Articles | Volume 24, issue 4
https://doi.org/10.5194/acp-24-2077-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-24-2077-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
19 Feb 2024
Research article |
| 19 Feb 2024
| 19 Feb 2024
How well do Earth system models reproduce the observed aerosol response to rapid emission reductions? A COVID-19 case study
Canadian Centre for Climate Modelling and Analysis, Environment and Climate Change, Victoria, British Columbia, Canada
School of Earth and Ocean Sciences, University of Victoria, Victoria, British Columbia, Canada
Nathan P. Gillett
Canadian Centre for Climate Modelling and Analysis, Environment and Climate Change, Victoria, British Columbia, Canada
Adam H. Monahan
School of Earth and Ocean Sciences, University of Victoria, Victoria, British Columbia, Canada
Knut von Salzen
Canadian Centre for Climate Modelling and Analysis, Environment and Climate Change, Victoria, British Columbia, Canada
Antonis Gkikas
Institute for Astronomy, Astrophysics, Space Applications and Remote Sensing, National Observatory of Athens (IAASARS/NOA), Athens, Greece
Research Centre for Atmospheric Physics and Climatology, Academy of Athens, Athens, Greece
Qianqian Song
Atmospheric and Oceanic Sciences Program, Princeton University, Princeton, NJ, USA
Zhibo Zhang
Physics Department, University of Maryland, Baltimore County, Baltimore, Maryland, USA
Goddard Earth Sciences Technology and Research II, University of Maryland, Baltimore County, Baltimore, MD 21250, USA
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Atmos. Chem. Phys., 23, 637–661, https://doi.org/10.5194/acp-23-637-2023, https://doi.org/10.5194/acp-23-637-2023, 2023
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This study summarizes recent research on ozone in the Arctic, a sensitive and rapidly warming region. We find that the seasonal cycles of near-surface atmospheric ozone are variable depending on whether they are near the coast, inland, or at high altitude. Several global model simulations were evaluated, and we found that because models lack some of the ozone chemistry that is important for the coastal Arctic locations, they do not accurately simulate ozone there.
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Atmos. Chem. Phys., 22, 15703–15727, https://doi.org/10.5194/acp-22-15703-2022, https://doi.org/10.5194/acp-22-15703-2022, 2022
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Sjoukje Y. Philip, Sarah F. Kew, Geert Jan van Oldenborgh, Faron S. Anslow, Sonia I. Seneviratne, Robert Vautard, Dim Coumou, Kristie L. Ebi, Julie Arrighi, Roop Singh, Maarten van Aalst, Carolina Pereira Marghidan, Michael Wehner, Wenchang Yang, Sihan Li, Dominik L. Schumacher, Mathias Hauser, Rémy Bonnet, Linh N. Luu, Flavio Lehner, Nathan Gillett, Jordis S. Tradowsky, Gabriel A. Vecchi, Chris Rodell, Roland B. Stull, Rosie Howard, and Friederike E. L. Otto
Earth Syst. Dynam., 13, 1689–1713, https://doi.org/10.5194/esd-13-1689-2022, https://doi.org/10.5194/esd-13-1689-2022, 2022
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Huilin Huang, Yun Qian, Ye Liu, Cenlin He, Jianyu Zheng, Zhibo Zhang, and Antonis Gkikas
Atmos. Chem. Phys., 22, 15469–15488, https://doi.org/10.5194/acp-22-15469-2022, https://doi.org/10.5194/acp-22-15469-2022, 2022
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Qianqian Song, Zhibo Zhang, Hongbin Yu, Jasper F. Kok, Claudia Di Biagio, Samuel Albani, Jianyu Zheng, and Jiachen Ding
Atmos. Chem. Phys., 22, 13115–13135, https://doi.org/10.5194/acp-22-13115-2022, https://doi.org/10.5194/acp-22-13115-2022, 2022
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Eleni Drakaki, Vassilis Amiridis, Alexandra Tsekeri, Antonis Gkikas, Emmanouil Proestakis, Sotirios Mallios, Stavros Solomos, Christos Spyrou, Eleni Marinou, Claire L. Ryder, Demetri Bouris, and Petros Katsafados
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State-of-the-art atmospheric dust models have limitations in accounting for a realistic dust size distribution (emission, transport). We modify the parameterization of the mineral dust cycle by including particles with diameter >20 μm, as indicated by observations over deserts. Moreover, we investigate the effects of reduced settling velocities of dust particles. Model results are evaluated using airborne and spaceborne dust measurements above Cabo Verde.
Cynthia H. Whaley, Rashed Mahmood, Knut von Salzen, Barbara Winter, Sabine Eckhardt, Stephen Arnold, Stephen Beagley, Silvia Becagli, Rong-You Chien, Jesper Christensen, Sujay Manish Damani, Xinyi Dong, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Fabio Giardi, Wanmin Gong, Jens Liengaard Hjorth, Lin Huang, Ulas Im, Yugo Kanaya, Srinath Krishnan, Zbigniew Klimont, Thomas Kühn, Joakim Langner, Kathy S. Law, Louis Marelle, Andreas Massling, Dirk Olivié, Tatsuo Onishi, Naga Oshima, Yiran Peng, David A. Plummer, Olga Popovicheva, Luca Pozzoli, Jean-Christophe Raut, Maria Sand, Laura N. Saunders, Julia Schmale, Sangeeta Sharma, Ragnhild Bieltvedt Skeie, Henrik Skov, Fumikazu Taketani, Manu A. Thomas, Rita Traversi, Kostas Tsigaridis, Svetlana Tsyro, Steven Turnock, Vito Vitale, Kaley A. Walker, Minqi Wang, Duncan Watson-Parris, and Tahya Weiss-Gibbons
Atmos. Chem. Phys., 22, 5775–5828, https://doi.org/10.5194/acp-22-5775-2022, https://doi.org/10.5194/acp-22-5775-2022, 2022
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Air pollutants, like ozone and soot, play a role in both global warming and air quality. Atmospheric models are often used to provide information to policy makers about current and future conditions under different emissions scenarios. In order to have confidence in those simulations, in this study we compare simulated air pollution from 18 state-of-the-art atmospheric models to measured air pollution in order to assess how well the models perform.
Hengqi Wang, Yiran Peng, Knut von Salzen, Yan Yang, Wei Zhou, and Delong Zhao
Geosci. Model Dev., 15, 2949–2971, https://doi.org/10.5194/gmd-15-2949-2022, https://doi.org/10.5194/gmd-15-2949-2022, 2022
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The aerosol activation scheme is an important part of the general circulation model, but evaluations using observed data are mostly regional. This research introduced a numerically efficient aerosol activation scheme and evaluated it by using stratus and stratocumulus cloud data sampled during multiple aircraft campaigns in Canada, Chile, Brazil, and China. The decent performance indicates that the scheme is suitable for simulations of cloud droplet number concentrations over wide conditions.
Po-Lun Ma, Bryce E. Harrop, Vincent E. Larson, Richard B. Neale, Andrew Gettelman, Hugh Morrison, Hailong Wang, Kai Zhang, Stephen A. Klein, Mark D. Zelinka, Yuying Zhang, Yun Qian, Jin-Ho Yoon, Christopher R. Jones, Meng Huang, Sheng-Lun Tai, Balwinder Singh, Peter A. Bogenschutz, Xue Zheng, Wuyin Lin, Johannes Quaas, Hélène Chepfer, Michael A. Brunke, Xubin Zeng, Johannes Mülmenstädt, Samson Hagos, Zhibo Zhang, Hua Song, Xiaohong Liu, Michael S. Pritchard, Hui Wan, Jingyu Wang, Qi Tang, Peter M. Caldwell, Jiwen Fan, Larry K. Berg, Jerome D. Fast, Mark A. Taylor, Jean-Christophe Golaz, Shaocheng Xie, Philip J. Rasch, and L. Ruby Leung
Geosci. Model Dev., 15, 2881–2916, https://doi.org/10.5194/gmd-15-2881-2022, https://doi.org/10.5194/gmd-15-2881-2022, 2022
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An alternative set of parameters for E3SM Atmospheric Model version 1 has been developed based on a tuning strategy that focuses on clouds. When clouds in every regime are improved, other aspects of the model are also improved, even though they are not the direct targets for calibration. The recalibrated model shows a lower sensitivity to anthropogenic aerosols and surface warming, suggesting potential improvements to the simulated climate in the past and future.
Antonis Gkikas, Emmanouil Proestakis, Vassilis Amiridis, Stelios Kazadzis, Enza Di Tomaso, Eleni Marinou, Nikos Hatzianastassiou, Jasper F. Kok, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 22, 3553–3578, https://doi.org/10.5194/acp-22-3553-2022, https://doi.org/10.5194/acp-22-3553-2022, 2022
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We present a comprehensive climatological analysis of dust optical depth (DOD) relying on the MIDAS dataset. MIDAS provides columnar mid-visible (550 nm) DOD at fine spatial resolution (0.1° × 0.1°) over a 15-year period (2003–2017). In the current study, the analysis is performed at various spatial (from regional to global) and temporal (from months to years) scales. More specifically, focus is given to specific regions hosting the major dust sources as well as downwind areas of the planet.
Julia Schmale, Sangeeta Sharma, Stefano Decesari, Jakob Pernov, Andreas Massling, Hans-Christen Hansson, Knut von Salzen, Henrik Skov, Elisabeth Andrews, Patricia K. Quinn, Lucia M. Upchurch, Konstantinos Eleftheriadis, Rita Traversi, Stefania Gilardoni, Mauro Mazzola, James Laing, and Philip Hopke
Atmos. Chem. Phys., 22, 3067–3096, https://doi.org/10.5194/acp-22-3067-2022, https://doi.org/10.5194/acp-22-3067-2022, 2022
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Long-term data sets of Arctic aerosol properties from 10 stations across the Arctic provide evidence that anthropogenic influence on the Arctic atmospheric chemical composition has declined in winter, a season which is typically dominated by mid-latitude emissions. The number of significant trends in summer is smaller than in winter, and overall the pattern is ambiguous with some significant positive and negative trends. This reflects the mixed influence of natural and anthropogenic emissions.
Justin A. Covert, David B. Mechem, and Zhibo Zhang
Atmos. Chem. Phys., 22, 1159–1174, https://doi.org/10.5194/acp-22-1159-2022, https://doi.org/10.5194/acp-22-1159-2022, 2022
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Stratocumulus play an important role in Earth's radiative balance. The simulation of these cloud systems in climate models is difficult due to the scale at which cloud microphysical processes occur compared with model grid sizes. In this study, we use large-eddy simulation to analyze subgrid-scale variability of cloud water and its implications on a cloud water to drizzle model enhancement factor E. We find current values of E may be too large and that E should be vertically dependent in models.
