Articles | Volume 18, issue 9
https://doi.org/10.5194/acp-18-6785-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-18-6785-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
16 May 2018
Research article |
| 16 May 2018
| 16 May 2018
Characterizing biospheric carbon balance using CO2 observations from the OCO-2 satellite
Department of Global Ecology, Carnegie Institution for Science, Stanford, CA, USA
now at: the Department of Environmental Health and Engineering, Johns Hopkins University, Baltimore, MD, USA
Anna M. Michalak
Department of Global Ecology, Carnegie Institution for Science, Stanford, CA, USA
Vineet Yadav
Jet Propulsion Laboratory, California Institute of Technology, Pasadena, CA, USA
Jovan M. Tadić
Lawrence Berkeley National Laboratory, Berkeley, CA, USA
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Changes in the carbon stocks of terrestrial ecosystems result in emissions and removals of CO2. These can be driven by anthropogenic activities (e.g., deforestation), natural processes (e.g., fires) or in response to rising CO2 (e.g., CO2 fertilization). This paper describes a dataset of CO2 emissions and removals derived from atmospheric CO2 observations. This pilot dataset informs current capabilities and future developments towards top-down monitoring and verification systems.
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Atmospheric inverse modeling describes the process of estimating greenhouse gas fluxes or air pollution emissions at the Earth's surface using observations of these gases collected in the atmosphere. The launch of new satellites, the expansion of surface observation networks, and a desire for more detailed maps of surface fluxes have yielded numerous computational and statistical challenges. This article describes computationally efficient methods for large-scale atmospheric inverse modeling.
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NASA's Orbiting Carbon Observatory 2 (OCO-2) satellite observes atmospheric CO2 globally. We use a multiple regression and inverse model to quantify the relationships between OCO-2 and environmental drivers within individual years for 2015–2018 and within seven global biomes. Our results point to limitations of current space-based observations for inferring environmental relationships but also indicate the potential to inform key relationships that are very uncertain in process-based models.
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New observations of greenhouse gases from satellites and aircraft provide an unprecedented window into global carbon sources and sinks. However, these new datasets also present enormous computational challenges due to the sheer number of observations. In this article, we discuss the challenges of estimating greenhouse gas source and sinks using very large atmospheric datasets and evaluate several strategies for overcoming these challenges.
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NASA's Orbiting Carbon Observatory 2 (OCO-2) satellite observes CO2 in the atmosphere. The satellite measures radiation, and these measurements are then converted to an estimate of atmospheric CO2. This conversion or retrieval algorithm has improved markedly since the satellite launch. We find that these improvements in the CO2 retrieval are having a potentially transformative effect on satellite-based estimates of the global biospheric carbon balance.
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Changes in the carbon stocks of terrestrial ecosystems result in emissions and removals of CO2. These can be driven by anthropogenic activities (e.g., deforestation), natural processes (e.g., fires) or in response to rising CO2 (e.g., CO2 fertilization). This paper describes a dataset of CO2 emissions and removals derived from atmospheric CO2 observations. This pilot dataset informs current capabilities and future developments towards top-down monitoring and verification systems.
Taewon Cho, Julianne Chung, Scot M. Miller, and Arvind K. Saibaba
Geosci. Model Dev., 15, 5547–5565, https://doi.org/10.5194/gmd-15-5547-2022, https://doi.org/10.5194/gmd-15-5547-2022, 2022
Short summary
Short summary
Atmospheric inverse modeling describes the process of estimating greenhouse gas fluxes or air pollution emissions at the Earth's surface using observations of these gases collected in the atmosphere. The launch of new satellites, the expansion of surface observation networks, and a desire for more detailed maps of surface fluxes have yielded numerous computational and statistical challenges. This article describes computationally efficient methods for large-scale atmospheric inverse modeling.
Xiaoling Liu, August L. Weinbren, He Chang, Jovan M. Tadić, Marikate E. Mountain, Michael E. Trudeau, Arlyn E. Andrews, Zichong Chen, and Scot M. Miller
Geosci. Model Dev., 14, 4683–4696, https://doi.org/10.5194/gmd-14-4683-2021, https://doi.org/10.5194/gmd-14-4683-2021, 2021
Short summary
Short summary
Observations of greenhouse gases have become far more numerous in recent years due to new satellite observations. The sheer size of these datasets makes it challenging to incorporate these data into statistical models and use these data to estimate greenhouse gas sources and sinks. In this paper, we develop an approach to reduce the size of these datasets while preserving the most information possible. We subsequently test this approach using satellite observations of carbon dioxide.
Dien Wu, John C. Lin, Henrique F. Duarte, Vineet Yadav, Nicholas C. Parazoo, Tomohiro Oda, and Eric A. Kort
Geosci. Model Dev., 14, 3633–3661, https://doi.org/10.5194/gmd-14-3633-2021, https://doi.org/10.5194/gmd-14-3633-2021, 2021
Short summary
Short summary
A model (SMUrF) is presented that estimates biogenic CO2 fluxes over cities around the globe to separate out biogenic fluxes from anthropogenic emissions. The model leverages satellite-based solar-induced fluorescence data and a machine-learning technique. We evaluate the biogenic fluxes against flux observations and show contrasts between biogenic and anthropogenic fluxes over cities, revealing urban–rural flux gradients, diurnal cycles, and the resulting imprints on atmospheric-column CO2.
Zichong Chen, Junjie Liu, Daven K. Henze, Deborah N. Huntzinger, Kelley C. Wells, Stephen Sitch, Pierre Friedlingstein, Emilie Joetzjer, Vladislav Bastrikov, Daniel S. Goll, Vanessa Haverd, Atul K. Jain, Etsushi Kato, Sebastian Lienert, Danica L. Lombardozzi, Patrick C. McGuire, Joe R. Melton, Julia E. M. S. Nabel, Benjamin Poulter, Hanqin Tian, Andrew J. Wiltshire, Sönke Zaehle, and Scot M. Miller
Atmos. Chem. Phys., 21, 6663–6680, https://doi.org/10.5194/acp-21-6663-2021, https://doi.org/10.5194/acp-21-6663-2021, 2021
Short summary
Short summary
NASA's Orbiting Carbon Observatory 2 (OCO-2) satellite observes atmospheric CO2 globally. We use a multiple regression and inverse model to quantify the relationships between OCO-2 and environmental drivers within individual years for 2015–2018 and within seven global biomes. Our results point to limitations of current space-based observations for inferring environmental relationships but also indicate the potential to inform key relationships that are very uncertain in process-based models.
Scot M. Miller, Arvind K. Saibaba, Michael E. Trudeau, Marikate E. Mountain, and Arlyn E. Andrews
Geosci. Model Dev., 13, 1771–1785, https://doi.org/10.5194/gmd-13-1771-2020, https://doi.org/10.5194/gmd-13-1771-2020, 2020
Short summary
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New observations of greenhouse gases from satellites and aircraft provide an unprecedented window into global carbon sources and sinks. However, these new datasets also present enormous computational challenges due to the sheer number of observations. In this article, we discuss the challenges of estimating greenhouse gas source and sinks using very large atmospheric datasets and evaluate several strategies for overcoming these challenges.
Scot M. Miller and Anna M. Michalak
Atmos. Chem. Phys., 20, 323–331, https://doi.org/10.5194/acp-20-323-2020, https://doi.org/10.5194/acp-20-323-2020, 2020
Short summary
Short summary
NASA's Orbiting Carbon Observatory 2 (OCO-2) satellite observes CO2 in the atmosphere. The satellite measures radiation, and these measurements are then converted to an estimate of atmospheric CO2. This conversion or retrieval algorithm has improved markedly since the satellite launch. We find that these improvements in the CO2 retrieval are having a potentially transformative effect on satellite-based estimates of the global biospheric carbon balance.
Peter J. Rayner, Anna M. Michalak, and Frédéric Chevallier
Atmos. Chem. Phys., 19, 13911–13932, https://doi.org/10.5194/acp-19-13911-2019, https://doi.org/10.5194/acp-19-13911-2019, 2019
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This paper describes the methods for combining models and data to understand how nutrients and pollutants move through natural systems. The methods are analogous to the process of weather forecasting in which previous information is combined with new observations and a model to improve our knowledge of the internal state of the physical system. The methods appear highly diverse but the paper shows that they are all examples of a single underlying formalism.
Ju-Mee Ryoo, Laura T. Iraci, Tomoaki Tanaka, Josette E. Marrero, Emma L. Yates, Inez Fung, Anna M. Michalak, Jovan Tadić, Warren Gore, T. Paul Bui, Jonathan M. Dean-Day, and Cecilia S. Chang
Atmos. Meas. Tech., 12, 2949–2966, https://doi.org/10.5194/amt-12-2949-2019, https://doi.org/10.5194/amt-12-2949-2019, 2019
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We designed cylindrical flights and computed the emission fluxes using a kriging method and Gauss's theorem over Sacramento, California. Differences in wind treatment and background affect the emission estimates by a factor of 1.5 to 7. The effects of the vertical layer average and the vertical mass transfer on the emission estimates are found to be small, esp. local scale. The result also suggests a closed-shape flight profile can better contain total emissions than a one-sided curtain flight.
Robert R. Bogue, Florian M. Schwandner, Joshua B. Fisher, Ryan Pavlick, Troy S. Magney, Caroline A. Famiglietti, Kerry Cawse-Nicholson, Vineet Yadav, Justin P. Linick, Gretchen B. North, and Eliecer Duarte
Biogeosciences, 16, 1343–1360, https://doi.org/10.5194/bg-16-1343-2019, https://doi.org/10.5194/bg-16-1343-2019, 2019
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This study examined rainforest responses to elevated CO2 coming from volcanoes in Costa Rica. Comparing tree species, we found that leaf function responded when exposed to increasing CO2 levels. The chemical signature of volcanic CO2 is different than background CO2. Trees exposed to volcanic CO2 also had chemical signatures which showed the influence of volcanic CO2: trees not only
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Nils Hase, Scot M. Miller, Peter Maaß, Justus Notholt, Mathias Palm, and Thorsten Warneke
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Inverse modeling uses atmospheric measurements to estimate emissions of greenhouse gases, which are key to understand the climate system. However, the measurement information alone is typically insufficient to provide reasonable emission estimates. Additional information is required. This article applies modern mathematical inversion techniques to formulate such additional knowledge. It is a prime example of how such tools can improve the quality of estimates compared to commonly used methods.
Kristal R. Verhulst, Anna Karion, Jooil Kim, Peter K. Salameh, Ralph F. Keeling, Sally Newman, John Miller, Christopher Sloop, Thomas Pongetti, Preeti Rao, Clare Wong, Francesca M. Hopkins, Vineet Yadav, Ray F. Weiss, Riley M. Duren, and Charles E. Miller
Atmos. Chem. Phys., 17, 8313–8341, https://doi.org/10.5194/acp-17-8313-2017, https://doi.org/10.5194/acp-17-8313-2017, 2017
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We present the first carbon dioxide (CO2) and methane (CH4) measurements from an extensive surface network as part of the Los Angeles Megacity Carbon Project. We describe methods that are essential for understanding carbon fluxes from complex urban environments. CO2 and CH4 levels are spatially and temporally variable, with urban sites showing significant enhancements relative to background. In 2015, the median afternoon enhancement near downtown Los Angeles was ~15 ppm CO2 and ~80 ppb CH4.
