Articles | Volume 20, issue 11
https://doi.org/10.5194/acp-20-7035-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-7035-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
15 Jun 2020
Research article |
| 15 Jun 2020
| 15 Jun 2020
Seasonal stratospheric ozone trends over 2000–2018 derived from several merged data sets
Space and Earth Observation Centre, Finnish Meteorological Institute, Helsinki, Finland
Viktoria F. Sofieva
Space and Earth Observation Centre, Finnish Meteorological Institute, Helsinki, Finland
Doug Degenstein
Institute of Space and Atmospheric Studies, University of Saskatchewan, Saskatoon, Saskatchewan, Canada
Chris Roth
Institute of Space and Atmospheric Studies, University of Saskatchewan, Saskatoon, Saskatchewan, Canada
Sean Davis
NOAA Earth System Research Laboratory Chemical Sciences Division,
Boulder, CO, USA
Lucien Froidevaux
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA, USA
Related authors
Viktoria F. Sofieva, Alexei Rozanov, Monika Szelag, John P. Burrows, Christian Retscher, Robert Damadeo, Doug Degenstein, Landon A. Rieger, and Adam Bourassa
Earth Syst. Sci. Data, 16, 5227–5241, https://doi.org/10.5194/essd-16-5227-2024, https://doi.org/10.5194/essd-16-5227-2024, 2024
Short summary
Short summary
Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived from data of six limb and occultation satellite instruments. The created aerosol climate record covers the period from October 1984 to December 2023. It can be used in various climate-related studies.
Miriam Sinnhuber, Christina Arras, Stefan Bender, Bernd Funke, Hanli Liu, Daniel R. Marsh, Thomas Reddmann, Eugene Rozanov, Timofei Sukhodolov, Monika E. Szelag, and Jan Maik Wissing
EGUsphere, https://doi.org/10.5194/egusphere-2024-2256, https://doi.org/10.5194/egusphere-2024-2256, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Formation of nitric oxide NO in the upper atmosphere varies with solar activity. Observations show that it starts a chain of processes in the entire atmosphere affecting the ozone layer and climate system. This is often underestimated in models. We compare five models which show large differences in simulated NO. Analysis of results point out problems related to the oxygen balance, and to the impact of atmospheric waves on dynamics. Both must be modeled well to reproduce the downward coupling.
Tuomas Häkkilä, Maxime Grandin, Markus Battarbee, Monika E. Szeląg, Markku Alho, Leo Kotipalo, Niilo Kalakoski, Pekka T. Verronen, and Minna Palmroth
Ann. Geophys. Discuss., https://doi.org/10.5194/angeo-2024-7, https://doi.org/10.5194/angeo-2024-7, 2024
Revised manuscript under review for ANGEO
Short summary
Short summary
We study the atmospheric impact of auroral electron precipitation, by the novel combination of both magnetospheric and atmospheric modelling. We first simulate fluxes of auroral electrons, and then use these fluxes to model their atmospheric impact. We find an increase of up to 200 % in thermospheric odd nitrogen, and a corresponding decrease in stratospheric ozone of around 0.7 %. The produced auroral electron precipitation is realistic, and shows the potential for future studies.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Didier Fussen, Christine Bingen, Filip Vanhellemont, Nina Mateshvili, Alexei Rozanov, and Christine Pohl
Atmos. Meas. Tech., 17, 3085–3101, https://doi.org/10.5194/amt-17-3085-2024, https://doi.org/10.5194/amt-17-3085-2024, 2024
Short summary
Short summary
We have developed the new multi-wavelength dataset of aerosol extinction profiles, which are retrieved from the averaged transmittance spectra by the Global Ozone Monitoring by Occultation of Stars instrument aboard Envisat. The retrieved aerosol extinction profiles are provided in the altitude range 10–40 km at 400, 440, 452, 470, 500, 525, 550, 672 and 750 nm for the period 2002–2012. FMI-GOMOSaero aerosol profiles have improved quality; they are in good agreement with other datasets.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Carlo Arosio, Alexei Rozanov, Mark Weber, Doug Degenstein, Adam Bourassa, Daniel Zawada, Michael Kiefer, Alexandra Laeng, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Christian Retscher, Robert Damadeo, and Jerry D. Lumpe
Atmos. Meas. Tech., 16, 1881–1899, https://doi.org/10.5194/amt-16-1881-2023, https://doi.org/10.5194/amt-16-1881-2023, 2023
Short summary
Short summary
The paper presents the updated SAGE-CCI-OMPS+ climate data record of monthly zonal mean ozone profiles. This dataset covers the stratosphere and combines measurements by nine limb and occultation satellite instruments (SAGE II, OSIRIS, MIPAS, SCIAMACHY, GOMOS, ACE-FTS, OMPS-LP, POAM III, and SAGE III/ISS). The update includes new versions of MIPAS, ACE-FTS, and OSIRIS datasets and introduces data from additional sensors (POAM III and SAGE III/ISS) and retrieval processors (OMPS-LP).
Viktoria F. Sofieva, Risto Hänninen, Mikhail Sofiev, Monika Szeląg, Hei Shing Lee, Johanna Tamminen, and Christian Retscher
Atmos. Meas. Tech., 15, 3193–3212, https://doi.org/10.5194/amt-15-3193-2022, https://doi.org/10.5194/amt-15-3193-2022, 2022
Short summary
Short summary
We present tropospheric ozone column datasets that have been created using combinations of total ozone column from OMI and TROPOMI with stratospheric ozone column datasets from several available limb-viewing instruments (MLS, OSIRIS, MIPAS, SCIAMACHY, OMPS-LP, GOMOS). The main results are (i) several methodological developments, (ii) new tropospheric ozone column datasets from OMI and TROPOMI, and (iii) a new high-resolution dataset of ozone profiles from limb satellite instruments.
Pekka T. Verronen, Antti Kero, Noora Partamies, Monika E. Szeląg, Shin-Ichiro Oyama, Yoshizumi Miyoshi, and Esa Turunen
Ann. Geophys., 39, 883–897, https://doi.org/10.5194/angeo-39-883-2021, https://doi.org/10.5194/angeo-39-883-2021, 2021
Short summary
Short summary
This paper is the first to simulate and analyse the pulsating aurorae impact on middle atmosphere on monthly/seasonal timescales. We find that pulsating aurorae have the potential to make a considerable contribution to the total energetic particle forcing and increase the impact on upper stratospheric odd nitrogen and ozone in the polar regions. Thus, it should be considered in atmospheric and climate simulations.
Viktoria F. Sofieva, Monika Szeląg, Johanna Tamminen, Erkki Kyrölä, Doug Degenstein, Chris Roth, Daniel Zawada, Alexei Rozanov, Carlo Arosio, John P. Burrows, Mark Weber, Alexandra Laeng, Gabriele P. Stiller, Thomas von Clarmann, Lucien Froidevaux, Nathaniel Livesey, Michel van Roozendael, and Christian Retscher
Atmos. Chem. Phys., 21, 6707–6720, https://doi.org/10.5194/acp-21-6707-2021, https://doi.org/10.5194/acp-21-6707-2021, 2021
Short summary
Short summary
The MErged GRIdded Dataset of Ozone Profiles is a long-term (2001–2018) stratospheric ozone profile climate data record with resolved longitudinal structure that combines the data from six limb satellite instruments. The dataset can be used for various analyses, some of which are discussed in the paper. In particular, regionally and vertically resolved ozone trends are evaluated, including trends in the polar regions.
Tuomas Häkkilä, Pekka T. Verronen, Luis Millán, Monika E. Szeląg, Niilo Kalakoski, and Antti Kero
Ann. Geophys., 38, 1299–1312, https://doi.org/10.5194/angeo-38-1299-2020, https://doi.org/10.5194/angeo-38-1299-2020, 2020
Short summary
Short summary
The atmospheric impacts of energetic particle precipitation (EPP) can be useful in understanding the uncertainties of measuring the precipitation. Hence, information on how strong of an EPP flux has observable atmospheric impacts is needed. In this study, we find such threshold flux values using odd hydrogen concentrations from both satellite observations and model simulations. We consider the effects of solar proton events and radiation belt electron precipitation in the middle atmosphere.
Jia Jia, Antti Kero, Niilo Kalakoski, Monika E. Szeląg, and Pekka T. Verronen
Atmos. Chem. Phys., 20, 14969–14982, https://doi.org/10.5194/acp-20-14969-2020, https://doi.org/10.5194/acp-20-14969-2020, 2020
Short summary
Short summary
Recent studies have reported up to a 10 % average decrease of lower stratospheric ozone at 20 km altitude following solar proton events (SPEs). Our study uses 49 events that occurred after the launch of Aura MLS (July 2004–now) and 177 events that occurred in the WACCM-D simulation period (Jan 1989–Dec 2012) to evaluate ozone changes following SPEs. The statistical and case-by-case studies show no solid evidence of SPE's direct impact on the lower stratospheric ozone.
Niilo Kalakoski, Pekka T. Verronen, Annika Seppälä, Monika E. Szeląg, Antti Kero, and Daniel R. Marsh
Atmos. Chem. Phys., 20, 8923–8938, https://doi.org/10.5194/acp-20-8923-2020, https://doi.org/10.5194/acp-20-8923-2020, 2020
Short summary
Short summary
Effects of solar proton events (SPEs) on middle atmosphere chemistry were studied using the WACCM-D chemistry–climate model, including an improved representation of lower ionosphere ion chemistry. This study includes 66 events in the years 1989–2012 and uses a statistical approach to determine the impact of the improved chemistry scheme. The differences shown highlight the importance of ion chemistry in models used to study energetic particle precipitation.
Pekka T. Verronen, Daniel R. Marsh, Monika E. Szeląg, and Niilo Kalakoski
Ann. Geophys., 38, 833–844, https://doi.org/10.5194/angeo-38-833-2020, https://doi.org/10.5194/angeo-38-833-2020, 2020
Short summary
Short summary
This paper is the first to study how the representation of the magnetic-local-time (MLT) dependency of electron precipitation impacts middle-atmospheric-ozone response on monthly timescales. We use a state-of-the-art chemistry–climate model with detailed lower-ionospheric chemistry for an advanced representation of atmospheric impacts of electron forcing. We find that the use of daily zonal-mean electron forcing will provide an accurate ozone response in long-term climate simulations.
Erkki Kyrölä, Monika E. Andersson, Pekka T. Verronen, Marko Laine, Simo Tukiainen, and Daniel R. Marsh
Atmos. Chem. Phys., 18, 5001–5019, https://doi.org/10.5194/acp-18-5001-2018, https://doi.org/10.5194/acp-18-5001-2018, 2018
Short summary
Short summary
In this work we compare three key constituents of the middle atmosphere (ozone, NO2, and NO3) from the GOMOS satellite instrument with the WACCM model. We find that in the stratosphere (below 50 km) ozone differences are very small, but in the mesosphere large deviations are found. GOMOS and WACCM NO2 agree reasonably well except in the polar areas. These differences can be connected to the solar particle storms. For NO3, WACCM results agree with GOMOS with a very high correlation.
Katja Matthes, Bernd Funke, Monika E. Andersson, Luke Barnard, Jürg Beer, Paul Charbonneau, Mark A. Clilverd, Thierry Dudok de Wit, Margit Haberreiter, Aaron Hendry, Charles H. Jackman, Matthieu Kretzschmar, Tim Kruschke, Markus Kunze, Ulrike Langematz, Daniel R. Marsh, Amanda C. Maycock, Stergios Misios, Craig J. Rodger, Adam A. Scaife, Annika Seppälä, Ming Shangguan, Miriam Sinnhuber, Kleareti Tourpali, Ilya Usoskin, Max van de Kamp, Pekka T. Verronen, and Stefan Versick
Geosci. Model Dev., 10, 2247–2302, https://doi.org/10.5194/gmd-10-2247-2017, https://doi.org/10.5194/gmd-10-2247-2017, 2017
Short summary
Short summary
The solar forcing dataset for climate model experiments performed for the upcoming IPCC report is described. This dataset provides the radiative and particle input of solar variability on a daily basis from 1850 through to 2300. With this dataset a better representation of natural climate variability with respect to the output of the Sun is provided which provides the most sophisticated and comprehensive respresentation of solar variability that has been used in climate model simulations so far.
Tamás Kovács, John M. C. Plane, Wuhu Feng, Tibor Nagy, Martyn P. Chipperfield, Pekka T. Verronen, Monika E. Andersson, David A. Newnham, Mark A. Clilverd, and Daniel R. Marsh
Geosci. Model Dev., 9, 3123–3136, https://doi.org/10.5194/gmd-9-3123-2016, https://doi.org/10.5194/gmd-9-3123-2016, 2016
Short summary
Short summary
This study was completed on D-region atmospheric model development. The sophisticated 3-D Whole Atmosphere Community Climate Model (WACCM) and the 1-D Sodynkalä Ion and Neutral Chemistry Model (SIC) were combined in order to provide a detailed, accurate model (WACCM-SIC) that considers the processes taking place in solar proton events. The original SIC model was reduced by mechanism reduction, which provided an accurate sub-mechanism (rSIC, WACCM-rSIC) of the original model.
P. T. Verronen, M. E. Andersson, A. Kero, C.-F. Enell, J. M. Wissing, E. R. Talaat, K. Kauristie, M. Palmroth, T. E. Sarris, and E. Armandillo
Ann. Geophys., 33, 381–394, https://doi.org/10.5194/angeo-33-381-2015, https://doi.org/10.5194/angeo-33-381-2015, 2015
Short summary
Short summary
Electron concentrations observed by EISCAT radars can be reasonable well represented using AIMOS v1.2 satellite-data-based ionization model and SIC D-region ion chemistry model. SIC-EISCAT difference varies from event to event, probably because the statistical nature of AIMOS ionization is not capturing all the spatio-temporal fine structure of electron precipitation. Below 90km, AIMOS overestimates electron ionization because of proton contamination of the satellite electron detectors.
Carlo Arosio, Viktoria Sofieva, Andrea Orfanoz-Cheuquelaf, Alexei Rozanov, Klaus-Peter Heue, Edward Malina, Ryan M. Stauffer, David Tarasick, Roeland Van Malderen, Jerry R. Ziemke, and Mark Weber
EGUsphere, https://doi.org/10.5194/egusphere-2024-3737, https://doi.org/10.5194/egusphere-2024-3737, 2024
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
Short summary
Short summary
Tropospheric ozone affects air quality and climate, being a pollutant and a greenhouse gas. We analysed satellite data of tropospheric ozone that combine two types of observations: one providing stratospheric ozone and another measuring total ozone. We compare common climatological features and study the influence of the tropopause (troposphere to stratosphere boundary) on the results. We also examine trends over the last 20 years and compare satellite data with ozonesondes to identify drifts.
Kimberlee Dubé, Susann Tegtmeier, Adam Bourassa, Daniel Zawada, Douglas Degenstein, William Randel, Sean Davis, Michael Schwartz, Nathaniel Livesey, and Anne Smith
Atmos. Chem. Phys., 24, 12925–12941, https://doi.org/10.5194/acp-24-12925-2024, https://doi.org/10.5194/acp-24-12925-2024, 2024
Short summary
Short summary
Greenhouse gas emissions that warm the troposphere also result in stratospheric cooling. The cooling rate is difficult to quantify above 35 km due to a deficit of long-term observational data with high vertical resolution in this region. We use satellite observations from several instruments, including a new temperature product from OSIRIS, to show that the upper stratosphere, from 35–60 km, cooled by 0.5 to 1 K per decade over 2005–2021 and by 0.6 K per decade over 1979–2021.
Viktoria F. Sofieva, Alexei Rozanov, Monika Szelag, John P. Burrows, Christian Retscher, Robert Damadeo, Doug Degenstein, Landon A. Rieger, and Adam Bourassa
Earth Syst. Sci. Data, 16, 5227–5241, https://doi.org/10.5194/essd-16-5227-2024, https://doi.org/10.5194/essd-16-5227-2024, 2024
Short summary
Short summary
Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived from data of six limb and occultation satellite instruments. The created aerosol climate record covers the period from October 1984 to December 2023. It can be used in various climate-related studies.
Miriam Sinnhuber, Christina Arras, Stefan Bender, Bernd Funke, Hanli Liu, Daniel R. Marsh, Thomas Reddmann, Eugene Rozanov, Timofei Sukhodolov, Monika E. Szelag, and Jan Maik Wissing
EGUsphere, https://doi.org/10.5194/egusphere-2024-2256, https://doi.org/10.5194/egusphere-2024-2256, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Formation of nitric oxide NO in the upper atmosphere varies with solar activity. Observations show that it starts a chain of processes in the entire atmosphere affecting the ozone layer and climate system. This is often underestimated in models. We compare five models which show large differences in simulated NO. Analysis of results point out problems related to the oxygen balance, and to the impact of atmospheric waves on dynamics. Both must be modeled well to reproduce the downward coupling.
Masatomo Fujiwara, Patrick Martineau, Jonathon S. Wright, Marta Abalos, Petr Šácha, Yoshio Kawatani, Sean M. Davis, Thomas Birner, and Beatriz M. Monge-Sanz
Atmos. Chem. Phys., 24, 7873–7898, https://doi.org/10.5194/acp-24-7873-2024, https://doi.org/10.5194/acp-24-7873-2024, 2024
Short summary
Short summary
A climatology of the major variables and terms of the transformed Eulerian-mean (TEM) momentum and thermodynamic equations from four global atmospheric reanalyses is evaluated. The spread among reanalysis TEM momentum balance terms is around 10 % in Northern Hemisphere winter and up to 50 % in Southern Hemisphere winter. The largest uncertainties in the thermodynamic equation (about 50 %) are in the vertical advection, which does not show a structure consistent with the differences in heating.
Mona Zolghadrshojaee, Susann Tegtmeier, Sean M. Davis, and Robin Pilch Kedzierski
Atmos. Chem. Phys., 24, 7405–7419, https://doi.org/10.5194/acp-24-7405-2024, https://doi.org/10.5194/acp-24-7405-2024, 2024
Short summary
Short summary
Satellite data challenge the idea of an overall cooling trend in the tropical tropopause layer. From 2002 to 2022, a warming trend was observed, diverging from earlier findings. Tropopause height changes indicate dynamic processes alongside radiative effects. Upper-tropospheric warming contrasts with lower-stratosphere temperatures. The study highlights the complex interplay of factors shaping temperature trends.
Robert P. Damadeo, Viktoria F. Sofieva, Alexei Rozanov, and Larry W. Thomason
Atmos. Meas. Tech., 17, 3669–3678, https://doi.org/10.5194/amt-17-3669-2024, https://doi.org/10.5194/amt-17-3669-2024, 2024
Short summary
Short summary
Comparing different aerosol data sets for scientific studies often requires converting aerosol extinction data between different wavelengths. A common approximation for the spectral behavior of aerosol is the Ångström formula; however, this introduces biases. Using measurements across many different wavelengths from a single instrument, we derive an empirical relationship to both characterize this bias and offer a correction for other studies that may employ this analysis approach.
Tuomas Häkkilä, Maxime Grandin, Markus Battarbee, Monika E. Szeląg, Markku Alho, Leo Kotipalo, Niilo Kalakoski, Pekka T. Verronen, and Minna Palmroth
Ann. Geophys. Discuss., https://doi.org/10.5194/angeo-2024-7, https://doi.org/10.5194/angeo-2024-7, 2024
Revised manuscript under review for ANGEO
Short summary
Short summary
We study the atmospheric impact of auroral electron precipitation, by the novel combination of both magnetospheric and atmospheric modelling. We first simulate fluxes of auroral electrons, and then use these fluxes to model their atmospheric impact. We find an increase of up to 200 % in thermospheric odd nitrogen, and a corresponding decrease in stratospheric ozone of around 0.7 %. The produced auroral electron precipitation is realistic, and shows the potential for future studies.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Didier Fussen, Christine Bingen, Filip Vanhellemont, Nina Mateshvili, Alexei Rozanov, and Christine Pohl
Atmos. Meas. Tech., 17, 3085–3101, https://doi.org/10.5194/amt-17-3085-2024, https://doi.org/10.5194/amt-17-3085-2024, 2024
Short summary
Short summary
We have developed the new multi-wavelength dataset of aerosol extinction profiles, which are retrieved from the averaged transmittance spectra by the Global Ozone Monitoring by Occultation of Stars instrument aboard Envisat. The retrieved aerosol extinction profiles are provided in the altitude range 10–40 km at 400, 440, 452, 470, 500, 525, 550, 672 and 750 nm for the period 2002–2012. FMI-GOMOSaero aerosol profiles have improved quality; they are in good agreement with other datasets.