Stavros-Andreas Logothetis, Vasileios Salamalikis, Antonis Gkikas, Stelios Kazadzis, Vassilis Amiridis, and Andreas Kazantzidis
Atmos. Chem. Phys., 21, 16499–16529, https://doi.org/10.5194/acp-21-16499-2021, https://doi.org/10.5194/acp-21-16499-2021, 2021
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This study investigates the temporal trends of dust optical depth (DOD; 550 nm) on global, regional and seasonal scales over a 15-year period (2003–2017) using the MIDAS (ModIs Dust AeroSol) dataset. The findings of this study revealed that the DOD was increased across the central Sahara and the Arabian Peninsula, with opposite trends over the eastern and western Sahara, the Thar and Gobi deserts, in the Bodélé Depression, and in the southern Mediterranean.
Qianqian Song, Zhibo Zhang, Hongbin Yu, Paul Ginoux, and Jerry Shen
Atmos. Chem. Phys., 21, 13369–13395, https://doi.org/10.5194/acp-21-13369-2021, https://doi.org/10.5194/acp-21-13369-2021, 2021
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We present a satellite-derived global dust climatological record over the last two decades, including the monthly mean visible dust optical depth (DAOD) and vertical distribution of dust extinction coefficient at a 2º × 5º spatial resolution derived from CALIOP and MODIS. In addition, the CALIOP climatological dataset also includes dust vertical extinction profiles. Based on these two datasets, we carried out a comprehensive comparative study of the spatial and temporal climatology of dust.
Hongbin Yu, Qian Tan, Lillian Zhou, Yaping Zhou, Huisheng Bian, Mian Chin, Claire L. Ryder, Robert C. Levy, Yaswant Pradhan, Yingxi Shi, Qianqian Song, Zhibo Zhang, Peter R. Colarco, Dongchul Kim, Lorraine A. Remer, Tianle Yuan, Olga Mayol-Bracero, and Brent N. Holben
Atmos. Chem. Phys., 21, 12359–12383, https://doi.org/10.5194/acp-21-12359-2021, https://doi.org/10.5194/acp-21-12359-2021, 2021
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This study characterizes a historic African dust intrusion into the Caribbean Basin in June 2020 using satellites and NASA GEOS. Dust emissions in West Africa were large albeit not extreme. However, a unique synoptic system accumulated the dust near the coast for about 4 d before it was ventilated. Although GEOS reproduced satellite-observed plume tracks well, it substantially underestimated dust emissions and did not lift up dust high enough for ensuing long-range transport.
Robin D. Lamboll, Chris D. Jones, Ragnhild B. Skeie, Stephanie Fiedler, Bjørn H. Samset, Nathan P. Gillett, Joeri Rogelj, and Piers M. Forster
Geosci. Model Dev., 14, 3683–3695, https://doi.org/10.5194/gmd-14-3683-2021, https://doi.org/10.5194/gmd-14-3683-2021, 2021
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Lockdowns to avoid the spread of COVID-19 have created an unprecedented reduction in human emissions. We can estimate the changes in emissions at a country level, but to make predictions about how this will affect our climate, we need more precise information about where the emissions happen. Here we combine older estimates of where emissions normally occur with very recent estimates of sector activity levels to enable different groups to make simulations of the climatic effects of lockdown.
Zhibo Zhang, Qianqian Song, David B. Mechem, Vincent E. Larson, Jian Wang, Yangang Liu, Mikael K. Witte, Xiquan Dong, and Peng Wu
Atmos. Chem. Phys., 21, 3103–3121, https://doi.org/10.5194/acp-21-3103-2021, https://doi.org/10.5194/acp-21-3103-2021, 2021
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This study investigates the small-scale variations and covariations of cloud microphysical properties, namely, cloud liquid water content and cloud droplet number concentration, in marine boundary layer clouds based on in situ observation from the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) campaign. We discuss the dependence of cloud variations on vertical location in cloud and the implications for warm-rain simulations in the global climate models.
Antonis Gkikas, Emmanouil Proestakis, Vassilis Amiridis, Stelios Kazadzis, Enza Di Tomaso, Alexandra Tsekeri, Eleni Marinou, Nikos Hatzianastassiou, and Carlos Pérez García-Pando
Atmos. Meas. Tech., 14, 309–334, https://doi.org/10.5194/amt-14-309-2021, https://doi.org/10.5194/amt-14-309-2021, 2021
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We present the development of the MIDAS (ModIs Dust AeroSol) data set, providing daily dust optical depth (DOD; 550 nm) at a global scale and fine spatial resolution (0.1° x 0.1°) over a 15-year period (2003–2017). It has been developed via the synergy of MODIS-Aqua and MERRA-2 data, while CALIOP and AERONET retrievals are used for its assessment. MIDAS upgrades existing dust observational capabilities, and it is suitable for dust climatological studies, model evaluation, and data assimilation.
Anna Gialitaki, Alexandra Tsekeri, Vassilis Amiridis, Romain Ceolato, Lucas Paulien, Anna Kampouri, Antonis Gkikas, Stavros Solomos, Eleni Marinou, Moritz Haarig, Holger Baars, Albert Ansmann, Tatyana Lapyonok, Anton Lopatin, Oleg Dubovik, Silke Groß, Martin Wirth, Maria Tsichla, Ioanna Tsikoudi, and Dimitris Balis
Atmos. Chem. Phys., 20, 14005–14021, https://doi.org/10.5194/acp-20-14005-2020, https://doi.org/10.5194/acp-20-14005-2020, 2020
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Stratospheric smoke particles are found to significantly depolarize incident light, while this effect is also accompanied by a strong spectral dependence. We utilize scattering simulations to show that this behaviour can be attributed to the near-spherical shape of the particles. We also examine whether an extension of the current AERONET scattering model to include the near-spherical shapes could be of benefit to the AERONET retrieval for stratospheric smoke associated with enhanced PLDR.
Landon A. Rieger, Jason N. S. Cole, John C. Fyfe, Stephen Po-Chedley, Philip J. Cameron-Smith, Paul J. Durack, Nathan P. Gillett, and Qi Tang
Geosci. Model Dev., 13, 4831–4843, https://doi.org/10.5194/gmd-13-4831-2020, https://doi.org/10.5194/gmd-13-4831-2020, 2020
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Recently, the stratospheric aerosol forcing dataset used as an input to the Coupled Model Intercomparison Project phase 6 was updated. This work explores the impact of those changes on the modelled historical climates in the CanESM5 and EAMv1 models. Temperature differences in the stratosphere shortly after the Pinatubo eruption are found to be significant, but surface temperatures and precipitation do not show a significant change.
Chenxi Wang, Steven Platnick, Kerry Meyer, Zhibo Zhang, and Yaping Zhou
Atmos. Meas. Tech., 13, 2257–2277, https://doi.org/10.5194/amt-13-2257-2020, https://doi.org/10.5194/amt-13-2257-2020, 2020
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A machine-learning (ML)-based approach that can be used for cloud mask and phase detection is developed. An all-day model that uses infrared (IR) observations and a daytime model that uses shortwave and IR observations from a passive instrument are trained separately for different surface types. The training datasets are selected by using reference pixel types from collocated space lidar. The ML approach is validated carefully and the overall performance is better than traditional methods.
Christine Aebi, Julian Gröbner, Stelios Kazadzis, Laurent Vuilleumier, Antonis Gkikas, and Niklaus Kämpfer
Atmos. Meas. Tech., 13, 907–923, https://doi.org/10.5194/amt-13-907-2020, https://doi.org/10.5194/amt-13-907-2020, 2020
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Clouds are one of the largest sources of uncertainties in climate models. The current study estimates the cloud optical thickness (COT), the effective droplet radius and the single scattering albedo of stratus–altostratus and cirrus–cirrostratus clouds in Payerne, Switzerland, by combining ground- and satellite-based measurements and radiative transfer models. The estimated values are thereafter compared with data retrieved from other methods. The mean COT is distinct for different seasons.
Neil C. Swart, Jason N. S. Cole, Viatcheslav V. Kharin, Mike Lazare, John F. Scinocca, Nathan P. Gillett, James Anstey, Vivek Arora, James R. Christian, Sarah Hanna, Yanjun Jiao, Warren G. Lee, Fouad Majaess, Oleg A. Saenko, Christian Seiler, Clint Seinen, Andrew Shao, Michael Sigmond, Larry Solheim, Knut von Salzen, Duo Yang, and Barbara Winter
Geosci. Model Dev., 12, 4823–4873, https://doi.org/10.5194/gmd-12-4823-2019, https://doi.org/10.5194/gmd-12-4823-2019, 2019
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The Canadian Earth System Model version 5 (CanESM5) is a global model developed to simulate historical climate change and variability, to make centennial-scale projections of future climate, and to produce initialized seasonal and decadal predictions. This paper describes the model components and quantifies the model performance. CanESM5 simulations contribute to the Coupled Model Intercomparison Project phase 6 (CMIP6) and will be employed for climate science applications in Canada.
Carsten Abraham, Amber M. Holdsworth, and Adam H. Monahan
Nonlin. Processes Geophys., 26, 401–427, https://doi.org/10.5194/npg-26-401-2019, https://doi.org/10.5194/npg-26-401-2019, 2019
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Atmospheric stably stratified boundary layers display transitions between regimes of sustained and intermittent turbulence. These transitions are not well represented in numerical weather prediction and climate models. A prototype explicitly stochastic turbulence parameterization simulating regime dynamics is presented and tested in an idealized model. Results demonstrate that the approach can improve the regime representation in models.
Chris D. Jones, Thomas L. Frölicher, Charles Koven, Andrew H. MacDougall, H. Damon Matthews, Kirsten Zickfeld, Joeri Rogelj, Katarzyna B. Tokarska, Nathan P. Gillett, Tatiana Ilyina, Malte Meinshausen, Nadine Mengis, Roland Séférian, Michael Eby, and Friedrich A. Burger
Geosci. Model Dev., 12, 4375–4385, https://doi.org/10.5194/gmd-12-4375-2019, https://doi.org/10.5194/gmd-12-4375-2019, 2019
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Global warming is simply related to the total emission of CO2 allowing us to define a carbon budget. However, information on the Zero Emissions Commitment is a key missing link to assess remaining carbon budgets to achieve the climate targets of the Paris Agreement. It was therefore decided that a small targeted MIP activity to fill this knowledge gap would be extremely valuable. This article formalises the experimental design alongside the other CMIP6 documentation papers.
Fei Lu, Nils Weitzel, and Adam H. Monahan
Nonlin. Processes Geophys., 26, 227–250, https://doi.org/10.5194/npg-26-227-2019, https://doi.org/10.5194/npg-26-227-2019, 2019
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ll-posedness of the inverse problem and sparse noisy data are two major challenges in the modeling of high-dimensional spatiotemporal processes. We present a Bayesian inference method with a strongly regularized posterior to overcome these challenges, enabling joint state-parameter estimation and quantifying uncertainty in the estimation. We demonstrate the method on a physically motivated nonlinear stochastic partial differential equation arising from paleoclimate construction.
