Articles | Volume 24, issue 20
https://doi.org/10.5194/acp-24-11775-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-11775-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
23 Oct 2024
Research article |
| 23 Oct 2024
| 23 Oct 2024
Impacts of tropical cyclone–heat wave compound events on surface ozone in eastern China: comparison between the Yangtze River and Pearl River deltas
Cuini Qi
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Joint International Research Laboratory of Climate and Environment Change, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, China
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Joint International Research Laboratory of Climate and Environment Change, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, China
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Joint International Research Laboratory of Climate and Environment Change, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, China
Huimin Li
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Joint International Research Laboratory of Climate and Environment Change, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, China
Hui Zhang
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Joint International Research Laboratory of Climate and Environment Change, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, China
Lili Ren
College of Environment and Ecology, Jiangsu Open University, Nanjing, Jiangsu, China
Xipeng Jin
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Joint International Research Laboratory of Climate and Environment Change, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, China
Chenchao Zhan
School of Atmospheric Physics, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, China
Jianping Tang
School of Atmospheric Sciences, Nanjing University, Nanjing, Jiangsu, China
Hong Liao
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Joint International Research Laboratory of Climate and Environment Change, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, Jiangsu, China
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Laura Hyesung Yang, Daniel J. Jacob, Ruijun Dang, Yujin J. Oak, Haipeng Lin, Jhoon Kim, Shixian Zhai, Nadia K. Colombi, Drew C. Pendergrass, Ellie Beaudry, Viral Shah, Xu Feng, Robert M. Yantosca, Heesung Chong, Junsung Park, Hanlim Lee, Won-Jin Lee, Soontae Kim, Eunhye Kim, Katherine R. Travis, James H. Crawford, and Hong Liao
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Xu Yue, Hao Zhou, Chenguang Tian, Yimian Ma, Yihan Hu, Cheng Gong, Hui Zheng, and Hong Liao
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We develop the interactive Model for Air Pollution and Land Ecosystems (iMAPLE). The model considers the full coupling between carbon and water cycles, dynamic fire emissions, wetland methane emissions, biogenic volatile organic compound emissions, and trait-based ozone vegetation damage. Evaluations show that iMAPLE is a useful tool for the study of the interactions among climate, chemistry, and ecosystems.
Yang Yang, Shaoxuan Mou, Hailong Wang, Pinya Wang, Baojie Li, and Hong Liao
Atmos. Chem. Phys., 24, 6509–6523, https://doi.org/10.5194/acp-24-6509-2024, https://doi.org/10.5194/acp-24-6509-2024, 2024
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The variations in anthropogenic aerosol concentrations and source contributions and their subsequent radiative impact in major emission regions during historical periods are quantified based on an aerosol-tagging system in E3SMv1. Due to the industrial development and implementation of economic policies, sources of anthropogenic aerosols show different variations, which has important implications for pollution prevention and control measures and decision-making for global collaboration.
Drew C. Pendergrass, Daniel J. Jacob, Yujin J. Oak, Jeewoo Lee, Minseok Kim, Jhoon Kim, Seoyoung Lee, Shixian Zhai, Hitoshi Irie, and Hong Liao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-172, https://doi.org/10.5194/essd-2024-172, 2024
Preprint withdrawn
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Fine particles suspended in the atmosphere are a major form of air pollution and an important public health burden. However, measurements of particulate matter are sparse in space and in places like East Asia monitors are established after regulatory policies to improve pollution have changed. In this paper, we use machine learning to fill in the gaps. We train an algorithm to predict pollution at the surface from the atmosphere’s opacity, then produce high resolution maps of data without gaps.
Hao Yang, Lei Chen, Hong Liao, Jia Zhu, Wenjie Wang, and Xin Li
Atmos. Chem. Phys., 24, 4001–4015, https://doi.org/10.5194/acp-24-4001-2024, https://doi.org/10.5194/acp-24-4001-2024, 2024
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The present study quantifies the response of aerosol–radiation interaction (ARI) to anthropogenic emission reduction from 2013 to 2017, with the main focus on the contribution to changed O3 concentrations over eastern China both in summer and winter using the WRF-Chem model. The weakened ARI due to decreased anthropogenic emission aggravates the summer (winter) O3 pollution by +0.81 ppb (+0.63 ppb), averaged over eastern China.
Feifan Yan, Hang Su, Yafang Cheng, Rujin Huang, Hong Liao, Ting Yang, Yuanyuan Zhu, Shaoqing Zhang, Lifang Sheng, Wenbin Kou, Xinran Zeng, Shengnan Xiang, Xiaohong Yao, Huiwang Gao, and Yang Gao
Atmos. Chem. Phys., 24, 2365–2376, https://doi.org/10.5194/acp-24-2365-2024, https://doi.org/10.5194/acp-24-2365-2024, 2024
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PM2.5 pollution is a major air quality issue deteriorating human health, and previous studies mostly focus on regions like the North China Plain and Yangtze River Delta. However, the characteristics of PM2.5 concentrations between these two regions are studied less often. Focusing on the transport corridor region, we identify an interesting seesaw transport phenomenon with stagnant weather conditions, conducive to PM2.5 accumulation over this region, resulting in large health effects.
Yang Yang, Yang Zhou, Hailong Wang, Mengyun Li, Huimin Li, Pinya Wang, Xu Yue, Ke Li, Jia Zhu, and Hong Liao
Atmos. Chem. Phys., 24, 1177–1191, https://doi.org/10.5194/acp-24-1177-2024, https://doi.org/10.5194/acp-24-1177-2024, 2024
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This study reveals that extreme ozone pollution over the North China Plain and Yangtze River Delta is due to the chemical production related to hot and dry conditions, and the regional transport explains the ozone pollution over the Sichuan Basin and Pearl River Delta. The frequency of meteorological conditions of the extreme ozone pollution increases from the past to the future. The sustainable scenario is the optimal path to retaining clean air in China in the future.
Xiaodong Xie, Jianlin Hu, Momei Qin, Song Guo, Min Hu, Dongsheng Ji, Hongli Wang, Shengrong Lou, Cheng Huang, Chong Liu, Hongliang Zhang, Qi Ying, Hong Liao, and Yuanhang Zhang
Atmos. Chem. Phys., 23, 10563–10578, https://doi.org/10.5194/acp-23-10563-2023, https://doi.org/10.5194/acp-23-10563-2023, 2023
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The atmospheric age of particles reflects how long particles have been formed and suspended in the atmosphere, which is closely associated with the evolution processes of particles. An analysis of the atmospheric age of PM2.5 provides a unique perspective on the evolution processes of different PM2.5 components. The results also shed lights on how to design effective emission control actions under unfavorable meteorological conditions.
