Articles | Volume 20, issue 12
https://doi.org/10.5194/acp-20-7217-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-7217-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
23 Jun 2020
Research article |
| 23 Jun 2020
| 23 Jun 2020
Heavy air pollution with a unique “non-stagnant” atmospheric boundary layer in the Yangtze River middle basin aggravated by regional transport of PM2.5 over China
Chao Yu
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
Southwest Electric Power Design Institute Co., Ltd, of China Power
Engineering Consulting Group, Chengdu, 610021, China
Tianliang Zhao
CORRESPONDING AUTHOR
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
Yongqing Bai
CORRESPONDING AUTHOR
Institute of Heavy Rain, China Meteorological Administration, Wuhan,
430205, China
Lei Zhang
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
Chengdu Academy of Environmental Sciences, Chengdu, 610031, China
Shaofei Kong
Department of Atmospheric Sciences, School of Environmental Studies, China University of Geosciences (Wuhan), 430074, Wuhan, China
Xingna Yu
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
Jinhai He
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
Chunguang Cui
Institute of Heavy Rain, China Meteorological Administration, Wuhan,
430205, China
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
Yinchang You
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
Guoxu Ma
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
Ming Wu
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
Jiacheng Chang
Collaborative Innovation Center on Forecast and Evaluation of
Meteorological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of
China Meteorological Administration, PREMIC, Nanjing University of
Information Science and Technology, Nanjing 210044, China
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Yongqing Bai, Tianliang Zhao, Yue Zhou, Jie Xiong, Weiyang Hu, Yao Gu, Lin Liu, Shaofei Kong, and Huang Zheng
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-708, https://doi.org/10.5194/acp-2020-708, 2020
Revised manuscript not accepted
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Xiaoning Xie, Anmin Duan, Zhengguo Shi, Xinzhou Li, Hui Sun, Xiaodong Liu, Xugeng Cheng, Tianliang Zhao, Huizheng Che, and Yangang Liu
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Yilun Chen, Guangcan Chen, Chunguang Cui, Aoqi Zhang, Rong Wan, Shengnan Zhou, Dongyong Wang, and Yunfei Fu
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The vertical evolution of the cloud effective radius reflects the precipitation-forming process. We developed an algorithm for retrieving it based on objective cloud-cluster identification rather than the subjective polygon of the conventional method. The profile shows completely different morphologies in different life stages of the cloud cluster, which is important in the characterization of the formation of precipitation and the temporal evolution of microphysical processes.
Jun Zhu, Xiangao Xia, Huizheng Che, Jun Wang, Zhiyuan Cong, Tianliang Zhao, Shichang Kang, Xuelei Zhang, Xingna Yu, and Yanlin Zhang
Atmos. Chem. Phys., 19, 14637–14656, https://doi.org/10.5194/acp-19-14637-2019, https://doi.org/10.5194/acp-19-14637-2019, 2019
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The long-term temporal–spatial variations of the aerosol optical properties over the Tibetan Plateau (TP) based on the multiple ground-based sun photometer sites and the MODIS product are presented. Besides, the aerosol pollution and aerosol transport processes over the TP are also analyzed by the observations and models. The results in this region could help reduce the assessment uncertainties of aerosol radiative forcing and provide more information on aerosol transportation.
Shixian Zhai, Daniel J. Jacob, Xuan Wang, Lu Shen, Ke Li, Yuzhong Zhang, Ke Gui, Tianliang Zhao, and Hong Liao
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Observed annual mean PM2.5 decreased by 30–50 % in China from 2013–2018. However, meteorologically PM2.5 variability complicates trend attribution. We used a stepwise multiple linear regression model to quantitatively separate contributions from anthropogenic emissions and meteorology. Results show that 88 % of the PM2.5 decrease across China is attributable to anthropogenic emission changes, and 12 % is attributable to meteorology.
Huang Zheng, Shaofei Kong, Fangqi Wu, Yi Cheng, Zhenzhen Niu, Shurui Zheng, Guowei Yang, Liquan Yao, Qin Yan, Jian Wu, Mingming Zheng, Nan Chen, Ke Xu, Yingying Yan, Dantong Liu, Delong Zhao, Tianliang Zhao, Yongqing Bai, Shuanglin Li, and Shihua Qi
Atmos. Chem. Phys., 19, 4499–4516, https://doi.org/10.5194/acp-19-4499-2019, https://doi.org/10.5194/acp-19-4499-2019, 2019
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This study simultaneously observed black carbon (BC) at five sites in central China and on the south edge of North China Plain, which have the most serious air pollution issues in China. The differences in BC properties between different air quality conditions and the property changes during transportation were studied. The main findings of this study were that during the downwind transportation of air, the BC mass concentration increased, whereas the absorption Ångström exponent decreased.
Junting Zhong, Xiaoye Zhang, Yaqiang Wang, Jizhi Wang, Xiaojing Shen, Hongsheng Zhang, Tijian Wang, Zhouqing Xie, Cheng Liu, Hengde Zhang, Tianliang Zhao, Junying Sun, Shaojia Fan, Zhiqiu Gao, Yubin Li, and Linlin Wang
Atmos. Chem. Phys., 19, 3287–3306, https://doi.org/10.5194/acp-19-3287-2019, https://doi.org/10.5194/acp-19-3287-2019, 2019
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In various haze regions in China, including the Guanzhong Plain, the middle and lower reaches of the Yangtze River, the Pearl River Delta, the Sichuan Basin, and the Northeast China Plain, heavy aerosol pollution episodes include inter-/trans-regional transport stages and cumulative stages (CSs). During CSs a two-way feedback mechanism exists between unfavorable meteorological conditions and cumulative aerosol pollution. This two-way feedback is further quantified and its magnitude is compared.
Jing Wang, Zhiwei Zhu, Li Qi, Qiaohua Zhao, Jinhai He, and Julian X. L. Wang
Atmos. Chem. Phys., 19, 1521–1535, https://doi.org/10.5194/acp-19-1521-2019, https://doi.org/10.5194/acp-19-1521-2019, 2019
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Less attention has been paid to haze weather during the autumn season. Here, we unravel the mechanism of how SST anomalies over the subtropical North Atlantic and western North Pacific drive the interannual variability of the autumnal haze days in the Beijing–Tianjin–Hebei region. The two pathways of SST anomaly forcings can result in an anticyclonic (cyclonic) anomaly over Northeast Asia, leading to a lower-level southerly (northerly) anomaly and in turn more (fewer) haze days in this region.
Yue Peng, Hong Wang, Yubin Li, Changwei Liu, Tianliang Zhao, Xiaoye Zhang, Zhiqiu Gao, Tong Jiang, Huizheng Che, and Meng Zhang
Atmos. Chem. Phys., 18, 17421–17435, https://doi.org/10.5194/acp-18-17421-2018, https://doi.org/10.5194/acp-18-17421-2018, 2018
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Two surface layer schemes are evaluated in eastern China based on observational flux data. The results indicate that the Li scheme better describes regional atmosphere stratification compared with the MM5 scheme, especially for the transition stage from unstable to stable atmosphere conditions, corresponding to PM2.5 accumulation. Our research suggests the potential improved possibilities for severe haze prediction in eastern China by coupling Li online into atmosphere chemical models.
Jun Hu, Yichen Li, Tianliang Zhao, Jane Liu, Xiao-Ming Hu, Duanyang Liu, Yongcheng Jiang, Jianming Xu, and Luyu Chang
Atmos. Chem. Phys., 18, 16239–16251, https://doi.org/10.5194/acp-18-16239-2018, https://doi.org/10.5194/acp-18-16239-2018, 2018
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Using observational and modeling studies, the importance of the mechanism driving regional O3 transport in the residual layer (RL) with respect to summer smog over the Yangtze River Delta region in eastern China was revealed. This mechanism was also examined in association with diurnal change in the atmospheric boundary layer. Regional O3 transport through the nocturnal RL is believed to have great implications for understanding urban and regional O3 pollution in this area.
