Articles | Volume 11, issue 15
https://doi.org/10.5194/acp-11-7561-2011
© Author(s) 2011. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-11-7561-2011
© Author(s) 2011. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
01 Aug 2011
Research article |
| 01 Aug 2011
Absorbing aerosol in the troposphere of the Western Arctic during the 2008 ARCTAS/ARCPAC airborne field campaigns
C. S. McNaughton
School of Ocean and Earth Science and Technology, University of Hawaii, Honolulu, HI, USA
A. D. Clarke
School of Ocean and Earth Science and Technology, University of Hawaii, Honolulu, HI, USA
S. Freitag
School of Ocean and Earth Science and Technology, University of Hawaii, Honolulu, HI, USA
V. N. Kapustin
School of Ocean and Earth Science and Technology, University of Hawaii, Honolulu, HI, USA
Y. Kondo
Research Center for Advanced Science and Technology, University of Tokyo, Tokyo, Japan
N. Moteki
Research Center for Advanced Science and Technology, University of Tokyo, Tokyo, Japan
L. Sahu
Research Center for Advanced Science and Technology, University of Tokyo, Tokyo, Japan
N. Takegawa
Research Center for Advanced Science and Technology, University of Tokyo, Tokyo, Japan
J. P. Schwarz
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
J. R. Spackman
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
L. Watts
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
G. Diskin
NASA Langley Research Center, Hampton, VA, USA
J. Podolske
NASA Ames Research Center, Moffett Field, CA, USA
J. S. Holloway
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
A. Wisthaler
Institute of Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
T. Mikoviny
Institute of Ion Physics and Applied Physics, University of Innsbruck, Innsbruck, Austria
J. de Gouw
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
C. Warneke
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
Cooperative Institute for Research in Environmental Sciences (CIRES) University of Colorado, Boulder, CO, USA
J. Jimenez
Cooperative Institute for Research in Environmental Sciences (CIRES) University of Colorado, Boulder, CO, USA
M. Cubison
Cooperative Institute for Research in Environmental Sciences (CIRES) University of Colorado, Boulder, CO, USA
S. G. Howell
School of Ocean and Earth Science and Technology, University of Hawaii, Honolulu, HI, USA
A. Middlebrook
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
R. Bahreini
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
B. E. Anderson
NASA Langley Research Center, Hampton, VA, USA
E. Winstead
NASA Langley Research Center, Hampton, VA, USA
K. L. Thornhill
NASA Langley Research Center, Hampton, VA, USA
D. Lack
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
J. Cozic
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
C. A. Brock
Chemical Sciences Division, NOAA Earth System Research Laboratory, Boulder, CO, USA
Related subject area
Subject: Aerosols | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Measurement report: Contribution of atmospheric new particle formation to ultrafine particle concentration, cloud condensation nuclei, and radiative forcing – results from 5-year observations in central Europe
Simulated contrail-processed aviation soot aerosols are poor ice-nucleating particles at cirrus temperatures
Biological and dust aerosols as sources of ice-nucleating particles in the eastern Mediterranean: source apportionment, atmospheric processing and parameterization
Quantifying the dust direct radiative effect in the southwestern United States: findings from multiyear measurements
How horizontal transport and turbulent mixing impact aerosol particle and precursor concentrations at a background site in the UAE
Markedly different impacts of primary emissions and secondary aerosol formation on aerosol mixing states revealed by simultaneous measurements of CCNC, H(/V)TDMA, and SP2
Vertically resolved aerosol variability at the Amazon Tall Tower Observatory under wet-season conditions
Vertical structure of a springtime smoky and humid troposphere over the southeast Atlantic from aircraft and reanalysis
Multi-year gradient measurements of sea spray fluxes over the Baltic Sea and the North Atlantic Ocean
Shipborne observations of black carbon aerosols in the western Arctic Ocean during summer and autumn 2016–2020: impact of boreal fires
Attribution of aerosol particle number size distributions to main sources using an 11-year urban dataset
Contribution of fluorescent primary biological aerosol particles to low-level Arctic cloud residuals
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Measurement report: A comparison of ground-level ice-nucleating-particle abundance and aerosol properties during autumn at contrasting marine and terrestrial locations
Vertical distribution of ice nucleating particles over the boreal forest of Hyytiälä, Finland
Efficient droplet activation of ambient black carbon particles in a suburban environment
Tropospheric sulfate from Cumbre Vieja (La Palma) observed over Cabo Verde contrasted with background conditions: a lidar case study of aerosol extinction, backscatter, depolarization and lidar ratio profiles at 355, 532 and 1064 nm
Measurements of particle emissions of an A350-941 burning 100 % sustainable aviation fuels in cruise
Occurrence, abundance, and formation of atmospheric tarballs from a wide range of wildfires in the western US
The radiative impact of biomass burning aerosols on dust emissions over Namibia and the long-range transport of smoke observed during the Aerosols, Radiation and Clouds in southern Africa (AEROCLO-sA) campaign
Ice-nucleating particles active below -24 °C in a Finnish boreal forest and their relationship to bioaerosols
Atmospheric Black Carbon in the metropolitan area of La Paz and El Alto, Bolivia: concentration levels and emission sources
Extending the wind profile beyond the surface layer by combining physical and machine learning approaches
Aerosol Size Distribution Properties Associated with Cold-Air Outbreaks in the Norwegian Arctic
Amazonian aerosol size distributions in a lognormal phase space: characteristics and trajectories
Long range transport of coarse mineral dust: an evaluation of the Met Office Unified Model against aircraft observations
Measurement report: Hygroscopicity of size-selected aerosol particles in the heavily polluted urban atmosphere of Delhi: impacts of chloride aerosol
Measurement report: In-situ vertical profiles of below-cloud aerosol over the central Greenland Ice Sheet
An observation-constrained estimation of brown carbon aerosol direct radiative effects
The Puy de Dôme ICe Nucleation Intercomparison Campaign (PICNIC): comparison between online and offline methods in ambient air
Optical properties and simple forcing efficiency of the organic aerosols and black carbon emitted by residential wood burning in rural central Europe
Particle phase state and aerosol liquid water greatly impact secondary aerosol formation: insights into phase transition and its role in haze events
Emerging extreme Saharan-dust events expand northward over the Atlantic and Europe prompting record-breaking PM10 and PM2.5 episodes
Measurement report: Nocturnal subsidence behind the cold front enhances surface particulate matter in plains regions: observations from the mobile multi-lidar system
Increase in precipitation scavenging contributes to long-term reductions of light-absorbing aerosol in the Arctic
Sea spray emissions from the Baltic Sea: comparison of aerosol eddy covariance fluxes and chamber-simulated sea spray emissions
Higher absorption enhancement of black carbon in summer shown by 2-year measurements at the high-altitude mountain site of Pic du Midi Observatory in the French Pyrenees
Variations of the atmospheric polycyclic aromatic hydrocarbon concentrations, sources, and health risk and the direct medical costs of lung cancer around the Bohai Sea against a background of pollution prevention and control in China
Characterization of aerosol over the Eastern Mediterranean by polarization sensitive Raman lidar measurements during A-LIFE – aerosol type classification and type separation
Changing optical properties of Black Carbon and Brown Carbon aerosols during long-range transport from the Indo-Gangetic Plain to the equatorial Indian Ocean
Introducing the novel concept of cumulative concentration roses for studying the transport of ultrafine particles from an airport to adjacent residential areas
Significant spatial gradients in new particle formation frequency in Greece during summer
Impact of desert dust on new particle formation events and the cloud condensation nuclei budget in dust-influenced areas
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Examining the vertical heterogeneity of aerosols over the Southern Great Plains
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Aerosol absorption using in situ filter-based photometers and ground-based sun photometry in the Po Valley urban atmosphere
Aerosol and dynamical contributions to cloud droplet formation in Arctic low-level clouds
Jia Sun, Markus Hermann, Kay Weinhold, Maik Merkel, Wolfram Birmili, Yifan Yang, Thomas Tuch, Harald Flentje, Björn Briel, Ludwig Ries, Cedric Couret, Michael Elsasser, Ralf Sohmer, Klaus Wirtz, Frank Meinhardt, Maik Schütze, Olaf Bath, Bryan Hellack, Veli-Matti Kerminen, Markku Kulmala, Nan Ma, and Alfred Wiedensohler
Atmos. Chem. Phys., 24, 10667–10687, https://doi.org/10.5194/acp-24-10667-2024, https://doi.org/10.5194/acp-24-10667-2024, 2024
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We investigated the characteristics of new particle formation (NPF) for various environments from urban background to high Alpine and the impacts of NPF on cloud condensation nuclei and aerosol radiative forcing. NPF features differ between site categories, implying the crucial role of local environmental factors such as the degree of emissions and meteorological conditions. The results also underscore the importance of local environments when assessing the impact of NPF on climate in models.
Baptiste Testa, Lukas Durdina, Jacinta Edebeli, Curdin Spirig, and Zamin A. Kanji
Atmos. Chem. Phys., 24, 10409–10424, https://doi.org/10.5194/acp-24-10409-2024, https://doi.org/10.5194/acp-24-10409-2024, 2024
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Aviation soot residuals released from contrails can become compacted upon sublimation of the ice crystals, generating new voids in the aggregates where ice nucleation can occur. Here we show that contrail-processed soot is highly compact but that it remains unable to form ice at a relative humidity different from that required for the formation of background cirrus from the more ubiquitous aqueous solution droplets, suggesting that it will not perturb cirrus cloud formation via ice nucleation.
Kunfeng Gao, Franziska Vogel, Romanos Foskinis, Stergios Vratolis, Maria I. Gini, Konstantinos Granakis, Anne-Claire Billault-Roux, Paraskevi Georgakaki, Olga Zografou, Prodromos Fetfatzis, Alexis Berne, Alexandros Papayannis, Konstantinos Eleftheridadis, Ottmar Möhler, and Athanasios Nenes
Atmos. Chem. Phys., 24, 9939–9974, https://doi.org/10.5194/acp-24-9939-2024, https://doi.org/10.5194/acp-24-9939-2024, 2024
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Ice nucleating particle (INP) concentrations are required for correct predictions of clouds and precipitation in a changing climate, but they are poorly constrained in climate models. We unravel source contributions to INPs in the eastern Mediterranean and find that biological particles are important, regardless of their origin. The parameterizations developed exhibit superior performance and enable models to consider biological-particle effects on INPs.
Alexandra Kuwano, Amato T. Evan, Blake Walkowiak, and Robert Frouin
Atmos. Chem. Phys., 24, 9843–9868, https://doi.org/10.5194/acp-24-9843-2024, https://doi.org/10.5194/acp-24-9843-2024, 2024
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The dust direct radiative effect is highly uncertain. Here we used new measurements collected over 3 years and during dust storms at a field site in a desert region in the southwestern United States to estimate the regional dust direct radiative effect. We also used novel soil mineralogy retrieved from an airborne spectrometer to estimate this parameter with model output. We find that, in this region, dust has a minimal net cooling effect on this region's climate.