Anna M. Michalak, Nina A. Randazzo, and Frédéric Chevallier
Atmos. Chem. Phys., 17, 7405–7421, https://doi.org/10.5194/acp-17-7405-2017, https://doi.org/10.5194/acp-17-7405-2017, 2017
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The use of inverse modeling for quantifying emissions of greenhouse gases is increasing. Estimates are very difficult to evaluate objectively, however, due to limited atmospheric observations and the lack of direct emissions measurements at compatible scales. Diagnostic tools have been proposed to partially circumvent these limitations. This paper presents the first systematic review of the scope and applicability of these tools for atmospheric inversions of long-lived greenhouse gases.
Scot M. Miller and Anna M. Michalak
Atmos. Chem. Phys., 17, 3963–3985, https://doi.org/10.5194/acp-17-3963-2017, https://doi.org/10.5194/acp-17-3963-2017, 2017
Short summary
Short summary
We reviewed recent efforts to estimate state- and national-scale carbon dioxide and methane emissions from individual anthropogenic source sectors in the United States. State and federal greenhouse gas regulations almost always target reductions from specific source sectors, and reliable emission estimates are important to support and evaluate these policies. We also describe a number of forward-looking opportunities that would improve sector-specific estimates.
Jovan M. Tadić, Xuemei Qiu, Scot Miller, and Anna M. Michalak
Geosci. Model Dev., 10, 709–720, https://doi.org/10.5194/gmd-10-709-2017, https://doi.org/10.5194/gmd-10-709-2017, 2017
Short summary
Short summary
We developed a new method to create contiguous maps from sparse and/or noisy satellite observations. This approach could be used to produce retroactive or real-time estimates of environmental data observed by satellites which exhibit spatio-temporal autocorrelations. The method could be applied in a standalone mode or as part of a broader satellite data processing package. Maps produced in this way could then be incorporated into physical and biogeochemical models of the Earth system.
Sander Houweling, Peter Bergamaschi, Frederic Chevallier, Martin Heimann, Thomas Kaminski, Maarten Krol, Anna M. Michalak, and Prabir Patra
Atmos. Chem. Phys., 17, 235–256, https://doi.org/10.5194/acp-17-235-2017, https://doi.org/10.5194/acp-17-235-2017, 2017
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The aim of this paper is to present an overview of inverse modeling methods, developed over the years, for estimating the global sources and sinks of the greenhouse gas methane from atmospheric measurements. It provides insight into how techniques and estimates have evolved over time, what the remaining shortcomings are, new developments, and promising future directions.
A. Anthony Bloom, Thomas Lauvaux, John Worden, Vineet Yadav, Riley Duren, Stanley P. Sander, and David S. Schimel
Atmos. Chem. Phys., 16, 15199–15218, https://doi.org/10.5194/acp-16-15199-2016, https://doi.org/10.5194/acp-16-15199-2016, 2016
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Understanding terrestrial carbon processes is a major challenge in climate science. We define the satellite system required to understand greenhouse gas biogeochemistry: our study is focused on Amazon wetland CH4 emissions. We find that future geostationary satellites will provide the CH4 measurements required to understand wetland CH4 processes. Low-earth orbit satellites will be unable to resolve wetland CH4 processes due to a low number of cloud-free CH4 measurements over the Amazon basin.
Vineet Yadav and Anna M. Michalak
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2016-204, https://doi.org/10.5194/gmd-2016-204, 2016
Revised manuscript has not been submitted
Short summary
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Multiplication of two matrices that consists of few non-zero entries is a fundamental operation in problems that involve estimation of greenhouse gas fluxes from atmospheric measurements. To increase computational efficiency of estimating these quantities, modification of the standard matrix multiplication algorithm for multiplying these matrices is proposed in this research.
Bjorn-Gustaf J. Brooks, Ankur R. Desai, Britton B. Stephens, Anna M. Michalak, and Jakob Zscheischler
Biogeosciences Discuss., https://doi.org/10.5194/bg-2016-223, https://doi.org/10.5194/bg-2016-223, 2016
Manuscript not accepted for further review
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CO2 is the primary greenhouse gas, and its abundance in the atmosphere tends to increase during disturbances like drought. This paper demonstrates how CO2 measurements are combined with models to determine not only how strongly different locations influence CO2 measurement stations, but also the capacity of those measurement stations to detect drought effects. Understanding detection sensitivity will help assess what kinds of changes and turnings points can be monitored using atmospheric CO2.
Scot M. Miller, Roisin Commane, Joe R. Melton, Arlyn E. Andrews, Joshua Benmergui, Edward J. Dlugokencky, Greet Janssens-Maenhout, Anna M. Michalak, Colm Sweeney, and Doug E. J. Worthy
Biogeosciences, 13, 1329–1339, https://doi.org/10.5194/bg-13-1329-2016, https://doi.org/10.5194/bg-13-1329-2016, 2016
Short summary
Short summary
We use atmospheric data from the US and Canada to examine seven wetland methane flux estimates. Relative to existing estimates, we find a methane source that is smaller in magnitude with a broader seasonal cycle. Furthermore, we estimate the largest fluxes over the Hudson Bay Lowlands, a spatial distribution that differs from commonly used remote sensing estimates of wetland location.
J. M. Tadić, X. Qiu, V. Yadav, and A. M. Michalak
Geosci. Model Dev., 8, 3311–3319, https://doi.org/10.5194/gmd-8-3311-2015, https://doi.org/10.5194/gmd-8-3311-2015, 2015
J. Ray, J. Lee, V. Yadav, S. Lefantzi, A. M. Michalak, and B. van Bloemen Waanders
Geosci. Model Dev., 8, 1259–1273, https://doi.org/10.5194/gmd-8-1259-2015, https://doi.org/10.5194/gmd-8-1259-2015, 2015
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The paper presents a statistical method (shrinkage) that can be used to estimate rough emission fields, e.g., fossil fuel CO2 emissions, from measurements of concentrations. This method is demonstrated in a test case where the emissions are modeled using wavelets. We find that the method can eliminate unnecessary complexity from the wavelet model, ensures non-negativity of the emissions, is computationally efficient and is, by construction, insensitive to prior guesses of the total emission.
S. M. Miller, M. N. Hayek, A. E. Andrews, I. Fung, and J. Liu
Atmos. Chem. Phys., 15, 2903–2914, https://doi.org/10.5194/acp-15-2903-2015, https://doi.org/10.5194/acp-15-2903-2015, 2015
Y. Wei, S. Liu, D. N. Huntzinger, A. M. Michalak, N. Viovy, W. M. Post, C. R. Schwalm, K. Schaefer, A. R. Jacobson, C. Lu, H. Tian, D. M. Ricciuto, R. B. Cook, J. Mao, and X. Shi
Geosci. Model Dev., 7, 2875–2893, https://doi.org/10.5194/gmd-7-2875-2014, https://doi.org/10.5194/gmd-7-2875-2014, 2014
J. Ray, V. Yadav, A. M. Michalak, B. van Bloemen Waanders, and S. A. McKenna
Geosci. Model Dev., 7, 1901–1918, https://doi.org/10.5194/gmd-7-1901-2014, https://doi.org/10.5194/gmd-7-1901-2014, 2014
S. M. Miller, A. M. Michalak, and P. J. Levi
Geosci. Model Dev., 7, 303–315, https://doi.org/10.5194/gmd-7-303-2014, https://doi.org/10.5194/gmd-7-303-2014, 2014
A. Chatterjee and A. M. Michalak
Atmos. Chem. Phys., 13, 11643–11660, https://doi.org/10.5194/acp-13-11643-2013, https://doi.org/10.5194/acp-13-11643-2013, 2013
V. Yadav and A. M. Michalak
Geosci. Model Dev., 6, 583–590, https://doi.org/10.5194/gmd-6-583-2013, https://doi.org/10.5194/gmd-6-583-2013, 2013
Related subject area
Subject: Gases | Research Activity: Remote Sensing | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Measurement report: Combined use of MAX-DOAS and AERONET ground-based measurements in Montevideo, Uruguay, for the detection of distant biomass burning
Quantifying CH4 emissions from coal mine aggregation areas in Shanxi, China, using TROPOMI observations and the wind-assigned anomaly method
Identifying episodic carbon monoxide emission events in the MOPITT measurement dataset
Quantifying effects of long-range transport of NO2 over Delhi using back trajectories and satellite data
Measurement report: Ammonia in Paris derived from ground-based open-path and satellite observations
Anthropogenic CO2 emission estimates in the Tokyo metropolitan area from ground-based CO2 column observations
Characterizing the tropospheric water vapor spatial variation and trend using 2007–2018 COSMIC radio occultation and ECMWF reanalysis data
Detecting nitrogen oxide emissions in Qatar and quantifying emission factors of gas-fired power plants – a 4-year study
Identifying and accounting for the Coriolis effect in satellite NO2 observations and emission estimates
Characterisations of Europe's integrated water vapour and assessments of atmospheric reanalyses using more than 2 decades of ground-based GPS
Ground-level gaseous pollutants (NO2, SO2, and CO) in China: daily seamless mapping and spatiotemporal variations
NH3 spatiotemporal variability over Paris, Mexico City, and Toronto, and its link to PM2.5 during pollution events
Multi-axis differential optical absorption spectroscopy (MAX-DOAS) observations of formaldehyde and nitrogen dioxide at three sites in Asia and comparison with the global chemistry transport model CHASER
Quantifying CH4 emissions in hard coal mines from TROPOMI and IASI observations using the wind-assigned anomaly method
Estimation of surface ammonia concentrations and emissions in China from the polar-orbiting Infrared Atmospheric Sounding Interferometer and the FY-4A Geostationary Interferometric Infrared Sounder
Interannual variability in the Australian carbon cycle over 2015–2019, based on assimilation of Orbiting Carbon Observatory-2 (OCO-2) satellite data
Source and variability of formaldehyde (HCHO) at northern high latitudes: an integrated satellite, aircraft, and model study
Volcanic SO2 layer height by TROPOMI/S5P: evaluation against IASI/MetOp and CALIOP/CALIPSO observations
Spaceborne tropospheric nitrogen dioxide (NO2) observations from 2005–2020 over the Yangtze River Delta (YRD), China: variabilities, implications, and drivers
Novel assessment of numerical forecasting model relative humidity with satellite probabilistic estimates
Influence of springtime atmospheric circulation types on the distribution of air pollutants in the Arctic
Technical note: Evaluation of profile retrievals of aerosols and trace gases for MAX-DOAS measurements under different aerosol scenarios based on radiative transfer simulations
Diurnal evolution of total column and surface atmospheric ammonia in the megacity of Paris, France, during an intense springtime pollution episode
The reduction in C2H6 from 2015 to 2020 over Hefei, eastern China, points to air quality improvement in China
Mapping the drivers of formaldehyde (HCHO) variability from 2015 to 2019 over eastern China: insights from Fourier transform infrared observation and GEOS-Chem model simulation
The impact of Los Angeles Basin pollution and stratospheric intrusions on the surrounding San Gabriel Mountains as seen by surface measurements, lidar, and numerical models
Sudden changes in nitrogen dioxide emissions over Greece due to lockdown after the outbreak of COVID-19
Monitoring CO emissions of the metropolis Mexico City using TROPOMI CO observations
Pollution trace gas distributions and their transport in the Asian monsoon upper troposphere and lowermost stratosphere during the StratoClim campaign 2017
Spatial distribution of enhanced BrO and its relation to meteorological parameters in Arctic and Antarctic sea ice regions
Trends of atmospheric water vapour in Switzerland from ground-based radiometry, FTIR and GNSS data
A Raman lidar tropospheric water vapour climatology and height-resolved trend analysis over Payerne, Switzerland
The potential of Orbiting Carbon Observatory-2 data to reduce the uncertainties in CO2 surface fluxes over Australia using a variational assimilation scheme
Observing carbon dioxide emissions over China's cities and industrial areas with the Orbiting Carbon Observatory-2
Observational evidence of moistening the lowermost stratosphere via isentropic mixing across the subtropical jet
Fourier transform infrared time series of tropospheric HCN in eastern China: seasonality, interannual variability, and source attribution
NH3 emissions from large point sources derived from CrIS and IASI satellite observations
Diurnal cycle of short-term fluctuations of integrated water vapour above Switzerland
Retrieval of total column and surface NO2 from Pandora zenith-sky measurements
MAX-DOAS measurements of tropospheric NO2 and HCHO in Nanjing and a comparison to ozone monitoring instrument observations
Consistency and representativeness of integrated water vapour from ground-based GPS observations and ERA-Interim reanalysis
Towards monitoring localized CO2 emissions from space: co-located regional CO2 and NO2 enhancements observed by the OCO-2 and S5P satellites
Variability of bulk water vapor content in the marine cloudy boundary layers from microwave and near-infrared imagery
Trends and trend reversal detection in 2 decades of tropospheric NO2 satellite observations
Satellite-derived sulfur dioxide (SO2) emissions from the 2014–2015 Holuhraun eruption (Iceland)
Emissions of methane in Europe inferred by total column measurements
On the interpretation of upper-tropospheric humidity based on a second-order retrieval from infrared radiances
Carbon monoxide air pollution on sub-city scales and along arterial roads detected by the Tropospheric Monitoring Instrument
Ground-based MAX-DOAS observations of tropospheric formaldehyde VCDs and comparisons with the CAMS model at a rural site near Beijing during APEC 2014
Trends in global tropospheric ozone inferred from a composite record of TOMS/OMI/MLS/OMPS satellite measurements and the MERRA-2 GMI simulation
Matías Osorio, Alejandro Agesta, Tim Bösch, Nicolás Casaballe, Andreas Richter, Leonardo M. A. Alvarado, and Erna Frins
Atmos. Chem. Phys., 24, 7447–7465, https://doi.org/10.5194/acp-24-7447-2024, https://doi.org/10.5194/acp-24-7447-2024, 2024
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This study concerns the detection and quantification of long-transport emissions of a biomass burning event, which represents a major source of air pollutants, due to the release of large amounts of aerosols and chemical species into the atmosphere. The quantification was done using ground-based observations (which play an important role in assessing the abundance of trace gases and aerosols) over Montevideo (Uruguay) and using satellite observations.