Xiaoning Xie, Xiaodong Liu, Huizheng Che, Xiaoxun Xie, Xinzhou Li, Zhengguo Shi, Hongli Wang, Tianliang Zhao, and Yangang Liu
Atmos. Chem. Phys., 18, 12683–12698, https://doi.org/10.5194/acp-18-12683-2018, https://doi.org/10.5194/acp-18-12683-2018, 2018
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This study extends our previous investigation in dust–radiation interactions to investigate SRF and its feedbacks on the regional climate and the dust cycle over east Asia by use of the CAM4-BAM. Our results show that SRF increases the east Asian dust emissions significantly by 13.7 % in the spring, in contrast to −7.6 % of decreased dust emissions by DRF. Hence, a significant feature of SRF on the Tibetan Plateau can create a positive feedback loop to enhance the dust cycle over east Asia.
Jian Wu, Shaofei Kong, Fangqi Wu, Yi Cheng, Shurui Zheng, Qin Yan, Huang Zheng, Guowei Yang, Mingming Zheng, Dantong Liu, Delong Zhao, and Shihua Qi
Atmos. Chem. Phys., 18, 11623–11646, https://doi.org/10.5194/acp-18-11623-2018, https://doi.org/10.5194/acp-18-11623-2018, 2018
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In order to support regional modeling impact on air quality and policy making on controlling open biomass burning emissions, accurate open biomass burning emissions were estimated from 2003 to 2015 with high spatial and temporal resolution. Multiple satellite data, updated biomass data and survey results were all used to improve the accuracy. In addition, management policies and all influencing factors in rural areas for open biomass burning emissions were considered.
Mingming Zheng, Shaofei Kong, Jianguo Bao, Ke Xu, Shurui Zheng, Guowei Yang, Jihong Quan, Lianxin Yuan, Nan Chen, Yiping Tian, Huang Zheng, Jian Wu, Dantong Liu, Delong Zhao, Qin Yan, Tianliang Zhao, and Shihua Qi
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2018-367, https://doi.org/10.5194/acp-2018-367, 2018
Preprint retracted
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In this paper, we study the aerosol acidity for different time scales, pollution episodes and air mass directions in a megacity of central China with high ambient temperature and relative humidity, and the impacting factors of pH were identified. This research is the first study concerning the aerosol acidity based on one-year online monitoring dataset with high resolution in central China, which is an important supplementary for the current aerosol acidity study around the world.
Shixian Zhai, Xingqin An, Tianliang Zhao, Zhaobin Sun, Wei Wang, Qing Hou, Zengyuan Guo, and Chao Wang
Atmos. Chem. Phys., 18, 6241–6258, https://doi.org/10.5194/acp-18-6241-2018, https://doi.org/10.5194/acp-18-6241-2018, 2018
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The GRAPES–CUACE aerosol adjoint model was developed and applied in detecting PM2.5 sources for haze events in eastern China (EC). The response time of Beijing PM2.5 pollution peaks to local and surrounding emissions is quantized for regional transport of air pollution over the EC. The adjoint results agreed well with the Models-3/CMAQ assessments. The adjoint method is powerful in simulating the receptor–source relationship and can be utilized in dynamic air quality control scheme design.
Huang Zheng, Shaofei Kong, Xinli Xing, Yao Mao, Tianpeng Hu, Yang Ding, Gang Li, Dantong Liu, Shuanglin Li, and Shihua Qi
Atmos. Chem. Phys., 18, 4567–4595, https://doi.org/10.5194/acp-18-4567-2018, https://doi.org/10.5194/acp-18-4567-2018, 2018
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This research is the first study concerning the 1-year online monitoring of volatile organic compounds in an oil–gas field in China. The VOC concentrations, compositions and ozone formation potential in this study are quite different from other research. The contributions of natural gas and the other four sources to total VOCs are quantified. The different timescale variations in different sources are described. This research broadens our knowledge of VOC behavior in this type of region.
Lei Zhang, Tianliang Zhao, Sunling Gong, Shaofei Kong, Lili Tang, Duanyang Liu, Yongwei Wang, Lianji Jin, Yunpeng Shan, Chenghao Tan, Yingjie Zhang, and Xiaomei Guo
Atmos. Chem. Phys., 18, 2065–2079, https://doi.org/10.5194/acp-18-2065-2018, https://doi.org/10.5194/acp-18-2065-2018, 2018
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An updated emission inventory of coal-fired power plants (UEIPP) based on online monitoring data in Jiangsu Province in China for the year of 2012 was implemented in the Multi-resolution Emission Inventory for China (MEIC). By employing the model WRF-Chem, two simulations were executed to assess the atmospheric environmental change by using the original MEIC and the MEIC with the UEIPP. Interestingly, when the UEIPP was used, the atmospheric oxidizing capacity significantly reinforced.
Delong Zhao, Mengyu Huang, Dantong Liu, Deping Ding, Ping Tian, Quan Liu, Wei Zhou, Jiujiang Sheng, Fei Wang, Kai Bi, Yan Yang, Xia Li, Yaqiong Hu, Xin Guo, Yang Gao, Hui He, Yunbo Chen, Shaofei Kong, and Jiayi Huang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-1118, https://doi.org/10.5194/acp-2017-1118, 2018
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This study for the first time reports the 3D distributions of black carbon and detailed physical properties in the boundary layer over the North China Plain, using intensive aircraft measurements in both hot and cold seasons. The BC mass in the planetary boundary layer (PBL) was found to be largely influenced by meteorology which modulated the local emission and regional transport.
Xiangde Xu, Xueliang Guo, Tianliang Zhao, Xingqin An, Yang Zhao, Jiannong Quan, Fei Mao, Yang Gao, Xinghong Cheng, Wenhui Zhu, and Yinjun Wang
Atmos. Chem. Phys., 17, 8011–8019, https://doi.org/10.5194/acp-17-8011-2017, https://doi.org/10.5194/acp-17-8011-2017, 2017
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Aerosols have complicated effects on clouds and precipitation, depending on many factors such as aerosol properties, topography and meteorological conditions. Most previous investigations of aerosol impacts on clouds and precipitation are primarily based on limited cases on relatively small spatial and temporal scales. The climate forcing of aerosols on precipitation in large-scale continental regions and their physical causes remain uncertain.
Zefeng Zhang, Yan Shen, Yanwei Li, Bin Zhu, and Xingna Yu
Atmos. Chem. Phys., 17, 4147–4157, https://doi.org/10.5194/acp-17-4147-2017, https://doi.org/10.5194/acp-17-4147-2017, 2017
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Aerosol particles and relative humidity are the main factors that affect atmospheric visibility. Due to the complexity of the physicochemical properties of aerosol particles, more and more instruments and cost were put into research, which limited the development of large area observation research. Thus, it is especially important to find the key parameters which affect the visibility and to establish the observation scheme.
Zhaopeng Luan, Yongxiang Han, Tianliang Zhao, Feng Liu, Chong Liu, Mark J. Rood, Xinghua Yang, Qing He, and Huichao Lu
Atmos. Meas. Tech., 10, 273–279, https://doi.org/10.5194/amt-10-273-2017, https://doi.org/10.5194/amt-10-273-2017, 2017
Chunpeng Leng, Junyan Duan, Chen Xu, Hefeng Zhang, Yifan Wang, Yanyu Wang, Xiang Li, Lingdong Kong, Jun Tao, Renjian Zhang, Tiantao Cheng, Shuping Zha, and Xingna Yu
Atmos. Chem. Phys., 16, 9221–9234, https://doi.org/10.5194/acp-16-9221-2016, https://doi.org/10.5194/acp-16-9221-2016, 2016
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Meteorological conditions, local anthropogenic emissions and aerosol properties played major roles in this historic winter haze weather formation. Aerosols the size of 600–1400 nm are mostly responsible for the impairment of atmospheric visibility. This study was performed by combining many on-line measurement techniques which were calibrated regularly to ensure reliability, and can act as a reference for forecasting and eliminating the occurrences of regional atmospheric pollutions in China.
X. Xu, T. Zhao, F. Liu, S. L. Gong, D. Kristovich, C. Lu, Y. Guo, X. Cheng, Y. Wang, and G. Ding
Atmos. Chem. Phys., 16, 1365–1375, https://doi.org/10.5194/acp-16-1365-2016, https://doi.org/10.5194/acp-16-1365-2016, 2016
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We study the climate modulation of the Tibetan Plateau (TP) on atmospheric environment in China with three key points. First a large-scale "susceptible region" for haze is climatologically identified over central-eastern China (CEC) harbored by the TP. Secondly, thermal anomalies of the TP induce the changes in meteorological drivers downstream for frequent haze events in CEC. Finally implications of the TP for the atmospheric environment have potential utility for development planning in China.
