Articles | Volume 22, issue 21
https://doi.org/10.5194/acp-22-14303-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-14303-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Nov 2022
Research article |
| 08 Nov 2022
| 08 Nov 2022
Stratospheric water vapour and ozone response to the quasi-biennial oscillation disruptions in 2016 and 2020
Mohamadou A. Diallo
CORRESPONDING AUTHOR
Institute of Energy and Climate Research, Stratosphere (IEK–7), Forschungszentrum Jülich, 52425 Jülich, Germany
Felix Ploeger
Institute of Energy and Climate Research, Stratosphere (IEK–7), Forschungszentrum Jülich, 52425 Jülich, Germany
Institute for Atmospheric and Environmental Research, University of Wuppertal, Wuppertal, Germany
Michaela I. Hegglin
Institute of Energy and Climate Research, Stratosphere (IEK–7), Forschungszentrum Jülich, 52425 Jülich, Germany
Institute for Atmospheric and Environmental Research, University of Wuppertal, Wuppertal, Germany
Department of Meteorology, University of Reading, Reading, UK
Manfred Ern
Institute of Energy and Climate Research, Stratosphere (IEK–7), Forschungszentrum Jülich, 52425 Jülich, Germany
Jens-Uwe Grooß
Institute of Energy and Climate Research, Stratosphere (IEK–7), Forschungszentrum Jülich, 52425 Jülich, Germany
Sergey Khaykin
Laboratoire Atmosphères, Milieux, Observations Spatiales, UMR CNRS 8190, IPSL, Sorbonne Univ./UVSQ, Guyancourt, France
Martin Riese
Institute of Energy and Climate Research, Stratosphere (IEK–7), Forschungszentrum Jülich, 52425 Jülich, Germany
Institute for Atmospheric and Environmental Research, University of Wuppertal, Wuppertal, Germany
Related authors
Sean M. Davis, William T. Ball, Yue Jia, Gabriel Chiodo, Justin A. Alsing, James Keeble, Hideharu Akiyoshi, Carlo Arosio, Ewa M. Bednarz, Andreas Chrysanthou, Melanie Coldewey-Egbers, Robert Damadeo, Sandip Dhomse, Mohamadou A. Diallo, Simone Dietmuller, Roland Eichinger, Stacey Frith, Birgit Hassler, Michaela I. Hegglin, Daan Hubert, Patrick Jöckel, Béatrice Josse, Natalya Kramarova, Diego Loyola, Eliane Maillard Barras, Marion Marchand, Olaf Morgenstern, David Plummer, Robert W. Portmann, Karen H. Rosenlof, Alexei Rozanov, Viktoria F. Sofieva, Johannes Staehelin, Timofei Sukhodolov, Kleareti Tourpali, Ronald J. Van der A, H. J. Ray Wang, Krzysztof Wargan, Shingo Watanabe, Mark Weber, Jeannette D. Wild, Yousuke Yamashita, and Jerry Ziemke
Atmos. Chem. Phys., 26, 13817–13843, https://doi.org/10.5194/acp-26-13817-2026, https://doi.org/10.5194/acp-26-13817-2026, 2026
Short summary
Short summary
This study investigates tropical ozone changes in models and satellite observations to determine how well they agree and whether observations can constrain model projections. At some levels, satellite records disagree significantly on the magnitude of ozone changes. While early and late 21st century trends are correlated across models, suggesting a potential emergent constraint, the spread in observations means they are unable to provide guidance on the credibility of model projections.
Jingyu Wang, Gabriel Chiodo, Blanca Ayarzagüena, William T. Ball, Mohamadou Diallo, Birgit Hassler, James Keeble, Peer Nowack, Clara Orbe, Sandro Vattioni, and Timofei Sukhodolov
Atmos. Chem. Phys., 25, 17819–17844, https://doi.org/10.5194/acp-25-17819-2025, https://doi.org/10.5194/acp-25-17819-2025, 2025
Short summary
Short summary
We analyzed the ozone response under elevated CO2 using the data from CMIP6 DECK experiments. We then examined the relations between ozone response and changes in temperature and circulation to identify the drivers of ozone change. The climate feedback of ozone is investigated through offline calculations and by comparing models with and without interactive chemistry. We find that ozone–climate interactions are important for Earth system models and thus should be considered in future model development.
Toyese Tunde Ayorinde, Cristiano Max Wrasse, Hisao Takahashi, Luiz Fernando Sapucci, Mohamadou A. Diallo, Cosme Alexandre Oliveira Barros Figueiredo, Diego Barros, Ligia Alves da Silva, Patrick Essien, and Anderson Vestena Bilibio
Atmos. Chem. Phys., 25, 12357–12378, https://doi.org/10.5194/acp-25-12357-2025, https://doi.org/10.5194/acp-25-12357-2025, 2025
Short summary
Short summary
We studied how the Intertropical Convergence Zone (ITCZ) interacts with atmospheric gravity waves high in the sky and how global climate patterns like El Niño affect them. Using RO, ERA5, and NCEP reanalysis data, we found that the ITCZ shifts with season but stays strong year-round, influencing weather and energy flow. Our findings show how climate patterns shape weather systems and help predict changes, improving understanding of the atmosphere and its effects on global climate.
Manfred Ern, Mohamadou A. Diallo, Dina Khordakova, Isabell Krisch, Peter Preusse, Oliver Reitebuch, Jörn Ungermann, and Martin Riese
Atmos. Chem. Phys., 23, 9549–9583, https://doi.org/10.5194/acp-23-9549-2023, https://doi.org/10.5194/acp-23-9549-2023, 2023
Short summary
Short summary
Quasi-biennial oscillation (QBO) of the stratospheric tropical winds is an important mode of climate variability but is not well reproduced in free-running climate models. We use the novel global wind observations by the Aeolus satellite and radiosondes to show that the QBO is captured well in three modern reanalyses (ERA-5, JRA-55, and MERRA-2). Good agreement is also found also between Aeolus and reanalyses for large-scale tropical wave modes in the upper troposphere and lower stratosphere.