Qiansi Tu, Frank Hase, Kai Qin, Jason Blake Cohen, Farahnaz Khosrawi, Xinrui Zou, Matthias Schneider, and Fan Lu
Atmos. Chem. Phys., 24, 4875–4894, https://doi.org/10.5194/acp-24-4875-2024, https://doi.org/10.5194/acp-24-4875-2024, 2024
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Four-year satellite observations of XCH4 are used to derive CH4 emissions in three regions of China’s coal-rich Shanxi province. The wind-assigned anomalies for two opposite wind directions are calculated, and the estimated emission rates are comparable to the current bottom-up inventory but lower than the CAMS and EDGAR inventories. This research enhances the understanding of emissions in Shanxi and supports climate mitigation strategies by validating emission inventories.
Paul S. Jeffery, James R. Drummond, Jiansheng Zou, and Kaley A. Walker
Atmos. Chem. Phys., 24, 4253–4263, https://doi.org/10.5194/acp-24-4253-2024, https://doi.org/10.5194/acp-24-4253-2024, 2024
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The MOPITT instrument has been monitoring carbon monoxide (CO) since March 2000. This dataset has been used for many applications; however, episodic emission events, which release large amounts of CO into the atmosphere, are a major source of uncertainty. This study presents a method for identifying these events by determining measurements that are unlikely to have typically arisen. The distribution and frequency of these flagged measurements in the MOPITT dataset are presented and discussed.
Ailish M. Graham, Richard J. Pope, Martyn P. Chipperfield, Sandip S. Dhomse, Matilda Pimlott, Wuhu Feng, Vikas Singh, Ying Chen, Oliver Wild, Ranjeet Sokhi, and Gufran Beig
Atmos. Chem. Phys., 24, 789–806, https://doi.org/10.5194/acp-24-789-2024, https://doi.org/10.5194/acp-24-789-2024, 2024
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Our paper uses novel satellite datasets and high-resolution emissions datasets alongside a back-trajectory model to investigate the balance of local and external sources influencing NOx air pollution changes in Delhi. We find in the post-monsoon season that NOx from local and non-local transport emissions contributes most to poor air quality in Delhi. Therefore, air quality mitigation strategies in Delhi and surrounding regions are used to control this issue.
Camille Viatte, Nadir Guendouz, Clarisse Dufaux, Arjan Hensen, Daan Swart, Martin Van Damme, Lieven Clarisse, Pierre Coheur, and Cathy Clerbaux
Atmos. Chem. Phys., 23, 15253–15267, https://doi.org/10.5194/acp-23-15253-2023, https://doi.org/10.5194/acp-23-15253-2023, 2023
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Ammonia (NH3) is an important air pollutant which, as a precursor of fine particulate matter, raises public health concerns. Models have difficulty predicting events of pollution associated with NH3 since ground-based observations of this gas are still relatively sparse and difficult to implement. We present the first relatively long (2.5 years) and continuous record of hourly NH3 concentrations in Paris to determine its temporal variabilities at different scales to unravel emission sources.
Hirofumi Ohyama, Matthias M. Frey, Isamu Morino, Kei Shiomi, Masahide Nishihashi, Tatsuya Miyauchi, Hiroko Yamada, Makoto Saito, Masanobu Wakasa, Thomas Blumenstock, and Frank Hase
Atmos. Chem. Phys., 23, 15097–15119, https://doi.org/10.5194/acp-23-15097-2023, https://doi.org/10.5194/acp-23-15097-2023, 2023
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We conducted a field campaign for CO2 column measurements in the Tokyo metropolitan area with three ground-based Fourier transform spectrometers. The model simulations using prior CO2 fluxes were generally in good agreement with the observations. We developed an urban-scale inversion system in which spatially resolved CO2 fluxes and a scaling factor of large point source emissions were estimated. The posterior total CO2 emissions agreed with emission inventories within the posterior uncertainty.
Xi Shao, Shu-Peng Ho, Xin Jing, Xinjia Zhou, Yong Chen, Tung-Chang Liu, Bin Zhang, and Jun Dong
Atmos. Chem. Phys., 23, 14187–14218, https://doi.org/10.5194/acp-23-14187-2023, https://doi.org/10.5194/acp-23-14187-2023, 2023
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Atmospheric water vapor plays an essential role in the global energy balance, hydrological cycle, and climate system. This paper characterizes and compares the global, latitudinal, and regional variabilities of COSMIC and ERA5 water vapor distribution, as well as the seasonality and long-term trends at selected pressure levels from 2007 to 2018. Evaluation of spatiotemporal variabilities of atmospheric water vapor ensures the qualities of COSMIC and reanalysis water vapor for climate studies.
Anthony Rey-Pommier, Frédéric Chevallier, Philippe Ciais, Jonilda Kushta, Theodoros Christoudias, I. Safak Bayram, and Jean Sciare
Atmos. Chem. Phys., 23, 13565–13583, https://doi.org/10.5194/acp-23-13565-2023, https://doi.org/10.5194/acp-23-13565-2023, 2023
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We use four years (2019–2022) of TROPOMI NO2 data to map NOx emissions in Qatar. We estimate average monthly emissions for the country and industrial facilities and derive an emission factor for the power sector. Monthly emissions have a weekly cycle reflecting the social norms in Qatar and an annual cycle consistent with the electricity production by gas-fired power plants. Their mean value is lower than the NOx emissions in global inventories but similar to the emissions reported for 2007.
Daniel A. Potts, Roger Timmis, Emma J. S. Ferranti, and Joshua D. Vande Hey
Atmos. Chem. Phys., 23, 4577–4593, https://doi.org/10.5194/acp-23-4577-2023, https://doi.org/10.5194/acp-23-4577-2023, 2023
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With the launch of the TROPOspheric Monitoring Instrument (TROPOMI) in 2017, it is now possible to observe pollutants emitted from individual industrial facilities on a daily basis around the globe. By using observations of nitrogen dioxide (NO2) from 16 different industrial sites, we show how the Coriolis effect influences the trajectory of these emission plumes as well as how the additional curvature can lead to a substantial underestimation of the calculated emissions.
Peng Yuan, Roeland Van Malderen, Xungang Yin, Hannes Vogelmann, Weiping Jiang, Joseph Awange, Bernhard Heck, and Hansjörg Kutterer
Atmos. Chem. Phys., 23, 3517–3541, https://doi.org/10.5194/acp-23-3517-2023, https://doi.org/10.5194/acp-23-3517-2023, 2023
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Water vapour plays an important role in various weather and climate processes. However, due to its large spatiotemporal variability, its high-accuracy quantification remains a challenge. In this study, 20+ years of GPS-derived integrated water vapour (IWV) retrievals in Europe were obtained. They were then used to characterise the temporal features of Europe's IWV and assess six atmospheric reanalyses. Results show that ERA5 outperforms the other reanalyses at most temporal scales.
Jing Wei, Zhanqing Li, Jun Wang, Can Li, Pawan Gupta, and Maureen Cribb
Atmos. Chem. Phys., 23, 1511–1532, https://doi.org/10.5194/acp-23-1511-2023, https://doi.org/10.5194/acp-23-1511-2023, 2023
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This study estimated the daily seamless 10 km ambient gaseous pollutants (NO2, SO2, and CO) across China using machine learning with extensive input variables measured on monitors, satellites, and models. Our dataset yields a high data quality via cross-validation at varying spatiotemporal scales and outperforms most previous related studies, making it most helpful to future (especially short-term) air pollution and environmental health-related studies.
Camille Viatte, Rimal Abeed, Shoma Yamanouchi, William C. Porter, Sarah Safieddine, Martin Van Damme, Lieven Clarisse, Beatriz Herrera, Michel Grutter, Pierre-Francois Coheur, Kimberly Strong, and Cathy Clerbaux
Atmos. Chem. Phys., 22, 12907–12922, https://doi.org/10.5194/acp-22-12907-2022, https://doi.org/10.5194/acp-22-12907-2022, 2022
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Large cities can experience high levels of fine particulate matter (PM2.5) pollution linked to ammonia (NH3) mainly emitted from agricultural activities. Using a combination of PM2.5 and NH3 measurements from in situ instruments, satellite infrared spectrometers, and atmospheric model simulations, we have demonstrated the role of NH3 and meteorological conditions on pollution events occurring over Paris, Toronto, and Mexico City.
