Articles | Volume 15, issue 1
Atmos. Chem. Phys., 15, 153–172, 2015
https://doi.org/10.5194/acp-15-153-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 15, 153–172, 2015
https://doi.org/10.5194/acp-15-153-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
09 Jan 2015
Research article
| 09 Jan 2015
Global and regional modeling of clouds and aerosols in the marine boundary layer during VOCALS: the VOCA intercomparison
M. C. Wyant et al.
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Michael S. Diamond, Pablo E. Saide, Paquita Zuidema, Andrew S. Ackerman, Sarah J. Doherty, Ann M. Fridlind, Hamish Gordon, Calvin Howes, Jan Kazil, Takanobu Yamaguchi, Jianhao Zhang, Graham Feingold, and Robert Wood
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-411, https://doi.org/10.5194/acp-2022-411, 2022
Preprint under review for ACP
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Smoke from southern Africa blankets the southeast Atlantic Ocean from June-October, overlying a major low-altitude cloud deck. The smoke affects Earth's radiation budget by absorbing and reflecting sunlight and changing cloud properties. We investigate smoke effects on the transition between overcast and scattered clouds in regional climate and large eddy simulation models and compare our results with observations from three recent international field campaigns.
Sagar Prasad Parajuli, Georgiy L. Stenchikov, Alexander Ukhov, Suleiman Mostamandi, Paul A. Kucera, Duncan Axisa, William I. Gustafson Jr., and Yannian Zhu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-164, https://doi.org/10.5194/acp-2022-164, 2022
Revised manuscript accepted for ACP
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Rainfall affects the distribution of surface and ground water resources, which are constantly declining over the Middle East and North Africa (MENA) region due to overexploitation. Here, we explored the effects of dust on rainfall using WRF-Chem model simulations. Although dust is considered a nuisance from an air quality perspective, our results highlight the more positive fundamental role of dust particles in modulating rainfall formation and distribution.
Lindsay M. Sheridan, Raghu Krishnamurthy, Gabriel Garcia Medina, Brian J. Gaudet, William I. Gustafson, Alicia M. Mahon, William J. Shaw, Rob K. Newsom, Mikhail Pekour, and Zhaoqing Yang
Wind Energ. Sci. Discuss., https://doi.org/10.5194/wes-2022-16, https://doi.org/10.5194/wes-2022-16, 2022
Preprint under review for WES
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Using observations from lidar buoys, five reanalysis and analysis models that support the wind energy community are validated offshore and at rotor-level heights along the California Pacific coast. The models are found to underestimate the observed wind resource. Occasions of large model error occur in conjunction with wind ramps, stable atmospheric conditions, wind speeds associated with peak turbine power production, and mischaracterization of the diurnal wind speed cycle in summer months.
Ville Leinonen, Harri Kokkola, Taina Yli-Juuti, Tero Mielonen, Thomas Kühn, Tuomo Nieminen, Simo Heikkinen, Tuuli Miinalainen, Tommi Bergman, Ken Carslaw, Stefano Decesari, Markus Fiebig, Tareq Hussein, Niku Kivekäs, Markku Kulmala, Ari Leskinen, Andreas Massling, Nikos Mihalopoulos, Jane P. Mulcahy, Steffen M. Noe, Twan van Noije, Fiona M. O'Connor, Colin O'Dowd, Dirk Olivie, Jakob B. Pernov, Tuukka Petäjä, Øyvind Seland, Michael Schulz, Catherine E. Scott, Henrik Skov, Erik Swietlicki, Thomas Tuch, Alfred Wiedensohler, Annele Virtanen, and Santtu Mikkonen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-225, https://doi.org/10.5194/acp-2022-225, 2022
Preprint under review for ACP
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We provide the first extensive comparison of detailed aerosol size distribution trends between in-situ observations from Europe and five different earth system models. We investigated commonly used aerosol modes (nucleation, Aitken, and accumulation) separately and were able to show the differences between measured and modeled trends and especially their seasonal patterns. This provides an important addition to earlier aerosol-cloud interaction model evaluation studies.
Sarah J. Doherty, Pablo E. Saide, Paquita Zuidema, Yohei Shinozuka, Gonzalo A. Ferrada, Hamish Gordon, Marc Mallet, Kerry Meyer, David Painemal, Steven G. Howell, Steffen Freitag, Amie Dobracki, James R. Podolske, Sharon P. Burton, Richard A. Ferrare, Calvin Howes, Pierre Nabat, Gregory R. Carmichael, Arlindo da Silva, Kristina Pistone, Ian Chang, Lan Gao, Robert Wood, and Jens Redemann
Atmos. Chem. Phys., 22, 1–46, https://doi.org/10.5194/acp-22-1-2022, https://doi.org/10.5194/acp-22-1-2022, 2022
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Between July and October, biomass burning smoke is advected over the southeastern Atlantic Ocean, leading to climate forcing. Model calculations of forcing by this plume vary significantly in both magnitude and sign. This paper compares aerosol and cloud properties observed during three NASA ORACLES field campaigns to the same in four models. It quantifies modeled biases in properties key to aerosol direct radiative forcing and evaluates how these biases propagate to biases in forcing.
Amie Dobracki, Paquita Zuidema, Steve Howell, Pablo Saide, Steffen Freitag, Allison C. Aiken, Sharon P. Burton, Arthur J. Sedlacek III, Jens Redemann, and Robert Wood
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-1081, https://doi.org/10.5194/acp-2021-1081, 2022
Preprint withdrawn
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The global maximum of shortwave-absorbing aerosol above cloud occurs above the southeast Atlantic, where the biomass-burning aerosol provides a distinct aerosol radiative warming of regional climate. The smoke aerosols are unusually highly absorbing of sunlight. This study seeks to understand the cause. We conclude the aerosol is already strongly absorbing at the fire emission source, but that chemical aging, through encouraging a net loss of organic aerosol, also contributes.
Jie Zhang, Kalli Furtado, Steven T. Turnock, Jane P. Mulcahy, Laura J. Wilcox, Ben B. Booth, David Sexton, Tongwen Wu, Fang Zhang, and Qianxia Liu
Atmos. Chem. Phys., 21, 18609–18627, https://doi.org/10.5194/acp-21-18609-2021, https://doi.org/10.5194/acp-21-18609-2021, 2021
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The CMIP6 ESMs systematically underestimate TAS anomalies in the NH midlatitudes, especially from 1960 to 1990. The anomalous cooling is concurrent in time and space with anthropogenic SO2 emissions. The spurious drop in TAS is attributed to the overestimated aerosol concentrations. The aerosol forcing sensitivity cannot well explain the inter-model spread of PHC biases. And the cloud-amount term accounts for most of the inter-model spread in aerosol forcing sensitivity.
Catherine Hardacre, Jane P. Mulcahy, Richard J. Pope, Colin G. Jones, Steven T. Rumbold, Can Li, Colin Johnson, and Steven T. Turnock
Atmos. Chem. Phys., 21, 18465–18497, https://doi.org/10.5194/acp-21-18465-2021, https://doi.org/10.5194/acp-21-18465-2021, 2021
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We investigate UKESM1's ability to represent the sulfur (S) cycle in the recent historical period. The S cycle is a key driver of historical radiative forcing. Earth system models such as UKESM1 should represent the S cycle well so that we can have confidence in their projections of future climate. We compare UKESM1 to observations of sulfur compounds, finding that the model generally performs well. We also identify areas for UKESM1’s development, focussing on how SO2 is removed from the air.
Anthony C. Jones, Adrian Hill, Samuel Remy, N. Luke Abraham, Mohit Dalvi, Catherine Hardacre, Alan J. Hewitt, Ben Johnson, Jane P. Mulcahy, and Steven T. Turnock
Atmos. Chem. Phys., 21, 15901–15927, https://doi.org/10.5194/acp-21-15901-2021, https://doi.org/10.5194/acp-21-15901-2021, 2021
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Ammonium nitrate is hard to model because it forms and evaporates rapidly. One approach is to relate its equilibrium concentration to temperature, humidity, and the amount of nitric acid and ammonia gases. Using this approach, we limit the rate at which equilibrium is reached using various condensation rates in a climate model. We show that ammonium nitrate concentrations are highly sensitive to the condensation rate. Our results will help improve the representation of nitrate in climate models.
Xinxin Ye, Pargoal Arab, Ravan Ahmadov, Eric James, Georg A. Grell, Bradley Pierce, Aditya Kumar, Paul Makar, Jack Chen, Didier Davignon, Greg R. Carmichael, Gonzalo Ferrada, Jeff McQueen, Jianping Huang, Rajesh Kumar, Louisa Emmons, Farren L. Herron-Thorpe, Mark Parrington, Richard Engelen, Vincent-Henri Peuch, Arlindo da Silva, Amber Soja, Emily Gargulinski, Elizabeth Wiggins, Johnathan W. Hair, Marta Fenn, Taylor Shingler, Shobha Kondragunta, Alexei Lyapustin, Yujie Wang, Brent Holben, David M. Giles, and Pablo E. Saide
Atmos. Chem. Phys., 21, 14427–14469, https://doi.org/10.5194/acp-21-14427-2021, https://doi.org/10.5194/acp-21-14427-2021, 2021
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Wildfire smoke has crucial impacts on air quality, while uncertainties in the numerical forecasts remain significant. We present an evaluation of 12 real-time forecasting systems. Comparison of predicted smoke emissions suggests a large spread in magnitudes, with temporal patterns deviating from satellite detections. The performance for AOD and surface PM2.5 and their discrepancies highlighted the role of accurately represented spatiotemporal emission profiles in improving smoke forecasts.
Josué Bock, Martine Michou, Pierre Nabat, Manabu Abe, Jane P. Mulcahy, Dirk J. L. Olivié, Jörg Schwinger, Parvadha Suntharalingam, Jerry Tjiputra, Marco van Hulten, Michio Watanabe, Andrew Yool, and Roland Séférian
Biogeosciences, 18, 3823–3860, https://doi.org/10.5194/bg-18-3823-2021, https://doi.org/10.5194/bg-18-3823-2021, 2021
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In this study we analyse surface ocean dimethylsulfide (DMS) concentration and flux to the atmosphere from four CMIP6 Earth system models over the historical and ssp585 simulations.
Our analysis of contemporary (1980–2009) climatologies shows that models better reproduce observations in mid to high latitudes. The models disagree on the sign of the trend of the global DMS flux from 1980 onwards. The models agree on a positive trend of DMS over polar latitudes following sea-ice retreat dynamics.
Kristina Pistone, Paquita Zuidema, Robert Wood, Michael Diamond, Arlindo M. da Silva, Gonzalo Ferrada, Pablo E. Saide, Rei Ueyama, Ju-Mee Ryoo, Leonhard Pfister, James Podolske, David Noone, Ryan Bennett, Eric Stith, Gregory Carmichael, Jens Redemann, Connor Flynn, Samuel LeBlanc, Michal Segal-Rozenhaimer, and Yohei Shinozuka
Atmos. Chem. Phys., 21, 9643–9668, https://doi.org/10.5194/acp-21-9643-2021, https://doi.org/10.5194/acp-21-9643-2021, 2021
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Using aircraft-based measurements off the Atlantic coast of Africa, we found the springtime smoke plume was strongly correlated with the amount of water vapor in the atmosphere (more smoke indicated more humidity). We see the same general feature in satellite-assimilated and free-running models. Our analysis suggests this relationship is not caused by the burning but originates due to coincident continental meteorology plus fires. This air is transported over the ocean without further mixing.
Behrooz Roozitalab, Gregory R. Carmichael, and Sarath K. Guttikunda
Atmos. Chem. Phys., 21, 2837–2860, https://doi.org/10.5194/acp-21-2837-2021, https://doi.org/10.5194/acp-21-2837-2021, 2021
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We used air quality modeling to study an extreme pollution episode in November 2017 in India. We found both local and regional emissions contribute to high pollution levels. The extreme pollution values were the result of agricultural fires in the northwest of India. Ozone should be considered in future air quality management strategies.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Fiona M. O'Connor, N. Luke Abraham, Mohit Dalvi, Gerd A. Folberth, Paul T. Griffiths, Catherine Hardacre, Ben T. Johnson, Ron Kahana, James Keeble, Byeonghyeon Kim, Olaf Morgenstern, Jane P. Mulcahy, Mark Richardson, Eddy Robertson, Jeongbyn Seo, Sungbo Shim, João C. Teixeira, Steven T. Turnock, Jonny Williams, Andrew J. Wiltshire, Stephanie Woodward, and Guang Zeng
Atmos. Chem. Phys., 21, 1211–1243, https://doi.org/10.5194/acp-21-1211-2021, https://doi.org/10.5194/acp-21-1211-2021, 2021
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This paper calculates how changes in emissions and/or concentrations of different atmospheric constituents since the pre-industrial era have altered the Earth's energy budget at the present day using a metric called effective radiative forcing. The impact of land use change is also assessed. We find that individual contributions do not add linearly, and different Earth system interactions can affect the magnitude of the calculated effective radiative forcing.
Gillian Thornhill, William Collins, Dirk Olivié, Ragnhild B. Skeie, Alex Archibald, Susanne Bauer, Ramiro Checa-Garcia, Stephanie Fiedler, Gerd Folberth, Ada Gjermundsen, Larry Horowitz, Jean-Francois Lamarque, Martine Michou, Jane Mulcahy, Pierre Nabat, Vaishali Naik, Fiona M. O'Connor, Fabien Paulot, Michael Schulz, Catherine E. Scott, Roland Séférian, Chris Smith, Toshihiko Takemura, Simone Tilmes, Kostas Tsigaridis, and James Weber
Atmos. Chem. Phys., 21, 1105–1126, https://doi.org/10.5194/acp-21-1105-2021, https://doi.org/10.5194/acp-21-1105-2021, 2021
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We find that increased temperatures affect aerosols and reactive gases by changing natural emissions and their rates of removal from the atmosphere. Changing the composition of these species in the atmosphere affects the radiative budget of the climate system and therefore amplifies or dampens the climate response of climate models of the Earth system. This study found that the largest effect is a dampening of climate change as warmer temperatures increase the emissions of cooling aerosols.
Gillian D. Thornhill, William J. Collins, Ryan J. Kramer, Dirk Olivié, Ragnhild B. Skeie, Fiona M. O'Connor, Nathan Luke Abraham, Ramiro Checa-Garcia, Susanne E. Bauer, Makoto Deushi, Louisa K. Emmons, Piers M. Forster, Larry W. Horowitz, Ben Johnson, James Keeble, Jean-Francois Lamarque, Martine Michou, Michael J. Mills, Jane P. Mulcahy, Gunnar Myhre, Pierre Nabat, Vaishali Naik, Naga Oshima, Michael Schulz, Christopher J. Smith, Toshihiko Takemura, Simone Tilmes, Tongwen Wu, Guang Zeng, and Jie Zhang
Atmos. Chem. Phys., 21, 853–874, https://doi.org/10.5194/acp-21-853-2021, https://doi.org/10.5194/acp-21-853-2021, 2021
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This paper is a study of how different constituents in the atmosphere, such as aerosols and gases like methane and ozone, affect the energy balance in the atmosphere. Different climate models were run using the same inputs to allow an easy comparison of the results and to understand where the models differ. We found the effect of aerosols is to reduce warming in the atmosphere, but this effect varies between models. Reactions between gases are also important in affecting climate.
Jane P. Mulcahy, Colin Johnson, Colin G. Jones, Adam C. Povey, Catherine E. Scott, Alistair Sellar, Steven T. Turnock, Matthew T. Woodhouse, Nathan Luke Abraham, Martin B. Andrews, Nicolas Bellouin, Jo Browse, Ken S. Carslaw, Mohit Dalvi, Gerd A. Folberth, Matthew Glover, Daniel P. Grosvenor, Catherine Hardacre, Richard Hill, Ben Johnson, Andy Jones, Zak Kipling, Graham Mann, James Mollard, Fiona M. O'Connor, Julien Palmiéri, Carly Reddington, Steven T. Rumbold, Mark Richardson, Nick A. J. Schutgens, Philip Stier, Marc Stringer, Yongming Tang, Jeremy Walton, Stephanie Woodward, and Andrew Yool
Geosci. Model Dev., 13, 6383–6423, https://doi.org/10.5194/gmd-13-6383-2020, https://doi.org/10.5194/gmd-13-6383-2020, 2020
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Aerosols are an important component of the Earth system. Here, we comprehensively document and evaluate the aerosol schemes as implemented in the physical and Earth system models, HadGEM3-GC3.1 and UKESM1. This study provides a useful characterisation of the aerosol climatology in both models, facilitating the understanding of the numerous aerosol–climate interaction studies that will be conducted for CMIP6 and beyond.