Sean M. Davis, William T. Ball, Yue Jia, Gabriel Chiodo, Justin A. Alsing, James Keeble, Hideharu Akiyoshi, Carlo Arosio, Ewa M. Bednarz, Andreas Chrysanthou, Melanie Coldewey-Egbers, Robert Damadeo, Sandip Dhomse, Mohamadou A. Diallo, Simone Dietmuller, Roland Eichinger, Stacey Frith, Birgit Hassler, Michaela I. Hegglin, Daan Hubert, Patrick Jöckel, Béatrice Josse, Natalya Kramarova, Diego Loyola, Eliane Maillard Barras, Marion Marchand, Olaf Morgenstern, David Plummer, Robert W. Portmann, Karen H. Rosenlof, Alexei Rozanov, Viktoria F. Sofieva, Johannes Staehelin, Timofei Sukhodolov, Kleareti Tourpali, Ronald J. Van der A, H. J. Ray Wang, Krzysztof Wargan, Shingo Watanabe, Mark Weber, Jeannette D. Wild, Yousuke Yamashita, and Jerry Ziemke
Atmos. Chem. Phys., 26, 13817–13843, https://doi.org/10.5194/acp-26-13817-2026, https://doi.org/10.5194/acp-26-13817-2026, 2026
Short summary
Short summary
This study investigates tropical ozone changes in models and satellite observations to determine how well they agree and whether observations can constrain model projections. At some levels, satellite records disagree significantly on the magnitude of ozone changes. While early and late 21st century trends are correlated across models, suggesting a potential emergent constraint, the spread in observations means they are unable to provide guidance on the credibility of model projections.
Qiaoyun Hu, Philippe Goloub, Igor Veselovskii, Thierry Podvin, Gaël Dubois, Sergey Khaykin, William Boissière, Fabrice Ducos, and Mikhail Korenskiy
Atmos. Chem. Phys., 26, 13027–13053, https://doi.org/10.5194/acp-26-13027-2026, https://doi.org/10.5194/acp-26-13027-2026, 2026
Short summary
Short summary
This study reports dual-site fluorescence lidar observations of long-range transported Canadian wildfire biomass burning aerosols (BBAs) from May to September 2023. Upper troposphere–lower stratosphere (UTLS) layers showed higher depolarization, lower Ångström exponents, and fluorescence redshift compared to tropospheric layers. Moderate correlations are found between layer altitude and BBA properties. Notably, limited hygroscopicity was found in more than 100 identified BBA layers. Cross-site comparison shows consistent fluorescence signatures.
Florian Voet, Felix Ploeger, Johannes C. Laube, Laura N. Saunders, Patrick E. Sheese, Attahir Mainika, Peter Preusse, Jens-Uwe Grooß, Kaley A. Walker, Susann Tegtmeier, and Michaela Imelda Hegglin
EGUsphere, https://doi.org/10.5194/egusphere-2026-4647, https://doi.org/10.5194/egusphere-2026-4647, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
We developed a better way to estimate how long air remains in the upper atmosphere, because satellite estimates can be too noisy to show long-term changes. Using measurements of several gases from a satellite, we found that combining them cuts uncertainty by about half and gives estimates with about 0.3 years of average uncertainty. Results for 2004–2021 show older air in the Northern Hemisphere and younger air in the tropics and Southern Hemisphere, suggesting slower circulation in the north.
Wolfgang Woiwode, Bärbel Vogel, Valentin Lauther, Jens-Uwe Grooß, Jeremy Harrison, Sören Johansson, Jörn Ungermann, Peter Braesicke, Markus Dick, Andreas Engel, Felix Friedl-Vallon, Norbert Glatthor, Thomas Gulde, Michael Höpfner, Markus Jesswein, Jan Kaumanns, Timo Keber, Anne Kleinert, Erik Kretschmer, Guido Maucher, Tom Neubert, Hans Nordmeyer, Christof Piesch, Felix Plöger, Peter Preusse, Markus Retzlaff, Sebastian Rhode, Heinz Rongen, Georg Schardt, Tanja Schuck, Björn-Martin Sinnhuber, Johannes Strobel, Franziska Trinkl, Ronja Van Luijt, Stefan Versick, C. Michael Volk, Gerald Wetzel, Peter Hoor, and Martin Riese
EGUsphere, https://doi.org/10.5194/egusphere-2026-3271, https://doi.org/10.5194/egusphere-2026-3271, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Filaments of CH2Cl2-rich air are revealed by airborne infrared limb-imaging observations in late summer 2023 above the North Pacific, Canada and Alaska and traced back to the Asian Summer Monsoon region. Involving new spectroscopic data, high CH2Cl2 levels were retrieved in the troposphere and moderate enhancements also in air masses with characteristics of the lowermost stratosphere. Mesoscale filaments are shown to transport substantial amounts of CH2Cl2 across the North Pacific.
Kimberlee Dubé, William Randel, Adam Bourassa, Susann Tegtmeier, Xinyue Wang, Jun Zhang, Eilidh Hlady, Meghan Brehon, Sergey Khaykin, and Douglas Degenstein
EGUsphere, https://doi.org/10.5194/egusphere-2026-4022, https://doi.org/10.5194/egusphere-2026-4022, 2026
Short summary
Short summary
The Hunga volcanic eruption in January 2022 increased the total stratospheric water vapor (H2O) mass by 10 %. The study uses satellite observations and models to track the transport of the Hunga H2O. We find that there is substantially more H2O in the observations than the model during 2024 and 2025, suggesting that the modelled transport across the lower stratosphere is too fast. We also find evidence that some of the H2O that reaches the lower stratosphere is mixed back into the tropics.
Jan Kaumanns, Florian Voet, Felix Ploeger, Peter Preuße, Jörn Ungermann, and Michaela Imelda Hegglin
EGUsphere, https://doi.org/10.5194/egusphere-2026-4183, https://doi.org/10.5194/egusphere-2026-4183, 2026
Short summary
Short summary
Age-of-Air (AoA) denotes the time an air parcel has spent inside the stratosphere and is an important diagnostic quantity for the Brewer Dobson Circulation (BDC). We present a novel approach using neural networks to accurately and robustly derive AoA from inert chemical species with considerable measurement noise even far beyond the training domain. We also present an alternative view of AoA by using autoencoders to derive a model-independent proxy quantity for it and validate its robustness.
