Articles | Volume 21, issue 3
https://doi.org/10.5194/acp-21-1861-2021
https://doi.org/10.5194/acp-21-1861-2021
Research article
 | 
10 Feb 2021
Research article |  | 10 Feb 2021

Simulation of radon-222 with the GEOS-Chem global model: emissions, seasonality, and convective transport

Bo Zhang, Hongyu Liu, James H. Crawford, Gao Chen, T. Duncan Fairlie, Scott Chambers, Chang-Hee Kang, Alastair G. Williams, Kai Zhang, David B. Considine, Melissa P. Sulprizio, and Robert M. Yantosca

Related authors

Investigating the role of typhoon-induced gravity waves and stratospheric hydration in the formation of tropopause cirrus clouds observed during the 2017 Asian monsoon
Amit Kumar Pandit, Jean-Paul Vernier, Thomas Duncan Fairlie, Kristopher M. Bedka, Melody A. Avery, Harish Gadhavi, Madineni Venkat Ratnam, Sanjeev Dwivedi, Kasimahanthi Amar Jyothi, Frank G. Wienhold, Holger Vömel, Hongyu Liu, Bo Zhang, Buduru Suneel Kumar, Tra Dinh, and Achuthan Jayaraman
EGUsphere, https://doi.org/10.5194/egusphere-2023-2236,https://doi.org/10.5194/egusphere-2023-2236, 2023
Short summary
Exploring the inorganic composition of the Asian Tropopause Aerosol Layer using medium-duration balloon flights
Hazel Vernier, Neeraj Rastogi, Hongyu Liu, Amit Kumar Pandit, Kris Bedka, Anil Patel, Madineni Venkat Ratnam, Buduru Suneel Kumar, Bo Zhang, Harish Gadhavi, Frank Wienhold, Gwenael Berthet, and Jean-Paul Vernier
Atmos. Chem. Phys., 22, 12675–12694, https://doi.org/10.5194/acp-22-12675-2022,https://doi.org/10.5194/acp-22-12675-2022, 2022
Short summary
North Atlantic Ocean SST-gradient-driven variations in aerosol and cloud evolution along Lagrangian cold-air outbreak trajectories
Kevin J. Sanchez, Bo Zhang, Hongyu Liu, Matthew D. Brown, Ewan C. Crosbie, Francesca Gallo, Johnathan W. Hair, Chris A. Hostetler, Carolyn E. Jordan, Claire E. Robinson, Amy Jo Scarino, Taylor J. Shingler, Michael A. Shook, Kenneth L. Thornhill, Elizabeth B. Wiggins, Edward L. Winstead, Luke D. Ziemba, Georges Saliba, Savannah L. Lewis, Lynn M. Russell, Patricia K. Quinn, Timothy S. Bates, Jack Porter, Thomas G. Bell, Peter Gaube, Eric S. Saltzman, Michael J. Behrenfeld, and Richard H. Moore
Atmos. Chem. Phys., 22, 2795–2815, https://doi.org/10.5194/acp-22-2795-2022,https://doi.org/10.5194/acp-22-2795-2022, 2022
Short summary
Observation and modeling of high-7Be concentration events at the surface in northern Europe associated with the instability of the Arctic polar vortex in early 2003
Erika Brattich, Hongyu Liu, Bo Zhang, Miguel Ángel Hernández-Ceballos, Jussi Paatero, Darko Sarvan, Vladimir Djurdjevic, Laura Tositti, and Jelena Ajtić
Atmos. Chem. Phys., 21, 17927–17951, https://doi.org/10.5194/acp-21-17927-2021,https://doi.org/10.5194/acp-21-17927-2021, 2021
Short summary
Aerosol responses to precipitation along North American air trajectories arriving at Bermuda
Hossein Dadashazar, Majid Alipanah, Miguel Ricardo A. Hilario, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Andrew J. Peters, Amy Jo Scarino, Michael Shook, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Bo Zhang, Luke Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 21, 16121–16141, https://doi.org/10.5194/acp-21-16121-2021,https://doi.org/10.5194/acp-21-16121-2021, 2021
Short summary

