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Volume 17, issue 3
Atmos. Chem. Phys., 17, 2347–2357, 2017
https://doi.org/10.5194/acp-17-2347-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 17, 2347–2357, 2017
https://doi.org/10.5194/acp-17-2347-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 14 Feb 2017

Research article | 14 Feb 2017

Formation of secondary organic aerosols from the ozonolysis of dihydrofurans

Yolanda Diaz-de-Mera et al.

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Subject: Aerosols | Research Activity: Laboratory Studies | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
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Cited articles

Alwe, H. D., Walavalkar, M. P., Sharma, Dhanya, A. S., and Naik P. D.: Tropospheric oxidation of cyclic unsaturated ethers in the day-time: Comparison of the reactions with Cl, OH and O3 based on the determination of their rate coefficients at 298 K, Atmos. Environ., 82, 113–120, 2014.
Anglada, J. M., González, J., and Torrent-Sucarrat, M.: Effects of the substituents on the reactivity of carbonyl oxides. A theoretical study on the reaction of substituted carbonyl oxides with water, Phys. Chem. Chem. Phys., 13, 13034–13045, 2011.
Aranda, A, Díaz-de-Mera, Y., Notario, A., Rodríguez D., and Rodríguez, A.: Fine and ultrafine particles in small cities. A case study in the south of Europe, Environ. Sci. Pollut. R., 22, 18477–18486, 2015.
Bartlett, R. J.: Coupled-cluster approach to molecular structure and spectra: a step toward predictive quantum chemistry, J. Phys. Chem., 93, 1697–1708, 1989.
Berndt, T, Jokinen, T., Sipilä, M., Mauldin, R. L., Herrmann, H., Stratmann, F., Junninen, H., and Kulmala, M.: H2SO4 formation from the gas-phase reaction of stabilized Criegee Intermediates with SO2: Influence of water vapour content and temperature, Atmos. Environ., 89, 603–612, 2014a.
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Criegee intermediates are involved in the formation of secondary organic aerosols. How? Recent works show that they contribute to the oxidation of SO2 to SO3. We have found that the studied ozonolysis reactions only led to nucleation in the presence of SO2, which behaved as a catalyst. So the role of SO2 to form SOA depends on the structure of the alkene. For these reactions, the formation of low-volatility organic acid is expected to be responsible for nucleation, since SO3 was not released.
Criegee intermediates are involved in the formation of secondary organic aerosols. How? Recent...
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