Articles | Volume 23, issue 15
https://doi.org/10.5194/acp-23-8993-2023
https://doi.org/10.5194/acp-23-8993-2023
Research article
 | 
11 Aug 2023
Research article |  | 11 Aug 2023

Anthropogenic amplification of biogenic secondary organic aerosol production

Yiqi Zheng, Larry W. Horowitz, Raymond Menzel, David J. Paynter, Vaishali Naik, Jingyi Li, and Jingqiu Mao

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Cited articles

Attwood, A. R., Washenfelder, R. A., Brock, C. A., Hu, W., Baumann, K., Campuzano-Jost, P., Day, D. A., Edgerton, E. S., Murphy, D. M., Palm, B. B., McComiskey, A., Wagner, N. L., De Sá, S. S., Ortega, A., Martin, S. T., Jimenez, J. L., and Brown, S. S.: Trends in sulfate and organic aerosol mass in the Southeast U.S.: Impact on aerosol optical depth and radiative forcing, Geophys. Res. Lett., 41, 7701–7709, https://doi.org/10.1002/2014GL061669, 2014. 
Bates, K. H. and Jacob, D. J.: A new model mechanism for atmospheric oxidation of isoprene: global effects on oxidants, nitrogen oxides, organic products, and secondary organic aerosol, Atmos. Chem. Phys., 19, 9613–9640, https://doi.org/10.5194/acp-19-9613-2019, 2019. 
Berkemeier, T., Takeuchi, M., Eris, G., and Ng, N. L.: Kinetic modeling of formation and evaporation of secondary organic aerosol from NO3 oxidation of pure and mixed monoterpenes, Atmos. Chem. Phys., 20, 15513–15535, https://doi.org/10.5194/acp-20-15513-2020, 2020. 
Blanchard, C. L., Hidy, G. M., Shaw, S., Baumann, K., and Edgerton, E. S.: Effects of emission reductions on organic aerosol in the southeastern United States, Atmos. Chem. Phys., 16, 215–238, https://doi.org/10.5194/acp-16-215-2016, 2016. 
Boyd, C. M., Nah, T., Xu, L., Berkemeier, T., and Ng, N. L.: Secondary Organic Aerosol (SOA) from Nitrate Radical Oxidation of Monoterpenes: Effects of Temperature, Dilution, and Humidity on Aerosol Formation, Mixing, and Evaporation, Environ. Sci. Technol., 51, 7831–7841, https://doi.org/10.1021/acs.est.7b01460, 2017. 
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Short summary
Biogenic secondary organic aerosols (SOAs) account for a large fraction of fine aerosol at the global scale. Using long-term measurements and a climate model, we investigate anthropogenic impacts on biogenic SOA at both decadal and centennial timescales. Results show that despite reductions in biogenic precursor emissions, SOA has been strongly amplified by anthropogenic emissions since the preindustrial era and exerts a cooling radiative forcing.
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