Yohei Shinozuka, Pablo E. Saide, Gonzalo A. Ferrada, Sharon P. Burton, Richard Ferrare, Sarah J. Doherty, Hamish Gordon, Karla Longo, Marc Mallet, Yan Feng, Qiaoqiao Wang, Yafang Cheng, Amie Dobracki, Steffen Freitag, Steven G. Howell, Samuel LeBlanc, Connor Flynn, Michal Segal-Rosenhaimer, Kristina Pistone, James R. Podolske, Eric J. Stith, Joseph Ryan Bennett, Gregory R. Carmichael, Arlindo da Silva, Ravi Govindaraju, Ruby Leung, Yang Zhang, Leonhard Pfister, Ju-Mee Ryoo, Jens Redemann, Robert Wood, and Paquita Zuidema
Atmos. Chem. Phys., 20, 11491–11526, https://doi.org/10.5194/acp-20-11491-2020, https://doi.org/10.5194/acp-20-11491-2020, 2020
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In the southeast Atlantic, well-defined smoke plumes from Africa advect over marine boundary layer cloud decks; both are most extensive around September, when most of the smoke resides in the free troposphere. A framework is put forth for evaluating the performance of a range of global and regional atmospheric composition models against observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) airborne mission in September 2016.
Prodromos Zanis, Dimitris Akritidis, Aristeidis K. Georgoulias, Robert J. Allen, Susanne E. Bauer, Olivier Boucher, Jason Cole, Ben Johnson, Makoto Deushi, Martine Michou, Jane Mulcahy, Pierre Nabat, Dirk Olivié, Naga Oshima, Adriana Sima, Michael Schulz, Toshihiko Takemura, and Konstantinos Tsigaridis
Atmos. Chem. Phys., 20, 8381–8404, https://doi.org/10.5194/acp-20-8381-2020, https://doi.org/10.5194/acp-20-8381-2020, 2020
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In this work, we use Coupled Model Intercomparison Project Phase 6 (CMIP6) simulations from 10 Earth system models (ESMs) and general circulation models (GCMs) to study the fast climate responses on pre-industrial climate, due to present-day aerosols. All models carried out two sets of simulations: a control experiment with all forcings set to the year 1850 and a perturbation experiment with all forcings identical to the control, except for aerosols with precursor emissions set to the year 2014.
Pablo E. Saide, Meng Gao, Zifeng Lu, Daniel L. Goldberg, David G. Streets, Jung-Hun Woo, Andreas Beyersdorf, Chelsea A. Corr, Kenneth L. Thornhill, Bruce Anderson, Johnathan W. Hair, Amin R. Nehrir, Glenn S. Diskin, Jose L. Jimenez, Benjamin A. Nault, Pedro Campuzano-Jost, Jack Dibb, Eric Heim, Kara D. Lamb, Joshua P. Schwarz, Anne E. Perring, Jhoon Kim, Myungje Choi, Brent Holben, Gabriele Pfister, Alma Hodzic, Gregory R. Carmichael, Louisa Emmons, and James H. Crawford
Atmos. Chem. Phys., 20, 6455–6478, https://doi.org/10.5194/acp-20-6455-2020, https://doi.org/10.5194/acp-20-6455-2020, 2020
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Air quality forecasts over the Korean Peninsula captured aerosol optical depth but largely overpredicted surface PM during a Chinese haze transport event. Model deficiency was related to the calculation of optical properties. In order to improve it, aerosol size representation needs to be refined in the calculations, and the representation of aerosol properties, such as size distribution, chemical composition, refractive index, hygroscopicity parameter, and density, needs to be improved.
Sungyeon Choi, Lok N. Lamsal, Melanie Follette-Cook, Joanna Joiner, Nickolay A. Krotkov, William H. Swartz, Kenneth E. Pickering, Christopher P. Loughner, Wyat Appel, Gabriele Pfister, Pablo E. Saide, Ronald C. Cohen, Andrew J. Weinheimer, and Jay R. Herman
Atmos. Meas. Tech., 13, 2523–2546, https://doi.org/10.5194/amt-13-2523-2020, https://doi.org/10.5194/amt-13-2523-2020, 2020
Sojin Lee, Chul Han Song, Kyung Man Han, Daven K. Henze, Kyunghwa Lee, Jinhyeok Yu, Jung-Hun Woo, Jia Jung, Yunsoo Choi, Pablo E. Saide, and Gregory R. Carmichael
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-116, https://doi.org/10.5194/gmd-2020-116, 2020
Revised manuscript not accepted
Alexander T. Archibald, Fiona M. O'Connor, Nathan Luke Abraham, Scott Archer-Nicholls, Martyn P. Chipperfield, Mohit Dalvi, Gerd A. Folberth, Fraser Dennison, Sandip S. Dhomse, Paul T. Griffiths, Catherine Hardacre, Alan J. Hewitt, Richard S. Hill, Colin E. Johnson, James Keeble, Marcus O. Köhler, Olaf Morgenstern, Jane P. Mulcahy, Carlos Ordóñez, Richard J. Pope, Steven T. Rumbold, Maria R. Russo, Nicholas H. Savage, Alistair Sellar, Marc Stringer, Steven T. Turnock, Oliver Wild, and Guang Zeng
Geosci. Model Dev., 13, 1223–1266, https://doi.org/10.5194/gmd-13-1223-2020, https://doi.org/10.5194/gmd-13-1223-2020, 2020
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Here we present a description and evaluation of the UKCA stratosphere–troposphere chemistry scheme (StratTrop vn 1.0) implemented in the UK Earth System Model (UKESM1). UKCA StratTrop represents a substantial step forward compared to previous versions of UKCA. We show here that it is fully suited to the challenges of representing interactions in a coupled Earth system model and identify key areas and components for future development that will make it even better in the future.
Meng Gao, Zirui Liu, Bo Zheng, Dongsheng Ji, Peter Sherman, Shaojie Song, Jinyuan Xin, Cheng Liu, Yuesi Wang, Qiang Zhang, Jia Xing, Jingkun Jiang, Zifa Wang, Gregory R. Carmichael, and Michael B. McElroy
Atmos. Chem. Phys., 20, 1497–1505, https://doi.org/10.5194/acp-20-1497-2020, https://doi.org/10.5194/acp-20-1497-2020, 2020
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We quantified the relative influences of anthropogenic emissions and meteorological conditions on PM2.5 concentrations in Beijing over the winters of 2002–2016. Meteorological conditions over the study period would have led to an increase of haze in Beijing, but the strict emission control measures have suppressed the unfavorable influences of the recent climate.
Meng Gao, Zhiwei Han, Zhining Tao, Jiawei Li, Jeong-Eon Kang, Kan Huang, Xinyi Dong, Bingliang Zhuang, Shu Li, Baozhu Ge, Qizhong Wu, Hyo-Jung Lee, Cheol-Hee Kim, Joshua S. Fu, Tijian Wang, Mian Chin, Meng Li, Jung-Hun Woo, Qiang Zhang, Yafang Cheng, Zifa Wang, and Gregory R. Carmichael
Atmos. Chem. Phys., 20, 1147–1161, https://doi.org/10.5194/acp-20-1147-2020, https://doi.org/10.5194/acp-20-1147-2020, 2020
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Topic 3 of the Model Inter-Comparison Study for Asia (MICS-Asia) Phase III examines how online coupled air quality models perform in simulating high aerosol pollution in the North China Plain region during wintertime haze events and evaluates the importance of aerosol radiative feedbacks. This paper discusses the estimates of aerosol radiative forcing, aerosol feedbacks, and possible causes for the differences among the models.
Lei Kong, Xiao Tang, Jiang Zhu, Zifa Wang, Joshua S. Fu, Xuemei Wang, Syuichi Itahashi, Kazuyo Yamaji, Tatsuya Nagashima, Hyo-Jung Lee, Cheol-Hee Kim, Chuan-Yao Lin, Lei Chen, Meigen Zhang, Zhining Tao, Jie Li, Mizuo Kajino, Hong Liao, Zhe Wang, Kengo Sudo, Yuesi Wang, Yuepeng Pan, Guiqian Tang, Meng Li, Qizhong Wu, Baozhu Ge, and Gregory R. Carmichael
Atmos. Chem. Phys., 20, 181–202, https://doi.org/10.5194/acp-20-181-2020, https://doi.org/10.5194/acp-20-181-2020, 2020
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Evaluation and uncertainty investigation of NO2, CO and NH3 modeling over China were conducted in this study using 14 chemical transport model results from MICS-Asia III. All models largely underestimated CO concentrations and showed very poor performance in reproducing the observed monthly variations of NH3 concentrations. Potential factors related to such deficiencies are investigated and discussed in this paper.
Laura E. Revell, Stefanie Kremser, Sean Hartery, Mike Harvey, Jane P. Mulcahy, Jonny Williams, Olaf Morgenstern, Adrian J. McDonald, Vidya Varma, Leroy Bird, and Alex Schuddeboom
Atmos. Chem. Phys., 19, 15447–15466, https://doi.org/10.5194/acp-19-15447-2019, https://doi.org/10.5194/acp-19-15447-2019, 2019
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Aerosols over the Southern Ocean consist primarily of sea salt and sulfate, yet are seasonally biased in our model. We test three sulfate chemistry schemes to investigate DMS oxidation, which forms sulfate aerosol. Simulated cloud droplet number concentrations improve using more complex sulfate chemistry. We also show that a new sea spray aerosol source function, developed from measurements made on a recent Southern Ocean research voyage, improves the model's simulation of aerosol optical depth.
Samuel Rémy, Zak Kipling, Johannes Flemming, Olivier Boucher, Pierre Nabat, Martine Michou, Alessio Bozzo, Melanie Ades, Vincent Huijnen, Angela Benedetti, Richard Engelen, Vincent-Henri Peuch, and Jean-Jacques Morcrette
Geosci. Model Dev., 12, 4627–4659, https://doi.org/10.5194/gmd-12-4627-2019, https://doi.org/10.5194/gmd-12-4627-2019, 2019
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This article describes the IFS-AER aerosol module used operationally in the Integrated Forecasting System (IFS) cycle 45R1, operated by the ECMWF in the framework of the Copernicus Atmospheric Monitoring Services (CAMS). We describe the different parameterizations for aerosol sources, sinks, and how the aerosols are integrated in the larger atmospheric composition forecasting system. The skill of PM and AOD simulations against observations is improved compared to the older cycle 40R2.
Jie Li, Tatsuya Nagashima, Lei Kong, Baozhu Ge, Kazuyo Yamaji, Joshua S. Fu, Xuemei Wang, Qi Fan, Syuichi Itahashi, Hyo-Jung Lee, Cheol-Hee Kim, Chuan-Yao Lin, Meigen Zhang, Zhining Tao, Mizuo Kajino, Hong Liao, Meng Li, Jung-Hun Woo, Jun-ichi Kurokawa, Zhe Wang, Qizhong Wu, Hajime Akimoto, Gregory R. Carmichael, and Zifa Wang
Atmos. Chem. Phys., 19, 12993–13015, https://doi.org/10.5194/acp-19-12993-2019, https://doi.org/10.5194/acp-19-12993-2019, 2019
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This study evaluated and intercompared 14 CTMs with ozone observations in East Asia, within the framework of the Model Inter-Comparison Study for ASIA Phase III (MICS-Asia III). Potential causes of the discrepancies between model results and observation were investigated by assessing the planetary boundary layer heights, emission fluxes, dry deposition, chemistry and vertical transport among models. Finally, a multi-model estimate of pollution distributions was provided.
Myungje Choi, Hyunkwang Lim, Jhoon Kim, Seoyoung Lee, Thomas F. Eck, Brent N. Holben, Michael J. Garay, Edward J. Hyer, Pablo E. Saide, and Hongqing Liu
Atmos. Meas. Tech., 12, 4619–4641, https://doi.org/10.5194/amt-12-4619-2019, https://doi.org/10.5194/amt-12-4619-2019, 2019
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Satellite-based aerosol optical depth (AOD) products have been improved continuously and available from multiple low Earth orbit sensors, such as MODIS, MISR, and VIIRS, and geostationary sensors, such as GOCI and AHI, over East Asia. These multi-satellite AOD products are validated, intercompared, analyzed, and integrated to understand different characteristics, such as quality and spatio-temporal coverage, focused on several aerosol transportation cases during the 2016 KORUS-AQ campaign.
David Walters, Anthony J. Baran, Ian Boutle, Malcolm Brooks, Paul Earnshaw, John Edwards, Kalli Furtado, Peter Hill, Adrian Lock, James Manners, Cyril Morcrette, Jane Mulcahy, Claudio Sanchez, Chris Smith, Rachel Stratton, Warren Tennant, Lorenzo Tomassini, Kwinten Van Weverberg, Simon Vosper, Martin Willett, Jo Browse, Andrew Bushell, Kenneth Carslaw, Mohit Dalvi, Richard Essery, Nicola Gedney, Steven Hardiman, Ben Johnson, Colin Johnson, Andy Jones, Colin Jones, Graham Mann, Sean Milton, Heather Rumbold, Alistair Sellar, Masashi Ujiie, Michael Whitall, Keith Williams, and Mohamed Zerroukat
Geosci. Model Dev., 12, 1909–1963, https://doi.org/10.5194/gmd-12-1909-2019, https://doi.org/10.5194/gmd-12-1909-2019, 2019
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Global Atmosphere (GA) configurations of the Unified Model (UM) and Global Land (GL) configurations of JULES are developed for use in any global atmospheric modelling application. We describe a recent iteration of these configurations, GA7/GL7, which includes new aerosol and snow schemes and addresses the four critical errors identified in GA6. GA7/GL7 will underpin the UK's contributions to CMIP6, and hence their documentation is important.
Marc Mallet, Pierre Nabat, Paquita Zuidema, Jens Redemann, Andrew Mark Sayer, Martin Stengel, Sebastian Schmidt, Sabrina Cochrane, Sharon Burton, Richard Ferrare, Kerry Meyer, Pablo Saide, Hiren Jethva, Omar Torres, Robert Wood, David Saint Martin, Romain Roehrig, Christina Hsu, and Paola Formenti
Atmos. Chem. Phys., 19, 4963–4990, https://doi.org/10.5194/acp-19-4963-2019, https://doi.org/10.5194/acp-19-4963-2019, 2019
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The model is able to represent LWP but not the LCF. AOD is consistent over the continent but also over ocean (ACAOD). Differences are observed in SSA due to the absence of internal mixing in ALADIN-Climate. A significant regional gradient of the forcing at TOA is observed. An intense positive forcing is simulated over Gabon. Results highlight the significant effect of enhanced moisture on BBA extinction. The surface dimming modifies the energy budget.
Daniel L. Goldberg, Pablo E. Saide, Lok N. Lamsal, Benjamin de Foy, Zifeng Lu, Jung-Hun Woo, Younha Kim, Jinseok Kim, Meng Gao, Gregory Carmichael, and David G. Streets
Atmos. Chem. Phys., 19, 1801–1818, https://doi.org/10.5194/acp-19-1801-2019, https://doi.org/10.5194/acp-19-1801-2019, 2019
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Using satellite data, we are able to estimate the emissions of NOx (NOx=NO+NO2), a toxic group of air pollutants, in the Seoul metropolitan area. We first develop an enhanced satellite product that better observes NO2 in urban regions. Using this new product, we derive NOx emissions to be twice as large as the emissions reported by the South Korean government. The implication is that the measures taken to reduce NOx emissions in South Korea have not been as effective as regulators have thought.
Maryam Abdi-Oskouei, Gabriele Pfister, Frank Flocke, Negin Sobhani, Pablo Saide, Alan Fried, Dirk Richter, Petter Weibring, James Walega, and Gregory Carmichael
Atmos. Chem. Phys., 18, 16863–16883, https://doi.org/10.5194/acp-18-16863-2018, https://doi.org/10.5194/acp-18-16863-2018, 2018
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This study presents a quantification of model uncertainties due to configurations and errors in the emission inventories. The analysis includes performing simulations with different configurations and comparisons with airborne and ground-based observations with a focus on capturing transport and emissions from the oil and gas sector. The presented results reflect the challenges that one may face when attempting to improve emission inventories by contrasting measured with modeled concentrations.
Elizabeth M. Lennartson, Jun Wang, Juping Gu, Lorena Castro Garcia, Cui Ge, Meng Gao, Myungje Choi, Pablo E. Saide, Gregory R. Carmichael, Jhoon Kim, and Scott J. Janz
Atmos. Chem. Phys., 18, 15125–15144, https://doi.org/10.5194/acp-18-15125-2018, https://doi.org/10.5194/acp-18-15125-2018, 2018
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This paper is among the first to study the diurnal variations of AOD, PM2.5, and their relationships in South Korea. We show that the PM2.5–AOD relationship has strong diurnal variations, and, hence, using AOD data retrieved from geostationary satellite can improve the monitoring of surface PM2.5 air quality on a daily basis as well as constrain the diurnal variation of aerosol emission.
Michael S. Diamond, Amie Dobracki, Steffen Freitag, Jennifer D. Small Griswold, Ashley Heikkila, Steven G. Howell, Mary E. Kacarab, James R. Podolske, Pablo E. Saide, and Robert Wood
Atmos. Chem. Phys., 18, 14623–14636, https://doi.org/10.5194/acp-18-14623-2018, https://doi.org/10.5194/acp-18-14623-2018, 2018
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Smoke from Africa can mix into clouds over the southeast Atlantic and create new droplets, which brightens the clouds, reflects more sunlight, and thus cools the region. Using aircraft data from a NASA field campaign, we find that cloud properties are correlated with smoke as expected when the smoke is below the clouds but not when smoke is above the clouds because it takes several days for clouds to mix smoke downward. We recommend methods that can track clouds as they move for future studies.