Y. C. Jiang, T. L. Zhao, J. Liu, X. D. Xu, C. H. Tan, X. H. Cheng, X. Y. Bi, J. B. Gan, J. F. You, and S. Z. Zhao
Atmos. Chem. Phys., 15, 13331–13338, https://doi.org/10.5194/acp-15-13331-2015, https://doi.org/10.5194/acp-15-13331-2015, 2015
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An O3 episode with high night-time O3 was observed before typhoon landing over southeastern China. Variations in the observed O3, NO2, CO and meteorology during Typhoon Hagibis event clearly suggest a substantial impact of the peripheral downdrafts in the tropical cyclone on the high O3 episode. This study provides observational evidence of typhoon-driven intrusion of O3 from the upper troposphere and lower stratosphere to surface air threatening to ambient air quality.
C. Jiang, H. Wang, T. Zhao, T. Li, and H. Che
Atmos. Chem. Phys., 15, 5803–5814, https://doi.org/10.5194/acp-15-5803-2015, https://doi.org/10.5194/acp-15-5803-2015, 2015
K. Ding, J. Liu, A. Ding, Q. Liu, T. L. Zhao, J. Shi, Y. Han, H. Wang, and F. Jiang
Atmos. Chem. Phys., 15, 2843–2866, https://doi.org/10.5194/acp-15-2843-2015, https://doi.org/10.5194/acp-15-2843-2015, 2015
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1. High CO abundances of 300-550 ppbv is shown in aircraft MOZAIC data between 700 and 300 hPa over East Asia in three episodes. Correspondingly, elevated CO is observed in satellite MOPITT data at similar altitudes.
2. GEOS-Chem and FLEXPART simulations reveal distinct uplifting processes for CO from fires and anthropogenic sources in the cases.
3. Topography in East Asia affects uplifting of CO in different ways.
4. The new version 5 MOPITT data can help diagnose vertical transport of CO.
S. F. Kong, L. Li, X. X. Li, Y. Yin, K. Chen, D. T. Liu, L. Yuan, Y. J. Zhang, Y. P. Shan, and Y. Q. Ji
Atmos. Chem. Phys., 15, 2167–2184, https://doi.org/10.5194/acp-15-2167-2015, https://doi.org/10.5194/acp-15-2167-2015, 2015
X. Xu, T. Zhao, C. Lu, Y. Guo, B. Chen, R. Liu, Y. Li, and X. Shi
Atmos. Chem. Phys., 14, 11287–11295, https://doi.org/10.5194/acp-14-11287-2014, https://doi.org/10.5194/acp-14-11287-2014, 2014
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The Tibetan Plateau (TP) with its thermal structure leads to dynamic processes of vapor transport, similar to the CISK mechanism of tropical cyclones.
Two CISK-like processes, contiguous horizontally but staggered vertically, in two ladders over the southern slopes and main platform of the TP relay the moist air over the TP. An integration of mechanical and thermal TP forcing is revealed in relation to the Asian summer monsoon circulation transporting water vapor from tropical oceans to the TP.
J. Liu, D. W. Tarasick, V. E. Fioletov, C. McLinden, T. Zhao, S. Gong, C. Sioris, J. J. Jin, G. Liu, and O. Moeini
Atmos. Chem. Phys., 13, 11441–11464, https://doi.org/10.5194/acp-13-11441-2013, https://doi.org/10.5194/acp-13-11441-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Pollution affects Arabian and Saharan dust optical properties in the eastern Mediterranean
Phase matrix characterization of long-range-transported Saharan dust using multiwavelength-polarized polar imaging nephelometry
Measurement report: The influence of particle number size distribution and hygroscopicity on the microphysical properties of cloud droplets at a mountain site
Measurement report: Long-term assessment of primary and secondary organic aerosols in the Shanghai megacity throughout China's Clean Air actions since 2010
The evolution of aerosol mixing state derived from a field campaign in Beijing: implications for particle aging timescales in urban atmospheres
Measurement report: Size-resolved particle effective density measured by an AAC-SMPS and implications for chemical composition
Measurement report: Aircraft observations of aerosol and microphysical quantities of stratocumulus in autumn over Guangxi Province, China – daylight variation, vertical distribution, and aerosol–cloud interactions
Hygroscopic aerosols amplify longwave downward radiation in the Arctic
Measurement report: Aerosol and cloud nuclei properties along the Central and Northern Great Barrier Reef: Impact of continental emissions
Measurement report: Optical and structural properties of atmospheric water-soluble organic carbon in China – insights from multi-site spectroscopic measurements
Measurement report: The variation properties of aerosol hygroscopic growth related to chemical composition during new particle formation days in a coastal city of Southeast China
In situ vertical observations of the layered structure of air pollution in a continental high-latitude urban boundary layer during winter
Size-resolved hygroscopicity and volatility properties of ambient urban aerosol particles measured by a volatility hygroscopicity tandem differential mobility analyzer system in Beijing
Terrestrial runoff is an important source of biological ice-nucleating particles in Arctic marine systems
Characterization of aerosol over the eastern Mediterranean by polarization-sensitive Raman lidar measurements during A-LIFE – aerosol type classification and type separation
Aerosol spectral optical properties in the Paris urban area and its peri-urban and forested surroundings during summer 2022 from ACROSS surface observations
Measurement report: An investigation of the spatiotemporal variability in aerosols in the mountainous terrain of the upper Colorado River basin using SAIL-Net
Contributions of the synoptic meteorology to the seasonal cloud condensation nuclei cycle over the Southern Ocean
Measurement report: Cloud condensation nuclei (CCN) activity in the South China Sea from shipborne observations during the summer and winter of 2021 – seasonal variation and anthropogenic influence
Differential characterization of air ions in boreal forest of Finland and megacity of eastern China
Source-Dependent Optical Properties and Molecular Characteristics of Atmospheric Brown Carbon
On-road vehicle emission measurements show a significant reduction of black carbon and nitrogen oxides emissions in Euro6c and 6d diesel-powered cars
Measurement report: A comparative analysis of an intensive incursion of fluorescing African dust particles over Puerto Rico and another over Spain
Measurement report: Analysis of aerosol optical depth variation at Zhongshan Station in Antarctica
External particle mixing influences hygroscopicity in a sub-urban area
Long-term observations of black carbon and carbon monoxide in the Poker Flat Research Range, central Alaska, with a focus on forest wildfire emissions
Origin, size distribution and hygroscopic properties of marine aerosols in the south-western Indian Ocean: report of 6 campaigns of shipborne observations
High ice-nucleating particle concentrations associated with Arctic haze in springtime cold-air outbreaks
CCN estimations at a high-altitude remote site: role of organic aerosol variability and hygroscopicity
Aerosol hygroscopicity over the southeast Atlantic Ocean during the biomass burning season – Part 1: From the perspective of scattering enhancement
Spatial, temporal, and meteorological impact of the 26 February 2023 dust storm: increase in particulate matter concentrations across New Mexico and West Texas
Large spatiotemporal variability in aerosol properties over central Argentina during the CACTI field campaign
Microphysical properties of refractory black carbon aerosols for different air masses at a central European background site
Quantification and characterization of primary biological aerosol particles and microbes aerosolized from Baltic seawater
Brownness of organics in anthropogenic biomass burning aerosols over South Asia
Multi-year black carbon observations and modeling close to the largest gas flaring and wildfire regions (Western Siberian Arctic)
Strong influence of Black Carbon on aerosol optical properties in Central Amazonia during the fire season
Source apportionment of particle number size distribution at the street canyon and urban background sites
Long-range transport of coarse mineral dust: an evaluation of the Met Office Unified Model against aircraft observations
Extreme Saharan dust events expand northward over the Atlantic and Europe, prompting record-breaking PM10 and PM2.5 episodes
Atmospheric black carbon in the metropolitan area of La Paz and El Alto, Bolivia: concentration levels and emission sources
Changing optical properties of black carbon and brown carbon aerosols during long-range transport from the Indo-Gangetic Plain to the equatorial Indian Ocean
Aerosol size distribution properties associated with cold-air outbreaks in the Norwegian Arctic
Ice-nucleating particles active below −24 °C in a Finnish boreal forest and their relationship to bioaerosols
Measurements of particle emissions of an A350-941 burning 100 % sustainable aviation fuels in cruise
Vertical distribution of ice nucleating particles over the boreal forest of Hyytiälä, Finland
Multi-year gradient measurements of sea spray fluxes over the Baltic Sea and the North Atlantic Ocean
Measurement report: In situ vertical profiles of below-cloud aerosol over the central Greenland Ice Sheet
Occurrence, abundance, and formation of atmospheric tarballs from a wide range of wildfires in the western US
Measurement report: Contribution of atmospheric new particle formation to ultrafine particle concentration, cloud condensation nuclei, and radiative forcing – results from 5-year observations in central Europe
Marilena Teri, Josef Gasteiger, Katharina Heimerl, Maximilian Dollner, Manuel Schöberl, Petra Seibert, Anne Tipka, Thomas Müller, Sudharaj Aryasree, Konrad Kandler, and Bernadett Weinzierl
Atmos. Chem. Phys., 25, 6633–6662, https://doi.org/10.5194/acp-25-6633-2025, https://doi.org/10.5194/acp-25-6633-2025, 2025
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The A-LIFE aircraft field experiment was carried out in the eastern Mediterranean in 2017. Using A-LIFE data, we studied the change in mineral dust optical properties due to mixing with anthropogenic aerosols. We found that increasing pollution affects dust optical properties, which has implications for identifying dust events and understanding their climate effects. We also show that optical properties of Saharan and Arabian dust are similar when comparing cases with equal pollution content.