Hossain Mohammed Syedul Hoque, Kengo Sudo, Hitoshi Irie, Alessandro Damiani, Manish Naja, and Al Mashroor Fatmi
Atmos. Chem. Phys., 22, 12559–12589, https://doi.org/10.5194/acp-22-12559-2022, https://doi.org/10.5194/acp-22-12559-2022, 2022
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Nitrogen dioxide (NO2) and formaldehyde (HCHO) are essential trace graces regulating tropospheric ozone chemistry. These trace constituents are measured using an optical passive remote sensing technique. In addition, NO2 and HCHO are simulated with a computer model and evaluated against the observations. Such evaluations are essential to assess model uncertainties and improve their predictability. The results yielded good agreement between the two datasets with some discrepancies.
Qiansi Tu, Matthias Schneider, Frank Hase, Farahnaz Khosrawi, Benjamin Ertl, Jaroslaw Necki, Darko Dubravica, Christopher J. Diekmann, Thomas Blumenstock, and Dianjun Fang
Atmos. Chem. Phys., 22, 9747–9765, https://doi.org/10.5194/acp-22-9747-2022, https://doi.org/10.5194/acp-22-9747-2022, 2022
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Three-year satellite observations and high-resolution model forecast of XCH4 are used to derive CH4 emissions in the USCB region, Poland – a region of intense coal mining activities. The wind-assigned anomalies for two opposite wind directions are calculated and the estimated emission rates are very close to the inventories and in reasonable agreement with the previous studies. Our method is quite robust and can serve as a simple method to estimate CH4 or CO2 emissions for other regions.
Pu Liu, Jia Ding, Lei Liu, Wen Xu, and Xuejun Liu
Atmos. Chem. Phys., 22, 9099–9110, https://doi.org/10.5194/acp-22-9099-2022, https://doi.org/10.5194/acp-22-9099-2022, 2022
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Ammonia (NH3) is the important alkaline gas and the key component of fine particulate matter. We used satellite-based observations to analyze the changes in hourly NH3 concentrations and estimated surface NH3 concentrations and NH3 emissions in China. This study shows enormous potential for using satellite data to estimate surface NH3 concentrations and NH3 emissions and provides an important reference for understanding NH3 variation in China.
Yohanna Villalobos, Peter J. Rayner, Jeremy D. Silver, Steven Thomas, Vanessa Haverd, Jürgen Knauer, Zoë M. Loh, Nicholas M. Deutscher, David W. T. Griffith, and David F. Pollard
Atmos. Chem. Phys., 22, 8897–8934, https://doi.org/10.5194/acp-22-8897-2022, https://doi.org/10.5194/acp-22-8897-2022, 2022
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We study the interannual variability in Australian carbon fluxes for 2015–2019 derived from OCO-2 satellite data. Our results suggest that Australia's semi-arid ecosystems are highly responsive to variations in climate drivers such as rainfall and temperature. We found that high rainfall and low temperatures recorded in 2016 led to an anomalous carbon sink over savanna and sparsely vegetated regions, while unprecedented dry and hot weather in 2019 led to anomalous carbon release.
Tianlang Zhao, Jingqiu Mao, William R. Simpson, Isabelle De Smedt, Lei Zhu, Thomas F. Hanisco, Glenn M. Wolfe, Jason M. St. Clair, Gonzalo González Abad, Caroline R. Nowlan, Barbara Barletta, Simone Meinardi, Donald R. Blake, Eric C. Apel, and Rebecca S. Hornbrook
Atmos. Chem. Phys., 22, 7163–7178, https://doi.org/10.5194/acp-22-7163-2022, https://doi.org/10.5194/acp-22-7163-2022, 2022
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Monitoring formaldehyde (HCHO) can help us understand Arctic vegetation change. Here, we compare satellite data and model and show that Alaska summertime HCHO is largely dominated by a background from methane oxidation during mild wildfire years and is dominated by wildfire (largely from direct emission of fire) during strong fire years. Consequently, it is challenging to use satellite HCHO to study vegetation change in the Arctic region.
Maria-Elissavet Koukouli, Konstantinos Michailidis, Pascal Hedelt, Isabelle A. Taylor, Antje Inness, Lieven Clarisse, Dimitris Balis, Dmitry Efremenko, Diego Loyola, Roy G. Grainger, and Christian Retscher
Atmos. Chem. Phys., 22, 5665–5683, https://doi.org/10.5194/acp-22-5665-2022, https://doi.org/10.5194/acp-22-5665-2022, 2022
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Volcanic eruptions eject large amounts of ash and trace gases into the atmosphere. The use of space-borne instruments enables the global monitoring of volcanic SO2 emissions in an economical and risk-free manner. The main aim of this paper is to present its extensive verification, accomplished within the ESA S5P+I: SO2LH project, over major recent volcanic eruptions, against collocated space-borne measurements, as well as assess its impact on the forecasts provided by CAMS.
Hao Yin, Youwen Sun, Justus Notholt, Mathias Palm, and Cheng Liu
Atmos. Chem. Phys., 22, 4167–4185, https://doi.org/10.5194/acp-22-4167-2022, https://doi.org/10.5194/acp-22-4167-2022, 2022
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In this study, we quantity the long-term variabilities and the underlying drivers of NO2 from 2005 to 2020 over the Yangtze River Delta (YRD), one of the most densely populated and highly industrialized city clusters in China. We reveal the significant effect of the Action Plan on the Prevention and Control of Air Pollution since 2013 adopted by the Chinese government to reduce NOx pollution. Our study can improve the understanding of pollution control measures on a regional scale.
Chloé Radice, Hélène Brogniez, Pierre-Emmanuel Kirstetter, and Philippe Chambon
Atmos. Chem. Phys., 22, 3811–3825, https://doi.org/10.5194/acp-22-3811-2022, https://doi.org/10.5194/acp-22-3811-2022, 2022
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A novel probabilistic approach is proposed to evaluate relative humidity (RH) profiles simulated by an atmospheric model with respect to satellite-based RH defined from probability distributions. It improves upon deterministic comparisons by enhancing the information content to enable a finer assessment of each model–observation discrepancy, highlighting significant departures within a deterministic confidence range. Geographical and vertical distributions of the model biases are discussed.
Manu Anna Thomas, Abhay Devasthale, and Tiina Nygård
Atmos. Chem. Phys., 21, 16593–16608, https://doi.org/10.5194/acp-21-16593-2021, https://doi.org/10.5194/acp-21-16593-2021, 2021
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The impact of transported pollutants and their spatial distribution in the Arctic are governed by the local atmospheric circulation or weather states. Therefore, we investigated eight different atmospheric circulation types observed during the spring season in the Arctic. Using satellite and reanalysis datasets, this study provides a comprehensive assessment of the typical circulation patterns that can lead to enhanced or reduced pollution concentrations in the different sectors of the Arctic.
Xin Tian, Yang Wang, Steffen Beirle, Pinhua Xie, Thomas Wagner, Jin Xu, Ang Li, Steffen Dörner, Bo Ren, and Xiaomei Li
Atmos. Chem. Phys., 21, 12867–12894, https://doi.org/10.5194/acp-21-12867-2021, https://doi.org/10.5194/acp-21-12867-2021, 2021
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The performances of two MAX-DOAS inversion algorithms were evaluated for various aerosol pollution scenarios. One inversion algorithm is based on optimal estimation; the other uses a parameterized approach. In this analysis, three types of profile shapes for aerosols and NO2 were considered: exponential, Boltzmann, and Gaussian. The evaluation results can effectively guide the application of the two inversion algorithms in the actual atmosphere and improve the accuracy of the actual inversion.
Rebecca D. Kutzner, Juan Cuesta, Pascale Chelin, Jean-Eudes Petit, Mokhtar Ray, Xavier Landsheere, Benoît Tournadre, Jean-Charles Dupont, Amandine Rosso, Frank Hase, Johannes Orphal, and Matthias Beekmann
Atmos. Chem. Phys., 21, 12091–12111, https://doi.org/10.5194/acp-21-12091-2021, https://doi.org/10.5194/acp-21-12091-2021, 2021
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Our work investigates the diurnal evolution of atmospheric ammonia concentrations during a major pollution event. It analyses it in regard of both chemical (gas–particle conversion) and physical (vertical mixing, meteorology) processes in the atmosphere. These mechanisms are key for understanding the evolution of the physicochemical state of the atmosphere; therefore, it clearly fits into the scope of Atmospheric Chemistry and Physics.
Youwen Sun, Hao Yin, Cheng Liu, Emmanuel Mahieu, Justus Notholt, Yao Té, Xiao Lu, Mathias Palm, Wei Wang, Changgong Shan, Qihou Hu, Min Qin, Yuan Tian, and Bo Zheng
Atmos. Chem. Phys., 21, 11759–11779, https://doi.org/10.5194/acp-21-11759-2021, https://doi.org/10.5194/acp-21-11759-2021, 2021
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The variability, sources, and transport of ethane (C2H6) over eastern China from 2015 to 2020 were studied using ground-based Fourier transform infrared (FTIR) spectroscopy and GEOS-Chem simulations. C2H6 variability is driven by both meteorological and emission factors. The reduction in C2H6 in recent years over eastern China points to air quality improvement in China.
Youwen Sun, Hao Yin, Cheng Liu, Lin Zhang, Yuan Cheng, Mathias Palm, Justus Notholt, Xiao Lu, Corinne Vigouroux, Bo Zheng, Wei Wang, Nicholas Jones, Changong Shan, Min Qin, Yuan Tian, Qihou Hu, Fanhao Meng, and Jianguo Liu
Atmos. Chem. Phys., 21, 6365–6387, https://doi.org/10.5194/acp-21-6365-2021, https://doi.org/10.5194/acp-21-6365-2021, 2021
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This study mapped the drivers of HCHO variability from 2015 to 2019 over eastern China. Hydroxyl (OH) radical production rates from HCHO photolysis were evaluated. The relative contributions of emitted and photochemical sources to the observed HCHO abundance were analyzed. Contributions of various emission sources and geographical regions to the observed HCHO summertime enhancements were determined.
Fernando Chouza, Thierry Leblanc, Mark Brewer, Patrick Wang, Sabino Piazzolla, Gabriele Pfister, Rajesh Kumar, Carl Drews, Simone Tilmes, Louisa Emmons, and Matthew Johnson
Atmos. Chem. Phys., 21, 6129–6153, https://doi.org/10.5194/acp-21-6129-2021, https://doi.org/10.5194/acp-21-6129-2021, 2021
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The tropospheric ozone lidar at the JPL Table Mountain Facility (TMF) was used to investigate the impact of Los Angeles (LA) Basin pollution transport and stratospheric intrusions in the planetary boundary layer on the San Gabriel Mountains. The results of this study indicate a dominant role of the LA Basin pollution on days when high ozone levels were observed at TMF (March–October period).
Maria-Elissavet Koukouli, Ioanna Skoulidou, Andreas Karavias, Isaak Parcharidis, Dimitris Balis, Astrid Manders, Arjo Segers, Henk Eskes, and Jos van Geffen
Atmos. Chem. Phys., 21, 1759–1774, https://doi.org/10.5194/acp-21-1759-2021, https://doi.org/10.5194/acp-21-1759-2021, 2021
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In recent years, satellite observations have contributed to monitoring air quality. During the first COVID-19 lockdown, lower levels of nitrogen dioxide were observed over Greece by S5P/TROPOMI for March and April 2020 (than the preceding year) due to decreased transport emissions. Taking meteorology into account, using LOTOS-EUROS CTM simulations, the resulting decline due to the lockdown was estimated to range between 0 % and −37 % for the five largest Greek cities, with an average of ~ −10 %.
