Articles | Volume 23, issue 21
https://doi.org/10.5194/acp-23-13555-2023
https://doi.org/10.5194/acp-23-13555-2023
Research article
 | 
30 Oct 2023
Research article |  | 30 Oct 2023

Effects of simulated secondary organic aerosol water on PM1 levels and composition over the US

Stylianos Kakavas, Spyros N. Pandis, and Athanasios Nenes

Related authors

Formation and chemical evolution of secondary organic aerosol in two different environments: a dual-chamber study
Andreas Aktypis, Dontavious J. Sippial, Christina N. Vasilakopoulou, Angeliki Matrali, Christos Kaltsonoudis, Andrea Simonati, Marco Paglione, Matteo Rinaldi, Stefano Decesari, and Spyros N. Pandis
Atmos. Chem. Phys., 24, 13769–13791, https://doi.org/10.5194/acp-24-13769-2024,https://doi.org/10.5194/acp-24-13769-2024, 2024
Short summary
Significant spatial and temporal variation of the concentrations and chemical composition of ultrafine particulate matter over Europe
Konstantinos Mataras, Evangelia Siouti, David Patoulias, and Spyros Pandis
EGUsphere, https://doi.org/10.5194/egusphere-2024-3357,https://doi.org/10.5194/egusphere-2024-3357, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Impact of meteorology and aerosol sources on PM2.5 and oxidative potential variability and levels in China
Jiemei Liu, Jesper H. Christensen, Zhuyun Ye, Shikui Dong, Camilla Geels, Jørgen Brandt, Athanasios Nenes, Yuan Yuan, and Ulas Im
Atmos. Chem. Phys., 24, 10849–10867, https://doi.org/10.5194/acp-24-10849-2024,https://doi.org/10.5194/acp-24-10849-2024, 2024
Short summary
Sensitivity of predicted ultrafine particle size distributions in Europe to different nucleation rate parameterizations using PMCAMx-UF v2.2
David Patoulias, Kalliopi Florou, and Spyros N. Pandis
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-145,https://doi.org/10.5194/gmd-2024-145, 2024
Revised manuscript under review for GMD
Short summary
Recent improvements and maximum covariance analysis of aerosol and cloud properties in the EC-Earth3-AerChem model
Manu Anna Thomas, Klaus Wyser, Shiyu Wang, Marios Chatziparaschos, Paraskevi Georgakaki, Montserrat Costa-Surós, Maria Gonçalves Ageitos, Maria Kanakidou, Carlos Pérez García-Pando, Athanasios Nenes, Twan van Noije, Philippe Le Sager, and Abhay Devasthale
Geosci. Model Dev., 17, 6903–6927, https://doi.org/10.5194/gmd-17-6903-2024,https://doi.org/10.5194/gmd-17-6903-2024, 2024
Short summary