Li Fang, Jianbing Jin, Arjo Segers, Hong Liao, Ke Li, Bufan Xu, Wei Han, Mijie Pang, and Hai Xiang Lin
Geosci. Model Dev., 16, 4867–4882, https://doi.org/10.5194/gmd-16-4867-2023, https://doi.org/10.5194/gmd-16-4867-2023, 2023
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Machine learning models have gained great popularity in air quality prediction. However, they are only available at air quality monitoring stations. In contrast, chemical transport models (CTM) provide predictions that are continuous in the 3D field. Owing to complex error sources, they are typically biased. In this study, we proposed a gridded prediction with high accuracy by fusing predictions from our regional feature selection machine learning prediction (RFSML v1.0) and a CTM prediction.
Zhenxin Liu, Yuanhao Chen, Yuhang Wang, Cheng Liu, Shuhua Liu, and Hong Liao
Geosci. Model Dev., 16, 4385–4403, https://doi.org/10.5194/gmd-16-4385-2023, https://doi.org/10.5194/gmd-16-4385-2023, 2023
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The heterogeneous layout of urban buildings leads to the complex wind field in and over the urban canopy. Large discrepancies between the observations and the current simulations result from misunderstanding the character of the wind field. The Inhomogeneous Wind Scheme in Urban Street (IWSUS) was developed to simulate the heterogeneity of the wind speed in a typical street and then improve the simulated energy budget in the lower atmospheric layer over the urban canopy.
Pengwei Li, Yang Yang, Hailong Wang, Su Li, Ke Li, Pinya Wang, Baojie Li, and Hong Liao
Atmos. Chem. Phys., 23, 5403–5417, https://doi.org/10.5194/acp-23-5403-2023, https://doi.org/10.5194/acp-23-5403-2023, 2023
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We use a novel technique that can attribute O3 to precursors to investigate O3 changes in the United States during 1995–2019. We found that the US domestic energy and surface transportation emission reductions are primarily responsible for the O3 decrease in summer. In winter, factors such as nitrogen oxide emission reduction in the context of its inhibition of ozone production, increased aviation and shipping activities, and large-scale circulation changes contribute to the O3 increases.
Shixian Zhai, Daniel J. Jacob, Drew C. Pendergrass, Nadia K. Colombi, Viral Shah, Laura Hyesung Yang, Qiang Zhang, Shuxiao Wang, Hwajin Kim, Yele Sun, Jin-Soo Choi, Jin-Soo Park, Gan Luo, Fangqun Yu, Jung-Hun Woo, Younha Kim, Jack E. Dibb, Taehyoung Lee, Jin-Seok Han, Bruce E. Anderson, Ke Li, and Hong Liao
Atmos. Chem. Phys., 23, 4271–4281, https://doi.org/10.5194/acp-23-4271-2023, https://doi.org/10.5194/acp-23-4271-2023, 2023
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Anthropogenic fugitive dust in East Asia not only causes severe coarse particulate matter air pollution problems, but also affects fine particulate nitrate. Due to emission control efforts, coarse PM decreased steadily. We find that the decrease of coarse PM is a major driver for a lack of decrease of fine particulate nitrate, as it allows more nitric acid to form fine particulate nitrate. The continuing decrease of coarse PM requires more stringent ammonia and nitrogen oxides emission controls.
Nadia K. Colombi, Daniel J. Jacob, Laura Hyesung Yang, Shixian Zhai, Viral Shah, Stuart K. Grange, Robert M. Yantosca, Soontae Kim, and Hong Liao
Atmos. Chem. Phys., 23, 4031–4044, https://doi.org/10.5194/acp-23-4031-2023, https://doi.org/10.5194/acp-23-4031-2023, 2023
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Surface ozone, detrimental to human and ecosystem health, is very high and increasing in South Korea. Using a global model of the atmosphere, we found that emissions from South Korea and China contribute equally to the high ozone observed. We found that in the absence of all anthropogenic emissions over East Asia, ozone is still very high, implying that the air quality standard in South Korea is not practically achievable unless this background external to East Asia can be decreased.
Yi Yang, Douglas Maraun, Albert Ossó, and Jianping Tang
Nat. Hazards Earth Syst. Sci., 23, 693–709, https://doi.org/10.5194/nhess-23-693-2023, https://doi.org/10.5194/nhess-23-693-2023, 2023
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This study quantifies the spatiotemporal variation and characteristics of compound long-duration dry and hot events in China over the 1961–2014 period. The results show that over the past few decades, there has been a substantial increase in the frequency of these compound events across most parts of China, which is dominated by rising temperatures. We detect a strong increase in the spatially contiguous areas experiencing concurrent dry and hot conditions.
Mengyun Li, Yang Yang, Hailong Wang, Huimin Li, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 23, 1533–1544, https://doi.org/10.5194/acp-23-1533-2023, https://doi.org/10.5194/acp-23-1533-2023, 2023
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Using the GEOS-Chem model, the impact of the quasi-biennial oscillation (QBO) on summertime tropospheric O3 in China is investigated. In the warm phases of sea surface temperature anomalies over the eastern tropical Pacific, the QBO has a significant positive correlation with near-surface O3 concentrations over central China. The QBO impacts on O3 pollution in China are mainly a result of changing vertical transport of O3.
Huimin Li, Yang Yang, Jianbing Jin, Hailong Wang, Ke Li, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 23, 1131–1145, https://doi.org/10.5194/acp-23-1131-2023, https://doi.org/10.5194/acp-23-1131-2023, 2023
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Future climate change will aggravate ozone pollution in Asia, especially in high-forcing scenarios. Ozone pollution in China will expand from North China to South China and extend into the cold season in a warmer future. The emphasis of this work is to quantify the impacts of future climate change on O3 pollution in Asia, which is of great significance for future O3 pollution mitigation strategies.
Chenchao Zhan, Min Xie, Hua Lu, Bojun Liu, Zheng Wu, Tijian Wang, Bingliang Zhuang, Mengmeng Li, and Shu Li
Atmos. Chem. Phys., 23, 771–788, https://doi.org/10.5194/acp-23-771-2023, https://doi.org/10.5194/acp-23-771-2023, 2023
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With the development of urbanization, urban land use and anthropogenic
emissions increase, affecting urban air quality and, in turn, the health risks associated with air pollutants. In this study, we systematically evaluate the impacts of urbanization on air quality and the corresponding health risks in a highly urbanized city with severe air pollution and complex terrain. This work focuses on the health risks caused by urbanization and can provide valuable insight for air pollution strategies.
