Articles | Volume 21, issue 6
Atmos. Chem. Phys., 21, 4709–4727, 2021
https://doi.org/10.5194/acp-21-4709-2021
Atmos. Chem. Phys., 21, 4709–4727, 2021
https://doi.org/10.5194/acp-21-4709-2021

Research article 26 Mar 2021

Research article | 26 Mar 2021

Pre-deliquescent water uptake in deposited nanoparticles observed with in situ ambient pressure X-ray photoelectron spectroscopy

Jack J. Lin et al.

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Cited articles

Ammann, M., Artiglia, L., and Bartels-Rausch, T.: X-Ray Excited Electron Spectroscopy to Study Gas–Liquid Interfaces of Atmospheric Relevance, in: Physical Chemistry of Gas-Liquid Interfaces, Elsevier, Amsterdam, Netherlands, 135–166, 2018. a
Antonsson, E., Patanen, M., Nicolas, C., Neville, J. J., Benkoula, S., Goel, A., and Miron, C.: Complete Bromide Surface Segregation in Mixed NaCl / NaBrAerosols Grown from Droplets, Phys. Rev. X, 5, 011025, https://doi.org/10.1103/PhysRevX.5.011025 2015. a
Archer, J., Walker, J., Gregson, F. K. A., Hardy, D. A., and Reid, J. P.: Drying Kinetics and Particle Formation from Dilute Colloidal Suspensions in Aerosol Droplets, Langmuir, 26, 12481–12493, 2020. a
Ault, A. P. and Axson, J. L.: Atmospheric Aerosol Chemistry: Spectroscopic and Microscopic Advances, Anal. Chem., 89, 430–452, 2016. a
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We used surface-sensitive X-ray photoelectron spectroscopy (XPS) to study laboratory-generated nanoparticles of atmospheric interest at 0–16 % relative humidity. XPS gives direct information about changes in the chemical state from the binding energies of probed elements. Our results indicate water adsorption and associated chemical changes at the particle surfaces well below deliquescence, with distinct features for different particle components and implications for atmospheric chemistry.
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