Related subject area

Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Rapid oxidation of phenolic compounds by O3 and HO: effects of the air–water interface and mineral dust in tropospheric chemical processes
Yanru Huo, Mingxue Li, Xueyu Wang, Jianfei Sun, Yuxin Zhou, Yuhui Ma, and Maoxia He
Atmos. Chem. Phys., 24, 12409–12423, https://doi.org/10.5194/acp-24-12409-2024,https://doi.org/10.5194/acp-24-12409-2024, 2024
Short summary
Modeling the contribution of leads to sea spray aerosol in the high Arctic
Rémy Lapere, Louis Marelle, Pierre Rampal, Laurent Brodeau, Christian Melsheimer, Gunnar Spreen, and Jennie L. Thomas
Atmos. Chem. Phys., 24, 12107–12132, https://doi.org/10.5194/acp-24-12107-2024,https://doi.org/10.5194/acp-24-12107-2024, 2024
Short summary
Importance of aerosol composition and aerosol vertical profiles in global spatial variation in the relationship between PM2.5 and aerosol optical depth
Haihui Zhu, Randall V. Martin, Aaron van Donkelaar, Melanie S. Hammer, Chi Li, Jun Meng, Christopher R. Oxford, Xuan Liu, Yanshun Li, Dandan Zhang, Inderjeet Singh, and Alexei Lyapustin
Atmos. Chem. Phys., 24, 11565–11584, https://doi.org/10.5194/acp-24-11565-2024,https://doi.org/10.5194/acp-24-11565-2024, 2024
Short summary
The co-benefits of a low-carbon future for PM2.5 and O3 air pollution in Europe
Connor J. Clayton, Daniel R. Marsh, Steven T. Turnock, Ailish M. Graham, Kirsty J. Pringle, Carly L. Reddington, Rajesh Kumar, and James B. McQuaid
Atmos. Chem. Phys., 24, 10717–10740, https://doi.org/10.5194/acp-24-10717-2024,https://doi.org/10.5194/acp-24-10717-2024, 2024
Short summary
Assessing the effectiveness of SO2, NOx, and NH3 emission reductions in mitigating winter PM2.5 in Taiwan using CMAQ
Ping-Chieh Huang, Hui-Ming Hung, Hsin-Chih Lai, and Charles C.-K. Chou
Atmos. Chem. Phys., 24, 10759–10772, https://doi.org/10.5194/acp-24-10759-2024,https://doi.org/10.5194/acp-24-10759-2024, 2024
Short summary

Cited articles

Baker, A., Kanakidou, M., Nenes, A., Myriokefalitakis, S., Croot, P.L., Duce, A. D., Gao, Y., Guieu, C., Ito, A., Jickells, T. D., Mahowald, N. M., Middag, R., Perron, M. M. G., Sarin, M. M., Shelley, R., and Turner, D. R.: Changing atmospheric acidity as a modulator of nutrient deposition and ocean biogeochemistry, Sci. Adv., 7, 1–9, https://doi.org/10.1126/sciadv.abd8800, 2021. 
Bian, Y. X., Zhao, C. S., Ma, N., Chen, J., and Xu, W. Y.: A study of aerosol liquid water content based on hygroscopicity measurements at high relative humidity in the North China Plain, Atmos. Chem. Phys., 14, 6417–6426, https://doi.org/10.5194/acp-14-6417-2014, 2014. 
Bougiatioti, A., Nikolaou, P., Stavroulas, I., Kouvarakis, G., Weber, R., Nenes, A., Kanakidou, M., and Mihalopoulos, N.: Particle water and pH in the eastern Mediterranean: source variability and implications for nutrient availability, Atmos. Chem. Phys., 16, 4579–4591, https://doi.org/10.5194/acp-16-4579-2016, 2016. 
Carlton, A. G. and Turpin, B. J.: Particle partitioning potential of organic compounds is highest in the Eastern US and driven by anthropogenic water, Atmos. Chem. Phys., 13, 10203–10214, https://doi.org/10.5194/acp-13-10203-2013, 2013. 
Chang, R. Y.-W., Slowik, J. G., Shantz, N. C., Vlasenko, A., Liggio, J., Sjostedt, S. J., Leaitch, W. R., and Abbatt, J. P. D.: The hygroscopicity parameter (κ) of ambient organic aerosol at a field site subject to biogenic and anthropogenic influences: relationship to degree of aerosol oxidation, Atmos. Chem. Phys., 10, 5047–5064, https://doi.org/10.5194/acp-10-5047-2010, 2010. 
Download
Short summary
Water uptake from organic species in aerosol can affect the partitioning of semi-volatile inorganic compounds but are not considered in global and chemical transport models. We address this with a version of the PM-CAMx model that considers such organic water effects and use it to carry out 1-year aerosol simulations over the continental US. We show that such organic water impacts can increase dry PM1 levels by up to 2 μg m-3 when RH levels and PM1 concentrations are high.
Altmetrics
Final-revised paper
Preprint