Eddy Poncet, Sergey Khaykin, Sophie Godin-Beekmann, and Thierry Leblanc
EGUsphere, https://doi.org/10.5194/egusphere-2026-4358, https://doi.org/10.5194/egusphere-2026-4358, 2026
Short summary
Short summary
High particles in the atmosphere affect climate and the ozone layer, so measurements from a new European-Japanese satellite, EarthCARE (launched 2024), need checking. We compared its laser data with a trusted instrument on the International Space Station and two ground stations, in clear, volcanic and wildfire conditions. A method using the satellite's raw signal stayed accurate even when particles were scarce, unlike the standard product, so we recommend it for reliable long-term monitoring.
Oleh Kachula, Bärbel Vogel, Gebhard Günther, Rolf Müller, and Felix Ploeger
EGUsphere, https://doi.org/10.5194/egusphere-2026-3509, https://doi.org/10.5194/egusphere-2026-3509, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Locating the boundary of the Asian summer monsoon anticyclone (ASMA) in the upper atmosphere is important for understanding how this system distributes pollutants. We show that while different methodologies generally agree on the boundary's location and shape, certain methods are preferred under specific conditions. These findings will be of broad interest to researchers studying large-scale atmospheric circulations in upper atmosphere.
Fatih Ekinci, Oliver Eppers, Oliver Appel, Felix Ploeger, Antonis Dragoneas, Sergej Molleker, Philipp Brauner, Hans-Christoph Lachnitt, Franziska Weyland, Linda Ort, Nicolas Emig, Hans-Christian Clemen, Laura Tomsche, Martin Ebert, Peter Hoor, Bärbel Vogel, Yafang Cheng, Johannes Schneider, Stephan Borrmann, and Franziska Köllner
Atmos. Chem. Phys., 26, 10399–10421, https://doi.org/10.5194/acp-26-10399-2026, https://doi.org/10.5194/acp-26-10399-2026, 2026
Short summary
Short summary
This study shows that aerosol transported from the Asian summer monsoon region can substantially alter the background composition of the extratropical lower stratosphere. Aircraft-based measurements and model simulations reveal a strong increase of ammonium nitrate aerosol from summer to autumn 2023 caused by transport of young air masses from South and East Asia. These particles can persist for months and undergo chemical aging.
Christoph Jacobi, Ales Kuchar, Manfred Ern, Toralf Renkwitz, Ralph Latteck, and Jorge L. Chau
Adv. Radio Sci., 24, 15–28, https://doi.org/10.5194/ars-24-15-2026, https://doi.org/10.5194/ars-24-15-2026, 2026
Short summary
Short summary
Analyses of more than four decades (1979–2024) of mean horizontal winds in the mesopause region at about 90 km altitude show long-term trends and an influence of the 11-year solar cycle. After the 1990s, both linear trends and the solar cycle effect change and strongly weaken, indicating a change in dynamics or solar forcing. Gravity wave proxies also show a solar cycle effect, which decreases after the 1990s.
Jan Kaumanns, Jörn Ungermann, Bärbel Vogel, Sören Johansson, Erik Kretschmer, Felix Plöger, Peter Preuße, Wolfgang Woiwode, and Martin Riese
Atmos. Chem. Phys., 26, 9083–9111, https://doi.org/10.5194/acp-26-9083-2026, https://doi.org/10.5194/acp-26-9083-2026, 2026
Short summary
Short summary
During the PHILEAS aircraft campaign a self-matching experiment was conducted to study the mixing of Asian Summer monsoon air into the upper troposphere – lower stratosphere. We present the first 3-D tomographic observations of this mixing for multiple trace gas species. We use advanced clustering to identify the types of air and their transport pathways, particularly into the stratosphere. Simulations of surface-origin tracers link several of these air types to different source regions.
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Irene Bartolome Garcia, Emmanuel Briaud, Rubel Chandra Das, Stéphane Chevrier, Nicolas Dumelié, Lilian Joly, Thomas Lecas, Pauline Marbach, Felix Ploeger, Jean-Baptiste Renard, Jean-Paul Vernier, Frank G. Wienhold, and Michaela I. Hegglin
Atmos. Chem. Phys., 26, 8981–8997, https://doi.org/10.5194/acp-26-8981-2026, https://doi.org/10.5194/acp-26-8981-2026, 2026
Short summary
Short summary
In October 2022, we detected volcanic particles in the stratosphere over France, linked to the January 2022 Hunga eruption in the South Pacific. Found between 17 and 23 km altitude, they were traced back to the tropics using trajectory simulations and satellite data. Their optical properties matched those in the Southern Hemisphere. The particles spread across the Northern Hemisphere, reflecting sunlight and slightly cooling the surface – a small but non-negligible effect.
Irina Petropavlovskikh, Martine De Mazière, Anne M. Thompson, Jeannette D. Wild, James W. Hannigan, Henry B. Selkirk, Reem A. Hannun, Wolfgang Steinbrecht, Jean-Christopher Lambert, Roeland Van Malderen, Elizabeth Asher, Raul R. Cordero, Sophie Godin-Beekmann, Daan Hubert, Sergey Khaykin, Karin Kreher, Thierry Leblanc, Emmanuel Mahieu, Eliane Maillard Barras, Glen McConville, Gerald Nedoluha, Ivan Ortega, Alberto Redondas Marrero, Gunther Seckmeyer, Ryan M. Stauffer, Sarah A. Strode, Kim Strong, Takafumi Sugita, Michel Van Roozendael, Voltaire Velazco, Corinne Vigouroux, and Bärbel Vogel
Atmos. Chem. Phys., 26, 8637–8675, https://doi.org/10.5194/acp-26-8637-2026, https://doi.org/10.5194/acp-26-8637-2026, 2026
Short summary
Short summary
This introduction to the special issue "Achievements and perspectives of the Network for the Detection of Atmospheric Composition Change after 35 years of operation” provides an overview of important research findings achieved under the NDACC objectives. The future of NDACC is discussed in the light of the evolution of the scientific questions, evolving collaborations with partners and Cooperating Networks, and the current landscape of gaps in satellite and ground-based observations.