Huibin Dai, Hong Liao, Ke Li, Xu Yue, Yang Yang, Jia Zhu, Jianbing Jin, Baojie Li, and Xingwen Jiang
Atmos. Chem. Phys., 23, 23–39, https://doi.org/10.5194/acp-23-23-2023, https://doi.org/10.5194/acp-23-23-2023, 2023
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We apply the 3-D global chemical transport model (GEOS-Chem) to simulate co-polluted days by O3 and PM2.5 (O3–PM2.5PDs) in Beijing–Tianjin–Hebei in 2013–2020 and investigate the chemical and physical characteristics of O3–PM2.5PDs by composited analyses of such days that are captured by both the observations and the model. We report for the first time the unique features in vertical distributions of aerosols during O3–PM2.5PDs and the physical and chemical characteristics of O3–PM2.5PDs.
Yang Yang, Liangying Zeng, Hailong Wang, Pinya Wang, and Hong Liao
Atmos. Chem. Phys., 22, 14489–14502, https://doi.org/10.5194/acp-22-14489-2022, https://doi.org/10.5194/acp-22-14489-2022, 2022
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Using an aerosol–climate model, dust pollution in China affected by different spatial and temporal types of El Niño are examined. Both eastern and central Pacific El Niño and short-duration El Niño increase winter dust concentrations over northern China, while long-duration El Niño decreases concentrations. Only long-duration El Niño events can significantly affect dust over China in the following spring. This study has profound implications for air pollution control and dust storm prediction.
Zhenqi Xu, Wei Feng, Yicheng Wang, Haoran Ye, Yuhang Wang, Hong Liao, and Mingjie Xie
Atmos. Chem. Phys., 22, 13739–13752, https://doi.org/10.5194/acp-22-13739-2022, https://doi.org/10.5194/acp-22-13739-2022, 2022
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This work uses a solvent (DMF) that can efficiently dissolve low-volatility OC to examine BrC absorption and sources, which will benefit future investigations on the physicochemical properties of large organic molecules. The study results also shed light on potential sources for methanol-insoluble OC. These results highlight the importance of testing different solvents to investigate the structures and light absorption of low-volatility BrC.
Li Fang, Jianbing Jin, Arjo Segers, Hai Xiang Lin, Mijie Pang, Cong Xiao, Tuo Deng, and Hong Liao
Geosci. Model Dev., 15, 7791–7807, https://doi.org/10.5194/gmd-15-7791-2022, https://doi.org/10.5194/gmd-15-7791-2022, 2022
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This study proposes a regional feature selection-based machine learning system to predict short-term air quality in China. The system has a tool that can figure out the importance of input data for better prediction. It provides large-scale air quality prediction that exhibits improved interpretability, fewer training costs, and higher accuracy compared with a standard machine learning system. It can act as an early warning for citizens and reduce exposure to PM2.5 and other air pollutants.
Chenguang Tian, Xu Yue, Jun Zhu, Hong Liao, Yang Yang, Yadong Lei, Xinyi Zhou, Hao Zhou, Yimian Ma, and Yang Cao
Atmos. Chem. Phys., 22, 12353–12366, https://doi.org/10.5194/acp-22-12353-2022, https://doi.org/10.5194/acp-22-12353-2022, 2022
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We quantify the impacts of fire aerosols on climate through direct, indirect, and albedo effects. In atmosphere-only simulations, we find global fire aerosols cause surface cooling and rainfall inhibition over many land regions. These fast atmospheric perturbations further lead to a reduction in regional leaf area index and lightning activities. By considering the feedback of fire aerosols on humidity, lightning, and leaf area index, we predict a slight reduction in fire emissions.
Shijie Cui, Dan Dan Huang, Yangzhou Wu, Junfeng Wang, Fuzhen Shen, Jiukun Xian, Yunjiang Zhang, Hongli Wang, Cheng Huang, Hong Liao, and Xinlei Ge
Atmos. Chem. Phys., 22, 8073–8096, https://doi.org/10.5194/acp-22-8073-2022, https://doi.org/10.5194/acp-22-8073-2022, 2022
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Refractory black carbon (rBC) aerosols are important to air quality and climate change. rBC can mix with many other species, which can significantly change its properties and impacts. We used a specific set of techniques to exclusively characterize rBC-containing (rBCc) particles in Shanghai. We elucidated their composition, sources and size distributions and factors that affect their properties. Our findings are very valuable for advancing the understanding of BC and controlling BC pollution.
Jiyuan Gao, Yang Yang, Hailong Wang, Pinya Wang, Huimin Li, Mengyun Li, Lili Ren, Xu Yue, and Hong Liao
Atmos. Chem. Phys., 22, 7131–7142, https://doi.org/10.5194/acp-22-7131-2022, https://doi.org/10.5194/acp-22-7131-2022, 2022
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China has been implementing a sequence of policies for clean air since the year 2013. The aerosol decline produced a 0.09 ± 0.10°C warming during 2013–2017 estimated in this study, and the increase in ozone in the lower troposphere during this time period accelerated the warming, leading to a total 0.16 ± 0.15°C temperature increase in eastern China. Residential emission reductions led to a cooling effect because of a substantial decrease in light-absorbing aerosols.
Jianbing Jin, Mijie Pang, Arjo Segers, Wei Han, Li Fang, Baojie Li, Haochuan Feng, Hai Xiang Lin, and Hong Liao
Atmos. Chem. Phys., 22, 6393–6410, https://doi.org/10.5194/acp-22-6393-2022, https://doi.org/10.5194/acp-22-6393-2022, 2022
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Super dust storms reappeared in East Asia last spring after being absent for one and a half decades. Accurate simulation of such super sandstorms is valuable, but challenging due to imperfect emissions. In this study, the emissions of these dust storms are estimated by assimilating multiple observations. The results reveal that emissions originated from both China and Mongolia. However, for northern China, long-distance transport from Mongolia contributes much more dust than Chinese deserts.
Haoran Zhang, Nan Li, Keqin Tang, Hong Liao, Chong Shi, Cheng Huang, Hongli Wang, Song Guo, Min Hu, Xinlei Ge, Mindong Chen, Zhenxin Liu, Huan Yu, and Jianlin Hu
Atmos. Chem. Phys., 22, 5495–5514, https://doi.org/10.5194/acp-22-5495-2022, https://doi.org/10.5194/acp-22-5495-2022, 2022
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We developed a new algorithm with low economic/technique costs to identify primary and secondary components of PM2.5. Our model was shown to be reliable by comparison with different observation datasets. We systematically explored the patterns and changes in the secondary PM2.5 pollution in China at large spatial and time scales. We believe that this method is a promising tool for efficiently estimating primary and secondary PM2.5, and has huge potential for future PM mitigation.