Hakase Hayashida, James R. Christian, Amber M. Holdsworth, Xianmin Hu, Adam H. Monahan, Eric Mortenson, Paul G. Myers, Olivier G. J. Riche, Tessa Sou, and Nadja S. Steiner
Geosci. Model Dev., 12, 1965–1990, https://doi.org/10.5194/gmd-12-1965-2019, https://doi.org/10.5194/gmd-12-1965-2019, 2019
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Ice algae, the primary producer in sea ice, play a fundamental role in shaping marine ecosystems and biogeochemical cycling of key elements in polar regions. In this study, we developed a process-based numerical model component representing sea-ice biogeochemistry for a sea ice–ocean coupled general circulation model. The model developed can be used to simulate the projected changes in sea-ice ecosystems and biogeochemistry in response to on-going rapid decline of the Arctic.
Antonio Di Noia, Otto P. Hasekamp, Bastiaan van Diedenhoven, and Zhibo Zhang
Atmos. Meas. Tech., 12, 1697–1716, https://doi.org/10.5194/amt-12-1697-2019, https://doi.org/10.5194/amt-12-1697-2019, 2019
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We present a neural network algorithm for the retrieval of cloud physical properties from multi-angle polarimetric measurements. We have trained the algorithm on a large dataset of synthetic measurements and applied it to a year of POLDER-3 data. A comparison against MODIS cloud products reveals that our algorithm is capable of performing cloud property retrievals on a global scale and possibly improves the estimates of cloud effective radius over land with respect to existing POLDER-3 products.
Zhibo Zhang, Hua Song, Po-Lun Ma, Vincent E. Larson, Minghuai Wang, Xiquan Dong, and Jianwu Wang
Atmos. Chem. Phys., 19, 1077–1096, https://doi.org/10.5194/acp-19-1077-2019, https://doi.org/10.5194/acp-19-1077-2019, 2019
Peng Wu, Baike Xi, Xiquan Dong, and Zhibo Zhang
Atmos. Chem. Phys., 18, 17405–17420, https://doi.org/10.5194/acp-18-17405-2018, https://doi.org/10.5194/acp-18-17405-2018, 2018
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Prescribed autoconversion and accretion enhancement factors in GCM warm-rain parameterizations contribute partially to the too-frequent and too-light problem in precipitation simulation. The two factors should be regime- and resolution-dependent. A decreased autoconversion enhancement factor and increased accretion enhancement factor in the Morrison and Gettleman (2008) scheme can improve the simulated precipitation frequency and intensity. The two factors for other schemes are also suggested.
Qianqian Song, Zhibo Zhang, Hongbin Yu, Seiji Kato, Ping Yang, Peter Colarco, Lorraine A. Remer, and Claire L. Ryder
Atmos. Chem. Phys., 18, 11303–11322, https://doi.org/10.5194/acp-18-11303-2018, https://doi.org/10.5194/acp-18-11303-2018, 2018
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Mineral dust is the most abundant atmospheric aerosol component in terms of dry mass. In this study, we integrate recent aircraft measurements of dust microphysical and optical properties with satellite retrievals of aerosol and radiative fluxes to quantify the dust direct radiative effects on the shortwave and longwave radiation at both the top of the atmosphere and the surface in the tropical North Atlantic during summer months.
Hua Song, Zhibo Zhang, Po-Lun Ma, Steven Ghan, and Minghuai Wang
Geosci. Model Dev., 11, 3147–3158, https://doi.org/10.5194/gmd-11-3147-2018, https://doi.org/10.5194/gmd-11-3147-2018, 2018
Daniel J. Miller, Zhibo Zhang, Steven Platnick, Andrew S. Ackerman, Frank Werner, Celine Cornet, and Kirk Knobelspiesse
Atmos. Meas. Tech., 11, 3689–3715, https://doi.org/10.5194/amt-11-3689-2018, https://doi.org/10.5194/amt-11-3689-2018, 2018
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Prior satellite comparisons of bispectral and polarimetric cloud droplet size retrievals exhibited systematic biases. However, similar airborne instrument retrievals have been found to be quite similar to one another. This study explains this discrepancy in terms of differing sensitivity to vertical profile, as well as spatial and angular resolution. This is accomplished by using a satellite retrieval simulator – an LES cloud model coupled to radiative transfer and cloud retrieval algorithms.
Antonis Gkikas, Vincenzo Obiso, Carlos Pérez García-Pando, Oriol Jorba, Nikos Hatzianastassiou, Lluis Vendrell, Sara Basart, Stavros Solomos, Santiago Gassó, and José Maria Baldasano
Atmos. Chem. Phys., 18, 8757–8787, https://doi.org/10.5194/acp-18-8757-2018, https://doi.org/10.5194/acp-18-8757-2018, 2018
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The present study investigates the direct radiative effects (DREs), induced during 20 intense Mediterranean desert dust outbreaks, based on regional short-term numerical simulations of the NMMB-MONARCH model: more specifically, (i) the DREs and their associated impacts on temperature and surface sensible and latent heat fluxes, (ii) the feedbacks on dust AOD and dust emissions, and (iii) the possible improvements in short-term forecasts (up to 84 h) of temperature and radiation.
Gerald M. Lohmann and Adam H. Monahan
Atmos. Meas. Tech., 11, 3131–3144, https://doi.org/10.5194/amt-11-3131-2018, https://doi.org/10.5194/amt-11-3131-2018, 2018
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Using high-resolution surface irradiance data with original temporal resolutions between 0.01 s and 1 s from six different locations in the Northern Hemisphere, we characterize the changes in representation of temporal variability resulting from time averaging. Our results indicate that a temporal averaging time scale of around 1 s marks a transition in representing single-point irradiance variability, such that longer averages result in substantial underestimates of variability.
Adam H. Monahan
Nonlin. Processes Geophys., 25, 335–353, https://doi.org/10.5194/npg-25-335-2018, https://doi.org/10.5194/npg-25-335-2018, 2018
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Bivariate probability density functions (pdfs) of wind speed characterize the relationship between speeds at two different locations or times. This study develops such pdfs of wind speed from distributions of the components, following a well-established approach for univariate distributions. The ability of these models to characterize example observed datasets is assessed. The mathematical complexity of these models suggests further extensions of this line of reasoning may not be practical.
Paul J. Kushner, Lawrence R. Mudryk, William Merryfield, Jaison T. Ambadan, Aaron Berg, Adéline Bichet, Ross Brown, Chris Derksen, Stephen J. Déry, Arlan Dirkson, Greg Flato, Christopher G. Fletcher, John C. Fyfe, Nathan Gillett, Christian Haas, Stephen Howell, Frédéric Laliberté, Kelly McCusker, Michael Sigmond, Reinel Sospedra-Alfonso, Neil F. Tandon, Chad Thackeray, Bruno Tremblay, and Francis W. Zwiers
The Cryosphere, 12, 1137–1156, https://doi.org/10.5194/tc-12-1137-2018, https://doi.org/10.5194/tc-12-1137-2018, 2018
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Here, the Canadian research network CanSISE uses state-of-the-art observations of snow and sea ice to assess how Canada's climate model and climate prediction systems capture variability in snow, sea ice, and related climate parameters. We find that the system performs well, accounting for observational uncertainty (especially for snow), model uncertainty, and chaotic climate variability. Even for variables like sea ice, where improvement is needed, useful prediction tools can be developed.
Heming Bai, Cheng Gong, Minghuai Wang, Zhibo Zhang, and Tristan L'Ecuyer
Atmos. Chem. Phys., 18, 1763–1783, https://doi.org/10.5194/acp-18-1763-2018, https://doi.org/10.5194/acp-18-1763-2018, 2018
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Precipitation susceptibility to aerosol perturbation plays a key role in understanding aerosol–cloud interactions and for constraining aerosol indirect effects. Here, multisensor aerosol and cloud products from A-Train satellites are analyzed to estimate precipitation susceptibility. Compared to precipitation intensity susceptibility, precipitation frequency susceptibility demonstrates relatively robust features across different retrieval products.
Hakase Hayashida, Nadja Steiner, Adam Monahan, Virginie Galindo, Martine Lizotte, and Maurice Levasseur
Biogeosciences, 14, 3129–3155, https://doi.org/10.5194/bg-14-3129-2017, https://doi.org/10.5194/bg-14-3129-2017, 2017
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In remote regions, cloud conditions may be strongly influenced by oceanic source of dimethylsulfide (DMS) produced by plankton and bacteria. In the Arctic, sea ice provides an additional source of these aerosols. The results of this study highlight the importance of taking into account both the sea-ice sulfur cycle and ecosystem in the flux estimates of oceanic DMS near the ice margins and identify key uncertainties in processes and rates that would be better constrained by new observations.
Daniel Mitchell, Krishna AchutaRao, Myles Allen, Ingo Bethke, Urs Beyerle, Andrew Ciavarella, Piers M. Forster, Jan Fuglestvedt, Nathan Gillett, Karsten Haustein, William Ingram, Trond Iversen, Viatcheslav Kharin, Nicholas Klingaman, Neil Massey, Erich Fischer, Carl-Friedrich Schleussner, John Scinocca, Øyvind Seland, Hideo Shiogama, Emily Shuckburgh, Sarah Sparrow, Dáithí Stone, Peter Uhe, David Wallom, Michael Wehner, and Rashyd Zaaboul
Geosci. Model Dev., 10, 571–583, https://doi.org/10.5194/gmd-10-571-2017, https://doi.org/10.5194/gmd-10-571-2017, 2017
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This paper provides an experimental design to assess impacts of a world that is 1.5 °C warmer than at pre-industrial levels. The design is a new way to approach impacts from the climate community, and aims to answer questions related to the recent Paris Agreement. In particular the paper provides a method for studying extreme events under relatively high mitigation scenarios.
Frank Werner, Galina Wind, Zhibo Zhang, Steven Platnick, Larry Di Girolamo, Guangyu Zhao, Nandana Amarasinghe, and Kerry Meyer
Atmos. Meas. Tech., 9, 5869–5894, https://doi.org/10.5194/amt-9-5869-2016, https://doi.org/10.5194/amt-9-5869-2016, 2016
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A research–level retrieval algorithm for cloud optical and microphysical properties is developed for the Advanced Spaceborne Thermal Emission and Reflection Radiometer (ASTER) aboard the Terra satellite. This yields reliable estimates of important cloud variables at a horizontal resolution of 30 m. Comparisons of the ASTER retrieval results with the operational cloud products from the Moderate Resolution Imaging Spectroradiometer (MODIS) show a high agreement for 48 example cloud fields.
Nathan P. Gillett, Hideo Shiogama, Bernd Funke, Gabriele Hegerl, Reto Knutti, Katja Matthes, Benjamin D. Santer, Daithi Stone, and Claudia Tebaldi
Geosci. Model Dev., 9, 3685–3697, https://doi.org/10.5194/gmd-9-3685-2016, https://doi.org/10.5194/gmd-9-3685-2016, 2016
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Detection and attribution of climate change is the process of determining the causes of observed climate changes, which has underpinned key conclusions on the role of human influence on climate in the reports of the Intergovernmental Panel on Climate Change (IPCC). This paper describes a coordinated set of climate model experiments that will form part of the Sixth Coupled Model Intercomparison Project and will support improved attribution of climate change in the next IPCC report.