Daniel Zawada, Kimberlee Dubé, Taran Warnock, Adam Bourassa, Susann Tegtmeier, and Douglas Degenstein
Atmos. Meas. Tech., 17, 1995–2010, https://doi.org/10.5194/amt-17-1995-2024, https://doi.org/10.5194/amt-17-1995-2024, 2024
Short summary
Short summary
There remain large uncertainties in long-term changes of stratospheric–atmospheric temperatures. We have produced a time series of more than 20 years of satellite-based temperature measurements from the OSIRIS instrument in the upper–middle stratosphere. The dataset is publicly available and intended to be used for a better understanding of changes in stratospheric temperatures.
Lukas Fehr, Chris McLinden, Debora Griffin, Daniel Zawada, Doug Degenstein, and Adam Bourassa
Geosci. Model Dev., 16, 7491–7507, https://doi.org/10.5194/gmd-16-7491-2023, https://doi.org/10.5194/gmd-16-7491-2023, 2023
Short summary
Short summary
This work highlights upgrades to SASKTRAN, a model that simulates sunlight interacting with the atmosphere to help measure trace gases. The upgrades were verified by detailed comparisons between different numerical methods. A case study was performed using SASKTRAN’s multidimensional capabilities, which found that ignoring horizontal variation in the atmosphere (a common practice in the field) can introduce non-negligible errors where there is snow or high pollution.
Kimberlee Dubé, Susann Tegtmeier, Adam Bourassa, Daniel Zawada, Douglas Degenstein, Patrick E. Sheese, Kaley A. Walker, and William Randel
Atmos. Chem. Phys., 23, 13283–13300, https://doi.org/10.5194/acp-23-13283-2023, https://doi.org/10.5194/acp-23-13283-2023, 2023
Short summary
Short summary
This paper presents a technique for understanding the causes of long-term changes in stratospheric composition. By using N2O as a proxy for stratospheric circulation in the model used to calculated trends, it is possible to separate the effects of dynamics and chemistry on observed trace gas trends. We find that observed HCl increases are due to changes in the stratospheric circulation, as are O3 decreases above 30 hPa in the Northern Hemisphere.
Ethan Runge, Jeff Langille, Daniel Zawada, Adam Bourassa, and Doug Degenstein
Atmos. Meas. Tech., 16, 3123–3139, https://doi.org/10.5194/amt-16-3123-2023, https://doi.org/10.5194/amt-16-3123-2023, 2023
Short summary
Short summary
The Limb Imaging Fourier Transform Spectrometer Experiment (LIFE) instrument takes vertical images of limb radiance across a wide mid-infrared spectral band from a stratospheric balloon. Measurements are used to infer vertical-trace-gas-profile retrievals of H2O, O3, HNO3, CH4, and N2O. Nearly time-/space-coincident observations from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) and Microwave Limb Sounder (MLS) instruments are compared to the LIFE results.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Carlo Arosio, Alexei Rozanov, Mark Weber, Doug Degenstein, Adam Bourassa, Daniel Zawada, Michael Kiefer, Alexandra Laeng, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Christian Retscher, Robert Damadeo, and Jerry D. Lumpe
Atmos. Meas. Tech., 16, 1881–1899, https://doi.org/10.5194/amt-16-1881-2023, https://doi.org/10.5194/amt-16-1881-2023, 2023
Short summary
Short summary
The paper presents the updated SAGE-CCI-OMPS+ climate data record of monthly zonal mean ozone profiles. This dataset covers the stratosphere and combines measurements by nine limb and occultation satellite instruments (SAGE II, OSIRIS, MIPAS, SCIAMACHY, GOMOS, ACE-FTS, OMPS-LP, POAM III, and SAGE III/ISS). The update includes new versions of MIPAS, ACE-FTS, and OSIRIS datasets and introduces data from additional sensors (POAM III and SAGE III/ISS) and retrieval processors (OMPS-LP).
Sean M. Davis, Nicholas Davis, Robert W. Portmann, Eric Ray, and Karen Rosenlof
Atmos. Chem. Phys., 23, 3347–3361, https://doi.org/10.5194/acp-23-3347-2023, https://doi.org/10.5194/acp-23-3347-2023, 2023
Short summary
Short summary
Ozone in the lower part of the stratosphere has not increased and has perhaps even continued to decline in recent decades. This study demonstrates that the amount of ozone in this region is highly sensitive to the amount of air upwelling into the stratosphere in the tropics and that simulations from a climate model nudged to historical meteorological fields often fail to accurately capture the variations in tropical upwelling that control short-term trends in lower-stratospheric ozone.
J. Douglas Goetz, Lars E. Kalnajs, Terry Deshler, Sean M. Davis, Martina Bramberger, and M. Joan Alexander
Atmos. Meas. Tech., 16, 791–807, https://doi.org/10.5194/amt-16-791-2023, https://doi.org/10.5194/amt-16-791-2023, 2023
Short summary
Short summary
An instrument for in situ continuous 2 km vertical profiles of temperature below high-altitude balloons was developed for high-temporal-resolution measurements within the upper troposphere and lower stratosphere using fiber-optic distributed temperature sensing. The mechanical, electrical, and temperature calibration systems were validated from a short mid-latitude constant-altitude balloon flight within the lower stratosphere. The instrument observed small-scale and inertial gravity waves.
Paul S. Jeffery, Kaley A. Walker, Chris E. Sioris, Chris D. Boone, Doug Degenstein, Gloria L. Manney, C. Thomas McElroy, Luis Millán, David A. Plummer, Niall J. Ryan, Patrick E. Sheese, and Jiansheng Zou
Atmos. Chem. Phys., 22, 14709–14734, https://doi.org/10.5194/acp-22-14709-2022, https://doi.org/10.5194/acp-22-14709-2022, 2022
Short summary
Short summary
The upper troposphere–lower stratosphere is one of the most variable regions in the atmosphere. To improve our understanding of water vapour and ozone concentrations in this region, climatologies have been developed from 14 years of measurements from three Canadian satellite instruments. Horizontal and vertical coordinates have been chosen to minimize the effects of variability. To aid in analysis, model simulations have been used to characterize differences between instrument climatologies.
Kimberlee Dubé, Daniel Zawada, Adam Bourassa, Doug Degenstein, William Randel, David Flittner, Patrick Sheese, and Kaley Walker
Atmos. Meas. Tech., 15, 6163–6180, https://doi.org/10.5194/amt-15-6163-2022, https://doi.org/10.5194/amt-15-6163-2022, 2022
Short summary
Short summary
Satellite observations are important for monitoring changes in atmospheric composition. Here we describe an improved version of the NO2 retrieval for the Optical Spectrograph and InfraRed Imager System. The resulting NO2 profiles are compared to those from the Atmospheric Chemistry Experiment – Fourier Transform Spectrometer and the Stratospheric Aerosol and Gas Experiment III on the International Space Station. All datasets agree within 20 % throughout the stratosphere.
Sophie Godin-Beekmann, Niramson Azouz, Viktoria F. Sofieva, Daan Hubert, Irina Petropavlovskikh, Peter Effertz, Gérard Ancellet, Doug A. Degenstein, Daniel Zawada, Lucien Froidevaux, Stacey Frith, Jeannette Wild, Sean Davis, Wolfgang Steinbrecht, Thierry Leblanc, Richard Querel, Kleareti Tourpali, Robert Damadeo, Eliane Maillard Barras, René Stübi, Corinne Vigouroux, Carlo Arosio, Gerald Nedoluha, Ian Boyd, Roeland Van Malderen, Emmanuel Mahieu, Dan Smale, and Ralf Sussmann
Atmos. Chem. Phys., 22, 11657–11673, https://doi.org/10.5194/acp-22-11657-2022, https://doi.org/10.5194/acp-22-11657-2022, 2022
Short summary
Short summary
An updated evaluation up to 2020 of stratospheric ozone profile long-term trends at extrapolar latitudes based on satellite and ground-based records is presented. Ozone increase in the upper stratosphere is confirmed, with significant trends at most latitudes. In this altitude region, a very good agreement is found with trends derived from chemistry–climate model simulations. Observed and modelled trends diverge in the lower stratosphere, but the differences are non-significant.
Niilo Kalakoski, Viktoria F. Sofieva, René Preusker, Claire Henocq, Matthieu Denisselle, Steffen Dransfeld, and Silvia Scifoni
Atmos. Meas. Tech., 15, 5129–5140, https://doi.org/10.5194/amt-15-5129-2022, https://doi.org/10.5194/amt-15-5129-2022, 2022
Short summary
Short summary
Geophysical validation of the Integrated Water Vapour (IWV) product from the Sentinel-3 Ocean and Land Colour Instrument (OLCI) was performed against reference observations from SUOMINET and IGRA databases. Results for cloud-free matchups over land show a wet bias of 7 %–10 % for OLCI, with a high correlation against the reference observations (0.98 against SUOMINET and 0.90 against IGRA). Special attention is given to validation of uncertainty estimates and cloud flagging.
Kristof Bognar, Susann Tegtmeier, Adam Bourassa, Chris Roth, Taran Warnock, Daniel Zawada, and Doug Degenstein
Atmos. Chem. Phys., 22, 9553–9569, https://doi.org/10.5194/acp-22-9553-2022, https://doi.org/10.5194/acp-22-9553-2022, 2022
Short summary
Short summary
We quantify recent changes in stratospheric ozone (outside the polar regions) using a combination of three satellite datasets. We find that upper stratospheric ozone have increased significantly since 2000, although the recovery shows an unexpected pause in the Northern Hemisphere. Combined with the likely decrease in ozone in the lower stratosphere, this presents an interesting challenge for predicting the future of the ozone layer.
Shlomi Ziskin Ziv, Chaim I. Garfinkel, Sean Davis, and Antara Banerjee
Atmos. Chem. Phys., 22, 7523–7538, https://doi.org/10.5194/acp-22-7523-2022, https://doi.org/10.5194/acp-22-7523-2022, 2022
Short summary
Short summary
Stratospheric water vapor is important for Earth's overall greenhouse effect and for ozone chemistry; however the factors governing its variability on interannual timescales are not fully known, and previous modeling studies have indicated that models struggle to capture this interannual variability. We demonstrate that nonlinear interactions are important for determining overall water vapor concentrations and also that models have improved in their ability to capture these connections.
Viktoria F. Sofieva, Risto Hänninen, Mikhail Sofiev, Monika Szeląg, Hei Shing Lee, Johanna Tamminen, and Christian Retscher
Atmos. Meas. Tech., 15, 3193–3212, https://doi.org/10.5194/amt-15-3193-2022, https://doi.org/10.5194/amt-15-3193-2022, 2022
Short summary
Short summary
We present tropospheric ozone column datasets that have been created using combinations of total ozone column from OMI and TROPOMI with stratospheric ozone column datasets from several available limb-viewing instruments (MLS, OSIRIS, MIPAS, SCIAMACHY, OMPS-LP, GOMOS). The main results are (i) several methodological developments, (ii) new tropospheric ozone column datasets from OMI and TROPOMI, and (iii) a new high-resolution dataset of ozone profiles from limb satellite instruments.
Julia Koch, Adam Bourassa, Nick Lloyd, Chris Roth, and Christian von Savigny
Atmos. Chem. Phys., 22, 3191–3202, https://doi.org/10.5194/acp-22-3191-2022, https://doi.org/10.5194/acp-22-3191-2022, 2022
Short summary
Short summary
The mesopause, the region of the earth's atmosphere between 85 and 100 km, is hard to access by direct measurements. Therefore we look for parameters that can be measured using satellite or ground-based measurements. In this study we researched sodium airglow, a phenomenon that occurs when sodium atoms are excited by chemical reactions. We compared satellite measurements of the airglow and resulting sodium concentration profiles to gain a better understanding of the sodium in that region.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Adam E. Bourassa, Doug A. Degenstein, Lucien Froidevaux, C. Thomas McElroy, Donal Murtagh, James M. Russell III, and Jiansheng Zou
Atmos. Meas. Tech., 15, 1233–1249, https://doi.org/10.5194/amt-15-1233-2022, https://doi.org/10.5194/amt-15-1233-2022, 2022
Short summary
Short summary
This study analyzes the quality of two versions (v3.6 and v4.1) of ozone concentration measurements from the ACE-FTS (Atmospheric Chemistry Experiment Fourier Transform Spectrometer), by comparing with data from five satellite instruments between 2004 and 2020. It was found that although the v3.6 data exhibit a better agreement than v4.1 with respect to the other instruments, v4.1 exhibits much better stability over time than v3.6. The stability of v4.1 makes it suitable for ozone trend studies.
Debora Griffin, Chris A. McLinden, Enrico Dammers, Cristen Adams, Chelsea E. Stockwell, Carsten Warneke, Ilann Bourgeois, Jeff Peischl, Thomas B. Ryerson, Kyle J. Zarzana, Jake P. Rowe, Rainer Volkamer, Christoph Knote, Natalie Kille, Theodore K. Koenig, Christopher F. Lee, Drew Rollins, Pamela S. Rickly, Jack Chen, Lukas Fehr, Adam Bourassa, Doug Degenstein, Katherine Hayden, Cristian Mihele, Sumi N. Wren, John Liggio, Ayodeji Akingunola, and Paul Makar
Atmos. Meas. Tech., 14, 7929–7957, https://doi.org/10.5194/amt-14-7929-2021, https://doi.org/10.5194/amt-14-7929-2021, 2021
Short summary
Short summary
Satellite-derived NOx emissions from biomass burning are estimated with TROPOMI observations. Two common emission estimation methods are applied, and sensitivity tests with model output were performed to determine the accuracy of these methods. The effect of smoke aerosols on TROPOMI NO2 columns is estimated and compared to aircraft observations from four different aircraft campaigns measuring biomass burning plumes in 2018 and 2019 in North America.
Anqi Li, Chris Z. Roth, Adam E. Bourassa, Douglas A. Degenstein, Kristell Pérot, Ole Martin Christensen, and Donal P. Murtagh
Earth Syst. Sci. Data, 13, 5115–5126, https://doi.org/10.5194/essd-13-5115-2021, https://doi.org/10.5194/essd-13-5115-2021, 2021
Short summary
Short summary
The nightglow emission originating from the vibrationally excited hydroxyl layer (about 85 km altitude) has been measured by the infrared imager (IRI) on the Odin satellite for more than 15 years. In this study, we document the retrieval steps, the resulting volume emission rates and the layer characteristics. Finally, we use the monthly zonal averages to demonstrate the fidelity of the data set. This unique, long-term data set will be valuable for studying various topics near the mesopause.
Nathaniel J. Livesey, William G. Read, Lucien Froidevaux, Alyn Lambert, Michelle L. Santee, Michael J. Schwartz, Luis F. Millán, Robert F. Jarnot, Paul A. Wagner, Dale F. Hurst, Kaley A. Walker, Patrick E. Sheese, and Gerald E. Nedoluha
Atmos. Chem. Phys., 21, 15409–15430, https://doi.org/10.5194/acp-21-15409-2021, https://doi.org/10.5194/acp-21-15409-2021, 2021
Short summary
Short summary
The Microwave Limb Sounder (MLS), an instrument on NASA's Aura mission launched in 2004, measures vertical profiles of the temperature and composition of Earth's "middle atmosphere" (the region from ~12 to ~100 km altitude). We describe how, among the 16 trace gases measured by MLS, the measurements of water vapor (H2O) and nitrous oxide (N2O) have started to drift since ~2010. The paper also discusses the origins of this drift and work to ameliorate it in a new version of the MLS dataset.
Pekka T. Verronen, Antti Kero, Noora Partamies, Monika E. Szeląg, Shin-Ichiro Oyama, Yoshizumi Miyoshi, and Esa Turunen
Ann. Geophys., 39, 883–897, https://doi.org/10.5194/angeo-39-883-2021, https://doi.org/10.5194/angeo-39-883-2021, 2021
Short summary
Short summary
This paper is the first to simulate and analyse the pulsating aurorae impact on middle atmosphere on monthly/seasonal timescales. We find that pulsating aurorae have the potential to make a considerable contribution to the total energetic particle forcing and increase the impact on upper stratospheric odd nitrogen and ozone in the polar regions. Thus, it should be considered in atmospheric and climate simulations.
Daniel Zawada, Ghislain Franssens, Robert Loughman, Antti Mikkonen, Alexei Rozanov, Claudia Emde, Adam Bourassa, Seth Dueck, Hannakaisa Lindqvist, Didier Ramon, Vladimir Rozanov, Emmanuel Dekemper, Erkki Kyrölä, John P. Burrows, Didier Fussen, and Doug Degenstein
Atmos. Meas. Tech., 14, 3953–3972, https://doi.org/10.5194/amt-14-3953-2021, https://doi.org/10.5194/amt-14-3953-2021, 2021
Short summary
Short summary
Satellite measurements of atmospheric composition often rely on computer tools known as radiative transfer models to model the propagation of sunlight within the atmosphere. Here we have performed a detailed inter-comparison of seven different radiative transfer models in a variety of conditions. We have found that the models agree remarkably well, at a level better than previously reported. This result provides confidence in our understanding of atmospheric radiative transfer.
Michaela I. Hegglin, Susann Tegtmeier, John Anderson, Adam E. Bourassa, Samuel Brohede, Doug Degenstein, Lucien Froidevaux, Bernd Funke, John Gille, Yasuko Kasai, Erkki T. Kyrölä, Jerry Lumpe, Donal Murtagh, Jessica L. Neu, Kristell Pérot, Ellis E. Remsberg, Alexei Rozanov, Matthew Toohey, Joachim Urban, Thomas von Clarmann, Kaley A. Walker, Hsiang-Jui Wang, Carlo Arosio, Robert Damadeo, Ryan A. Fuller, Gretchen Lingenfelser, Christopher McLinden, Diane Pendlebury, Chris Roth, Niall J. Ryan, Christopher Sioris, Lesley Smith, and Katja Weigel
Earth Syst. Sci. Data, 13, 1855–1903, https://doi.org/10.5194/essd-13-1855-2021, https://doi.org/10.5194/essd-13-1855-2021, 2021
Short summary
Short summary
An overview of the SPARC Data Initiative is presented, to date the most comprehensive assessment of stratospheric composition measurements spanning 1979–2018. Measurements of 26 chemical constituents obtained from an international suite of space-based limb sounders were compiled into vertically resolved, zonal monthly mean time series. The quality and consistency of these gridded datasets are then evaluated using a climatological validation approach and a range of diagnostics.
Viktoria F. Sofieva, Monika Szeląg, Johanna Tamminen, Erkki Kyrölä, Doug Degenstein, Chris Roth, Daniel Zawada, Alexei Rozanov, Carlo Arosio, John P. Burrows, Mark Weber, Alexandra Laeng, Gabriele P. Stiller, Thomas von Clarmann, Lucien Froidevaux, Nathaniel Livesey, Michel van Roozendael, and Christian Retscher
Atmos. Chem. Phys., 21, 6707–6720, https://doi.org/10.5194/acp-21-6707-2021, https://doi.org/10.5194/acp-21-6707-2021, 2021
Short summary
Short summary
The MErged GRIdded Dataset of Ozone Profiles is a long-term (2001–2018) stratospheric ozone profile climate data record with resolved longitudinal structure that combines the data from six limb satellite instruments. The dataset can be used for various analyses, some of which are discussed in the paper. In particular, regionally and vertically resolved ozone trends are evaluated, including trends in the polar regions.
