Treatment of non-ideality in the SPACCIM multiphase model – Part 2: Impacts on the multiphase chemical processing in deliquesced aerosol particles

Rusumdar, Ahmad Jhony; Tilgner, Andreas; Wolke, Ralf; Herrmann, Hartmut

doi:https://doi.org/10.5194/acp-20-10351-2020

Articles | Volume 20, issue 17

https://doi.org/10.5194/acp-20-10351-2020

© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

Special issue:

Simulation chambers as tools in atmospheric research (AMT/ACP/GMD...

https://doi.org/10.5194/acp-20-10351-2020

© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

Articles | Volume 20, issue 17

Research article

|

07 Sep 2020

Research article |

| 07 Sep 2020

Treatment of non-ideality in the SPACCIM multiphase model – Part 2: Impacts on the multiphase chemical processing in deliquesced aerosol particles

Ahmad Jhony Rusumdar, Andreas Tilgner, Ralf Wolke, and Hartmut Herrmann

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Final revised paper (published on 07 Sep 2020)
Supplement to the final revised paper
Preprint (discussion started on 28 Oct 2019)
Supplement to the preprint

Interactive discussion

Status: closed

AC: Author comment | RC: Referee comment | SC: Short comment | EC: Editor comment

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- Supplement

RC1: 'Review of the paper by A. Rusumbar et al., "Treatment of non-ideality in the multiphase model SPACCIM-Part2"', Anonymous Referee #1, 09 Jan 2020
- AC1: 'Response to Reviewer 1', Hartmut Herrmann, 25 Mar 2020
- AC3: 'Manuscript version with tracked changes', Hartmut Herrmann, 25 Mar 2020
RC2: 'Review of acp-2019-819', Anonymous Referee #2, 22 Jan 2020
- AC2: 'Response to Reviewer 2', Hartmut Herrmann, 25 Mar 2020
- AC4: 'Manuscript with tracked changes', Hartmut Herrmann, 25 Mar 2020

Peer-review completion

AR: Author's response | RR: Referee report | ED: Editor decision

AR by Hartmut Herrmann on behalf of the Authors (25 Mar 2020) Author's response Manuscript

ED: Publish as is (06 Apr 2020) by Christian George

Short summary

In the present study, simulations with the SPACCIM-SpactMod multiphase chemistry model are performed. The investigations aim at assessing the impact of a detailed treatment of non-ideality in multiphase models dealing with aqueous aerosol chemistry. The model studies demonstrate that the inclusion of non-ideality considerably affects the multiphase chemical processing of transition metal ions, oxidants, and related chemical subsystems such as organic chemistry in aqueous aerosols.