Elena Bazo, Daniel Pérez-Ramírez, Antonio Valenzuela, J. Vanderlei Martins, Gloria Titos, Alberto Cazorla, Fernando Rejano, Diego Patrón, Arlett Díaz-Zurita, Francisco José García-Izquierdo, David Fuertes, Lucas Alados-Arboledas, and Francisco José Olmo
Atmos. Chem. Phys., 25, 6325–6352, https://doi.org/10.5194/acp-25-6325-2025, https://doi.org/10.5194/acp-25-6325-2025, 2025
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This works analyzes the aerosol scattering phase function for transported Saharan dust to the city of Granada – located in southwestern Europe. We use the novel technique polar imaging nephelometry that helps to determine the phase functions using a CMOS camera. The capability of measuring with polarized light helps to infer new properties about the mixture of Saharan dust particles with those of anthropogenic origin.
Xiaojing Shen, Quan Liu, Junying Sun, Wanlin Kong, Qianli Ma, Bing Qi, Lujie Han, Yangmei Zhang, Linlin Liang, Lei Liu, Shuo Liu, Xinyao Hu, Jiayuan Lu, Aoyuan Yu, Huizheng Che, and Xiaoye Zhang
Atmos. Chem. Phys., 25, 5711–5725, https://doi.org/10.5194/acp-25-5711-2025, https://doi.org/10.5194/acp-25-5711-2025, 2025
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In this work, an automatic switched inlet system was developed and employed to investigate the aerosols and cloud droplets at a mountain site with frequent cloud processes. It showed different characteristics of cloud residual and interstitial particles. Stronger particle hygroscopicity reduced liquid water content and smaller cloud droplet diameters. This investigation contributes to understanding aerosol–cloud interactions by assessing the impact of aerosol particles on cloud microphysics.
Haifeng Yu, Yunhua Chang, Lin Cheng, Yusen Duan, and Jianlin Hu
Atmos. Chem. Phys., 25, 5355–5369, https://doi.org/10.5194/acp-25-5355-2025, https://doi.org/10.5194/acp-25-5355-2025, 2025
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This study presents long-term measurements and comprehensive analysis of carbonaceous aerosols in fine particles in Shanghai. We further estimated primary and secondary carbon levels, examining their temporal variations on interannual, monthly, seasonal, and diurnal scales. Through rigorous statistical analysis and correlation studies with meteorological parameters and pollutant concentrations, the origins, formation mechanisms, and spatial distribution patterns of secondary organic carbon were elucidated.
Jieyao Liu, Fang Zhang, Jingye Ren, Lu Chen, Anran Zhang, Zhe Wang, Songjian Zou, Honghao Xu, and Xingyan Yue
Atmos. Chem. Phys., 25, 5075–5086, https://doi.org/10.5194/acp-25-5075-2025, https://doi.org/10.5194/acp-25-5075-2025, 2025
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Particle mixing states and aging timescales are important for the evaluation of aerosol climate effects, but they are poorly parameterized in current models. We unravel the evolution of real-time mixing states and the aging timescale of size-resolved particles based on field measurements in urban Beijing. This study provides an observational basis for accurately parameterizing the aging timescale of aerosol particles in climate models.
Yao Song, Jing Wei, Wenlong Zhao, Jinmei Ding, Xiangyu Pei, Fei Zhang, Zhengning Xu, Ruifang Shi, Ya Wei, Lu Zhang, Lingling Jin, and Zhibin Wang
Atmos. Chem. Phys., 25, 4755–4766, https://doi.org/10.5194/acp-25-4755-2025, https://doi.org/10.5194/acp-25-4755-2025, 2025
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This study investigates the size-resolved effective density (ρeff) of aerosol particles in Hangzhou using a tandem aerodynamic aerosol classifier and scanning mobility particle sizer system. The ρeff values ranged from 1.47 to 1.63 g cm-3, increasing with particle diameter. The relationship between ρeff and the particle diameter varies due to differences in the chemical composition of the particles. A new method to derive the size-resolved chemical composition of particles from ρeff is proposed.
Sihan Liu, Honglei Wang, Delong Zhao, Wei Zhou, Yuanmou Du, Zhengguo Zhang, Peng Cheng, Tianliang Zhao, Yue Ke, Zihao Wu, and Mengyu Huang
Atmos. Chem. Phys., 25, 4151–4165, https://doi.org/10.5194/acp-25-4151-2025, https://doi.org/10.5194/acp-25-4151-2025, 2025
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To understand the effect of aerosols on the vertical distribution of stratocumulus microphysical quantities in southwest China, the daily variation characteristics and formation mechanism of the vertical profiles of stratocumulus microphysical characteristics in this region were described using the data of nine cloud-crossing aircraft observations over Guangxi from 10 October to 3 November 2020.
Denghui Ji, Mathias Palm, Matthias Buschmann, Kerstin Ebell, Marion Maturilli, Xiaoyu Sun, and Justus Notholt
Atmos. Chem. Phys., 25, 3889–3904, https://doi.org/10.5194/acp-25-3889-2025, https://doi.org/10.5194/acp-25-3889-2025, 2025
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Our study explores how certain aerosols, like sea salt, affect infrared heat radiation in the Arctic, potentially speeding up warming. We used advanced technology to measure aerosol composition and found that these particles grow with humidity, significantly increasing their heat-trapping effect in the infrared region, especially in winter. Our findings suggest these aerosols could be a key factor in Arctic warming, emphasizing the importance of understanding aerosols for climate prediction.
E. Johanna Horchler, Joel Alroe, Luke Harrison, Luke Cravigan, Daniel P. Harrison, and Zoran D. Ristovski
EGUsphere, https://doi.org/10.5194/egusphere-2025-465, https://doi.org/10.5194/egusphere-2025-465, 2025
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Aerosols play a role in global climate by interacting with incoming solar radiation and by taking up water vapour from the atmosphere to form clouds. Enhancing local-scale cloud cover can reduce sea surface temperatures. Coral bleaching events increased in the Great Barrier Reef (GBR) as sea surface temperatures rise. Our study found that the number of aerosols and the cloud forming ability over the GBR increased if the aerosols were transported from inland Australia rather than the ocean.
Haibiao Chen, Caiqing Yan, Liubin Huang, Lin Du, Yang Yue, Xinfeng Wang, Qingcai Chen, Mingjie Xie, Junwen Liu, Fengwen Wang, Shuhong Fang, Qiaoyun Yang, Hongya Niu, Mei Zheng, Yan Wu, and Likun Xue
Atmos. Chem. Phys., 25, 3647–3667, https://doi.org/10.5194/acp-25-3647-2025, https://doi.org/10.5194/acp-25-3647-2025, 2025
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A comprehensive understanding of the optical properties of brown carbon (BrC) is essential to accurately assess its climatic effects. Based on multi-site spectroscopic measurements, this study demonstrated the significant spatial heterogeneity in the optical and structural properties of water-soluble organic carbon (WSOC) in different regions of China and revealed factors affecting WSOC light absorption and the relationship between fluorophores and light absorption of WSOC.