Pinya Wang, Yang Yang, Huimin Li, Lei Chen, Ruijun Dang, Daokai Xue, Baojie Li, Jianping Tang, L. Ruby Leung, and Hong Liao
Atmos. Chem. Phys., 22, 4705–4719, https://doi.org/10.5194/acp-22-4705-2022, https://doi.org/10.5194/acp-22-4705-2022, 2022
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China is now suffering from both severe ozone (O3) pollution and heat events. We highlight that North China Plain is the hot spot of the co-occurrences of extremes in O3 and high temperatures in China. Such coupled extremes exhibit an increasing trend during 2014–2019 and will continue to increase until the middle of this century. And the coupled extremes impose more severe health impacts to human than O3 pollution occurring alone because of elevated O3 levels and temperatures.
Hao Yang, Lei Chen, Hong Liao, Jia Zhu, Wenjie Wang, and Xin Li
Atmos. Chem. Phys., 22, 4101–4116, https://doi.org/10.5194/acp-22-4101-2022, https://doi.org/10.5194/acp-22-4101-2022, 2022
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Aerosols can influence O3 through aerosol–radiation interactions, including aerosol–photolysis interaction (API) and aerosol–radiation feedback (ARF). The weakened photolysis rates and changed meteorological conditions reduce surface-layer O3 concentrations by up to 9.3–11.4 ppb, with API and ARF contributing 74.6 %–90.0 % and 10.0 %–25.4 % of the O3 decrease in three episodes, respectively, which indicates that API is the dominant way for O3 reduction related to aerosol–radiation interactions.
Drew C. Pendergrass, Shixian Zhai, Jhoon Kim, Ja-Ho Koo, Seoyoung Lee, Minah Bae, Soontae Kim, Hong Liao, and Daniel J. Jacob
Atmos. Meas. Tech., 15, 1075–1091, https://doi.org/10.5194/amt-15-1075-2022, https://doi.org/10.5194/amt-15-1075-2022, 2022
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This paper uses a machine learning algorithm to infer high-resolution maps of particulate air quality in eastern China, Japan, and the Korean peninsula, using data from a geostationary satellite along with meteorology. We then perform an extensive evaluation of this inferred air quality and use it to diagnose trends in the region. We hope this paper and the associated data will be valuable to other scientists interested in epidemiology, air quality, remote sensing, and machine learning.
Donglin Chen, Hong Liao, Yang Yang, Lei Chen, Delong Zhao, and Deping Ding
Atmos. Chem. Phys., 22, 1825–1844, https://doi.org/10.5194/acp-22-1825-2022, https://doi.org/10.5194/acp-22-1825-2022, 2022
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The black carbon (BC) vertical profile plays a critical role in BC–meteorology interaction, which also influences PM2.5 concentrations. More BC mass was assigned into high altitudes (above 1000 m) in the model, which resulted in a stronger cooling effect near the surface, a larger temperature inversion below 421 m, more reductions in PBLH, and a larger increase in near-surface PM2.5 in the daytime caused by the direct radiative effect of BC.
Chenchao Zhan and Min Xie
Atmos. Chem. Phys., 22, 1351–1371, https://doi.org/10.5194/acp-22-1351-2022, https://doi.org/10.5194/acp-22-1351-2022, 2022
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The changes of land use and anthropogenic heat (AH) derived from urbanization can affect meteorology and in turn O3 evolution. In this study, we briefly describe the general features of O3 pollution in the Yangtze River Delta (YRD) based on in situ observational data. Then, the impacts of land use and anthropogenic heat on O3 via changing the meteorological factors and local circulations are investigated in this region using the WRF-Chem model.
Yulu Qiu, Zhiqiang Ma, Ke Li, Mengyu Huang, Jiujiang Sheng, Ping Tian, Jia Zhu, Weiwei Pu, Yingxiao Tang, Tingting Han, Huaigang Zhou, and Hong Liao
Atmos. Chem. Phys., 21, 17995–18010, https://doi.org/10.5194/acp-21-17995-2021, https://doi.org/10.5194/acp-21-17995-2021, 2021
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Photochemical pollution over the North China Plain (NCP) is attracting much concern. Our observations at a rural site in the NCP identified high peroxyacetyl nitrate (PAN) concentrations, even on cold days. Increased acetaldehyde concentration and hydroxyl radical production rates drive fast PAN formation. Moreover, our study emphasizes the importance of formaldehyde photolysis in PAN formation and calls for implementing strict volatile organic compound controls after summer over the NCP.
Jianping Guo, Jian Zhang, Kun Yang, Hong Liao, Shaodong Zhang, Kaiming Huang, Yanmin Lv, Jia Shao, Tao Yu, Bing Tong, Jian Li, Tianning Su, Steve H. L. Yim, Ad Stoffelen, Panmao Zhai, and Xiaofeng Xu
Atmos. Chem. Phys., 21, 17079–17097, https://doi.org/10.5194/acp-21-17079-2021, https://doi.org/10.5194/acp-21-17079-2021, 2021
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The planetary boundary layer (PBL) is the lowest part of the troposphere, and boundary layer height (BLH) is the depth of the PBL and is of critical importance to the dispersion of air pollution. The study presents the first near-global BLH climatology by using high-resolution (5-10 m) radiosonde measurements. The variations in BLH exhibit large spatial and temporal dependence, with a peak at 17:00 local solar time. The most promising reanalysis product is ERA-5 in terms of modeling BLH.
Shixian Zhai, Daniel J. Jacob, Jared F. Brewer, Ke Li, Jonathan M. Moch, Jhoon Kim, Seoyoung Lee, Hyunkwang Lim, Hyun Chul Lee, Su Keun Kuk, Rokjin J. Park, Jaein I. Jeong, Xuan Wang, Pengfei Liu, Gan Luo, Fangqun Yu, Jun Meng, Randall V. Martin, Katherine R. Travis, Johnathan W. Hair, Bruce E. Anderson, Jack E. Dibb, Jose L. Jimenez, Pedro Campuzano-Jost, Benjamin A. Nault, Jung-Hun Woo, Younha Kim, Qiang Zhang, and Hong Liao
Atmos. Chem. Phys., 21, 16775–16791, https://doi.org/10.5194/acp-21-16775-2021, https://doi.org/10.5194/acp-21-16775-2021, 2021
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Geostationary satellite aerosol optical depth (AOD) has tremendous potential for monitoring surface fine particulate matter (PM2.5). Our study explored the physical relationship between AOD and PM2.5 by integrating data from surface networks, aircraft, and satellites with the GEOS-Chem chemical transport model. We quantitatively showed that accurate simulation of aerosol size distributions, boundary layer depths, relative humidity, coarse particles, and diurnal variations in PM2.5 are essential.