Viktoria F. Sofieva, Hei Shing Lee, Johanna Tamminen, Christophe Lerot, Fabian Romahn, and Diego G. Loyola
Atmos. Meas. Tech., 14, 2993–3002, https://doi.org/10.5194/amt-14-2993-2021, https://doi.org/10.5194/amt-14-2993-2021, 2021
Short summary
Short summary
Our paper discusses the structure function method, which allows validation of random uncertainties in the data and, at the same time, probing of the small-scale natural variability. We applied this method to the clear-sky total ozone measurements by TROPOMI Sentinel-5P satellite instrument and found that the TROPOMI random error estimation is adequate. The discussed method is a powerful tool, which can be used in various applications.
Lars E. Kalnajs, Sean M. Davis, J. Douglas Goetz, Terry Deshler, Sergey Khaykin, Alex St. Clair, Albert Hertzog, Jerome Bordereau, and Alexey Lykov
Atmos. Meas. Tech., 14, 2635–2648, https://doi.org/10.5194/amt-14-2635-2021, https://doi.org/10.5194/amt-14-2635-2021, 2021
Short summary
Short summary
This work introduces a novel instrument system for high-resolution atmospheric profiling, which lowers and retracts a suspended instrument package beneath drifting long-duration balloons. During a 100 d circumtropical flight, the instrument collected over a hundred 2 km profiles of temperature, water vapor, clouds, and aerosol at 1 m resolution, yielding unprecedented geographic sampling and vertical resolution measurements of the tropical tropopause layer.
James Keeble, Birgit Hassler, Antara Banerjee, Ramiro Checa-Garcia, Gabriel Chiodo, Sean Davis, Veronika Eyring, Paul T. Griffiths, Olaf Morgenstern, Peer Nowack, Guang Zeng, Jiankai Zhang, Greg Bodeker, Susannah Burrows, Philip Cameron-Smith, David Cugnet, Christopher Danek, Makoto Deushi, Larry W. Horowitz, Anne Kubin, Lijuan Li, Gerrit Lohmann, Martine Michou, Michael J. Mills, Pierre Nabat, Dirk Olivié, Sungsu Park, Øyvind Seland, Jens Stoll, Karl-Hermann Wieners, and Tongwen Wu
Atmos. Chem. Phys., 21, 5015–5061, https://doi.org/10.5194/acp-21-5015-2021, https://doi.org/10.5194/acp-21-5015-2021, 2021
Short summary
Short summary
Stratospheric ozone and water vapour are key components of the Earth system; changes to both have important impacts on global and regional climate. We evaluate changes to these species from 1850 to 2100 in the new generation of CMIP6 models. There is good agreement between the multi-model mean and observations, although there is substantial variation between the individual models. The future evolution of both ozone and water vapour is strongly dependent on the assumed future emissions scenario.
Chaim I. Garfinkel, Ohad Harari, Shlomi Ziskin Ziv, Jian Rao, Olaf Morgenstern, Guang Zeng, Simone Tilmes, Douglas Kinnison, Fiona M. O'Connor, Neal Butchart, Makoto Deushi, Patrick Jöckel, Andrea Pozzer, and Sean Davis
Atmos. Chem. Phys., 21, 3725–3740, https://doi.org/10.5194/acp-21-3725-2021, https://doi.org/10.5194/acp-21-3725-2021, 2021
Short summary
Short summary
Water vapor is the dominant greenhouse gas in the atmosphere, and El Niño is the dominant mode of variability in the ocean–atmosphere system. The connection between El Niño and water vapor above ~ 17 km is unclear, with single-model studies reaching a range of conclusions. This study examines this connection in 12 different models. While there are substantial differences among the models, all models appear to capture the fundamental physical processes correctly.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Doug A. Degenstein, Felicia Kolonjari, David Plummer, Douglas E. Kinnison, Patrick Jöckel, and Thomas von Clarmann
Atmos. Meas. Tech., 14, 1425–1438, https://doi.org/10.5194/amt-14-1425-2021, https://doi.org/10.5194/amt-14-1425-2021, 2021
Short summary
Short summary
Output from climate chemistry models (CMAM, EMAC, and WACCM) is used to estimate the expected geophysical variability of ozone concentrations between coincident satellite instrument measurement times and geolocations. We use the Canadian ACE-FTS and OSIRIS instruments as a case study. Ensemble mean estimates are used to optimize coincidence criteria between the two instruments, allowing for the use of more coincident profiles while providing an estimate of the geophysical variation.
Kimberlee Dubé, Adam Bourassa, Daniel Zawada, Douglas Degenstein, Robert Damadeo, David Flittner, and William Randel
Atmos. Meas. Tech., 14, 557–566, https://doi.org/10.5194/amt-14-557-2021, https://doi.org/10.5194/amt-14-557-2021, 2021
Short summary
Short summary
SAGE III/ISS measures profiles of NO2; however the algorithm to convert raw measurements to NO2 concentration neglects variations caused by changes in chemistry over the course of a day. We devised a procedure to account for these diurnal variations and assess their impact on NO2 measurements from SAGE III/ISS. We find that the new NO2 concentration is more than 10 % lower than NO2 from the standard algorithm below 30 km, showing that this effect is important to consider at lower altitudes.
Tuomas Häkkilä, Pekka T. Verronen, Luis Millán, Monika E. Szeląg, Niilo Kalakoski, and Antti Kero
Ann. Geophys., 38, 1299–1312, https://doi.org/10.5194/angeo-38-1299-2020, https://doi.org/10.5194/angeo-38-1299-2020, 2020
Short summary
Short summary
The atmospheric impacts of energetic particle precipitation (EPP) can be useful in understanding the uncertainties of measuring the precipitation. Hence, information on how strong of an EPP flux has observable atmospheric impacts is needed. In this study, we find such threshold flux values using odd hydrogen concentrations from both satellite observations and model simulations. We consider the effects of solar proton events and radiation belt electron precipitation in the middle atmosphere.
Seidai Nara, Tomohiro O. Sato, Takayoshi Yamada, Tamaki Fujinawa, Kota Kuribayashi, Takeshi Manabe, Lucien Froidevaux, Nathaniel J. Livesey, Kaley A. Walker, Jian Xu, Franz Schreier, Yvan J. Orsolini, Varavut Limpasuvan, Nario Kuno, and Yasuko Kasai
Atmos. Meas. Tech., 13, 6837–6852, https://doi.org/10.5194/amt-13-6837-2020, https://doi.org/10.5194/amt-13-6837-2020, 2020
Short summary
Short summary
In the atmosphere, more than 80 % of chlorine compounds are anthropogenic. Hydrogen chloride (HCl), the main stratospheric chlorine reservoir, is useful to estimate the total budget of the atmospheric chlorine compounds. We report, for the first time, the HCl vertical distribution from the middle troposphere to the lower thermosphere using a high-sensitivity SMILES measurement; the data quality is quantified by comparisons with other measurements and via theoretical error analysis.
Jia Jia, Antti Kero, Niilo Kalakoski, Monika E. Szeląg, and Pekka T. Verronen
Atmos. Chem. Phys., 20, 14969–14982, https://doi.org/10.5194/acp-20-14969-2020, https://doi.org/10.5194/acp-20-14969-2020, 2020
Short summary
Short summary
Recent studies have reported up to a 10 % average decrease of lower stratospheric ozone at 20 km altitude following solar proton events (SPEs). Our study uses 49 events that occurred after the launch of Aura MLS (July 2004–now) and 177 events that occurred in the WACCM-D simulation period (Jan 1989–Dec 2012) to evaluate ozone changes following SPEs. The statistical and case-by-case studies show no solid evidence of SPE's direct impact on the lower stratospheric ozone.
Anqi Li, Chris Z. Roth, Kristell Pérot, Ole Martin Christensen, Adam Bourassa, Doug A. Degenstein, and Donal P. Murtagh
Atmos. Meas. Tech., 13, 6215–6236, https://doi.org/10.5194/amt-13-6215-2020, https://doi.org/10.5194/amt-13-6215-2020, 2020
Short summary
Short summary
The OSIRIS IR imager, one of the instruments on the Odin satellite, routinely measures the oxygen airglow at 1.27 μm. In this study, we primarily focus on the steps done for retrieving the calibrated IRA band limb radiance, the volume emission rate of O2(a1∆g) and finally the ozone number density. Specifically, we use a novel approach to address the issue of the measurements that were made close to the local sunrise, where the O2(a1∆g) diverges from the equilibrium state.
Stephanie Evan, Jerome Brioude, Karen Rosenlof, Sean M. Davis, Holger Vömel, Damien Héron, Françoise Posny, Jean-Marc Metzger, Valentin Duflot, Guillaume Payen, Hélène Vérèmes, Philippe Keckhut, and Jean-Pierre Cammas
Atmos. Chem. Phys., 20, 10565–10586, https://doi.org/10.5194/acp-20-10565-2020, https://doi.org/10.5194/acp-20-10565-2020, 2020
Short summary
Short summary
The role of deep convection in the southwest Indian Ocean (the 3rd most active tropical cyclone basin) on the composition of the tropical tropopause layer (TTL) and the climate system is less understood due to scarce observations. Balloon-borne lidar and satellite measurements in the southwest Indian Ocean were used to study tropical cyclones' influence on TTL composition. This study compares the impact of a tropical storm and cyclone on the humidification of the TTL over the SW Indian Ocean.
Thomas von Clarmann, Douglas A. Degenstein, Nathaniel J. Livesey, Stefan Bender, Amy Braverman, André Butz, Steven Compernolle, Robert Damadeo, Seth Dueck, Patrick Eriksson, Bernd Funke, Margaret C. Johnson, Yasuko Kasai, Arno Keppens, Anne Kleinert, Natalya A. Kramarova, Alexandra Laeng, Bavo Langerock, Vivienne H. Payne, Alexei Rozanov, Tomohiro O. Sato, Matthias Schneider, Patrick Sheese, Viktoria Sofieva, Gabriele P. Stiller, Christian von Savigny, and Daniel Zawada
Atmos. Meas. Tech., 13, 4393–4436, https://doi.org/10.5194/amt-13-4393-2020, https://doi.org/10.5194/amt-13-4393-2020, 2020
Short summary
Short summary
Remote sensing of atmospheric state variables typically relies on the inverse solution of the radiative transfer equation. An adequately characterized retrieval provides information on the uncertainties of the estimated state variables as well as on how any constraint or a priori assumption affects the estimate. This paper summarizes related techniques and provides recommendations for unified error reporting.
Niilo Kalakoski, Pekka T. Verronen, Annika Seppälä, Monika E. Szeląg, Antti Kero, and Daniel R. Marsh
Atmos. Chem. Phys., 20, 8923–8938, https://doi.org/10.5194/acp-20-8923-2020, https://doi.org/10.5194/acp-20-8923-2020, 2020
Short summary
Short summary
Effects of solar proton events (SPEs) on middle atmosphere chemistry were studied using the WACCM-D chemistry–climate model, including an improved representation of lower ionosphere ion chemistry. This study includes 66 events in the years 1989–2012 and uses a statistical approach to determine the impact of the improved chemistry scheme. The differences shown highlight the importance of ion chemistry in models used to study energetic particle precipitation.
Pekka T. Verronen, Daniel R. Marsh, Monika E. Szeląg, and Niilo Kalakoski
Ann. Geophys., 38, 833–844, https://doi.org/10.5194/angeo-38-833-2020, https://doi.org/10.5194/angeo-38-833-2020, 2020
Short summary
Short summary
This paper is the first to study how the representation of the magnetic-local-time (MLT) dependency of electron precipitation impacts middle-atmospheric-ozone response on monthly timescales. We use a state-of-the-art chemistry–climate model with detailed lower-ionospheric chemistry for an advanced representation of atmospheric impacts of electron forcing. We find that the use of daily zonal-mean electron forcing will provide an accurate ozone response in long-term climate simulations.
Jeffery Langille, Adam Bourassa, Laura L. Pan, Daniel Letros, Brian Solheim, Daniel Zawada, and Doug Degenstein
Atmos. Chem. Phys., 20, 5477–5486, https://doi.org/10.5194/acp-20-5477-2020, https://doi.org/10.5194/acp-20-5477-2020, 2020
Short summary
Short summary
Water vapour (WV) is a highly variable and extremely important trace gas in Earth’s atmosphere. Due to its radiative and chemical properties, it is coupled to the climate in an extremely complex manner. This is especially true in the lowermost stratosphere (LMS). Despite its importance, the physical processes that control mixing and the distribution of WV in the LMS are poorly understood. This study provides observational evidence of moistening the LMS via mixing across the subtropical jet.
Kevin M. Grise and Sean M. Davis
Atmos. Chem. Phys., 20, 5249–5268, https://doi.org/10.5194/acp-20-5249-2020, https://doi.org/10.5194/acp-20-5249-2020, 2020
Short summary
Short summary
As Earth's climate warms, the tropical overturning circulation (Hadley circulation) is projected to expand, potentially pushing subtropical dry zones further poleward. This study examines projections of the Hadley circulation from the latest generation of computer models and finds several notable differences from older models. For example, the Northern Hemisphere circulation has expanded northward at a greater rate in recent decades than would be expected from increasing greenhouse gases alone.
Nicholas A. Davis, Sean M. Davis, Robert W. Portmann, Eric Ray, Karen H. Rosenlof, and Pengfei Yu
Geosci. Model Dev., 13, 717–734, https://doi.org/10.5194/gmd-13-717-2020, https://doi.org/10.5194/gmd-13-717-2020, 2020
Short summary
Short summary
Large-scale waves drive upward motion in the tropical stratosphere, with major impacts on stratospheric chemistry and climate. However, some of the modeling methods which attempt to simulate the past evolution of the stratosphere do not seem to be able to recreate important trends. We believe this is due to disagreements between the basic climate of the model and observations, but if the method is constructed more carefully, the disagreement becomes smaller and the trends become more realistic.
Mikhail Sofiev, Rostislav Kouznetsov, Risto Hänninen, and Viktoria F. Sofieva
Atmos. Chem. Phys., 20, 1839–1847, https://doi.org/10.5194/acp-20-1839-2020, https://doi.org/10.5194/acp-20-1839-2020, 2020
Short summary
Short summary
An episode of anomalously low ozone concentrations in the stratosphere over northern Europe occurred on 3–5 November 2018. The 30 % reduction of the ozone layer was predicted by the global chemistry-transport model of the Finnish Meteorological Institute driven by weather forecasts of ECMWF. The reduction was subsequently observed by ozone monitoring satellites. The episode was caused by a storm in the northern Atlantic, which uplifted air from the troposphere to stratosphere.
Susann Tegtmeier, James Anstey, Sean Davis, Rossana Dragani, Yayoi Harada, Ioana Ivanciu, Robin Pilch Kedzierski, Kirstin Krüger, Bernard Legras, Craig Long, James S. Wang, Krzysztof Wargan, and Jonathon S. Wright
Atmos. Chem. Phys., 20, 753–770, https://doi.org/10.5194/acp-20-753-2020, https://doi.org/10.5194/acp-20-753-2020, 2020
Short summary
Short summary
The tropical tropopause layer is an important atmospheric region right in between the troposphere and the stratosphere. We evaluate the representation of this layer in reanalyses data sets, which create a complete picture of the state of Earth's atmosphere using atmospheric modeling and available observations. The recent reanalyses show realistic temperatures in the tropical tropopause layer. However, where the temperature is lowest, the so-called cold point, the reanalyses are too cold.
William T. Ball, Justin Alsing, Johannes Staehelin, Sean M. Davis, Lucien Froidevaux, and Thomas Peter
Atmos. Chem. Phys., 19, 12731–12748, https://doi.org/10.5194/acp-19-12731-2019, https://doi.org/10.5194/acp-19-12731-2019, 2019
Short summary
Short summary
We analyse long-term stratospheric ozone (60° S–60° N) trends over the 1985–2018 period. Previous work has suggested that lower stratosphere ozone declined over 1998–2016. We demonstrate that a large ozone upsurge in 2017 is likely related to QBO variability, but that lower stratospheric ozone trends likely remain lower in 2018 than in 1998. Tropical stratospheric ozone (30° S–30° N) shows highly probable decreases in both the lower stratosphere and in the integrated stratospheric ozone layer.
Ohad Harari, Chaim I. Garfinkel, Shlomi Ziskin Ziv, Olaf Morgenstern, Guang Zeng, Simone Tilmes, Douglas Kinnison, Makoto Deushi, Patrick Jöckel, Andrea Pozzer, Fiona M. O'Connor, and Sean Davis
Atmos. Chem. Phys., 19, 9253–9268, https://doi.org/10.5194/acp-19-9253-2019, https://doi.org/10.5194/acp-19-9253-2019, 2019
Short summary
Short summary
Ozone depletion in the Antarctic has been shown to influence surface conditions, but the effects of ozone depletion in the Arctic on surface climate are unclear. We show that Arctic ozone does influence surface climate in both polar regions and tropical regions, though the proximate cause of these surface impacts is not yet clear.
Elizaveta Malinina, Alexei Rozanov, Landon Rieger, Adam Bourassa, Heinrich Bovensmann, John P. Burrows, and Doug Degenstein
Atmos. Meas. Tech., 12, 3485–3502, https://doi.org/10.5194/amt-12-3485-2019, https://doi.org/10.5194/amt-12-3485-2019, 2019
Short summary
Short summary
This paper covers the problems related to the derivation of aerosol extinction coefficients and Ångström exponents from space-borne instruments working in limb and occultation viewing geometries. Aerosol extinction coefficients and Ångström exponents were calculated from the SCIAMACHY aerosol particle size data set. The results were compared with the data from SAGE II and OSIRIS. The Ångström exponent in the tropical regions and its dependency on particle size parameters are discussed.
Jerry R. Ziemke, Luke D. Oman, Sarah A. Strode, Anne R. Douglass, Mark A. Olsen, Richard D. McPeters, Pawan K. Bhartia, Lucien Froidevaux, Gordon J. Labow, Jacquie C. Witte, Anne M. Thompson, David P. Haffner, Natalya A. Kramarova, Stacey M. Frith, Liang-Kang Huang, Glen R. Jaross, Colin J. Seftor, Mathew T. Deland, and Steven L. Taylor
Atmos. Chem. Phys., 19, 3257–3269, https://doi.org/10.5194/acp-19-3257-2019, https://doi.org/10.5194/acp-19-3257-2019, 2019
Short summary
Short summary
Both a 38-year merged satellite record of tropospheric ozone from TOMS/OMI/MLS/OMPS and a MERRA-2 GMI model simulation show large increases of 6–7 Dobson units from the Near East to India–East Asia and eastward over the Pacific. These increases in tropospheric ozone are attributed to increases in pollution over the region over the last several decades. Secondary 38-year increases of 4–5 Dobson units with both GMI model and satellite measurements occur over central African–tropical Atlantic.
Alain Hauchecorne, Laurent Blanot, Robin Wing, Philippe Keckhut, Sergey Khaykin, Jean-Loup Bertaux, Mustapha Meftah, Chantal Claud, and Viktoria Sofieva
Atmos. Meas. Tech., 12, 749–761, https://doi.org/10.5194/amt-12-749-2019, https://doi.org/10.5194/amt-12-749-2019, 2019
Short summary
Short summary
This paper presents a new dataset of temperature profiles in the upper stratosphere and mesosphere acquired with the GOMOS spectrometer on board the European satellite ENVISAT. The principle is to observe the scattering of sunlight by air molecules at the Earth limb. The observed signal is proportional to the atmospheric density from which the temperature is derived. This technique provides a new source of information on temperature where satellite observations are sparse.
Viktoria F. Sofieva, Francis Dalaudier, Alain Hauchecorne, and Valery Kan
Atmos. Meas. Tech., 12, 585–598, https://doi.org/10.5194/amt-12-585-2019, https://doi.org/10.5194/amt-12-585-2019, 2019
Short summary
Short summary
This paper describes the temperature profiles in the stratosphere obtained from unique stellar scintillation measurements by the GOMOS instrument operated on board Envisat in 2002–2012. The high-resolution temperature profiles (HRTPs) are retrieved with a very good vertical resolution of ~ 200 m and a high accuracy of ~ 1–3 K for altitudes 15–32 km as well as a global coverage. HRTPs can be assimilated into atmospheric models and used in analyses of internal gravity wave activity.