Meng Gao, Zhiwei Han, Zirui Liu, Meng Li, Jinyuan Xin, Zhining Tao, Jiawei Li, Jeong-Eon Kang, Kan Huang, Xinyi Dong, Bingliang Zhuang, Shu Li, Baozhu Ge, Qizhong Wu, Yafang Cheng, Yuesi Wang, Hyo-Jung Lee, Cheol-Hee Kim, Joshua S. Fu, Tijian Wang, Mian Chin, Jung-Hun Woo, Qiang Zhang, Zifa Wang, and Gregory R. Carmichael
Atmos. Chem. Phys., 18, 4859–4884, https://doi.org/10.5194/acp-18-4859-2018, https://doi.org/10.5194/acp-18-4859-2018, 2018
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Topic 3 of the Model Inter-Comparison Study for Asia (MICS-Asia) Phase III examines how online coupled air quality models perform in simulating high aerosol pollution in the North China Plain region during wintertime haze events and evaluates the importance of aerosol radiative and microphysical feedbacks. A comprehensive overview of the MICS-ASIA III Topic 3 study design is presented.
Stefano Galmarini, Brigitte Koffi, Efisio Solazzo, Terry Keating, Christian Hogrefe, Michael Schulz, Anna Benedictow, Jan Jurgen Griesfeller, Greet Janssens-Maenhout, Greg Carmichael, Joshua Fu, and Frank Dentener
Atmos. Chem. Phys., 17, 1543–1555, https://doi.org/10.5194/acp-17-1543-2017, https://doi.org/10.5194/acp-17-1543-2017, 2017
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We present an overview of the coordinated global numerical modelling experiments performed during 2012–2016 by the Task Force on Hemispheric Transport of Air Pollution (TF HTAP), the regional experiments by the Air Quality Model Evaluation International Initiative (AQMEII) over Europe and North America, and the Model Intercomparison Study for Asia (MICS-Asia). Given the organizational complexity of bringing together these three initiatives, the experiment organization is presented.
Meng Li, Qiang Zhang, Jun-ichi Kurokawa, Jung-Hun Woo, Kebin He, Zifeng Lu, Toshimasa Ohara, Yu Song, David G. Streets, Gregory R. Carmichael, Yafang Cheng, Chaopeng Hong, Hong Huo, Xujia Jiang, Sicong Kang, Fei Liu, Hang Su, and Bo Zheng
Atmos. Chem. Phys., 17, 935–963, https://doi.org/10.5194/acp-17-935-2017, https://doi.org/10.5194/acp-17-935-2017, 2017
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An anthropogenic emission inventory for Asia is developed for the years 2008 and 2010 to support the Model Inter-Comparison Study for Asia (MICS-Asia) and the Task Force on Hemispheric Transport of Air Pollution (TF HTAP) projects by a mosaic of up-to-date regional emission inventories. The total Asian emissions in 2010 are estimated as follows: 51.3 Tg SO2, 52.1 Tg NOx, 336.5 Tg CO, 67.0 Tg NMVOC, 28.7 Tg NH3, 31.7 Tg PM10, 22.7 Tg PM2.5, 3.5 Tg BC, 8.3 Tg OC, and 17.3 Pg CO2.
Ben T. Johnson, James M. Haywood, Justin M. Langridge, Eoghan Darbyshire, William T. Morgan, Kate Szpek, Jennifer K. Brooke, Franco Marenco, Hugh Coe, Paulo Artaxo, Karla M. Longo, Jane P. Mulcahy, Graham W. Mann, Mohit Dalvi, and Nicolas Bellouin
Atmos. Chem. Phys., 16, 14657–14685, https://doi.org/10.5194/acp-16-14657-2016, https://doi.org/10.5194/acp-16-14657-2016, 2016
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Biomass burning is a large source of carbonaceous aerosols, which scatter and absorb solar radiation, and modify cloud properties. We evaluate the simulation of biomass burning aerosol processes and properties in the HadGEM3 climate model using observations, including those from the South American Biomass Burning Analysis. We find that modelled aerosol optical depths are underestimated unless aerosol emissions (Global Fire Emission Database v3) are increased by a factor of 1.6–2.0.
Meng Gao, Gregory R. Carmichael, Pablo E. Saide, Zifeng Lu, Man Yu, David G. Streets, and Zifa Wang
Atmos. Chem. Phys., 16, 11837–11851, https://doi.org/10.5194/acp-16-11837-2016, https://doi.org/10.5194/acp-16-11837-2016, 2016
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The WRF-Chem model was used to examine how the winter PM2.5 concentrations change in response to changes in emissions and meteorology in North China from 1960 to 2010. The discussions in this study indicate that dramatic changes in emissions are the main cause of increasing haze events in North China, and long-term trends in atmospheric circulations maybe another important cause. We also found aerosol feedbacks have been significantly enhanced from 1960 to 2010, due to higher aerosol loadings.
Dan Chen, Zhiquan Liu, Jerome Fast, and Junmei Ban
Atmos. Chem. Phys., 16, 10707–10724, https://doi.org/10.5194/acp-16-10707-2016, https://doi.org/10.5194/acp-16-10707-2016, 2016
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Extreme haze events occurred frequently over China recently, and adequately predicting peak PM2.5 concentrations is still challenging. In this study, the sulfate–nitrate–ammonium relevant heterogeneous reactions were parameterized for the first time in the WRF-Chem model. We evaluated the performance of WRF-Chem and used the model to investigate the sensitivity of heterogeneous reactions on simulated peak sulfate, nitrate, and ammonium concentrations in the vicinity of Beijing during October 2014.
Chun Zhao, Maoyi Huang, Jerome D. Fast, Larry K. Berg, Yun Qian, Alex Guenther, Dasa Gu, Manish Shrivastava, Ying Liu, Stacy Walters, Gabriele Pfister, Jiming Jin, John E. Shilling, and Carsten Warneke
Geosci. Model Dev., 9, 1959–1976, https://doi.org/10.5194/gmd-9-1959-2016, https://doi.org/10.5194/gmd-9-1959-2016, 2016
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In this study, the latest version of MEGAN is coupled within CLM4 in WRF-Chem. In this implementation, MEGAN shares a consistent vegetation map with CLM4. This improved modeling framework is used to investigate the impact of two land surface schemes on BVOCs and examine the sensitivity of BVOCs to vegetation distributions in California. This study indicates that more effort is needed to obtain the most appropriate and accurate land cover data sets for climate and air quality models.
N. Huneeus, S. Basart, S. Fiedler, J.-J. Morcrette, A. Benedetti, J. Mulcahy, E. Terradellas, C. Pérez García-Pando, G. Pejanovic, S. Nickovic, P. Arsenovic, M. Schulz, E. Cuevas, J. M. Baldasano, J. Pey, S. Remy, and B. Cvetkovic
Atmos. Chem. Phys., 16, 4967–4986, https://doi.org/10.5194/acp-16-4967-2016, https://doi.org/10.5194/acp-16-4967-2016, 2016
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Five dust models are evaluated regarding their performance in predicting an intense Saharan dust outbreak affecting western and northern Europe (NE). Models predict the onset and evolution of the event for all analysed lead times. On average, differences among the models are larger than differences in lead times for each model. The models tend to underestimate the long-range transport towards NE. This is partly due to difficulties in simulating the vertical dust distribution and horizontal wind.
Franco Marenco, Ben Johnson, Justin M. Langridge, Jane Mulcahy, Angela Benedetti, Samuel Remy, Luke Jones, Kate Szpek, Jim Haywood, Karla Longo, and Paulo Artaxo
Atmos. Chem. Phys., 16, 2155–2174, https://doi.org/10.5194/acp-16-2155-2016, https://doi.org/10.5194/acp-16-2155-2016, 2016
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A widespread and persistent smoke layer was observed in the Amazon
region during the biomass burning season, spanning a distance of 2200 km
and a period of 14 days. The larger smoke content was typically found
in elevated layers, from 1–1.5 km to 4–6 km.
Measurements have been compared to model predictions, and the latter
were able to reproduce the general features of the smoke layer, but
with some differences which are analysed and described in the paper.
L. Kleinman, C. Kuang, A. Sedlacek, G. Senum, S. Springston, J. Wang, Q. Zhang, J. Jayne, J. Fast, J. Hubbe, J. Shilling, and R. Zaveri
Atmos. Chem. Phys., 16, 1729–1746, https://doi.org/10.5194/acp-16-1729-2016, https://doi.org/10.5194/acp-16-1729-2016, 2016
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Atmospheric measurements of total organic aerosol (OA) and tracers of anthropogenic and biogenic emissions are used to quantify synergistic effects (A–B interactions) between two classes of precursors in the formation of OA. Regressions are consistent with the Sacramento plume composed mainly of modern carbon, and OA correlating best with an anthropogenic tracer. It is found that meteorological conditions during a pollution episode can mimic effects of A–B interactions.
M. Gao, G. R. Carmichael, Y. Wang, P. E. Saide, M. Yu, J. Xin, Z. Liu, and Z. Wang
Atmos. Chem. Phys., 16, 1673–1691, https://doi.org/10.5194/acp-16-1673-2016, https://doi.org/10.5194/acp-16-1673-2016, 2016
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The WRF-Chem model was applied to study the 2010 winter haze in North China. Air pollutants outside Beijing contributed about 64.5 % to the PM2.5 levels in Beijing during this haze event, and most of them are from south Hebei, Tianjin city, Shandong and Henan provinces. In addition, aerosol feedback has important impacts on surface temperature, Relative Humidity (RH) and wind speeds, and these meteorological variables affect aerosol distribution and formation in turn.
G. Roberts, M. J. Wooster, W. Xu, P. H. Freeborn, J.-J. Morcrette, L. Jones, A. Benedetti, H. Jiangping, D. Fisher, and J. W. Kaiser
Atmos. Chem. Phys., 15, 13241–13267, https://doi.org/10.5194/acp-15-13241-2015, https://doi.org/10.5194/acp-15-13241-2015, 2015
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Characterising the dynamics of wildfires at high temporal resolution is best achieved using observations from geostationary satellite sensors. The SEVIRI Fire Radiative Power (FRP) products have been developed using such imagery at up to 15-minute temporal frequency. These data are used to estimate wildfire fuel consumption and to the characterise smoke emissions from the 2007 Peloponnese "mega fires" within an atmospheric transport model.
A. Lupascu, R. Easter, R. Zaveri, M. Shrivastava, M. Pekour, J. Tomlinson, Q. Yang, H. Matsui, A. Hodzic, Q. Zhang, and J. D. Fast
Atmos. Chem. Phys., 15, 12283–12313, https://doi.org/10.5194/acp-15-12283-2015, https://doi.org/10.5194/acp-15-12283-2015, 2015
S. R. Kolusu, J. H. Marsham, J. Mulcahy, B. Johnson, C. Dunning, M. Bush, and D. V. Spracklen
Atmos. Chem. Phys., 15, 12251–12266, https://doi.org/10.5194/acp-15-12251-2015, https://doi.org/10.5194/acp-15-12251-2015, 2015
L. Zhang, D. K. Henze, G. A. Grell, G. R. Carmichael, N. Bousserez, Q. Zhang, O. Torres, C. Ahn, Z. Lu, J. Cao, and Y. Mao
Atmos. Chem. Phys., 15, 10281–10308, https://doi.org/10.5194/acp-15-10281-2015, https://doi.org/10.5194/acp-15-10281-2015, 2015
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We attempt to reduce uncertainties in BC emissions and improve BC model simulations by developing top-down, spatially resolved, estimates of BC emissions through assimilation of OMI observations of aerosol absorption optical depth (AAOD) with the GEOS-Chem model and its adjoint for April and October of 2006. Despite the limitations and uncertainties, using OMI AAOD to constrain BC sources we are able to improve model representation of BC distributions, particularly over China.
H. S. Chen, Z. F. Wang, J. Li, X. Tang, B. Z. Ge, X. L. Wu, O. Wild, and G. R. Carmichael
Geosci. Model Dev., 8, 2857–2876, https://doi.org/10.5194/gmd-8-2857-2015, https://doi.org/10.5194/gmd-8-2857-2015, 2015
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A new global nested atmospheric mercury transport model was developed and introduced. Model performance was found significantly better in North America and Europe than in East Asia. Nested simulation has been conducted in East Asia and shows improved skill at capturing the high spatial variability of Hg concentrations and deposition. The trans-boundary transport of Chinese primary anthropogenic mercury emissions was quantified for the first time.
Y. Shinozuka, A. D. Clarke, A. Nenes, A. Jefferson, R. Wood, C. S. McNaughton, J. Ström, P. Tunved, J. Redemann, K. L. Thornhill, R. H. Moore, T. L. Lathem, J. J. Lin, and Y. J. Yoon
Atmos. Chem. Phys., 15, 7585–7604, https://doi.org/10.5194/acp-15-7585-2015, https://doi.org/10.5194/acp-15-7585-2015, 2015
A. H. Berner, C. S. Bretherton, and R. Wood
Atmos. Chem. Phys., 15, 5851–5871, https://doi.org/10.5194/acp-15-5851-2015, https://doi.org/10.5194/acp-15-5851-2015, 2015
R. Kumar, M. C. Barth, V. S. Nair, G. G. Pfister, S. Suresh Babu, S. K. Satheesh, K. Krishna Moorthy, G. R. Carmichael, Z. Lu, and D. G. Streets
Atmos. Chem. Phys., 15, 5415–5428, https://doi.org/10.5194/acp-15-5415-2015, https://doi.org/10.5194/acp-15-5415-2015, 2015
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We examine differences in the surface BC between the Bay of Bengal (BoB) and the Arabian Sea (AS) and identify dominant sources of BC in South Asia during ICARB. Anthropogenic emissions were the main source of BC during ICARB and had about 5 times stronger influence on the BoB compared to the AS. Regional-scale transport contributes up to 25% of BC mass concentrations in western and eastern India, suggesting that surface BC mass concentrations cannot be linked directly to the local emissions.
M. Bocquet, H. Elbern, H. Eskes, M. Hirtl, R. Žabkar, G. R. Carmichael, J. Flemming, A. Inness, M. Pagowski, J. L. Pérez Camaño, P. E. Saide, R. San Jose, M. Sofiev, J. Vira, A. Baklanov, C. Carnevale, G. Grell, and C. Seigneur
Atmos. Chem. Phys., 15, 5325–5358, https://doi.org/10.5194/acp-15-5325-2015, https://doi.org/10.5194/acp-15-5325-2015, 2015
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Data assimilation is used in atmospheric chemistry models to improve air quality forecasts, construct re-analyses of concentrations, and perform inverse modeling. Coupled chemistry meteorology models (CCMM) are atmospheric chemistry models that simulate meteorological processes and chemical transformations jointly. We review here the current status of data assimilation in atmospheric chemistry models, with a particular focus on future prospects for data assimilation in CCMM.
E. Cuevas, C. Camino, A. Benedetti, S. Basart, E. Terradellas, J. M. Baldasano, J. J. Morcrette, B. Marticorena, P. Goloub, A. Mortier, A. Berjón, Y. Hernández, M. Gil-Ojeda, and M. Schulz
Atmos. Chem. Phys., 15, 3991–4024, https://doi.org/10.5194/acp-15-3991-2015, https://doi.org/10.5194/acp-15-3991-2015, 2015
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Atmospheric mineral dust from a MACC-II short reanalysis (2007-2008) has been evaluated over northern Africa and the Middle East using satellite aerosol products, AERONET data, in situ PM10 concentrations, and extinction vertical profiles. The MACC-II AOD spatial and temporal variability shows good agreement with satellite sensors and AERONET. We find a good agreement in averaged extinction vertical profiles between MACC-II and lidars. MACC correctly reproduces daily to interannual PM10.
L. Marelle, J.-C. Raut, J. L. Thomas, K. S. Law, B. Quennehen, G. Ancellet, J. Pelon, A. Schwarzenboeck, and J. D. Fast
Atmos. Chem. Phys., 15, 3831–3850, https://doi.org/10.5194/acp-15-3831-2015, https://doi.org/10.5194/acp-15-3831-2015, 2015
L. K. Berg, M. Shrivastava, R. C. Easter, J. D. Fast, E. G. Chapman, Y. Liu, and R. A. Ferrare
Geosci. Model Dev., 8, 409–429, https://doi.org/10.5194/gmd-8-409-2015, https://doi.org/10.5194/gmd-8-409-2015, 2015
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This work presents a new methodology for representing regional-scale impacts of cloud processing on both aerosol and trace gases in sub-grid-scale convective clouds. Using the new methodology, we can better simulate the aerosol lifecycle over large areas. The results presented in this work highlight the potential change in column-integrated amounts of black carbon, organic aerosol, and sulfate aerosol, which were found to range from -50% for black carbon to +40% for sulfate.