Tobias Borsdorff, Agustín García Reynoso, Gilberto Maldonado, Bertha Mar-Morales, Wolfgang Stremme, Michel Grutter, and Jochen Landgraf
Atmos. Chem. Phys., 20, 15761–15774, https://doi.org/10.5194/acp-20-15761-2020, https://doi.org/10.5194/acp-20-15761-2020, 2020
Sören Johansson, Michael Höpfner, Oliver Kirner, Ingo Wohltmann, Silvia Bucci, Bernard Legras, Felix Friedl-Vallon, Norbert Glatthor, Erik Kretschmer, Jörn Ungermann, and Gerald Wetzel
Atmos. Chem. Phys., 20, 14695–14715, https://doi.org/10.5194/acp-20-14695-2020, https://doi.org/10.5194/acp-20-14695-2020, 2020
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We present high-resolution measurements of pollutant trace gases (PAN, C2H2, and HCOOH) in the Asian monsoon UTLS from the airborne limb imager GLORIA during StratoClim 2017. Enhancements are observed up to 16 km altitude, and PAN and C2H2 even up to 18 km. Two atmospheric models, CAMS and EMAC, reproduce the pollutant's large-scale structures but not finer structures. Convection is investigated using backward trajectories of the models ATLAS and TRACZILLA with advanced detection of convection.
Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows
Atmos. Chem. Phys., 20, 12285–12312, https://doi.org/10.5194/acp-20-12285-2020, https://doi.org/10.5194/acp-20-12285-2020, 2020
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In this study, we present spatial distributions of occurrence frequency of enhanced total BrO column and various meteorological parameters affecting it in the Arctic and Antarctic sea ice regions by using 10 years of GOME-2 measurements and meteorological model data. Statistical analysis using the long-term dataset shows clear differences in the meteorological conditions between the mean field and the situation of enhanced total BrO columns in both polar sea ice regions.
Leonie Bernet, Elmar Brockmann, Thomas von Clarmann, Niklaus Kämpfer, Emmanuel Mahieu, Christian Mätzler, Gunter Stober, and Klemens Hocke
Atmos. Chem. Phys., 20, 11223–11244, https://doi.org/10.5194/acp-20-11223-2020, https://doi.org/10.5194/acp-20-11223-2020, 2020
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With global warming, water vapour increases in the atmosphere. Water vapour is an important gas because it is a natural greenhouse gas and affects the formation of clouds, rain and snow. How much water vapour increases can vary in different regions of the world. To verify if it increases as expected on a regional scale, we analysed water vapour measurements in Switzerland. We found that water vapour generally increases as expected from temperature changes, except in winter.
Shannon Hicks-Jalali, Robert J. Sica, Giovanni Martucci, Eliane Maillard Barras, Jordan Voirin, and Alexander Haefele
Atmos. Chem. Phys., 20, 9619–9640, https://doi.org/10.5194/acp-20-9619-2020, https://doi.org/10.5194/acp-20-9619-2020, 2020
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We have calculated an 11.5-year water vapour climatology using the Raman Lidar for Meteorological Observations (RALMO), located in Payerne, Switzerland. The climatology shows that the highest water vapour concentrations are in the summer months and the lowest in the winter months. We present for the first time height-resolved water vapour trends, which show that water vapour increases specific humidity by between 5 % and 15 % per decade depending on the altitude.
Yohanna Villalobos, Peter Rayner, Steven Thomas, and Jeremy Silver
Atmos. Chem. Phys., 20, 8473–8500, https://doi.org/10.5194/acp-20-8473-2020, https://doi.org/10.5194/acp-20-8473-2020, 2020
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Estimated carbon fluxes for Australia are subject to considerable uncertainty. We ran simulation experiments over Australia to determine how much these uncertainties can be constrained using satellite data. We found that the satellite data has the potential to reduce these uncertainties up to 80 % across the whole continent. For 1 month, this percentage corresponds to 0.51 Pg C y-1 for Australia. This method could lead to significantly more accurate estimates of Australia's carbon budget.
Bo Zheng, Frédéric Chevallier, Philippe Ciais, Grégoire Broquet, Yilong Wang, Jinghui Lian, and Yuanhong Zhao
Atmos. Chem. Phys., 20, 8501–8510, https://doi.org/10.5194/acp-20-8501-2020, https://doi.org/10.5194/acp-20-8501-2020, 2020
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The Paris Climate Agreement requires all parties to report CO2 emissions regularly. Given the self-reporting nature of this system, it is critical to evaluate the emission reports with independent observation systems. Here we present the direct observations of city CO2 plumes from space and the quantification of CO2 emissions from these observations over the largest emitter country China. The emissions from 46 hot-spot regions representing 13 % of China's total emissions can be well constrained.
Jeffery Langille, Adam Bourassa, Laura L. Pan, Daniel Letros, Brian Solheim, Daniel Zawada, and Doug Degenstein
Atmos. Chem. Phys., 20, 5477–5486, https://doi.org/10.5194/acp-20-5477-2020, https://doi.org/10.5194/acp-20-5477-2020, 2020
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Water vapour (WV) is a highly variable and extremely important trace gas in Earth’s atmosphere. Due to its radiative and chemical properties, it is coupled to the climate in an extremely complex manner. This is especially true in the lowermost stratosphere (LMS). Despite its importance, the physical processes that control mixing and the distribution of WV in the LMS are poorly understood. This study provides observational evidence of moistening the LMS via mixing across the subtropical jet.
Youwen Sun, Cheng Liu, Lin Zhang, Mathias Palm, Justus Notholt, Hao Yin, Corinne Vigouroux, Erik Lutsch, Wei Wang, Changong Shan, Thomas Blumenstock, Tomoo Nagahama, Isamu Morino, Emmanuel Mahieu, Kimberly Strong, Bavo Langerock, Martine De Mazière, Qihou Hu, Huifang Zhang, Christof Petri, and Jianguo Liu
Atmos. Chem. Phys., 20, 5437–5456, https://doi.org/10.5194/acp-20-5437-2020, https://doi.org/10.5194/acp-20-5437-2020, 2020
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We present multiyear time series of ground-based Fourier-transform infrared spectroscopy measurements of HCN in densely populated eastern China. The seasonality and interannual variability of tropospheric HCN columns were investigated. The potential sources that drive the observed HCN seasonality and interannual variability were determined using a GEOS-Chem tagged CO simulation, global fire maps, and potential source contribution function values calculated using HYSPLIT back trajectories.
Enrico Dammers, Chris A. McLinden, Debora Griffin, Mark W. Shephard, Shelley Van Der Graaf, Erik Lutsch, Martijn Schaap, Yonatan Gainairu-Matz, Vitali Fioletov, Martin Van Damme, Simon Whitburn, Lieven Clarisse, Karen Cady-Pereira, Cathy Clerbaux, Pierre Francois Coheur, and Jan Willem Erisman
Atmos. Chem. Phys., 19, 12261–12293, https://doi.org/10.5194/acp-19-12261-2019, https://doi.org/10.5194/acp-19-12261-2019, 2019
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Ammonia is an essential molecule in the environment, but at its current levels it is unsustainable. However, the emissions are highly uncertain. We explore the use of satellites to estimate the ammonia lifetime and emissions around point sources to help improve the budget. The same method applied to different satellite instruments shows consistent results. Comparison to the emission inventories shows that those are underestimating emissions of point sources by on average a factor of 2.5.
Klemens Hocke, Leonie Bernet, Jonas Hagen, Axel Murk, Matthias Renker, and Christian Mätzler
Atmos. Chem. Phys., 19, 12083–12090, https://doi.org/10.5194/acp-19-12083-2019, https://doi.org/10.5194/acp-19-12083-2019, 2019
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The Tropospheric Water Radiometer (TROWARA) observed an enhanced intensity of short-term integrated water vapour (IWV) fluctuations during daytime in summer. These IWV fluctuations are possibly related to latent heat flux and thermal convective activity in the lower troposphere. The observed climatology and spectra of IWV fluctuations might be useful for modelling studies of water vapour convection in the atmospheric boundary layer at mid latitudes.
Xiaoyi Zhao, Debora Griffin, Vitali Fioletov, Chris McLinden, Jonathan Davies, Akira Ogyu, Sum Chi Lee, Alexandru Lupu, Michael D. Moran, Alexander Cede, Martin Tiefengraber, and Moritz Müller
Atmos. Chem. Phys., 19, 10619–10642, https://doi.org/10.5194/acp-19-10619-2019, https://doi.org/10.5194/acp-19-10619-2019, 2019
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New nitrogen dioxide (NO2) retrieval algorithms are developed for Pandora zenith-sky measurements. A column-to-surface conversion look-up table was produced for the Pandora instruments; therefore, quick and practical Pandora-based surface NO2 concentration data can be obtained for air quality monitoring purposes. It is demonstrated that the surface NO2 concentration is controlled not only by the planetary boundary layer height but also by both boundary layer dynamics and photochemistry.
Ka Lok Chan, Zhuoru Wang, Aijun Ding, Klaus-Peter Heue, Yicheng Shen, Jing Wang, Feng Zhang, Yining Shi, Nan Hao, and Mark Wenig
Atmos. Chem. Phys., 19, 10051–10071, https://doi.org/10.5194/acp-19-10051-2019, https://doi.org/10.5194/acp-19-10051-2019, 2019
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The paper presents long-term observations of atmospheric nitrogen dioxide (NO2) and formaldehyde (HCHO) in Nanjing using a MAX-DOAS instrument. The measurements were performed from April 2013 to February 2017. The MAX-DOAS measurements of NO2 and HCHO are used to validate OMI satellite observations and to investigate the influences of region transport of air pollutants on the air quality in Nanjing.
Olivier Bock and Ana C. Parracho
Atmos. Chem. Phys., 19, 9453–9468, https://doi.org/10.5194/acp-19-9453-2019, https://doi.org/10.5194/acp-19-9453-2019, 2019
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We examine the consistency of global IWV data from ERA-Interim reanalysis and 16 years of GPS observations. Representativeness differences are found to be a dominant error source, with a strong dependence on geographic, topographic, and climatic features, which explain both average and extreme differences. A methodology for reducing the representativeness errors and detecting the extreme, outlying, cases is discussed.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Sven Krautwurst, Christopher W. O'Dell, Andreas Richter, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 19, 9371–9383, https://doi.org/10.5194/acp-19-9371-2019, https://doi.org/10.5194/acp-19-9371-2019, 2019
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The quantification of anthropogenic emissions with current CO2 satellite sensors is difficult, but NO2 is co-emitted, making it a suitable tracer of recently emitted CO2. We analyze enhancements of CO2 and NO2 observed by OCO-2 and S5P and estimate the CO2 plume cross-sectional fluxes that we compare with emission databases. Our results demonstrate the usefulness of simultaneous satellite observations of CO2 and NO2 as envisaged for the European Copernicus anthropogenic CO2 monitoring mission
Luis F. Millán, Matthew D. Lebsock, and Joao Teixeira
Atmos. Chem. Phys., 19, 8491–8502, https://doi.org/10.5194/acp-19-8491-2019, https://doi.org/10.5194/acp-19-8491-2019, 2019
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The synergy of the collocated Advanced Microwave Scanning Radiometer (AMSR) and the Moderate Resolution Imaging Spectroradiometer (MODIS) provides daily global estimates of marine boundary layer water vapor. AMSR provides the total column water vapor, while MODIS provides the water vapor above the cloud layers. The difference between the two gives the vapor between the surface and the cloud top, which may be interpreted as the boundary layer water vapor.