Jeffery Langille, Daniel Letros, Adam Bourassa, Brian Solheim, Doug Degenstein, Fabien Dupont, Daniel Zawada, and Nick D. Lloyd
Atmos. Meas. Tech., 12, 431–455, https://doi.org/10.5194/amt-12-431-2019, https://doi.org/10.5194/amt-12-431-2019, 2019
Short summary
Short summary
The SHOW instrument is a prototype satellite concept that is being developed through collaboration between the University of Saskatchewan, the Canadian Space Agency, and ABB Inc. to provide high vertical resolution (< 200 m) measurements of UTLS water vapour with < 1 ppm accuracy. This paper presents suborbital measurements obtained during a demonstration flight aboard NASA's ER-2 aircraft. These measurements are validated through a comparison with coincident radiosonde measurements.
Ori Adam, Kevin M. Grise, Paul Staten, Isla R. Simpson, Sean M. Davis, Nicholas A. Davis, Darryn W. Waugh, Thomas Birner, and Alison Ming
Geosci. Model Dev., 11, 4339–4357, https://doi.org/10.5194/gmd-11-4339-2018, https://doi.org/10.5194/gmd-11-4339-2018, 2018
Short summary
Short summary
Due to incoherent methodologies, estimates of tropical width variations differ significantly across studies. Here, methods for eight commonly-used metrics of the tropical width are implemented in the Tropical-width Diagnostics (TropD) code package. The method compilation and analysis provide tools and information which help reduce the methodological component of the uncertainty associated with calculations of the tropical width.
Birgit Hassler, Stefanie Kremser, Greg E. Bodeker, Jared Lewis, Kage Nesbit, Sean M. Davis, Martyn P. Chipperfield, Sandip S. Dhomse, and Martin Dameris
Earth Syst. Sci. Data, 10, 1473–1490, https://doi.org/10.5194/essd-10-1473-2018, https://doi.org/10.5194/essd-10-1473-2018, 2018
Alexandra Laeng, Ellen Eckert, Thomas von Clarmann, Michael Kiefer, Daan Hubert, Gabriele Stiller, Norbert Glatthor, Manuel López-Puertas, Bernd Funke, Udo Grabowski, Johannes Plieninger, Sylvia Kellmann, Andrea Linden, Stefan Lossow, Arne Babenhauserheide, Lucien Froidevaux, and Kaley Walker
Atmos. Meas. Tech., 11, 4693–4705, https://doi.org/10.5194/amt-11-4693-2018, https://doi.org/10.5194/amt-11-4693-2018, 2018
Short summary
Short summary
MIPAS was an IR limb emission spectrometer on the Envisat platform. From 2002 to 2012, it performed pole-to-pole measurements of ozone during day and night. ESA recently released the new version 7 of Level 1 MIPAS spectra, which is expected to reduce the long-term drift of the MIPAS Level 2 data. We evaluate the long-term stability of ozone Level 2 data from the KIT IMK processor. Our results indicate that MIPAS data are now even more suited for trend studies, alone or as part of merged data.
Landon A. Rieger, Elizaveta P. Malinina, Alexei V. Rozanov, John P. Burrows, Adam E. Bourassa, and Doug A. Degenstein
Atmos. Meas. Tech., 11, 3433–3445, https://doi.org/10.5194/amt-11-3433-2018, https://doi.org/10.5194/amt-11-3433-2018, 2018
Short summary
Short summary
This paper compares aerosol extinction records from two limb scattering instruments, OSIRIS and SCIAMACHY, to that from the occultation instrument SAGE II. Differences are investigated through modelling and retrieval studies and important sources of systematic errors are quantified. It is found that the largest biases come from uncertainties in the aerosol size distribution and the aerosol particle concentration at altitudes above 30 km.
Natalya A. Kramarova, Pawan K. Bhartia, Glen Jaross, Leslie Moy, Philippe Xu, Zhong Chen, Matthew DeLand, Lucien Froidevaux, Nathaniel Livesey, Douglas Degenstein, Adam Bourassa, Kaley A. Walker, and Patrick Sheese
Atmos. Meas. Tech., 11, 2837–2861, https://doi.org/10.5194/amt-11-2837-2018, https://doi.org/10.5194/amt-11-2837-2018, 2018
Short summary
Short summary
The Ozone Mapping and Profiler Suite (OMPS) Limb Profiler (LP) is a newly designed research sensor aiming to continue high vertical resolution ozone records from space-borne sensors. In summer 2017 all LP measurements were processed with the new version 2.5 algorithm. In this paper we provide a description of the key changes implemented in the new algorithm and evaluate the quality of ozone retrievals by comparing with independent satellite profile measurements (MLS, ACE-FTS and OSIRIS).
Christos Zerefos, John Kapsomenakis, Kostas Eleftheratos, Kleareti Tourpali, Irina Petropavlovskikh, Daan Hubert, Sophie Godin-Beekmann, Wolfgang Steinbrecht, Stacey Frith, Viktoria Sofieva, and Birgit Hassler
Atmos. Chem. Phys., 18, 6427–6440, https://doi.org/10.5194/acp-18-6427-2018, https://doi.org/10.5194/acp-18-6427-2018, 2018
Short summary
Short summary
We point out the representativeness of single lidar stations for zonally averaged ozone profile variations in the middle/upper stratosphere. We examine the contribution of chemistry and natural proxies to ozone profile trends. Above 10 hPa an “inflection point” between 1997–99 marks the end of significant negative ozone trends, followed by a recent period of positive ozone change in 1998–2015. Below 15 hPa the pre-1998 negative ozone trends tend to become insignificant as we move to 2015.
Daniel J. Zawada, Landon A. Rieger, Adam E. Bourassa, and Douglas A. Degenstein
Atmos. Meas. Tech., 11, 2375–2393, https://doi.org/10.5194/amt-11-2375-2018, https://doi.org/10.5194/amt-11-2375-2018, 2018
Short summary
Short summary
The Ozone Mapping and Profiler Suite Limb Profiler measures scattered sunlight, which is then inverted to obtain vertical profiles of ozone in the atmosphere. We have developed a new algorithm for inverting the data which is better suited for areas with large horizontal ozone gradients, such as the polar vortex. Data from the full currently 5-year mission have been processed and are publicly available.
Manuel López-Puertas, Maya García-Comas, Bernd Funke, Angela Gardini, Gabriele P. Stiller, Thomas von Clarmann, Norbert Glatthor, Alexandra Laeng, Martin Kaufmann, Viktoria F. Sofieva, Lucien Froidevaux, Kaley A. Walker, and Masato Shiotani
Atmos. Meas. Tech., 11, 2187–2212, https://doi.org/10.5194/amt-11-2187-2018, https://doi.org/10.5194/amt-11-2187-2018, 2018
Short summary
Short summary
This paper describes the inversion of O3 data from MIPAS middle atmosphere spectra which requires non-LTE. The O3 dataset comprises from 20 to 100 km, has a pole-to-pole latitude coverage, day and nighttime, and span from 2005 until 2012. A validation of the data against other satellite measurements and an overall description of O3 is also presented. This is an important dataset for the community and describes the major characteristics of stratospheric and mesospheric O3.
Erkki Kyrölä, Monika E. Andersson, Pekka T. Verronen, Marko Laine, Simo Tukiainen, and Daniel R. Marsh
Atmos. Chem. Phys., 18, 5001–5019, https://doi.org/10.5194/acp-18-5001-2018, https://doi.org/10.5194/acp-18-5001-2018, 2018
Short summary
Short summary
In this work we compare three key constituents of the middle atmosphere (ozone, NO2, and NO3) from the GOMOS satellite instrument with the WACCM model. We find that in the stratosphere (below 50 km) ozone differences are very small, but in the mesosphere large deviations are found. GOMOS and WACCM NO2 agree reasonably well except in the polar areas. These differences can be connected to the solar particle storms. For NO3, WACCM results agree with GOMOS with a very high correlation.
Chaim I. Garfinkel, Amit Gordon, Luke D. Oman, Feng Li, Sean Davis, and Steven Pawson
Atmos. Chem. Phys., 18, 4597–4615, https://doi.org/10.5194/acp-18-4597-2018, https://doi.org/10.5194/acp-18-4597-2018, 2018
Short summary
Short summary
The impact of El Niño in the lower stratosphere is nonlinear in spring. While moderate El Niño events lead to cooling in this region,
strong El Niño events appear to lead to warming, and hence the water vapor response is nonlinear too. The net effect is that strong
El Nino events, such as in 1997/1998 and 2015/2016, lead to qualitatively different water vapor impacts as compared to moderate
El Nino events.
Valery Kan, Michael E. Gorbunov, and Viktoria F. Sofieva
Atmos. Meas. Tech., 11, 663–680, https://doi.org/10.5194/amt-11-663-2018, https://doi.org/10.5194/amt-11-663-2018, 2018
Short summary
Short summary
We discuss the relationships that link the observed fluctuation spectra of the amplitude and phase of signals used for the radio occultation sounding of the Earth's atmosphere with the spectra of atmospheric inhomogeneities. We demonstrate that the main contribution into the radio signal fluctuations comes from the internal gravity waves. These results may serve as the basis for the global monitoring of the wave activity in the stratosphere and upper troposphere.
William T. Ball, Justin Alsing, Daniel J. Mortlock, Johannes Staehelin, Joanna D. Haigh, Thomas Peter, Fiona Tummon, Rene Stübi, Andrea Stenke, John Anderson, Adam Bourassa, Sean M. Davis, Doug Degenstein, Stacey Frith, Lucien Froidevaux, Chris Roth, Viktoria Sofieva, Ray Wang, Jeannette Wild, Pengfei Yu, Jerald R. Ziemke, and Eugene V. Rozanov
Atmos. Chem. Phys., 18, 1379–1394, https://doi.org/10.5194/acp-18-1379-2018, https://doi.org/10.5194/acp-18-1379-2018, 2018
Short summary
Short summary
Using a robust analysis, with artefact-corrected ozone data, we confirm upper stratospheric ozone is recovering following the Montreal Protocol, but that lower stratospheric ozone (50° S–50° N) has continued to decrease since 1998, and the ozone layer as a whole (60° S–60° N) may be lower today than in 1998. No change in total column ozone may be due to increasing tropospheric ozone. State-of-the-art models do not reproduce lower stratospheric ozone decreases.
Adam E. Bourassa, Chris Z. Roth, Daniel J. Zawada, Landon A. Rieger, Chris A. McLinden, and Douglas A. Degenstein
Atmos. Meas. Tech., 11, 489–498, https://doi.org/10.5194/amt-11-489-2018, https://doi.org/10.5194/amt-11-489-2018, 2018
Short summary
Short summary
OSIRIS satellite measurements of ozone in the stratosphere are corrected for slowly varying errors. These changes make the OSIRIS data compare better with other satellite measurements over the long term and make an impact on our understanding of the recovery of the ozone layer.
Craig S. Long, Masatomo Fujiwara, Sean Davis, Daniel M. Mitchell, and Corwin J. Wright
Atmos. Chem. Phys., 17, 14593–14629, https://doi.org/10.5194/acp-17-14593-2017, https://doi.org/10.5194/acp-17-14593-2017, 2017
Short summary
Short summary
As part of the SPARC Reanalysis Intercomparison Project, we evaluate the temperature and wind structure of all the recent and past reanalyses with 2.5-degree monthly zonal mean data sets from 1979–2014. There is a distinct change in the temperature structure in the stratosphere in 1998. Zonal winds are in greater agreement than temperatures. All reanalyses have issues analysing the tropical stratospheric winds. Caution is advised for using reanalysis temperatures for trend detection.
Sean M. Davis, Michaela I. Hegglin, Masatomo Fujiwara, Rossana Dragani, Yayoi Harada, Chiaki Kobayashi, Craig Long, Gloria L. Manney, Eric R. Nash, Gerald L. Potter, Susann Tegtmeier, Tao Wang, Krzysztof Wargan, and Jonathon S. Wright
Atmos. Chem. Phys., 17, 12743–12778, https://doi.org/10.5194/acp-17-12743-2017, https://doi.org/10.5194/acp-17-12743-2017, 2017
Short summary
Short summary
Ozone and water vapor in the stratosphere are important gases that affect surface climate and absorb incoming solar ultraviolet radiation. These gases are represented in reanalyses, which create a complete picture of the state of Earth's atmosphere using limited observations. We evaluate reanalysis water vapor and ozone fidelity by intercomparing them, and comparing them to independent observations. Generally reanalyses do a good job at representing ozone, but have problems with water vapor.
Viktoria F. Sofieva, Erkki Kyrölä, Marko Laine, Johanna Tamminen, Doug Degenstein, Adam Bourassa, Chris Roth, Daniel Zawada, Mark Weber, Alexei Rozanov, Nabiz Rahpoe, Gabriele Stiller, Alexandra Laeng, Thomas von Clarmann, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Claus Zehner, Robert Damadeo, Joseph Zawodny, Natalya Kramarova, and Pawan K. Bhartia
Atmos. Chem. Phys., 17, 12533–12552, https://doi.org/10.5194/acp-17-12533-2017, https://doi.org/10.5194/acp-17-12533-2017, 2017
Short summary
Short summary
We present a merged dataset of ozone profiles from several satellite instruments: SAGE II, GOMOS, SCIAMACHY, MIPAS, OSIRIS, ACE-FTS and OMPS. For merging, we used the latest versions of the original ozone datasets.
The merged SAGE–CCI–OMPS dataset is used for evaluating ozone trends in the stratosphere through multiple linear regression. Negative ozone trends in the upper stratosphere are observed before 1997 and positive trends are found after 1997.
Wolfgang Steinbrecht, Lucien Froidevaux, Ryan Fuller, Ray Wang, John Anderson, Chris Roth, Adam Bourassa, Doug Degenstein, Robert Damadeo, Joe Zawodny, Stacey Frith, Richard McPeters, Pawan Bhartia, Jeannette Wild, Craig Long, Sean Davis, Karen Rosenlof, Viktoria Sofieva, Kaley Walker, Nabiz Rahpoe, Alexei Rozanov, Mark Weber, Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Natalya Kramarova, Sophie Godin-Beekmann, Thierry Leblanc, Richard Querel, Daan Swart, Ian Boyd, Klemens Hocke, Niklaus Kämpfer, Eliane Maillard Barras, Lorena Moreira, Gerald Nedoluha, Corinne Vigouroux, Thomas Blumenstock, Matthias Schneider, Omaira García, Nicholas Jones, Emmanuel Mahieu, Dan Smale, Michael Kotkamp, John Robinson, Irina Petropavlovskikh, Neil Harris, Birgit Hassler, Daan Hubert, and Fiona Tummon
Atmos. Chem. Phys., 17, 10675–10690, https://doi.org/10.5194/acp-17-10675-2017, https://doi.org/10.5194/acp-17-10675-2017, 2017
Short summary
Short summary
Thanks to the 1987 Montreal Protocol and its amendments, ozone-depleting chlorine (and bromine) in the stratosphere has declined slowly since the late 1990s. Improved and extended long-term ozone profile observations from satellites and ground-based stations confirm that ozone is responding as expected and has increased by about 2 % per decade since 2000 in the upper stratosphere, around 40 km altitude. At lower altitudes, however, ozone has not changed significantly since 2000.
Christopher J. Merchant, Frank Paul, Thomas Popp, Michael Ablain, Sophie Bontemps, Pierre Defourny, Rainer Hollmann, Thomas Lavergne, Alexandra Laeng, Gerrit de Leeuw, Jonathan Mittaz, Caroline Poulsen, Adam C. Povey, Max Reuter, Shubha Sathyendranath, Stein Sandven, Viktoria F. Sofieva, and Wolfgang Wagner
Earth Syst. Sci. Data, 9, 511–527, https://doi.org/10.5194/essd-9-511-2017, https://doi.org/10.5194/essd-9-511-2017, 2017
Short summary
Short summary
Climate data records (CDRs) contain data describing Earth's climate and should address uncertainty in the data to communicate what is known about climate variability or change and what range of doubt exists. This paper discusses good practice for including uncertainty information in CDRs for the essential climate variables (ECVs) derived from satellite data. Recommendations emerge from the shared experience of diverse ECV projects within the European Space Agency Climate Change Initiative.
Cristen Adams, Adam E. Bourassa, Chris A. McLinden, Chris E. Sioris, Thomas von Clarmann, Bernd Funke, Landon A. Rieger, and Douglas A. Degenstein
Atmos. Chem. Phys., 17, 8063–8080, https://doi.org/10.5194/acp-17-8063-2017, https://doi.org/10.5194/acp-17-8063-2017, 2017
Short summary
Short summary
We measured the relationship between volcanic aerosol and trace gases in the stratosphere using the OSIRIS and MIPAS satellite instruments between 2002 and 2014. We found that levels of stratospheric NO2 and N2O5 both decreased significantly in the presence of volcanic aerosol. These decreases were consistent with the modeling results.
Katja Matthes, Bernd Funke, Monika E. Andersson, Luke Barnard, Jürg Beer, Paul Charbonneau, Mark A. Clilverd, Thierry Dudok de Wit, Margit Haberreiter, Aaron Hendry, Charles H. Jackman, Matthieu Kretzschmar, Tim Kruschke, Markus Kunze, Ulrike Langematz, Daniel R. Marsh, Amanda C. Maycock, Stergios Misios, Craig J. Rodger, Adam A. Scaife, Annika Seppälä, Ming Shangguan, Miriam Sinnhuber, Kleareti Tourpali, Ilya Usoskin, Max van de Kamp, Pekka T. Verronen, and Stefan Versick
Geosci. Model Dev., 10, 2247–2302, https://doi.org/10.5194/gmd-10-2247-2017, https://doi.org/10.5194/gmd-10-2247-2017, 2017
Short summary
Short summary
The solar forcing dataset for climate model experiments performed for the upcoming IPCC report is described. This dataset provides the radiative and particle input of solar variability on a daily basis from 1850 through to 2300. With this dataset a better representation of natural climate variability with respect to the output of the Sun is provided which provides the most sophisticated and comprehensive respresentation of solar variability that has been used in climate model simulations so far.
Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Bianca Maria Dinelli, Anu Dudhia, Piera Raspollini, Norbert Glatthor, Udo Grabowski, Viktoria Sofieva, Lucien Froidevaux, Kaley A. Walker, and Claus Zehner
Atmos. Meas. Tech., 10, 1511–1518, https://doi.org/10.5194/amt-10-1511-2017, https://doi.org/10.5194/amt-10-1511-2017, 2017
Short summary
Short summary
A MIPAS instrument was flown in 2002–2012 on the Envisat satellite and measured atmospheric composition. There exist four processors retrieving atmospheric profiles from MIPAS spectra. We performed a mathematically clean merging of 2007–2008 datasets of ozone from these four processors. The merged product was compared with ozone datasets from ACE-FTS and MLS instruments. The advantages and the shortcomings of this merged product are discussed.
Christopher E. Sioris, Landon A. Rieger, Nicholas D. Lloyd, Adam E. Bourassa, Chris Z. Roth, Douglas A. Degenstein, Claude Camy-Peyret, Klaus Pfeilsticker, Gwenaël Berthet, Valéry Catoire, Florence Goutail, Jean-Pierre Pommereau, and Chris A. McLinden
Atmos. Meas. Tech., 10, 1155–1168, https://doi.org/10.5194/amt-10-1155-2017, https://doi.org/10.5194/amt-10-1155-2017, 2017
Short summary
Short summary
A new OSIRIS NO2 retrieval algorithm is described and validated using > 40 balloon-based profile measurements. The validation results indicate a slight improvement relative to the existing operational algorithm in terms of the bias versus the balloon data, particularly in the lower stratosphere. The implication is that this new algorithm should replace the operational one. The motivation was to combine spectral fitting and the SaskTRAN radiative transfer model to achieve an improved product.