Jan-Erik Tesdal, James R. Christian, Adam H. Monahan, and Knut von Salzen
Atmos. Chem. Phys., 16, 10847–10864, https://doi.org/10.5194/acp-16-10847-2016, https://doi.org/10.5194/acp-16-10847-2016, 2016
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A global atmosphere model with explicit representation of aerosol processes is used to assess uncertainties in the climate impact of ocean DMS efflux and the role of spatial and temporal variability of the DMS flux in the effect on climate. The radiative effect of sulfate is nearly linearly related to global total DMS flux. Removing the spatial or temporal variability of DMS flux changes the global radiation budget, but the effect is of second-order importance relative to the global mean flux.
Antonis Gkikas, Sara Basart, Nikos Hatzianastassiou, Eleni Marinou, Vassilis Amiridis, Stelios Kazadzis, Jorge Pey, Xavier Querol, Oriol Jorba, Santiago Gassó, and José Maria Baldasano
Atmos. Chem. Phys., 16, 8609–8642, https://doi.org/10.5194/acp-16-8609-2016, https://doi.org/10.5194/acp-16-8609-2016, 2016
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This study presents the 3-D structures of intense Mediterranean desert dust outbreaks, over the period Mar 2000–Feb 2013. The desert dust (DD) episodes are identified through an objective and dynamic algorithm, which utilizes satellite retrievals (MODIS, TOMS and OMI) as inputs. The performance of the satellite algorithm is evaluated vs. AERONET and PM10 data. The geometrical characteristics of the identified DD episodes are analyzed using the collocated CALIOP profiles as a complementary tool.
Gerald M. Lohmann, Adam H. Monahan, and Detlev Heinemann
Atmos. Chem. Phys., 16, 6365–6379, https://doi.org/10.5194/acp-16-6365-2016, https://doi.org/10.5194/acp-16-6365-2016, 2016
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Increasing numbers of photovoltaic (PV) power systems call for the characterization of irradiance variability with very high spatiotemporal resolution. We use 1 Hz irradiance data recorded by as many as 99 pyranometers and show mixed sky conditions to differ substantially from clear and overcast skies. For example, the probabilities of strong fluctuations and their respective spatial autocorrelation structures are appreciably distinct under mixed conditions.
Zhibo Zhang, Kerry Meyer, Hongbin Yu, Steven Platnick, Peter Colarco, Zhaoyan Liu, and Lazaros Oreopoulos
Atmos. Chem. Phys., 16, 2877–2900, https://doi.org/10.5194/acp-16-2877-2016, https://doi.org/10.5194/acp-16-2877-2016, 2016
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The frequency of occurrence and shortwave direct radiative effects (DRE) of above-cloud aerosols (ACAs) over global oceans are investigated using 8 years of collocated CALIOP and MODIS observations. We estimated that ACAs have a global ocean annual mean diurnally averaged cloudy-sky DRE of 0.015 W m−2 (range of −0.03 to 0.06 W m−2) at TOA. The DREs at surface and within atmosphere are −0.15 W m−2 (range of −0.09 to −0.21 W m−2), and 0.17 W m−2 (range of 0.11 to 0.24 W m−2), respectively.
M. B. Korras-Carraca, N. Hatzianastassiou, C. Matsoukas, A. Gkikas, and C. D. Papadimas
Atmos. Chem. Phys., 15, 13113–13132, https://doi.org/10.5194/acp-15-13113-2015, https://doi.org/10.5194/acp-15-13113-2015, 2015
M. Taylor, S. Kazadzis, A. Tsekeri, A. Gkikas, and V. Amiridis
Atmos. Meas. Tech., 7, 3151–3175, https://doi.org/10.5194/amt-7-3151-2014, https://doi.org/10.5194/amt-7-3151-2014, 2014
Z. Zhang, K. Meyer, S. Platnick, L. Oreopoulos, D. Lee, and H. Yu
Atmos. Meas. Tech., 7, 1777–1789, https://doi.org/10.5194/amt-7-1777-2014, https://doi.org/10.5194/amt-7-1777-2014, 2014
A. Gkikas, N. Hatzianastassiou, N. Mihalopoulos, V. Katsoulis, S. Kazadzis, J. Pey, X. Querol, and O. Torres
Atmos. Chem. Phys., 13, 12135–12154, https://doi.org/10.5194/acp-13-12135-2013, https://doi.org/10.5194/acp-13-12135-2013, 2013
V. Amiridis, U. Wandinger, E. Marinou, E. Giannakaki, A. Tsekeri, S. Basart, S. Kazadzis, A. Gkikas, M. Taylor, J. Baldasano, and A. Ansmann
Atmos. Chem. Phys., 13, 12089–12106, https://doi.org/10.5194/acp-13-12089-2013, https://doi.org/10.5194/acp-13-12089-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Dust-producing weather patterns of the North American Great Plains
High-resolution air quality maps for Bucharest using a mixed-effects modeling framework
Construction and application of a pollen emissions model based on phenology and random forests
The impact of uncertainty in black carbon's refractive index on simulated optical depth and radiative forcing
Characterization of brown carbon absorption in different European environments through source contribution analysis
Accounting for the black carbon aging process in a two-way coupled meteorology–air quality model
The effectiveness of solar radiation management using fine sea spray across multiple climatic regions
A global dust emission dataset for estimating dust radiative forcings in climate models
Tropospheric aerosols over the western North Atlantic Ocean during the winter and summer deployments of ACTIVATE 2020: life cycle, transport, and distribution
Spatial and temporal evolution of future atmospheric reactive nitrogen deposition in China under different climate change mitigation strategies
Steady-state mixing state of black carbon aerosols from a particle-resolved model
Distinctive dust weather intensities in North China resulted from two types of atmospheric circulation anomalies
Biomass burning emission analysis based on MODIS aerosol optical depth and AeroCom multi-model simulations: implications for model constraints and emission inventories
Quasi-weekly oscillation of regional PM2.5 transport over China driven by the synoptic-scale disturbance of the East Asian winter monsoon circulation
Solar radiation estimation in West Africa: impact of dust conditions during the 2021 dry season
Machine Learning Assisted Inference of the Particle Charge Fraction and the Ion-induced Nucleation Rates during New Particle Formation Events
Gaps in our understanding of ice-nucleating particle sources exposed by global simulation of the UK Earth System Model
The role of interfacial tension in the size-dependent phase separation of atmospheric aerosol particles
Warming effects of reduced sulfur emissions from shipping
The key role of atmospheric absorption in the Asian summer monsoon response to dust emissions in CMIP6 models
Multi-model effective radiative forcing of the 2020 sulfur cap for shipping
Exploring the Aerosol Activation Properties in a Coastal Area Using Cloud and Particle-resolving Models
Representation of iron aerosol size distributions of anthropogenic emissions is critical in evaluating atmospheric soluble iron input to the ocean
Revealing dominant patterns of aerosol regimes in the lower troposphere and their evolution from preindustrial times to the future in global climate model simulations
A Novel Method to Quantify the Uncertainty Contribution of Aerosol-Radiative Interaction Factors
Improving estimation of a record-breaking east Asian dust storm emission with lagged aerosol Ångström exponent observations
Impact of biomass burning aerosols (BBA) on the tropical African climate in an ocean–atmosphere–aerosol coupled climate model
Retrieval of refractive index and water content for the coating materials of aged black carbon aerosol based on optical properties: a theoretical analysis
Impact of post monsoon crop residue burning on PM2.5 over North India: Optimizing emissions using a high-density in situ surface observation network
Predicting hygroscopic growth of organosulfur aerosol particles using COSMOtherm
Dust aerosol from the Aralkum Desert influences the radiation budget and atmospheric dynamics of Central Asia
Global modeling of aerosol nucleation with a semi-explicit chemical mechanism for highly oxygenated organic molecules (HOMs)
How to trace the origins of short-lived atmospheric species in the Arctic
Synergistic effects of the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) on dust activities in North China during the following spring
Aerosol composition, air quality, and boundary layer dynamics in the urban background of Stuttgart in winter
Response of the link between ENSO and the East Asian winter monsoon to Asian anthropogenic aerosols
Measurement report: Source attribution and estimation of black carbon levels in an urban hotspot of the central Po Valley – an integrated approach combining high-resolution dispersion modelling and micro-aethalometers
Modeling CMAQ dry deposition treatment over Western Pacific: A distinct characteristic of mineral dust and anthropogenic aerosol
Microphysical modelling of aerosol scavenging by different types of clouds: description and validation of the approach
Insights into the sources of ultrafine particle numbers at six European urban sites obtained by investigating COVID-19 lockdowns
In-plume and out-of-plume analysis of aerosol–cloud interactions derived from the 2014–2015 Holuhraun volcanic eruption
Impacts of atmospheric circulation patterns and cloud inhibition on aerosol radiative effect and boundary layer structure during winter air pollution in Sichuan Basin, China
Modeling simulation of aerosol light absorption over the Beijing-Tianjin-Hebei region: the impact of mixing state and aging processes
Investigating the sign of stratocumulus adjustments to aerosols in the ICON global storm-resolving model
A model study investigating the sensitivity of aerosol forcing to the volatilities of semi-volatile organic compounds
An Investigation of the Impact of Canadian wildfires on US Air Quality using Satellite, Model and Ground Measurements
Decomposing the effective radiative forcing of anthropogenic aerosols based on CMIP6 Earth system models
Modeling impacts of dust mineralogy on fast climate response
Uncertainties in laboratory-measured shortwave refractive indices of mineral dust aerosols and derived optical properties: a theoretical assessment
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
Stuart Evans
Atmos. Chem. Phys., 25, 4833–4845, https://doi.org/10.5194/acp-25-4833-2025, https://doi.org/10.5194/acp-25-4833-2025, 2025
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This study of the North American Great Plains identifies the various weather patterns responsible for blowing dust in all parts of the region using a weather pattern classification. In the southwestern plains passing cold fronts are the primary cause of dust; in the understudied northern plains, summertime patterns and southerly pre-frontal winds are most important in the west and east, respectively. These results are valuable to understanding and forecasting dust in this complex source region.
Camelia Talianu, Jeni Vasilescu, Doina Nicolae, Alexandru Ilie, Andrei Dandocsi, Anca Nemuc, and Livio Belegante
Atmos. Chem. Phys., 25, 4639–4654, https://doi.org/10.5194/acp-25-4639-2025, https://doi.org/10.5194/acp-25-4639-2025, 2025
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For Bucharest, Romania's capital, mobile measurements during two intensive campaigns and mixed-effect LUR (land-use regression) models to derive seasonal maps of near-surface PM10, NO2 and UFPs (ultrafine particles) have successfully been used. The model's performance was evaluated, demonstrating its potential for high-resolution mapping in other cities with well-characterized urban structures and diverse in situ monitoring stations.