Phoebe Noble, Haruka Okui, Joan Alexander, Manfred Ern, Neil P. Hindley, Lars Hoffmann, Laura Holt, Annelize van Niekerk, Riwal Plougonven, Inna Polichtchouk, Claudia C. Stephan, Martina Bramberger, Milena Corcos, William Putnam, Christopher Kruse, and Corwin J. Wright
Atmos. Chem. Phys., 26, 7607–7630, https://doi.org/10.5194/acp-26-7607-2026, https://doi.org/10.5194/acp-26-7607-2026, 2026
Short summary
Short summary
Gravity waves are small-scale processes that drive the circulation in the middle and upper atmosphere. In this work, we assess 3 new high-resolution (3-5km horizontal resolution) models against satellite data. Generally, models capture the spatial patterns and represent stratospheric northern hemisphere mountain generated waves well. However, they still underestimate amplitudes globally and struggle with the representation of southern hemispheric convective waves.
Dimitri Trapon, Holger Baars, Sebastian Bley, Albert Ansmann, Michael Rennie, Sergey Khaykin, and Michael Sicard
EGUsphere, https://doi.org/10.5194/egusphere-2026-2575, https://doi.org/10.5194/egusphere-2026-2575, 2026
Short summary
Short summary
The study presents observations of the 2022 Hunga volcanic aerosol in the stratosphere made by the European Space Agency’s Aeolus satellite. Aeolus tracks the long-range transported plumes that circumnavigate the Earth at distinct latitudes and altitudes up to 30 km. Vertical gradient of optical properties measured with the ultraviolet lidar signal are shown, such as decreasing trends over time. This helps to understand the stratospheric residence time of aerosols in the Southern Hemisphere.
Raphaël Lebrun, Yevgeny Derimian, François Ravetta, Jérôme Bureau, and Sergey Khaykin
EGUsphere, https://doi.org/10.5194/egusphere-2026-2006, https://doi.org/10.5194/egusphere-2026-2006, 2026
Short summary
Short summary
Fueled by climate change, some recent extreme wildfires have been observed to inject unprecedented levels of aerosols in the stratosphere. Partly composed of carbon, these aerosols absorb solar light and change the energy balance of the atmosphere. Using observations and radiative modeling, we show the stratospheric aerosols from the 2020 Australian wildfire have warmed the atmosphere by 0.08 to 0.19 W.m−2 globally over a year, as they tend to reduce the albedo effect of underlying clouds.
Shubhajyoti Roy, Satheesh P. R. Chandran, Suvarna Fadnavis, Vijay Sagar, Michaela I. Hegglin, Rolf Müller, and Prashant Chavan
Atmos. Chem. Phys., 26, 7047–7059, https://doi.org/10.5194/acp-26-7047-2026, https://doi.org/10.5194/acp-26-7047-2026, 2026
Short summary
Short summary
We show that stratospheric ozone intrusions associated with sudden stratospheric warming events occurring concurrent with the westerly phase of the Quasi-biennial oscillation enhance ozone in the upper troposphere and lower stratosphere over South Asia. The ozone enhancement increases ozone radiative forcing by 0.09±0.05 W m-2 over South Asia. This increase in ozone radiative forcing potentially exacerbates regional climate warming.
Bärbel Vogel, Valentin Lauther, Franziska Köllner, Fatih Ekinci, Christian Rolf, Johannes Strobel, Ronja van Luijt, C. Michael Volk, Stephan Borrmann, Antonis Dragoneas, Oliver Eppers, Sergej Molleker, Peter Hoor, Linda Ort, Franziska Weyland, Andreas Zahn, Jan Clemens, Gebhard Günther, Oleh Kachula, Rolf Müller, Felix Ploeger, and Martin Riese
Atmos. Chem. Phys., 26, 6283–6319, https://doi.org/10.5194/acp-26-6283-2026, https://doi.org/10.5194/acp-26-6283-2026, 2026
Short summary
Short summary
This work highlights the impact of the Asian summer monsoon on the chemical composition of the upper troposphere and lower stratosphere. Measurements of trace gases and aerosol particles uplifted by the Asian summer monsoon to higher altitudes are sparse. Here, we had the opportunity to use a whole suite of different measured trace gases and the chemical composition of aerosols, in combination with simulations, to better understand the complex transport and mixing processes in this region.
Marta Abalos, Thomas Birner, Andreas Chrysanthou, Sean Davis, Alvaro de la Cámara, Sandip Dhomse, Hella Garny, Michaela I. Hegglin, Daan Hubert, Oksana Ivaniha, James Keeble, Marianna Linz, Daniele Minganti, Jessica Neu, David Plummer, Laura Saunders, Kasturi Shah, Gabriele Stiller, Kleareti Tourpali, Darryn Waugh, Nathan Luke Abraham, Hideharu Akiyoshi, Martyn P. Chipperfield, Patrick Jöckel, Béatrice Josse, Marion Marchand, Patrick Martineau, Olaf Morgenstern, Timofei Sukhodolov, Shingo Watanabe, and Yousuke Yamashita
Atmos. Chem. Phys., 26, 5249–5291, https://doi.org/10.5194/acp-26-5249-2026, https://doi.org/10.5194/acp-26-5249-2026, 2026
Short summary
Short summary
Accurate representation of stratospheric transport in Chemistry-Climate Models is essential for reliable climate projections. This study evaluates three generations of models using observational data and reanalyses, identifying persistent biases and their potential causes. Some biases persist or even worsen in newer models. These findings highlight key limitations and inform efforts to improve models and advance understanding through process-based studies and enhanced observations.