S. Kulkarni, N. Sobhani, J. P. Miller-Schulze, M. M. Shafer, J. J. Schauer, P. A. Solomon, P. E. Saide, S. N. Spak, Y. F. Cheng, H. A. C. Denier van der Gon, Z. Lu, D. G. Streets, G. Janssens-Maenhout, C. Wiedinmyer, J. Lantz, M. Artamonova, B. Chen, S. Imashev, L. Sverdlik, J. T. Deminter, B. Adhikary, A. D'Allura, C. Wei, and G. R. Carmichael
Atmos. Chem. Phys., 15, 1683–1705, https://doi.org/10.5194/acp-15-1683-2015, https://doi.org/10.5194/acp-15-1683-2015, 2015
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This study presents a regional-scale modeling analysis of aerosols in the Central Asia region including detailed characterization of seasonal source region and sector contributions along with the predicted changes in distribution of aerosols using 2030 future emission scenarios. The influence of long transport and impact of varied emission sources including dust, biomass burning, and anthropogenic sources on the regional aerosol distributions and the associated transport pathways are discussed.
W. R. Sessions, J. S. Reid, A. Benedetti, P. R. Colarco, A. da Silva, S. Lu, T. Sekiyama, T. Y. Tanaka, J. M. Baldasano, S. Basart, M. E. Brooks, T. F. Eck, M. Iredell, J. A. Hansen, O. C. Jorba, H.-M. H. Juang, P. Lynch, J.-J. Morcrette, S. Moorthi, J. Mulcahy, Y. Pradhan, M. Razinger, C. B. Sampson, J. Wang, and D. L. Westphal
Atmos. Chem. Phys., 15, 335–362, https://doi.org/10.5194/acp-15-335-2015, https://doi.org/10.5194/acp-15-335-2015, 2015
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T. Amnuaylojaroen, M. C. Barth, L. K. Emmons, G. R. Carmichael, J. Kreasuwun, S. Prasitwattanaseree, and S. Chantara
Atmos. Chem. Phys., 14, 12983–13012, https://doi.org/10.5194/acp-14-12983-2014, https://doi.org/10.5194/acp-14-12983-2014, 2014
S. Nordmann, Y. F. Cheng, G. R. Carmichael, M. Yu, H. A. C. Denier van der Gon, Q. Zhang, P. E. Saide, U. Pöschl, H. Su, W. Birmili, and A. Wiedensohler
Atmos. Chem. Phys., 14, 12683–12699, https://doi.org/10.5194/acp-14-12683-2014, https://doi.org/10.5194/acp-14-12683-2014, 2014
S. Archer-Nicholls, D. Lowe, S. Utembe, J. Allan, R. A. Zaveri, J. D. Fast, Ø. Hodnebrog, H. Denier van der Gon, and G. McFiggans
Geosci. Model Dev., 7, 2557–2579, https://doi.org/10.5194/gmd-7-2557-2014, https://doi.org/10.5194/gmd-7-2557-2014, 2014
X. Wang, C. L. Heald, D. A. Ridley, J. P. Schwarz, J. R. Spackman, A. E. Perring, H. Coe, D. Liu, and A. D. Clarke
Atmos. Chem. Phys., 14, 10989–11010, https://doi.org/10.5194/acp-14-10989-2014, https://doi.org/10.5194/acp-14-10989-2014, 2014
P. Marrapu, Y. Cheng, G. Beig, S. Sahu, R. Srinivas, and G. R. Carmichael
Atmos. Chem. Phys., 14, 10619–10630, https://doi.org/10.5194/acp-14-10619-2014, https://doi.org/10.5194/acp-14-10619-2014, 2014
H. Matsui, M. Koike, Y. Kondo, J. D. Fast, and M. Takigawa
Atmos. Chem. Phys., 14, 10315–10331, https://doi.org/10.5194/acp-14-10315-2014, https://doi.org/10.5194/acp-14-10315-2014, 2014
J. D. Fast, J. Allan, R. Bahreini, J. Craven, L. Emmons, R. Ferrare, P. L. Hayes, A. Hodzic, J. Holloway, C. Hostetler, J. L. Jimenez, H. Jonsson, S. Liu, Y. Liu, A. Metcalf, A. Middlebrook, J. Nowak, M. Pekour, A. Perring, L. Russell, A. Sedlacek, J. Seinfeld, A. Setyan, J. Shilling, M. Shrivastava, S. Springston, C. Song, R. Subramanian, J. W. Taylor, V. Vinoj, Q. Yang, R. A. Zaveri, and Q. Zhang
Atmos. Chem. Phys., 14, 10013–10060, https://doi.org/10.5194/acp-14-10013-2014, https://doi.org/10.5194/acp-14-10013-2014, 2014
V. H. Almanza, L. T. Molina, G. Li, J. Fast, and G. Sosa
Atmos. Chem. Phys., 14, 8483–8499, https://doi.org/10.5194/acp-14-8483-2014, https://doi.org/10.5194/acp-14-8483-2014, 2014
C. R. Terai, C. S. Bretherton, R. Wood, and G. Painter
Atmos. Chem. Phys., 14, 8071–8088, https://doi.org/10.5194/acp-14-8071-2014, https://doi.org/10.5194/acp-14-8071-2014, 2014
C. Knote, A. Hodzic, J. L. Jimenez, R. Volkamer, J. J. Orlando, S. Baidar, J. Brioude, J. Fast, D. R. Gentner, A. H. Goldstein, P. L. Hayes, W. B. Knighton, H. Oetjen, A. Setyan, H. Stark, R. Thalman, G. Tyndall, R. Washenfelder, E. Waxman, and Q. Zhang
Atmos. Chem. Phys., 14, 6213–6239, https://doi.org/10.5194/acp-14-6213-2014, https://doi.org/10.5194/acp-14-6213-2014, 2014
A. J. Scarino, M. D. Obland, J. D. Fast, S. P. Burton, R. A. Ferrare, C. A. Hostetler, L. K. Berg, B. Lefer, C. Haman, J. W. Hair, R. R. Rogers, C. Butler, A. L. Cook, and D. B. Harper
Atmos. Chem. Phys., 14, 5547–5560, https://doi.org/10.5194/acp-14-5547-2014, https://doi.org/10.5194/acp-14-5547-2014, 2014
S. G. Howell, A. D. Clarke, S. Freitag, C. S. McNaughton, V. Kapustin, V. Brekovskikh, J.-L. Jimenez, and M. J. Cubison
Atmos. Chem. Phys., 14, 5073–5087, https://doi.org/10.5194/acp-14-5073-2014, https://doi.org/10.5194/acp-14-5073-2014, 2014
G. W. Mann, K. S. Carslaw, C. L. Reddington, K. J. Pringle, M. Schulz, A. Asmi, D. V. Spracklen, D. A. Ridley, M. T. Woodhouse, L. A. Lee, K. Zhang, S. J. Ghan, R. C. Easter, X. Liu, P. Stier, Y. H. Lee, P. J. Adams, H. Tost, J. Lelieveld, S. E. Bauer, K. Tsigaridis, T. P. C. van Noije, A. Strunk, E. Vignati, N. Bellouin, M. Dalvi, C. E. Johnson, T. Bergman, H. Kokkola, K. von Salzen, F. Yu, G. Luo, A. Petzold, J. Heintzenberg, A. Clarke, J. A. Ogren, J. Gras, U. Baltensperger, U. Kaminski, S. G. Jennings, C. D. O'Dowd, R. M. Harrison, D. C. S. Beddows, M. Kulmala, Y. Viisanen, V. Ulevicius, N. Mihalopoulos, V. Zdimal, M. Fiebig, H.-C. Hansson, E. Swietlicki, and J. S. Henzing
Atmos. Chem. Phys., 14, 4679–4713, https://doi.org/10.5194/acp-14-4679-2014, https://doi.org/10.5194/acp-14-4679-2014, 2014
J. P. Mulcahy, D. N. Walters, N. Bellouin, and S. F. Milton
Atmos. Chem. Phys., 14, 4749–4778, https://doi.org/10.5194/acp-14-4749-2014, https://doi.org/10.5194/acp-14-4749-2014, 2014
P.-L. Ma, P. J. Rasch, J. D. Fast, R. C. Easter, W. I. Gustafson Jr., X. Liu, S. J. Ghan, and B. Singh
Geosci. Model Dev., 7, 755–778, https://doi.org/10.5194/gmd-7-755-2014, https://doi.org/10.5194/gmd-7-755-2014, 2014
V. Cesnulyte, A. V. Lindfors, M. R. A. Pitkänen, K. E. J. Lehtinen, J.-J. Morcrette, and A. Arola
Atmos. Chem. Phys., 14, 593–608, https://doi.org/10.5194/acp-14-593-2014, https://doi.org/10.5194/acp-14-593-2014, 2014
S. Freitag, A. D. Clarke, S. G. Howell, V. N. Kapustin, T. Campos, V. L. Brekhovskikh, and J. Zhou
Atmos. Meas. Tech., 7, 107–128, https://doi.org/10.5194/amt-7-107-2014, https://doi.org/10.5194/amt-7-107-2014, 2014
A. Baklanov, K. Schlünzen, P. Suppan, J. Baldasano, D. Brunner, S. Aksoyoglu, G. Carmichael, J. Douros, J. Flemming, R. Forkel, S. Galmarini, M. Gauss, G. Grell, M. Hirtl, S. Joffre, O. Jorba, E. Kaas, M. Kaasik, G. Kallos, X. Kong, U. Korsholm, A. Kurganskiy, J. Kushta, U. Lohmann, A. Mahura, A. Manders-Groot, A. Maurizi, N. Moussiopoulos, S. T. Rao, N. Savage, C. Seigneur, R. S. Sokhi, E. Solazzo, S. Solomos, B. Sørensen, G. Tsegas, E. Vignati, B. Vogel, and Y. Zhang
Atmos. Chem. Phys., 14, 317–398, https://doi.org/10.5194/acp-14-317-2014, https://doi.org/10.5194/acp-14-317-2014, 2014
P. E. Saide, G. R. Carmichael, Z. Liu, C. S. Schwartz, H. C. Lin, A. M. da Silva, and E. Hyer
Atmos. Chem. Phys., 13, 10425–10444, https://doi.org/10.5194/acp-13-10425-2013, https://doi.org/10.5194/acp-13-10425-2013, 2013
R. C. Moffet, T. C. Rödel, S. T. Kelly, X. Y. Yu, G. T. Carroll, J. Fast, R. A. Zaveri, A. Laskin, and M. K. Gilles
Atmos. Chem. Phys., 13, 10445–10459, https://doi.org/10.5194/acp-13-10445-2013, https://doi.org/10.5194/acp-13-10445-2013, 2013
M. Lefèvre, A. Oumbe, P. Blanc, B. Espinar, B. Gschwind, Z. Qu, L. Wald, M. Schroedter-Homscheidt, C. Hoyer-Klick, A. Arola, A. Benedetti, J. W. Kaiser, and J.-J. Morcrette
Atmos. Meas. Tech., 6, 2403–2418, https://doi.org/10.5194/amt-6-2403-2013, https://doi.org/10.5194/amt-6-2403-2013, 2013
A. D. Clarke, S. Freitag, R. M. C. Simpson, J. G. Hudson, S. G. Howell, V. L. Brekhovskikh, T. Campos, V. N. Kapustin, and J. Zhou
Atmos. Chem. Phys., 13, 7511–7529, https://doi.org/10.5194/acp-13-7511-2013, https://doi.org/10.5194/acp-13-7511-2013, 2013
R. Blot, A. D. Clarke, S. Freitag, V. Kapustin, S. G. Howell, J. B. Jensen, L. M. Shank, C. S. McNaughton, and V. Brekhovskikh
Atmos. Chem. Phys., 13, 7263–7278, https://doi.org/10.5194/acp-13-7263-2013, https://doi.org/10.5194/acp-13-7263-2013, 2013
R. C. George, R. Wood, C. S. Bretherton, and G. Painter
Atmos. Chem. Phys., 13, 6305–6328, https://doi.org/10.5194/acp-13-6305-2013, https://doi.org/10.5194/acp-13-6305-2013, 2013
P. Nabat, S. Somot, M. Mallet, I. Chiapello, J. J. Morcrette, F. Solmon, S. Szopa, F. Dulac, W. Collins, S. Ghan, L. W. Horowitz, J. F. Lamarque, Y. H. Lee, V. Naik, T. Nagashima, D. Shindell, and R. Skeie
Atmos. Meas. Tech., 6, 1287–1314, https://doi.org/10.5194/amt-6-1287-2013, https://doi.org/10.5194/amt-6-1287-2013, 2013
J. L. Thomas, J.-C. Raut, K. S. Law, L. Marelle, G. Ancellet, F. Ravetta, J. D. Fast, G. Pfister, L. K. Emmons, G. S. Diskin, A. Weinheimer, A. Roiger, and H. Schlager
Atmos. Chem. Phys., 13, 3825–3848, https://doi.org/10.5194/acp-13-3825-2013, https://doi.org/10.5194/acp-13-3825-2013, 2013
C. H. Twohy, J. R. Anderson, D. W. Toohey, M. Andrejczuk, A. Adams, M. Lytle, R. C. George, R. Wood, P. Saide, S. Spak, P. Zuidema, and D. Leon
Atmos. Chem. Phys., 13, 2541–2562, https://doi.org/10.5194/acp-13-2541-2013, https://doi.org/10.5194/acp-13-2541-2013, 2013
N. Bellouin, J. Quaas, J.-J. Morcrette, and O. Boucher
Atmos. Chem. Phys., 13, 2045–2062, https://doi.org/10.5194/acp-13-2045-2013, https://doi.org/10.5194/acp-13-2045-2013, 2013
J. E. Shilling, R. A. Zaveri, J. D. Fast, L. Kleinman, M. L. Alexander, M. R. Canagaratna, E. Fortner, J. M. Hubbe, J. T. Jayne, A. Sedlacek, A. Setyan, S. Springston, D. R. Worsnop, and Q. Zhang
Atmos. Chem. Phys., 13, 2091–2113, https://doi.org/10.5194/acp-13-2091-2013, https://doi.org/10.5194/acp-13-2091-2013, 2013
M. Huang, G. R. Carmichael, T. Chai, R. B. Pierce, S. J. Oltmans, D. A. Jaffe, K. W. Bowman, A. Kaduwela, C. Cai, S. N. Spak, A. J. Weinheimer, L. G. Huey, and G. S. Diskin
Atmos. Chem. Phys., 13, 359–391, https://doi.org/10.5194/acp-13-359-2013, https://doi.org/10.5194/acp-13-359-2013, 2013
Related subject area
Subject: Clouds and Precipitation | Research Activity: Atmospheric Modelling | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Warm and moist air intrusions into the winter Arctic: a Lagrangian view on the near-surface energy budgets
Convective updrafts near sea-breeze fronts
Evaluation of modelled summertime convective storms using polarimetric radar observations
Evaluating seasonal and regional distribution of snowfall in regional climate model simulations in the Arctic
Modeling impacts of ice-nucleating particles from marine aerosols on mixed-phase orographic clouds during 2015 ACAPEX field campaign
Influences of an entrainment–mixing parameterization on numerical simulations of cumulus and stratocumulus clouds
Investigation of ice cloud modeling capabilities for the irregularly shaped Voronoi ice scattering models in climate simulations
Assessing the potential for simplification in global climate model cloud microphysics
Technical note: Parameterising cloud base updraft velocity of marine stratocumuli
Radiative and microphysical responses of clouds to an anomalous increase in fire particles over the Maritime Continent in 2015
Intricate relations among particle collision, relative motion and clustering in turbulent clouds: computational observation and theory
The effect of marine ice-nucleating particles on mixed-phase clouds
A strong statistical link between aerosol indirect effects and the self-similarity of rainfall distributions
Quantifying albedo susceptibility biases in shallow clouds
Primary and secondary ice production: interactions and their relative importance
Microphysical processes producing high ice water contents (HIWCs) in tropical convective clouds during the HAIC-HIWC field campaign: dominant role of secondary ice production
Importance of aerosols and shape of the cloud droplet size distribution for convective clouds and precipitation
Secondary ice production processes in wintertime alpine mixed-phase clouds
Multi-thermals and high concentrations of secondary ice: a modelling study of convective clouds during the Ice in Clouds Experiment – Dust (ICE-D) campaign
Arctic mixed-phase clouds sometimes dissipate due to insufficient aerosol: evidence from observations and idealized simulations
Subgrid-scale horizontal and vertical variation of cloud water in stratocumulus clouds: a case study based on LES and comparisons with in situ observations
A vertical transport window of water vapor in the troposphere over the Tibetan Plateau with implications for global climate change
Impact of Holuhraun volcano aerosols on clouds in cloud-system resolving simulations
Box model trajectory studies of contrail formation using a particle-based cloud microphysics scheme
Updraft dynamics and microphysics: on the added value of the cumulus thermal reference frame in simulations of aerosol–deep convection interactions
Demistify: a large-eddy simulation (LES) and single-column model (SCM) intercomparison of radiation fog
Case study of a moisture intrusion over the Arctic with the ICOsahedral Non-hydrostatic (ICON) model: resolution dependence of its representation
New investigations on homogeneous ice nucleation: the effects of water activity and water saturation formulations
Cloud droplet formation at the base of tropical convective clouds: closure between modeling and measurement results of ACRIDICON–CHUVA
Impacts of long-range-transported mineral dust on summertime convective cloud and precipitation: a case study over the Taiwan region
Model emulation to understand the joint effects of ice-nucleating particles and secondary ice production on deep convective anvil cirrus
Improving the representation of aggregation in a two-moment microphysical scheme with statistics of multi-frequency Doppler radar observations
Overview towards improved understanding of the mechanisms leading to heavy precipitation in the western Mediterranean: lessons learned from HyMeX
Midlatitude mixed-phase stratocumulus clouds and their interactions with aerosols: how ice processes affect microphysical, dynamic, and thermodynamic development in those clouds and interactions?