Jiangtao Li, Xingqin An, Zhaobin Sun, Caihua Ye, Qing Hou, Yuxin Zhao, and Zhe Liu
Atmos. Chem. Phys., 25, 3583–3602, https://doi.org/10.5194/acp-25-3583-2025, https://doi.org/10.5194/acp-25-3583-2025, 2025
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Climate change and pollution have intensified pollen allergies. We developed a pollen emissions model using phenology and random forests. Key factors affecting annual pollen emissions include temperature, relative humidity and sunshine hours. Pollen dispersal starts around 10 August, peaks around 30 August and ends by 25 September, lasting about 45 d. Over time, annual pollen emissions exhibit significant fluctuations and a downward trend.
Ruth A. R. Digby, Knut von Salzen, Adam H. Monahan, Nathan P. Gillett, and Jiangnan Li
Atmos. Chem. Phys., 25, 3109–3130, https://doi.org/10.5194/acp-25-3109-2025, https://doi.org/10.5194/acp-25-3109-2025, 2025
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The refractive index of black carbon (BCRI), which determines how much energy black carbon absorbs and scatters, is difficult to measure, and different climate models use different values. We show that varying the BCRI across commonly used values can increase absorbing aerosol optical depth by 42 % and the warming effect from interactions between black carbon and radiation by 47 %, an appreciable fraction of the overall spread between models reported in recent literature assessments.
Hector Navarro-Barboza, Jordi Rovira, Vincenzo Obiso, Andrea Pozzer, Marta Via, Andres Alastuey, Xavier Querol, Noemi Perez, Marjan Savadkoohi, Gang Chen, Jesus Yus-Díez, Matic Ivancic, Martin Rigler, Konstantinos Eleftheriadis, Stergios Vratolis, Olga Zografou, Maria Gini, Benjamin Chazeau, Nicolas Marchand, Andre S. H. Prevot, Kaspar Dallenbach, Mikael Ehn, Krista Luoma, Tuukka Petäjä, Anna Tobler, Jaroslaw Necki, Minna Aurela, Hilkka Timonen, Jarkko Niemi, Olivier Favez, Jean-Eudes Petit, Jean-Philippe Putaud, Christoph Hueglin, Nicolas Pascal, Aurélien Chauvigné, Sébastien Conil, Marco Pandolfi, and Oriol Jorba
Atmos. Chem. Phys., 25, 2667–2694, https://doi.org/10.5194/acp-25-2667-2025, https://doi.org/10.5194/acp-25-2667-2025, 2025
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Brown carbon (BrC) absorbs ultraviolet (UV) and visible light, influencing climate. This study explores BrC's imaginary refractive index (k) using data from 12 European sites. Residential emissions are a major organic aerosol (OA) source in winter, while secondary organic aerosol (SOA) dominates in summer. Source-specific k values were derived, improving model accuracy. The findings highlight BrC's climate impact and emphasize source-specific constraints in atmospheric models.
Yuzhi Jin, Jiandong Wang, Chao Liu, David C. Wong, Golam Sarwar, Kathleen M. Fahey, Shang Wu, Jiaping Wang, Jing Cai, Zeyuan Tian, Zhouyang Zhang, Jia Xing, Aijun Ding, and Shuxiao Wang
Atmos. Chem. Phys., 25, 2613–2630, https://doi.org/10.5194/acp-25-2613-2025, https://doi.org/10.5194/acp-25-2613-2025, 2025
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Black carbon (BC) affects climate and the environment, and its aging process alters its properties. Current models, like WRF-CMAQ, lack full accounting for it. We developed the WRF-CMAQ-BCG model to better represent BC aging by introducing bare and coated BC species and their conversion. The WRF-CMAQ-BCG model introduces the capability to simulate BC mixing states and bare and coated BC wet deposition, and it improves the accuracy of BC mass concentration and aerosol optics.
Zhe Song, Shaocai Yu, Pengfei Li, Ningning Yao, Lang Chen, Yuhai Sun, Boqiong Jiang, and Daniel Rosenfeld
Atmos. Chem. Phys., 25, 2473–2494, https://doi.org/10.5194/acp-25-2473-2025, https://doi.org/10.5194/acp-25-2473-2025, 2025
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Our results with injected sea salt aerosols for five open oceans show that sea salt aerosols with low injection amounts dominate shortwave radiation, mainly through indirect effects. As indirect aerosol effects saturate with increasing injection rates, direct effects exceed indirect effects. This implies that marine cloud brightening is best implemented in areas with extensive cloud cover, while aerosol direct scattering effects remain dominant when clouds are scarce.
Danny M. Leung, Jasper F. Kok, Longlei Li, David M. Lawrence, Natalie M. Mahowald, Simone Tilmes, and Erik Kluzek
Atmos. Chem. Phys., 25, 2311–2331, https://doi.org/10.5194/acp-25-2311-2025, https://doi.org/10.5194/acp-25-2311-2025, 2025
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This study derives a gridded dust emission dataset for 1841–2000 by employing a combination of observed dust from core records and reanalyzed global dust cycle constraints. We evaluate the ability of global models to replicate the observed historical dust variability by using the emission dataset to force a historical simulation in an Earth system model. We show that prescribing our emissions forces the model to better match observations than other mechanistic models.
Hongyu Liu, Bo Zhang, Richard H. Moore, Luke D. Ziemba, Richard A. Ferrare, Hyundeok Choi, Armin Sorooshian, David Painemal, Hailong Wang, Michael A. Shook, Amy Jo Scarino, Johnathan W. Hair, Ewan C. Crosbie, Marta A. Fenn, Taylor J. Shingler, Chris A. Hostetler, Gao Chen, Mary M. Kleb, Gan Luo, Fangqun Yu, Mark A. Vaughan, Yongxiang Hu, Glenn S. Diskin, John B. Nowak, Joshua P. DiGangi, Yonghoon Choi, Christoph A. Keller, and Matthew S. Johnson
Atmos. Chem. Phys., 25, 2087–2121, https://doi.org/10.5194/acp-25-2087-2025, https://doi.org/10.5194/acp-25-2087-2025, 2025
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We use the GEOS-Chem model to simulate aerosol distributions and properties over the western North Atlantic Ocean (WNAO) during the winter and summer deployments in 2020 of the NASA ACTIVATE mission. Model results are evaluated against aircraft, ground-based, and satellite observations. The improved understanding of life cycle, composition, transport pathways, and distribution of aerosols has important implications for characterizing aerosol–cloud–meteorology interactions over WNAO.
Mingrui Ma, Jiachen Cao, Dan Tong, Bo Zheng, and Yu Zhao
Atmos. Chem. Phys., 25, 2147–2166, https://doi.org/10.5194/acp-25-2147-2025, https://doi.org/10.5194/acp-25-2147-2025, 2025
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We combined two global climate change pathways and three national emission control scenarios to analyze the future evolution of reactive nitrogen (Nr) deposition till the 2060s in China with air quality modeling. We show China’s clean air and carbon neutrality policies would overcome the adverse effects of climate change and efficiently reduce Nr deposition. The outflow of Nr fluxes from mainland China to the west Pacific would also be clearly reduced from continuous stringent emission controls.
Zhouyang Zhang, Jiandong Wang, Jiaping Wang, Nicole Riemer, Chao Liu, Yuzhi Jin, Zeyuan Tian, Jing Cai, Yueyue Cheng, Ganzhen Chen, Bin Wang, Shuxiao Wang, and Aijun Ding
Atmos. Chem. Phys., 25, 1869–1881, https://doi.org/10.5194/acp-25-1869-2025, https://doi.org/10.5194/acp-25-1869-2025, 2025
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Black carbon (BC) exerts notable warming effects. We use a particle-resolved model to investigate the long-term behavior of the BC mixing state, revealing its compositions, coating thickness distribution, and optical properties all stabilize with a characteristic time of less than 1 d. This study can effectively simplify the description of the BC mixing state, which facilitates the precise assessment of the optical properties of BC aerosols in global and chemical transport models.
Qianyi Huo, Zhicong Yin, Xiaoqing Ma, and Huijun Wang
Atmos. Chem. Phys., 25, 1711–1724, https://doi.org/10.5194/acp-25-1711-2025, https://doi.org/10.5194/acp-25-1711-2025, 2025
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Dust days during the spring seasons of 2015–2023 in North China were classified into Mongolian cyclone and cold high types depending on the presence of the Mongolian cyclone. The Mongolian cyclone type led to more frequent and severe dust weather, indicated by PM10 concentrations. To comprehensively forecast the two types of dust weather, a common predictor was established based on 500 hPa anomalous circulation systems, offering insights for dust weather forecasting and climate prediction.
Mariya Petrenko, Ralph Kahn, Mian Chin, Susanne E. Bauer, Tommi Bergman, Huisheng Bian, Gabriele Curci, Ben Johnson, Johannes W. Kaiser, Zak Kipling, Harri Kokkola, Xiaohong Liu, Keren Mezuman, Tero Mielonen, Gunnar Myhre, Xiaohua Pan, Anna Protonotariou, Samuel Remy, Ragnhild Bieltvedt Skeie, Philip Stier, Toshihiko Takemura, Kostas Tsigaridis, Hailong Wang, Duncan Watson-Parris, and Kai Zhang
Atmos. Chem. Phys., 25, 1545–1567, https://doi.org/10.5194/acp-25-1545-2025, https://doi.org/10.5194/acp-25-1545-2025, 2025
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We compared smoke plume simulations from 11 global models to each other and to satellite smoke amount observations aimed at constraining smoke source strength. In regions where plumes are thick and background aerosol is low, models and satellites compare well. However, the input emission inventory tends to underestimate in many places, and particle property and loss rate assumptions vary enormously among models, causing uncertainties that require systematic in situ measurements to resolve.
Yongqing Bai, Tianliang Zhao, Kai Meng, Yue Zhou, Jie Xiong, Xiaoyun Sun, Lijuan Shen, Yanyu Yue, Yan Zhu, Weiyang Hu, and Jingyan Yao
Atmos. Chem. Phys., 25, 1273–1287, https://doi.org/10.5194/acp-25-1273-2025, https://doi.org/10.5194/acp-25-1273-2025, 2025
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We proposed a composite statistical method to identify the quasi-weekly oscillation (QWO) of regional PM2.5 transport over China in winter from 2015 to 2019. The QWO of regional PM2.5 transport is constrained by synoptic-scale disturbances of the East Asian winter monsoon circulation with the periodic activities of the Siberian high, providing a new insight into the understanding of regional pollutant transport with meteorological drivers in atmospheric environment changes.
Léo Clauzel, Sandrine Anquetin, Christophe Lavaysse, Gilles Bergametti, Christel Bouet, Guillaume Siour, Rémy Lapere, Béatrice Marticorena, and Jennie Thomas
Atmos. Chem. Phys., 25, 997–1021, https://doi.org/10.5194/acp-25-997-2025, https://doi.org/10.5194/acp-25-997-2025, 2025
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Solar energy production in West Africa is set to rise and needs accurate solar radiation estimates which are affected by desert dust. This work analyses a March 2021 dust event using a modelling strategy incorporating desert dust. Results show that considering desert dust cuts errors in solar radiation estimates by 75 % and reduces surface solar radiation by 18 %. This highlights the importance of incorporating dust aerosols into solar forecasting for better accuracy.
