Articles | Volume 25, issue 7
https://doi.org/10.5194/acp-25-3873-2025
https://doi.org/10.5194/acp-25-3873-2025
Research article
 | 
03 Apr 2025
Research article |  | 03 Apr 2025

Surface temperature dependence of stratospheric sulfate aerosol clear-sky forcing and feedback

Ravikiran Hegde, Moritz Günther, Hauke Schmidt, and Clarissa Kroll

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Cited articles

Andronova, N. G., Rozanov, E. V., Yang, F., Schlesinger, M. E., and Stenchikov, G. L.: Radiative forcing by volcanic aerosols from 1850 to 1994, J. Geophys. Res.-Atmos., 104, 16807–16826, https://doi.org/10.1029/1999JD900165, 1999. a, b, c
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Aubry, T. J., Staunton-Sykes, J., Marshall, L. R., Haywood, J., Abraham, N. L., and Schmidt, A.: Climate change modulates the stratospheric volcanic sulfate aerosol lifecycle and radiative forcing from tropical eruptions, Nat. Commun., 12, 4708, https://doi.org/10.1038/s41467-021-24943-7, 2021. a, b, c, d
Aubry, T. J., Farquharson, J. I., Rowell, C. R., Watt, S. F. L., Pinel, V., Beckett, F., Fasullo, J., Hopcroft, P. O., Pyle, D. M., Schmidt, A., and Sykes, J. S.: Impact of climate change on volcanic processes: current understanding and future challenges, B. Volcanol., 84, 58, https://doi.org/10.1007/s00445-022-01562-8, 2022. a, b
Bloch-Johnson, J., Rugenstein, M., Stolpe, M. B., Rohrschneider, T., Zheng, Y., and Gregory, J. M.: Climate sensitivity increases under higher CO2 levels due to feedback temperature dependence, Geophys. Res. Lett., 48, e2020GL089074, https://doi.org/10.1029/2020GL089074, 2021. a, b, c
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Using a one-dimensional radiative–convective equilibrium model, we show that in clear-sky conditions, stratospheric sulfate aerosol forcing weakens with increasing surface temperature while CO2 forcing varies much less. This effect arises as sulfate aerosol, unlike CO2, absorbs mainly at wavelengths where the atmosphere is optically thin. It thereby masks the surface emission, which increases with warming. The spectral masking also results in weaker radiative feedback when aerosol is present.
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