Gwenaël Berthet, Fabrice Jégou, Valéry Catoire, Gisèle Krysztofiak, Jean-Baptiste Renard, Adam E. Bourassa, Doug A. Degenstein, Colette Brogniez, Marcel Dorf, Sebastian Kreycy, Klaus Pfeilsticker, Bodo Werner, Franck Lefèvre, Tjarda J. Roberts, Thibaut Lurton, Damien Vignelles, Nelson Bègue, Quentin Bourgeois, Daniel Daugeron, Michel Chartier, Claude Robert, Bertrand Gaubicher, and Christophe Guimbaud
Atmos. Chem. Phys., 17, 2229–2253, https://doi.org/10.5194/acp-17-2229-2017, https://doi.org/10.5194/acp-17-2229-2017, 2017
Short summary
Short summary
Since the last major volcanic event, i.e. the Pinatubo eruption in 1991, only
moderateeruptions have regularly injected sulfur into the stratosphere, typically enhancing the aerosol loading for several months. We investigate here for the first time the chemical perturbation associated with the Sarychev eruption in June 2009, using balloon-borne instruments and model calculations. Some chemical compounds are significantly affected by the aerosols, but the impact on stratospheric ozone is weak.
Sergey M. Khaykin, Sophie Godin-Beekmann, Philippe Keckhut, Alain Hauchecorne, Julien Jumelet, Jean-Paul Vernier, Adam Bourassa, Doug A. Degenstein, Landon A. Rieger, Christine Bingen, Filip Vanhellemont, Charles Robert, Matthew DeLand, and Pawan K. Bhartia
Atmos. Chem. Phys., 17, 1829–1845, https://doi.org/10.5194/acp-17-1829-2017, https://doi.org/10.5194/acp-17-1829-2017, 2017
Short summary
Short summary
The article is devoted to the long-term evolution and variability of stratospheric aerosol, which plays an important role in climate change and the ozone layer. We use 22-year long continuous observations using laser radar soundings in southern France and satellite-based observations to distinguish between natural aerosol variability (caused by volcanic eruptions) and human-induced change in aerosol concentration. An influence of growing pollution above Asia on stratospheric aerosol is found.
Masatomo Fujiwara, Jonathon S. Wright, Gloria L. Manney, Lesley J. Gray, James Anstey, Thomas Birner, Sean Davis, Edwin P. Gerber, V. Lynn Harvey, Michaela I. Hegglin, Cameron R. Homeyer, John A. Knox, Kirstin Krüger, Alyn Lambert, Craig S. Long, Patrick Martineau, Andrea Molod, Beatriz M. Monge-Sanz, Michelle L. Santee, Susann Tegtmeier, Simon Chabrillat, David G. H. Tan, David R. Jackson, Saroja Polavarapu, Gilbert P. Compo, Rossana Dragani, Wesley Ebisuzaki, Yayoi Harada, Chiaki Kobayashi, Will McCarty, Kazutoshi Onogi, Steven Pawson, Adrian Simmons, Krzysztof Wargan, Jeffrey S. Whitaker, and Cheng-Zhi Zou
Atmos. Chem. Phys., 17, 1417–1452, https://doi.org/10.5194/acp-17-1417-2017, https://doi.org/10.5194/acp-17-1417-2017, 2017
Short summary
Short summary
We introduce the SPARC Reanalysis Intercomparison Project (S-RIP), review key concepts and elements of atmospheric reanalysis systems, and summarize the technical details of and differences among 11 of these systems. This work supports scientific studies and intercomparisons of reanalysis products by collecting these background materials and technical details into a single reference. We also address several common misunderstandings and points of confusion regarding reanalyses.
Viktoria F. Sofieva, Iolanda Ialongo, Janne Hakkarainen, Erkki Kyrölä, Johanna Tamminen, Marko Laine, Daan Hubert, Alain Hauchecorne, Francis Dalaudier, Jean-Loup Bertaux, Didier Fussen, Laurent Blanot, Gilbert Barrot, and Angelika Dehn
Atmos. Meas. Tech., 10, 231–246, https://doi.org/10.5194/amt-10-231-2017, https://doi.org/10.5194/amt-10-231-2017, 2017
Short summary
Short summary
This paper presents a new ozone profile inversion algorithm for GOMOS/Envisat satellite data. This algorithm is enhanced with a DOAS-type method at visible wavelengths in the upper troposphere and the lower stratosphere. The new GOMOS ozone profiles have a significantly improved data quality in the UTLS compared to the official IPF V6 ozone profiles. The paper describes the inversion algorithm and present inter-comparisons with ozonesonde and satellite measurements.
Michael R. Giordano, Lars E. Kalnajs, Anita Avery, J. Douglas Goetz, Sean M. Davis, and Peter F. DeCarlo
Atmos. Chem. Phys., 17, 1–20, https://doi.org/10.5194/acp-17-1-2017, https://doi.org/10.5194/acp-17-1-2017, 2017
Short summary
Short summary
This paper summarizes two field measurements of particles and gases made in coastal Antarctica and represents the first real-time composition measurements of particles in this understudied area of the world. Using the combined data from both field measurements, we find that there is a constant background of particles in coastal Antarctica and that they are mostly sulfate. Seasonal transitions from winter to spring add additional particles, and that from spring to summer adds additional sulfate.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Chris A. McLinden, Peter F. Bernath, Adam E. Bourassa, John P. Burrows, Doug A. Degenstein, Bernd Funke, Didier Fussen, Gloria L. Manney, C. Thomas McElroy, Donal Murtagh, Cora E. Randall, Piera Raspollini, Alexei Rozanov, James M. Russell III, Makoto Suzuki, Masato Shiotani, Joachim Urban, Thomas von Clarmann, and Joseph M. Zawodny
Atmos. Meas. Tech., 9, 5781–5810, https://doi.org/10.5194/amt-9-5781-2016, https://doi.org/10.5194/amt-9-5781-2016, 2016
Short summary
Short summary
This study validates version 3.5 of the ACE-FTS NOy species data sets by comparing diurnally scaled ACE-FTS data to correlative data from 11 other satellite limb sounders. For all five species examined (NO, NO2, HNO3, N2O5, and ClONO2), there is good agreement between ACE-FTS and the other data sets in various regions of the atmosphere. In these validated regions, these NOy data products can be used for further investigation into the composition, dynamics, and climate of the stratosphere.
Sean M. Davis, Karen H. Rosenlof, Birgit Hassler, Dale F. Hurst, William G. Read, Holger Vömel, Henry Selkirk, Masatomo Fujiwara, and Robert Damadeo
Earth Syst. Sci. Data, 8, 461–490, https://doi.org/10.5194/essd-8-461-2016, https://doi.org/10.5194/essd-8-461-2016, 2016
Short summary
Short summary
This paper describes the construction of the Stratospheric Water and Ozone Satellite Homogenized (SWOOSH) database, whose main feature is a combined data product created by homogenizing multiple satellite records. This motivation for SWOOSH is that in order to study multiyear to decadal variability in ozone and water vapor concentrations, it is necessary to have a continuous and smooth record without artificial jumps in the data.
Filip Vanhellemont, Nina Mateshvili, Laurent Blanot, Charles Étienne Robert, Christine Bingen, Viktoria Sofieva, Francis Dalaudier, Cédric Tétard, Didier Fussen, Emmanuel Dekemper, Erkki Kyrölä, Marko Laine, Johanna Tamminen, and Claus Zehner
Atmos. Meas. Tech., 9, 4687–4700, https://doi.org/10.5194/amt-9-4687-2016, https://doi.org/10.5194/amt-9-4687-2016, 2016
Short summary
Short summary
The GOMOS instrument on Envisat has delivered a valuable aerosol extinction data set for the Earth's upper troposphere and stratosphere, from 2002 to 2012. However, at many optical wavelengths, data quality was not optimal. This article describes the AerGOM retrieval algorithm that was built to solve the problem and presents a first look at the reprocessed GOMOS data, clearly demonstrating the improvement. Multi-wavelength studies of atmospheric aerosol–cloud properties will now be possible.
Tamás Kovács, John M. C. Plane, Wuhu Feng, Tibor Nagy, Martyn P. Chipperfield, Pekka T. Verronen, Monika E. Andersson, David A. Newnham, Mark A. Clilverd, and Daniel R. Marsh
Geosci. Model Dev., 9, 3123–3136, https://doi.org/10.5194/gmd-9-3123-2016, https://doi.org/10.5194/gmd-9-3123-2016, 2016
Short summary
Short summary
This study was completed on D-region atmospheric model development. The sophisticated 3-D Whole Atmosphere Community Climate Model (WACCM) and the 1-D Sodynkalä Ion and Neutral Chemistry Model (SIC) were combined in order to provide a detailed, accurate model (WACCM-SIC) that considers the processes taking place in solar proton events. The original SIC model was reduced by mechanism reduction, which provided an accurate sub-mechanism (rSIC, WACCM-rSIC) of the original model.
Dale F. Hurst, William G. Read, Holger Vömel, Henry B. Selkirk, Karen H. Rosenlof, Sean M. Davis, Emrys G. Hall, Allen F. Jordan, and Samuel J. Oltmans
Atmos. Meas. Tech., 9, 4447–4457, https://doi.org/10.5194/amt-9-4447-2016, https://doi.org/10.5194/amt-9-4447-2016, 2016
Short summary
Short summary
This study compares stratospheric water vapor measurements by the Aura Microwave Limb Sounder (MLS) and balloon-borne frost point hygrometers (FPs) at five sites that launch two different types of FPs. The results demonstrate that FP and MLS measurements have been diverging at statistically significant rates of 0.6 to 1.5 % per year since approximately 2010. Similarities in the divergences at different sites suggest a positive drift in MLS retrievals since approximately 2010.
Cristen Adams, Elise N. Normand, Chris A. McLinden, Adam E. Bourassa, Nicholas D. Lloyd, Douglas A. Degenstein, Nickolay A. Krotkov, Maria Belmonte Rivas, K. Folkert Boersma, and Henk Eskes
Atmos. Meas. Tech., 9, 4103–4122, https://doi.org/10.5194/amt-9-4103-2016, https://doi.org/10.5194/amt-9-4103-2016, 2016
Short summary
Short summary
A new "OMI-minus-OSIRIS" (OmO) prototype dataset for tropospheric NO2 was created by combining information from the OMI satellite instrument, which is sensitive to NO2 in both the troposphere and stratosphere, with information from the OSIRIS satellite instrument, which measures NO2 in the stratosphere. This paper demonstrates that this approach is feasible and could be applied to future geostationary missions.
Nicholas A. Davis, Dian J. Seidel, Thomas Birner, Sean M. Davis, and Simone Tilmes
Atmos. Chem. Phys., 16, 10083–10095, https://doi.org/10.5194/acp-16-10083-2016, https://doi.org/10.5194/acp-16-10083-2016, 2016
Short summary
Short summary
In the Hadley cells, air rises at the Equator and sinks over the subtropics, drying the air and creating deserts on land. We investigated simple climate model experiments and found that the Hadley cells expand in response to increasing carbon dioxide. The climate of some models warms more than others, and these models also have greater Hadley cell expansion. This expansion could shift deserts toward more populated areas, with potentially major impacts on water resources and surface climate.
Daan Hubert, Jean-Christopher Lambert, Tijl Verhoelst, José Granville, Arno Keppens, Jean-Luc Baray, Adam E. Bourassa, Ugo Cortesi, Doug A. Degenstein, Lucien Froidevaux, Sophie Godin-Beekmann, Karl W. Hoppel, Bryan J. Johnson, Erkki Kyrölä, Thierry Leblanc, Günter Lichtenberg, Marion Marchand, C. Thomas McElroy, Donal Murtagh, Hideaki Nakane, Thierry Portafaix, Richard Querel, James M. Russell III, Jacobo Salvador, Herman G. J. Smit, Kerstin Stebel, Wolfgang Steinbrecht, Kevin B. Strawbridge, René Stübi, Daan P. J. Swart, Ghassan Taha, David W. Tarasick, Anne M. Thompson, Joachim Urban, Joanna A. E. van Gijsel, Roeland Van Malderen, Peter von der Gathen, Kaley A. Walker, Elian Wolfram, and Joseph M. Zawodny
Atmos. Meas. Tech., 9, 2497–2534, https://doi.org/10.5194/amt-9-2497-2016, https://doi.org/10.5194/amt-9-2497-2016, 2016
Short summary
Short summary
A more detailed understanding of satellite O3 profile data records is vital for further progress in O3 research. To this end, we made a comprehensive assessment of 14 limb/occultation profilers using ground-based reference data. The mutual consistency of satellite O3 in terms of bias, short-term variability and decadal stability is generally good over most of the stratosphere. However, we identified some exceptions that impact the quality of recently merged data sets and ozone trend assessments.
Niilo Kalakoski, Jukka Kujanpää, Viktoria Sofieva, Johanna Tamminen, Margherita Grossi, and Pieter Valks
Atmos. Meas. Tech., 9, 1533–1544, https://doi.org/10.5194/amt-9-1533-2016, https://doi.org/10.5194/amt-9-1533-2016, 2016
B. J. Elash, A. E. Bourassa, P. R. Loewen, N. D. Lloyd, and D. A. Degenstein
Atmos. Meas. Tech., 9, 1261–1277, https://doi.org/10.5194/amt-9-1261-2016, https://doi.org/10.5194/amt-9-1261-2016, 2016
A. Kauppi, O. N. E. Tuinder, S. Tukiainen, V. Sofieva, and J. Tamminen
Atmos. Meas. Tech., 9, 249–261, https://doi.org/10.5194/amt-9-249-2016, https://doi.org/10.5194/amt-9-249-2016, 2016
Short summary
Short summary
This paper presents a comparison of operational vertical ozone profiles retrieved by OPERA algorithm from the GOME-2 measurements on board Metop-A with space borne high-vertical-resolution ozone profiles by GOMOS, OSIRIS and MLS. The overall agreement of ozone profiles from GOME-2 and reference instruments is within 15 % below 35–40 km depending on latitude. The GOME-2 ozone profiles from non-degradation corrected radiances have a tendency to underestimate the ozone concentration above 30 km.
D. Pendlebury, D. Plummer, J. Scinocca, P. Sheese, K. Strong, K. Walker, and D. Degenstein
Atmos. Chem. Phys., 15, 12465–12485, https://doi.org/10.5194/acp-15-12465-2015, https://doi.org/10.5194/acp-15-12465-2015, 2015
Short summary
Short summary
The CMAM30 data set takes a chemistry-climate model and relaxes the dynamics to reanalysis, which can then provide chemistry fields not available from the reanalysis data set. This paper addresses this gap by comparing temperature, water vapour, ozone and methane to satellite data to determine and document any biases in the model fields. The lack of ozone destruction and dehydration in the SH polar vortex is shown to be due to the treatment of polar stratosphere clouds in the model.
F. Deng, D. B. A. Jones, T. W. Walker, M. Keller, K. W. Bowman, D. K. Henze, R. Nassar, E. A. Kort, S. C. Wofsy, K. A. Walker, A. E. Bourassa, and D. A. Degenstein
Atmos. Chem. Phys., 15, 11773–11788, https://doi.org/10.5194/acp-15-11773-2015, https://doi.org/10.5194/acp-15-11773-2015, 2015
Short summary
Short summary
The upper troposphere and lower stratosphere (UTLS) is characterized by strong gradients in the distribution of long-lived tracers, which are sensitive to discrepancies in transport in models. We found that our model overestimates CO2 in the polar UTLS through comparison of modeled CO2 with aircraft observations. We then corrected the modeled CO2 and quantified the impact of the correction on the flux estimates using an atmospheric model together with atmospheric CO2 measured from a satellite.
N. Rahpoe, M. Weber, A. V. Rozanov, K. Weigel, H. Bovensmann, J. P. Burrows, A. Laeng, G. Stiller, T. von Clarmann, E. Kyrölä, V. F. Sofieva, J. Tamminen, K. Walker, D. Degenstein, A. E. Bourassa, R. Hargreaves, P. Bernath, J. Urban, and D. P. Murtagh
Atmos. Meas. Tech., 8, 4369–4381, https://doi.org/10.5194/amt-8-4369-2015, https://doi.org/10.5194/amt-8-4369-2015, 2015
Short summary
Short summary
The analyses among six satellite instruments measuring ozone reveals that the relative drift between the sensors is not significant in the stratosphere and we conclude that merging of data from these instruments is possible. The merged ozone profiles can then be ingested in global climate models for long-term forecasts of ozone and climate change in the atmosphere. The added drift uncertainty is estimated at about 3% per decade (1 sigma) and should be applied in the calculation of ozone trends.
N. R. P. Harris, B. Hassler, F. Tummon, G. E. Bodeker, D. Hubert, I. Petropavlovskikh, W. Steinbrecht, J. Anderson, P. K. Bhartia, C. D. Boone, A. Bourassa, S. M. Davis, D. Degenstein, A. Delcloo, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, N. Jones, M. J. Kurylo, E. Kyrölä, M. Laine, S. T. Leblanc, J.-C. Lambert, B. Liley, E. Mahieu, A. Maycock, M. de Mazière, A. Parrish, R. Querel, K. H. Rosenlof, C. Roth, C. Sioris, J. Staehelin, R. S. Stolarski, R. Stübi, J. Tamminen, C. Vigouroux, K. A. Walker, H. J. Wang, J. Wild, and J. M. Zawodny
Atmos. Chem. Phys., 15, 9965–9982, https://doi.org/10.5194/acp-15-9965-2015, https://doi.org/10.5194/acp-15-9965-2015, 2015
Short summary
Short summary
Trends in the vertical distribution of ozone are reported for new and recently revised data sets. The amount of ozone-depleting compounds in the stratosphere peaked in the second half of the 1990s. We examine the trends before and after that peak to see if any change in trend is discernible. The previously reported decreases are confirmed. Furthermore, the downward trend in upper stratospheric ozone has not continued. The possible significance of any increase is discussed in detail.
D. J. Zawada, S. R. Dueck, L. A. Rieger, A. E. Bourassa, N. D. Lloyd, and D. A. Degenstein
Atmos. Meas. Tech., 8, 2609–2623, https://doi.org/10.5194/amt-8-2609-2015, https://doi.org/10.5194/amt-8-2609-2015, 2015
P. T. Verronen, M. E. Andersson, A. Kero, C.-F. Enell, J. M. Wissing, E. R. Talaat, K. Kauristie, M. Palmroth, T. E. Sarris, and E. Armandillo
Ann. Geophys., 33, 381–394, https://doi.org/10.5194/angeo-33-381-2015, https://doi.org/10.5194/angeo-33-381-2015, 2015
Short summary
Short summary
Electron concentrations observed by EISCAT radars can be reasonable well represented using AIMOS v1.2 satellite-data-based ionization model and SIC D-region ion chemistry model. SIC-EISCAT difference varies from event to event, probably because the statistical nature of AIMOS ionization is not capturing all the spatio-temporal fine structure of electron precipitation. Below 90km, AIMOS overestimates electron ionization because of proton contamination of the satellite electron detectors.
F. Tummon, B. Hassler, N. R. P. Harris, J. Staehelin, W. Steinbrecht, J. Anderson, G. E. Bodeker, A. Bourassa, S. M. Davis, D. Degenstein, S. M. Frith, L. Froidevaux, E. Kyrölä, M. Laine, C. Long, A. A. Penckwitt, C. E. Sioris, K. H. Rosenlof, C. Roth, H.-J. Wang, and J. Wild
Atmos. Chem. Phys., 15, 3021–3043, https://doi.org/10.5194/acp-15-3021-2015, https://doi.org/10.5194/acp-15-3021-2015, 2015
Short summary
Short summary
Understanding ozone trends in the vertical is vital in terms of assessing the success of the Montreal Protocol. This paper compares and analyses the long-term trends in stratospheric ozone from seven new merged satellite data sets. The data sets largely agree well with each other, particularly for the negative trends seen in the early period 1984-1997. For the 1998-2011 period there is less agreement, but a clear shift from negative to mostly positive trends.