Pan Wang, Yue Zhao, Jiandong Wang, Veli-Matti Kerminen, Jingkun Jiang, and Chenxi Li
EGUsphere, https://doi.org/10.5194/egusphere-2024-3666, https://doi.org/10.5194/egusphere-2024-3666, 2025
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We developed a numerical model to explore how the charge state of newly formed atmospheric particles evolves during growth and how this relates to ion-induced nucleation rates. We identify the governing factors of particle charging and further apply neural networks to predict particle charge states and estimate ion induced nucleation rates. This study offers insights into particle charging dynamics and introduces new methods for assessing ion induced nucleation in atmospheric research.
Ross J. Herbert, Alberto Sanchez-Marroquin, Daniel P. Grosvenor, Kirsty J. Pringle, Stephen R. Arnold, Benjamin J. Murray, and Kenneth S. Carslaw
Atmos. Chem. Phys., 25, 291–325, https://doi.org/10.5194/acp-25-291-2025, https://doi.org/10.5194/acp-25-291-2025, 2025
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Aerosol particles that help form ice in clouds vary in number and type around the world and with time. However, in many weather and climate models cloud ice is not linked to aerosols that are known to nucleate ice. Here we report the first steps towards representing ice-nucleating particles within the UK Earth System Model. We conclude that in addition to ice nucleation by sea spray and mineral components of soil dust, we also need to represent ice nucleation by the organic components of soils.
Ryan Schmedding and Andreas Zuend
Atmos. Chem. Phys., 25, 327–346, https://doi.org/10.5194/acp-25-327-2025, https://doi.org/10.5194/acp-25-327-2025, 2025
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Four different approaches for computing the interfacial tension between liquid phases in aerosol particles were tested for particles with diameters from 10 nm to more than 5 μm. Antonov's rule led to the strongest reductions in the onset relative humidity of liquid–liquid phase separation and reproduced measured interfacial tensions for highly immiscible systems. A modified form of the Butler equation was able to best reproduce measured interfacial tensions in more miscible systems.
Masaru Yoshioka, Daniel P. Grosvenor, Ben B. B. Booth, Colin P. Morice, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 13681–13692, https://doi.org/10.5194/acp-24-13681-2024, https://doi.org/10.5194/acp-24-13681-2024, 2024
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A 2020 regulation has reduced sulfur emissions from shipping by about 80 %, leading to a decrease in atmospheric aerosols that have a cooling effect primarily by affecting cloud properties and amounts. Our climate model simulations predict a global temperature increase of 0.04 K over the next 3 decades as a result, which could contribute to surpassing the Paris Agreement's 1.5 °C target. Reduced aerosols may have also contributed to the recent temperature spikes.
Alcide Zhao, Laura J. Wilcox, and Claire L. Ryder
Atmos. Chem. Phys., 24, 13385–13402, https://doi.org/10.5194/acp-24-13385-2024, https://doi.org/10.5194/acp-24-13385-2024, 2024
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Climate models include desert dust aerosols, which cause atmospheric heating and can change circulation patterns. We assess the effect of dust on the Indian and east Asian summer monsoons through multi-model experiments isolating the effect of dust in current climate models for the first time. Dust atmospheric heating results in a southward shift of western Pacific equatorial rainfall and an enhanced Indian summer monsoon. This shows the importance of accurate dust representation in models.
Ragnhild Bieltvedt Skeie, Rachael Byrom, Øivind Hodnebrog, Caroline Jouan, and Gunnar Myhre
Atmos. Chem. Phys., 24, 13361–13370, https://doi.org/10.5194/acp-24-13361-2024, https://doi.org/10.5194/acp-24-13361-2024, 2024
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In 2020, new regulations by the International Maritime Organization regarding sulfur emissions came into force, reducing emissions of SO2 from the shipping sector by approximately 80 %. In this study, we use multiple models to calculate how much the Earth energy balance changed due to the emission reduction or the so-called effective radiative forcing. The calculated effective radiative forcing is weak, comparable to the effect of the increase in CO2 over the last 2 to 3 years.
Ge Yu, Yueya Wang, Zhe Wang, and Xiaoming Shi
EGUsphere, https://doi.org/10.5194/egusphere-2024-3581, https://doi.org/10.5194/egusphere-2024-3581, 2024
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Studying the cloud-forming capacity of aerosols is crucial in climate research. The PartMC model can provide detailed particle information and help these studies. This model is integrated with the ideal meteorological Cloud Model 1 (CM1) to simulate the aerosols at cloud-forming locations. Significant changes are revealed in the hygroscopicity distribution of aerosols within ascending air parcels. Additionally, different ascent times also affect aerosol aging processes.
Mingxu Liu, Hitoshi Matsui, Douglas S. Hamilton, Sagar D. Rathod, Kara D. Lamb, and Natalie M. Mahowald
Atmos. Chem. Phys., 24, 13115–13127, https://doi.org/10.5194/acp-24-13115-2024, https://doi.org/10.5194/acp-24-13115-2024, 2024
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Atmospheric aerosol deposition provides bioavailable iron to promote marine primary production, yet the estimates of its fluxes remain highly uncertain. This study, by performing global aerosol simulations, demonstrates that iron-containing particle size upon emission is a critical factor in regulating soluble iron input to open oceans. Further observational constraints on this are needed to reduce modeling uncertainties.
Jingmin Li, Mattia Righi, Johannes Hendricks, Christof G. Beer, Ulrike Burkhardt, and Anja Schmidt
Atmos. Chem. Phys., 24, 12727–12747, https://doi.org/10.5194/acp-24-12727-2024, https://doi.org/10.5194/acp-24-12727-2024, 2024
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Aiming to understand underlying patterns and trends in aerosols, we characterize the spatial patterns and long-term evolution of lower tropospheric aerosols by clustering multiple aerosol properties from preindustrial times to the year 2050 under three Shared
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Socioeconomic Pathway scenarios. The results provide a clear and condensed picture of the spatial extent and distribution of aerosols for different time periods and emission scenarios.
Bishuo He and Chunsheng Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-3441, https://doi.org/10.5194/egusphere-2024-3441, 2024
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Factor-uncertainty analysis helps us understand their impacts on complex systems. Traditional methods have many limitations. This study introduces a new method to measure how each factor contributes to uncertainty. It gains insights into the role of each variable and works for all multi-factor systems. As an application, we analyzed how aerosols affect solar radiation and identified the key factors. These analyses can improve our understanding of the role of aerosols in climate change.
Yueming Cheng, Tie Dai, Junji Cao, Daisuke Goto, Jianbing Jin, Teruyuki Nakajima, and Guangyu Shi
Atmos. Chem. Phys., 24, 12643–12659, https://doi.org/10.5194/acp-24-12643-2024, https://doi.org/10.5194/acp-24-12643-2024, 2024
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In March 2021, east Asia experienced an outbreak of severe dust storms after an absence of 1.5 decades. Here, we innovatively used the time-lagged ground-based aerosol size information with the fixed-lag ensemble Kalman smoother to optimize dust emission and reproduce the dust storm. This work is valuable for not only the quantification of health damage, aviation risks, and profound impacts on the Earth's system but also revealing the climatic driving force and the process of desertification.
Marc Mallet, Aurore Voldoire, Fabien Solmon, Pierre Nabat, Thomas Drugé, and Romain Roehrig
Atmos. Chem. Phys., 24, 12509–12535, https://doi.org/10.5194/acp-24-12509-2024, https://doi.org/10.5194/acp-24-12509-2024, 2024
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This study investigates the interactions between smoke aerosols and climate in tropical Africa using a coupled ocean–atmosphere–aerosol climate model. The work shows that smoke plumes have a significant impact by increasing the low-cloud fraction, decreasing the ocean and continental surface temperature and reducing the precipitation of coastal western Africa. It also highlights the role of the ocean temperature response and its feedbacks for the September–November season.
Jia Liu, Cancan Zhu, Donghui Zhou, and Jinbao Han
Atmos. Chem. Phys., 24, 12341–12354, https://doi.org/10.5194/acp-24-12341-2024, https://doi.org/10.5194/acp-24-12341-2024, 2024
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The hydrophilic coatings of aged black carbon (BC) particles absorb moisture during the hygroscopic growth process, but it is difficult to characterize how much water is absorbed under different relative humidities (RHs). In this study, we propose a method to obtain the water content in the coatings based on the equivalent complex refractive index retrieved from optical properties. This method is verified from a theoretical perspective, and it performs well for thickly coated BC at high RHs.
Mizuo Kajino, Kentaro Ishijima, Joseph Ching, Kazuyo Yamaji, Rio Ishikawa, Tomoki Kajikawa, Tanbir Singh, Tomoki Nakayama, Yutaka Matsumi, Koyo Kojima, Prabir K. Patra, and Sachiko Hayashida
EGUsphere, https://doi.org/10.5194/egusphere-2024-1811, https://doi.org/10.5194/egusphere-2024-1811, 2024
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Air pollution in Delhi during post monsoon period is severe and association with intensive crop residue burning (CRB) over Punjab state has attracted attention. However, the relationship has been unclear as the CRB emissions conventionally derived from satellites were underestimated due to clouds and haze over the region. We evaluated the impact of CRB on PM2.5 as about 50 %, based on a combination of numerical modeling and high-density observation network using low-cost sensors we installed.
Zijun Li, Angela Buchholz, and Noora Hyttinen
Atmos. Chem. Phys., 24, 11717–11725, https://doi.org/10.5194/acp-24-11717-2024, https://doi.org/10.5194/acp-24-11717-2024, 2024
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Evaluating organosulfur (OS) hygroscopicity is important for assessing aerosol–cloud climate interactions in the post-fossil-fuel future, when SO2 emissions decrease and OS compounds become increasingly important. Here a state-of-the-art quantum-chemistry-based method was used to predict the hygroscopic growth factors (HGFs) of a group of atmospherically relevant OS compounds and their mixtures with (NH4)2SO4. A good agreement was observed between their model-estimated and experimental HGFs.
Jamie R. Banks, Bernd Heinold, and Kerstin Schepanski
Atmos. Chem. Phys., 24, 11451–11475, https://doi.org/10.5194/acp-24-11451-2024, https://doi.org/10.5194/acp-24-11451-2024, 2024
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The Aralkum is a new desert in Central Asia formed by the desiccation of the Aral Sea. This has created a source of atmospheric dust, with implications for the balance of solar and thermal radiation. Simulating these effects using a dust transport model, we find that Aralkum dust adds radiative cooling effects to the surface and atmosphere on average but also adds heating events. Increases in surface pressure due to Aralkum dust strengthen the Siberian High and weaken the summer Asian heat low.