Zhen Yang, Bärbel Vogel, Felix Plöger, Zhixuan Bai, Dan Li, Sabine Griessbach, Lars Hoffmann, Frank G. Wienhold, Elizabeth Asher, Alexandre A. Baron, Katie R. Smith, Troy Thornberry, Jianchun Bian, and Michaela I. Hegglin
Atmos. Chem. Phys., 26, 4749–4769, https://doi.org/10.5194/acp-26-4749-2026, https://doi.org/10.5194/acp-26-4749-2026, 2026
Short summary
Short summary
Balloon measurements over Lhasa, China, combined with satellite guided modelling, tracked aerosol from the 2019 Raikoke eruption through the Asian summer monsoon anticyclone. We find two altitude dependent routes into the anticyclone. It partly blocks transport but also allows entry and mixing, explaining the gradual weakening of the layers. Balloon measurements over Boulder, United States, outside the anticyclone, provide an independent check outside the region.
Samuel Trémoulu, Fabrice Chane Ming, Alain Hauchecorne, Sergey Khaykin, Mathieu Ratynski, and Philippe Keckhut
Atmos. Meas. Tech., 19, 1039–1058, https://doi.org/10.5194/amt-19-1039-2026, https://doi.org/10.5194/amt-19-1039-2026, 2026
Short summary
Short summary
We developed a new method to better detect and study small-scale gravity waves in the middle atmosphere using lidar data. This technique more clearly reveals wave patterns than older methods and gives more accurate energy estimates, especially high up near the stratopause. Our approach helps scientists understand how these waves behave and interact across different scales, improving knowledge of atmospheric dynamics.
Arun Jo Mathew, Sebastian Rhode, Manfred Ern, Maniyatt Pramitha, and Peter Preusse
Atmos. Meas. Tech., 19, 949–964, https://doi.org/10.5194/amt-19-949-2026, https://doi.org/10.5194/amt-19-949-2026, 2026
Short summary
Short summary
The atmosphere hosts a multitude of waves, among which Atmospheric Gravity wave separation from satellite measurements requires removal of global scale waves and tides. The present study describes the open access software GLOFI (GLObal wave FIt) which uses the 2D spectral decomposition to perform this removal. It is validated on simulated temperature observations synthesised for ESA (European Space Agency) Earth Explorer 11 candidate CAIRT (Changing-Atmosphere Infra-Red Tomography Explorer).
Sergey Khaykin, Michaël Sicard, Thierry Leblanc, Tetsu Sakai, Nickolay Balugin, Gwenaël Berthet, Stëphane Chevrier, Fernando Chouza, Artem Feofilov, Dominique Gantois, Sophie Godin-Beekmann, Arezki Haddouche, Yoshitaka Jin, Isamu Morino, Nicolas Kadygrov, Thomas Lecas, Ben Liley, Richard Querel, Ghasssan Taha, and Vladimir Yushkov
Atmos. Chem. Phys., 26, 607–622, https://doi.org/10.5194/acp-26-607-2026, https://doi.org/10.5194/acp-26-607-2026, 2026
Short summary
Short summary
In April 2024, the Ruang volcano in Indonesia sent large amounts of gas and particles high into the atmosphere, which then spread worldwide. Using the new European EarthCARE satellite and its advanced laser instrument ATLID (Atmospheric LIDar), together with ground and balloon observations, we tracked how these particles doubled levels in the tropics and spread into both hemispheres. The study shows ATLID’s power to reveal how eruptions can affect climate, clouds, and ozone for more than a year.
Liliana Guidetti, Erika Brattich, Simone Ceccherini, Michaela I. Hegglin, Piera Raspollini, Cecilia Tirelli, Nicola Zoppetti, and Ugo Cortesi
Atmos. Meas. Tech., 19, 167–184, https://doi.org/10.5194/amt-19-167-2026, https://doi.org/10.5194/amt-19-167-2026, 2026
Short summary
Short summary
The Complete Data Fusion algorithm is applied to observations from the Michelson Interferometer for Passive Atmospheric Sounding and the Infrared Atmospheric Sounding Interferometer to generate and validate a new ozone dataset against ozone soundings across multiple latitudes. The fusion propagates stratospheric limb information into the troposphere. The dataset shows increased information content and lower uncertainty, improving the study of stratosphere–troposphere ozone intrusions.
Paul Konopka, Felix Ploeger, Francesco D'Amato, Teresa Campos, Marc von Hobe, Shawn B. Honomichl, Peter Hoor, Laura L. Pan, Michelle L. Santee, Silvia Viciani, Kaley A. Walker, and Michaela I. Hegglin
Atmos. Chem. Phys., 25, 17973–17996, https://doi.org/10.5194/acp-25-17973-2025, https://doi.org/10.5194/acp-25-17973-2025, 2025
Short summary
Short summary
We present an improved version of the Chemical Lagrangian Model of the Stratosphere (CLaMS-3.0), which better represents transport from the lower atmosphere to the upper troposphere and lower stratosphere. By refining grid resolution and improving convection representation, the model more accurately simulates carbon monoxide transport. Comparisons with satellite and in situ observations highlight its ability to capture seasonal variations and improve our understanding of atmospheric transport.
Jingyu Wang, Gabriel Chiodo, Blanca Ayarzagüena, William T. Ball, Mohamadou Diallo, Birgit Hassler, James Keeble, Peer Nowack, Clara Orbe, Sandro Vattioni, and Timofei Sukhodolov
Atmos. Chem. Phys., 25, 17819–17844, https://doi.org/10.5194/acp-25-17819-2025, https://doi.org/10.5194/acp-25-17819-2025, 2025
Short summary
Short summary
We analyzed the ozone response under elevated CO2 using the data from CMIP6 DECK experiments. We then examined the relations between ozone response and changes in temperature and circulation to identify the drivers of ozone change. The climate feedback of ozone is investigated through offline calculations and by comparing models with and without interactive chemistry. We find that ozone–climate interactions are important for Earth system models and thus should be considered in future model development.