Tracking the influence of cloud condensation nuclei on summer diurnal precipitating systems over complex topography in Taiwan
Revisiting adiabatic fraction estimations in cumulus clouds: high-resolution simulations with a passive tracer
Impact of hygroscopic seeding on the initiation of precipitation formation: results of a hybrid bin microphysics parcel model
Aerosol–cloud interactions: the representation of heterogeneous ice activation in cloud models
Sensitivity of precipitation formation to secondary ice production in winter orographic mixed-phase clouds
Environmental sensitivities of shallow-cumulus dilution – Part 2: Vertical wind profile
Supersaturation, buoyancy, and deep convection dynamics
How does the Environment Modulate Aerosol Impacts on Tropical Sea Breeze Convective Systems?
Statistical properties of a stochastic model of eddy hopping
Understanding the model representation of clouds based on visible and infrared satellite observations
Impact of high- and low-vorticity turbulence on cloud–environment mixing and cloud microphysics processes
Preconditioning of overcast-to-broken cloud transitions by riming in marine cold air outbreaks
Aitken mode particles as CCN in aerosol- and updraft-sensitive regimes of cloud droplet formation
Ice multiplication from ice–ice collisions in the high Arctic: sensitivity to ice habit, rimed fraction, ice type and uncertainties in the numerical description of the process
Contrail formation within cirrus: high-resolution simulations using ICON-LEM
The climate impact of COVID-19-induced contrail changes
Cheng You, Michael Tjernström, and Abhay Devasthale
Atmos. Chem. Phys., 22, 8037–8057, https://doi.org/10.5194/acp-22-8037-2022, https://doi.org/10.5194/acp-22-8037-2022, 2022
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In winter when solar radiation is absent in the Arctic, the poleward transport of heat and moisture into the high Arctic becomes the main contribution of Arctic warming. Over completely frozen ocean sectors, total surface energy budget is dominated by net long-wave heat, while over the Barents Sea, with an open ocean to the south, total net surface energy budget is dominated by the surface turbulent heat.
Shizuo Fu, Richard Rotunno, and Huiwen Xue
Atmos. Chem. Phys., 22, 7727–7738, https://doi.org/10.5194/acp-22-7727-2022, https://doi.org/10.5194/acp-22-7727-2022, 2022
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The convective updrafts near the sea-breeze fronts (SBFs) play important roles in initiating deep convection, but their characteristics are not well understood. By performing large-eddy simulations, we explain why the updrafts near the SBF are larger than but have similar strength to the updrafts ahead of the SBF. The results should also apply to other boundary-layer convergence zones similar to the SBF.
Prabhakar Shrestha, Silke Trömel, Raquel Evaristo, and Clemens Simmer
Atmos. Chem. Phys., 22, 7593–7618, https://doi.org/10.5194/acp-22-7593-2022, https://doi.org/10.5194/acp-22-7593-2022, 2022
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The study makes use of ensemble numerical simulations with forward operator to evaluate the simulated cloud and precipitation processes with radar observations. While comparing model data with radar has its own challenges due to errors in the forward operator and processed radar measurements, the model was generally found to underestimate the high reflectivity, width/magnitude (value) of ZDR columns and high precipitation.
Annakaisa von Lerber, Mario Mech, Annette Rinke, Damao Zhang, Melanie Lauer, Ana Radovan, Irina Gorodetskaya, and Susanne Crewell
Atmos. Chem. Phys., 22, 7287–7317, https://doi.org/10.5194/acp-22-7287-2022, https://doi.org/10.5194/acp-22-7287-2022, 2022
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Snowfall is an important climate indicator. However, microphysical snowfall processes are challenging for atmospheric models. In this study, the performance of a regional climate model is evaluated in modeling the spatial and temporal distribution of Arctic snowfall when compared to CloudSat satellite observations. Excellent agreement in averaged annual snowfall rates is found, and the shown methodology offers a promising diagnostic tool to investigate the shown differences further.
Yun Lin, Jiwen Fan, Pengfei Li, Lai-yung Ruby Leung, Paul J. DeMott, Lexie Goldberger, Jennifer Comstock, Ying Liu, Jong-Hoon Jeong, and Jason Tomlinson
Atmos. Chem. Phys., 22, 6749–6771, https://doi.org/10.5194/acp-22-6749-2022, https://doi.org/10.5194/acp-22-6749-2022, 2022
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How sea spray aerosols may affect cloud and precipitation over the region by acting as ice-nucleating particles (INPs) is unknown. We explored the effects of INPs from marine aerosols on orographic cloud and precipitation for an atmospheric river event observed during the 2015 ACAPEX field campaign. The marine INPs enhance the formation of ice and snow, leading to less shallow warm clouds but more mixed-phase and deep clouds. This work suggests models need to consider the impacts of marine INPs.
Xiaoqi Xu, Chunsong Lu, Yangang Liu, Shi Luo, Xin Zhou, Satoshi Endo, Lei Zhu, and Yuan Wang
Atmos. Chem. Phys., 22, 5459–5475, https://doi.org/10.5194/acp-22-5459-2022, https://doi.org/10.5194/acp-22-5459-2022, 2022
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A new entrainment–mixing parameterization which can be directly implemented in microphysics schemes without requiring the relative humidity of the entrained air is proposed based on the explicit mixing parcel model. The parameterization is implemented in the two-moment microphysics scheme and exhibits different effects on different types of clouds and even on different stages of stratocumulus clouds, which are affected by turbulent dissipation rate and aerosol concentration.
Ming Li, Husi Letu, Yiran Peng, Hiroshi Ishimoto, Yanluan Lin, Takashi Y. Nakajima, Anthony J. Baran, Zengyuan Guo, Yonghui Lei, and Jiancheng Shi
Atmos. Chem. Phys., 22, 4809–4825, https://doi.org/10.5194/acp-22-4809-2022, https://doi.org/10.5194/acp-22-4809-2022, 2022
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To build on the previous investigations of the Voronoi model in the remote sensing retrievals of ice cloud products, this paper developed an ice cloud parameterization scheme based on the single-scattering properties of the Voronoi model and evaluate it through simulations with the Community Integrated Earth System Model (CIESM). Compared with four representative ice cloud schemes, results show that the Voronoi model has good capabilities of ice cloud modeling in the climate model.
Ulrike Proske, Sylvaine Ferrachat, David Neubauer, Martin Staab, and Ulrike Lohmann
Atmos. Chem. Phys., 22, 4737–4762, https://doi.org/10.5194/acp-22-4737-2022, https://doi.org/10.5194/acp-22-4737-2022, 2022
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Cloud microphysical processes shape cloud properties and are therefore important to represent in climate models. Their parameterization has grown more complex, making the model results more difficult to interpret. Using sensitivity analysis we test how the global aerosol–climate model ECHAM-HAM reacts to changes to these parameterizations. The model is sensitive to the parameterization of ice crystal autoconversion but not to, e.g., self-collection, suggesting that it may be simplified.
Jaakko Ahola, Tomi Raatikainen, Muzaffer Ege Alper, Jukka-Pekka Keskinen, Harri Kokkola, Antti Kukkurainen, Antti Lipponen, Jia Liu, Kalle Nordling, Antti-Ilari Partanen, Sami Romakkaniemi, Petri Räisänen, Juha Tonttila, and Hannele Korhonen
Atmos. Chem. Phys., 22, 4523–4537, https://doi.org/10.5194/acp-22-4523-2022, https://doi.org/10.5194/acp-22-4523-2022, 2022
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Clouds are important for the climate, and cloud droplets have a significant role in cloud properties. Cloud droplets form when air rises and cools and water vapour condenses on small particles that can be natural or of anthropogenic origin. Currently, the updraft velocity, meaning how fast the air rises, is poorly represented in global climate models. In our study, we show three methods that will improve the depiction of updraft velocity and which properties are vital to updrafts.
Azusa Takeishi and Chien Wang
Atmos. Chem. Phys., 22, 4129–4147, https://doi.org/10.5194/acp-22-4129-2022, https://doi.org/10.5194/acp-22-4129-2022, 2022
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Nanometer- to micrometer-sized particles in the atmosphere, namely aerosols, play a crucial role in cloud formation as cloud droplets form on aerosols. This study uses a weather forecasting model to examine the impacts of a large emission of aerosol particles from biomass burning activities over Southeast Asia. We find that additional cloud droplets brought by fire-emitted particles can lead to taller and more reflective convective clouds with increased rainfall.
Ewe-Wei Saw and Xiaohui Meng
Atmos. Chem. Phys., 22, 3779–3788, https://doi.org/10.5194/acp-22-3779-2022, https://doi.org/10.5194/acp-22-3779-2022, 2022
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Collision–coagulation of small droplets in turbulent clouds leads to the production of rain. Turbulence causes droplet clustering and higher relative droplet velocities, and these should enhance the collision–coagulation rate. We find, surprisingly, that collision–coagulation starkly diminishes clustering and strongly alters relative velocities. We provide a theory that explains this result. Our results call for a new perspective on how we understand particle/droplet collision in clouds.
Tomi Raatikainen, Marje Prank, Jaakko Ahola, Harri Kokkola, Juha Tonttila, and Sami Romakkaniemi
Atmos. Chem. Phys., 22, 3763–3778, https://doi.org/10.5194/acp-22-3763-2022, https://doi.org/10.5194/acp-22-3763-2022, 2022
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Mineral dust or similar ice-nucleating particles (INPs) are needed to initiate cloud droplet freezing at temperatures common in shallow clouds. In this work we examine how INPs that are released from the sea surface impact marine clouds. Our high-resolution simulations show that turbulent updraughts carry these particles effectively up to the clouds, where they initiate cloud droplet freezing. Sea surface INP emissions become more important with decreasing background dust INP concentrations.
Kalli Furtado and Paul Field
Atmos. Chem. Phys., 22, 3391–3407, https://doi.org/10.5194/acp-22-3391-2022, https://doi.org/10.5194/acp-22-3391-2022, 2022
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The complex processes involved mean that no simple answer to this
question has so far been discovered: do aerosols increase or decrease precipitation? Using high-resolution weather simulations, we find a self-similar property of rainfall that is not affected by aerosols. Using this invariant, we can collapse all our simulations to a single curve. So, although aerosol effects on rain are many, there may be a universal constraint on the number of degrees of freedom needed to represent them.
Graham Feingold, Tom Goren, and Takanobu Yamaguchi
Atmos. Chem. Phys., 22, 3303–3319, https://doi.org/10.5194/acp-22-3303-2022, https://doi.org/10.5194/acp-22-3303-2022, 2022
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The evaluation of radiative forcing associated with aerosol–cloud interactions remains a significant source of uncertainty in future climate projections. Using high-resolution numerical model output, we mimic typical satellite retrieval methodologies to show that data aggregation can introduce significant error (hundreds of percent) in the cloud albedo susceptibility metric. Spatial aggregation errors tend to be countered by temporal aggregation errors.
Xi Zhao and Xiaohong Liu
Atmos. Chem. Phys., 22, 2585–2600, https://doi.org/10.5194/acp-22-2585-2022, https://doi.org/10.5194/acp-22-2585-2022, 2022
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The goal of this study is to investigate the relative importance and interactions of primary and secondary ice production in the Arctic mixed-phase clouds. Our results show that the SIP is not only a result of ice crystals produced from ice nucleation, but also competes with the ice production; conversely, strong ice nucleation also suppresses SIP.
Yongjie Huang, Wei Wu, Greg M. McFarquhar, Ming Xue, Hugh Morrison, Jason Milbrandt, Alexei V. Korolev, Yachao Hu, Zhipeng Qu, Mengistu Wolde, Cuong Nguyen, Alfons Schwarzenboeck, and Ivan Heckman
Atmos. Chem. Phys., 22, 2365–2384, https://doi.org/10.5194/acp-22-2365-2022, https://doi.org/10.5194/acp-22-2365-2022, 2022
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Numerous small ice crystals in tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. Previous numerical simulations failed to reproduce this phenomenon and hypothesized that key microphysical processes are still lacking in current models to realistically simulate the phenomenon. This study uses numerical experiments to confirm the dominant role of secondary ice production in the formation of these large numbers of small ice crystals.
Christian Barthlott, Amirmahdi Zarboo, Takumi Matsunobu, and Christian Keil
Atmos. Chem. Phys., 22, 2153–2172, https://doi.org/10.5194/acp-22-2153-2022, https://doi.org/10.5194/acp-22-2153-2022, 2022
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The relative impact of cloud condensation nuclei (CCN) concentrations and the shape parameter of the cloud droplet size distribution is evaluated in realistic convection-resolving simulations. We find that an increase in the shape parameter can produce almost as large a variation in precipitation as a CCN increase from maritime to polluted conditions. The choice of the shape parameter may be more important than previously thought for determining cloud radiative characteristics.
Paraskevi Georgakaki, Georgia Sotiropoulou, Étienne Vignon, Anne-Claire Billault-Roux, Alexis Berne, and Athanasios Nenes
Atmos. Chem. Phys., 22, 1965–1988, https://doi.org/10.5194/acp-22-1965-2022, https://doi.org/10.5194/acp-22-1965-2022, 2022
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The modelling study focuses on the importance of ice multiplication processes in orographic mixed-phase clouds, which is one of the least understood cloud types in the climate system. We show that the consideration of ice seeding and secondary ice production through ice–ice collisional breakup is essential for correct predictions of precipitation in mountainous terrain, with important implications for radiation processes.
Zhiqiang Cui, Alan Blyth, Yahui Huang, Gary Lloyd, Thomas Choularton, Keith Bower, Paul Field, Rachel Hawker, and Lindsay Bennett
Atmos. Chem. Phys., 22, 1649–1667, https://doi.org/10.5194/acp-22-1649-2022, https://doi.org/10.5194/acp-22-1649-2022, 2022
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High concentrations of ice particles were observed at temperatures greater than about –8 C. The default scheme of the secondary ice production cannot explain the high concentrations. Relaxing the conditions for secondary ice production or considering dust aerosol alone is insufficient to produce the observed amount of ice particles. It is likely that multi-thermals play an important role in producing very high concentrations of secondary ice particles in some tropical clouds.
Lucas J. Sterzinger, Joseph Sedlar, Heather Guy, Ryan R. Neely III, and Adele L. Igel
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-36, https://doi.org/10.5194/acp-2022-36, 2022
Revised manuscript accepted for ACP
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Aerosol particles are required for cloud droplets to form. The Arctic atmosphere often has much fewer aerosol than at lower latitudes. In this study, we investigate whether aerosol concentrations can drop so low as to no longer support a cloud. We use observations to initialize idealized model simulations to investigate a "worse case scenario" where all aerosol are removed from the environment instantaneously. We find that this mechanism is possible in two cases and unlikely in the third.
Justin A. Covert, David B. Mechem, and Zhibo Zhang
Atmos. Chem. Phys., 22, 1159–1174, https://doi.org/10.5194/acp-22-1159-2022, https://doi.org/10.5194/acp-22-1159-2022, 2022
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Stratocumulus play an important role in Earth's radiative balance. The simulation of these cloud systems in climate models is difficult due to the scale at which cloud microphysical processes occur compared with model grid sizes. In this study, we use large-eddy simulation to analyze subgrid-scale variability of cloud water and its implications on a cloud water to drizzle model enhancement factor E. We find current values of E may be too large and that E should be vertically dependent in models.
Xiangde Xu, Chan Sun, Deliang Chen, Tianliang Zhao, Jianjun Xu, Shengjun Zhang, Juan Li, Bin Chen, Yang Zhao, Hongxiong Xu, Lili Dong, Xiaoyun Sun, and Yan Zhu
Atmos. Chem. Phys., 22, 1149–1157, https://doi.org/10.5194/acp-22-1149-2022, https://doi.org/10.5194/acp-22-1149-2022, 2022
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A vertical transport window of tropospheric vapor exists on the Tibetan Plateau (TP). The TP's thermal forcing drives the vertical transport
windowof vapor in the troposphere. The effects of the TP's vertical transport window of vapor are of importance in global climate change.