Baojie Li, Lei Chen, Weishou Shen, Jianbing Jin, Teng Wang, Pinya Wang, Yang Yang, and Hong Liao
Atmos. Chem. Phys., 21, 15883–15900, https://doi.org/10.5194/acp-21-15883-2021, https://doi.org/10.5194/acp-21-15883-2021, 2021
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This study focused on improving fertilizer-application-related NH3 emission inventories. We comprehensively evaluated the dates and times of fertilizer application to the major crops in China, improved the spatial allocation methods for NH3 emissions from croplands with different rice types, and established a NH3 emission inventory for mainland China in 2016. The inventory showed a higher level of accuracy than other inventories based on evaluation using the WRF-Chem and observation data.
Lili Ren, Yang Yang, Hailong Wang, Pinya Wang, Lei Chen, Jia Zhu, and Hong Liao
Atmos. Chem. Phys., 21, 15431–15445, https://doi.org/10.5194/acp-21-15431-2021, https://doi.org/10.5194/acp-21-15431-2021, 2021
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Due to the COVID-19 pandemic, human activities were strictly restricted in China. Even though anthropogenic aerosol emissions largely decreased, haze events still occurred. Our results shows that PM2.5 over the North China Plain is largely contributed by local sources. For other regions in China, PM2.5 is largely contributed from nonlocal sources. As emission reduction is a future goal, aerosol long-range transport and unfavorable meteorology are increasingly important to air quality.
Cited articles
Ainsworth, E. A., Yendrek, C. R., Sitch, S., Collins, W. J., and Emberson, L. D.: The Effects of Tropospheric Ozone on Net Primary Productivity and Implications for Climate Change, Annu. Rev. Plant Biol., 63, 637–661, https://doi.org/10.1146/annurev-arplant-042110-103829, 2012.
Ashmore, M. R.: Assessing the future global impacts of ozone on vegetation, Plant Cell Environ., 28, 949–964, https://doi.org/10.1111/j.1365-3040.2005.01341.x, 2005.
Banta, R. M., Senff, C. J., Alvarez, R. J., Langford, A. O., Parrish, D. D., Trainer, M. K., Darby, L. S., Hardesty, R. M., Lambeth, B., and Neuman, J. A.: Dependence of daily peak O3 concentrations near Houston, Texas on environmental factors: Wind speed, temperature, and boundary-layer depth, Atmos. Environ., 45, 162–173, https://doi.org/10.1016/j.atmosenv.2010.09.030, 2011.
Chen, L., Liao, H., Zhu, J., Li, K., Bai, Y., Yue, X., Yang, Y., Hu, J., and Zhang, M.: Increases in ozone-related mortality in China over 2013–2030 attributed to historical ozone deterioration and future population aging, Sci. Total Environ., 858, 159972, https://doi.org/10.1016/j.scitotenv.2022.159972, 2023.
China Meteorological Administration (CMA): Daily Timed Data from automated weather stations in China, https://data.cma.cn/en/?r=data/detail&dataCode=A.0012.0001, last access: 22 May 2022.
Dai, H., Huang, G., Wang, J., and Zeng, H.: VAR-tree model based spatio-temporal characterization and prediction of O3 concentration in China, Ecotox. Environ. Safe., 257, 114960, https://doi.org/10.1016/j.ecoenv.2023.114960, 2023.
Ding, H., Kong, L., You, Y., Mao, J., Chen, W., Chen, D., Chang, M., and Wang, X.: Effects of tropical cyclones with different tracks on ozone pollution over the Pearl River Delta region, Atmos. Res., 286, 106680, https://doi.org/10.1016/j.atmosres.2023.106680, 2023.
Feng, Z., Hu, E., Wang, X., Jiang, L., and Liu, X.: Ground-level O3 pollution and its impacts on food crops in China: A review, Environ. Pollut., 199, 42–48, https://doi.org/10.1016/j.envpol.2015.01.016, 2015.
Fu, Y. and Liao, H.: Impacts of land use and land cover changes on biogenic emissions of volatile organic compounds in China from the late 1980s to the mid-2000s: implications for tropospheric ozone and secondary organic aerosol, Tellus B, 66, 24987, https://doi.org/10.3402/tellusb.v66.24987, 2014.
Fu, Y., Liao, H., and Yang, Y.: Interannual and Decadal Changes in Tropospheric Ozone in China and the Associated Chemistry-Climate Interactions: A Review, Adv. Atmos. Sci., 36, 975–993, https://doi.org/10.1007/s00376-019-8216-9, 2019.
Gelaro, R., McCarty, W., Suárez, M. J., Todling, R., Molod, A., Takacs, L., Randles, C. A., Darmenov, A., Bosilovich, M. G., Reichle, R., Wargan, K., Coy, L., Cullather, R., Draper, C., Akella, S., Buchard, V., Conaty, A., Da Silva, A. M., Gu W., Kim, G., Koster, R., Lucchesi, R., Merkova, D., Nielsen, J., Partyka, G., Pawson, S., Putman, W., Rienecker, M., Schubert, S. D., Sienkiewicz, M., and Zhao, B.: The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2), J. Climate, 30, 5419–5454, https://doi.org/10.1175/JCLI-D-16-0758.1, 2017.
Gong, C. and Liao, H.: A typical weather pattern for ozone pollution events in North China, Atmos. Chem. Phys., 19, 13725–13740, https://doi.org/10.5194/acp-19-13725-2019, 2019.
Gori, A., Lin, N., Xi, D., and Emanuel, K.: Tropical cyclone climatology change greatly exacerbates US extreme rainfall–surge hazard, Nat. Clim. Change, 12, 171–178, https://doi.org/10.1038/s41558-021-01272-7, 2022.
Gu, X., Wang, T., and Li, C.: Elevated ozone decreases the multifunctionality of belowground ecosystems, Glob. Change Biol., 29, 890–908, https://doi.org/10.1111/gcb.16507, 2023.
Guenther, A. B., Jiang, X., Heald, C. L., Sakulyanontvittaya, T., Duhl, T., Emmons, L. K., and Wang, X.: The Model of Emissions of Gases and Aerosols from Nature version 2.1 (MEGAN2.1): an extended and updated framework for modeling biogenic emissions, Geosci. Model Dev., 5, 1471–1492, https://doi.org/10.5194/gmd-5-1471-2012, 2012.
Han, W., Wang, Y., and Liu, L.: The relationship between pre-landfall intensity change and post-landfall weakening of tropical cyclones over China, Front. Earth Sci., 10, 1082181, https://doi.org/10.3389/feart.2022.1082181, 2022.
Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A., Muñoz-Sabater, J., Nicolas, J., Peubey, C., Radu, R., Schepers, D., Simmons, A., Soci, C., Abdalla, S., Abellan, X., Balsamo, G., Bechtold, P., Biavati, G., Bidlot, J., Bonavita, M., De Chiara, G., Dahlgren, P., Dee, D., Diamantakis, M., Dragani, R., Flemming, J., Forbes, R., Fuentes, M., Geer, A., Haimberger, L., Healy, S., Hogan, R. J., Hólm, E., Janisková, M., Keeley, S., Laloyaux, P., Lopez, P., Lupu, C., Radnoti, G., de Rosnay, P., Rozum, I., Vamborg, F., Villaume, S., and Thépaut, J.-N.: The ERA5 global reanalysis, Q. J. Roy. Meteor. Soc., 146, 1999–2049, https://doi.org/10.1002/qj.3803, 2020.