A. Laeng, U. Grabowski, T. von Clarmann, G. Stiller, N. Glatthor, M. Höpfner, S. Kellmann, M. Kiefer, A. Linden, S. Lossow, V. Sofieva, I. Petropavlovskikh, D. Hubert, T. Bathgate, P. Bernath, C. D. Boone, C. Clerbaux, P. Coheur, R. Damadeo, D. Degenstein, S. Frith, L. Froidevaux, J. Gille, K. Hoppel, M. McHugh, Y. Kasai, J. Lumpe, N. Rahpoe, G. Toon, T. Sano, M. Suzuki, J. Tamminen, J. Urban, K. Walker, M. Weber, and J. Zawodny
Atmos. Meas. Tech., 7, 3971–3987, https://doi.org/10.5194/amt-7-3971-2014, https://doi.org/10.5194/amt-7-3971-2014, 2014
D. W. Fahey, R.-S. Gao, O. Möhler, H. Saathoff, C. Schiller, V. Ebert, M. Krämer, T. Peter, N. Amarouche, L. M. Avallone, R. Bauer, Z. Bozóki, L. E. Christensen, S. M. Davis, G. Durry, C. Dyroff, R. L. Herman, S. Hunsmann, S. M. Khaykin, P. Mackrodt, J. Meyer, J. B. Smith, N. Spelten, R. F. Troy, H. Vömel, S. Wagner, and F. G. Wienhold
Atmos. Meas. Tech., 7, 3177–3213, https://doi.org/10.5194/amt-7-3177-2014, https://doi.org/10.5194/amt-7-3177-2014, 2014
V. F. Sofieva, J. Tamminen, E. Kyrölä, A. Laeng, T. von Clarmann, F. Dalaudier, A. Hauchecorne, J.-L. Bertaux, G. Barrot, L. Blanot, D. Fussen, and F. Vanhellemont
Atmos. Meas. Tech., 7, 2147–2158, https://doi.org/10.5194/amt-7-2147-2014, https://doi.org/10.5194/amt-7-2147-2014, 2014
A. E. Bourassa, D. A. Degenstein, W. J. Randel, J. M. Zawodny, E. Kyrölä, C. A. McLinden, C. E. Sioris, and C. Z. Roth
Atmos. Chem. Phys., 14, 6983–6994, https://doi.org/10.5194/acp-14-6983-2014, https://doi.org/10.5194/acp-14-6983-2014, 2014
V. F. Sofieva, N. Kalakoski, S.-M. Päivärinta, J. Tamminen, M. Laine, and L. Froidevaux
Atmos. Meas. Tech., 7, 1891–1900, https://doi.org/10.5194/amt-7-1891-2014, https://doi.org/10.5194/amt-7-1891-2014, 2014
V. Kan, V. F. Sofieva, and F. Dalaudier
Atmos. Meas. Tech., 7, 1861–1872, https://doi.org/10.5194/amt-7-1861-2014, https://doi.org/10.5194/amt-7-1861-2014, 2014
B. Hassler, I. Petropavlovskikh, J. Staehelin, T. August, P. K. Bhartia, C. Clerbaux, D. Degenstein, M. De Mazière, B. M. Dinelli, A. Dudhia, G. Dufour, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, J. Granville, N. R. P. Harris, K. Hoppel, D. Hubert, Y. Kasai, M. J. Kurylo, E. Kyrölä, J.-C. Lambert, P. F. Levelt, C. T. McElroy, R. D. McPeters, R. Munro, H. Nakajima, A. Parrish, P. Raspollini, E. E. Remsberg, K. H. Rosenlof, A. Rozanov, T. Sano, Y. Sasano, M. Shiotani, H. G. J. Smit, G. Stiller, J. Tamminen, D. W. Tarasick, J. Urban, R. J. van der A, J. P. Veefkind, C. Vigouroux, T. von Clarmann, C. von Savigny, K. A. Walker, M. Weber, J. Wild, and J. M. Zawodny
Atmos. Meas. Tech., 7, 1395–1427, https://doi.org/10.5194/amt-7-1395-2014, https://doi.org/10.5194/amt-7-1395-2014, 2014
C. E. Sioris, C. A. McLinden, V. E. Fioletov, C. Adams, J. M. Zawodny, A. E. Bourassa, C. Z. Roth, and D. A. Degenstein
Atmos. Chem. Phys., 14, 3479–3496, https://doi.org/10.5194/acp-14-3479-2014, https://doi.org/10.5194/acp-14-3479-2014, 2014
L. A. Rieger, A. E. Bourassa, and D. A. Degenstein
Atmos. Meas. Tech., 7, 777–780, https://doi.org/10.5194/amt-7-777-2014, https://doi.org/10.5194/amt-7-777-2014, 2014
E. Eckert, T. von Clarmann, M. Kiefer, G. P. Stiller, S. Lossow, N. Glatthor, D. A. Degenstein, L. Froidevaux, S. Godin-Beekmann, T. Leblanc, S. McDermid, M. Pastel, W. Steinbrecht, D. P. J. Swart, K. A. Walker, and P. F. Bernath
Atmos. Chem. Phys., 14, 2571–2589, https://doi.org/10.5194/acp-14-2571-2014, https://doi.org/10.5194/acp-14-2571-2014, 2014
L. A. Rieger, A. E. Bourassa, and D. A. Degenstein
Atmos. Meas. Tech., 7, 507–522, https://doi.org/10.5194/amt-7-507-2014, https://doi.org/10.5194/amt-7-507-2014, 2014
C. Gebhardt, A. Rozanov, R. Hommel, M. Weber, H. Bovensmann, J. P. Burrows, D. Degenstein, L. Froidevaux, and A. M. Thompson
Atmos. Chem. Phys., 14, 831–846, https://doi.org/10.5194/acp-14-831-2014, https://doi.org/10.5194/acp-14-831-2014, 2014
V. F. Sofieva, J. Tamminen, E. Kyrölä, T. Mielonen, P. Veefkind, B. Hassler, and G.E. Bodeker
Atmos. Chem. Phys., 14, 283–299, https://doi.org/10.5194/acp-14-283-2014, https://doi.org/10.5194/acp-14-283-2014, 2014
C. Adams, A. E. Bourassa, V. Sofieva, L. Froidevaux, C. A. McLinden, D. Hubert, J.-C. Lambert, C. E. Sioris, and D. A. Degenstein
Atmos. Meas. Tech., 7, 49–64, https://doi.org/10.5194/amt-7-49-2014, https://doi.org/10.5194/amt-7-49-2014, 2014
E. N. Normand, J. T. Wiensz, A. E. Bourassa, and D. A. Degenstein
Atmos. Meas. Tech., 6, 3359–3368, https://doi.org/10.5194/amt-6-3359-2013, https://doi.org/10.5194/amt-6-3359-2013, 2013
V. F. Sofieva, N. Rahpoe, J. Tamminen, E. Kyrölä, N. Kalakoski, M. Weber, A. Rozanov, C. von Savigny, A. Laeng, T. von Clarmann, G. Stiller, S. Lossow, D. Degenstein, A. Bourassa, C. Adams, C. Roth, N. Lloyd, P. Bernath, R. J. Hargreaves, J. Urban, D. Murtagh, A. Hauchecorne, F. Dalaudier, M. van Roozendael, N. Kalb, and C. Zehner
Earth Syst. Sci. Data, 5, 349–363, https://doi.org/10.5194/essd-5-349-2013, https://doi.org/10.5194/essd-5-349-2013, 2013
E. Kyrölä, M. Laine, V. Sofieva, J. Tamminen, S.-M. Päivärinta, S. Tukiainen, J. Zawodny, and L. Thomason
Atmos. Chem. Phys., 13, 10645–10658, https://doi.org/10.5194/acp-13-10645-2013, https://doi.org/10.5194/acp-13-10645-2013, 2013
C. Tétard, D. Fussen, F. Vanhellemont, C. Bingen, E. Dekemper, N. Mateshvili, D. Pieroux, C. Robert, E. Kyrölä, J. Tamminen, V. Sofieva, A. Hauchecorne, F. Dalaudier, J.-L. Bertaux, O. Fanton d'Andon, G. Barrot, L. Blanot, A. Dehn, and L. Saavedra de Miguel
Atmos. Meas. Tech., 6, 2953–2964, https://doi.org/10.5194/amt-6-2953-2013, https://doi.org/10.5194/amt-6-2953-2013, 2013
A. Wiacek, R. V. Martin, A. E. Bourassa, N. D. Lloyd, and D. A. Degenstein
Atmos. Meas. Tech., 6, 2761–2776, https://doi.org/10.5194/amt-6-2761-2013, https://doi.org/10.5194/amt-6-2761-2013, 2013
C. Adams, A. E. Bourassa, A. F. Bathgate, C. A. McLinden, N. D. Lloyd, C. Z. Roth, E. J. Llewellyn, J. M. Zawodny, D. E. Flittner, G. L. Manney, W. H. Daffer, and D. A. Degenstein
Atmos. Meas. Tech., 6, 1447–1459, https://doi.org/10.5194/amt-6-1447-2013, https://doi.org/10.5194/amt-6-1447-2013, 2013
J. T. Wiensz, D. A. Degenstein, N. D. Lloyd, and A. E. Bourassa
Atmos. Meas. Tech., 6, 105–119, https://doi.org/10.5194/amt-6-105-2013, https://doi.org/10.5194/amt-6-105-2013, 2013
C. Adams, K. Strong, X. Zhao, A. E. Bourassa, W. H. Daffer, D. Degenstein, J. R. Drummond, E. E. Farahani, A. Fraser, N. D. Lloyd, G. L. Manney, C. A. McLinden, M. Rex, C. Roth, S. E. Strahan, K. A. Walker, and I. Wohltmann
Atmos. Chem. Phys., 13, 611–624, https://doi.org/10.5194/acp-13-611-2013, https://doi.org/10.5194/acp-13-611-2013, 2013
Related subject area
Subject: Gases | Research Activity: Remote Sensing | Altitude Range: Stratosphere | Science Focus: Physics (physical properties and processes)
Total ozone trends at three northern high-latitude stations
Case study on the influence of synoptic-scale processes on the paired H2O–O3 distribution in the UTLS across a North Atlantic jet stream
Dynamical linear modeling estimates of long-term ozone trends from homogenized Dobson Umkehr profiles at Arosa/Davos, Switzerland
Zonally asymmetric influences of the quasi-biennial oscillation on stratospheric ozone
Stratospheric ozone trends for 1984–2021 in the SAGE II–OSIRIS–SAGE III/ISS composite dataset
Analyzing ozone variations and uncertainties at high latitudes during sudden stratospheric warming events using MERRA-2
Impacts of tropical cyclones on the thermodynamic conditions in the tropical tropopause layer observed by A-Train satellites
Investigation and amelioration of long-term instrumental drifts in water vapor and nitrous oxide measurements from the Aura Microwave Limb Sounder (MLS) and their implications for studies of variability and trends
3-D tomographic observations of Rossby wave breaking over the North Atlantic during the WISE aircraft campaign in 2017
Is there a direct solar proton impact on lower-stratospheric ozone?
Small-scale variability of stratospheric ozone during the sudden stratospheric warming 2018/2019 observed at Ny-Ålesund, Svalbard
Evidence for energetic particle precipitation and quasi-biennial oscillation modulations of the Antarctic NO2 springtime stratospheric column from OMI observations
Stratospheric ozone trends for 1985–2018: sensitivity to recent large variability
Interannual variations of water vapor in the tropical upper troposphere and the lower and middle stratosphere and their connections to ENSO and QBO
Ground-based ozone profiles over central Europe: incorporating anomalous observations into the analysis of stratospheric ozone trends
Response of stratospheric water vapor and ozone to the unusual timing of El Niño and the QBO disruption in 2015–2016
Assessing stratospheric transport in the CMAM30 simulations using ACE-FTS measurements
Water vapour and methane coupling in the stratosphere observed using SCIAMACHY solar occultation measurements
Evidence for a continuous decline in lower stratospheric ozone offsetting ozone layer recovery
MLS measurements of stratospheric hydrogen cyanide during the 2015–2016 El Niño event
What controls the seasonal cycle of columnar methane observed by GOSAT over different regions in India?
An “island” in the stratosphere – on the enhanced annual variation of water vapour in the middle and upper stratosphere in the southern tropics and subtropics
CCl4 distribution derived from MIPAS ESA v7 data: intercomparisons, trend, and lifetime estimation
Results from the validation campaign of the ozone radiometer GROMOS-C at the NDACC station of Réunion island
Trend analysis of the 20-year time series of stratospheric ozone profiles observed by the GROMOS microwave radiometer at Bern
Is there a solar signal in lower stratospheric water vapour?
Trajectory mapping of middle atmospheric water vapor by a mini network of NDACC instruments
Sunset–sunrise difference in solar occultation ozone measurements (SAGE II, HALOE, and ACE–FTS) and its relationship to tidal vertical winds
Tracing the second stage of ozone recovery in the Antarctic ozone-hole with a "big data" approach to multivariate regressions
Total ozone trends and variability during 1979–2012 from merged data sets of various satellites
Trends in stratospheric ozone derived from merged SAGE II and Odin-OSIRIS satellite observations
Evaluation of the use of five laboratory-determined ozone absorption cross sections in Brewer and Dobson retrieval algorithms
Decadal-scale responses in middle and upper stratospheric ozone from SAGE II version 7 data
Validation of ozone monthly zonal mean profiles obtained from the version 8.6 Solar Backscatter Ultraviolet algorithm
Stratospheric lifetimes of CFC-12, CCl4, CH4, CH3Cl and N2O from measurements made by the Atmospheric Chemistry Experiment-Fourier Transform Spectrometer (ACE-FTS)
Volcanic SO2 fluxes derived from satellite data: a survey using OMI, GOME-2, IASI and MODIS
Stratospheric ozone interannual variability (1995–2011) as observed by lidar and satellite at Mauna Loa Observatory, HI and Table Mountain Facility, CA
Chemical ozone losses in Arctic and Antarctic polar winter/spring season derived from SCIAMACHY limb measurements 2002–2009
Development of a climate record of tropospheric and stratospheric column ozone from satellite remote sensing: evidence of an early recovery of global stratospheric ozone
A-train CALIOP and MLS observations of early winter Antarctic polar stratospheric clouds and nitric acid in 2008
Ozone zonal asymmetry and planetary wave characterization during Antarctic spring
A global climatology of tropospheric and stratospheric ozone derived from Aura OMI and MLS measurements
Sulphur dioxide as a volcanic ash proxy during the April–May 2010 eruption of Eyjafjallajökull Volcano, Iceland
Analysis of HCl and ClO time series in the upper stratosphere using satellite data sets
Retrieval of atmospheric parameters from GOMOS data
Multi sensor reanalysis of total ozone
GOMOS data characterisation and error estimation
Technical Note: Time-dependent limb-darkening calibration for solar occultation instruments
Simultaneous measurements of OClO, NO2 and O3 in the Arctic polar vortex by the GOMOS instrument
Leonie Bernet, Tove Svendby, Georg Hansen, Yvan Orsolini, Arne Dahlback, Florence Goutail, Andrea Pazmiño, Boyan Petkov, and Arve Kylling
Atmos. Chem. Phys., 23, 4165–4184, https://doi.org/10.5194/acp-23-4165-2023, https://doi.org/10.5194/acp-23-4165-2023, 2023
Short summary
Short summary
After the severe destruction of the ozone layer, the amount of ozone in the stratosphere is expected to increase again. At northern high latitudes, however, such a recovery has not been detected yet. To assess ozone changes in that region, we analyse the amount of ozone above specific locations (total ozone) measured at three stations in Norway. We found that total ozone increases significantly at two Arctic stations, which may be an indication of ozone recovery at northern high latitudes.
Andreas Schäfler, Michael Sprenger, Heini Wernli, Andreas Fix, and Martin Wirth
Atmos. Chem. Phys., 23, 999–1018, https://doi.org/10.5194/acp-23-999-2023, https://doi.org/10.5194/acp-23-999-2023, 2023
Short summary
Short summary
In this study, airborne lidar profile measurements of H2O and O3 across a midlatitude jet stream are combined with analyses in tracer–trace space and backward trajectories. We highlight that transport and mixing processes in the history of the observed air masses are governed by interacting tropospheric weather systems on synoptic timescales. We show that these weather systems play a key role in the high variability of the paired H2O and O3 distributions near the tropopause.
Eliane Maillard Barras, Alexander Haefele, René Stübi, Achille Jouberton, Herbert Schill, Irina Petropavlovskikh, Koji Miyagawa, Martin Stanek, and Lucien Froidevaux
Atmos. Chem. Phys., 22, 14283–14302, https://doi.org/10.5194/acp-22-14283-2022, https://doi.org/10.5194/acp-22-14283-2022, 2022
Short summary
Short summary
Intercomparisons of three Dobson and three Brewer spectrophotometers at Arosa/Davos, Switzerland, are used for the homogenization of the longest Umkehr ozone profiles time series worldwide. Dynamic linear modeling (DLM) reveals a significant positive trend after 2004 in the upper stratosphere, a persistent negative trend between 25 and 30 km in the middle stratosphere, and a negative trend at 20 km in the lower stratosphere, with different levels of significance depending on the dataset.
Wuke Wang, Jin Hong, Ming Shangguan, Hongyue Wang, Wei Jiang, and Shuyun Zhao
Atmos. Chem. Phys., 22, 13695–13711, https://doi.org/10.5194/acp-22-13695-2022, https://doi.org/10.5194/acp-22-13695-2022, 2022
Short summary
Short summary
The ozone layer protects the life on the Earth by absorbing the ultraviolet (UV) radiation. Beside the long-term trend, there are strong interannual fluctuations in stratospheric ozone. The quasi-biennial oscillation (QBO) is an important interannual mode in the stratosphere. We show some new zonally asymmetric features of its impacts on stratospheric ozone using satellite data, ERA5 reanalysis, and model simulations, which is helpful for predicting the regional UV radiation at the surface.
Kristof Bognar, Susann Tegtmeier, Adam Bourassa, Chris Roth, Taran Warnock, Daniel Zawada, and Doug Degenstein
Atmos. Chem. Phys., 22, 9553–9569, https://doi.org/10.5194/acp-22-9553-2022, https://doi.org/10.5194/acp-22-9553-2022, 2022
Short summary
Short summary
We quantify recent changes in stratospheric ozone (outside the polar regions) using a combination of three satellite datasets. We find that upper stratospheric ozone have increased significantly since 2000, although the recovery shows an unexpected pause in the Northern Hemisphere. Combined with the likely decrease in ozone in the lower stratosphere, this presents an interesting challenge for predicting the future of the ozone layer.
Shima Bahramvash Shams, Von P. Walden, James W. Hannigan, William J. Randel, Irina V. Petropavlovskikh, Amy H. Butler, and Alvaro de la Cámara
Atmos. Chem. Phys., 22, 5435–5458, https://doi.org/10.5194/acp-22-5435-2022, https://doi.org/10.5194/acp-22-5435-2022, 2022
Short summary
Short summary
Large-scale atmospheric circulation has a strong influence on ozone in the Arctic, and certain anomalous dynamical events, such as sudden stratospheric warmings, cause dramatic alterations of the large-scale circulation. A reanalysis model is evaluated and then used to investigate the impact of sudden stratospheric warmings on mid-atmospheric ozone. Results show that the position of the cold jet stream over the Arctic before these events influences the variability of ozone.
Jing Feng and Yi Huang
Atmos. Chem. Phys., 21, 15493–15518, https://doi.org/10.5194/acp-21-15493-2021, https://doi.org/10.5194/acp-21-15493-2021, 2021
Short summary
Short summary
This study conducts a comprehensive analysis of thermodynamic fields above tropical cyclones. Using a synergistic retrieval method, we develop the first infrared hyperspectra-based dataset of collocated temperature and water vapor profiles above deep convective clouds. It discloses the unique impacts of convective overshoots on the tropical tropopause layer (TTL). Challenging conventional views, our study suggests that convective hydration may be limited by the radiative balance above cyclones.