Mahnoosh Haghighatnasab, Jan Kretzschmar, Karoline Block, and Johannes Quaas
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-38, https://doi.org/10.5194/acp-2022-38, 2022
Revised manuscript accepted for ACP
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The impact of aerosols emitted by the Holuhraun volcanic eruption on liquid clouds was assessed from a pair of cloud-system resolving simulations along with satellite retrievals. Inside and outside the plume were compared in terms of their statistical distributions. Analyses indicated enhancement for cloud droplet number concentration inside the volcano plume in model simulations and satellite retrievals while there was on average a small effect on both liquid water path and cloud fraction.
Andreas Bier, Simon Unterstrasser, and Xavier Vancassel
Atmos. Chem. Phys., 22, 823–845, https://doi.org/10.5194/acp-22-823-2022, https://doi.org/10.5194/acp-22-823-2022, 2022
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We investigate contrail formation in an aircraft plume with a particle-based multi-trajectory 0D model. Due to the high plume heterogeneity, contrail ice crystals form first near the plume edge and then in the plume centre. The number of ice crystals varies strongly with ambient conditions and soot properties near the contrail formation threshold. Our results imply that the multi-trajectory approach does not necessarily lead to improved scientific results compared to a single mean trajectory.
Daniel Hernandez-Deckers, Toshihisa Matsui, and Ann M. Fridlind
Atmos. Chem. Phys., 22, 711–724, https://doi.org/10.5194/acp-22-711-2022, https://doi.org/10.5194/acp-22-711-2022, 2022
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We investigate how the concentration of aerosols (small particles that serve as seeds for cloud droplets) affect the dynamics of simulated clouds using two different frameworks, i.e., the traditional selection of cloudy rising grid points and tracking small-scale coherent rising features (cumulus thermals). By doing so, we find that these cumulus thermals reveal useful information about the coupling between internal cloud circulations and cloud droplet and raindrop formation.
Ian Boutle, Wayne Angevine, Jian-Wen Bao, Thierry Bergot, Ritthik Bhattacharya, Andreas Bott, Leo Ducongé, Richard Forbes, Tobias Goecke, Evelyn Grell, Adrian Hill, Adele L. Igel, Innocent Kudzotsa, Christine Lac, Bjorn Maronga, Sami Romakkaniemi, Juerg Schmidli, Johannes Schwenkel, Gert-Jan Steeneveld, and Benoît Vié
Atmos. Chem. Phys., 22, 319–333, https://doi.org/10.5194/acp-22-319-2022, https://doi.org/10.5194/acp-22-319-2022, 2022
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Fog forecasting is one of the biggest problems for numerical weather prediction. By comparing many models used for fog forecasting with others used for fog research, we hoped to help guide forecast improvements. We show some key processes that, if improved, will help improve fog forecasting, such as how water is deposited on the ground. We also showed that research models were not themselves a suitable baseline for comparison, and we discuss what future observations are required to improve them.
Hélène Bresson, Annette Rinke, Mario Mech, Daniel Reinert, Vera Schemann, Kerstin Ebell, Marion Maturilli, Carolina Viceto, Irina Gorodetskaya, and Susanne Crewell
Atmos. Chem. Phys., 22, 173–196, https://doi.org/10.5194/acp-22-173-2022, https://doi.org/10.5194/acp-22-173-2022, 2022
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Arctic warming is pronounced, and one factor in this is the poleward atmospheric transport of heat and moisture. This study assesses the 4D structure of an Arctic moisture intrusion event which occurred in June 2017. For the first time, high-resolution pan-Arctic ICON simulations are performed and compared with global models, reanalysis, and observations. Results show the added value of high resolution in the event representation and the impact of the intrusion on the surface energy fluxes.
Manuel Baumgartner, Christian Rolf, Jens-Uwe Grooß, Julia Schneider, Tobias Schorr, Ottmar Möhler, Peter Spichtinger, and Martina Krämer
Atmos. Chem. Phys., 22, 65–91, https://doi.org/10.5194/acp-22-65-2022, https://doi.org/10.5194/acp-22-65-2022, 2022
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An important mechanism for the appearance of ice particles in the upper troposphere at low temperatures is homogeneous nucleation. This process is commonly described by the
Koop line, predicting the humidity at freezing. However, laboratory measurements suggest that the freezing humidities are above the Koop line, motivating the present study to investigate the influence of different physical parameterizations on the homogeneous freezing with the help of a detailed numerical model.
Ramon Campos Braga, Barbara Ervens, Daniel Rosenfeld, Meinrat O. Andreae, Jan-David Förster, Daniel Fütterer, Lianet Hernández Pardo, Bruna A. Holanda, Tina Jurkat-Witschas, Ovid O. Krüger, Oliver Lauer, Luiz A. T. Machado, Christopher Pöhlker, Daniel Sauer, Christiane Voigt, Adrian Walser, Manfred Wendisch, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 21, 17513–17528, https://doi.org/10.5194/acp-21-17513-2021, https://doi.org/10.5194/acp-21-17513-2021, 2021
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Interactions of aerosol particles with clouds represent a large uncertainty in estimates of climate change. Properties of aerosol particles control their ability to act as cloud condensation nuclei. Using aerosol measurements in the Amazon, we performed model studies to compare predicted and measured cloud droplet number concentrations at cloud bases. Our results confirm previous estimates of particle hygroscopicity in this region.
Yanda Zhang, Fangqun Yu, Gan Luo, Jiwen Fan, and Shuai Liu
Atmos. Chem. Phys., 21, 17433–17451, https://doi.org/10.5194/acp-21-17433-2021, https://doi.org/10.5194/acp-21-17433-2021, 2021
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This paper explores the impacts of dust on summertime convective cloud and precipitation through a numerical experiment. The result indicates that the long-range-transported dust can notably affect the properties of convective cloud and precipitation by enhancing immersion freezing and invigorating convection. We also analyze the different dust effects predicted by the Morrison and SBM schemes, which are partially attributed to the saturation adjustment approach utilized in the bulk schemes.
Rachel E. Hawker, Annette K. Miltenberger, Jill S. Johnson, Jonathan M. Wilkinson, Adrian A. Hill, Ben J. Shipway, Paul R. Field, Benjamin J. Murray, and Ken S. Carslaw
Atmos. Chem. Phys., 21, 17315–17343, https://doi.org/10.5194/acp-21-17315-2021, https://doi.org/10.5194/acp-21-17315-2021, 2021
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We find that ice-nucleating particles (INPs), aerosols that can initiate the freezing of cloud droplets, cause substantial changes to the properties of radiatively important convectively generated anvil cirrus. The number concentration of INPs had a large effect on ice crystal number concentration while the INP temperature dependence controlled ice crystal size and cloud fraction. The results indicate information on INP number and source is necessary for the representation of cloud glaciation.
Markus Karrer, Axel Seifert, Davide Ori, and Stefan Kneifel
Atmos. Chem. Phys., 21, 17133–17166, https://doi.org/10.5194/acp-21-17133-2021, https://doi.org/10.5194/acp-21-17133-2021, 2021
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Modeling precipitation is of great relevance, e.g., for mitigating damage caused by extreme weather. A key component in accurate precipitation modeling is aggregation, i.e., sticking together of snowflakes. Simulating aggregation is difficult due to multiple parameters that are not well-known. Knowing how these parameters affect aggregation can help its simulation. We put new parameters in the model and select a combination of parameters with which the model can simulate observations better.
Samira Khodayar, Silvio Davolio, Paolo Di Girolamo, Cindy Lebeaupin Brossier, Emmanouil Flaounas, Nadia Fourrie, Keun-Ok Lee, Didier Ricard, Benoit Vie, Francois Bouttier, Alberto Caldas-Alvarez, and Veronique Ducrocq
Atmos. Chem. Phys., 21, 17051–17078, https://doi.org/10.5194/acp-21-17051-2021, https://doi.org/10.5194/acp-21-17051-2021, 2021
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Heavy precipitation (HP) constitutes a major meteorological threat in the western Mediterranean. Every year, recurrent events affect the area with fatal consequences. Despite this being a well-known issue, open questions still remain. The understanding of the underlying mechanisms and the modeling representation of the events must be improved. In this article we present the most recent lessons learned from the Hydrological Cycle in the Mediterranean Experiment (HyMeX).
Seoung Soo Lee, Kyung-Ja Ha, Manguttathil Gopalakrishnan Manoj, Mohammad Kamruzzaman, Hyungjun Kim, Nobuyuki Utsumi, Youtong Zheng, Byung-Gon Kim, Chang Hoon Jung, Junshik Um, Jianping Guo, Kyoung Ock Choi, and Go-Un Kim
Atmos. Chem. Phys., 21, 16843–16868, https://doi.org/10.5194/acp-21-16843-2021, https://doi.org/10.5194/acp-21-16843-2021, 2021
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Using a modeling framework, a midlatitude stratocumulus cloud system is simulated. It is found that cloud mass in the system becomes very low due to interactions between ice and liquid particles compared to that in the absence of ice particles. It is also found that interactions between cloud mass and aerosols lead to a reduction in cloud mass in the system, and this is contrary to an aerosol-induced increase in cloud mass in the absence of ice particles.
Yu-Hung Chang, Wei-Ting Chen, Chien-Ming Wu, Christopher Moseley, and Chia-Chun Wu
Atmos. Chem. Phys., 21, 16709–16725, https://doi.org/10.5194/acp-21-16709-2021, https://doi.org/10.5194/acp-21-16709-2021, 2021
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The impacts of increasing cloud condensation nuclei on summertime diurnal precipitation in weak synoptic weather over complex topography in Taiwan were investigated by applying object-based tracking analyses to semi-realistic large-eddy simulations. In hotspots of orographic locking processes, rain initiation is delayed, which prolongs the development of local circulation and convection. For this organized regime, the occurrence of extreme diurnal precipitating systems is notably enhanced.
Eshkol Eytan, Ilan Koren, Orit Altaratz, Mark Pinsky, and Alexander Khain
Atmos. Chem. Phys., 21, 16203–16217, https://doi.org/10.5194/acp-21-16203-2021, https://doi.org/10.5194/acp-21-16203-2021, 2021
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Describing cloud mixing processes is among the most challenging fronts in cloud physics. Therefore, the adiabatic fraction (AF) that serves as a mixing measure is a valuable metric. We use high-resolution (10 m) simulations of single clouds with a passive tracer to test the skill of different methods used to derive AF. We highlight a method that is insensitive to the available cloud samples and allows considering microphysical effects on AF estimations in different environmental conditions.
Istvan Geresdi, Lulin Xue, Sisi Chen, Youssef Wehbe, Roelof Bruintjes, Jared A. Lee, Roy M. Rasmussen, Wojciech W. Grabowski, Noemi Sarkadi, and Sarah A. Tessendorf
Atmos. Chem. Phys., 21, 16143–16159, https://doi.org/10.5194/acp-21-16143-2021, https://doi.org/10.5194/acp-21-16143-2021, 2021
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By releasing soluble aerosols into the convective clouds, cloud seeding potentially enhances rainfall. The seeding impacts are hard to quantify with observations only. Numerical models that represent the detailed physics of aerosols, cloud and rain formation are used to investigate the seeding impacts on rain enhancement under different natural aerosol backgrounds and using different seeding materials. Our results indicate that seeding may enhance rainfall under certain conditions.
Bernd Kärcher and Claudia Marcolli
Atmos. Chem. Phys., 21, 15213–15220, https://doi.org/10.5194/acp-21-15213-2021, https://doi.org/10.5194/acp-21-15213-2021, 2021
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Aerosol–cloud interactions play an important role in climate change. Simulations of the competition between homogeneous solution droplet freezing and heterogeneous ice nucleation can be compromised by the misapplication of ice-active particle fractions frequently derived from laboratory measurements or parametrizations. Our study frames the problem and establishes a solution that is easy to implement in cloud models.
Zane Dedekind, Annika Lauber, Sylvaine Ferrachat, and Ulrike Lohmann
Atmos. Chem. Phys., 21, 15115–15134, https://doi.org/10.5194/acp-21-15115-2021, https://doi.org/10.5194/acp-21-15115-2021, 2021
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The RACLETS campaign combined cloud and snow research to improve the understanding of precipitation formation in clouds. A numerical weather prediction model, COSMO, was used to assess the importance of ice crystal enhancement by ice–ice collisions for cloud properties. We found that the number of ice crystals increased by 1 to 3 orders of magnitude when ice–ice collisions were permitted to occur, reducing localized regions of high precipitation and, thereby, improving the model performance.
Sonja Drueke, Daniel J. Kirshbaum, and Pavlos Kollias
Atmos. Chem. Phys., 21, 14039–14058, https://doi.org/10.5194/acp-21-14039-2021, https://doi.org/10.5194/acp-21-14039-2021, 2021
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This numerical study provides insights into the sensitivity of shallow-cumulus dilution to geostrophic vertical wind profile. The cumulus dilution is strongly sensitive to vertical wind shear in the cloud layer, with shallow cumuli being more diluted in sheared environments. On the other hand, wind shear in the subcloud layer leads to less diluted cumuli. The sensitivities are explained by jointly considering the impacts of vertical velocity and the properties of the entrained air.
Wojciech W. Grabowski and Hugh Morrison
Atmos. Chem. Phys., 21, 13997–14018, https://doi.org/10.5194/acp-21-13997-2021, https://doi.org/10.5194/acp-21-13997-2021, 2021
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The paper provides a discussion of key elements of moist convective dynamics: cloud buoyancy, latent heating, precipitation, and entrainment. The motivation comes from recent discussions concerning differences in convective dynamics in polluted and pristine environments.
J. Minnie Park and Susan C. van den Heever
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-693, https://doi.org/10.5194/acp-2021-693, 2021
Revised manuscript accepted for ACP
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This study explores how increased aerosol particles impact tropical sea breeze cloud systems under different environments and how a range of environments modulate these cloud responses. Overall, sea breeze flows and clouds that develop therein become weaker due to interactions between aerosols, sunlight, and land surface. In addition, surface rainfall also decreases with more aerosol particles. Weakening of cloud and rain with more aerosols are found irrespective of 130 different environments.
Izumi Saito, Takeshi Watanabe, and Toshiyuki Gotoh
Atmos. Chem. Phys., 21, 13119–13130, https://doi.org/10.5194/acp-21-13119-2021, https://doi.org/10.5194/acp-21-13119-2021, 2021
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We provide various statistical properties for the stochastic model
of eddy hopping, which is a novel cloud microphysical model that
accounts for the effect of the supersaturation fluctuation at unresolved
scales on the growth of cloud droplets and on spectral broadening
in a turbulent cloud. Our results indicate that the model can be
improved to have better fidelity to the reference data and to require
less computational cost.
Stefan Geiss, Leonhard Scheck, Alberto de Lozar, and Martin Weissmann
Atmos. Chem. Phys., 21, 12273–12290, https://doi.org/10.5194/acp-21-12273-2021, https://doi.org/10.5194/acp-21-12273-2021, 2021
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This study demonstrates the benefits of using both visible and infrared satellite channels to evaluate clouds in numerical weather prediction models. Combining these highly resolved observations provides significantly more and complementary information than using only infrared observations. The visible observations are particularly sensitive to subgrid water clouds, which are not well constrained by other observations.
Bipin Kumar, Rahul Ranjan, Man-Kong Yau, Sudarsan Bera, and Suryachandra A. Rao
Atmos. Chem. Phys., 21, 12317–12329, https://doi.org/10.5194/acp-21-12317-2021, https://doi.org/10.5194/acp-21-12317-2021, 2021
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The characteristics of turbulent clouds are affected by the entrainment of ambient dry air and its subsequent mixing. A turbulent flow generates vorticities of different intensities, and regions with high vorticity (HV) and low vorticity (LV) exist. This study provides a detailed analysis of different properties of turbulent flows and cloud droplets in the HV and LV regions in order to understand the impact of vorticity production on cloud microphysical and mixing processes.
Florian Tornow, Andrew S. Ackerman, and Ann M. Fridlind
Atmos. Chem. Phys., 21, 12049–12067, https://doi.org/10.5194/acp-21-12049-2021, https://doi.org/10.5194/acp-21-12049-2021, 2021
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Cold air outbreaks affect the local energy budget by forming bright boundary layer clouds that, once it rains, evolve into dimmer, broken cloud fields that are depleted of condensation nuclei – an evolution consistent with closed-to-open cell transitions. We find that cloud ice accelerates this evolution, primarily via riming prior to rain onset, which (1) reduces liquid water, (2) reduces condensation nuclei, and (3) leads to early precipitation cooling and moistening below cloud.
Mira L. Pöhlker, Minghui Zhang, Ramon Campos Braga, Ovid O. Krüger, Ulrich Pöschl, and Barbara Ervens
Atmos. Chem. Phys., 21, 11723–11740, https://doi.org/10.5194/acp-21-11723-2021, https://doi.org/10.5194/acp-21-11723-2021, 2021
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Clouds cool our atmosphere. The role of small aerosol particles in affecting them represents one of the largest uncertainties in current estimates of climate change. Traditionally it is assumed that cloud droplets only form particles of diameters ~ 100 nm (
accumulation mode). Previous studies suggest that this can also occur in smaller particles (
Aitken mode). Our study provides a general framework to estimate under which aerosol and cloud conditions Aitken mode particles affect clouds.