Benjamin W. Clouser, Laszlo C. Sarkozy, Clare E. Singer, Carly C. KleinStern, Adrien Desmoulin, Dylan Gaeta, Sergey Khaykin, Stephen Gabbard, Stephen Shertz, and Elisabeth J. Moyer
Atmos. Meas. Tech., 18, 6465–6491, https://doi.org/10.5194/amt-18-6465-2025, https://doi.org/10.5194/amt-18-6465-2025, 2025
Short summary
Short summary
The water molecule comes in several different varieties, which are nearly indistinguishable in daily life. However, slight differences between the water molecule types can be exploited to achieve better scientific understanding of parts of Earth's atmosphere. In this work we describe the design, construction, and operation of an instrument meant to measure these molecules aboard research aircraft up to altitudes of 20 km.
Frederik Harzer, Hella Garny, Felix Ploeger, J. Moritz Menken, and Thomas Birner
Atmos. Chem. Phys., 25, 14909–14921, https://doi.org/10.5194/acp-25-14909-2025, https://doi.org/10.5194/acp-25-14909-2025, 2025
Short summary
Short summary
We study ozone transport in the extratropical lowermost stratosphere using potential temperature as vertical coordinate, thereby distinguishing adiabatic and diabatic processes. We find that on top of known dominant transport processes (quasi-horizontal mixing, slow diabatic descent) vertical mixing plays an important role near the tropopause. Our findings are relevant for understanding ozone's role in climate including its imprint on tropospheric ozone via stratosphere-troposphere air exchange.
Hongyue Wang, Mijeong Park, Mengchu Tao, Cristina Peña-Ortiz, Nuria P. Plaza-Martin, Felix Ploeger, and Paul Konopka
Atmos. Chem. Phys., 25, 14703–14718, https://doi.org/10.5194/acp-25-14703-2025, https://doi.org/10.5194/acp-25-14703-2025, 2025
Short summary
Short summary
We investigate how water vapor in the upper atmosphere gains moisture during the Asian and North American monsoons using a simplified modeling approach. Our results show that the Asian monsoon is mainly controlled by large-scale temperature, whereas the North American monsoon may be more influenced by convective moistening. These differences point to distinct mechanisms shaping moisture transport in the two monsoon systems.
Sergey Khaykin, Slimane Bekki, Sophie Godin-Beekmann, Michael D. Fromm, Philippe Goloub, Qiaoyun Hu, Béatrice Josse, Alexandra Laeng, Mehdi Meziane, David A. Peterson, Sophie Pelletier, and Valérie Thouret
Atmos. Chem. Phys., 25, 14551–14571, https://doi.org/10.5194/acp-25-14551-2025, https://doi.org/10.5194/acp-25-14551-2025, 2025
Short summary
Short summary
In 2023, massive wildfires in Canada injected huge amounts of smoke into the atmosphere. Surprisingly, despite their intensity, the smoke did not rise very high but lingered at flight cruising altitudes, causing widespread pollution. This study shows how two different pathways lifted smoke into the lower stratosphere and reveals new insights into how wildfires affect air quality and climate, challenging what we thought we knew about fire and atmospheric impacts.
Gerald Wetzel, Anne Kleinert, Sören Johansson, Felix Friedl-Vallon, Michael Höpfner, Jörn Ungermann, Tom Neubert, Valéry Catoire, Cyril Crevoisier, Andreas Engel, Thomas Gulde, Patrick Jacquet, Oliver Kirner, Erik Kretschmer, Thomas Kulessa, Johannes C. Laube, Guido Maucher, Hans Nordmeyer, Christof Piesch, Peter Preusse, Markus Retzlaff, Georg Schardt, Johan Schillings, Herbert Schneider, Axel Schönfeld, Tanja Schuck, Wolfgang Woiwode, Martin Riese, and Peter Braesicke
Atmos. Meas. Tech., 18, 5873–5894, https://doi.org/10.5194/amt-18-5873-2025, https://doi.org/10.5194/amt-18-5873-2025, 2025
Short summary
Short summary
We present vertical trace gas profiles from the first balloon flight of the newly developed GLORIA-B limb-imaging Fourier-Transform spectrometer. Longer-lived gases are compared to external measurements to assess the quality of the GLORIA-B observations. Diurnal changes of photochemically active species are compared to model simulations. GLORIA-B demonstrates the capability of balloon-borne limb imaging to provide high-resolution vertical profiles of trace gases up to the middle stratosphere.
Mathieu Ratynski, Sergey Khaykin, Alain Hauchecorne, M. Joan Alexander, Alexis Mariaccia, Philippe Keckhut, and Antoine Mangin
Atmos. Chem. Phys., 25, 13769–13798, https://doi.org/10.5194/acp-25-13769-2025, https://doi.org/10.5194/acp-25-13769-2025, 2025
Short summary
Short summary
This study investigates how tropical convection generates gravity waves, which play a key role in transporting energy across the atmosphere. By combining Aeolus satellite data with ERA5 reanalysis data and radio occultation measurements, we identified significant wave activity overlooked by ERA5, particularly over the Indian Ocean. Aeolus fills major gaps in wind data, offering a clearer picture of wave dynamics and challenging assumptions about their behavior, thereby improving climate models.
Rasul Baikhadzhaev, Felix Ploeger, Peter Preusse, Manfred Ern, and Thomas Birner
Atmos. Chem. Phys., 25, 12753–12777, https://doi.org/10.5194/acp-25-12753-2025, https://doi.org/10.5194/acp-25-12753-2025, 2025
Short summary
Short summary
Across four reanalyses, the shallow branch of the stratospheric overturning circulation was found to be driven by planetary waves 1 to 3, and the deep branch of the circulation was found to be driven by smaller-scale waves (wave 4 and higher). However, the height of the level separating the branches is dependent on the reanalysis considered. Thus, using the appropriate separation levels in model inter-comparisons could reduce the spread between models regarding climatology and trends in the circulation.