Aristeidis K. Georgoulias, Ronald J. van der A, Piet Stammes, K. Folkert Boersma, and Henk J. Eskes
Atmos. Chem. Phys., 19, 6269–6294, https://doi.org/10.5194/acp-19-6269-2019, https://doi.org/10.5194/acp-19-6269-2019, 2019
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In this paper, a ∼21-year self-consistent global dataset from four different satellite sensors is compiled for the first time to study the long-term tropospheric NO2 patterns and trends. A novel method capable of detecting the year when a reversal of trends happened shows that tropospheric NO2 concentrations switched from positive to negative trends and vice versa over several regions around the globe during the last 2 decades.
Elisa Carboni, Tamsin A. Mather, Anja Schmidt, Roy G. Grainger, Melissa A. Pfeffer, Iolanda Ialongo, and Nicolas Theys
Atmos. Chem. Phys., 19, 4851–4862, https://doi.org/10.5194/acp-19-4851-2019, https://doi.org/10.5194/acp-19-4851-2019, 2019
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The 2014–2015 Holuhraun eruption was the largest in Iceland for 200 years, emitting huge quantities of gas into the troposphere, at times overwhelming European anthropogenic emissions. Infrared Atmospheric sounding Interferometer data are used to derive the first time series of daily sulfur dioxide mass and vertical distribution over the eruption period. A scheme is used to estimate sulfur dioxide fluxes, the total erupted mass, and how long the sulfur dioxide remains in the atmosphere.
Debra Wunch, Dylan B. A. Jones, Geoffrey C. Toon, Nicholas M. Deutscher, Frank Hase, Justus Notholt, Ralf Sussmann, Thorsten Warneke, Jeroen Kuenen, Hugo Denier van der Gon, Jenny A. Fisher, and Joannes D. Maasakkers
Atmos. Chem. Phys., 19, 3963–3980, https://doi.org/10.5194/acp-19-3963-2019, https://doi.org/10.5194/acp-19-3963-2019, 2019
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We used five atmospheric observatories in Europe measuring total column dry-air mole fractions of methane and carbon monoxide to infer methane emissions in the area between the observatories. We find that the methane emissions are overestimated by the state-of-the-art inventories, and that this is likely due, at least in part, to the inventory disaggregation. We find that there is significant uncertainty in the carbon monoxide inventories that requires further investigation.
Klaus Gierens and Kostas Eleftheratos
Atmos. Chem. Phys., 19, 3733–3746, https://doi.org/10.5194/acp-19-3733-2019, https://doi.org/10.5194/acp-19-3733-2019, 2019
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We derive a new method to retrieve upper-tropospheric humidity (UTH) from High-resolution Infrared Radiation Sounder (HIRS) channel 12 brightness temperatures. With the new method we solve an old problem, namely that the wavelength change that occurred between HIRS 2 on NOAA 14 and HIRS 3 on NOAA 15 led to the retrieval of many more events with high UTH; that is, the time series shows strong jumps at high UTH values. This old problem is solved with the new retrieval.
Tobias Borsdorff, Joost aan de Brugh, Sudhanshu Pandey, Otto Hasekamp, Ilse Aben, Sander Houweling, and Jochen Landgraf
Atmos. Chem. Phys., 19, 3579–3588, https://doi.org/10.5194/acp-19-3579-2019, https://doi.org/10.5194/acp-19-3579-2019, 2019
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The Tropospheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor satellite provides carbon monoxide (CO) total column concentrations based on measurements in the 2.3 μm spectral range with a spatial resolution of 7 km x 7 km and daily global coverage. In this study, we analyzed local CO enhancements in an area around Iran from 1 November to 20 December 2017 using the WRF model and evaluated CO emissions from the cities of Tehran, Yerevan, Urmia, and Tabriz.
Xin Tian, Pinhua Xie, Jin Xu, Yang Wang, Ang Li, Fengcheng Wu, Zhaokun Hu, Cheng Liu, and Qiong Zhang
Atmos. Chem. Phys., 19, 3375–3393, https://doi.org/10.5194/acp-19-3375-2019, https://doi.org/10.5194/acp-19-3375-2019, 2019
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We used the MAX-DOAS instrument installed at the UCAS, Beijing, to evaluate effects on HCHO. The daily variation, transport, sources, and the effect of APEC emission control measures on HCHO were analyzed. Dependences of HCHO VCDs on wind fields indicated that the HCHO values were affected by the transport of pollutants from the south. The results from comparing the MAX-DOAS with the CAMS model indicate the CAMS model can simulate the effects of transport and the secondary sources of HCHO well.
Jerry R. Ziemke, Luke D. Oman, Sarah A. Strode, Anne R. Douglass, Mark A. Olsen, Richard D. McPeters, Pawan K. Bhartia, Lucien Froidevaux, Gordon J. Labow, Jacquie C. Witte, Anne M. Thompson, David P. Haffner, Natalya A. Kramarova, Stacey M. Frith, Liang-Kang Huang, Glen R. Jaross, Colin J. Seftor, Mathew T. Deland, and Steven L. Taylor
Atmos. Chem. Phys., 19, 3257–3269, https://doi.org/10.5194/acp-19-3257-2019, https://doi.org/10.5194/acp-19-3257-2019, 2019
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Both a 38-year merged satellite record of tropospheric ozone from TOMS/OMI/MLS/OMPS and a MERRA-2 GMI model simulation show large increases of 6–7 Dobson units from the Near East to India–East Asia and eastward over the Pacific. These increases in tropospheric ozone are attributed to increases in pollution over the region over the last several decades. Secondary 38-year increases of 4–5 Dobson units with both GMI model and satellite measurements occur over central African–tropical Atlantic.
Cited articles
Baker, D. F., Bösch, H., Doney, S. C., O'Brien, D., and Schimel, D. S.:
Carbon source/sink information provided by column CO2 measurements from
the Orbiting Carbon Observatory, Atmos. Chem. Phys., 10, 4145–4165,
https://doi.org/10.5194/acp-10-4145-2010, 2010. a, b, c
Basu, S., Guerlet, S., Butz, A., Houweling, S., Hasekamp, O., Aben, I.,
Krummel, P., Steele, P., Langenfelds, R., Torn, M., Biraud, S., Stephens, B.,
Andrews, A., and Worthy, D.: Global CO2 fluxes estimated from GOSAT
retrievals of total column CO2, Atmos. Chem. Phys., 13, 8695–8717,
https://doi.org/10.5194/acp-13-8695-2013, 2013. a
Basu, S., Krol, M., Butz, A., Clerbaux, C., Sawa, Y., Machida, T., Matsueda,
H., Frankenberg, C., Hasekamp, O. P., and Aben, I.: The seasonal variation of
the CO2 flux over Tropical Asia estimated from GOSAT, CONTRAIL, and IASI,
Geophys. Res. Lett., 41, 1809–1815, https://doi.org/10.1002/2013GL059105, 2014. a
Chatterjee, A., Gierach, M. M., Sutton, A. J., Feely, R. A., Crisp, D.,
Eldering, A., Gunson, M. R., O'Dell, C. W., Stephens, B. B.,
and Schimel, D. S.: Influence of El Niño on atmospheric CO2 over the
tropical Pacific Ocean: Findings from NASA's OCO-2 mission,
Science, 358, eaam5776, https://doi.org/10.1126/science.aam5776, 2017. a
Chevallier, F., Bron, F.-M., and Rayner, P. J.: Contribution of the Orbiting
Carbon Observatory to the estimation of CO2 sources and sinks: Theoretical
study in a variational data assimilation framework, J. Geophys. Res.-Atmos., 112, d09307, https://doi.org/10.1029/2006JD007375, 2007. a, b
Crisp, D., Atlas, R., Breon, F.-M., Brown, L., Burrows, J., Ciais, P., Connor,
B., Doney, S., Fung, I., Jacob, D., Miller, C., O'Brien, D., Pawson, S.,
Randerson, J., Rayner, P., Salawitch, R., Sander, S., Sen, B., Stephens, G.,
Tans, P., Toon, G., Wennberg, P., Wofsy, S., Yung, Y., Kuang, Z., Chudasama,
B., Sprague, G., Weiss, B., Pollock, R., Kenyon, D., and Schroll, S.: The
Orbiting Carbon Observatory (OCO) mission, Adv. Space Res., 34, 700–709,
https://doi.org/10.1016/j.asr.2003.08.062, 2004. a
Crisp, D., Pollock, H. R., Rosenberg, R., Chapsky, L., Lee, R. A. M.,
Oyafuso, F. A., Frankenberg, C., O'Dell, C. W., Bruegge, C. J., Doran, G. B.,
Eldering, A., Fisher, B. M., Fu, D., Gunson, M. R., Mandrake, L., Osterman,
G. B., Schwandner, F. M., Sun, K., Taylor, T. E., Wennberg, P. O., and Wunch,
D.: The on-orbit performance of the Orbiting Carbon Observatory-2 (OCO-2)
instrument and its radiometrically calibrated products, Atmos. Meas. Tech.,
10, 59–81, https://doi.org/10.5194/amt-10-59-2017, 2017. a
Crowell, S: The OCO-2 Level 4 Flux Product, Poster presented at the OCO-2
Science Team Meeting, Boulder, Colorado, 2017. a
Deng, F., Jones, D. B. A., Henze, D. K., Bousserez, N., Bowman, K. W.,
Fisher, J. B., Nassar, R., O'Dell, C., Wunch, D., Wennberg, P. O., Kort, E.