Georgia Sotiropoulou, Luisa Ickes, Athanasios Nenes, and Annica M. L. Ekman
Atmos. Chem. Phys., 21, 9741–9760, https://doi.org/10.5194/acp-21-9741-2021, https://doi.org/10.5194/acp-21-9741-2021, 2021
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Mixed-phase clouds are a large source of uncertainty in projections of the Arctic climate. This is partly due to the poor representation of the cloud ice formation processes. Implementing a parameterization for ice multiplication due to mechanical breakup upon collision of two ice particles in a high-resolution model improves cloud ice phase representation; however, cloud liquid remains overestimated.
Pooja Verma and Ulrike Burkhardt
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-497, https://doi.org/10.5194/acp-2021-497, 2021
Revised manuscript accepted for ACP
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This paper investigates contrail ice formation within cirrus and the impact of natural cirrus on the contrail formation in the high-resolution ICON-LEM over Germany. The formation of contrail ice crystals often leads to changes in cirrus ice crystal number concentrations of a few orders of magnitude. Contrail formation is affected by pre-existing cirrus leading to increased ice nucleation rates and larger ice crystal survival rate specifically in optically thick cirrus.
Andrew Gettelman, Chieh-Chieh Chen, and Charles G. Bardeen
Atmos. Chem. Phys., 21, 9405–9416, https://doi.org/10.5194/acp-21-9405-2021, https://doi.org/10.5194/acp-21-9405-2021, 2021
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The COVID-19 pandemic caused significant economic disruption in 2020 and severely impacted air traffic. We use a climate model to evaluate the effect of the reductions in aviation on climate in 2020. Contrails, in general, warm the planet, and COVID-19-related reductions in contrails cooled the land surface in 2020. The timing of reductions in aviation was important, and this may change how we think about the future effects of contrails.
Cited articles
Abdul-Razzak, H. and Ghan, S. J.: A parameterization of aerosol activation. 3. Sectional representation, J. Geophys. Res., 107, AAC 1-1–AAC 1-6, 2002.
Abel, S. J., Walters, D. N., and Allen, G.: Evaluation of stratocumulus cloud prediction in the Met Office forecast model during VOCALS-REx, Atmos. Chem. Phys., 10, 10541–10559, https://doi.org/10.5194/acp-10-10541-2010, 2010.
Ackermann, I. J., Hass, H., Memmesheimer, M., Ebel, A., Binkowski, F. S., and Shankar, U.: Modal aerosol dynamics model for Europe: development and first applications, Atmos. Environ., 32, 2981–2999, https://doi.org/10.1016/S1352-2310(98)00006-5, 1998.
Allen, G., Coe, H., Clarke, A., Bretherton, C., Wood, R., Abel, S. J., Barrett, P., Brown, P., George, R., Freitag, S., McNaughton, C., Howell, S., Shank, L., Kapustin, V., Brekhovskikh, V., Kleinman, L., Lee, Y.-N., Springston, S., Toniazzo, T., Krejci, R., Fochesatto, J., Shaw, G., Krecl, P., Brooks, B., McMeeking, G., Bower, K. N., Williams, P. I., Crosier, J., Crawford, I., Connolly, P., Allan, J. D., Covert, D., Bandy, A. R., Russell, L. M., Trembath, J., Bart, M., McQuaid, J. B., Wang, J., and Chand, D.: South East Pacific atmospheric composition and variability sampled along 20° S during VOCALS-REx, Atmos. Chem. Phys., 11, 5237–5262, https://doi.org/10.5194/acp-11-5237-2011, 2011.
Bellouin, N., Boucher, O., Haywood, J., Johnson, C., Jones, A., Rae, J., and Woodward, S.: Improved representation of aerosols for HadGEM2, Tech. Note 73, Hadley Cent, Met Office, Exeter, UK, 43 pp., 2007.
Bellouin, N., Rae, J., Jones, A., Johnson, C., Haywood, J., and Boucher., O.: Aerosol forcing in the Climate Model Intercomparison Project CMIP5 simulations by HadGEM2-ES and the role of ammonium nitrate, J. Geophys. Res., 116, D20206, https://doi.org/10.1029/2011JD016074, 2011.
Blot, R., Clarke, A. D., Freitag, S., Kapustin, V., Howell, S. G., Jensen, J. B., Shank, L. M., McNaughton, C. S., and Brekhovskikh, V.: Ultrafine sea spray aerosol over the southeastern Pacific: open-ocean contributions to marine boundary layer CCN, Atmos. Chem. Phys., 13, 7263–7278, https://doi.org/10.5194/acp-13-7263-2013, 2013.
Bond, T. C., Bhardwaj, E., Dong, R., Jogani, R., Jung, S., Roden, C., Streets, D. G., and Trautmann, N. M.: Historical emissions of black and organic carbon aerosol from energy-related combustion, 1850–2000, Global Biogeochem. Cy., 21, GB2018, https://doi.org/10.1029/2006GB002840, 2007.
Boyle, J., Klein, S., Zhang, G., Xie, S., and Wei, X.: Climate model forecast experiments for TOGA COARE., Mon. Weather Rev., 136, 808–832, https://doi.org/10.1175/2007MWR2145.1, 2008.
Bretherton, C. S. and Park, S.: A new moist turbulence parameterization in the Community Atmosphere Model, J. Climate, 22, 3422-3448, 2009.
Bretherton, C. S., Uttal, T., Fairall, C. W., Yuter, S., Weller, R., Baumgardner, D., Comstock, K., Wood, R., and Raga, G.: The EPIC 2001 stratocumulus study, B. Am. Meteorol. Soc., 85, 967–977, 2004.
Bretherton, C. S., Wood, R., George, R. C., Leon, D., Allen, G., and Zheng, X.: Southeast Pacific stratocumulus clouds, precipitation and boundary layer structure sampled along 20° S during VOCALS-REx, Atmos. Chem. Phys., 10, 10639–10654, https://doi.org/10.5194/acp-10-10639-2010, 2010.
Burleyson, C. D., de Szoeke, S. P., Yuter, S. E., Wilbanks, M., and Brewer, W. A.: Ship-based observations of the diurnal cycle of southeast Pacific marine stratocumulus clouds and precipitation, J. Atmos. Sci., 70, 3876–3894, https://doi.org/10.1175/JAS-D-13-01.1, 2013.
Chang, J. S., Binkowski, F. S., Seaman, N. L, McHenry, J. N, Samson, P. J., Stockwell, W. R., Walcek, C. J., Madronich, S., Middleton, P. B., Pleim, J. E., and Lansford, H. H.: The regional acid deposition model and engineering model. State-of-Science/Technology, Report 4, National Acid Precipitation Assessment Program, Washington DC, 1989.
Chapman, E. G., Gustafson Jr., W. I., Easter, R. C., Barnard, J. C., Ghan, S. J., Pekour, M. S., and Fast, J. D.: Coupling aerosol-cloud-radiative processes in the WRF-Chem model: Investigating the radiative impact of elevated point sources, Atmos. Chem. Phys., 9, 945–964, https://doi.org/10.5194/acp-9-945-2009, 2009.
Chou, M. D., Suarez, M. J., Ho, C. H., Yan, M. M. H., and Lee, K. T.: Parameterizations for cloud overlapping and shortwave single-scattering properties for use in general circulation and cloud ensemble models, J. Climate, 11, 202–214, 1998.
Clarke, A. D., Owens, S. R., and Zhou, J.: An ultrafine sea-salt flux from breaking waves: Implications for cloud condensation nuclei in the remote marine atmosphere., J. Geophys. Res., 111, D06202, https://doi.org/10.1029/2005JD006565, 2006.
Clarke, A. D., Freitag, S., Brekhovskikh, V., Campos, T., Snider, J. R., Kasputin, V., Howell, S., Shank, L., and McNaughton, C.: Combustion aerosol, entrainment, and clouds in the VOCALS region, CLIVAR Exchanges, 15, 25–28, 2010.
Collins, W. D., Bitz, C. M., Blackmon, M. L., Bonan, G. B., Bretherton, C. S., Carton, J. A., Chang, P., Doney, S. C., Hack, J. J., Henderson, T. B., Kiehl, J. T., Large, W. G., McKenna, D. S., Santer, B. D., and Smith, R. D.: The community climate system model version 3 (CCSM3), J. Climate, 19, 2122–2143, 2006.
Cooke, W. F., Liousse, C., and Cachier, H.: Construction of a 1° × 1° fossil fuel emission data set for carbonaceous aerosol and implementation and radiative impact in the ECHAM4 model, J. Geophys. Res., 104, 22137–22162, https://doi.org/10.1029/1999JD900187, 1999.
Davies, T., Cullen, M. J. P., Malcolm, A. J., Mawson, M. H., Staniforth, A., White, A. A., and Wood, N.: A new dynamical core for the Met Office's global and regional modeling of the atmosphere, Q. J. Roy. Meteor. Soc., 131, 1759–1782, 2005.
Davies, D. K., Ilavajahala, S., Wong, M. M., and Justice, C. O.: Fire Information for Resource Management System: Archiving and distributing MODIS active fire data, IEEE T. Geosci. Remote Sens., 47, 72–79, https://doi.org/10.1109/TGRS.2008.2002076, 2009.
Detering, H. W. and Etling, D.: Application of the E-ϵ turbulence model to the atmospheric boundary layer, Bound.-Lay. Meteor., 33, 113–133, 1985.
de Szoeke, S. P., Yuter, S., Mechem, D., Fairall, C. W., Burleyson, C. D., and Zuidema, P.: Observations of stratocumulus clouds and their effect on the eastern pacific surface heat budget along 20° S, J. Climate, 25, 8542–8567, https://doi.org/10.1175/JCLI-D-11-00618.1, 2012.
Diehl, T., Heil, A., Chin, M., Pan, X., Streets, D., Schultz, M., and Kinne, S.: Anthropogenic, biomass burning, and volcanic emissions of black carbon, organic carbon, and SO2 from 1980 to 2010 for hindcast model experiments, Atmos. Chem. Phys. Discuss., 12, 24895–24954, https://doi.org/10.5194/acpd-12-24895-2012, 2012.
Donner, L. J., Wyman, B. L., Hemler, R. S., Horowitz, L. W., Ming, Y., Zhao, M., Golaz, J.-C., Ginoux, P. Lin, S.-J., Schwarzkopf, M. D., Austin, J., Alaka, G., Cooke, W. F., Delworth, T. L., Freidenreich, S. M., Gordon, C. T., Griffies, S. M., Held, I. M., Hurlin, W. J., Klein, S. A., Knutson, T. R., Langenhorst, A. R., Lee, H.-C., Lin, Y., Magi, B. I., Malyshev, S. L., Milly, P. C. D., Naik, V., Nath, M. J., Pincus, R., Ploshay, J. J., Ramaswamy, V., Seman, C. J., Shevliakova, E., Sirutis, J. J., Stern, W. F., Stouffer, R. J., Wilson, R. J., Winton, M., Wittenberg, A. T., Zeng, F.: The dynamical core, physical parameterizations, and basic simulation characteristics of the atmospheric component AM3 of the GFDL Global Coupled Model CM3, J. Climate., 24, 3484–3519, https://doi.org/10.1175/2011JCLI3955.1, 2011.
Edwards, J. M. and Slingo, A.: Studies with a flexible new radiation code. I: Choosing a configuration for a large-scale model, Q. J. Roy. Meteor. Soc., 122, 689–719, 1996.
Emmons, L. K., Walters, S., Hess, P. G., Lamarque, J.-F., Pfister, G. G., Fillmore, D., Granier, C., Guenther, A., Kinnison, D., Laepple, T., Orlando, J., Tie, X., Tyndall, G., Wiedinmyer, C., Baughcum, S. L., and Kloster, S.: Description and evaluation of the Model for Ozone and Related chemical Tracers, version 4 (MOZART-4), Geosci. Model Dev., 3, 43–67, https://doi.org/10.5194/gmd-3-43-2010, 2010.
Freidenreich, S. M. and Ramaswamy, V.: A new multiple-band solar radiative parameterization for general circulation models, J. Geophys. Res., 104, 31389–31409, 1999.
George, R. C. and Wood, R.: Subseasonal variability of low cloud radiative properties over the southeast Pacific Ocean, Atmos. Chem. Phys., 10, 4047–4063, https://doi.org/10.5194/acp-10-4047-2010, 2010.
George, R. C., Wood, R., Bretherton, C. S., and Painter, G.: Development and impact of hooks of high droplet concentration on remote southeast Pacific stratocumulus, Atmos. Chem. Phys., 13, 6305–6328, https://doi.org/10.5194/acp-13-6305-2013, 2013.
Gettelman, A., Morrison, H., and Ghan, S. J.: A new two-moment bulk stratiform cloud microphysics scheme in the Community Atmospheric Model, Version 3 (CAM3). Part II: Single-column and global results, J. Climate, 21, 3660–3679, 2008.
Gong, S. L., Barrie, L. A., and Blanchet, J.-P.: Modeling sea-salt aerosols in the atmosphere. 1. Model development, J. Geophys. Res., 102, 3805–3818, 1997.
Guenther, A., Karl, T., Harley, P., Wiedinmyer, C., Palmer, P. I., and Geron, C.: Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions of Gases and Aerosols from Nature), Atmos. Chem. Phys., 6, 3181–3210, https://doi.org/10.5194/acp-6-3181-2006, 2006.
Hannay, C., Williamson, D. L., Hack, J. J., Kiehl, J. T., Olson, J. G., Klein, S. A., Bretherton, C. S., and Köhler, M.: Evaluation of forecasted Southeast Pacific stratocumulus in the NCAR, GFDL, and ECMWF models, J. Climate, 22, 2871–2889, https://doi.org/10.1175/2008JCLI2479.1, 2009.
Holtslag, A. A. M. and Boville, B. A.: Local versus nonlocal boundary-layer diffusion in a global climate model, J. Climate, 6, 1825–1842, 1993.
Hong, S.-Y., Noh, Y., and Dudhia, J.: A new vertical diffusion package with an explicit treatment of entrainment processes, Mon. Weather Rev., 134, 2318–2341, 2006.
Hudson, J. G., Noble, S., and Jha, V.: Stratus cloud supersaturations, Geophys. Res. Lett., 37, L21813, https://doi.org/10.1029/2010GL045197, 2010.
Iacono, M. J., Delamere, J. S., Mlawer, E. J., Shephard, M. W., Clough, S. A., and Collins, W. D.: Radiative forcing by long-lived greenhouse gases: Calculations with the AER radiative transfer models, J. Geophys. Res., 113, D13103, https://doi.org/10.1029/2008JD009944, 2008.
Junker, C. and Liousse, C.: A global emission inventory of carbonaceous aerosol from historic records of fossil fuel and biofuel consumption for the period 1860–1997, Atmos. Chem. Phys., 8, 1195–1207, https://doi.org/10.5194/acp-8-1195-2008, 2008.
Köhler, M., Ahlgrimm, M., and Beljaars, A.: Unified treatment of dry convective and stratocumulus-topped boundary layers in the ECMWF model, Q. J. Roy. Meteor. Soc., 137, 43–57, https://doi.org/10.1002/qj.713, 2011.
Lauer, A., Eyring, V., Hendricks, J., Jöckel, P., and Lohmann, U.: Global model simulations of the impact of ocean-going ships on aerosols, clouds, and the radiation budget, Atmos. Chem. Phys., 7, 5061–5079, https://doi.org/10.5194/acp-7-5061-2007, 2007.
Lauer, A., Wang, Y., Phillips, V. T. J., McNaughton, C. S., Bennartz, R., and Clarke, A. D.: Simulating marine boundary layer clouds over the eastern Pacific in a regional climate model with double-moment cloud microphysics, J. Geophys. Res., 114, D21205, https://doi.org/10.1029/2009JD012201, 2009.
Lamarque, J.-F., Kiehl, J. T., Brasseur, G. P., Butler, T., Cameron-Smith, P., Collins, W. D., Collins, W. J., Granier, C., Hauglustaine, D., Hess, P. G., Holland, E. A., Horowitz, L., Lawrence, M. G., McKenna, D., Merilees, P., Prather, M. J., Rasch, P. J., Rotman, D., Shindell, D., and Thornton, P.: Assessing future nitrogen deposition and carbon cycle feedback using a multimodel approach: analysis of nitrogen deposition, J. Geophys. Res., 110, D19303, https://doi.org/10.1029/2005JD005825, 2005.