Hersbach, H., Bell, B., Berrisford, P., Biavati, G., Horányi, A., Muñoz Sabater, J., Nicolas, J., Peubey, C., Radu, R., Rozum, I., Schepers, D., Simmons, A., Soci, C., Dee, D., and Thépaut, J.-N.: ERA5 hourly data on pressure levels from 1940 to present, Copernicus Climate Change Service (C3S) Climate Data Store (CDS) [data set], https://doi.org/10.24381/cds.bd0915c6, 2023.
Hoesly, R. M., Smith, S. J., Feng, L., Klimont, Z., Janssens-Maenhout, G., Pitkanen, T., Seibert, J. J., Vu, L., Andres, R. J., Bolt, R. M., Bond, T. C., Dawidowski, L., Kholod, N., Kurokawa, J.-I., Li, M., Liu, L., Lu, Z., Moura, M. C. P., O'Rourke, P. R., and Zhang, Q.: Historical (1750–2014) anthropogenic emissions of reactive gases and aerosols from the Community Emissions Data System (CEDS), Geosci. Model Dev., 11, 369–408, https://doi.org/10.5194/gmd-11-369-2018, 2018.
Huang, C., Chen, C. H., Li, L., Cheng, Z., Wang, H. L., Huang, H. Y., Streets, D. G., Wang, Y. J., Zhang, G. F., and Chen, Y. R.: Emission inventory of anthropogenic air pollutants and VOC species in the Yangtze River Delta region, China, Atmos. Chem. Phys., 11, 4105–4120, https://doi.org/10.5194/acp-11-4105-2011, 2011.
Huang, J., Pan, X., Guo, X., and Li, G.: Health impact of China's Air Pollution Prevention and Control Action Plan: an analysis of national air quality monitoring and mortality data, Lancet Planet. Health, 2, e313–e323, https://doi.org/10.1016/S2542-5196(18)30141-4, 2018.
Jacob, D. J., Logan, J. A., and Murti, P. P.: Effect of rising Asian emissions on surface ozone in the United States, Geophys. Res. Lett., 26, 2175–2178, https://doi.org/10.1029/1999GL900450, 1999.
Jammalamadaka, S. R. and Lund, U. J.: The effect of wind direction on ozone levels: a case study, Environ. Ecol. Stat., 13, 287–298, https://doi.org/10.1007/s10651-004-0012-7, 2006.
Ji, X., Chen, G., Chen, J., Xu, L., Lin, Z., Zhang, K., Fan, X., Li, M., Zhang, F., Wang, H., Huang, Z., and Hong, Y.: Meteorological impacts on the unexpected ozone pollution in coastal cities of China during the unprecedented hot summer of 2022, Sci. Total Environ., 914, 170035, https://doi.org/10.1016/j.scitotenv.2024.170035, 2024.
Jiang, Z., Li, J., Lu, X., Gong, C., Zhang, L., and Liao, H.: Impact of western Pacific subtropical high on ozone pollution over eastern China, Atmos. Chem. Phys., 21, 2601–2613, https://doi.org/10.5194/acp-21-2601-2021, 2021.
Kavassalis, S. C. and Murphy, J. G.: Understanding ozone-meteorology correlations: A role for dry deposition, Geophys. Res. Lett., 44, 2922–2931, https://doi.org/10.1002/2016GL071791, 2017.
Li, K., Jacob, D. J., Liao, H., Shen, L., Zhang, Q., and Bates, K. H.: Anthropogenic drivers of 2013–2017 trends in summer surface ozone in China, P. Natl. Acad. Sci. USA, 116, 422–427, https://doi.org/10.1073/pnas.1812168116, 2019.
Li, M., Yu, S., Chen, X., Li, Z., Zhang, Y., Wang, L., Liu, W., Li, P., Lichtfouse, E., Rosenfeld, D., and Seinfeld, J. H.: Large scale control of surface ozone by relative humidity observed during warm seasons in China, Environ. Chem. Lett., 19, 3981–3989, https://doi.org/10.1007/s10311-021-01265-0, 2021.
Lin, X., Yuan, Z., Yang, L., Luo, H., and Li, W.: Impact of Extreme Meteorological Events on Ozone in the Pearl River Delta, China, Aerosol Air Qual. Res., 19, 1307–1324, https://doi.org/10.4209/aaqr.2019.01.0027, 2019.
Liu, H., Liu, S., Xue, B., Lv, Z., Meng, Z., Yang, X., Xue, T., Yu, Q., and He, K.: Ground-level ozone pollution and its health impacts in China, Atmos. Environ., 173, 223–230, https://doi.org/10.1016/j.atmosenv.2017.11.014, 2018.
Lu, X., Zhang, L., Chen, Y., Zhou, M., Zheng, B., Li, K., Liu, Y., Lin, J., Fu, T.-M., and Zhang, Q.: Exploring 2016–2017 surface ozone pollution over China: source contributions and meteorological influences, Atmos. Chem. Phys., 19, 8339–8361, https://doi.org/10.5194/acp-19-8339-2019, 2019.
Lu, X., Yu, H., Ying, M., Zhao, B., Zhang, S., Lin, L., Bai, L., and Wan, R.: Western North Pacific Tropical Cyclone Database Created by the China Meteorological Administration, Adv. Atmos. Sci., 38, 690–699, https://doi.org/10.1007/s00376-020-0211-7, 2021 (data available at: https://tcdata.typhoon.org.cn/zjljsjj.html).
Luo, M. and Lau, N.-C.: Heat Waves in Southern China: Synoptic Behavior, Long-Term Change, and Urbanization Effects, J. Climate, 30, 703–720, https://doi.org/10.1175/JCLI-D-16-0269.1, 2017.
Ma, M., Gao, Y., Wang, Y., Zhang, S., Leung, L. R., Liu, C., Wang, S., Zhao, B., Chang, X., Su, H., Zhang, T., Sheng, L., Yao, X., and Gao, H.: Substantial ozone enhancement over the North China Plain from increased biogenic emissions due to heat waves and land cover in summer 2017, Atmos. Chem. Phys., 19, 12195–12207, https://doi.org/10.5194/acp-19-12195-2019, 2019.
Matthews, T., Wilby, R. L., and Murphy, C.: An emerging tropical cyclone–deadly heat compound hazard, Nat. Clim. Change, 9, 602–606, https://doi.org/10.1038/s41558-019-0525-6, 2019.