Jutta Kesti, Ewan J. O'Connor, Anne Hirsikko, John Backman, Maria Filioglou, Anu-Maija Sundström, Juha Tonttila, Heikki Lihavainen, Hannele Korhonen, and Eija Asmi
Atmos. Chem. Phys., 24, 9369–9386, https://doi.org/10.5194/acp-24-9369-2024, https://doi.org/10.5194/acp-24-9369-2024, 2024
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The study combines aerosol particle measurements at the surface and vertical profiling of the atmosphere with a scanning Doppler lidar to investigate how particle transportation together with boundary layer evolution can affect particle and SO2 concentrations at the surface in the Arabian Peninsula region. The instrumentation enabled us to see elevated nucleation mode particle and SO2 concentrations at the surface when air masses transported from polluted areas are mixed in the boundary layer.
Jiangchuan Tao, Biao Luo, Weiqi Xu, Gang Zhao, Hanbin Xu, Biao Xue, Miaomiao Zhai, Wanyun Xu, Huarong Zhao, Sanxue Ren, Guangsheng Zhou, Li Liu, Ye Kuang, and Yele Sun
Atmos. Chem. Phys., 24, 9131–9154, https://doi.org/10.5194/acp-24-9131-2024, https://doi.org/10.5194/acp-24-9131-2024, 2024
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Using simultaneous measurements of DMA–CCNC, H(/V)TDMA, and DMA–SP2, impacts of primary emissions and secondary aerosol formations on changes in aerosol physicochemical properties were comprehensively investigated. It was found that intercomparisons among aerosol mixing-state parameters derived from different techniques can help us gain more insight into aerosol physical properties which, in turn, will aid the investigation of emission characteristics and secondary aerosol formation pathways.
Marco A. Franco, Rafael Valiati, Bruna A. Holanda, Bruno B. Meller, Leslie A. Kremper, Luciana V. Rizzo, Samara Carbone, Fernando G. Morais, Janaína P. Nascimento, Meinrat O. Andreae, Micael A. Cecchini, Luiz A. T. Machado, Milena Ponczek, Ulrich Pöschl, David Walter, Christopher Pöhlker, and Paulo Artaxo
Atmos. Chem. Phys., 24, 8751–8770, https://doi.org/10.5194/acp-24-8751-2024, https://doi.org/10.5194/acp-24-8751-2024, 2024
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The Amazon wet-season atmosphere was studied at the Amazon Tall Tower Observatory site, revealing vertical variations (between 60 and 325 m) in natural aerosols. Daytime mixing contrasted with nighttime stratification, with distinct rain-induced changes in aerosol populations. Notably, optical property recovery at higher levels was faster, while near-canopy aerosols showed higher scattering efficiency. These findings enhance our understanding of aerosol impacts on climate dynamics.
Kristina Pistone, Eric M. Wilcox, Paquita Zuidema, Marco Giordano, James Podolske, Samuel E. LeBlanc, Meloë Kacenelenbogen, Steven G. Howell, and Steffen Freitag
Atmos. Chem. Phys., 24, 7983–8005, https://doi.org/10.5194/acp-24-7983-2024, https://doi.org/10.5194/acp-24-7983-2024, 2024
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The springtime southeast Atlantic atmosphere contains lots of smoke from continental fires. This smoke travels with water vapor; more smoke means more humidity. We use aircraft observations and models to describe how the values change through the season and over the region. We sort the atmosphere into different types by vertical structure and amount of smoke and humidity. Since our work shows how frequently these components coincide, it helps to better quantify heating effects over this region.
Piotr Markuszewski, E. Douglas Nilsson, Julika Zinke, E. Monica Mårtensson, Matthew Salter, Przemysław Makuch, Małgorzata Kitowska, Iwona Niedźwiecka-Wróbel, Violetta Drozdowska, Dominik Lis, Tomasz Petelski, Luca Ferrero, and Jacek Piskozub
EGUsphere, https://doi.org/10.5194/egusphere-2024-1254, https://doi.org/10.5194/egusphere-2024-1254, 2024
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Sea spray aerosol whipped up from the sea surface, is an important compound of the atmospheric boundary layer. Our research provides new insights into the study of sea spray emission in the Baltic Sea and North Atlantic. We investigated the impact of environmental factors on sea spray fluxes. We observed that in case of increased marine biological activity in the Baltic Sea, sea spray flux is suppressed. We also observed evidence of sea surface temperature influence on sea spray emission.
Yange Deng, Hiroshi Tanimoto, Kohei Ikeda, Sohiko Kameyama, Sachiko Okamoto, Jinyoung Jung, Young Jun Yoon, Eun Jin Yang, and Sung-Ho Kang
Atmos. Chem. Phys., 24, 6339–6357, https://doi.org/10.5194/acp-24-6339-2024, https://doi.org/10.5194/acp-24-6339-2024, 2024
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Black carbon (BC) aerosols play important roles in Arctic climate change, yet they are not well understood because of limited observational data. We observed BC mass concentrations (mBC) in the western Arctic Ocean during summer and early autumn 2016–2020. The mean mBC in 2019 was much higher than in other years. Biomass burning was likely the dominant BC source. Boreal fire BC transport occurring near the surface and/or in the mid-troposphere contributed to high-BC events in the Arctic Ocean.
Máté Vörösmarty, Philip K. Hopke, and Imre Salma
Atmos. Chem. Phys., 24, 5695–5712, https://doi.org/10.5194/acp-24-5695-2024, https://doi.org/10.5194/acp-24-5695-2024, 2024
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The World Health Organization identified ultrafine particles, which make up most of the particle number concentrations, as a potential risk factor for humans. The sources of particle numbers are very different from those of the particulate matter mass. We performed source apportionment of size-segregated particle number concentrations over the diameter range of 6–1000 nm in Budapest for 11 full years. Six source types were identified, characterized and quantified.
Gabriel Pereira Freitas, Ben Kopec, Kouji Adachi, Radovan Krejci, Dominic Heslin-Rees, Karl Espen Yttri, Alun Hubbard, Jeffrey M. Welker, and Paul Zieger
Atmos. Chem. Phys., 24, 5479–5494, https://doi.org/10.5194/acp-24-5479-2024, https://doi.org/10.5194/acp-24-5479-2024, 2024
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Bioaerosols can participate in ice formation within clouds. In the Arctic, where global warming manifests most, they may become more important as their sources prevail for longer periods of the year. We have directly measured bioaerosols within clouds for a full year at an Arctic mountain site using a novel combination of cloud particle sampling and single-particle techniques. We show that bioaerosols act as cloud seeds and may influence the presence of ice within clouds.
Andreas Petzold, Ulrich Bundke, Anca Hienola, Paolo Laj, Cathrine Lund Myhre, Alex Vermeulen, Angeliki Adamaki, Werner Kutsch, Valerie Thouret, Damien Boulanger, Markus Fiebig, Markus Stocker, Zhiming Zhao, and Ari Asmi
Atmos. Chem. Phys., 24, 5369–5388, https://doi.org/10.5194/acp-24-5369-2024, https://doi.org/10.5194/acp-24-5369-2024, 2024
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Easy and fast access to long-term and high-quality observational data is recognised as fundamental to environmental research and the development of climate forecasting and assessment services. We discuss the potential new directions in atmospheric sciences offered by the atmosphere-centric European research infrastructures ACTRIS, IAGOS, and ICOS, building on their capabilities for standardised provision of data through open access combined with tools and methods of data-intensive science.
Elise K. Wilbourn, Larissa Lacher, Carlos Guerrero, Hemanth S. K. Vepuri, Kristina Höhler, Jens Nadolny, Aidan D. Pantoya, Ottmar Möhler, and Naruki Hiranuma
Atmos. Chem. Phys., 24, 5433–5456, https://doi.org/10.5194/acp-24-5433-2024, https://doi.org/10.5194/acp-24-5433-2024, 2024
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Ambient ice particles were measured at terrestrial and temperate marine sites. Ice particles were more abundant in the former site, while the fraction of ice particles relative to total ambient particles, representing atmospheric ice nucleation efficiency, was higher in the latter site. Ice nucleation parameterizations were developed as a function of examined freezing temperatures from two sites for our study periods (autumn).
Zoé Brasseur, Julia Schneider, Janne Lampilahti, Ville Vakkari, Victoria A. Sinclair, Christina J. Williamson, Carlton Xavier, Dmitri Moisseev, Markus Hartmann, Pyry Poutanen, Markus Lampimäki, Markku Kulmala, Tuukka Petäjä, Katrianne Lehtipalo, Erik S. Thomson, Kristina Höhler, Ottmar Möhler, and Jonathan Duplissy
EGUsphere, https://doi.org/10.5194/egusphere-2024-1272, https://doi.org/10.5194/egusphere-2024-1272, 2024
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Ice nucleating particles (INPs) strongly influence the formation of clouds by initiating the formation of ice crystals. However, very little is known concerning the vertical distribution of INPs in the atmosphere. Here, we present aircraft measurements of INP concentrations above the Finnish boreal forest. Results show that near-surface INPs are efficiently transported and mixed within the boundary layer, and occasionally reach the free troposphere.
Ping Tian, Dantong Liu, Kang Hu, Yangzhou Wu, Mengyu Huang, Hui He, Jiujiang Sheng, Chenjie Yu, Dawei Hu, and Deping Ding
Atmos. Chem. Phys., 24, 5149–5164, https://doi.org/10.5194/acp-24-5149-2024, https://doi.org/10.5194/acp-24-5149-2024, 2024
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The results provide direct evidence of efficient droplet activation of black carbon (BC). The cloud condensation nuclei (CCN) activation fraction of BC was higher than for all particles, suggesting higher CCN activity of BC, even though its hygroscopicity is lower. Our research reveals that the evolution of BC's hygroscopicity and its CCN activation properties through atmospheric aging can be effectively characterized by the photochemical age.
Henriette Gebauer, Athena Augusta Floutsi, Moritz Haarig, Martin Radenz, Ronny Engelmann, Dietrich Althausen, Annett Skupin, Albert Ansmann, Cordula Zenk, and Holger Baars
Atmos. Chem. Phys., 24, 5047–5067, https://doi.org/10.5194/acp-24-5047-2024, https://doi.org/10.5194/acp-24-5047-2024, 2024
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Sulfate aerosol from the volcanic eruption at La Palma in 2021 was observed over Cabo Verde. We characterized the aerosol burden based on a case study of lidar and sun photometer observations. We compared the volcanic case to the typical background conditions (reference case) to quantify the volcanic pollution. We show the first ever measurements of the extinction coefficient, lidar ratio and depolarization ratio at 1064 nm for volcanic sulfate.
Rebecca Katharina Dischl, Daniel Sauer, Christiane Voigt, Theresa Harlaß, Felicitas Sakellariou, Raphael Satoru Märkl, Ulrich Schumann, Monika Scheibe, Stefan Kaufmann, Anke Roiger, Andreas Dörnbrack, Charles Renard, Maxime Gauthier, Peter Swann, Paul Madden, Darren Luff, Mark Johnson, Denise Ahrens, Reetu Sallinen, Tobias Schripp, Georg Eckel, Uwe Bauder, and Patrick Le Clercq
EGUsphere, https://doi.org/10.5194/egusphere-2024-1224, https://doi.org/10.5194/egusphere-2024-1224, 2024
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In-flight measurements of aircraft emissions burning 100 % sustainable aviation fuel (SAF) show reduced particle number concentrations up to 41 % compared to conventional jet fuel. Particle emissions are dependent on engine power setting, flight altitude and fuel composition. Engine models show a good correlation with measurement results. Future increased prevalence of SAF can positively influence the climate impact of aviation.