Toyese Tunde Ayorinde, Cristiano Max Wrasse, Hisao Takahashi, Luiz Fernando Sapucci, Mohamadou A. Diallo, Cosme Alexandre Oliveira Barros Figueiredo, Diego Barros, Ligia Alves da Silva, Patrick Essien, and Anderson Vestena Bilibio
Atmos. Chem. Phys., 25, 12357–12378, https://doi.org/10.5194/acp-25-12357-2025, https://doi.org/10.5194/acp-25-12357-2025, 2025
Short summary
Short summary
We studied how the Intertropical Convergence Zone (ITCZ) interacts with atmospheric gravity waves high in the sky and how global climate patterns like El Niño affect them. Using RO, ERA5, and NCEP reanalysis data, we found that the ITCZ shifts with season but stays strong year-round, influencing weather and energy flow. Our findings show how climate patterns shape weather systems and help predict changes, improving understanding of the atmosphere and its effects on global climate.
Ales Kuchar, Gunter Stober, Dimitry Pokhotelov, Huixin Liu, Han-Li Liu, Manfred Ern, Damian Murphy, Diego Janches, Tracy Moffat-Griffin, Nicholas Mitchell, and Christoph Jacobi
EGUsphere, https://doi.org/10.5194/egusphere-2025-2827, https://doi.org/10.5194/egusphere-2025-2827, 2025
Short summary
Short summary
We studied how the healing of the Antarctic ozone layer is affecting winds high above the South Pole. Using ground-based radar, satellite data, and computer models, we found that winds in the upper atmosphere have become stronger over the past two decades. These changes appear to be linked to shifts in the lower atmosphere caused by ozone recovery. Our results show that human efforts to repair the ozone layer are also influencing climate patterns far above Earth’s surface.
Christoph Jacobi, Khalil Karami, Ales Kuchar, Manfred Ern, Toralf Renkwitz, Ralph Latteck, and Jorge L. Chau
Adv. Radio Sci., 23, 21–31, https://doi.org/10.5194/ars-23-21-2025, https://doi.org/10.5194/ars-23-21-2025, 2025
Short summary
Short summary
Half-hourly mean winds have been obtained using ground-based low-frequency and very high frequency radio observations of the mesopause region at Collm, Germany, since 1984. Long-term changes of wind variances, which are proxies for short-period atmospheric gravity waves, have been analysed. Gravity wave amplitudes increase with time in winter, but mainly decrease in summer. The trends are consistent with mean wind changes according to wave theory.
Mingzhao Liu, Lars Hoffmann, Jens-Uwe Grooß, Zhongyin Cai, Sabine Grießbach, and Yi Heng
Atmos. Chem. Phys., 25, 4403–4418, https://doi.org/10.5194/acp-25-4403-2025, https://doi.org/10.5194/acp-25-4403-2025, 2025
Short summary
Short summary
We studied the transport and chemical decomposition of volcanic SO2, focusing on the 2019 Raikoke event. By comparing two different chemistry modeling schemes, we found that including complex chemical reactions leads to a more accurate prediction of how long SO2 stays in the atmosphere. This research helps improve our understanding of volcanic pollution and its impact on air quality and climate, providing better tools for scientists to track and predict the movement of these pollutants.
Patrick Konjari, Christian Rolf, Michaela I. Hegglin, Susanne Rohs, Yun Li, Andreas Zahn, Harald Bönisch, Philippe Nedelec, Martina Krämer, and Andreas Petzold
Atmos. Chem. Phys., 25, 4269–4289, https://doi.org/10.5194/acp-25-4269-2025, https://doi.org/10.5194/acp-25-4269-2025, 2025
Short summary
Short summary
This study introduces a new method to derive adjusted water vapor (H2O) climatologies for the upper tropopshere and lower statosphere (UT/LS) using data from 60 000 flights under the IAGOS program. Biases in the IAGOS water vapour dataset are adjusted, based on the more accurate IAGOS-CARIBIC data. The resulting highly resolved H2O climatologies will contribute to a better understanding of the H2O variability in the UT/LS and its connection to various transport and mixing processes.
Laura N. Saunders, Kaley A. Walker, Gabriele P. Stiller, Thomas von Clarmann, Florian Haenel, Hella Garny, Harald Bönisch, Chris D. Boone, Ariana E. Castillo, Andreas Engel, Johannes C. Laube, Marianna Linz, Felix Ploeger, David A. Plummer, Eric A. Ray, and Patrick E. Sheese
Atmos. Chem. Phys., 25, 4185–4209, https://doi.org/10.5194/acp-25-4185-2025, https://doi.org/10.5194/acp-25-4185-2025, 2025
Short summary
Short summary
We present a 17-year stratospheric age-of-air dataset derived from ACE-FTS satellite measurements of sulfur hexafluoride. This is the longest continuous, global, and vertically resolved age of air time series available to date. In this paper, we show that this dataset agrees well with age-of-air datasets based on measurements from other instruments. We also present trends in the midlatitude lower stratosphere that indicate changes in the global circulation that are predicted by climate models.
Florian Voet, Felix Ploeger, Johannes Laube, Peter Preusse, Paul Konopka, Jens-Uwe Grooß, Jörn Ungermann, Björn-Martin Sinnhuber, Michael Höpfner, Bernd Funke, Gerald Wetzel, Sören Johansson, Gabriele Stiller, Eric Ray, and Michaela I. Hegglin
Atmos. Chem. Phys., 25, 3541–3565, https://doi.org/10.5194/acp-25-3541-2025, https://doi.org/10.5194/acp-25-3541-2025, 2025
Short summary
Short summary
This study refines estimates of the stratospheric “age of air”, a measure of how long air circulates in the stratosphere. By analyzing correlations between trace gases measurable by satellites, the research introduces a method that reduces uncertainties and detects small-scale atmospheric features. This improved understanding of stratospheric circulation is crucial for better climate models and predictions, enhancing our ability to assess the impacts of climate change on the atmosphere.
Ziming Wang, Luca Bugliaro, Klaus Gierens, Michaela I. Hegglin, Susanne Rohs, Andreas Petzold, Stefan Kaufmann, and Christiane Voigt
Atmos. Chem. Phys., 25, 2845–2861, https://doi.org/10.5194/acp-25-2845-2025, https://doi.org/10.5194/acp-25-2845-2025, 2025
Short summary
Short summary
Upper-tropospheric relative humidity bias in the ERA5 weather model is corrected by 10 % by an artificial neural network using aircraft in-service humidity data and thermodynamic and dynamical variables. The improved skills of the weather model will advance cirrus research, weather forecasts, and measures for contrail reduction.