Meng, K., Zhao, T., Xu, X., Hu, Y., Zhao, Y., Zhang, L., Pang, Y., Ma, X., Bai, Y., Zhao, Y., and Zhen, S.: Anomalous surface O3 changes in North China Plain during the northwestward movement of a landing typhoon, Sci. Total Environ., 820, 153196, https://doi.org/10.1016/j.scitotenv.2022.153196, 2022.
Meng, X., Wang, W., Shi, S., Zhu, S., Wang, P., Chen, R., Xiao, Q., Xue, T., Geng, G., Zhang, Q., Kan, H., and Zhang, H.: Evaluating the spatiotemporal ozone characteristics with high-resolution predictions in mainland China, 2013–2019, Environ. Pollut., 299, 118865, https://doi.org/10.1016/j.envpol.2022.118865, 2022.
Ni, Y., Yang, Y., Wang, H., Li, H., Li, M., and Wang, P.: Contrasting changes in ozone during 2019–2021 between eastern China and the other regions of China, Sci. Total Environ., 908, 168272, https://doi.org/10.2139/ssrn.4563723, 2024.
Ouyang, S., Deng, T., Liu, R., Chen, J., He, G., Leung, J. C.-H., Wang, N., and Liu, S. C.: Impact of a subtropical high and a typhoon on a severe ozone pollution episode in the Pearl River Delta, China, Atmos. Chem. Phys., 22, 10751–10767, https://doi.org/10.5194/acp-22-10751-2022, 2022.
Pye, H. O. T., Liao, H., Wu, S., Mickley, L. J., Jacob, D. J., Henze, D. K., and Seinfeld, J. H.: Effect of changes in climate and emissions on future sulfate-nitrate-ammonium aerosol levels in the United States, J. Geophys. Res.-Atmos., 114, 2008JD010701, https://doi.org/10.1029/2008JD010701, 2009.
Qu, K., Wang, X., Yan, Y., Shen, J., Xiao, T., Dong, H., Zeng, L., and Zhang, Y.: A comparative study to reveal the influence of typhoons on the transport, production and accumulation of O3 in the Pearl River Delta, China, Atmos. Chem. Phys., 21, 11593–11612, https://doi.org/10.5194/acp-21-11593-2021, 2021.
Sherwen, T., Schmidt, J. A., Evans, M. J., Carpenter, L. J., Großmann, K., Eastham, S. D., Jacob, D. J., Dix, B., Koenig, T. K., Sinreich, R., Ortega, I., Volkamer, R., Saiz-Lopez, A., Prados-Roman, C., Mahajan, A. S., and Ordóñez, C.: Global impacts of tropospheric halogens (Cl, Br, I) on oxidants and composition in GEOS-Chem, Atmos. Chem. Phys., 16, 12239–12271, https://doi.org/10.5194/acp-16-12239-2016, 2016.
Shu, L., Xie, M., Wang, T., Gao, D., Chen, P., Han, Y., Li, S., Zhuang, B., and Li, M.: Integrated studies of a regional ozone pollution synthetically affected by subtropical high and typhoon system in the Yangtze River Delta region, China, Atmos. Chem. Phys., 16, 15801–15819, https://doi.org/10.5194/acp-16-15801-2016, 2016.
The International GEOS-Chem User Community: geoschem/GCClassic: GEOS-Chem 13.4.1 (13.4.1), Zenodo [data set], https://doi.org/10.5281/zenodo.6564702, 2022.
Tuleya, R. E., Bender, M. A., and Kurihara, Y.: A Simulation Study of the Landfall of Tropical Cyclones, Mon. Weather Rev., 112, 124–136, https://doi.org/10.1175/1520-0493(1984)112<0124:ASSOTL>2.0.CO;2, 1984.
Turner, M. C., Jerrett, M., Pope, C. A., Krewski, D., Gapstur, S. M., Diver, W. R., Beckerman, B. S., Marshall, J. D., Su, J., Crouse, D. L., and Burnett, R. T.: Long-Term Ozone Exposure and Mortality in a Large Prospective Study, Am. J. Resp. Crit. Care, 193, 1134–1142, https://doi.org/10.1164/rccm.201508-1633OC, 2016.
van der Werf, G. R., Randerson, J. T., Giglio, L., van Leeuwen, T. T., Chen, Y., Rogers, B. M., Mu, M., van Marle, M. J. E., Morton, D. C., Collatz, G. J., Yokelson, R. J., and Kasibhatla, P. S.: Global fire emissions estimates during 1997–2016, Earth Syst. Sci. Data, 9, 697–720, https://doi.org/10.5194/essd-9-697-2017, 2017.
Wang, N., Huang, X., Xu, J., Wang, T., Tan, Z., and Ding, A.: Typhoon-boosted biogenic emission aggravates cross-regional ozone pollution in China, Sci. Adv., 8, eabl6166, https://doi.org/10.1126/sciadv.abl6166, 2022.
Wang, P., Tang, J., Wang, S., Dong, X., and Fang, J.: Regional heatwaves in china: a cluster analysis, Clim. Dynam., 50, 1901–1917, https://doi.org/10.1007/s00382-017-3728-4, 2018.
Wang, P., Hui, P., Xue, D., and Tang, J.: Future projection of heat waves over China under global warming within the CORDEX-EA-II project, Clim. Dynam., 53, 957–973, https://doi.org/10.1007/s00382-019-04621-7, 2019a.
Wang, P., Leung, L. R., Lu, J., Song, F., and Tang, J.: Extreme wet-bulb temperatures in China: The significant role of moisture, J. Geophys. Res.-Atmos., 124, 11944–11960, https://doi.org/10.1029/2019JD031477, 2019b.
Wang, P., Yang, Y., Li, H., Chen, L., Dang, R., Xue, D., Li, B., Tang, J., Leung, L. R., and Liao, H.: North China Plain as a hot spot of ozone pollution exacerbated by extreme high temperatures, Atmos. Chem. Phys., 22, 4705–4719, https://doi.org/10.5194/acp-22-4705-2022, 2022.
Wang, P., Yang, Y., Xue, D., Qu, Y., Tang, J., Leung, L. R., and Liao, H.: Increasing Compound Hazards of Tropical Cyclones and Heatwaves over Southeastern Coast of China under Climate Warming, J. Climate, 36, 2243–2257, https://doi.org/10.1175/JCLI-D-22-0279.1, 2023.
Wang, T., Xue, L., Brimblecombe, P., Lam, Y. F., Li, L., and Zhang, L.: Ozone pollution in China: A review of concentrations, meteorological influences, chemical precursors, and effects, Sci. Total Environ., 575, 1582–1596, https://doi.org/10.1016/j.scitotenv.2016.10.081, 2017.
