Articles | Volume 20, issue 17
https://doi.org/10.5194/acp-20-10351-2020
https://doi.org/10.5194/acp-20-10351-2020
Research article
 | 
07 Sep 2020
Research article |  | 07 Sep 2020

Treatment of non-ideality in the SPACCIM multiphase model – Part 2: Impacts on the multiphase chemical processing in deliquesced aerosol particles

Ahmad Jhony Rusumdar, Andreas Tilgner, Ralf Wolke, and Hartmut Herrmann

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Cited articles

Adriano, D. C. and Johnson, A. H.: Acidic Precipitation: Biological and Ecological Effects, Springer New York, 85–136, 1989. 
Akimoto, H.: Global Air Quality and Pollution, Science, 302, 1716–1719, https://doi.org/10.1126/science.1092666, 2003. 
Amundson, N. R., Caboussat, A., He, J. W., Martynenko, A. V., Savarin, V. B., Seinfeld, J. H., and Yoo, K. Y.: A new inorganic atmospheric aerosol phase equilibrium model (UHAERO), Atmos. Chem. Phys., 6, 975–992, https://doi.org/10.5194/acp-6-975-2006, 2006. 
Amundson, N. R., Caboussat, A., He, J. W., Martynenko, A. V., Landry, C., Tong, C., and Seinfeld, J. H.: A new atmospheric aerosol phase equilibrium model (UHAERO): organic systems, Atmos. Chem. Phys., 7, 4675–4698, https://doi.org/10.5194/acp-7-4675-2007, 2007. 
Andreae, M. O. and Crutzen, P. J.: Atmospheric Aerosols: Biogeochemical Sources and Role in Atmospheric Chemistry, Science, 276, 1052, https://doi.org/10.1126/science.276.5315.1052, 1997. 
Short summary
In the present study, simulations with the SPACCIM-SpactMod multiphase chemistry model are performed. The investigations aim at assessing the impact of a detailed treatment of non-ideality in multiphase models dealing with aqueous aerosol chemistry. The model studies demonstrate that the inclusion of non-ideality considerably affects the multiphase chemical processing of transition metal ions, oxidants, and related chemical subsystems such as organic chemistry in aqueous aerosols.
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