Lamarque, J.-F., Bond, T. C., Eyring, V., Granier, C., Heil, A., Klimont, Z., Lee, D., Liousse, C., Mieville, A., Owen, B., Schultz, M. G., Shindell, D., Smith, S. J., Stehfest, E., Van Aardenne, J., Cooper, O. R., Kainuma, M., Mahowald, N., McConnell, J. R., Naik, V., Riahi, K., and van Vuuren, D. P.: Historical (1850–2000) gridded anthropogenic and biomass burning emissions of reactive gases and aerosols: methodology and application, Atmos. Chem. Phys., 10, 7017–7039, https://doi.org/10.5194/acp-10-7017-2010, 2010.
Langland, R. H. and Liou, C.-S.: Implementation of an E-ϵ parameterization of vertical subgrid-scale mixing in a regional model, Mon. Weather Rev., 124, 905–918, 1996.
Liousse, C., Penner, J. E., Chuang, C., Walton, J. J., Eddleman, H., and Cachier, H.: A global three-dimensional model study of carbonaceous aerosols, J. Geophys. Res., 101, 19411–19432, https://doi.org/10.1029/95JD03426, 1996.
Lock, A. P., Brown, A. R., Bush, M. R., Martin, G. M., and Smith, R. N. B.: A new boundary layer mixing scheme. Part I: scheme description and single-column model tests, Mon. Weather Rev., 128, 3187–3199, 2000.
Mahowald, N. M., Lamarque, J.-F., Tie, X. X., and Wolff, E.: Sea-salt aerosol response to climate change: Last Glacial Maximum, preindustrial, and doubled carbon dioxide climates, J. Geophys. Res., 111, D05303, https://doi.org/10.1029/2005JD006459, 2006.
Mårtensson, E. M., Nilsson, E. D., de Leeuw, G., Cohen, L. H., and Hansson, H. C.: Laboratory simulations are parameterization of the primary marine aerosol production, J. Geophys. Res., 108, 4297, https://doi.org/10.1029/2002JD002263, 2003.
Martin, G. M., Johnson, D. W., and Spice, A.: The measurement and parameterization of effective radius of droplets in warm stratocumulus clouds, J. Atmos. Sci., 51, 1823–1842, 1994.
McNaughton, C. S.: Constraining climate model simulations of aerosol size distributions over the North Pacific and North America using in-situ airborne measurements, PhD thesis, Univ. of Hawaii at Manoa, Honolulu, Hawaii, USA, available at: http://hdl.handle.net/10125/20817 (last access: 5 January 2015), 2008.
Mechoso, C. R., Wood, R., Weller, R., Bretherton, C. S., Clarke, A. D., Coe., H., Fairall, C., Farrar, J. T., Feingold, G., Garreaud, R., Grados, C., McWilliams, J., de Szoeke, S. P., Yuter, S. E., and Zuidema, P.: Ocean-cloud-atmosphere-land interactions in the southeastern pacific: The VOCALS Program, B. Am. Meteorol. Soc., 95, 357–375, https://doi.org/10.1175/BAMS-D-11-00246.1, 2014.
Mena-Carrasco, M., Oliva, E., Saide, P., Spak, S. N., de la Maza, C., Osses, M., Tolvett, S., Campbell, J. E., Tsao, T. C.-C., and Molina, L. T.: Estimating the health benefits from natural gas use in transport and heating in Santiago, Chile, Sci. Total Environ., 429, 257–265, https://doi.org/10.1016/j.scitotenv.2012.04.037, 2012.
Ming, Y., V. Ramaswamy, V., Donner, L. J., and Phillips, V. T. J.: A new parameterization of cloud droplet activation applicable to general circulation models, J. Atmos. Sci., 63, 1348–1356, 2006.
Mlawer, E. J., Taubman, S. J., Brown, P. D., Iacono, M. J., and Clough, S. A.: Radiative transfer for inhomogeneous atmosphere: RRTM, a validated correlated-k model for the longwave, J. Geophys. Res., 102, 16663–16682, 1997.
Monahan, E. C., Spiel, D. E., and Davidson, K. L.: A model of marine aerosol generation via whitecaps and wave disruption, in: Oceanic Whitecaps and Their Role in Air-Sea Exchange Processes, edited by: Monahan, E. C. and Mac Niocaill, G., 167–193, Springer, New York, 1986.
Morcrette, J.-J., Barker, H. W., Cole, J. N. S., Iacono, M. J., and Pincus, R.: Impact of a new radiation package, McRad, in the ECMWF Integrated Forecasting System, Mon. Weather Rev., 136, 4773–4798, https://doi.org/10.1175/2008MWR2363.1, 2008.
Morcrette, J.-J., Boucher, O., Jones, L., Salmond, D., Bechtold, P., Beljaars, A., Benedetti, A., Bonet, A., Kaiser, J. W., Razinger, M., Schulz, M., Serrar, S., Simmons, A. J., Sofiev, M., Suttie, M., Tompkins, A. M., and Untch, A.: Aerosol analysis and forecast in the ECMWF Integrated Forecast System: Forward modelling, J. Geophys. Res., 114, D06206, https://doi.org/10.1029/2008JD011235, 2009.
Morrison, H. and Gettelman, A.: A new two-moment bulk stratiform cloud microphysics scheme in the Community Atmosphere Model, version 3 (CAM3). Part I: description and numerical tests, J. Climate, 21, 3642–3659, 2008.
Nakanishi, M. and Niino, H.: An improved Mellor-Yamada level-3 model with condensation physics: its design and verification, Bound. Lay. Meteorol., 112, 1–31, 2004.
Nightingale, P. D., Malin, G., Law, C. S., Watson, A. J., Liss, P. S., Liddicoat, M. I., Boutin, J., and Upstill-Goddard, R. C.: In situ evaluation of air-sea gas exchange parameterizations using novel conservative and volatile tracers, Global Biogeochem. Cy., 14, 373–387, 2000.
Ovchinnikov, M., Easter, R. C., and Gustafson, W. I.: Untangling dynamical and microphysical controls for the structure of stratocumulus, Geophys. Res. Lett., 40, 4432–4436, https://doi.org/10.1002/grl.50810, 2013.
Park, S. and Bretherton, C. S.: The University of Washington shallow convection and moist turbulence schemes and their impact on climate simulations with the community atmosphere model, J. Climate, 22, 3449–3469, 2009.
Phillips, T. J., Potter, G. L., Williamson, D. L., Cederwall, R. T., Boyle, J. S., Fiorino, M., Hnilo, J. J., Olson, J. G., Xie, S., and Yio, J. J.: Evaluating parameterizations in general circulation models: climate simulation meets weather prediction, B. Am. Meteorol. Soc., 85, 1903–1915, https://doi.org/10.1175/BAMS-85-12-1903, 2004.
Phillips, V. T. J., Donner, L. J., and Garner, S. T.: Nucleation processes in deep convection simulated by a cloud-system-resolving model with double-moment bulk microphysics, J. Atmos. Sci., 64, 738–761, https://doi.org/10.1175/JAS3869.1, 2007.
Phillips, V. T. J., DeMott, P. J., and Andronache, C.: An empirical parameterization of heterogeneous ice nucleation for multiple chemical species of aerosol, J. Atmos. Sci., 65, 2757–2783, https://doi.org/10.1175/2007JAS2546.1, 2008.
Phillips, V. T. J., Andronache, C., Christner, B., Morris, C. E., Sands, D. C., Bansemer, A., Lauer, A., McNaughton, C., and Seman, C.: Potential impacts from biological aerosols on ensembles of continental clouds simulated numerically, Biogeosciences, 6, 987–1014, https://doi.org/10.5194/bg-6-987-2009, 2009.
Rapp, A. D., Lebsock, M., and L'Ecuyer, T.: Low cloud precipitation climatology in the southeastern Pacific marine stratocumulus region using CloudSat, Environ. Res. Lett., 8, 014027, https://doi.org/10.1088/1748-9326/8/1/014027, 2013.
Rasch, P. J. and Kristjánsson, J. E.: A comparison of the CCM3 model climate using diagnosed and predicted condensate parameterizations, J. Climate, 11, 1587–1614, 1998.
Richter, I. and Mechoso, C. R.: Orographic influences on subtropical stratocumulus, J. Atmos. Sci., 63, 2585–2601, 2006.
Rotstayn, L. D.: A physically based scheme for the treatment of stratiform clouds and precipitation in large-scale models. I: Description and evaluation of the microphysical processes, Q. J. Roy. Meteor. Soc., 123, 1227–1282, 1997.
Rotstayn, L. D.: On the "tuning" of autoconversion parameterizations in climate models, J. Geophys. Res., 105, 15495–15507, 2000.
Saide, P. E., Spak, S. N., Carmichael, G. R., Mena-Carrasco, M. A., Yang, Q., Howell, S., Leon, D. C., Snider, J. R., Bandy, A. R., Collett, J. L., Benedict, K. B., de Szoeke, S. P., Hawkins, L. N., Allen, G., Crawford, I., Crosier, J., and Springston, S. R.: Evaluating WRF-Chem aerosol indirect effects in Southeast Pacific marine stratocumulus during VOCALS-REx, Atmos. Chem. Phys., 12, 3045–3064, https://doi.org/10.5194/acp-12-3045-2012, 2012.
Schell B., Ackermann, I. J., Hass, H., Binkowski, F. S., and Ebel, A.: Modeling the formation of secondary organic aerosol within a comprehensive air quality model system, J. Geophys. Res., 106, 28275–28293, 2001.
Schwarzkopf, M. D. and Ramaswamy, V.: Radiative effects of CH4, N2O, halocarbons, and the foreign-broadened H2O continuum: A GCM experiment, J. Geophys., Res., 104, 9467–9488, 1999.
Shank, L. M., Howell, S., Clarke, A. D., Freitag, S., Brekhovskikh, V., Kapustin, V., McNaughton, C., Campos, T., and Wood, R.: Organic matter and non-refractory aerosol over the remote Southeast Pacific: oceanic and combustion sources, Atmos. Chem. Phys., 12, 557–576, https://doi.org/10.5194/acp-12-557-2012, 2012.
Shipway, B. J. and Hill, A. A.: Diagnosis of systematic differences between multiple parametrizations of warm rain microphysics using a kinematic framework, Q. J. Roy. Meteorol. Soc., 138, 2196–2211, 2012.
Smith, S. J., Pitcher, H., and Wigley, T. M. L.: Global and regional anthropogenic sulfur dioxide emissions, Global Biogeochem. Cy., 29, 99–119, 2001.
Smith, S. J., Andres, R., Conception, E., and Lurz, J.: Historical sulfur dioxide emissions 1850–2000: methods and results, Technical report, Pacific Northwest National Laboratory, Joint Global Change Research Institute, College Park, MD, USA, 2004.
Snider, J. R., Guibert S., Brenguier, J.-L., and Putaud, J.-P.: Aerosol activation in marine stratocumulus clouds: 2. Köhler and parcel theory closure studies, J. Geophys. Res., 108, 8629, https://doi.org/10.1029/2002JD002692, 2003.
Solomon, S., Qin, D., Manning, M., Marquis, M., Averyt, K. B., Tignor, M., Miller, H. L. Jr., and Chen, Z. (Eds).: Climate Change 2007: The Physical Science Basis, Cambridge University Press, 996 pp., 2007.
Twohy, C. H., Anderson, J. R., Toohey, D. W., Andrejczuk, M., Adams, A., Lytle, M., George, R. C., Wood, R., Saide, P., Spak, S., Zuidema, P., and Leon, D.: Impacts of aerosol particles on the microphysical and radiative properties of stratocumulus clouds over the southeast Pacific Ocean, Atmos. Chem. Phys., 13, 2541–2562, https://doi.org/10.5194/acp-13-2541-2013, 2013.
Wang, S., O'Neill, L. W., Jiang, Q., de Szoeke, S. P., Hong, X., Jin, H., Thompson, W. T., and Zheng, X.: A regional real-time forecast of marine boundary layers during VOCALS-REx, Atmos. Chem. Phys., 11, 421–437, https://doi.org/10.5194/acp-11-421-2011, 2011.
Wilson, D. R. and Ballard, S. P.: A microphysically based precipitation scheme for the UK Meteorological Office Unified Model, Q. J. Roy. Met. Soc., 125, 1607–1636, 1999.
Wood, R., Comstock, K. K., Bretherton, C. S., Cornish, C., Tomlinson, J., Collins D. R., and Fairall, C.: Open cellular structure in marine stratocumulus cloud sheets, J. Geophys. Res., 113, D12207, https://doi.org/10.1029/2007JD009371, 2008
Wood, R., Mechoso, C. R., Bretherton, C. S., Weller, R. A., Huebert, B., Straneo, F., Albrecht, B. A., Coe, H., Allen, G., Vaughan, G., Daum, P., Fairall, C., Chand, D., Gallardo Klenner, L., Garreaud, R., Grados, C., Covert, D. S., Bates, T. S., Krejci, R., Russell, L. M., de Szoeke, S., Brewer, A., Yuter, S. E., Springston, S. R., Chaigneau, A., Toniazzo, T., Minnis, P., Palikonda, R., Abel, S. J., Brown, W. O. J., Williams, S., Fochesatto, J., Brioude, J., and Bower, K. N.: The VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx): goals, platforms, and field operations, Atmos. Chem. Phys., 11, 627–654, https://doi.org/10.5194/acp-11-627-2011, 2011a.
Wood, R., Bretherton, C. S., Leon, D., Clarke, A. D., Zuidema, P., Allen, G., and Coe, H.: An aircraft case study of the spatial transition from closed to open mesoscale cellular convection over the Southeast Pacific, Atmos. Chem. Phys., 11, 2341–2370, https://doi.org/10.5194/acp-11-2341-2011, 2011b.
Wood, R., Leon, D., Lebsock, M., Snider, J., and Clarke, A. D.: Precipitation driving of droplet concentration variability in marine low clouds, J. Geophys. Res., 117, D19210, https://doi.org/10.1029/2012JD018305, 2012.
Wyant, M. C., Wood, R., Bretherton, C. S., Mechoso, C. R., Bacmeister, J., Balmaseda, M. A., Barrett, B., Codron, F., Earnshaw, P., Fast, J., Hannay, C., Kaiser, J. W., Kitagawa, H., Klein, S. A., Köhler, M., Manganello, J., Pan, H.-L., Sun, F., Wang, S., and Wang, Y.: The PreVOCA experiment: modeling the lower troposphere in the Southeast Pacific, Atmos. Chem. Phys., 10, 4757–4774, https://doi.org/10.5194/acp-10-4757-2010, 2010.
Yang, M., Huebert, B. J., Blomquist, B. W., Howell, S. G., Shank, L. M., McNaughton, C. S., Clarke, A. D., Hawkins, L. N., Russell, L. M., Covert, D. S., Coffman, D. J., Bates, T. S., Quinn, P. K., Zagorac, N., Bandy, A. R., de Szoeke, S. P., Zuidema, P. D., Tucker, S. C., Brewer, W. A., Benedict, K. B., and Collett, J. L.: Atmospheric sulfur cycling in the southeastern Pacific – longitudinal distribution, vertical profile, and diel variability observed during VOCALS-REx, Atmos. Chem. Phys., 11, 5079–5097, https://doi.org/10.5194/acp-11-5079-2011, 2011.
Yang, Q., W. I. Gustafson Jr., Fast, J. D., Wang, H., Easter, R. C., Morrison, H., Lee, Y.-N., Chapman, E. G., Spak, S. N., and Mena-Carrasco, M. A.: Assessing regional scale predictions of aerosols, marine stratocumulus, and their interactions during VOCALS-REx using WRF-Chem, Atmos. Chem. Phys., 11, 11951–11975, https://doi.org/10.5194/acp-11-11951-2011, 2011.
Yang, Q., Gustafson Jr., W. I., Fast, J. D., Wang, H., Easter, R. C., Wang, M., Ghan, S. J., Berg, L. K., Leung, L. R., and Morrison, H.: Impact of natural and anthropogenic aerosols on stratocumulus and precipitation in the Southeast Pacific: a regional modelling study using WRF-Chem, Atmos. Chem. Phys., 12, 8777–8796, https://doi.org/10.5194/acp-12-8777-2012, 2012.
Zaveri, R. A. and Peters, L. K.: A new lumped structure photochemical mechanism for large-scale applications, J. Geophys. Res., 104, 30387–30415, 1999.
Zaveri, R. A., Easter, R. C., Fast, J. D., and Peters, L.: Model for simulating aerosol interactions and chemistry (MOSAIC), J. Geophys. Res., 113, D13204, https://doi.org/10.1029/2007JD008782, 2008.
Zuidema, P., Leon, D., Pazmany, A., and Cadeddu, M.: Aircraft millimeter-wave passive sensing of cloud liquid water and water vapor during VOCALS-REx, Atmos. Chem. Phys., 12, 355–369, https://doi.org/10.5194/acp-12-355-2012, 2012.
Short summary
Simulations from a group of GCMs, forecast models, and regional models are compared with aircraft and ship observations of the marine boundary layer (MBL) in the southeast Pacific region during the VOCALS-REx field campaign of October-November 2008. Gradients of cloud, aerosol, and chemical properties in and above the MBL extending from the Peruvian coast westward along 20 degrees south are compared during the period.
Simulations from a group of GCMs, forecast models, and regional models are compared with...
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