in the GeoMIP and IMPLICC model intercomparison studies for climate engineering by stratospheric sulfate injection and marine cloud brightening via sea salt are analysed and compared to the reference scenario RCP4.5. The focus is on extremes in surface temperature and precipitation. It is found that the extreme changes mostly follow the mean changes and that extremes are also in general well mitigated, except for in polar regions.
U. Niemeier and C. Timmreck
Atmos. Chem. Phys., 15, 9129–9141, https://doi.org/10.5194/acp-15-9129-2015, https://doi.org/10.5194/acp-15-9129-2015, 2015
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The injection of sulfur dioxide is considered as an option for solar radiation management. We have calculated the effects of SO2 injections up to 100 Tg(S)/y. Our calculations show that the forcing efficiency of the injection decays exponentially. This result implies that SO2 injections in the order of 6 times Mt. Pinatubo eruptions per year are required to keep temperatures constant at that anticipated for 2020, whilst maintaining business as usual emission conditions.
R. Hommel, C. Timmreck, M. A. Giorgetta, and H. F. Graf
Atmos. Chem. Phys., 15, 5557–5584, https://doi.org/10.5194/acp-15-5557-2015, https://doi.org/10.5194/acp-15-5557-2015, 2015
M. Toohey, K. Krüger, M. Bittner, C. Timmreck, and H. Schmidt
Atmos. Chem. Phys., 14, 13063–13079, https://doi.org/10.5194/acp-14-13063-2014, https://doi.org/10.5194/acp-14-13063-2014, 2014
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Earth system model simulations are used to investigate the impact of volcanic aerosol forcing on stratospheric dynamics, e.g. the Northern Hemisphere (NH) polar vortex. We find that mechanisms linking aerosol heating and high-latitude dynamics are not as direct as often assumed; high-latitude effects result from changes in stratospheric circulation and related vertical motions. The simulated responses also show evidence of being sensitive to the structure of the volcanic forcing used.
F. Arfeuille, B. P. Luo, P. Heckendorn, D. Weisenstein, J. X. Sheng, E. Rozanov, M. Schraner, S. Brönnimann, L. W. Thomason, and T. Peter
Atmos. Chem. Phys., 13, 11221–11234, https://doi.org/10.5194/acp-13-11221-2013, https://doi.org/10.5194/acp-13-11221-2013, 2013
S. Fadnavis, K. Semeniuk, L. Pozzoli, M. G. Schultz, S. D. Ghude, S. Das, and R. Kakatkar
Atmos. Chem. Phys., 13, 8771–8786, https://doi.org/10.5194/acp-13-8771-2013, https://doi.org/10.5194/acp-13-8771-2013, 2013
D. N. Bernstein, J. D. Neelin, Q. B. Li, and D. Chen
Atmos. Chem. Phys., 13, 6373–6390, https://doi.org/10.5194/acp-13-6373-2013, https://doi.org/10.5194/acp-13-6373-2013, 2013
M. Toohey, K. Krüger, U. Niemeier, and C. Timmreck
Atmos. Chem. Phys., 11, 12351–12367, https://doi.org/10.5194/acp-11-12351-2011, https://doi.org/10.5194/acp-11-12351-2011, 2011
J. M. English, O. B. Toon, M. J. Mills, and F. Yu
Atmos. Chem. Phys., 11, 9303–9322, https://doi.org/10.5194/acp-11-9303-2011, https://doi.org/10.5194/acp-11-9303-2011, 2011
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Short summary
An artificial stratospheric sulfur layer heats the lower stratosphere which impacts stratospheric dynamics and transport. The quasi-biennial oscillation shuts down due to the heated sulfur layer which impacts the meridional transport of the sulfate aerosols. The tropical confinement of the sulfate is stronger and the radiative forcing efficiency of the aerosol layer decreases compared to previous studies, as does the forcing when increasing the injection height.
An artificial stratospheric sulfur layer heats the lower stratosphere which impacts...
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