Lingjun Li, Mengren Li, Xiaolong Fan, Yuping Chen, Ziyi Lin, Anqi Hou, Siqing Zhang, Ronghua Zheng, and Jinsheng Chen
Atmos. Chem. Phys., 25, 3669–3685, https://doi.org/10.5194/acp-25-3669-2025, https://doi.org/10.5194/acp-25-3669-2025, 2025
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Here, we show differences and variations in the aerosol scattering hygroscopic growth factor (f(RH)) between new particle formation (NPF) and non-NPF days and the effect of aerosol chemical compositions on f(RH) in Xiamen with in situ observations. The findings are helpful for the further understanding of aerosol hygroscopicity in a coastal city and the use of hygroscopic growth factors in models of air quality and climate change.
Roman Pohorsky, Andrea Baccarini, Natalie Brett, Brice Barret, Slimane Bekki, Gianluca Pappaccogli, Elsa Dieudonné, Brice Temime-Roussel, Barbara D'Anna, Meeta Cesler-Maloney, Antonio Donateo, Stefano Decesari, Kathy S. Law, William R. Simpson, Javier Fochesatto, Steve R. Arnold, and Julia Schmale
Atmos. Chem. Phys., 25, 3687–3715, https://doi.org/10.5194/acp-25-3687-2025, https://doi.org/10.5194/acp-25-3687-2025, 2025
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This study presents an analysis of vertical measurements of pollution in an Alaskan city during winter. It investigates the relationship between the atmospheric structure and the layering of aerosols and trace gases. Results indicate an overall very shallow surface mixing layer. The height of this layer is strongly influenced by a local shallow wind. The study also provides information on the pollution chemical composition at different altitudes, including pollution signatures from power plants.
Aoyuan Yu, Xiaojing Shen, Qianli Ma, Jiayuan Lu, Xinyao Hu, Yangmei Zhang, Quan Liu, Linlin Liang, Lei Liu, Shuo Liu, Hongfei Tong, Huizheng Che, Xiaoye Zhang, and Junying Sun
Atmos. Chem. Phys., 25, 3389–3412, https://doi.org/10.5194/acp-25-3389-2025, https://doi.org/10.5194/acp-25-3389-2025, 2025
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In this work, we utilized a volatility hygroscopicity tandem differential mobility analyzer (VH-TDMA) to investigate, for the first time, the hygroscopicity and volatility of submicron aerosols, as well as their hygroscopicity after heating, in urban Beijing during the autumn of 2023. We analyzed the size-resolved characteristics of hygroscopicity and volatility, the relationship between hygroscopic and volatile properties, and the hygroscopicity of heated submicron aerosols.
Corina Wieber, Lasse Z. Jensen, Leendert Vergeynst, Lorenz Meire, Thomas Juul-Pedersen, Kai Finster, and Tina Šantl-Temkiv
Atmos. Chem. Phys., 25, 3327–3346, https://doi.org/10.5194/acp-25-3327-2025, https://doi.org/10.5194/acp-25-3327-2025, 2025
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The Arctic region is subject to profound changes due to a warming climate. Ice-nucleating particles (INPs) in the seawater can get transported to the atmosphere and impact cloud formation. However, the sources of characteristics of INPs in the marine areas are poorly understood. We investigated the INPs in seawater from Greenlandic fjords and identified a seasonal variability, with highly active INPs originating from terrestrial sources such as glacial and soil runoff.
Silke Groß, Volker Freudenthaler, Moritz Haarig, Albert Ansmann, Carlos Toledano, David Mateos, Petra Seibert, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Josef Gasteiger, Maximilian Dollner, Anne Tipka, Manuel Schöberl, Marilena Teri, and Bernadett Weinzierl
Atmos. Chem. Phys., 25, 3191–3211, https://doi.org/10.5194/acp-25-3191-2025, https://doi.org/10.5194/acp-25-3191-2025, 2025
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Aerosols contribute to the largest uncertainties in climate change predictions. The eastern Mediterranean is a hotspot for aerosols with natural and anthropogenic contributions. We present lidar measurements performed during A-LIFE (Absorbing aerosol layers in a changing climate: aging, lifetime and dynamics) to characterize aerosols and aerosol mixtures. We extend current lidar classification and separation schemes and compare them to classification schemes using different methods.
Ludovico Di Antonio, Claudia Di Biagio, Paola Formenti, Aline Gratien, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Patrice Coll, Barbara D'Anna, Joel F. de Brito, David O. De Haan, Juliette R. Dignum, Shravan Deshmukh, Olivier Favez, Pierre-Marie Flaud, Cecile Gaimoz, Lelia N. Hawkins, Julien Kammer, Brigitte Language, Franck Maisonneuve, Griša Močnik, Emilie Perraudin, Jean-Eudes Petit, Prodip Acharja, Laurent Poulain, Pauline Pouyes, Eva Drew Pronovost, Véronique Riffault, Kanuri I. Roundtree, Marwa Shahin, Guillaume Siour, Eric Villenave, Pascal Zapf, Gilles Foret, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 25, 3161–3189, https://doi.org/10.5194/acp-25-3161-2025, https://doi.org/10.5194/acp-25-3161-2025, 2025
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The spectral complex refractive index (CRI) and single scattering albedo were retrieved from submicron aerosol measurements at three sites within the greater Paris area during the ACROSS field campaign (June–July 2022). Measurements revealed urban emission impact on surrounding areas. CRI full period averages at 520 nm were 1.41 – 0.037i (urban), 1.52 – 0.038i (peri-urban), and 1.50 – 0.025i (rural). Organic aerosols dominated the aerosol mass and contributed up to 22 % of absorption at 370 nm.
Leah D. Gibson, Ezra J. T. Levin, Ethan Emerson, Nick Good, Anna Hodshire, Gavin McMeeking, Kate Patterson, Bryan Rainwater, Tom Ramin, and Ben Swanson
Atmos. Chem. Phys., 25, 2745–2762, https://doi.org/10.5194/acp-25-2745-2025, https://doi.org/10.5194/acp-25-2745-2025, 2025
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From fall 2021 to summer 2023, SAIL-Net, a network of six aerosol measurement nodes, was deployed in the East River watershed (Colorado, USA) to study aerosol variability across space and time in mountainous terrain. We found that aerosol variability is influenced by elevation differences, with the most representative site in the region changing seasonally, suggesting aerosol spatial variability also varies seasonally. This work offers a blueprint for future studies in other mountainous regions.
Tahereh Alinejadtabrizi, Yi Huang, Francisco Lang, Steven Siems, Michael Manton, Luis Ackermann, Melita Keywood, Ruhi Humphries, Paul Krummel, Alastair Williams, and Greg Ayers
Atmos. Chem. Phys., 25, 2631–2648, https://doi.org/10.5194/acp-25-2631-2025, https://doi.org/10.5194/acp-25-2631-2025, 2025
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Clouds over the Southern Ocean are crucial to Earth's energy balance, but understanding the factors that control them is complex. Our research examines how weather patterns affect tiny particles called cloud condensation nuclei (CCN), which influence cloud properties. Using data from Kennaook / Cape Grim, we found that winter air from Antarctica brings cleaner conditions with lower CCN, while summer patterns from Australia transport more particles. Precipitation also helps reduce CCN in winter.
Hengjia Ou, Mingfu Cai, Yongyun Zhang, Xue Ni, Baoling Liang, Qibin Sun, Shixin Mai, Cuizhi Sun, Shengzhen Zhou, Haichao Wang, Jiaren Sun, and Jun Zhao
Atmos. Chem. Phys., 25, 2495–2513, https://doi.org/10.5194/acp-25-2495-2025, https://doi.org/10.5194/acp-25-2495-2025, 2025
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Two shipborne observations in the South China Sea (SCS) in summer and winter 2021 were conducted. Our study found aerosol hygroscopicity is higher in the SCS in summer than winter, with significant influences from various terrestrial air masses. Aerosol size distribution had a stronger effect on activation ratio than aerosol hygroscopicity in summer and vice versa in winter. Our study provides valuable information to enhance our understanding of cloud condensation nuclei activities in the SCS.