Related subject area

Subject: Gases | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Observational and model evidence for a prominent stratospheric influence on variability in tropospheric nitrous oxide
Cynthia D. Nevison, Qing Liang, Paul A. Newman, Britton B. Stephens, Geoff Dutton, Xin Lan, Roisin Commane, Yenny Gonzalez, and Eric Kort
Atmos. Chem. Phys., 24, 10513–10529, https://doi.org/10.5194/acp-24-10513-2024,https://doi.org/10.5194/acp-24-10513-2024, 2024
Short summary
Estimation of Canada's methane emissions: inverse modelling analysis using the Environment and Climate Change Canada (ECCC) measurement network
Misa Ishizawa, Douglas Chan, Doug Worthy, Elton Chan, Felix Vogel, Joe R. Melton, and Vivek K. Arora
Atmos. Chem. Phys., 24, 10013–10038, https://doi.org/10.5194/acp-24-10013-2024,https://doi.org/10.5194/acp-24-10013-2024, 2024
Short summary
Spatiotemporal source apportionment of ozone pollution over the Greater Bay Area
Yiang Chen, Xingcheng Lu, and Jimmy C. H. Fung
Atmos. Chem. Phys., 24, 8847–8864, https://doi.org/10.5194/acp-24-8847-2024,https://doi.org/10.5194/acp-24-8847-2024, 2024
Short summary
Potential of 14C-based vs. ΔCO-based ΔffCO2 observations to estimate urban fossil fuel CO2 (ffCO2) emissions
Fabian Maier, Christian Rödenbeck, Ingeborg Levin, Christoph Gerbig, Maksym Gachkivskyi, and Samuel Hammer
Atmos. Chem. Phys., 24, 8183–8203, https://doi.org/10.5194/acp-24-8183-2024,https://doi.org/10.5194/acp-24-8183-2024, 2024
Short summary
On the uncertainty of anthropogenic aromatic volatile organic compound emissions: model evaluation and sensitivity analysis
Kevin Oliveira, Marc Guevara, Oriol Jorba, Hervé Petetin, Dene Bowdalo, Carles Tena, Gilbert Montané Pinto, Franco López, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7137–7177, https://doi.org/10.5194/acp-24-7137-2024,https://doi.org/10.5194/acp-24-7137-2024, 2024
Short summary

Cited articles

Allen, D. J., Rood, R. B., Thompson, A. M., and Hudson, R.D.: Three-dimensional radon-222 calculations using assimilated meteorological data and a convective mixing algorithm, J. Geophys. Res.-Atmos., 101, 6871–6881, 1996. 
Balkanski, Y. J., Jacob, D. J., Arimoto, R., and Kritz, M. A.: Distribution of 222 Rn over the North Pacific: implications for continental influences, J. Atmos. Chem., 14, 353–374, 1992. 
Balkanski, Y. J., Jacob, D. J., Gardner, G. M., Graustein, W. C., and Turekian, K. K.: Transport and residence times of tropospheric aerosols inferred from a global three-dimensional simulation of 210Pb, J. Geophys. Res.-Atmos., 98, 20573–20586, https://doi.org/10.1029/93jd02456, 1993. 
Bey, I., Jacob, D. J., Yantosca, R. M., Logan, J. A., Field, B. D., Fiore, A. M., Li, Q. B., Liu, H. G. Y., Mickley, L. J., and Schultz, M. G.: Global modeling of tropospheric chemistry with assimilated meteorology: Model description and evaluation, J. Geophys. Res., 106, 23073–23095, https://doi.org/10.1029/2001JD000807, 2001. 
Botha, R., Labuschagne, C., Williams, A. G., Bosman, G., Brunke, E. G., Rossouw, A., and Lindsay, R.: Characterising fifteen years of continuous atmospheric radon activity observations at Cape Point (South Africa), Atmos. Environ., 176, 30–39, 2018. 
Download
Short summary
We simulate atmospheric 222Rn using the GEOS-Chem model to improve understanding of 222Rn emissions and characterize convective transport in the model. We demonstrate the potential of a customized global 222Rn emission scenario to improve simulated surface 222Rn concentrations and seasonality. We assess convective transport using observed 222Rn vertical profiles. Results have important implications for using chemical transport models to interpret the transport of trace gases and aerosols.
Altmetrics
Final-revised paper
Preprint