Kouji Adachi, Jack E. Dibb, Joseph M. Katich, Joshua P. Schwarz, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Jeff Peischl, Christopher D. Holmes, and James Crawford
EGUsphere, https://doi.org/10.5194/egusphere-2024-880, https://doi.org/10.5194/egusphere-2024-880, 2024
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We examined aerosol particles from wildfires and identified tarballs (TBs) during the FIREX-AQ campaign. This study revealed the compositions, abundance, sizes, and mixing states of TBs and showed that TBs formed as the smoke aged for up to 5 h. This study provides measurements of TBs from various biomass burning and ages and enhances the knowledge of TB emissions and our understanding of their climate impact.
Cyrille Flamant, Jean-Pierre Chaboureau, Marco Gaetani, Kerstin Schepanski, and Paola Formenti
Atmos. Chem. Phys., 24, 4265–4288, https://doi.org/10.5194/acp-24-4265-2024, https://doi.org/10.5194/acp-24-4265-2024, 2024
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In the austral dry season, the atmospheric composition over southern Africa is dominated by biomass burning aerosols and terrigenous aerosols (so-called mineral dust). This study suggests that the radiative effect of biomass burning aerosols needs to be taken into account to properly forecast dust emissions in Namibia.
Franziska Vogel, Michael P. Adams, Larissa Lacher, Polly Foster, Grace C. E. Porter, Barbara Bertozzi, Kristina Höhler, Julia Schneider, Tobias Schorr, Nsikanabasi S. Umo, Jens Nadolny, Zoé Brasseur, Paavo Heikkilä, Erik S. Thomson, Nicole Büttner, Martin I. Daily, Romy Fösig, Alexander D. Harrison, Jorma Keskinen, Ulrike Proske, Jonathan Duplissy, Markku Kulmala, Tuukka Petäjä, Ottmar Möhler, and Benjamin J. Murray
EGUsphere, https://doi.org/10.5194/egusphere-2024-853, https://doi.org/10.5194/egusphere-2024-853, 2024
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Primary ice formation in clouds strongly influences their properties, hence it is important to understand the sources of ice-nucleating particles (INPs) and their variability. We present 2 months INP measurements in a Finnish boreal forest using a new semi-autonomous INP counting device based on gas expansion. These results show strong variability in INP concentrations, and we present a case that the INP we observe are, at least some of the time, of biological origin.
Valeria Mardoñez-Balderrama, Griša Močnik, Marco Pandolfi, Robin Modini, Fernando Velarde, Laura Renzi, Angela Marinoni, Jean-Luc Jaffrezo, Isabel Moreno R., Diego Aliaga, Federico Bianchi, Claudia Mohr, Martin Gysel-Beer, Patrick Ginot, Radovan Krejci, Alfred Widensohler, Gaëlle Uzu, Marcos Andrade, and Paolo Laj
EGUsphere, https://doi.org/10.5194/egusphere-2024-770, https://doi.org/10.5194/egusphere-2024-770, 2024
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Levels of black carbon (BC) are scarcely reported in the southern hemisphere, especially in high-altitude conditions. This study provides insight on the concentration level, variability, and optical properties of BC in the cities of La Paz and El Alto, and at the station GAW Chacaltaya Mountain station. Two methods of source apportionment of absorption were tested and compared showing traffic as the main contributor to absorption in the urban area, additionally to biomass and open waste burning.
Boming Liu, Xin Ma, Jianping Guo, Renqiang Wen, Hui Li, Shikuan Jin, Yingying Ma, Xiaoran Guo, and Wei Gong
Atmos. Chem. Phys., 24, 4047–4063, https://doi.org/10.5194/acp-24-4047-2024, https://doi.org/10.5194/acp-24-4047-2024, 2024
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Accurate wind profile estimation, especially for the lowest few hundred meters of the atmosphere, is of great significance for the weather, climate, and renewable energy sector. We propose a novel method that combines the power-law method with the random forest algorithm to extend wind profiles beyond the surface layer. Compared with the traditional algorithm, this method has better stability and spatial applicability and can be used to obtain the wind profiles on different land cover types.
Abigail S. Williams, Jeramy L. Dedrick, Lynn M. Russell, Florian Tornow, Israel Silber, Ann M. Fridlind, Benjamin Swanson, Paul J. DeMott, Paul Zieger, and Radovan Krejci
EGUsphere, https://doi.org/10.5194/egusphere-2024-584, https://doi.org/10.5194/egusphere-2024-584, 2024
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The measured aerosol size distribution modes reveal distinct properties characteristic of cold-air outbreaks in the Norwegian Arctic. We find higher sea spray number concentration, smaller Hoppel minima, lower effective supersaturations, and accumulation mode particle scavenging during cold-air outbreaks. These results advance our understanding of cold-air outbreak aerosol-cloud interactions in order to improve their accurate representation in models.
Gabriela R. Unfer, Luiz A. T. Machado, Paulo Artaxo, Marco A. Franco, Leslie A. Kremper, Mira L. Pöhlker, Ulrich Pöschl, and Christopher Pöhlker
Atmos. Chem. Phys., 24, 3869–3882, https://doi.org/10.5194/acp-24-3869-2024, https://doi.org/10.5194/acp-24-3869-2024, 2024
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Amazonian aerosols and their interactions with precipitation were studied by understanding them in a 3D space based on three parameters that characterize the concentration and size distribution of aerosols. The results showed characteristic arrangements regarding seasonal and diurnal cycles, as well as when interacting with precipitation. The use of this 3D space appears to be a promising tool for aerosol population analysis and for model validation and parameterization.
Natalie Georgina Ratcliffe, Claire Louise Ryder, Nicolas Bellouin, Stephanie Woodward, Anthony Jones, Ben Johnson, Bernadett Weinzierl, Lisa-Maria Wieland, and Josef Gasteiger
EGUsphere, https://doi.org/10.5194/egusphere-2024-806, https://doi.org/10.5194/egusphere-2024-806, 2024
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Large mineral dust particles are more abundant in the atmosphere than expected and have different impacts on the environment than small particles, which are better represented in climate models. We use aircraft measurements to assess a climate model representation of large dust transport. We find that the model underestimates the amount of large dust at all stages of transport and that fast removal of the large particles increases this underestimation with distance from the Sahara.
Anil Kumar Mandariya, Ajit Ahlawat, Mohammed Haneef, Nisar Ali Baig, Kanan Patel, Joshua Apte, Lea Hildebrandt Ruiz, Alfred Wiedensohler, and Gazala Habib
Atmos. Chem. Phys., 24, 3627–3647, https://doi.org/10.5194/acp-24-3627-2024, https://doi.org/10.5194/acp-24-3627-2024, 2024
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The current study explores the temporal variation of size-selected particle hygroscopicity in Delhi for the first time. Here, we report that the high volume fraction contribution of ammonium chloride to aerosol governs the high aerosol hygroscopicity and associated liquid water content based on the experimental data. The episodically high ammonium chloride present in Delhi's atmosphere could lead to haze and fog formation under high relative humidity in the region.
Heather Guy, Andrew S. Martin, Erik Olson, Ian M. Brooks, and Ryan R. Neely III
EGUsphere, https://doi.org/10.5194/egusphere-2024-733, https://doi.org/10.5194/egusphere-2024-733, 2024
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Aerosol particles impact cloud properties which influence Greenland Ice Sheet melt. Understanding the aerosol population that interacts with clouds is important for constraining future melt. Measurements of aerosols at cloud height over Greenland are rare, and surface measurements are often used to investigate cloud-aerosol interactions. We use a tethered balloon to measure aerosols up to cloud base and show that surface measurements are often not equivalent to those just below the cloud.
Yueyue Cheng, Chao Liu, Jiandong Wang, Jiaping Wang, Zhouyang Zhang, Li Chen, Dafeng Ge, Caijun Zhu, Jinbo Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 3065–3078, https://doi.org/10.5194/acp-24-3065-2024, https://doi.org/10.5194/acp-24-3065-2024, 2024
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Brown carbon (BrC), a light-absorbing aerosol, plays a pivotal role in influencing global climate. However, assessing BrC radiative effects remains challenging because the required observational data are hardly accessible. Here we develop a new BrC radiative effect estimation method combining conventional observations and numerical models. Our findings reveal that BrC absorbs up to a third of the sunlight at 370 nm that black carbon does, highlighting its importance in aerosol radiative effects.
Larissa Lacher, Michael P. Adams, Kevin Barry, Barbara Bertozzi, Heinz Bingemer, Cristian Boffo, Yannick Bras, Nicole Büttner, Dimitri Castarede, Daniel J. Cziczo, Paul J. DeMott, Romy Fösig, Megan Goodell, Kristina Höhler, Thomas C. J. Hill, Conrad Jentzsch, Luis A. Ladino, Ezra J. T. Levin, Stephan Mertes, Ottmar Möhler, Kathryn A. Moore, Benjamin J. Murray, Jens Nadolny, Tatjana Pfeuffer, David Picard, Carolina Ramírez-Romero, Mickael Ribeiro, Sarah Richter, Jann Schrod, Karine Sellegri, Frank Stratmann, Benjamin E. Swanson, Erik S. Thomson, Heike Wex, Martin J. Wolf, and Evelyn Freney
Atmos. Chem. Phys., 24, 2651–2678, https://doi.org/10.5194/acp-24-2651-2024, https://doi.org/10.5194/acp-24-2651-2024, 2024
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Aerosol particles that trigger ice formation in clouds are important for the climate system but are very rare in the atmosphere, challenging measurement techniques. Here we compare three cloud chambers and seven methods for collecting aerosol particles on filters for offline analysis at a mountaintop station. A general good agreement of the methods was found when sampling aerosol particles behind a whole air inlet, supporting their use for obtaining data that can be implemented in models.
Andrea Cuesta-Mosquera, Kristina Glojek, Griša Močnik, Luka Drinovec, Asta Gregorič, Martin Rigler, Matej Ogrin, Baseerat Romshoo, Kay Weinhold, Maik Merkel, Dominik van Pinxteren, Hartmut Herrmann, Alfred Wiedensohler, Mira Pöhlker, and Thomas Müller
Atmos. Chem. Phys., 24, 2583–2605, https://doi.org/10.5194/acp-24-2583-2024, https://doi.org/10.5194/acp-24-2583-2024, 2024
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This study evaluated the air pollution and climate impacts of residential-wood-burning particle emissions from a rural European site. The authors investigate the optical and physical properties that connect the aerosol emissions with climate by evaluating atmospheric radiative impacts via simple-forcing calculations. The study contributes to reducing the lack of information on the understanding of the optical properties of air pollution from anthropogenic sources.