Tinghan Zhang, Ximeng Qi, Janne Lampilahti, Liangduo Chen, Xuguang Chi, Wei Nie, Xin Huang, Zehao Zou, Wei Du, Tom Kokkonen, Tuukka Petäjä, Katrianne Lehtipalo, Veli-Matti Kerminen, Aijun Ding, and Markku Kulmala
EGUsphere, https://doi.org/10.5194/egusphere-2024-3370, https://doi.org/10.5194/egusphere-2024-3370, 2025
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By comparing air ions at two “flagship” sites —the SMEAR II site in the boreal forest of Finland and the SORPES site in a megacity in eastern China—we characterized ion concentrations and their roles in new particle formation (NPF) across contrasting environments. The ion-induced fraction was much higher in clean areas. However, earlier activation of charged particles and high ion-induced fraction during quiet NPF at SORPES imply a non-negligible role for ion-induced NPF in polluted areas.
Jinghao Zhai, Yin Zhang, Pengfei Liu, Yujie Zhang, Antai Zhang, Yaling Zeng, Baohua Cai, Jingyi Zhang, Chunbo Xing, Honglong Yang, Xiaofei Wang, Jianhuai Ye, Chen Wang, Tzung-May Fu, Lei Zhu, Huizhong Shen, Shu Tao, and Xin Yang
EGUsphere, https://doi.org/10.5194/egusphere-2025-463, https://doi.org/10.5194/egusphere-2025-463, 2025
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Our findings show that BrC's optical properties vary by source. Secondary BrC from ozone pollution had the lowest absorption but highest wavelength dependence, while BrC from biomass combustion had the highest absorption with the lowest wavelength dependence. Molecular analysis indicated that CHON species from biomass burning had the strongest light absorption. These insights enhance the accuracy of climate models by highlighting source-specific optical properties of BrC.
Irena Ježek Brecelj, Asta Gregorič, Lucijan Zgonik, Tjaša Rutar, Matic Ivančič, Balint Alfoldy, Griša Močnik, and Martin Rigler
EGUsphere, https://doi.org/10.5194/egusphere-2024-3553, https://doi.org/10.5194/egusphere-2024-3553, 2025
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Following a major car industry scandal involving diesel emissions tests, Europe introduced new testing procedures. However, concerns remained about their effectiveness. Our independent study examined real-world vehicle emissions and revealed encouraging findings: modern diesel cars perform as well as, or even better than, gasoline cars in terms of nitrogen oxides emissions. We found the same pattern for soot particles, challenging common perceptions about diesel's environmental impact.
Bighnaraj Sarangi, Darrel Baumgardner, Ana Isabel Calvo, Benjamin Bolaños-Rosero, Roberto Fraile, Alberto Rodríguez-Fernández, Delia Fernández-González, Carlos Blanco-Alegre, Cátia Gonçalves, Estela D. Vicente, and Olga L. Mayol-Bracero
Atmos. Chem. Phys., 25, 843–865, https://doi.org/10.5194/acp-25-843-2025, https://doi.org/10.5194/acp-25-843-2025, 2025
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Measurements of fluorescing aerosol particle properties have been made during two major African dust events, one over the island of Puerto Rico and the other over the city of León, Spain. The measurements were made with two wideband integrated bioaerosol spectrometers. A significant change in the background aerosol properties, at both locations, is observed when the dust is in the respective regions.
Lijing Chen, Lei Zhang, Yong She, Zhaoliang Zeng, Yu Zheng, Biao Tian, Wenqian Zhang, Zhaohui Liu, Huizheng Che, and Minghu Ding
Atmos. Chem. Phys., 25, 727–739, https://doi.org/10.5194/acp-25-727-2025, https://doi.org/10.5194/acp-25-727-2025, 2025
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Aerosol optical depth (AOD) at Zhongshan Station varies seasonally, with lower values in summer and higher values in winter. Winter and spring AOD increases due to reduced fine-mode particles, while summer and autumn increases are linked to particle growth. Diurnal AOD variation correlates positively with temperature but negatively with wind speed and humidity. Backward trajectories show that aerosols on high-AOD (low-AOD) days primarily originate from the ocean (interior Antarctica).
Shravan Deshmukh, Laurent Poulain, Birgit Wehner, Silvia Henning, Jean-Eudes Petit, Pauline Fombelle, Olivier Favez, Hartmut Herrmann, and Mira Pöhlker
Atmos. Chem. Phys., 25, 741–758, https://doi.org/10.5194/acp-25-741-2025, https://doi.org/10.5194/acp-25-741-2025, 2025
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Aerosol hygroscopicity has been investigated at a sub-urban site in Paris; analysis shows the sub-saturated regime's measured hygroscopicity and the chemically derived hygroscopic growth, shedding light on the large effect of external particle mixing and its influence on predicting hygroscopicity.
Takeshi Kinase, Fumikazu Taketani, Masayuki Takigawa, Chunmao Zhu, Yongwon Kim, Petr Mordovskoi, and Yugo Kanaya
Atmos. Chem. Phys., 25, 143–156, https://doi.org/10.5194/acp-25-143-2025, https://doi.org/10.5194/acp-25-143-2025, 2025
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Boreal forest wildfires in interior Alaska represent an important black carbon (BC) source for the Arctic and surrounding regions. We observed BC and carbon monoxide (CO) concentrations in the Poker Flat Research Range since 2016 and found a positive correlation between the observed BC / ∆CO ratio and fire radiative power (FRP) observed in Alaska and Canada. Our finding suggests the BC emission factor and/or inventory could be potentially improved by using FRP.
Meredith Dournaux, Pierre Tulet, Joris Pianezze, Jérome Brioude, Jean-Marc Metzger, and Melilotus Thyssen
EGUsphere, https://doi.org/10.5194/egusphere-2024-3747, https://doi.org/10.5194/egusphere-2024-3747, 2025
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Aerosol measurements collected during six oceanographic campaigns carried out in 2021 and 2023 in the southwest Indian Ocean are presented and analyzed in this paper. The results highlight a large variability in the aerosol concentration, size and water vapor affinity depending on in-situ conditions and air mass transport over the ocean. Marine aerosol chemical composition is highly variable over this region, and should be considered to better study their impacts on regional weather and climate.
Erin N. Raif, Sarah L. Barr, Mark D. Tarn, James B. McQuaid, Martin I. Daily, Steven J. Abel, Paul A. Barrett, Keith N. Bower, Paul R. Field, Kenneth S. Carslaw, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 14045–14072, https://doi.org/10.5194/acp-24-14045-2024, https://doi.org/10.5194/acp-24-14045-2024, 2024
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Ice-nucleating particles (INPs) allow ice to form in clouds at temperatures warmer than −35°C. We measured INP concentrations over the Norwegian and Barents seas in weather events where cold air is ejected from the Arctic. These concentrations were among the highest measured in the Arctic. It is likely that the INPs were transported to the Arctic from distant regions. These results show it is important to consider hemispheric-scale INP processes to understand INP concentrations in the Arctic.
Fernando Rejano, Andrea Casans, Marta Via, Juan Andrés Casquero-Vera, Sonia Castillo, Hassan Lyamani, Alberto Cazorla, Elisabeth Andrews, Daniel Pérez-Ramírez, Andrés Alastuey, Francisco Javier Gómez-Moreno, Lucas Alados-Arboledas, Francisco José Olmo, and Gloria Titos
Atmos. Chem. Phys., 24, 13865–13888, https://doi.org/10.5194/acp-24-13865-2024, https://doi.org/10.5194/acp-24-13865-2024, 2024
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This study provides valuable insights to improve cloud condensation nuclei (CCN) estimations at a high-altitude remote site which is influenced by nearby urban pollution. Understanding the factors that affect CCN estimations is essential to improve the CCN data coverage worldwide and assess aerosol–cloud interactions on a global scale. This is crucial for improving climate models, since aerosol–cloud interactions are the most important source of uncertainty in climate projections.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Junying Sun, Ye Kuang, Paola Formenti, and Steven G. Howell
Atmos. Chem. Phys., 24, 13849–13864, https://doi.org/10.5194/acp-24-13849-2024, https://doi.org/10.5194/acp-24-13849-2024, 2024
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Using airborne measurements over the southeast Atlantic Ocean, we examined how much moisture aerosols take up during Africa’s biomass burning season. Our study revealed the important role of organic aerosols and introduced a predictive model for moisture uptake, accounting for organics, sulfate, and black carbon, summarizing results from various campaigns. These findings improve our understanding of aerosol–moisture interactions and their radiative effects in this climatically critical region.