Xinyue Shao, Minghuai Wang, Xinyi Dong, Yaman Liu, Wenxiang Shen, Stephen R. Arnold, Leighton A. Regayre, Meinrat O. Andreae, Mira L. Pöhlker, Duseong S. Jo, Man Yue, and Ken S. Carslaw
Atmos. Chem. Phys., 24, 11365–11389, https://doi.org/10.5194/acp-24-11365-2024, https://doi.org/10.5194/acp-24-11365-2024, 2024
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Highly oxygenated organic molecules (HOMs) play an important role in atmospheric new particle formation (NPF). By semi-explicitly coupling the chemical mechanism of HOMs and a comprehensive nucleation scheme in a global climate model, the updated model shows better agreement with measurements of nucleation rate, growth rate, and NPF event frequency. Our results reveal that HOM-driven NPF leads to a considerable increase in particle and cloud condensation nuclei burden globally.
Anderson Da Silva, Louis Marelle, Jean-Christophe Raut, Yvette Gramlich, Karolina Siegel, Sophie L. Haslett, Claudia Mohr, and Jennie L. Thomas
EGUsphere, https://doi.org/10.5194/egusphere-2024-2839, https://doi.org/10.5194/egusphere-2024-2839, 2024
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Particles sources in polar climates are unclear, affecting climate representation in models. This study introduces an evaluated method for tracking particles with backtrajectory modeling. Tests on simulated particles allowed to show that traditional detection methods often misidentify sources. An improved method that accurately traces origins of aerosol particles in the Arctic is presented. The study recommends using this enhanced method for better source identification of atmospheric species.
Falei Xu, Shuang Wang, Yan Li, and Juan Feng
Atmos. Chem. Phys., 24, 10689–10705, https://doi.org/10.5194/acp-24-10689-2024, https://doi.org/10.5194/acp-24-10689-2024, 2024
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This study examines how the winter North Atlantic Oscillation (NAO) and El Niño–Southern Oscillation (ENSO) affect dust activities in North China during the following spring. The results show that the NAO and ENSO, particularly in their negative phases, greatly influence dust activities. When both are negative, their combined effect on dust activities is even greater. This research highlights the importance of these climate patterns in predicting spring dust activities in North China.
Hengheng Zhang, Wei Huang, Xiaoli Shen, Ramakrishna Ramisetty, Junwei Song, Olga Kiseleva, Christopher Claus Holst, Basit Khan, Thomas Leisner, and Harald Saathoff
Atmos. Chem. Phys., 24, 10617–10637, https://doi.org/10.5194/acp-24-10617-2024, https://doi.org/10.5194/acp-24-10617-2024, 2024
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Our study unravels how stagnant winter conditions elevate aerosol levels in Stuttgart. Cloud cover at night plays a pivotal role, impacting morning air quality. Validating a key model, our findings aid accurate air quality predictions, crucial for effective pollution mitigation in urban areas.
Zixuan Jia, Massimo A. Bollasina, Wenjun Zhang, and Ying Xiang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2770, https://doi.org/10.5194/egusphere-2024-2770, 2024
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Using multi-model mean data from regional aerosol perturbation experiments, we find that increased Asian sulfate aerosols strengthen the link between ENSO and the East Asian winter monsoon. In coupled simulations, aerosol-induced broad cooling increases ENSO amplitude by affecting the tropical Pacific mean state, contributing to increase monsoon interannual variability. These results provide important implications to reduce uncertainties in future projections of regional extreme variability.
Giorgio Veratti, Alessandro Bigi, Michele Stortini, Sergio Teggi, and Grazia Ghermandi
Atmos. Chem. Phys., 24, 10475–10512, https://doi.org/10.5194/acp-24-10475-2024, https://doi.org/10.5194/acp-24-10475-2024, 2024
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In a study of two consecutive winter seasons, we used measurements and modelling tools to identify the levels and sources of black carbon pollution in a medium-sized urban area of the Po Valley, Italy. Our findings show that biomass burning and traffic-related emissions (especially from Euro 4 diesel cars) significantly contribute to BC concentrations. This research offers crucial insights for policymakers and urban planners aiming to improve air quality in cities.
Steven Soon-Kai Kong, Joshua S. Fu, Neng-Huei Lin, Guey-Rong Sheu, and Wei-Syun Huang
EGUsphere, https://doi.org/10.5194/egusphere-2024-2549, https://doi.org/10.5194/egusphere-2024-2549, 2024
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The accuracy of the chemical transport model, a key focus of our research, is strongly dependent on the dry deposition parameterization. Our finding shows that the refined CMAQ dust model correlated well with the ground and high altitude in-situ measurements by implementing the suggested dry deposition schemes. Furthermore, we reveal the mixing state of two types of aerosols at the upper level, a finding supported by both the optimized model and measurement.
Pascal Lemaitre, Arnaud Quérel, Alexis Dépée, Alice Guerra Devigne, Marie Monier, Thibault Hiron, Chloé Soto Minguez, Daniel Hardy, and Andrea Flossmann
Atmos. Chem. Phys., 24, 9713–9732, https://doi.org/10.5194/acp-24-9713-2024, https://doi.org/10.5194/acp-24-9713-2024, 2024
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A new in-cloud scavenging scheme is proposed. It is based on a microphysical model of cloud formation and may be applied to long-distance atmospheric transport models (> 100 km) and climatic models. This model is applied to the two most extreme precipitating cloud types in terms of both relative humidity and vertical extension: cumulonimbus and stratus.
Alex Rowell, James Brean, David C. S. Beddows, Tuukka Petäjä, Máté Vörösmarty, Imre Salma, Jarkko V. Niemi, Hanna E. Manninen, Dominik van Pinxteren, Thomas Tuch, Kay Weinhold, Zongbo Shi, and Roy M. Harrison
Atmos. Chem. Phys., 24, 9515–9531, https://doi.org/10.5194/acp-24-9515-2024, https://doi.org/10.5194/acp-24-9515-2024, 2024
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Different sources of airborne particles in the atmospheres of four European cities were distinguished by recognising their particle size distributions using a statistical procedure, positive matrix factorisation. The various sources responded differently to the changes in emissions associated with COVID-19 lockdowns, and the reasons are investigated. While traffic emissions generally decreased, particles formed from reactions of atmospheric gases decreased in some cities but increased in others.
Amy H. Peace, Ying Chen, George Jordan, Daniel G. Partridge, Florent Malavelle, Eliza Duncan, and Jim M. Haywood
Atmos. Chem. Phys., 24, 9533–9553, https://doi.org/10.5194/acp-24-9533-2024, https://doi.org/10.5194/acp-24-9533-2024, 2024
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Natural aerosols from volcanic eruptions can help us understand how anthropogenic aerosols modify climate. We use observations and model simulations of the 2014–2015 Holuhraun eruption plume to examine aerosol–cloud interactions in September 2014. We find a shift to clouds with smaller, more numerous cloud droplets in the first 2 weeks of the eruption. In the third week, the background meteorology and previous conditions experienced by air masses modulate the aerosol perturbation to clouds.
Hua Lu, Min Xie, Bingliang Zhuang, Danyang Ma, Bojun Liu, Yangzhihao Zhan, Tijian Wang, Shu Li, Mengmeng Li, and Kuanguang Zhu
Atmos. Chem. Phys., 24, 8963–8982, https://doi.org/10.5194/acp-24-8963-2024, https://doi.org/10.5194/acp-24-8963-2024, 2024
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To identify cloud, aerosol, and planetary boundary layer (PBL) interactions from an air quality perspective, we summarized two pollution patterns characterized by denser liquid cloud and by obvious cloud radiation interaction (CRI). Numerical simulation experiments showed CRI could cause a 50 % reduction in aerosol radiation interaction (ARI) under a low-trough system. The results emphasized the nonnegligible role of CRI and its inhibition of ARI under wet and cloudy pollution synoptic patterns.
Huiyun Du, Jie Li, Xueshun Chen, Gabriele Curci, Fangqun Yu, Yele Sun, Xu Dao, Song Guo, Zhe Wang, Wenyi Yang, Lianfang Wei, and Zifa Wang
EGUsphere, https://doi.org/10.5194/egusphere-2024-1432, https://doi.org/10.5194/egusphere-2024-1432, 2024
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Inadequate consideration of mixing state and coatings on BC hinders aerosol radiation forcing quantification. While core-shell mixing results match observations closely, partial internal mixing and coating are more realistic. The fraction of embedded BC and coating aerosols resolved by a microphysics module were used to constrain the mixing state. This led to a 30~43 % absorption enhancement decrease over Northern China, offering valuable insights for the assessment of BC's radiative effects.
Emilie Fons, Ann Kristin Naumann, David Neubauer, Theresa Lang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 8653–8675, https://doi.org/10.5194/acp-24-8653-2024, https://doi.org/10.5194/acp-24-8653-2024, 2024
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Aerosols can modify the liquid water path (LWP) of stratocumulus and, thus, their radiative effect. We compare storm-resolving model and satellite data that disagree on the sign of LWP adjustments and diagnose this discrepancy with causal inference. We find that strong precipitation, the absence of wet scavenging, and cloud deepening under a weak inversion contribute to positive LWP adjustments to aerosols in the model, despite weak negative effects from cloud-top entrainment enhancement.
Muhammed Irfan, Thomas Kühn, Taina Yli-Juuti, Anton Laakso, Eemeli Holopainen, Douglas R. Worsnop, Annele Virtanen, and Harri Kokkola
Atmos. Chem. Phys., 24, 8489–8506, https://doi.org/10.5194/acp-24-8489-2024, https://doi.org/10.5194/acp-24-8489-2024, 2024
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The study examines how the volatility of semi-volatile organic compounds affects secondary organic aerosol (SOA) formation and climate. Our simulations show that uncertainties in these volatilities influence aerosol mass and climate impacts. Accurate representation of these compounds in climate models is crucial for predicting global climate patterns.
Zhixin Xue, Nair Udaysankar, and Sundar Christopher
EGUsphere, https://doi.org/10.5194/egusphere-2024-1781, https://doi.org/10.5194/egusphere-2024-1781, 2024
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Canadian wildfires degrade US air quality through long-range smoke transport. This study uses surface, satellite, and numerical models to assess the PM2.5 increase due to Canadian fires during 2018 fire season. Satellite data, often limited by cloud cover, was supplemented with high-resolution simulated data to fill gaps. Weather systems significantly influenced smoke movement. Canadian fires led to a notable rise in PM2.5 levels across various US regions during the 2018 summer wildfire events.
Alkiviadis Kalisoras, Aristeidis K. Georgoulias, Dimitris Akritidis, Robert J. Allen, Vaishali Naik, Chaincy Kuo, Sophie Szopa, Pierre Nabat, Dirk Olivié, Twan van Noije, Philippe Le Sager, David Neubauer, Naga Oshima, Jane Mulcahy, Larry W. Horowitz, and Prodromos Zanis
Atmos. Chem. Phys., 24, 7837–7872, https://doi.org/10.5194/acp-24-7837-2024, https://doi.org/10.5194/acp-24-7837-2024, 2024
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Effective radiative forcing (ERF) is a metric for estimating how human activities and natural agents change the energy flow into and out of the Earth’s climate system. We investigate the anthropogenic aerosol ERF, and we estimate the contribution of individual processes to the total ERF using simulations from Earth system models within the Coupled Model Intercomparison Project Phase 6 (CMIP6). Our findings highlight that aerosol–cloud interactions drive ERF variability during the last 150 years.