Xiangxinyue Meng, Zhijun Wu, Jingchuan Chen, Yanting Qiu, Taomou Zong, Mijung Song, Jiyi Lee, and Min Hu
Atmos. Chem. Phys., 24, 2399–2414, https://doi.org/10.5194/acp-24-2399-2024, https://doi.org/10.5194/acp-24-2399-2024, 2024
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Our study revealed that particles predominantly exist in a semi-solid or solid state during clean winter days with RH below 30 %. However, a non-liquid to a liquid phase transition occurred when the aerosol liquid water (ALW) mass fraction surpassed 15 % (dry mass) at transition RH thresholds ranging from 40 % to 60 %. We also provide insights into the increasingly important roles of particle phase state variation and ALW in secondary particulate growth during haze formation in Beijing, China.
Sergio Rodríguez and Jessica López-Darias
EGUsphere, https://doi.org/10.5194/egusphere-2023-3083, https://doi.org/10.5194/egusphere-2023-3083, 2024
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Extreme Saharan-dust events have expanded northward to the Atlantic and Europe, prompting the most intense PM10 and PM2.5 events ever recorded in the governmental air quality network of Spain. The events occurred during hemispheric anomalies characterised by subtropical anticyclones shifted to higher latitudes, anomalous low pressures expanding beyond the tropic and a mid-latitude amplified Rossby-waves undulation, resembling the circulation anomalies due to the anthropogenic global warming.
Yiming Wang, Haolin Wang, Yujie Qin, Xinqi Xu, Guowen He, Nanxi Liu, Shengjie Miao, Xiao Lu, Haichao Wang, and Shaojia Fan
Atmos. Chem. Phys., 24, 2267–2285, https://doi.org/10.5194/acp-24-2267-2024, https://doi.org/10.5194/acp-24-2267-2024, 2024
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We conducted a vertical measurement of winter PM2.5 using a mobile multi-lidar system in four cities. Combined with the surface PM2.5 data, the ERA5 reanalysis data, and GEOS-Chem simulations during Dec 2018–Feb 2019, we found that transport nocturnal PM2.5 enhancement by subsidence (T-NPES) events widely occurred with high frequencies in plains regions in eastern China but happened less often in basin regions like Xi’an and Chengdu. We propose a conceptual model of the T-NPES events.
Dominic Heslin-Rees, Peter Tunved, Johan Ström, Roxana Cremer, Paul Zieger, Ilona Riipinen, Annica M. L. Ekman, Konstantinos Eleftheriadis, and Radovan Krejci
Atmos. Chem. Phys., 24, 2059–2075, https://doi.org/10.5194/acp-24-2059-2024, https://doi.org/10.5194/acp-24-2059-2024, 2024
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Light-absorbing atmospheric particles (e.g. black carbon – BC) exert a warming effect on the Arctic climate. We show that the amount of particle light absorption decreased from 2002 to 2023. We conclude that in addition to reductions in emissions of BC, wet removal plays a role in the long-term reduction of BC in the Arctic, given the increase in surface precipitation experienced by air masses arriving at the site. The potential impact of biomass burning events is shown to have increased.
Julika Zinke, Ernst Douglas Nilsson, Piotr Markuszewski, Paul Zieger, Eva Monica Mårtensson, Anna Rutgersson, Erik Nilsson, and Matthew Edward Salter
Atmos. Chem. Phys., 24, 1895–1918, https://doi.org/10.5194/acp-24-1895-2024, https://doi.org/10.5194/acp-24-1895-2024, 2024
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We conducted two research campaigns in the Baltic Sea, during which we combined laboratory sea spray simulation experiments with flux measurements on a nearby island. To combine these two methods, we scaled the laboratory measurements to the flux measurements using three different approaches. As a result, we derived a parameterization that is dependent on wind speed and wave state for particles with diameters 0.015–10 μm. This parameterization is applicable to low-salinity waters.
Sarah Tinorua, Cyrielle Denjean, Pierre Nabat, Thierry Bourrianne, Véronique Pont, François Gheusi, and Emmanuel Leclerc
Atmos. Chem. Phys., 24, 1801–1824, https://doi.org/10.5194/acp-24-1801-2024, https://doi.org/10.5194/acp-24-1801-2024, 2024
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At a French high-altitude site, where many complex interactions between black carbon (BC), radiation, clouds and snow impact climate, 2 years of refractive BC (rBC) and aerosol optical and microphysical measurements have been made. We observed strong seasonal rBC properties variations, with an enhanced absorption in summer compared to winter. The combination of rBC emission sources, transport pathways, atmospheric dynamics and chemical processes explains the rBC light absorption seasonality.
Wenwen Ma, Rong Sun, Xiaoping Wang, Zheng Zong, Shizhen Zhao, Zeyu Sun, Chongguo Tian, Jianhui Tang, Song Cui, Jun Li, and Gan Zhang
Atmos. Chem. Phys., 24, 1509–1523, https://doi.org/10.5194/acp-24-1509-2024, https://doi.org/10.5194/acp-24-1509-2024, 2024
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This is the first report of long-term atmospheric PAH monitoring around the Bohai Sea. The results showed that the concentrations of PAHs in the atmosphere around the Bohai Sea decreased from June 2014 to May 2019, especially the concentrations of highly toxic PAHs. This indicates that the contributions from PAH sources changed to a certain extent in different areas, and it also led to reductions in the related health risk and medical costs following pollution prevention and control.
Silke Groß, Volker Freudenthaler, Moritz Haarig, Albert Ansmann, Carlos Toledano, David Mateos, Petra Seibert, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Josef Gasteiger, Maximilian Dollner, Anne Tipka, Manuel Schöberl, Marilena Teri, and Bernadett Weinzierl
EGUsphere, https://doi.org/10.5194/egusphere-2024-140, https://doi.org/10.5194/egusphere-2024-140, 2024
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Aerosols contribute to the largest uncertainties in climate change predictions. Especially absorbing aerosols propose difficulties in our understanding. The eastern Mediterranean is a hot spot for aerosols with natural and anthropogenic contributions. We present lidar measurements performed during the A-LIFE field experiment to characterize aerosols and aerosol mixtures. We extend current classification and separation schemes and compare different classification schemes.
Krishnakant Budhavant, Mohanan Remani Manoj, Samuel Mwaniki Gaita, Henry Holmstrand, Abdus Salam, Ahmed Muslim, Sreedharan K. Satheesh, and Orjan Gustafsson
EGUsphere, https://doi.org/10.5194/egusphere-2024-104, https://doi.org/10.5194/egusphere-2024-104, 2024
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The South Asian Pollution Experiment-2018 utilized access to 3 strategically located atmospheric receptor observatories. These observational constraints revealed opposite trends during long-range transport in BC-MAC and BrC-MAC. Models estimating the climate effects of particularly BC aerosols may have underestimated the ambient BC-MAC over distant and extensive receptor areas, which could contribute to the discrepancy between aerosol absorption predicted by models constrained by observations.
Julius Seidler, Markus N. Friedrich, Christoph K. Thomas, and Anke C. Nölscher
Atmos. Chem. Phys., 24, 137–153, https://doi.org/10.5194/acp-24-137-2024, https://doi.org/10.5194/acp-24-137-2024, 2024
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Here, we study the transport of ultrafine particles (UFPs) from an airport to two new adjacent measuring sites for 1 year. The number of UFPs in the air and the diurnal variation are typical urban. Winds from the airport show increased number concentrations. Additionally, considering wind frequencies, we estimate that, from all UFPs measured at the two sites, 10 %–14 % originate from the airport and/or other UFP sources from between the airport and site.
Andreas Aktypis, Christos Kaltsonoudis, David Patoulias, Panayiotis Kalkavouras, Angeliki Matrali, Christina N. Vasilakopoulou, Evangelia Kostenidou, Kalliopi Florou, Nikos Kalivitis, Aikaterini Bougiatioti, Konstantinos Eleftheriadis, Stergios Vratolis, Maria I. Gini, Athanasios Kouras, Constantini Samara, Mihalis Lazaridis, Sofia-Eirini Chatoutsidou, Nikolaos Mihalopoulos, and Spyros N. Pandis
Atmos. Chem. Phys., 24, 65–84, https://doi.org/10.5194/acp-24-65-2024, https://doi.org/10.5194/acp-24-65-2024, 2024
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Extensive continuous particle number size distribution measurements took place during two summers (2020 and 2021) at 11 sites in Greece for the investigation of the frequency and the spatial extent of new particle formation. The frequency during summer varied from close to zero in southwestern Greece to more than 60 % in the northern, central, and eastern regions. The spatial variability can be explained by the proximity of the sites to coal-fired power plants and agricultural areas.
Juan Andrés Casquero-Vera, Daniel Pérez-Ramírez, Hassan Lyamani, Fernando Rejano, Andrea Casans, Gloria Titos, Francisco José Olmo, Lubna Dada, Simo Hakala, Tareq Hussein, Katrianne Lehtipalo, Pauli Paasonen, Antti Hyvärinen, Noemí Pérez, Xavier Querol, Sergio Rodríguez, Nikos Kalivitis, Yenny González, Mansour A. Alghamdi, Veli-Matti Kerminen, Andrés Alastuey, Tuukka Petäjä, and Lucas Alados-Arboledas
Atmos. Chem. Phys., 23, 15795–15814, https://doi.org/10.5194/acp-23-15795-2023, https://doi.org/10.5194/acp-23-15795-2023, 2023
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Here we present the first study of the effect of mineral dust on the inhibition/promotion of new particle formation (NPF) events in different dust-influenced areas. Unexpectedly, we show that the occurrence of NPF events is highly frequent during mineral dust outbreaks, occurring even during extreme dust outbreaks. We also show that the occurrence of NPF events during mineral dust outbreaks significantly affects the potential cloud condensation nuclei budget.
Kevin R. Barry, Thomas C. J. Hill, Marina Nieto-Caballero, Thomas A. Douglas, Sonia M. Kreidenweis, Paul J. DeMott, and Jessie M. Creamean
Atmos. Chem. Phys., 23, 15783–15793, https://doi.org/10.5194/acp-23-15783-2023, https://doi.org/10.5194/acp-23-15783-2023, 2023
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Ice-nucleating particles (INPs) are important for the climate due to their influence on cloud properties. To understand potential land-based sources of them in the Arctic, we carried out a survey near the northernmost point of Alaska, a landscape connected to the permafrost (thermokarst). Permafrost contained high concentrations of INPs, with the largest values near the coast. The thermokarst lakes were found to emit INPs, and the water contained elevated concentrations.
Yang Wang, Chanakya Bagya Ramesh, Scott E. Giangrande, Jerome Fast, Xianda Gong, Jiaoshi Zhang, Ahmet Tolga Odabasi, Marcus Vinicius Batista Oliveira, Alyssa Matthews, Fan Mei, John E. Shilling, Jason Tomlinson, Die Wang, and Jian Wang
Atmos. Chem. Phys., 23, 15671–15691, https://doi.org/10.5194/acp-23-15671-2023, https://doi.org/10.5194/acp-23-15671-2023, 2023
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We report the vertical profiles of aerosol properties over the Southern Great Plains (SGP), a region influenced by shallow convective clouds, land–atmosphere interactions, boundary layer turbulence, and the aerosol life cycle. We examined the processes that drive the aerosol population and distribution in the lower troposphere over the SGP. This study helps improve our understanding of aerosol–cloud interactions and the model representation of aerosol processes.