Mary C. Robinson, Kaitlin Schueth, and Karin Ardon-Dryer
Atmos. Chem. Phys., 24, 13733–13750, https://doi.org/10.5194/acp-24-13733-2024, https://doi.org/10.5194/acp-24-13733-2024, 2024
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On 26 February 2023, New Mexico and West Texas were impacted by a severe dust storm. To analyze this storm, 28 meteorological stations and 19 PM2.5 and PM10 stations were used. Dust particles were in the air for 16 h, and dust storm conditions lasted for up to 120 min. Hourly PM2.5 and PM10 concentrations were up to 518 and 9983 µg m−3, respectively. For Lubbock, Texas, the maximum PM2.5 concentrations were the highest ever recorded.
Jerome D. Fast, Adam C. Varble, Fan Mei, Mikhail Pekour, Jason Tomlinson, Alla Zelenyuk, Art J. Sedlacek III, Maria Zawadowicz, and Louisa Emmons
Atmos. Chem. Phys., 24, 13477–13502, https://doi.org/10.5194/acp-24-13477-2024, https://doi.org/10.5194/acp-24-13477-2024, 2024
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Aerosol property measurements recently collected on the ground and by a research aircraft in central Argentina during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) campaign exhibit large spatial and temporal variability. These measurements coupled with coincident meteorological information provide a valuable data set needed to evaluate and improve model predictions of aerosols in a traditionally data-sparse region of South America.
Yifan Yang, Thomas Müller, Laurent Poulain, Samira Atabakhsh, Bruna A. Holanda, Jens Voigtländer, Shubhi Arora, and Mira L. Pöhlker
EGUsphere, https://doi.org/10.5194/egusphere-2024-3539, https://doi.org/10.5194/egusphere-2024-3539, 2024
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Black carbon (BC) is the major atmospheric aerosol that can absorb light and influence climate. We measured the physical properties of BC at a background site in Germany. In summer, BC particles were smaller and the mixture with other atmospheric components occurred during the daytime. In winter, emissions from residential heating significantly influenced BC's properties. Understanding these characteristics of BC can help improve aerosol optics simulation accuracy.
Julika Zinke, Gabriel Pereira Freitas, Rachel Ann Foster, Paul Zieger, Ernst Douglas Nilsson, Piotr Markuszewski, and Matthew Edward Salter
Atmos. Chem. Phys., 24, 13413–13428, https://doi.org/10.5194/acp-24-13413-2024, https://doi.org/10.5194/acp-24-13413-2024, 2024
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Bioaerosols, which can influence climate and human health, were studied in the Baltic Sea. In May and August 2021, we used a sea spray simulation chamber during two ship-based campaigns to collect and measure these aerosols. We found that microbes were enriched in air compared to seawater. Bacterial diversity was analysed using DNA sequencing. Our methods provided consistent estimates of microbial emission fluxes, aligning with previous studies.
Chimurkar Navinya, Taveen Singh Kapoor, Gupta Anurag, Chandra Venkataraman, Harish C. Phuleria, and Rajan K. Chakrabarty
Atmos. Chem. Phys., 24, 13285–13297, https://doi.org/10.5194/acp-24-13285-2024, https://doi.org/10.5194/acp-24-13285-2024, 2024
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Brown carbon (BrC) aerosols show an order-of-magnitude variation in their light absorption strength. Our understanding of BrC from real-world biomass burning remains limited, complicating the determination of its radiative impact. Our study reports absorption properties of BrC emitted from four major biomass burning sources using field measurements in India. It develops an absorption parameterization for BrC and examines the spatial variability in BrC's absorption strength across India.
Olga B. Popovicheva, Marina A. Chichaeva, Nikolaos Evangeliou, Sabine Eckhardt, Evangelia Diapouli, and Nikolay S. Kasimov
EGUsphere, https://doi.org/10.5194/egusphere-2024-3124, https://doi.org/10.5194/egusphere-2024-3124, 2024
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High-quality measurements of light-absorbing carbon were performed at the polar aerosol station "Island Bely” (Western Siberian Arctic) from 2019 to 2022. The maximum light absorption coefficients were seen in summer due to gas flaring contribution, which is the most significant source in the region. However, the increasing Siberian wildfires had a special share in carbon contribution to this high Arctic station with a persistent smoke layer extending over the whole troposphere in summer.
Rafael Stern, Joel F. de Brito, Samara Carbone, Luciana Varanda Rizzo, Jonathan Daniel Muller, and Paulo Artaxo
EGUsphere, https://doi.org/10.5194/egusphere-2024-3339, https://doi.org/10.5194/egusphere-2024-3339, 2024
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Our work reveals the impact of forest fires on climate. We found that particles related to direct emissions from fires, beyond the well-known effect of absorbing light and thus heating the atmosphere, are also very efficient in scattering light, which causes an atmospheric cooling effect. In our remote study site, most of the particles presented a different chemical composition then particles directly emitted by the fires, but those were the main responsible for total light extinction.
Sami D. Harni, Minna Aurela, Sanna Saarikoski, Jarkko V. Niemi, Harri Portin, Hanna Manninen, Ville Leinonen, Pasi Aalto, Phil K. Hopke, Tuukka Petäjä, Topi Rönkkö, and Hilkka Timonen
Atmos. Chem. Phys., 24, 12143–12160, https://doi.org/10.5194/acp-24-12143-2024, https://doi.org/10.5194/acp-24-12143-2024, 2024
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In this study, particle number size distribution data were used in a novel way in positive matrix factorization analysis to find aerosol source profiles in the area. Measurements were made in Helsinki at a street canyon and urban background sites between February 2015 and June 2019. Five different aerosol sources were identified. These sources underline the significance of traffic-related emissions in urban environments despite recent improvements in emission reduction technologies.
Natalie G. Ratcliffe, Claire L. Ryder, Nicolas Bellouin, Stephanie Woodward, Anthony Jones, Ben Johnson, Lisa-Maria Wieland, Maximilian Dollner, Josef Gasteiger, and Bernadett Weinzierl
Atmos. Chem. Phys., 24, 12161–12181, https://doi.org/10.5194/acp-24-12161-2024, https://doi.org/10.5194/acp-24-12161-2024, 2024
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Large mineral dust particles are more abundant in the atmosphere than expected and have different impacts on the environment than small particles, which are better represented in climate models. We use aircraft measurements to assess a climate model representation of large-dust transport. We find that the model underestimates the amount of large dust at all stages of transport and that fast removal of the large particles increases this underestimation with distance from the Sahara.
Sergio Rodríguez and Jessica López-Darias
Atmos. Chem. Phys., 24, 12031–12053, https://doi.org/10.5194/acp-24-12031-2024, https://doi.org/10.5194/acp-24-12031-2024, 2024
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Extreme Saharan dust events expanded northward to the Atlantic and Europe, prompting record-breaking PM10 and PM2.5 events. These episodes are caused by low-to-high dipole meteorology during hemispheric anomalies characterized by subtropical anticyclones shifting to higher latitudes, anomalous low pressures beyond the tropics and amplified Rossby waves. Extreme dust events occur in a paradoxical context of a multidecadal decrease in dust emissions, a topic that requires further investigation.
Valeria Mardoñez-Balderrama, Griša Močnik, Marco Pandolfi, Robin L. Modini, Fernando Velarde, Laura Renzi, Angela Marinoni, Jean-Luc Jaffrezo, Isabel Moreno R., Diego Aliaga, Federico Bianchi, Claudia Mohr, Martin Gysel-Beer, Patrick Ginot, Radovan Krejci, Alfred Wiedensohler, Gaëlle Uzu, Marcos Andrade, and Paolo Laj
Atmos. Chem. Phys., 24, 12055–12077, https://doi.org/10.5194/acp-24-12055-2024, https://doi.org/10.5194/acp-24-12055-2024, 2024
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Levels of black carbon (BC) are scarcely reported in the Southern Hemisphere, especially in high-altitude conditions. This study provides insight into the concentration level, variability, and optical properties of BC in La Paz and El Alto and at the Chacaltaya Global Atmosphere Watch Station. Two methods of source apportionment of absorption were tested and compared showing traffic as the main contributor to absorption in the urban area, in addition to biomass and open waste burning.