Wang, T., Zhong, Z., Sun, Y., and Wang, J.: Impacts of tropical cyclones on the meridional movement of the western Pacific subtropical high, Atmos. Sci. Lett., 20, e893, https://doi.org/10.1002/asl.893, 2019.
Wang, W., Zhou, W., Li, X., Wang, X., and Wang, D.: Synoptic-scale characteristics and atmospheric controls of summer heat waves in China, Clim. Dynam., 46, 2923–2941, https://doi.org/10.1007/s00382-015-2741-8, 2016.
Wang, X., Chen, F., Wu, Z., Zhang, M., Tewari, M., Guenther, A., and Wiedinmyer, C.: Impacts of weather conditions modified by urban expansion on surface ozone: Comparison between the Pearl River Delta and Yangtze River Delta regions, Adv. Atmos. Sci., 26, 962–972, https://doi.org/10.1007/s00376-009-8001-2, 2009.
Wang, Z., Hu, B., Zhang, C., Atkinson, P. M., Wang, Z., Xu, K., Chang, J., Fang, X., Jiang, Y., and Shi, Z.: How the Air Clean Plan and carbon mitigation measures co-benefited China in PM2.5 reduction and health from 2014 to 2020, Environ. Int., 169, 107510, https://doi.org/10.1016/j.envint.2022.107510, 2022.
Wei, J. and Li, Z.: ChinaHighO3: Big Data Seamless 1 km Ground-level MDA8 O3 Dataset for China (2000–Present) (2 (2000–2023)), Zenodo [data set], https://doi.org/10.5281/zenodo.13342827, 2024.
Wei, J., Li, Z., Li, K., Dickerson, R. R., Pinker, R. T., Wang, J., Liu, X., Sun, L., Xue, W., and Cribb, M.: Full-coverage mapping and spatiotemporal variations of ground-level ozone (O3) pollution from 2013 to 2020 across China, Remote Sens. Environ., 270, 112775, https://doi.org/10.1016/j.rse.2021.112775, 2022.
Wei, X., Lam, K. S., Cao, C., Li, H., and He, J.: Dynamics of the Typhoon Haitang Related High Ozone Episode over Hong Kong, Adv. Atmos. Sci., 2016, 6089154, https://doi.org/10.1155/2016/6089154, 2016.
Wu, J., Chen, Y., Liao, Z., Gao, X., Zhai, P., and Hu, Y.: Increasing risk from landfalling tropical cyclone-heatwave compound events to coastal and inland China, Environ. Res. Lett., 17, 105007, https://doi.org/10.1088/1748-9326/ac9747, 2022.
Xiao, Y. F., Duan, Z. D., Xiao, Y. Q., Ou, J. P., Chang, L., and Li, Q. S.: Typhoon wind hazard analysis for southeast China coastal regions, Struct. Saf., 33, 286–295, https://doi.org/10.1016/j.strusafe.2011.04.003, 2011.
Yang, Y., Liao, H., and Li, J.: Impacts of the East Asian summer monsoon on interannual variations of summertime surface-layer ozone concentrations over China, Atmos. Chem. Phys., 14, 6867–6879, https://doi.org/10.5194/acp-14-6867-2014, 2014.
Yang, Y., Li, M., Wang, H., Li, H., Wang, P., Li, K., Gao, M., and Liao, H.: ENSO modulation of summertime tropospheric ozone over China, Environ. Res. Lett., 17, 034020, https://doi.org/10.1088/1748-9326/ac54cd, 2022.
Yin, Z., Cao, B., and Wang, H.: Dominant patterns of summer ozone pollution in eastern China and associated atmospheric circulations, Atmos. Chem. Phys., 19, 13933–13943, https://doi.org/10.5194/acp-19-13933-2019, 2019.
Ying, M., Zhang, W., Yu, H., Lu, X., Feng, J., Fan, Y., Zhu, Y., and Chen, D.: An Overview of the China Meteorological Administration Tropical Cyclone Database, J. Atmos. Ocean. Tech., 31, 287–301, https://doi.org/10.1175/JTECH-D-12-00119.1, 2014 (data available at: https://tcdata.typhoon.org.cn/zjljsjj.html).
Zhan, C. and Xie, M.: Exploring the link between ozone pollution and stratospheric intrusion under the influence of tropical cyclone Ampil, Sci. Total Environ., 828, 154261, https://doi.org/10.1016/j.scitotenv.2022.154261, 2022.
Zhan, C., Xie, M., Huang, C., Liu, J., Wang, T., Xu, M., Ma, C., Yu, J., Jiao, Y., Li, M., Li, S., Zhuang, B., Zhao, M., and Nie, D.: Ozone affected by a succession of four landfall typhoons in the Yangtze River Delta, China: major processes and health impacts, Atmos. Chem. Phys., 20, 13781–13799, https://doi.org/10.5194/acp-20-13781-2020, 2020.
Zhang, J., Gao, Y., Luo, K., Leung, L. R., Zhang, Y., Wang, K., and Fan, J.: Impacts of compound extreme weather events on ozone in the present and future, Atmos. Chem. Phys., 18, 9861–9877, https://doi.org/10.5194/acp-18-9861-2018, 2018.
Zhang, M., Yang, Y., Zhan, C., Zong, L., Gul, C., and Wang, M.: Tropical cyclone-related heatwave episodes in the Greater Bay Area, China: Synoptic patterns and urban-rural disparities, Weather and Climate Extremes, 44, 100656, https://doi.org/10.1016/j.wace.2024.100656, 2024.
Zhang, Y., Dai, J., Li, Q., Chen, T., Mu, J., Brasseur, G., Wang, T., and Xue, L.: Biogenic volatile organic compounds enhance ozone production and complicate control efforts: Insights from long-term observations in Hong Kong, Atmos. Environ., 309, 119917, https://doi.org/10.1016/j.atmosenv.2023.119917, 2023.
Zhou, Y., Yang, Y., Wang, H., Wang, J., Li, M., Li, H., Wang, P., Zhu, J., Li, K., and Liao, H.: Summer ozone pollution in China affected by the intensity of Asian monsoon systems, Sci. Total Environ., 849, 157785, https://doi.org/10.1016/j.scitotenv.2022.157785, 2022.
Short summary
We investigate extremely hot weather impacts on surface ozone over the southeastern coast of China with and without tropical cyclones. Compared to hot days alone, ozone concentration decreased notably in the Yangtze River Delta (YRD) but increased in the Pearl River Delta (PRD) during tropical cyclones and hot days. The YRD benefited from strong and clean sea winds aiding ozone elimination. In contrast, the PRD experienced strong northeasterly winds that potentially transport ozone pollution.
We investigate extremely hot weather impacts on surface ozone over the southeastern coast of...
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