Stefania Gilardoni, Dominic Heslin-Rees, Mauro Mazzola, Vito Vitale, Michael Sprenger, and Radovan Krejci
Atmos. Chem. Phys., 23, 15589–15607, https://doi.org/10.5194/acp-23-15589-2023, https://doi.org/10.5194/acp-23-15589-2023, 2023
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Models still fail in reproducing black carbon (BC) temporal variability in the Arctic. Analysis of equivalent BC concentrations in the European Arctic shows that BC seasonal variability is modulated by the efficiency of removal by precipitation during transport towards high latitudes. Short-term variability is controlled by synoptic-scale circulation patterns. The advection of warm air from lower latitudes is an effective pollution transport pathway during summer.
Markku Kulmala, Anna Lintunen, Hanna Lappalainen, Annele Virtanen, Chao Yan, Ekaterina Ezhova, Tuomo Nieminen, Ilona Riipinen, Risto Makkonen, Johanna Tamminen, Anu-Maija Sundström, Antti Arola, Armin Hansel, Kari Lehtinen, Timo Vesala, Tuukka Petäjä, Jaana Bäck, Tom Kokkonen, and Veli-Matti Kerminen
Atmos. Chem. Phys., 23, 14949–14971, https://doi.org/10.5194/acp-23-14949-2023, https://doi.org/10.5194/acp-23-14949-2023, 2023
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To be able to meet global grand challenges, we need comprehensive open data with proper metadata. In this opinion paper, we describe the SMEAR (Station for Measuring Earth surface – Atmosphere Relations) concept and include several examples (cases), such as new particle formation and growth, feedback loops and the effect of COVID-19, and what has been learned from these investigations. The future needs and the potential of comprehensive observations of the environment are summarized.
Weilun Zhao, Ying Li, Gang Zhao, Song Guo, Nan Ma, Shuya Hu, and Chunsheng Zhao
Atmos. Chem. Phys., 23, 14889–14902, https://doi.org/10.5194/acp-23-14889-2023, https://doi.org/10.5194/acp-23-14889-2023, 2023
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Studies have concentrated on particles containing black carbon (BC) smaller than 700 nm because of technical limitations. In this study, BC-containing particles larger than 700 nm (BC>700) were measured, highlighting their importance to total BC mass and absorption. The contribution of BC>700 to the BC direct radiative effect was estimated, highlighting the necessity to consider the whole size range of BC-containing particles in the model estimation of BC radiative effects.
Alessandro Bigi, Giorgio Veratti, Elisabeth Andrews, Martine Collaud Coen, Lorenzo Guerrieri, Vera Bernardoni, Dario Massabò, Luca Ferrero, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 23, 14841–14869, https://doi.org/10.5194/acp-23-14841-2023, https://doi.org/10.5194/acp-23-14841-2023, 2023
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Atmospheric particles include compounds that play a key role in the greenhouse effect and air toxicity. Concurrent observations of these compounds by multiple instruments are presented, following deployment within an urban environment in the Po Valley, one of Europe's pollution hotspots. The study compares these data, highlighting the impact of ground emissions, mainly vehicular traffic and biomass burning, on the absorption of sun radiation and, ultimately, on climate change and air quality.
Ghislain Motos, Gabriel Freitas, Paraskevi Georgakaki, Jörg Wieder, Guangyu Li, Wenche Aas, Chris Lunder, Radovan Krejci, Julie Thérèse Pasquier, Jan Henneberger, Robert Oscar David, Christoph Ritter, Claudia Mohr, Paul Zieger, and Athanasios Nenes
Atmos. Chem. Phys., 23, 13941–13956, https://doi.org/10.5194/acp-23-13941-2023, https://doi.org/10.5194/acp-23-13941-2023, 2023
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Low-altitude clouds play a key role in regulating the climate of the Arctic, a region that suffers from climate change more than any other on the planet. We gathered meteorological and aerosol physical and chemical data over a year and utilized them for a parameterization that help us unravel the factors driving and limiting the efficiency of cloud droplet formation. We then linked this information to the sources of aerosol found during each season and to processes of cloud glaciation.
Cited articles
ACIA: Impacts of a Warming Arctic: Arctic Climate Impact Assessment, Cambridge University Press, New York, USA, 2004.
Adler, G., Riziq, A. A., Erlick, C., and Rudich, Y.: Effect of intrinsic organic carbon on the optical properties of fresh diesel soot, Proc. Natl. Acad. Sci., 107(15), 6699–6704, https://doi.org/10.1073/pnas.0903311106, 2010.
Anderson, T. L. and Ogren, J. A: Determining aerosol radiative properties using a TSI 3563 integrating nephelometer, Aerosol Sci. Technol., $29$, 57–69, https://doi.org/10.1080/02786829808965551, 1998.
Anderson, T. L., Masonis, S. J., Covert, D. S., Ahlquist, N. C., Howell, S. G., Clarke, A. D., and McNaughton, C. S.: Variability of aerosol optical properties derived from in situ aircraft measurements during ACE-Asia, J. Geophys. Res., 108(D23), 8647, https://doi.org/10.1029/2002jd003247, 2003.
Anderson, T. L., Covert, D. S., Wheeler, J. D., Harris, J. M., Perry, K. D., Trost, B. E., Jaffe, D. J., and Ogren, J. A.: Aerosol backscatter fraction and single scattering albedo: Measured values and uncertainties at a coastal station in the Pacific Northwest, J. Geophys. Res., 104(D21), 26793–26807, https://doi.org/10.1029/1999jd900172, 1999.
Andreae, M. O. and Gelencsér, A.: Black carbon or brown carbon? The nature of light-absorbing carbonaceous aerosols, Atmos. Chem. Phys., 6, 3131–3148, http://dx.doi.org/10.5194/acp-6-3131-2006https://doi.org/10.5194/acp-6-3131-2006, 2006.
Arnott, W. P., Hamasha, K., Moosmuller, H., Sheridan, P. J., and Ogren, J. A.: Towards aerosol light-absorption measurements with a 7-wavelength aethalometer: Evaluation with a photoacoustic instrument and 3-wavelength nephelometer, Aerosol Sci. Technol., 39, 17–29, https://doi.org/10.1080/027868290901972, 2005.
Baumgardner, D., Kok, G., and Raga, G.: Warming of the Arctic lower stratosphere by light absorbing particles, Geophys. Res. Lett., 31(6), 1–4, L06117, https://doi.org/10.1029/2003GL018883, 2004.
Bokoye, A. I., Royer, A., O'Neill, N. T., and McArthur, L. J. B.: A North American Arctic aerosol climatology using ground-based sunphotometry, Arctic, 55(3), 215–228, 2002.
Bond, T. C., Anderson, T. L., and Campbell, D.: Calibration and intercomparison of filter-based measurements of visible light absorption by aerosols, Aerosol Sci. Technol., 30(6), 582–600, 1999.
Bond, T. C., Habib, G., and Bergstrom, R. W.: Limitations in the Enhancement of Visible Light Absorption due to Mixing State, J. Geophys. Res., 111, D20211, https://doi.org/10.1029/2006JD007315, 2006.
Bourdages, L., Duck, T. J., Lesins, G., Drummond, J. R., and Eloranta, E. W.: Physical properties of High Arctic tropospheric particles during winter, Atmos. Chem. Phys., 9, 6881–6897, https://doi.org/6810.5194/acp-6889-6881-2009, 2009.
Brock, C. A., Schroder, F., Karcher, B., Petzold, A., Busen, R., and Fiebig, M.: Ultrafine particle size distributions measured in aircraft exhaust plumes, J. Geophys. Res., 105(D21), 26555–26567, https://doi.org/10.1029/2000JD900360, 2000.
Brock, C. A., Sullivan, A. P., Peltier, R. E., Weber, R. J., Wollny, A., de Gouw, J. A., Middlebrook, A. M., Atlas, E. L., Stohl, A., Trainer, M. K., Cooper, O. R., Fehsenfeld, F. C., Frost, G. J., Holloway, J. S., Hübler, G., Neuman, J. A., Ryerson, T. B., Warneke, C., and Wilson, J. C.: Sources of particulate matter in the northeastern United States in summer: 2. Evolution of chemical and microphysical properties, J. Geophys. Res., 113(D8), D08302, https://doi.org/10.1029/2007jd009241, 2008.
Brock, C. A., Cozic, J., Bahreini, R., Froyd, K. D., Middlebrook, A. M., McComiskey, A., Brioude, J., Cooper, O. R., Stohl, A., Aikin, K. C., de Gouw, J. A., Fahey, D. W., Ferrare, R. A., Gao, R.-S., Gore, W., Holloway, J. S., Hübler, G., Jefferson, A., Lack, D. A., Lance, S., Moore, R. H., Murphy, D. M., Nenes, A., Novelli, P. C., Nowak, J. B., Ogren, J. A., Peischl, J., Pierce, R. B., Pilewskie, P., Quinn, P. K., Ryerson, T. B., Schmidt, K. S., Schwarz, J. P., Sodemann, H., Spackman, J. R., Stark, H., Thomson, D. S., Thornberry, T., Veres, P., Watts, L. A., Warneke, C., and Wollny, A. G.: Characteristics, sources, and transport of aerosols measured in spring 2008 during the aerosol, radiation, and cloud processes affecting Arctic Climate (ARCPAC) Project, Atmos. Chem. Phys., 11, 2423–2453, http://dx.doi.org/10.5194/acp-11-2423-2011https://doi.org/10.5194/acp-11-2423-2011, 2011.
Canagaratna, M. R., Jayne, J. T., Jimenez, J. L., Allan, J. D., Alfarra, M. R., Zhang, Q., Onasch, T. B., Drewnick, F., Coe, H., Middlebrook, A., Delia, A. E., Williams, L. R., Trimborn, A., Northway, M. J., DeCarlo, P. F., Kolb, C. E., Davidovits, P., and Worsnop, D. R.: Chemical and Microphysical Characterization of Ambient Aerosols with the Aerodyne Aerosol Mass Spectrometer, Mass Spectrom. Rev., 26, 185–222, https://doi.org/10.1002/mas.20115, 2007.
Cappa, C. D., Lack, D. A., Burkholder, J. B., and Ravishankara, A. R.: Bias in Filter-Based Aerosol Light Absorption Measurements Due to Organic Aerosol Loading: Evidence from Laboratory Measurements, Aerosol Sci. Technol., 42, 1022–1032, https://doi.org/10.1080/02786820802389277, 2008.
Clarke, A. D. and Kapustin, V. N.: Hemispheric Aerosol Vertical Profiles: Anthropogenic Impacts on Optical Depth and Cloud Nuclei, Science, 329(1488), https://doi.org/10.1126/science.1188838, 2010.
Clarke, A. D. and Noone, K. J.: Soot in the Arctic Snowpack – a Cause for Perturbations in Radiative-Transfer, Atmos. Environ., 19(12), 2045–2053, 1985.
Clarke, A. D., Charlson, R. J., and Radke, L. F.: Airborne Observations of Arctic Aerosol .4. Optical-Properties of Arctic Haze, Geophys. Res. Lett., 11(5), 405–408, 1984.
Clarke, A. D., Shinozuka, Y., Kapustin, V. N., Howell, S., Huebert, B., Doherty, S., Anderson, T., Covert, D., Anderson, J., Hua, X., Moore II, K. G., McNaughton, C., Carmichael, G., and Weber, R.: Size distributions and mixtures of dust and black carbon aerosol in Asian outflow: Physiochemistry and optical properties, J. Geophys. Res., $109$(D15), D15S09, https://doi.org/10.1029/2003jd004378, 2004.