Nathaniel J. Livesey, William G. Read, Lucien Froidevaux, Alyn Lambert, Michelle L. Santee, Michael J. Schwartz, Luis F. Millán, Robert F. Jarnot, Paul A. Wagner, Dale F. Hurst, Kaley A. Walker, Patrick E. Sheese, and Gerald E. Nedoluha
Atmos. Chem. Phys., 21, 15409–15430, https://doi.org/10.5194/acp-21-15409-2021, https://doi.org/10.5194/acp-21-15409-2021, 2021
Short summary
Short summary
The Microwave Limb Sounder (MLS), an instrument on NASA's Aura mission launched in 2004, measures vertical profiles of the temperature and composition of Earth's "middle atmosphere" (the region from ~12 to ~100 km altitude). We describe how, among the 16 trace gases measured by MLS, the measurements of water vapor (H2O) and nitrous oxide (N2O) have started to drift since ~2010. The paper also discusses the origins of this drift and work to ameliorate it in a new version of the MLS dataset.
Lukas Krasauskas, Jörn Ungermann, Peter Preusse, Felix Friedl-Vallon, Andreas Zahn, Helmut Ziereis, Christian Rolf, Felix Plöger, Paul Konopka, Bärbel Vogel, and Martin Riese
Atmos. Chem. Phys., 21, 10249–10272, https://doi.org/10.5194/acp-21-10249-2021, https://doi.org/10.5194/acp-21-10249-2021, 2021
Short summary
Short summary
A Rossby wave (RW) breaking event was observed over the North Atlantic during the WISE measurement campaign in October 2017. Infrared limb sounding measurements of trace gases in the lower stratosphere, including high-resolution 3-D tomographic reconstruction, revealed complex spatial structures in stratospheric tracers near the polar jet related to previous RW breaking events. Backward-trajectory analysis and tracer correlations were used to study mixing and stratosphere–troposphere exchange.
Jia Jia, Antti Kero, Niilo Kalakoski, Monika E. Szeląg, and Pekka T. Verronen
Atmos. Chem. Phys., 20, 14969–14982, https://doi.org/10.5194/acp-20-14969-2020, https://doi.org/10.5194/acp-20-14969-2020, 2020
Short summary
Short summary
Recent studies have reported up to a 10 % average decrease of lower stratospheric ozone at 20 km altitude following solar proton events (SPEs). Our study uses 49 events that occurred after the launch of Aura MLS (July 2004–now) and 177 events that occurred in the WACCM-D simulation period (Jan 1989–Dec 2012) to evaluate ozone changes following SPEs. The statistical and case-by-case studies show no solid evidence of SPE's direct impact on the lower stratospheric ozone.
Franziska Schranz, Jonas Hagen, Gunter Stober, Klemens Hocke, Axel Murk, and Niklaus Kämpfer
Atmos. Chem. Phys., 20, 10791–10806, https://doi.org/10.5194/acp-20-10791-2020, https://doi.org/10.5194/acp-20-10791-2020, 2020
Short summary
Short summary
We measured middle-atmospheric ozone, water vapour and zonal and meridional wind with two ground-based microwave radiometers which are located at Ny-Alesund, Svalbard, in the Arctic. In this article we present measurements of the small-scale horizontal ozone gradients during winter 2018/2019. We found a distinct seasonal variation of the ozone gradients which is linked to the planetary wave activity. We further present the signatures of the SSW in the ozone, water vapour and wind measurements.
Emily M. Gordon, Annika Seppälä, and Johanna Tamminen
Atmos. Chem. Phys., 20, 6259–6271, https://doi.org/10.5194/acp-20-6259-2020, https://doi.org/10.5194/acp-20-6259-2020, 2020
Short summary
Short summary
The Sun constantly emits high-energy charged particles that produce the ozone destroying chemical NOx in the polar atmosphere. NOx is transported to the stratosphere, where the ozone layer is. Satellite observations show that the NOx gases remain in the atmosphere longer than previously reported. This is influenced by the strength of atmospheric large-scale dynamics, suggesting that there are specific times when this type of solar influence on the Antarctic atmosphere becomes more pronounced.
William T. Ball, Justin Alsing, Johannes Staehelin, Sean M. Davis, Lucien Froidevaux, and Thomas Peter
Atmos. Chem. Phys., 19, 12731–12748, https://doi.org/10.5194/acp-19-12731-2019, https://doi.org/10.5194/acp-19-12731-2019, 2019
Short summary
Short summary
We analyse long-term stratospheric ozone (60° S–60° N) trends over the 1985–2018 period. Previous work has suggested that lower stratosphere ozone declined over 1998–2016. We demonstrate that a large ozone upsurge in 2017 is likely related to QBO variability, but that lower stratospheric ozone trends likely remain lower in 2018 than in 1998. Tropical stratospheric ozone (30° S–30° N) shows highly probable decreases in both the lower stratosphere and in the integrated stratospheric ozone layer.
Edward W. Tian, Hui Su, Baijun Tian, and Jonathan H. Jiang
Atmos. Chem. Phys., 19, 9913–9926, https://doi.org/10.5194/acp-19-9913-2019, https://doi.org/10.5194/acp-19-9913-2019, 2019
Short summary
Short summary
We study the interannual (2–7-year) water vapor variations in the tropical upper troposphere and the lower and middle stratosphere and their connections to El Nino–Southern Oscillation (ENSO) and quasi-biennial oscillation (QBO) using the Aura Microwave Limb Sounder (MLS) data and time-lag regression analysis and composite analysis. We found that ENSO is more important in the upper troposphere and near the tropopause, while QBO is more important in the lower and middle stratosphere.
Leonie Bernet, Thomas von Clarmann, Sophie Godin-Beekmann, Gérard Ancellet, Eliane Maillard Barras, René Stübi, Wolfgang Steinbrecht, Niklaus Kämpfer, and Klemens Hocke
Atmos. Chem. Phys., 19, 4289–4309, https://doi.org/10.5194/acp-19-4289-2019, https://doi.org/10.5194/acp-19-4289-2019, 2019
Short summary
Short summary
After severe ozone depletion, upper stratospheric ozone has started to recover in recent years. However, stratospheric ozone trends from various data sets still show differences. To partly explain such differences, we investigate how the trends are affected by different factors, for example, anomalies in the data. We show how trend estimates can be improved by considering such anomalies and present updated stratospheric ozone trends from ground data measured in central Europe.
Mohamadou Diallo, Martin Riese, Thomas Birner, Paul Konopka, Rolf Müller, Michaela I. Hegglin, Michelle L. Santee, Mark Baldwin, Bernard Legras, and Felix Ploeger
Atmos. Chem. Phys., 18, 13055–13073, https://doi.org/10.5194/acp-18-13055-2018, https://doi.org/10.5194/acp-18-13055-2018, 2018
Short summary
Short summary
The unprecedented timing of an El Niño event aligned with the disrupted QBO in 2015–2016 caused a perturbation to the stratospheric circulation, affecting trace gases. This paper resolves the puzzling response of the lower stratospheric water vapor by showing that the QBO disruption reversed the lower stratosphere moistening triggered by the alignment of the El Niño event with a westerly QBO in early boreal winter.
Felicia Kolonjari, David A. Plummer, Kaley A. Walker, Chris D. Boone, James W. Elkins, Michaela I. Hegglin, Gloria L. Manney, Fred L. Moore, Diane Pendlebury, Eric A. Ray, Karen H. Rosenlof, and Gabriele P. Stiller
Atmos. Chem. Phys., 18, 6801–6828, https://doi.org/10.5194/acp-18-6801-2018, https://doi.org/10.5194/acp-18-6801-2018, 2018
Short summary
Short summary
We used satellite observations and model simulations of CFC-11, CFC-12, and N2O to investigate stratospheric transport, which is important for predicting the recovery of the ozone layer and future climate. We found that sampling can impact results and that the model consistently overestimates concentrations of these gases in the lower stratosphere, consistent with a too rapid Brewer–Dobson circulation. An issue with mixing in the tropical lower stratosphere in June–July–August was also found.
Stefan Noël, Katja Weigel, Klaus Bramstedt, Alexei Rozanov, Mark Weber, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 18, 4463–4476, https://doi.org/10.5194/acp-18-4463-2018, https://doi.org/10.5194/acp-18-4463-2018, 2018
Short summary
Short summary
The combined analysis of stratospheric methane and water vapour data derived from SCIAMACHY solar occultation measurements shows the expected anti-correlation and a clear temporal variation related to waves in equatorial zonal winds. Above about 20 km most of the additional water vapour is attributed to the oxidation of methane. The SCIAMACHY data confirm that at lower altitudes water vapour and methane are transported from the tropics to higher latitudes.
William T. Ball, Justin Alsing, Daniel J. Mortlock, Johannes Staehelin, Joanna D. Haigh, Thomas Peter, Fiona Tummon, Rene Stübi, Andrea Stenke, John Anderson, Adam Bourassa, Sean M. Davis, Doug Degenstein, Stacey Frith, Lucien Froidevaux, Chris Roth, Viktoria Sofieva, Ray Wang, Jeannette Wild, Pengfei Yu, Jerald R. Ziemke, and Eugene V. Rozanov
Atmos. Chem. Phys., 18, 1379–1394, https://doi.org/10.5194/acp-18-1379-2018, https://doi.org/10.5194/acp-18-1379-2018, 2018
Short summary
Short summary
Using a robust analysis, with artefact-corrected ozone data, we confirm upper stratospheric ozone is recovering following the Montreal Protocol, but that lower stratospheric ozone (50° S–50° N) has continued to decrease since 1998, and the ozone layer as a whole (60° S–60° N) may be lower today than in 1998. No change in total column ozone may be due to increasing tropospheric ozone. State-of-the-art models do not reproduce lower stratospheric ozone decreases.
Hugh C. Pumphrey, Norbert Glatthor, Peter F. Bernath, Christopher D. Boone, James W. Hannigan, Ivan Ortega, Nathaniel J. Livesey, and William G. Read
Atmos. Chem. Phys., 18, 691–703, https://doi.org/10.5194/acp-18-691-2018, https://doi.org/10.5194/acp-18-691-2018, 2018
Short summary
Short summary
The Microwave Limb Sounder (MLS) is a satellite instrument that has been measuring the amount of various gases in the atmosphere since 2004. In late 2015 and 2016 it observed unusual amounts of hydrogen cyanide (HCN), a gas produced when vegetation is burned. We compare the MLS observations to similar observations from other instruments. The excess HCN is shown to come from fires in Indonesia. There are more fires than usual in 2015–16 due to a drought caused by an El Niño event.
Naveen Chandra, Sachiko Hayashida, Tazu Saeki, and Prabir K. Patra
Atmos. Chem. Phys., 17, 12633–12643, https://doi.org/10.5194/acp-17-12633-2017, https://doi.org/10.5194/acp-17-12633-2017, 2017
Short summary
Short summary
This study shows difficulties in interpreting columnar dry-air mole fractions of methane (XCH4) for surface emissions of CH4 over the South Asia region, without separating the role of chemistry and transport. Using a chemistry-transport model, we suggest that a link between surface emissions and higher levels of XCH4 is not always valid in this region of complex monsoonal meteorology, although there is often a fair correlation between the seasonal variations in surface emissions and XCH4.
Stefan Lossow, Hella Garny, and Patrick Jöckel
Atmos. Chem. Phys., 17, 11521–11539, https://doi.org/10.5194/acp-17-11521-2017, https://doi.org/10.5194/acp-17-11521-2017, 2017
Massimo Valeri, Flavio Barbara, Chris Boone, Simone Ceccherini, Marco Gai, Guido Maucher, Piera Raspollini, Marco Ridolfi, Luca Sgheri, Gerald Wetzel, and Nicola Zoppetti
Atmos. Chem. Phys., 17, 10143–10162, https://doi.org/10.5194/acp-17-10143-2017, https://doi.org/10.5194/acp-17-10143-2017, 2017
Short summary
Short summary
Atmospheric emissions of CCl4 are regulated by the Montreal Protocol due to its role as a strong ozone-depleting substance. The molecule is the subject of recent increased interest as a consequence of the discrepancy between atmospheric observations and reported production and consumption. We use MIPAS/ENVISAT data (2002–2012) to estimate CCl4 trends and lifetime. At 50 hPa we find a decline of about 30–35 % per decade. In the lower stratosphere our lifetime estimate is 47 (39–61) years.
Susana Fernandez, Rolf Rüfenacht, Niklaus Kämpfer, Thierry Portafaix, Françoise Posny, and Guillaume Payen
Atmos. Chem. Phys., 16, 7531–7543, https://doi.org/10.5194/acp-16-7531-2016, https://doi.org/10.5194/acp-16-7531-2016, 2016
Short summary
Short summary
We present a new ground based microwave radiometer for campaigns, GROMOS-C. It measures the vertical distribution of ozone in the middle atmosphere by observing spectra at 110.836 GHz. The paper presents a validation campaign that took place on La Réunion Island. The ozone retrieved profiles are validated against ozone profiles from the Microwave Limb Sounder, the ozone lidar located in the observatory, ozone profiles from weekly radiosondes and with ECMWF model data.
L. Moreira, K. Hocke, E. Eckert, T. von Clarmann, and N. Kämpfer
Atmos. Chem. Phys., 15, 10999–11009, https://doi.org/10.5194/acp-15-10999-2015, https://doi.org/10.5194/acp-15-10999-2015, 2015
Short summary
Short summary
GROMOS (GROund-based Millimeter-wave Ozone Spectrometer) has provided ozone profiles for the NDACC (Network for the Detection of Atmospheric Composition Change) at Bern since 1994. We performed a trend analysis of our 20-year time series of stratospheric ozone profiles with a multilinear parametric trend estimation method. With our estimated ozone trends we are able to support the stratospheric ozone turnaround, besides a statistically significant negative trend in the lower mesosphere.
T. Schieferdecker, S. Lossow, G. P. Stiller, and T. von Clarmann
Atmos. Chem. Phys., 15, 9851–9863, https://doi.org/10.5194/acp-15-9851-2015, https://doi.org/10.5194/acp-15-9851-2015, 2015
Short summary
Short summary
A merged data set of HALOE and MIPAS lower stratospheric water vapour has been constructed. Multivariate linear regression shows that the merged time series can best be explained if a proxy for the 11-year solar cycle is considered. The amplitude of the solar cycle signal in water vapour is slightly higher than that which can be explained by the known solar cycle variation of cold-point temperatures.
M. Lainer, N. Kämpfer, B. Tschanz, G. E. Nedoluha, S. Ka, and J. J. Oh
Atmos. Chem. Phys., 15, 9711–9730, https://doi.org/10.5194/acp-15-9711-2015, https://doi.org/10.5194/acp-15-9711-2015, 2015
Short summary
Short summary
We use water vapor profiles from ground-based microwave radiometers at five locations distributed over the Northern Hemisphere and operated in the frame of NDACC (Network for the Detection of Atmospheric Composition Change) to generate hemispheric water vapor maps based on the so-called trajectory mapping technique. The novelty is to show that a mini network of instruments is capable of providing information about the hemispheric distribution of water vapor under most conditions.
T. Sakazaki, M. Shiotani, M. Suzuki, D. Kinnison, J. M. Zawodny, M. McHugh, and K. A. Walker
Atmos. Chem. Phys., 15, 829–843, https://doi.org/10.5194/acp-15-829-2015, https://doi.org/10.5194/acp-15-829-2015, 2015
Short summary
Short summary
The solar occultation measurements measure the atmosphere at sunrise (SR) and sunset (SS). It has been reported that there is a significant difference in the observed amount of stratospheric ozone between SR and SS. This study first revealed that this difference can be largely explained by diurnal variations in ozone, particularly those caused by vertical transport by the atmospheric tidal winds. Our results would be helpful for the construction of combined data sets from SR and SS profiles.
A. T. J. de Laat, R. J. van der A, and M. van Weele
Atmos. Chem. Phys., 15, 79–97, https://doi.org/10.5194/acp-15-79-2015, https://doi.org/10.5194/acp-15-79-2015, 2015
Short summary
Short summary
Recent research suggests the Antarctic ozone hole has started to shrink due to decreasing ozone-depleting substances. Because it could be questioned how robust these results are, we provide an assessment of uncertainties in both the underlying ozone observational records and the detection-attribution method. Although Antarctic ozone concentrations are definitely increasing slowly, the formal identification of recovery is not yet justified, although this will likely become possible this decade.
W. Chehade, M. Weber, and J. P. Burrows
Atmos. Chem. Phys., 14, 7059–7074, https://doi.org/10.5194/acp-14-7059-2014, https://doi.org/10.5194/acp-14-7059-2014, 2014
A. E. Bourassa, D. A. Degenstein, W. J. Randel, J. M. Zawodny, E. Kyrölä, C. A. McLinden, C. E. Sioris, and C. Z. Roth
Atmos. Chem. Phys., 14, 6983–6994, https://doi.org/10.5194/acp-14-6983-2014, https://doi.org/10.5194/acp-14-6983-2014, 2014
A. Redondas, R. Evans, R. Stuebi, U. Köhler, and M. Weber
Atmos. Chem. Phys., 14, 1635–1648, https://doi.org/10.5194/acp-14-1635-2014, https://doi.org/10.5194/acp-14-1635-2014, 2014
E. E. Remsberg
Atmos. Chem. Phys., 14, 1039–1053, https://doi.org/10.5194/acp-14-1039-2014, https://doi.org/10.5194/acp-14-1039-2014, 2014
N. A. Kramarova, S. M. Frith, P. K. Bhartia, R. D. McPeters, S. L. Taylor, B. L. Fisher, G. J. Labow, and M. T. DeLand
Atmos. Chem. Phys., 13, 6887–6905, https://doi.org/10.5194/acp-13-6887-2013, https://doi.org/10.5194/acp-13-6887-2013, 2013
A. T. Brown, C. M. Volk, M. R. Schoeberl, C. D. Boone, and P. F. Bernath
Atmos. Chem. Phys., 13, 6921–6950, https://doi.org/10.5194/acp-13-6921-2013, https://doi.org/10.5194/acp-13-6921-2013, 2013
N. Theys, R. Campion, L. Clarisse, H. Brenot, J. van Gent, B. Dils, S. Corradini, L. Merucci, P.-F. Coheur, M. Van Roozendael, D. Hurtmans, C. Clerbaux, S. Tait, and F. Ferrucci
Atmos. Chem. Phys., 13, 5945–5968, https://doi.org/10.5194/acp-13-5945-2013, https://doi.org/10.5194/acp-13-5945-2013, 2013
G. Kirgis, T. Leblanc, I. S. McDermid, and T. D. Walsh
Atmos. Chem. Phys., 13, 5033–5047, https://doi.org/10.5194/acp-13-5033-2013, https://doi.org/10.5194/acp-13-5033-2013, 2013
T. Sonkaew, C. von Savigny, K.-U. Eichmann, M. Weber, A. Rozanov, H. Bovensmann, J. P. Burrows, and J.-U. Grooß
Atmos. Chem. Phys., 13, 1809–1835, https://doi.org/10.5194/acp-13-1809-2013, https://doi.org/10.5194/acp-13-1809-2013, 2013
J. R. Ziemke and S. Chandra
Atmos. Chem. Phys., 12, 5737–5753, https://doi.org/10.5194/acp-12-5737-2012, https://doi.org/10.5194/acp-12-5737-2012, 2012
A. Lambert, M. L. Santee, D. L. Wu, and J. H. Chae
Atmos. Chem. Phys., 12, 2899–2931, https://doi.org/10.5194/acp-12-2899-2012, https://doi.org/10.5194/acp-12-2899-2012, 2012
I. Ialongo, V. Sofieva, N. Kalakoski, J. Tamminen, and E. Kyrölä
Atmos. Chem. Phys., 12, 2603–2614, https://doi.org/10.5194/acp-12-2603-2012, https://doi.org/10.5194/acp-12-2603-2012, 2012
J. R. Ziemke, S. Chandra, G. J. Labow, P. K. Bhartia, L. Froidevaux, and J. C. Witte
Atmos. Chem. Phys., 11, 9237–9251, https://doi.org/10.5194/acp-11-9237-2011, https://doi.org/10.5194/acp-11-9237-2011, 2011
H. E. Thomas and A. J. Prata
Atmos. Chem. Phys., 11, 6871–6880, https://doi.org/10.5194/acp-11-6871-2011, https://doi.org/10.5194/acp-11-6871-2011, 2011
A. Jones, J. Urban, D. P. Murtagh, C. Sanchez, K. A. Walker, N. J. Livesey, L. Froidevaux, and M. L. Santee
Atmos. Chem. Phys., 11, 5321–5333, https://doi.org/10.5194/acp-11-5321-2011, https://doi.org/10.5194/acp-11-5321-2011, 2011
E. Kyrölä, J. Tamminen, V. Sofieva, J. L. Bertaux, A. Hauchecorne, F. Dalaudier, D. Fussen, F. Vanhellemont, O. Fanton d'Andon, G. Barrot, M. Guirlet, A. Mangin, L. Blanot, T. Fehr, L. Saavedra de Miguel, and R. Fraisse
Atmos. Chem. Phys., 10, 11881–11903, https://doi.org/10.5194/acp-10-11881-2010, https://doi.org/10.5194/acp-10-11881-2010, 2010
R. J. van der A, M. A. F. Allaart, and H. J. Eskes
Atmos. Chem. Phys., 10, 11277–11294, https://doi.org/10.5194/acp-10-11277-2010, https://doi.org/10.5194/acp-10-11277-2010, 2010
J. Tamminen, E. Kyrölä, V. F. Sofieva, M. Laine, J.-L. Bertaux, A. Hauchecorne, F. Dalaudier, D. Fussen, F. Vanhellemont, O. Fanton-d'Andon, G. Barrot, A. Mangin, M. Guirlet, L. Blanot, T. Fehr, L. Saavedra de Miguel, and R. Fraisse
Atmos. Chem. Phys., 10, 9505–9519, https://doi.org/10.5194/acp-10-9505-2010, https://doi.org/10.5194/acp-10-9505-2010, 2010
S. P. Burton, L. W. Thomason, and J. M. Zawodny
Atmos. Chem. Phys., 10, 1–8, https://doi.org/10.5194/acp-10-1-2010, https://doi.org/10.5194/acp-10-1-2010, 2010
C. Tétard, D. Fussen, C. Bingen, N. Capouillez, E. Dekemper, N. Loodts, N. Mateshvili, F. Vanhellemont, E. Kyrölä, J. Tamminen, V. Sofieva, A. Hauchecorne, F. Dalaudier, J.-L. Bertaux, O. Fanton d'Andon, G. Barrot, M. Guirlet, T. Fehr, and L. Saavedra
Atmos. Chem. Phys., 9, 7857–7866, https://doi.org/10.5194/acp-9-7857-2009, https://doi.org/10.5194/acp-9-7857-2009, 2009
Cited articles
Ball, W. T., Alsing, J., Mortlock, D. J., Staehelin, J., Haigh, J. D., Peter, T., Tummon, F., Stübi, R., Stenke, A., Anderson, J., Bourassa, A., Davis, S. M., Degenstein, D., Frith, S., Froidevaux, L., Roth, C., Sofieva, V., Wang, R., Wild, J., Yu, P., Ziemke, J. R., and Rozanov, E. V.: Evidence for a continuous decline in lower stratospheric ozone offsetting ozone layer recovery, Atmos. Chem. Phys., 18, 1379–1394, https://doi.org/10.5194/acp-18-1379-2018, 2018.