Qianqian Song, Paul Ginoux, María Gonçalves Ageitos, Ron L. Miller, Vincenzo Obiso, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 7421–7446, https://doi.org/10.5194/acp-24-7421-2024, https://doi.org/10.5194/acp-24-7421-2024, 2024
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We implement and simulate the distribution of eight dust minerals in the GFDL AM4.0 model. We found that resolving the eight minerals reduces dust absorption compared to the homogeneous dust used in the standard GFDL AM4.0 model that assumes a globally uniform hematite content of 2.7 % by volume. Resolving dust mineralogy results in significant impacts on radiation, land surface temperature, surface winds, and precipitation over North Africa in summer.
Senyi Kong, Zheng Wang, and Lei Bi
Atmos. Chem. Phys., 24, 6911–6935, https://doi.org/10.5194/acp-24-6911-2024, https://doi.org/10.5194/acp-24-6911-2024, 2024
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The retrieval of refractive indices of dust aerosols from laboratory optical measurements is commonly done assuming spherical particles. This paper aims to investigate the uncertainties in the shortwave refractive indices and corresponding optical properties by considering non-spherical and inhomogeneous models for dust samples. The study emphasizes the significance of using non-spherical models for simulating dust aerosols.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
Atmos. Chem. Phys., 24, 6787–6807, https://doi.org/10.5194/acp-24-6787-2024, https://doi.org/10.5194/acp-24-6787-2024, 2024
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In this study, we diagnose uncertainties in carbon monoxide and organic carbon emissions from four inventories for seven major wildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Cited articles
Acharya, P., Barik, G., Gayen, B. K., Bar, S., Maiti, A., Sarkar, A., Ghosh, S., De, S. K., and Sreekesh, S.: Revisiting the Levels of Aerosol Optical Depth in South-Southeast Asia, Europe and USA amid the COVID-19 Pandemic Using Satellite Observations, Environ. Res., 193, 110514, https://doi.org/10.1016/j.envres.2020.110514, 2021. a, b
Acosta Navarro, J. C., Ekman, A. M. L., Pausata, F. S. R., Lewinschal, A., Varma, V., Seland, Ø., Gauss, M., Iversen, T., Kirkevåg, A., Riipinen, I., and Hansson, H. C.: Future Response of Temperature and Precipitation to Reduced Aerosol Emissions as Compared with Increased Greenhouse Gas Concentrations, J. Climate, 30, 939–954, https://doi.org/10.1175/JCLI-D-16-0466.1, 2017. a
Al-Abadleh, H. A., Lysy, M., Neil, L., Patel, P., Mohammed, W., and Khalaf, Y.: Rigorous Quantification of Statistical Significance of the COVID-19 Lockdown Effect on Air Quality: The Case from Ground-Based Measurements in Ontario, Canada, J. Hazard. Mat., 413, 125445, https://doi.org/10.1016/j.jhazmat.2021.125445, 2021. a
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Chang, Y., Huang, R.-J., Ge, X., Huang, X., Hu, J., Duan, Y., Zou, Z., Liu, X., and Lehmann, M. F.: Puzzling Haze Events in China During the Coronavirus (COVID-19) Shutdown, Geophys. Res. Lett., 47, e2020GL088533, https://doi.org/10.1029/2020GL088533, 2020. a, b
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Deroubaix, A., Brasseur, G., Gaubert, B., Labuhn, I., Menut, L., Siour, G., and Tuccella, P.: Response of surface ozone concentration to emission reduction and meteorology during the COVID-19 lockdown in Europe, Meteorol. Appl., 28, e1990, https://doi.org/10.1002/met.1990, 2021. a
Diamond, M. S. and Wood, R.: Limited Regional Aerosol and Cloud Microphysical Changes Despite Unprecedented Decline in Nitrogen Oxide Pollution During the February 2020 COVID-19 Shutdown in China, Geophys. Res. Lett., 47, e2020GL088913, https://doi.org/10.1029/2020GL088913, 2020. a, b, c
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Eyring, V., Bony, S., Meehl, G. A., Senior, C. A., Stevens, B., Stouffer, R. J., and Taylor, K. E.: Overview of the Coupled Model Intercomparison Project Phase 6 (CMIP6) experimental design and organization, Geosci. Model Dev., 9, 1937–1958, https://doi.org/10.5194/gmd-9-1937-2016, 2016. a
Eyring, V., Gillett, N., Achuta Rao, K., Barimalala, R., Barreiro Parrillo, M., Bellouin, N., Cassou, C., Durack, P., Kosaka, Y., McGregor, S., Min, S., Morgenstern, O., and Sun, Y.: Human Influence on the Climate System, p. 423–552, Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, https://doi.org/10.1017/9781009157896.005, 2021. a
Fasullo, J. T., Rosenbloom, N., Buchholz, R. R., Danabasoglu, G., Lawrence, D. M., and Lamarque, J.-F.: Coupled Climate Responses to Recent Australian Wildfire and COVID-19 Emissions Anomalies Estimated in CESM2, Geophys. Res. Lett., 48, e2021GL097420, https://doi.org/10.1029/2021GL093841, 2021. a, b
Fiedler, S., Wyser, K., Rogelj, J., and van Noije, T.: Radiative Effects of Reduced Aerosol Emissions during the COVID-19 Pandemic and the Future Recovery, Atmos. Res., 264, 105866, https://doi.org/10.1016/j.atmosres.2021.105866, 2021. a, b
Field, R. D., Hickman, J. E., Geogdzhayev, I. V., Tsigaridis, K., and Bauer, S. E.: Changes in satellite retrievals of atmospheric composition over eastern China during the 2020 COVID-19 lockdowns, Atmos. Chem. Phys., 21, 18333–18350, https://doi.org/10.5194/acp-21-18333-2021, 2021. a, b, c, d
Forster, P. M., Forster, H. I., Evans, M. J., Gidden, M. J., Jones, C. D., Keller, C. A., Lamboll, R. D., Quéré, C. L., Rogelj, J., Rosen, D., Schleussner, C.-F., Richardson, T. B., Smith, C. J., and Turnock, S. T.: Current and Future Global Climate Impacts Resulting from COVID-19, Nat. Clim. Chang., 10, 913–919, https://doi.org/10.1038/s41558-020-0883-0, 2020. a, b, c, d, e
Fyfe, J. C., Kharin, V. V., Swart, N., Flato, G. M., Sigmond, M., and Gillett, N. P.: Quantifying the Influence of Short-Term Emission Reductions on Climate, Sci. Adv., 7, eabf7133, https://doi.org/10.1126/sciadv.abf7133, 2021. a, b
Gao, J., Yang, Y., Wang, H., Wang, P., Li, H., Li, M., Ren, L., Yue, X., and Liao, H.: Fast climate responses to emission reductions in aerosol and ozone precursors in China during 2013–2017, Atmos. Chem. Phys., 22, 7131–7142, https://doi.org/10.5194/acp-22-7131-2022, 2022. a
Gaubert, B., Bouarar, I., Doumbia, T., Liu, Y., Stavrakou, T., Deroubaix, A., Darras, S., Elguindi, N., Granier, C., Lacey, F., Müller, J.-F., Shi, X., Tilmes, S., Wang, T., and Brasseur, G. P.: Global Changes in Secondary Atmospheric Pollutants During the 2020 COVID-19 Pandemic, J. Geophys. Res.-Atmos., 126, e2020JD034213, https://doi.org/10.1029/2020JD034213, 2021. a
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Gettelman, A., Chen, C.-C., and Bardeen, C. G.: The climate impact of COVID-19-induced contrail changes, Atmos. Chem. Phys., 21, 9405–9416, https://doi.org/10.5194/acp-21-9405-2021, 2021. a, b
Gkatzelis, G. I., Gilman, J. B., Brown, S. S., Eskes, H., Gomes, A. R., Lange, A. C., McDonald, B. C., Peischl, J., Petzold, A., Thompson, C. R., and Kiendler-Scharr, A.: The Global Impacts of COVID-19 Lockdowns on Urban Air Pollution, Elem. Sci. Anthr., 9, 00176, https://doi.org/10.1525/elementa.2021.00176, 2021. a, b
Gkikas, A., Proestakis, E., Amiridis, V., Kazadzis, S., Di Tomaso, E., Tsekeri, A., Marinou, E., Hatzianastassiou, N., and Pérez García-Pando, C.: ModIs Dust AeroSol (MIDAS): a global fine-resolution dust optical depth data set, Atmos. Meas. Tech., 14, 309–334, https://doi.org/10.5194/amt-14-309-2021, 2021. a, b, c, d
Goldberg, D. L., Anenberg, S. C., Griffin, D., McLinden, C. A., Lu, Z., and Streets, D. G.: Disentangling the Impact of the COVID-19 Lockdowns on Urban NO2 From Natural Variability, Geophys. Res. Lett., 47, e2020GL089269, https://doi.org/10.1029/2020GL089269, 2020. a, b
Gouda, K., Gogeri, I., and ThippaReddy, A.: Assessment of Aerosol Optical Depth over Indian Subcontinent during COVID-19 lockdown (March–May 2020), Environ. Monit. Assess., 194, 1573–2959, https://doi.org/10.1007/s10661-022-09855-3, 2022. a
Griffin, D., McLinden, C. A., Racine, J., Moran, M. D., Fioletov, V., Pavlovic, R., Mashayekhi, R., Zhao, X., and Eskes, H.: Assessing the Impact of Corona-Virus-19 on Nitrogen Dioxide Levels over Southern Ontario, Canada, Remote Sens., 12, 4112, https://doi.org/10.3390/rs12244112, 2020. a
Hajima, T., Watanabe, M., Yamamoto, A., Tatebe, H., Noguchi, M. A., Abe, M., Ohgaito, R., Ito, A., Yamazaki, D., Okajima, H., Ito, A., Takata, K., Ogochi, K., Watanabe, S., and Kawamiya, M.: Development of the MIROC-ES2L Earth system model and the evaluation of biogeochemical processes and feedbacks, Geosci. Model Dev., 13, 2197–2244, https://doi.org/10.5194/gmd-13-2197-2020, 2020. a
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Short summary
The COVID-19 lockdowns reduced aerosol emissions. We ask whether these reductions affected regional aerosol optical depth (AOD) and compare the observed changes to predictions from Earth system models. Only India has an observed AOD reduction outside of typical variability. Models overestimate the response in some regions, but when key biases have been addressed, the agreement is improved. Our results suggest that current models can realistically predict the effects of future emission changes.
The COVID-19 lockdowns reduced aerosol emissions. We ask whether these reductions affected...
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