Clarke, A. D., McNaughton, C., Kapustin, V., Shinozuka, Y., Howell, S., Dibb, J., Zhou, J., Anderson, B., Brekhovskikh, V., Turner, H., and Pinkerton, M.: Biomass burning and pollution aerosol over North America: Organic components and their influence on spectral optical properties and humidification response, J. Geophys. Res., 112(D12), D12S18, https://doi.org/10.1029/2006jd007777, 2007.
Crounse, J. D., DeCarlo, P. F., Blake, D. R., Emmons, L. K., Campos, T. L., Apel, E. C., Clarke, A. D., Weinheimer, A. J., McCabe, D. C., Yokelson, R. J., Jimenez, J. L., and Wennberg, P. O.: Biomass burning and urban air pollution over the Central Mexican Plateau, Atmos. Chem. Phys., 9, 4929–4944, https://doi.org/10.5194/acp-9-4929-2009, 2009.
de Gouw, J. A. and Jimenez, J. L.: Organic aerosols in the Earth's atmosphere, Environ. Sci. Technol., $43$, 7614–7618, https://doi.org/10.1021/es9006004, 2009.
de Gouw, J. A. and Warneke, C.: Measurements of volatile organic compounds in the Earth's atmosphere using proton-transfer-reaction mass spectrometery, Mass Spectrom. Rev., 26, 223–257, https://doi.org/10.1002/mas.20119, 2007.
de Gouw, J. A., Cooper, O. R., Warneke, C., Hudson, P. K., Fehsenfeld, F. C., Holloway, J. S., Hubler, G., Nicks Jr., D. K., Nowak, J. B., Parrish, D. D., Ryerson, T. B., and Trainer, M.: Chemical composition of airmasses transported from Asia to the U.S. West Coast during ITCT 2K2: Fossil fuel combustion versus biomass-burning signatures, J. Geophys. Res., 109, D23S20, https://doi.org/10.1029/2003JD004202, 2004.
DeCarlo, P. F., Kimmel, R. E., Trimborn, A., Northway, M. J., Jayne, J. T., Aiken, A. C., Gonin, M., Fuhrer, K., Horvath, T., Docherty, K. S., Worsnop, D. R., and Jimenez, J. L.: Field-Deployable, High-Resolution, Time-of-Flight Aerosol Mass Spectrometer, Anal. Chem., $78$, 8281–8289, https://doi.org/10.1021/ac061249n, 2006.
DeCarlo, P. F., Ulbrich, I. M., Crounse, J., de Foy, B., Dunlea, E. J., Aiken, A. C., Knapp, D., Weinheimer, A. J., Campos, T., Wennberg, P. O., and Jimenez, J. L.: Investigation of the sources and processing of organic aerosol over the Central Mexican Plateau from aircraft measurements during MILAGRO, Atmos. Chem. Phys., 10, 5257–5280, https://doi.org/10.5194/acp-10-5257-2010, 2010.
Dunlea, E. J., DeCarlo, P. F., Aiken, A. C., Kimmel, R. E., Peltier, R. E., Weber, R. J., Tomlinson, J. M., Collins, D. R., Shinozuka, Y., McNaughton, C. S., Howell, S. G., Clarke, A. D., Emmons, L. K., Apel, E. C., Pfister, G., van Donkelaar, A., Martin, R. V., Millet, D. B., Heald, C. L., and Jimenez J. L.: Evolution of Asian Aerosols during Transpacific Transport in INTEX-B, Atmos. Chem. Phys., $9$, 7257–7287, https://doi.org/10.5194/acp-9-7257-2009, 2009.
Fisher, J. A., Jacob, D. J., Purdy, M. T., Kopacz, M., Le Sager, P., Carouge, C., Holmes, C. D., Yantosca, R. M., Batchelor, R. L., Strong, K., Diskin, G. S., Fuelberg, H. E., Holloway, J. S., Hyer, E. J., McMillan, W. W., Warner, J., Streets, D. G., Zhang, Q., Wang, Y., and Wu, S.: Source attribution and interannual variability of Arctic pollution in spring constrained by aircraft (ARCTAS, ARCPAC) and satellite (AIRS) observations of carbon monoxide, Atmos. Chem. Phys., 10, 977–996, https://doi.org/10.5194/acp-10-977-2010, 2010.
Flanner, M. G., Zender, C. S., Hess, P. G., Mahowald, N. M., Painter, T. H., Ramanathan, V., and Rasch, P. J.: Springtime warming and reduced snow cover from carbonaceous particles, Atmos. Chem. Phys., 9, 2481–2497, https://doi.org/10.5194/acp-9-2481-2009, 2009.
Fromm, M., Lindsey, D. T., Servranckx, R., Yue, G., Trickl, T., Sica, R., Doucet, P., and Godin-Beekmann, S.: The untold story of pyrocumulonimbus, B Am. Meteorol. Soc., $91$(9), 1193–1209, https://doi.org/1110.1175/2010BAMS3004.1191, 2010.
Froyd, K. D., Murphy, D. M., Sanford, T. J., Thomson, D. S., Wilson, J. C., Pfister, L., and Lait, L.: Aerosol composition of the tropical upper troposphere, Atmos. Chem. Phys., 9, 4363–4385, https://doi.org/10.5194/acp-9-4363-2009, 2009.
Fuelberg, H. E., Harrigan, D. L., and Sessions, W.: A meteorological overview of the ARCTAS 2008 mission, Atmos. Chem. Phys., 10, 817–842, https://doi.org/10.5194/acp-10-817-2010, 2010.
Fuller, K., Malm, W. C., and Kriedenweiss, S. M.: Effects of mixing on extinction by carbonaceous particles, J. Geophys. Res., 104, 15941–15954, 1999.
Gong, S. L., Zhao, T. L., Sharma, S., Toom-Sauntry, D., Lavoue, D., Zhang, X. B., Leaitch, W. R., and Barrie, L. A.: Identification of trends and interannual varia bility of sulfate and black carbon in the Canadian High Arctic: 1981–2007, J. Geophys. Res., 115, D07305, https://doi.org/10.1029/2009JD01294, 20103.
Graber, E. R. and Rudich, Y.: Atmospheric HULIS: How humic-like are they? A comprehensive and critical review, Atmos. Chem. Phys., 6, 729–753, https://doi.org/10.5194/acp-6-729-2006, 2006.
Guan, H., Esswein, R., Lopez, J., Bergstrom, R., Warnock, A., Follette-Cook, M., Fromm, M., and Iraci, L. T.: A multi-decadal history of biomass burning plume heights identified using aerosol index measurements, Atmos. Chem. Phys., 10, 6461–6469, https://doi.org/10.5194/acp-10-6461-2010, 2010.
Gyawali, M., Arnott, W. P., Lewis, K., and Moosmüller, H.: In situ aerosol optics in Reno, NV, USA during and after the summer 2008 California wildfires and the influence of absorbing and non-absorbing organic coatings on spectral light absorption, Atmos. Chem. Phys., 9, 8007–8015, https://doi.org/10.5194/acp-9-8007-2009, 2009.
Hansen, J. and Nazarenko, L.: Soot climate forcing via snow and ice albedos, Proc. Natl. Acad. Sci. USA, 101(2), 423–428, https://doi.org/10.1073/pnas.2237157100, 2004.
Haywood, J. M. and Shine, K. P.: The effect of anthropogenic sulfate and soot aerosol on the clear sky planetary radiation budget, Geophys. Res. Lett., $22$(5), 603–606, 1995.
Hegg, Dean A., Warren, Stephen G., Grenfell, Thomas C., Sarah J Doherty, and Clarke, Antony D.: Sources of light-absorbing aerosol in arctic snow and their seasonal variation, Atmos. Chem. Phys., 10, 10923–10938, https://doi.org/10.5194/acp-10-10923-2010, 2010.
Huebert, B. J., Bates, T., Russell, P. B., Shi, G., Kim, Y. J., Kawamura, K., Carmichael, G., and Nakajima, T.: An overview of ACE-Asia: Strategies for quantifying the relationships between Asian aerosols and their climatic impacts, J. Geophys. Res., 108(D23), 8633, https://doi.org/10.1029/2003jd003550, 2003.
Huebert, B. J., Bertram, T., Kline, J., Howell, S., Eatough, D., and Blomquist, B.: Measurements of organic and elemental carbon in Asian outflow during ACE-Asia from the NSF/NCAR C-130, J. Geophys. Res., 109(D19), D19S11, https://doi.org/10.1029/2004jd004700, 2004a.
Huebert, B. J., Howell, S. G., Covert, D., Bertram, T., Clarke, A., Anderson, J. R., Lafleur, B. G., Seebaugh, W. R., Wilson, J. C., Gesler, D., Blomquist, B., and Fox, J.: PELTI: Measuring the Passing Efficiency of an Airborne Low Turbulence Aerosol Inlet, Aerosol Sci. Technol., $38$(8), 803–826, https://doi.org/10.1080/027868290500823, 2004b.
IPCC: Technical Summary, in Climate Change 2007: The Physical Science Basis. Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Solomon, D. Q. S., Manning, M., Chen, Z., Marquis, M., Averyt, K. B., Tignor, M., and Miller, H. L., Cambridge University Press, Cambridge, UK and New York, NY, USA, 2007.
Ishii, S., Shibata, T., Nagai, T., Mizutani, K., Itabe, T., Hirota, M., Fujimoto, T., and Uchino, O.: Arctic haze and clouds observed by lidar during four winter seasons of 1993–1997 at Eureka Canada, Atmos. Environ., $33$(16), 2459–2470, https://doi.org/10.1016/S1352-2310(98)00397-5, 1999.
Jacob, D. J., Crawford, J. H., Maring, H., Clarke, A. D., Dibb, J. E., Emmons, L. K., Ferrare, R. A., Hostetler, C. A., Russell, P. B., Singh, H. B., Thompson, A. M., Shaw, G. E., McCauley, E., Pederson, J. R., and Fisher, J. A.: The Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) mission: design, execution, and first results, Atmos. Chem. Phys., 10, 5191–5212, https://doi.org/10.5194/acp-10-5191-2010, 2010.
Kanakidou, M., Seinfeld, J. H., Pandis, S. N., Barnes, I., Dentener, F. J., Facchini, M. C., Van Dingenen, R., Ervens, B., Nenes, A., Nielsen, C. J., Swietlicki, E., Putaud, J. P., Balkanski, Y., Fuzzi, S., Horth, J., Moortgat, G. K., Winterhalter, R., Myhre, C. E. L., Tsigaridis, K., Vignati, E., Stephanou, E. G., and Wilson, J.: Organic aerosol and global climate modelling: a review, Atmos. Chem. Phys., 5, 1053–1123, https://doi.org/10.5194/acp-5-1053-2005, 2005.