Ball, W. T., Chiodo, G., Abalos, M., and Alsing, J.: Inconsistencies between chemistry climate model and observed lower stratospheric trends since 1998, Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-734, in review, 2019.
Bourassa, A. E., Degenstein, D. A., Randel, W. J., Zawodny, J. M., Kyrölä, E., McLinden, C. A., Sioris, C. E., and Roth, C. Z.: Trends in stratospheric ozone derived from merged SAGE II and Odin-OSIRIS satellite observations, Atmos. Chem. Phys., 14, 6983–6994, https://doi.org/10.5194/acp-14-6983-2014, 2014.
Brasseur, G. P. and Solomon, S.: Aeronomy of the Middle Atmosphere, 3rd
edn., D. Reidel Publishing Company, Dordrecht, 2005.
Brewer, A. W.: Evidence for a world circulation provided by the measurements
of helium and water vapor distribution in the stratosphere, Q. J. Roy.
Meteor. Soc., 75, 351–363, 1949.
Butchart, N., Scaife, A. A., Bourqui, M., Grandpré, J., Hare, S. H. E.,
Kettleborough, J., Langematz, U., Manzini, E., Sassi, F., Shibata, K.,
Shindell, D., and Sigmond, M.: Simulations of anthropogenic change in the
strength of the Brewer-Dobson circulation, Clim. Dynam., 27, 727–741,
https://doi.org/10.1007/s00382-006-0162-4, 2006.
Chipperfield, M. P. and Jones, R. L.: Relative influences of atmospheric
chemistry and transport on Arctic ozone trends, Nature, 400, 3–6, 1999.
Cochrane, D. and Orcutt, G. H.: Application of Least Squares Regression to
Relationships Containing Auto-Correlated Error Terms, J. Am. Stat. Assoc.,
44, 32–61, https://doi.org/10.1080/01621459.1949.10483290, 1949.
Davis, S. M., Rosenlof, K. H., Hassler, B., Hurst, D. F., Read, W. G., Vömel, H., Selkirk, H., Fujiwara, M., and Damadeo, R.: The Stratospheric Water and Ozone Satellite Homogenized (SWOOSH) database: a long-term database for climate studies, Earth Syst. Sci. Data, 8, 461–490, https://doi.org/10.5194/essd-8-461-2016, 2016.
Dobson, G. M. B.: Origin and distribution of polyatomic molecules in the
atmosphere, P. Roy. Soc. A-Math. Phy., 236, 187–193, 1956.
ESA: Climate Change Initiative (CCI), available at: http://www.esa-ozone-cci.org, last access: 1 June 2020.
Froidevaux, L., Anderson, J., Wang, H.-J., Fuller, R. A., Schwartz, M. J., Santee, M. L., Livesey, N. J., Pumphrey, H. C., Bernath, P. F., Russell III, J. M., and McCormick, M. P.: Global OZone Chemistry And Related trace gas Data records for the Stratosphere (GOZCARDS): methodology and sample results with a focus on HCl, H2O, and O3, Atmos. Chem. Phys., 15, 10471–10507, https://doi.org/10.5194/acp-15-10471-2015, 2015.
Froidevaux, L., Kinnison, D. E., Wang, R., Anderson, J., and Fuller, R. A.: Evaluation of CESM1 (WACCM) free-running and specified dynamics atmospheric composition simulations using global multispecies satellite data records, Atmos. Chem. Phys., 19, 4783–4821, https://doi.org/10.5194/acp-19-4783-2019, 2019.
Funatsu, B. M., Claud, C., Keckhut, P., Hauchecorne, A., and Leblanc, T.:
Regional and seasonal stratospheric temperature trends in the last decade
(2002–2014) from AMSU observations, J. Geophys. Res., 121, 8172–8185,
https://doi.org/10.1002/2015JD024305, 2016.
Gabis, I. P.: Seasonal dependence of the quasi-biennial oscillation (QBO): New evidence from IGRA data, J. Atmos. Sol.-Terr. Phy., 179, 316–336, https://doi.org/10.1016/j.jastp.2018.08.012, 2018
Garcia, R. R. and Randel, W. J.: Acceleration of the Brewer–Dobson
circulation due to increases in greenhouse gases, J. Atmos. Sci., 65,
2731–2739, https://doi.org/10.1175/2008JAS2712.1, 2008.
Gettelman, A., Hegglin, M. I., Son, S.-W., Kim, J., Fujiwara, M., Birner,
T., Kremser, S., Rex, M., Añel, J. A., Akiyoshi, H., Austin, J., Bekki,
S., Braesike, P., Brühl, C., Butchart, N., Chipperfield, M., Dameris,
M., Dhomse, S., Garny, H., Hardiman, S. C., Jöckel, P., Kinnison, D. E.,
Lamarque, J. F., Mancini, E., Marchand, M., Michou, M., Morgenstern, O.,
Pawson, S., Pitari, G., Plummer, D., Pyle, J. A., Rozanov, E., Scinocca, J.,
Shepherd, T. G., Shibata, K., Smale, D., Teyssèdre, H., and Tian, W.:
Multimodel assessment of the upper troposphere and lower stratosphere:
Tropics and global trends, J. Geophys. Res. Atmos., 115, D00M08,
https://doi.org/10.1029/2009JD013638, 2010.
Han, Y., Tian, W., Chipperfield, M. P., Zhang, J., Wang, F., Sang, W., Luo, J., Feng, W., Chrysanthou, A., and Tian, H.: Attribution of the hemispheric asymmetries in trends of stratospheric trace gases inferred from Microwave Limb Sounder (MLS) measurements, J. Geophys. Res.-Atmos., 124, 6283–6293, https://doi.org/10.1029/2018JD029723, 2019.
Harris, N. R. P., Hassler, B., Tummon, F., Bodeker, G. E., Hubert, D., Petropavlovskikh, I., Steinbrecht, W., Anderson, J., Bhartia, P. K., Boone, C. D., Bourassa, A., Davis, S. M., Degenstein, D., Delcloo, A., Frith, S. M., Froidevaux, L., Godin-Beekmann, S., Jones, N., Kurylo, M. J., Kyrölä, E., Laine, M., Leblanc, S. T., Lambert, J.-C., Liley, B., Mahieu, E., Maycock, A., de Mazière, M., Parrish, A., Querel, R., Rosenlof, K. H., Roth, C., Sioris, C., Staehelin, J., Stolarski, R. S., Stübi, R., Tamminen, J., Vigouroux, C., Walker, K. A., Wang, H. J., Wild, J., and Zawodny, J. M.: Past changes in the vertical distribution of ozone – Part 3: Analysis and interpretation of trends, Atmos. Chem. Phys., 15, 9965–9982, https://doi.org/10.5194/acp-15-9965-2015, 2015.
Hauchecorne, A., Bertaux, J. L., Dalaudier, F., Keckhut, P., Lemennais, P., Bekki, S., Marchand, M., Lebrun, J. C., Kyrölä, E., Tamminen, J., Sofieva, V., Fussen, D., Vanhellemont, F., Fanton d'Andon, O., Barrot, G., Blanot, L., Fehr, T., and Saavedra de Miguel, L.: Response of tropical stratospheric O3, NO2 and NO3 to the equatorial Quasi-Biennial Oscillation and to temperature as seen from GOMOS/ENVISAT, Atmos. Chem. Phys., 10, 8873–8879, https://doi.org/10.5194/acp-10-8873-2010, 2010.
Hu, Y. and Fu, Q.: Stratospheric warming in Southern Hemisphere high latitudes since 1979, Atmos. Chem. Phys., 9, 4329–4340, https://doi.org/10.5194/acp-9-4329-2009, 2009.
Khaykin, S. M., Funatsu, B. M., Hauchecorne, A., Godin-Beekmann, S., Claud,
C., Keckhut, P., Pazmino, A., Gleisner, H., Nielsen, J. K., Syndergaard, S.,
and Lauritsen, K. B.: Postmillennium changes in stratospheric temperature
consistently resolved by GPS radio occultation and AMSU observations,
Geophys. Res. Lett., 44, 7510–7518, https://doi.org/10.1002/2017GL074353, 2017.
Kyrölä, E., Laine, M., Sofieva, V., Tamminen, J., Päivärinta, S.-M., Tukiainen, S., Zawodny, J., and Thomason, L.: Combined SAGE II–GOMOS ozone profile data set for 1984–2011 and trend analysis of the vertical distribution of ozone, Atmos. Chem. Phys., 13, 10645–10658, https://doi.org/10.5194/acp-13-10645-2013, 2013.
Li, F., Austin, J., and Wilson, J.: The strength of the Brewer-Dobson
circulation in a changing climate: Coupled chemistry-climate model
simulations, J. Climate, 21, 40–57, https://doi.org/10.1175/2007JCLI1663.1, 2008.
Mahieu, E., Chipperfield, M. P., Notholt, J., Reddmann, T., Anderson, J.,
Bernath, P. F., Blumenstock, T., Coffey, M. T., Dhomse, S. S., Feng, W.,
Franco, B., Froidevaux, L., Griffith, D. W. T., Hannigan, J. W., Hase, F.,
Hossaini, R., Jones, N. B., Morino, I., Murata, I., Nakajima, H., Palm, M.,
Paton-Walsh, C., Russell, J. M., Schneider, M., Servais, C., Smale, D., and
Walker, K. A.: Recent Northern Hemisphere stratospheric HCl increase due to
atmospheric circulation changes, Nature, 515, 104–107,
https://doi.org/10.1038/nature13857, 2014.
McLinden, C. A. and Fioletov, V.: Quantifying trends in stratospheric ozone: Complications due to stratospheric cooling, Geophys. Res. Lett., 38, L03808, https://doi.org/10.1029/2010GL046012, 2011.
Nair, P. J., Froidevaux, L., Kuttippurath, J., Zawodny, J. M., Russell, J.
M., Steinbrecht, W., Claude, H., Leblanc, T., van Gijsel, J. A. E., Johnson,
B., Swart, D. P. J., Thomas, A., Querel, R., Wang, R., and Anderson, J.:
Subtropical and midlatitude ozone trends in the stratosphere: Implications
for recovery, J. Geophys. Res., 120, 7247–7257,
https://doi.org/10.1002/2014JD022371, 2015.
NASA: GES DISC, available at: https://disc.gsfc.nasa.gov, last access: 1 June 2020.
Neu, J. L., Hegglin, M. I., Tegtmeier, S., Bourassa, A., Degenstein, D.,
Froidevaux, L., Fuller, R., Funke, B., Gille, J., Jones, A., Rozanov, A.,
Toohey, M., von Clarmann, T., Walker, K. A., and Worden, J. R.: The SPARC
Data Initiative: Comparison of upper troposphere/lower stratosphere ozone
climatologies from limb-viewing instruments and the nadir-viewing
Tropospheric Emission Spectrometer, J. Geophys. Res.-Atmos., 119,
6971–6990, https://doi.org/10.1002/2013JD020822, 2014.
Newchurch, M. J., Yang, E.-S., Cunnold, D. M., Reinsel, G. C., Zawodny, J.
M., and Russell, J. M.: Evidence for slowdown in stratospheric ozone loss:
First stage of ozone recovery, J. Geophys. Res., 108, 4507,
https://doi.org/10.1029/2003JD003471, 2003.
Petropavlovskikh, I., Godin-Beekmann, S., Hubert, D., Damadeo, R., Hassler,
B., and Sofieva, V.: SPARC/IO3C/GAW Report on Long-term Ozone Trends and
Uncertainties in the Stratosphere, edited by: Kenntner, M. and Ziegele, B., SPARC Report No. 9, GAW Report No. 241, WCRP Report 17/2018, https://doi.org/10.17874/f899e57a20b, 2019.
Randel, W. J. and Thompson, A. M.: Interannual variability and trends in
tropical ozone derived from SAGE II satellite data and SHADOZ ozonesondes,
J. Geophys. Res., 116, D07303, https://doi.org/10.1029/2010JD015195, 2011.
Randel, W. J., Smith, A. K., Wu, F., Zou, C. Z., and Qian, H.: Stratospheric
temperature trends over 1979–2015 derived from combined SSU, MLS, and SABER
satellite observations, J. Climate, 29, 4843–4859,
https://doi.org/10.1175/JCLI-D-15-0629.1, 2016.
Schnadt, C., Dameris, M., Ponater, M., Hein, R., Grewe, V., and Steil, B.:
Interaction of atmospheric chemistry and climate and its impact on
stratospheric ozone, Clim. Dynam., 18, 501–517,
https://doi.org/10.1007/s00382-001-0190-z, 2002.
Sigmond, M., Siegmund, P. C., Manzini, E., and Kelder, H.: A simulation of
the separate climate effects of middle-atmospheric and tropospheric CO2 doubling, J. Climate, 17, 2352–2367,
https://doi.org/10.1175/1520-0442(2004)017<2352:ASOTSC>2.0.CO;2, 2004.
Sofieva, V. F., Kyrölä, E., Laine, M., Tamminen, J., Degenstein, D., Bourassa, A., Roth, C., Zawada, D., Weber, M., Rozanov, A., Rahpoe, N., Stiller, G., Laeng, A., von Clarmann, T., Walker, K. A., Sheese, P., Hubert, D., van Roozendael, M., Zehner, C., Damadeo, R., Zawodny, J., Kramarova, N., and Bhartia, P. K.: Merged SAGE II, Ozone_cci and OMPS ozone profile dataset and evaluation of ozone trends in the stratosphere, Atmos. Chem. Phys., 17, 12533–12552, https://doi.org/10.5194/acp-17-12533-2017, 2017.
Solomon, S., Ivy, D. J., Kinnison, D., Mills, M. J., Neely III, R. R., and Schmidt, A.: Emergence of healing in the Antarctic ozone layer, Science, 353, 269–274, https://doi.org/10.1126/science.aae0061, 2016
Steinbrecht, W., Froidevaux, L., Fuller, R., Wang, R., Anderson, J., Roth, C., Bourassa, A., Degenstein, D., Damadeo, R., Zawodny, J., Frith, S., McPeters, R., Bhartia, P., Wild, J., Long, C., Davis, S., Rosenlof, K., Sofieva, V., Walker, K., Rahpoe, N., Rozanov, A., Weber, M., Laeng, A., von Clarmann, T., Stiller, G., Kramarova, N., Godin-Beekmann, S., Leblanc, T., Querel, R., Swart, D., Boyd, I., Hocke, K., Kämpfer, N., Maillard Barras, E., Moreira, L., Nedoluha, G., Vigouroux, C., Blumenstock, T., Schneider, M., García, O., Jones, N., Mahieu, E., Smale, D., Kotkamp, M., Robinson, J., Petropavlovskikh, I., Harris, N., Hassler, B., Hubert, D., and Tummon, F.: An update on ozone profile trends for the period 2000 to 2016, Atmos. Chem. Phys., 17, 10675–10690, https://doi.org/10.5194/acp-17-10675-2017, 2017.
Thompson, D. W. J. and Solomon, S.: Understanding recent stratospheric
climate change, J. Climate, 22, 1934–1943, https://doi.org/10.1175/2008JCLI2482.1,
2009.
Tummon, F., Hassler, B., Harris, N. R. P., Staehelin, J., Steinbrecht, W., Anderson, J., Bodeker, G. E., Bourassa, A., Davis, S. M., Degenstein, D., Frith, S. M., Froidevaux, L., Kyrölä, E., Laine, M., Long, C., Penckwitt, A. A., Sioris, C. E., Rosenlof, K. H., Roth, C., Wang, H.-J., and Wild, J.: Intercomparison of vertically resolved merged satellite ozone data sets: interannual variability and long-term trends, Atmos. Chem. Phys., 15, 3021–3043, https://doi.org/10.5194/acp-15-3021-2015, 2015.
WMO: Scientific Assessment of Ozone Depletion: 2018, Global Ozone Research and Monitoring Project, Report No. 58, 590 pp., Geneva, Switzerland, 2018.
Zawada, D. J., Rieger, L. A., Bourassa, A. E., and Degenstein, D. A.: Tomographic retrievals of ozone with the OMPS Limb Profiler: algorithm description and preliminary results, Atmos. Meas. Tech., 11, 2375–2393, https://doi.org/10.5194/amt-11-2375-2018, 2018.
Short summary
We analyze seasonal dependence of stratospheric ozone trends over 2000–2018. We demonstrate that the mid-latitude upper stratospheric ozone recovery maximizes during local winters and equinoxes. In the tropics, a very strong seasonal dependence of ozone trends is observed at all altitudes. We found hemispheric asymmetry of summertime ozone trend patterns below 35 km. The seasonal dependence of ozone trends and stratospheric temperature trends shows a clear inter-relation of the trend patterns.
We analyze seasonal dependence of stratospheric ozone trends over 2000–2018. We demonstrate that...
Altmetrics
Final-revised paper
Preprint