A., Wofsy, S. C., Blumenstock, T., Deutscher, N. M., Griffith, D. W. T.,
Hase, F., Heikkinen, P., Sherlock, V., Strong, K., Sussmann, R., and Warneke,
T.: Inferring regional sources and sinks of atmospheric CO2 from GOSAT
XCO2
data, Atmos. Chem. Phys., 14, 3703–3727,
https://doi.org/10.5194/acp-14-3703-2014, 2014. a
Eldering, A., Boland, S., Solish, B., Crisp, D., Kahn, P., and Gunson, M.: High
precision atmospheric CO2 measurements from space: The design and
implementation of OCO-2, in: 2012 IEEE Aerospace Conference, 1–10,
https://doi.org/10.1109/AERO.2012.6187176, 2012. a
Eldering, A., O'Dell, C. W., Wennberg, P. O., Crisp, D., Gunson, M. R.,
Viatte, C., Avis, C., Braverman, A., Castano, R., Chang, A., Chapsky, L.,
Cheng, C., Connor, B., Dang, L., Doran, G., Fisher, B., Frankenberg, C., Fu,
D., Granat, R., Hobbs, J., Lee, R. A. M., Mandrake, L., McDuffie, J., Miller,
C. E., Myers, V., Natraj, V., O'Brien, D., Osterman, G. B., Oyafuso, F.,
Payne, V. H., Pollock, H. R., Polonsky, I., Roehl, C. M., Rosenberg, R.,
Schwandner, F., Smyth, M., Tang, V., Taylor, T. E., To, C., Wunch, D., and
Yoshimizu, J.: The Orbiting Carbon Observatory-2: first 18 months of science
data products, Atmos. Meas. Tech., 10, 549–563,
https://doi.org/10.5194/amt-10-549-2017, 2017a. a, b
Eldering, A., Wennberg, P. O., Crisp, D., Schimel, D. S., Gunson, M. R.,
Chatterjee, A., Liu, J., Schwandner, F. M., Sun, Y., O'Dell,
C. W., Frankenberg, C., Taylor, T., Fisher, B., Osterman, G. B., Wunch, D.,
Hakkarainen, J., Tamminen, J., and Weir, B.: The Orbiting Carbon
Observatory-2 early science investigations of regional carbon dioxide fluxes,
Science, 358, eaam5745, https://doi.org/10.1126/science.aam5745, 2017b. a
European Commission, Joint Research Centre (JRC)/Netherlands Environmental
Assessment Agency (PBL): Emission Database for Global Atmospheric Research
(EDGAR), release EDGARv4.2 FT2010,
available at: http://edgar.jrc.ec.europa.eu (last access: 27 April 2018), 2013. a
Fang, Y. and Michalak, A. M.: Atmospheric observations inform CO2 flux
responses to enviroclimatic drivers, Global Biogeochem. Cy., 29, 555–566,
https://doi.org/10.1002/2014GB005034, 2015. a
Fang, Y., Michalak, A. M., Shiga, Y. P., and Yadav, V.: Using atmospheric
observations to evaluate the spatiotemporal variability of CO2 fluxes
simulated by terrestrial biospheric models, Biogeosciences, 11, 6985–6997,
https://doi.org/10.5194/bg-11-6985-2014, 2014. a, b, c, d
Fisher, J. B., Sikka, M., Huntzinger, D. N., Schwalm, C., and Liu, J.:
Technical note: 3-hourly temporal downscaling of monthly global terrestrial
biosphere model net ecosystem exchange, Biogeosciences, 13, 4271–4277,
https://doi.org/10.5194/bg-13-4271-2016, 2016. a
Fisher, J. B., Sikka, M., Huntzinger, D. N., Schwalm, C. R., Liu, J., Wei,
Y., Cook, R. B., Michalak, A. M., Schaefer, K., Jacobson, A. R., Arain, M.
A., Ciais, P., El-Masri, B., Hayes, D. J., Huang, M., Huang, S., Ito, A.,
Jain, A. K., Lei, H., Lu, C., Maignan, F., Mao, J., Parazoo, N. C., Peng, C.,
Peng, S., Poulter, B., Ricciuto, D. M., Tian, H., Shi, X., Wang, W., Zeng,
N., Zhao F., and Zhu, Q.: CMS: Modeled Net Ecosystem Exchange at 3-hourly
Time Steps, 2004–2010, ORNL Distributed Active Archive Center, available at:
https://doi.org/10.3334/ornldaac/1315 (last access: 27 April 2018), 2016. a
Giglio, L., Randerson, J. T., and van der Werf, G. R.: Analysis of daily,
monthly, and annual burned area using the fourth-generation global fire
emissions database (GFED4), J. Geophys. Res.-Biogeo., 118, 317–328,
https://doi.org/10.1002/jgrg.20042, 2013. a
Gourdji, S. M., Mueller, K. L., Schaefer, K., and Michalak, A. M.: Global
monthly averaged CO2 fluxes recovered using a geostatistical inverse
modeling approach: 2. Results including auxiliary environmental data, J.
Geophys. Res.-Atmos., 113, d21115, https://doi.org/10.1029/2007JD009733, 2008. a, b, c
Gourdji, S. M., Mueller, K. L., Yadav, V., Huntzinger, D. N., Andrews, A. E.,
Trudeau, M., Petron, G., Nehrkorn, T., Eluszkiewicz, J., Henderson, J., Wen,
D., Lin, J., Fischer, M., Sweeney, C., and Michalak, A. M.: North American
CO2 exchange: inter-comparison of modeled estimates with results from a
fine-scale atmospheric inversion, Biogeosciences, 9, 457–475,
https://doi.org/10.5194/bg-9-457-2012, 2012. a, b, c
Guerlet, S., Basu, S., Butz, A., Krol, M., Hahne, P., Houweling, S., Hasekamp,
O. P., and Aben, I.: Reduced carbon uptake during the 2010 Northern
Hemisphere summer from GOSAT, Geophys. Res. Lett., 40, 2378–2383,
https://doi.org/10.1002/grl.50402, 2013. a
Gurney, K. R., Law, R. M., Denning, A. S., Rayner, P. J. et al.: Towards
robust
regional estimates of CO2 sources and sinks using atmospheric transport
models, Nature, 415, 626–630, https://doi.org/10.1038/415626a, 2002. a
Gurney, K. R., Mendoza, D. L., Zhou, Y., Fischer, M. L., Miller, C. C.,
Geethakumar, S., and de la Rue du Can, S.: High resolution fossil fuel combustion CO2 emission fluxes for the United States, Environ. Sci. Technol.,
43, 5535–5541, https://doi.org/10.1021/es900806c, 2009. a
Hammerling, D. M., Kawa, S. R., Schaefer, K., Doney, S., and Michalak, A. M.:
Detectability of CO2 flux signals by a space-based lidar mission, J.
Geophys. Res.-Atmos., 120, 1794–1807, https://doi.org/10.1002/2014JD022483, 2015. a, b
Heymann, J., Reuter, M., Buchwitz, M., Schneising, O., Bovensmann, H., Burrows,
J. P., Massart, S., Kaiser, J. W., and Crisp, D.: CO2 emission of
Indonesian fires in 2015 estimated from satellite-derived atmospheric CO2
concentrations, Geophys. Res. Lett., 44, 1537–1544,
https://doi.org/10.1002/2016GL072042, 2017. a
Houweling, S., Baker, D., Basu, S., Boesch, H., Butz, A., Chevallier, F., Deng,
F., Dlugokencky, E. J., Feng, L., Ganshin, A., Hasekamp, O., Jones, D.,
Maksyutov, S., Marshall, J., Oda, T., O'Dell, C. W., Oshchepkov, S., Palmer,
P. I., Peylin, P., Poussi, Z., Reum, F., Takagi, H., Yoshida, Y., and
Zhuravlev, R.: An intercomparison of inverse models for estimating sources
and sinks of CO2 using GOSAT measurements, J. Geophys. Res.-Atmos.,
120, 5253–5266, https://doi.org/10.1002/2014JD022962, 2015. a, b, c
Huete, A., Didan, K., Miura, T., Rodriguez, E., Gao, X., and Ferreira, L.:
Overview of the radiometric and biophysical performance of the MODIS
vegetation indices, Remote Sens. Environ., 83, 195–213,
https://doi.org/10.1016/S0034-4257(02)00096-2, 2002. a
Huntzinger, D. N., Schwalm, C., Michalak, A. M., Schaefer, K., King, A. W.,
Wei, Y., Jacobson, A., Liu, S., Cook, R. B., Post, W. M., Berthier, G.,
Hayes, D., Huang, M., Ito, A., Lei, H., Lu, C., Mao, J., Peng, C. H., Peng,
S., Poulter, B., Riccuito, D., Shi, X., Tian, H., Wang, W., Zeng, N., Zhao,
F., and Zhu, Q.: The North American Carbon Program Multi-Scale Synthesis and
Terrestrial Model Intercomparison Project – Part 1: Overview and
experimental design, Geosci. Model Dev., 6, 2121–2133,
https://doi.org/10.5194/gmd-6-2121-2013, 2013. a, b
Japan Aerospace Exploration Agency: GOSAT-2: Greenhouse gas Observing
SATellite-2, available at:
http://global.jaxa.jp/activity/pr/brochure/files/sat38.pdf, last
access: 10 July 2017. a
Joiner, J., Guanter, L., Lindstrot, R., Voigt, M., Vasilkov, A. P.,
Middleton, E. M., Huemmrich, K. F., Yoshida, Y., and Frankenberg, C.: Global
monitoring of terrestrial chlorophyll fluorescence from
moderate-spectral-resolution near-infrared satellite measurements:
methodology, simulations, and application to GOME-2, Atmos. Meas. Tech., 6,
2803–2823, https://doi.org/10.5194/amt-6-2803-2013, 2013. a
Kawa, S. R., Erickson, D. J., Pawson, S., and Zhu, Z.: Global CO2 transport
simulations using meteorological data from the NASA data assimilation system,
J. Geophys. Res.-Atmos., 109, d18312, https://doi.org/10.1029/2004JD004554, 2004. a
Law, R. M., Peters, W., Rödenbeck, C., Aulagnier, C., Baker, I., Bergmann,
D. J., Bousquet, P., Brandt, J., Bruhwiler, L., Cameron-Smith, P. J.,
Christensen, J. H., Delage, F., Denning, A. S., Fan, S., Geels, C.,
Houweling, S., Imasu, R., Karstens, U., Kawa, S. R., Kleist, J., Krol, M. C.,
Lin, S.-J., Lokupitiya, R., Maki, T., Maksyutov, S., Niwa, Y., Onishi, R.,
Parazoo, N., Patra, P. K., Pieterse, G., Rivier, L., Satoh, M., Serrar, S.,
Taguchi, S., Takigawa, M., Vautard, R., Vermeulen, A. T., and Zhu, Z.:
TransCom model simulations of hourly atmospheric CO2: Experimental
overview and diurnal cycle results for 2002, Global Biogeochem. Cy., 22, gB3009, https://doi.org/10.1029/2007GB003050, 2008. a
Liu, J., Fung, I., Kalnay, E., and Kang, J.-S.: CO2 transport uncertainties
from the uncertainties in meteorological fields, Geophys. Res. Lett., 38, l12808,
https://doi.org/10.1029/2011GL047213, 2011. a, b, c
Liu, J., Bowman, K. W., Lee, M., Henze, D. K., Bousserez, N., Brix, H.,
Collatz, G. J., Menemenlis, D., Ott, L., Pawson, S., Jones, D., and Nassar,
R.: Carbon monitoring system flux estimation and attribution: impact of
ACOS-GOSAT XCO2 sampling on the inference of terrestrial biospheric
sources and sinks, Tellus B, 66, 22486,
https://doi.org/10.3402/tellusb.v66.22486, 2014.