Krishnakant Budhavant, Mohanan Remani Manoj, Hari Ram Chandrika Rajendran Nair, Samuel Mwaniki Gaita, Henry Holmstrand, Abdus Salam, Ahmed Muslim, Sreedharan Krishnakumari Satheesh, and Örjan Gustafsson
Atmos. Chem. Phys., 24, 11911–11925, https://doi.org/10.5194/acp-24-11911-2024, https://doi.org/10.5194/acp-24-11911-2024, 2024
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The South Asian Pollution Experiment 2018 used access to three strategically located receptor observatories. Observational constraints revealed opposing trends in the mass absorption cross sections of black carbon (BC MAC) and brown carbon (BrC MAC) during long-range transport. Models estimating the climate effects of BC aerosols may have underestimated the ambient BC MAC over distant receptor areas, leading to discrepancies in aerosol absorption predicted by observation-constrained models.
Abigail S. Williams, Jeramy L. Dedrick, Lynn M. Russell, Florian Tornow, Israel Silber, Ann M. Fridlind, Benjamin Swanson, Paul J. DeMott, Paul Zieger, and Radovan Krejci
Atmos. Chem. Phys., 24, 11791–11805, https://doi.org/10.5194/acp-24-11791-2024, https://doi.org/10.5194/acp-24-11791-2024, 2024
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The measured aerosol size distribution modes reveal distinct properties characteristic of cold-air outbreaks in the Norwegian Arctic. We find higher sea spray number concentrations, smaller Hoppel minima, lower effective supersaturations, and accumulation-mode particle scavenging during cold-air outbreaks. These results advance our understanding of cold-air outbreak aerosol–cloud interactions in order to improve their accurate representation in models.
Franziska Vogel, Michael P. Adams, Larissa Lacher, Polly B. Foster, Grace C. E. Porter, Barbara Bertozzi, Kristina Höhler, Julia Schneider, Tobias Schorr, Nsikanabasi S. Umo, Jens Nadolny, Zoé Brasseur, Paavo Heikkilä, Erik S. Thomson, Nicole Büttner, Martin I. Daily, Romy Fösig, Alexander D. Harrison, Jorma Keskinen, Ulrike Proske, Jonathan Duplissy, Markku Kulmala, Tuukka Petäjä, Ottmar Möhler, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 11737–11757, https://doi.org/10.5194/acp-24-11737-2024, https://doi.org/10.5194/acp-24-11737-2024, 2024
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Primary ice formation in clouds strongly influences their properties; hence, it is important to understand the sources of ice-nucleating particles (INPs) and their variability. We present 2 months of INP measurements in a Finnish boreal forest using a new semi-autonomous INP counting device based on gas expansion. These results show strong variability in INP concentrations, and we present a case that the INPs we observe are, at least some of the time, of biological origin.
Rebecca Dischl, Daniel Sauer, Christiane Voigt, Theresa Harlaß, Felicitas Sakellariou, Raphael Märkl, Ulrich Schumann, Monika Scheibe, Stefan Kaufmann, Anke Roiger, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Mark Johnson, Denise Ahrens, Reetu Sallinen, Tobias Schripp, Georg Eckel, Uwe Bauder, and Patrick Le Clercq
Atmos. Chem. Phys., 24, 11255–11273, https://doi.org/10.5194/acp-24-11255-2024, https://doi.org/10.5194/acp-24-11255-2024, 2024
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In-flight measurements of aircraft emissions burning 100 % sustainable aviation fuel (SAF) show reduced particle number concentrations up to 41 % compared to conventional jet fuel. Particle emissions are dependent on engine power setting, flight altitude, and fuel composition. Engine models show a good correlation with measurement results. Future increased prevalence of SAF can positively influence the climate impact of aviation.
Zoé Brasseur, Julia Schneider, Janne Lampilahti, Ville Vakkari, Victoria A. Sinclair, Christina J. Williamson, Carlton Xavier, Dmitri Moisseev, Markus Hartmann, Pyry Poutanen, Markus Lampimäki, Markku Kulmala, Tuukka Petäjä, Katrianne Lehtipalo, Erik S. Thomson, Kristina Höhler, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 24, 11305–11332, https://doi.org/10.5194/acp-24-11305-2024, https://doi.org/10.5194/acp-24-11305-2024, 2024
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Ice-nucleating particles (INPs) strongly influence the formation of clouds by initiating the formation of ice crystals. However, very little is known about the vertical distribution of INPs in the atmosphere. Here, we present aircraft measurements of INP concentrations above the Finnish boreal forest. Results show that near-surface INPs are efficiently transported and mixed within the boundary layer and occasionally reach the free troposphere.
Piotr Markuszewski, E. Douglas Nilsson, Julika Zinke, E. Monica Mårtensson, Matthew Salter, Przemysław Makuch, Małgorzata Kitowska, Iwona Niedźwiecka-Wróbel, Violetta Drozdowska, Dominik Lis, Tomasz Petelski, Luca Ferrero, and Jacek Piskozub
Atmos. Chem. Phys., 24, 11227–11253, https://doi.org/10.5194/acp-24-11227-2024, https://doi.org/10.5194/acp-24-11227-2024, 2024
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Our research provides new insights into the study of sea spray aerosol (SSA) emissions in the Baltic Sea and North Atlantic. We observed that SSA flux is suppressed during increased marine biological activity in the Baltic Sea. At the same time, the influence of wave age showed higher SSA emissions in the Baltic Sea for younger waves compared to the Atlantic Ocean. These insights underscore the complex interplay between biological activity and physical dynamics in regulating SSA emissions.
Heather Guy, Andrew S. Martin, Erik Olson, Ian M. Brooks, and Ryan R. Neely III
Atmos. Chem. Phys., 24, 11103–11114, https://doi.org/10.5194/acp-24-11103-2024, https://doi.org/10.5194/acp-24-11103-2024, 2024
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Aerosol particles impact cloud properties which influence Greenland Ice Sheet melt. Understanding the aerosol population that interacts with clouds is important for constraining future melt. Measurements of aerosols at cloud height over Greenland are rare, and surface measurements are often used to investigate cloud–aerosol interactions. We use a tethered balloon to measure aerosols up to cloud base and show that surface measurements are often not equivalent to those just below the cloud.
Kouji Adachi, Jack E. Dibb, Joseph M. Katich, Joshua P. Schwarz, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Jeff Peischl, Christopher D. Holmes, and James Crawford
Atmos. Chem. Phys., 24, 10985–11004, https://doi.org/10.5194/acp-24-10985-2024, https://doi.org/10.5194/acp-24-10985-2024, 2024
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We examined aerosol particles from wildfires and identified tarballs (TBs) from the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) campaign. This study reveals the compositions, abundance, sizes, and mixing states of TBs and shows that TBs formed as the smoke aged for up to 5 h. This study provides measurements of TBs from various biomass-burning events and ages, enhancing our knowledge of TB emissions and our understanding of their climate impact.
Jia Sun, Markus Hermann, Kay Weinhold, Maik Merkel, Wolfram Birmili, Yifan Yang, Thomas Tuch, Harald Flentje, Björn Briel, Ludwig Ries, Cedric Couret, Michael Elsasser, Ralf Sohmer, Klaus Wirtz, Frank Meinhardt, Maik Schütze, Olaf Bath, Bryan Hellack, Veli-Matti Kerminen, Markku Kulmala, Nan Ma, and Alfred Wiedensohler
Atmos. Chem. Phys., 24, 10667–10687, https://doi.org/10.5194/acp-24-10667-2024, https://doi.org/10.5194/acp-24-10667-2024, 2024
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We investigated the characteristics of new particle formation (NPF) for various environments from urban background to high Alpine and the impacts of NPF on cloud condensation nuclei and aerosol radiative forcing. NPF features differ between site categories, implying the crucial role of local environmental factors such as the degree of emissions and meteorological conditions. The results also underscore the importance of local environments when assessing the impact of NPF on climate in models.
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Short summary
This study investigated the ambient PM2.5 variations over Wuhan, a typical urban Yangtze River middle basin (YRMB) region in central eastern China in January 2016. Through an analysis of observational data of the environment and meteorology, as well as via a FLEXPART-WRF simulation, it heavy air pollution is revealed with the unique “non-stagnant” atmospheric boundary layer in the YRMB region aggravated by regional transport of PM2.5 over central and eastern China.
This study investigated the ambient PM2.5 variations over Wuhan, a typical urban Yangtze River...
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