Kinne, S., Schulz, M., Textor, C., Guibert, S., Balkanski, Y., Bauer, S. E., Berntsen, T., Berglen, T. F., Boucher, O., Chin, M., Collins, W., Dentener, F., Diehl, T., Easter, R., Feichter, J., Fillmore, D., Ghan, S., Ginoux, P., Gong, S., Grini, A., Hendricks, J., Herzog, M., Horowitz, L., Isaksen, I., Iversen, T., Kirkevåg, A., Kloster, S., Koch, D., Kristjansson, J. E., Krol, M., Lauer, A., Lamarque, J. F., Lesins, G., Liu, X., Lohmann, U., Montanaro, V., Myhre, G., Penner, J., Pitari, G., Reddy, S., Seland, O., Stier, P., Takemura, T., and Tie, X.: An AeroCom initial assessment –optical properties in aerosol component modules of global models, Atmos. Chem. Phys., 6, 1815–1834, http://dx.doi.org/10.5194/acp-6-1815-2006https://doi.org/10.5194/acp-6-1815-2006, 2006.
Kirchstetter, T. W., Novakov, T., and Hobbs, P. V.: Evidence that the spectral dependence of light absorption by aerosols is affected by organic carbon, J. Geophys. Res., 109, D21208, https://doi.org/10.1029/2004JD004999, 2004.
Kline, J., Huebert, B., Howell, S., Blomquist, B., Zhuang, J., Bertram, T., and Carrillo, J.: Aerosol composition and size versus altitude measured from the C-130 during ACE-Asia, J. Geophys. Res., 109(D19), D19S08, https://doi.org/10.1029/2004jd004540, 2004.
Koch, D., Schulz, M., Kinne, S., McNaughton, C., Spackman, J. R., Balkanski, Y., Bauer, S., Berntsen, T., Bond, T. C., Boucher, O., Chin, M., Clarke, A., De Luca, N., Dentener, F., Diehl, T., Dubovik, O., Easter, R., Fahey, D. W., Feichter, J., Fillmore, D., Freitag, S., Ghan, S., Ginoux, P., Gong, S., Horowitz, L., Iversen, T., Kirkevåg, A., Klimont, Z., Kondo, Y., Krol, M., Liu, X., Miller, R., Montanaro, V., Moteki, N., Myhre, G., Penner, J. E., Perlwitz, J., Pitari, G., Reddy, S., Sahu, L., Sakamoto, H., Schuster, G., Schwarz, J. P., Seland, Ø., Stier, P., Takegawa, N., Takemura, T., Textor, C., van Aardenne, J. A., and Zhao, Y.: Evaluation of black carbon estimations in global aerosol models, Atmos. Chem. Phys., 9, 9001–9026, http://dx.doi.org/10.5194/acp-9-9001-2009https://doi.org/10.5194/acp-9-9001-2009, 2009.
Kondo, Y., Sahu, L., Kuwata, M., Miyazaki, Y., Takegawa, N., Moteki, N., Imaru, J., Han, S., Nakayama, T., Kim Oang, N. T., Hu, M., Kim, Y. J., and Kita, K.: Stabilization of the Mass Absorption Cross Section of Black Carbon for Filter-Based Absorption Photometry by the use of a Heated Inlet, Aerosol Sci. Technol., 43, 741–756, https://doi.org/10.1080/02786820902889879, 2009.
Kondo, Y., Sahu, L., Moteki, N., Khan, F., Takegawa, N., Liu, X., Koike, M., and Miyakawa, T.: Consistency and traceability of black carbon measurements made by laser-induced incandescence, thermal-optical transmittance, and filter-based photo-aborption techniques, Aerosol Sci. Technol., 45(2), 294–312, https://doi.org/10.1080/02786826.2010.533215, 2011.
Lack, D. A. and Cappa, C. D.: Impact of brown and clear carbon on light absorption enhancement, single scatter albedo and absorption wavelength dependence of black carbon, Atmos. Chem. Phys., 10, 4207–4220, https://doi.org/10.5194/acp-10-4207-2010, 2010.
Lack, D. A., Cappa, C. D., Covert, D. C., Baynard, T., Massoli, P., Sierau, B., Bates, T. S., Quinn, P. K., Lovejoy, E. R., and Ravishankara, A. R.: Bias in Filter-Based Aerosol Light Absorption Measurements Due to Organic Aerosol Loading: Evidence from Ambient Measurements, Aerosol Sci. Technol., 42, 1033–1041, https://doi.org/10.1080/02786820802389277, 2008.
Lafon, S., Sokolik, I., Rajot, J., Caquineau, S., and Gaudichet, A.: Characterization of iron oxides in mineral dust aerosols: Implications for light absorption, J. Geophys. Res., 111, D21207, https://doi.org/10.1029/2005JD007016, 2006.
Leaitch, W. R., Hoff, R. M., and MacPherson, J. I.: , Airborne and lidar measurements of aerosol and c loud particles in the troposphere over Alert Canada in April 1986, J. Atmos. Chem., 9(1–3), 187–211, https://doi.org/10.1007/BF00052832, 1989.
Li, Z., Chen, H., Cribb, M., Dickerson, R. R., Holben, B., Li, C., Lu, D., Luo, Y., Maring, H., Shi, G., Tsay, S. C., Wang, P., Wang, Y., Xia, X., Zheng, Y., Yuan, T., and Zhao, F.: Preface to special section on East Asian Studies of Tropospheric Aerosols: An International Regional Experiment (EAST-AIRE), J. Geophys. Res., 112, D22S00, https://doi.org/10.1029/2007JD008853, 2007.
Lindinger, W., Hansel, A., and Jordan, A.: Proton-transer-reaction mass spectrometry (PTR-MS) on-line monitoring of volatile organic compounds at pptv levels, Chemical Society Reviews, 27, 347–354, 1998.
Mader, B., Flagan, R. C., and Seinfeld, J. H.: Airborne measurements of atmospheric carbonaceous aerosols during ACE-Asia, J. Geophys. Res., 107, 4704, https://doi.org/10.1029/2002JD002221, 2002.
Mayol-Bracero, O. L., Gabriel, R., Andreae, M. O., Kirchstetter, T. W., Novakov, T., Ogren, J., Sheridan, P., and Streets, D. G.: Carbonaceous aerosols over the Indian Ocean during the Indian Ocean Experiment (INDOEX): Chemical characterization, optical properties, and probable sources, J. Geophys. Res., 107(D19), INX2 29-21-INX22 29-21, https://doi.org/10.1029/2000JD000039, 2002.
McNaughton, C. S.: Constraining climate model simulations of aerosol size distributoins over the North Pacific and North America using in-situ airborne measurements, PhD Dissertation thesis, University of Hawaii, Honolulu, 408 pp., 2008.
McNaughton, C. S., Clarke, A. D., Howell, S. G., Pinkerton, M., Anderson, B. E., Thornhill, L., Hudgins, C., Winstead, E., Dibb, J. E., Scheuer, E., and Maring, H.: Results from the DC-8 Inlet Characterization Experiment (DICE): Airborne versus surface sampling of mineral dust and sea salt aerosols, Aerosol Sci. Technol., 41(2), 136–159, https://doi.org/10.1080/02786820601118406, 2007.
McNaughton, C. S., Clarke, A. D., Kapustin, V., Shinozuka, Y., Howell, S. G., Anderson, B. E., Winstead, E., Dibb, J., Scheuer, E., Cohen, R. C., Wooldridge, P., Perring, A., Huey, L. G., Kim, S., Jimenez, J. L., Dunlea, E. J., DeCarlo, P. F., Wennberg, P. O., Crounse, J. D., Weinheimer, A. J., and Flocke, F.: Observations of heterogeneous reactions between Asian pollution and mineral dust over the Eastern North Pacific during INTEX-B, Atmos. Chem. Phys., 9, 8283–8308, https://doi.org/10.5194/acp-9-8283-2009, 2009.
Menon, S., Koch, D., Beig, G., Sahu, S., Fasullo, J., and Orlikowski, D.: Black carbon aerosols and the third polar ice cap, Atmos. Chem. Phys., 10, 4559–4571, https://doi.org/4510.5194/acp-4510-4559-2010, 2010.
Middlebrook, A. M., Bahreini, R., Brioude, J., Brock, C. A., Cozic, J. A., De Gouw, J. A., Froyd, K. D., Holloway, J. S., Lack, D. A., Lance, S. M., Murphy, D. M., Ryerson, T. B., Schwarz, J. P., Spackman, J. R., Thomson, D. S., Thornberry, T. D., Veres, P., and Warneke, C.: The Influence of Distant Fires on the Chemical Properties of Arctic Aerosol During the Spring of 2008, in 2008 AGU Fall Meeting edited, American Geophysical Union, San Fransisco, California, USA, 2008.
Moteki, N. and Kondo, Y.: Effects of mixing state on black carbon measurement by Laser-Induced Incandescence, Aerosol Sci. Technol., 41, 398–417, https://doi.org/10.1080/02786820701199728, 2007.
Moteki, N., Kondo, Y., Miyazaki, Y., Takegawa, N., Komazaki, Y., Kurata, G., Shirai, T., Blake, D. R., Miyakawa, T., and Koike, M.: Evolution of mixing state of black carbon particles: Aircraft measurements over the western Pacific in March 2004, Geophys. Res. Lett., 34, L11803, https://doi.org/10.1029/2006GL028943, 2007.
Quinn, P. K., Shaw, G., Andrews, E., Dutton, E. G., Ruoho-Airola, T., and Gong, S. L.: Arctic haze: current trends and knowledge gaps, Tellus B – Chem. Phys. Meteorol., 59(1), 99–114, https://doi.org/10.1111/j.1600-0889.2006.00238.x, 2007.
Rogers, D. C., DeMott, P. J., and Kreidenweis, S. M.: Airborne measurements of tropospheric ice-nucleating aerosol particles in the Arctic spring, J. Geophys. Res., 106(D14), 15053–15064, https://doi.org/10.1029/2000JD900790, 2001.
Schauer, J. J., Mader, B. T., Deminter, J. T., Heidemann, G., Bae, M. S., Seinfeld, J. H., Flagan, R. C., Cary, R. A., Smith, D., Huebert, B. J., Bertram, T., Howell, S., Kline, J. T., Quinn, P., Bates, T., Turpin, B., Lim, H. J., Yu, J. Z., Yang, H., and Keywood, M. D.: ACE-Asia intercomparison of a thermal-optical method for the determination of particle-phase organic and elemental carbon, Environ. Sci. Technol., 37(5), 993–1001, https://doi.org/10.1021/es020622f, 2003.
Scheuer, E., Talbot, R. W., Dibb, J. E., Seid, G. K., DeBell, L., and Lefer, B.: Seasonal distributions of fine aerosol sulfate in the North American Arctic basin during TOPSE, J. Geophys. Res., 108(D4), 8370, https://doi.org/10.1029/2001JD001364, 2003.
Schnaiter, M., Gimmler, M., Llamas, I., Linke, C., Jager, C., and Mutschke H.: Strong spectral dependence of light absorption by organic carbon particles formed by propane combustion, Atmos. Chem. Phys., 6, 2981–2990, https://doi.org/10.5194/acp-6-2981-2006, 2006.
Schnaiter, M., Linke, C., Mohler, O., Naumann, K. H., Saathoff, H., Wagner, R., Schurath, U., and Wehner, B.: Absorption amplification of black carbon internally mixed secondary organic aerosol, J. Geophys. Res., 110, D19204, https://doi.org/10.1029/2005JD006046, 2005.