Liu, J., Bowman, K. W., Schimel, D. S., Parazoo, N. C., Jiang, Z., Lee, M.,
Bloom, A. A., Wunch, D., Frankenberg, C., Sun, Y., O'Dell,
C. W., Gurney, K. R., Menemenlis, D., Gierach, M., Crisp, D., and Eldering,
A.: Contrasting carbon cycle responses of the tropical continents to the
2015–2016 El Niño, Science, 358, eaam5690,
https://doi.org/10.1126/science.aam5690, 2017. a, b
Maksyutov, S., Takagi, H., Valsala, V. K., Saito, M., Oda, T., Saeki, T.,
Belikov, D. A., Saito, R., Ito, A., Yoshida, Y., Morino, I., Uchino, O.,
Andres, R. J., and Yokota, T.: Regional CO2 flux estimates for 2009–2010
based on GOSAT and ground-based CO2 observations, Atmos. Chem. Phys., 13,
9351–9373, https://doi.org/10.5194/acp-13-9351-2013, 2013. a
Miller, S. M., Hayek, M. N., Andrews, A. E., Fung, I., and Liu, J.: Biases in
atmospheric CO2 estimates from correlated meteorology modeling errors,
Atmos. Chem. Phys., 15, 2903–2914, https://doi.org/10.5194/acp-15-2903-2015,
2015. a, b
NASA Jet Propulsion Laboratory: Orbiting Carbon Observatory 3,
available at: http://www.jpl.nasa.gov/missions/orbiting-carbon-observatory-3-oco-3/, last access: 30 August 2017. a
Nassar, R., Hill, T. G., McLinden, C. A., Wunch, D., Jones, D. B. A., and
Crisp, D.: Quantifying CO2 Emissions From Individual Power Plants From
Space, Geophys. Res. Lett., 44, 10045–10053,
https://doi.org/10.1002/2017GL074702, 2017. a
NOAA Global Monitoring Division: Global Greenhouse Gas Reference Network,
available at: https://www.esrl.noaa.gov/gmd/ccgg/ggrn.php, last access:
24 August 2017. a
Olivier, J., Janssens-Maenhout, G., Munteam, M., and Peters, J.: Trends in
global CO2 emissions; 2014 Report, PBL Netherlands Environmental
Assessment Agency; European Commission, Joint Research Centre, Ispra, Italy, available at: http://edgar.jrc.ec.europa.eu/news_docs/jrc-2014-trends-in-global-co2-emissions-2014-report-93171.pdf (last access: 30 August 2017),
2014. a
Olsen, S. C. and Randerson, J. T.: Differences between surface and column
atmospheric CO2 and implications for carbon cycle research, J. Geophys. Res.-Atmos., 109, d02301, https://doi.org/10.1029/2003JD003968,
2004. a, b
Olson, D. M., Dinerstein, E., Wikramanayake, E. D., Burgess, N. D., Powell, G.
V. N., Underwood, E. C., D'amico, J. A., Itoua, I., Strand, H. E., Morrison,
J. C., Loucks, C. J., Allnutt, T. F., Ricketts, T. H., Kura, Y., Lamoreux,
J. F., Wettengel, W. W., Hedao, P., and Kassem, K. R.: Terrestrial ecoregions of the world: A new map of life on Earth, BioScience, 51, 933–938,
https://doi.org/10.1641/0006-3568(2001)051[0933:TEOTWA]2.0.CO;2,
2001. a
Parazoo, N. C., Bowman, K., Frankenberg, C., Lee, J.-E., Fisher, J. B., Worden,
J., Jones, D. B. A., Berry, J., Collatz, G. J., Baker, I. T., Jung, M., Liu,
J., Osterman, G., O'Dell, C., Sparks, A., Butz, A., Guerlet, S., Yoshida, Y.,
Chen, H., and Gerbig, C.: Interpreting seasonal changes in the carbon balance
of southern Amazonia using measurements of XCO2 and chlorophyll fluorescence
from GOSAT, Geophys. Res. Lett., 40, 2829–2833, https://doi.org/10.1002/grl.50452,
2013. a, b
Patra, P. K., Crisp, D., Kaiser, J. W., Wunch, D., Saeki, T., Ichii, K.,
Sekiya, T., Wennberg, P. O., Feist, D. G., Pollard, D. F., Griffith, D.
W. T., Velazco, V. A., De Maziere, M., Sha, M. K., Roehl, C., Chatterjee, A.,
and Ishijima, K.: The Orbiting Carbon Observatory (OCO-2) tracks 2–3
peta-gram increase in carbon release to the atmosphere during the 2014–2016
El Niño, Sci. Rep.-UK, 7, 13567,
https://doi.org/10.1038/s41598-017-13459-0, 2017. a
Peylin, P., Law, R. M., Gurney, K. R., Chevallier, F., Jacobson, A. R., Maki,
T., Niwa, Y., Patra, P. K., Peters, W., Rayner, P. J., Rödenbeck, C., van
der Laan-Luijkx, I. T., and Zhang, X.: Global atmospheric carbon budget:
results from an ensemble of atmospheric CO2 inversions, Biogeosciences,
10, 6699–6720, https://doi.org/10.5194/bg-10-6699-2013, 2013. a
Ramsey, F. and Schafer, D.: The Statistical Sleuth: A Course in Methods of Data
Analysis, Cengage Learning, Boston, MA, 2012. a
Rayner, P. J. and O'Brien, D. M.: The utility of remotely sensed CO2
concentration data in surface source inversions, Geophys. Res.
Lett., 28, 175–178,
https://doi.org/10.1029/2000GL011912, 2001. a
Rienecker, M. M., Suarez, M. J., Gelaro, R., Todling, R., Bacmeister, J., Liu,
E., Bosilovich, M. G., Schubert, S. D., Takacs, L., Kim, G.-K., Bloom, S.,
Chen, J., Collins, D., Conaty, A., da Silva, A., Gu, W., Joiner, J., Koster,
R. D., Lucchesi, R., Molod, A., Owens, T., Pawson, S., Pegion, P., Redder,
C. R., Reichle, R., Robertson, F. R., Ruddick, A. G., Sienkiewicz, M., and
Woollen, J.: MERRA: NASA's Modern-Era Retrospective Analysis for Research and
Applications, J. Climate, 24, 3624–3648, https://doi.org/10.1175/JCLI-D-11-00015.1,
2011. a
Saeki, T., Maksyutov, S., Saito, M., Valsala, V., Oda, T., Andres, R. J.,
Belikov, D., Tans, P., Dlugokencky, E., Yoshida, Y., Morino, I., Uchino, O.,
and Yokota, T.: Inverse modeling of CO2 fluxes using GOSAT data and
multi-year ground-based observations, SOLA, 9, 45–50,
https://doi.org/10.2151/sola.2013-011, 2013. a
Schuh, A. E., Denning, A. S., Corbin, K. D., Baker, I. T., Uliasz, M.,
Parazoo, N., Andrews, A. E., and Worthy, D. E. J.: A regional high-resolution
carbon flux inversion of North America for 2004, Biogeosciences, 7,
1625–1644, https://doi.org/10.5194/bg-7-1625-2010, 2010. a
Schwarz, G.: Estimating the dimension of a model, Ann. Stat., 6, 461–464,
available at: http://www.jstor.org/stable/2958889 (last access: 27 April 2018), 1978. a
Shiga, Y. P., Michalak, A. M., Randolph Kawa, S., and Engelen, R. J.: In-situ
CO2 monitoring network evaluation and design: A criterion based on
atmospheric CO2 variability, J. Geophys. Res.-Atmos., 118, 2007–2018,
https://doi.org/10.1002/jgrd.50168, 2013. a
Shiga, Y. P., Michalak, A. M., Gourdji, S. M., Mueller, K. L., and Yadav, V.:
Detecting fossil fuel emissions patterns from subcontinental regions using
North American in situ CO2 measurements, Geophys. Res. Lett., 41,
4381–4388, https://doi.org/10.1002/2014GL059684, 2014. a, b
Takagi, H., Saeki, T., Oda, T., Saito, M., Valsala, V., Belikov, D., Saito, R.,
Yoshida, Y., Morino, I., Uchino, O., Andres, R. J., Yokota, T., and
Maksyutov, S.: On the benefit of GOSAT observations to the estimation of
regional CO2 fluxes, SOLA, 7, 161–164, https://doi.org/10.2151/sola.2011-041, 2011.
a
Takahashi, T., Sutherland, S., and Kozyr, A.: Global Ocean Surface Water
Partial Pressure of CO2 Database: Measurements Performed During 1957–2015
(Version 2015), ORNL/CDIAC-160, NDP-088(V2015), Oak Ridge
National Laboratory, U.S. Department of Energy, Oak Ridge, Tennesee,
https://doi.org/10.3334/CDIAC/OTG.NDP088(V2015), 2016. a
van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Mu, M.,
Kasibhatla, P. S., Morton, D. C., DeFries, R. S., Jin, Y., and van Leeuwen,
T. T.: Global fire emissions and the contribution of deforestation, savanna,
forest, agricultural, and peat fires (1997–2009), Atmos. Chem. Phys., 10,
11707–11735, https://doi.org/10.5194/acp-10-11707-2010, 2010. a
Worden, J. R., Doran, G., Kulawik, S., Eldering, A., Crisp, D., Frankenberg,
C., O'Dell, C., and Bowman, K.: Evaluation and attribution of OCO-2 XCO2
uncertainties, Atmos. Meas. Tech., 10, 2759–2771,
https://doi.org/10.5194/amt-10-2759-2017, 2017. a
Wunch, D., Wennberg, P. O., Toon, G. C., Connor, B. J., Fisher, B., Osterman,
G. B., Frankenberg, C., Mandrake, L., O'Dell, C., Ahonen, P., Biraud, S. C.,
Castano, R., Cressie, N., Crisp, D., Deutscher, N. M., Eldering, A., Fisher,
M. L., Griffith, D. W. T., Gunson, M., Heikkinen, P., Keppel-Aleks, G.,
Kyrö, E., Lindenmaier, R., Macatangay, R., Mendonca, J., Messerschmidt,
J., Miller, C. E., Morino, I., Notholt, J., Oyafuso, F. A., Rettinger, M.,
Robinson, J., Roehl, C. M., Salawitch, R. J., Sherlock, V., Strong, K.,
Sussmann, R., Tanaka, T., Thompson, D. R., Uchino, O., Warneke, T., and
Wofsy, S. C.: A method for evaluating bias in global measurements of CO2
total columns from space, Atmos. Chem. Phys., 11, 12317–12337,
https://doi.org/10.5194/acp-11-12317-2011, 2011. a
Wunch, D., Wennberg, P. O., Osterman, G., Fisher, B., Naylor, B., Roehl, C.
M., O'Dell, C., Mandrake, L., Viatte, C., Kiel, M., Griffith, D. W. T.,
Deutscher, N. M., Velazco, V. A., Notholt, J., Warneke, T., Petri, C., De
Maziere, M., Sha, M. K., Sussmann, R., Rettinger, M., Pollard, D., Robinson,
J., Morino, I., Uchino, O., Hase, F., Blumenstock, T., Feist, D. G., Arnold,
S. G., Strong, K., Mendonca, J., Kivi, R., Heikkinen, P., Iraci, L.,
Podolske, J., Hillyard, P. W., Kawakami, S., Dubey, M. K., Parker, H. A.,
Sepulveda, E., García, O. E., Te, Y., Jeseck, P., Gunson, M. R., Crisp,
D., and Eldering, A.: Comparisons of the Orbiting Carbon Observatory-2
(OCO-2) XCO2 measurements with TCCON, Atmos. Meas. Tech., 10,
2209–2238, https://doi.org/10.5194/amt-10-2209-2017, 2017. a, b
Yokota, T., Yoshida, Y., Eguchi, N., Ota, Y., Tanaka, T., Watanabe, H., and
Maksyutov, S.: Global Concentrations of CO2 and CH4 Retrieved from
GOSAT: First Preliminary Results, SOLA, 5, 160–163,
https://doi.org/10.2151/sola.2009-041, 2009. a
Zucchini, W.: An Introduction to Model Selection, J. Math. Psychol., 44,
41–61, https://doi.org/10.1006/jmps.1999.1276, 2000. a
Short summary
NASA's Orbiting Carbon Observatory 2 (OCO-2) satellite observes CO2 in the atmosphere globally. We evaluate the extent to which current OCO-2 observations can inform scientific understanding of the biospheric carbon balance. We find that current observations are best-equipped to constrain the biospheric carbon balance across continental or hemispheric regions and provide limited information on smaller regions.
NASA's Orbiting Carbon Observatory 2 (OCO-2) satellite observes CO2 in the atmosphere globally....
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