Schwarz, J. P., Gao, R. S., Fahey, D. W., Thomson, D. S., Watts, L. A., Wilson, J. C., Reeves, J. M., Darbeheshti, M., Baumgardner, D. G., Kok, G. L., Chung, S. H., Schulz, M., Hendricks, J., Lauer, A., Karcher, B., Slowik, J. G., Rosenlof, K. H., Thompson, T. L., Langford, A. O., Loewenstein, M., and Aikin, K. C.: Single-particle measurements of midlatitude black carbon and light-scattering aerosols from the boundary layer to the lower stratosphere, J. Geophys. Res., 111, D16207, https://doi.org/10.1029/2006JD007076, 2006.
Sharma, S., Andrews, E., Barrie, L. A., Ogren, J. A., and Lavoue, D.: Variations and sources of the equivalent black carbon in the high Arctic revealed by long-term observations at Alert and Barrow: 1989–2003, J. Geophys. Res.-Atmos., 111(D14), 1–15, D14208, https://doi.org/10.1029/2005JD006581, 2006.
Shaw, G. E.: The Arctic Haze Phenomenon, B Am. Meteorol. Soc., 76(12), 2403–2414, https://doi.org/10.1175/1520-0477(1995)076<2403:TAHP>2.0.CO;2, 1995.
Shinozuka, Y., Clarke, A. D., Howell, S. G., Kapustin, V. N., McNaughton, C. S., Zhou, J., and Anderson, B. E.: Aircraft profiles of aerosol microphysics and optical properties over North America: Aerosol optical depth and its association with PM2.5 and water uptake, J. Geophys. Res., 112, D12S20, https://doi.org/10.1029/2006JD007918, 2007.
Slowik, J. G., Cross, E. S., Han, J. H., Davidovits, P., Onasch, T. B., Jayne, J. T., Williams, L. R., Canagaratna, M. R., Worsnop, D. R., Chakrabarty, R. K., Moosmuller, H., Arnott, W. P., Schwarz, J. P., Gao, R. S., Fahey, D. W., Kok, G. L., and Petzold, A.: An inter-comparison of instruments measuring black carbon content of soot particles, Aerosol Sci. Technol., 41(3), 295–314, https://doi.org/10.1080/02786820701197078, 2007.
Sokolik, I. N. and Toon, O. B.: Direct radiative forcing by anthropogenic airborne mineral aerosols, Nature, 381, 681–683, https://doi.org/10.1038/381681a0, 1996.
Solomon, S., Plattner, G. K., Knutti, R., and Friedlingstein, P.: Irreversible climate change due to carbon dioxide emissions, PNAS, 106, 1704–1709, https://doi.org/10.1073/pnas.0812721106, 2009.
Spackman, J. R., Gao, R. S., Neff, W. D., Schwarz, J. P., Watts, L. A., Fahey, D. W., Holloway, J. S., Ryerson, T. B., Peischl, J., and Brock, C. A.: Aircraft observations of enhancement and depletion of black carbon mass in the springtime Arctic, Atmos. Chem. Phys., 10, 9667–9680, https://doi.org/10.5194/acp-10-9667-2010, 2010.
Sprung, D., Jost, C., Reiner, T., Hansel, A., and Wisthaler, A.: Acetone and acetonitrile in the tropical Indian Ocean boundary layer and free troposphere: Aircraft-based intercomparison of AP-CIMS and PTR-MS measurements, J. Geophys. Res., 106(D22), 28511–28527, https://doi.org/10.1029/2000JD900599, 2001.
Stephens, M., Turner, N., and Sandberg, J.: Particle identification by Laser Induced Incandescence in a solid state laser cavity, Appl. Opt., 42, 3726–3736, https://doi.org/10.1364/AO.42.003726, 2003.
Stocks, B. J., Fosberg, M. A., Lynham, T. J., Mearns, L., Wotton, B. M., Yang, Q., Jin, J. Z., Lawrence, K., Hartley, G. R., Mason, J. A., and McKenney, D. W.: Climate change and forest fire potential in Russian and Canadian boreal forests, Clim. Change, 38(1), 1–13, 1998.
Stohl, A.: Characteristics of atmospheric transport into the Arctic troposphere, J. Geophys. Res.-Atmos., 111(D11), 1–17, D11306, https://doi.org/10.1029/2005JD006888, 2006.
Subramanian, R., Roden, C. A., Bopari, P., and Bond, T. C.: Yellow Beads and Missing Particles: Trouble Ahead for Filter-Based Absorption Measurements, Aerosol Sci. Technol., 41, 630–637, https://doi.org/10.1080/02786820701344589, 2007.
Subramanian, R., Kok, G. L., Baumgardner, D., Clarke, A., Shinozuka, Y., Campos, T. L., Heizer, C. G., Stephens, B. B., de Foy, B., Voss, P. B., and Zaveri, R. A.: Black carbon over Mexico: the effect of atmospheric transport on mixing state, mass absorption cross-section, and BC/CO ratios, Atmos. Chem. Phys., 10, 219–237, https://doi.org/10.5194/acp-10-219-2010, 2010.
Textor, C., Schulz, M., Guibert, S., Kinne, S., Balkanski, Y., Bauer, S., Berntsen, T., Berglen, T., Boucher, O., Chin, M., Dentener, F., Diehl, T., Easter, R., Feichter, H., Fillmore, D., Ghan, S., Ginoux, P., Gong, S., Grini, A., Hendricks, J., Horowitz, L., Huang, P., Isaksen, I., Iversen, I., Kloster, S., Koch, D., Kirkevåg, A., Kristjansson, J. E., Krol, M., Lauer, A., Lamarque, J. F., Liu, X., Montanaro, V., Myhre, G., Penner, J., Pitari, G., Reddy, S., Seland, Ø., Stier, P., Takemura, T., and Tie, X.: Analysis and quantification of the diversities of aerosol life cycles within AeroCom, Atmos. Chem. Phys., 6, 1777–1813, https://doi.org/10.5194/acp-6-1777-2006, 2006.
Tomasi, C., Vitale, V., Lupi, A., Di Carmine, C., Campanelli, M., Herber, A., Treffeisen, R., Stone, R. S., Andrews, E., Sharma, S., Radionov, V. F., von Heyningen-Huene, W., Stebel, K., Hansen, G. H., Myhre, C. L., Wehrli, C., Aaltonen, V., Lihavainen, H., Virkkula, A., Hillamo, R., Strom, J., Toledano, C., Cachorro, V. E., Ortiz, P., de Frutos, A. M., Blindheim, S., Frioud, M., Gausa, M., Zielinski, T., Petelski, T., and Yamanouchi, T.: Aerosol in polar regions: A historical overview based on optical depth and in-situ observations, J. Geophys. Res., 112, D16205, https://doi.org/10.1029/2007JD008432, 2007.
Virkkula, A.: Correction of the Calibration of the 3-wavelength Particle Soot Absorption Photometer (3λ PSAP), Aerosol Sci. Technol., 44(8), 706–712, https://doi.org/10.1080/02786826.02782010, 2010.
Virkkula, A., Ahlquist, N. C., Covert, D. S., Arnott, W. P., Sheridan, P. J., Quinn, P. K., and Coffman, D. J.: Modification, Calibration and a Field Test of an Instrument for Measuring Light Absorption by Particles, Aerosol Sci. Technol., 39(1), 68–83, https://doi.org/10.1080/027868290901963, 2005.
Warneke, C., De Gouw, J. A., Stohl, A., Cooper, O. R., Goldan, P. D., Kuster, W. C., Holloway, J. S., Williams, E. J., Lerner, B. M., McKeen, S. A., Trainer, M., Fehsenfeld, F. C., Atlas, E. L., Donnelly, S. G., Stroud, V., Lueb, A., and Kato, S.: Biomass burning and anthropogenic sources of CO over New England in summer 2004, J. Geophys. Res., 111, D23S15, https://doi.org/10.1029/2005JD006878, 2006.
Warneke, C., Bahreini, R., Brioude, J., Brock, C. A., De Gouw, J. A., Fahey, D. W., Froyd, K. D., Holloway, J. S., Middlebrook, A., Miller, L., Montzka, S., Murphy, D. M., Peischl, J., Ryerson, T. B., Schwarz, J. P., Spackman, J. R. and Veres, P.: Biomass burning in Siberia and Kazakhstan as an important source for haze over the Alaskan Arctic in April 2008, Geophys. Res. Lett., 36, L02813, https://doi.org/10.1029/2008GL036194, 2009.
Warneke, C., Froyd, K. D., Brioude, J., Bahreini, R., Brock, C. A., Cozic, J., De Gouw, J. A., Fahey, D. W., Ferrare, R., Holloway, J. S., Middlebrook, A. M., Miller, L., Montzka, S., Schwarz, J. P., Sodemann, H., Spackman, J. R., and Stohl, A.: An important contribution to sprintime Arctic aerosol from biomass burning in Russia, Geophys. Res. Lett., 37, L01801, https://doi.org/10.1029/2009GL041816, 2010.
Westerling, A. L., Hidalgo, H. G., Cayan, D. R., and Swetnam, T. W.: Warming and Earlier Spring Increase Western US Forest Wildfire Activity, Science, 313, 940–943, https://doi.org/10.1126/science.1128834, 2006.
Wilson, J. C., Lafleur, B., Hilvert, G. H., Seabaugh, W. R., Fox, W. J., Brock, C. A., Huebert, B. J., Geseler, D. R., Muller, J., and Reeves, J. M.: Function and performance of a low turbulence inlet for sampling super-micron particles from aircraft platforms, Aerosol Sci. Technol., 38, 790–802, https://doi.org/10.1080/027868290500841, 2004.
Xu, B., Cao, J. J., Hansen, J., Yao, T., Joswia, D. R., Wang, N., Wu, G., Wang, M., Zhao, H., Yang, W., Liu, X., and He, J.: Black soot and the survival of Tibetan glaciers, Proc. Natl. Acad. Sci. USA, 106(52), 22114–22118, https://doi.org/10.21073/pnas.0910444106, 2009.
Yamanouchi, T., Treffeisen, R., Herber, A., Shiobara, M., Yamagata, S., Hara, K., Sato, K., Yabuki, M., Tomikawa, Y., Rinke, A., Neuber, R., Schumachter, R., Kriews, M., Strom, J., Schrems, O., and Gernandt, H.: Arctic Study of Tropospheric Aerosol and Radiation (ASTAR) 2000: Arctic haze case study, Tellus B – Chem. Phys. Meteorol., 57(2), 141–152, https://doi.org/10.1111/j.1600-0889.2005.00140.x, 2005.
Yang, M.: Separation of light absorption to black carbon, brown carbon, and mineral dust – interpretations of atmospheric measurements near Beijing, MS Thesis, University of Hawaii at Manoa, Honolulu, Hawaii, USA, 2007.
Yang, M., Howell, S. G., Zhuang, J., and Huebert, B. J.: Attribution of aerosol light absorption to black carbon, brown carbon, and dust in China – interpretations of atmospheric measurements during EAST-AIRE, Atmos. Chem. Phys., 9, 2035–2050, https://doi.org/10.5194/acp-2035-2009, 2009.
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