Dioumacor Faye, Felipe M. de Andrade, Roberto Suárez-Moreno, Dahirou Wane, Michaela I. Hegglin, Abdou L. Dieng, François Kaly, Redouane Lguensat, and Amadou T. Gaye
EGUsphere, https://doi.org/10.5194/egusphere-2024-4040, https://doi.org/10.5194/egusphere-2024-4040, 2025
Preprint archived
Short summary
Short summary
This study evaluates machine learning (ML) methods to improve subseasonal-to-seasonal (S2S) rainfall forecasts in Senegal during the West African monsoon. Using high-resolution precipitation data and atmospheric-oceanic reanalysis, we show that ML models like ridge regression outperform traditional climate models. These methods enhance prediction accuracy and efficiency, offering valuable tools for climate risk management and water resource planning.
Kimberlee Dubé, Susann Tegtmeier, Felix Ploeger, and Kaley A. Walker
Atmos. Chem. Phys., 25, 1433–1447, https://doi.org/10.5194/acp-25-1433-2025, https://doi.org/10.5194/acp-25-1433-2025, 2025
Short summary
Short summary
The transport rate of air in the stratosphere has changed in response to human emissions of greenhouse gases and ozone-depleting substances. This transport rate can be approximated using measurements of long-lived trace gases. We use observations and model results to derive anomalies and trends in the mean rate of stratospheric air transport. We find that air in the Northern Hemisphere aged by up to 0.3 years per decade relative to air in the Southern Hemisphere over 2004–2017.
Franziska Weyland, Peter Hoor, Daniel Kunkel, Thomas Birner, Felix Plöger, and Katharina Turhal
Atmos. Chem. Phys., 25, 1227–1252, https://doi.org/10.5194/acp-25-1227-2025, https://doi.org/10.5194/acp-25-1227-2025, 2025
Short summary
Short summary
The lowermost stratosphere (LMS) plays an important role in the Earth's climate, containing strong gradients of ozone and water vapor. Our results indicate that the thermodynamic structure of the LMS was changing between 1979–2019 in response to anthropogenic climate change and the recovery of stratospheric ozone, also indicating large-scale circulation changes. We find that both the upper and the lower LMS boundaries show an (upward) trend, which has implications for the LMS mass.
Xiaolu Yan, Paul Konopka, Felix Ploeger, and Aurélien Podglajen
Atmos. Chem. Phys., 25, 1289–1305, https://doi.org/10.5194/acp-25-1289-2025, https://doi.org/10.5194/acp-25-1289-2025, 2025
Short summary
Short summary
Our study finds that the air mass fractions (AMFs) from the Asian boundary layer (ABL) to the polar regions are about 1.5 times larger than those from the same latitude band in the Southern Hemisphere. The transport of AMFs from the ABL to the polar vortex primarily occurs above 20 km and over timescales exceeding 2 years. Our analysis reveals a strong correlation between the polar pollutants and the AMFs from the ABL. About 20 % of SF6 in the polar stratosphere originates from the ABL.
Xiaodan Ma, Jianping Huang, Michaela I. Hegglin, Patrick Jöckel, and Tianliang Zhao
Atmos. Chem. Phys., 25, 943–958, https://doi.org/10.5194/acp-25-943-2025, https://doi.org/10.5194/acp-25-943-2025, 2025
Short summary
Short summary
Our research explored changes in ozone levels in the northwest Pacific region over 30 years, revealing a significant increase in the middle-to-upper troposphere, especially during spring and summer. This rise is influenced by both stratospheric and tropospheric sources, which affect climate and air quality in East Asia. This work underscores the need for continued study to understand underlying mechanisms.
Katharina Turhal, Felix Plöger, Jan Clemens, Thomas Birner, Franziska Weyland, Paul Konopka, and Peter Hoor
Atmos. Chem. Phys., 24, 13653–13679, https://doi.org/10.5194/acp-24-13653-2024, https://doi.org/10.5194/acp-24-13653-2024, 2024
Short summary
Short summary
The tropopause separates the troposphere, where many greenhouse gases originate, from the stratosphere. This study examines a tropopause defined by potential vorticity – an analogue for angular momentum that changes sharply in the subtropics, creating a transport barrier. Between 1980 and 2017, this tropopause shifted poleward at lower altitudes and equatorward above, suggesting height-dependent changes in atmospheric circulation that may affect greenhouse gas distribution and global warming.
Yiran Zhang-Liu, Rolf Müller, Jens-Uwe Grooß, Sabine Robrecht, Bärbel Vogel, Abdul Mannan Zafar, and Ralph Lehmann
Atmos. Chem. Phys., 24, 12557–12574, https://doi.org/10.5194/acp-24-12557-2024, https://doi.org/10.5194/acp-24-12557-2024, 2024
Short summary
Short summary
HCl null cycles in Antarctica are important for maintaining high values of ozone-destroying chlorine in Antarctic spring. These HCl null cycles are not affected by (1) using the most recent recommendations of chemical kinetics (compared to older recommendations), (2) accounting for dehydration in the Antarctic winter vortex, and (3) considering the observed (but unexplained) depletion of HCl in mid-winter in the Antarctic vortex throughout Antarctic winter.
Sebastian Rhode, Peter Preusse, Jörn Ungermann, Inna Polichtchouk, Kaoru Sato, Shingo Watanabe, Manfred Ern, Karlheinz Nogai, Björn-Martin Sinnhuber, and Martin Riese
Atmos. Meas. Tech., 17, 5785–5819, https://doi.org/10.5194/amt-17-5785-2024, https://doi.org/10.5194/amt-17-5785-2024, 2024
Short summary
Short summary
We investigate the capabilities of a proposed satellite mission, CAIRT, for observing gravity waves throughout the middle atmosphere and present the necessary methodology for in-depth wave analysis. Our findings suggest that such a satellite mission is highly capable of resolving individual wave parameters and could give new insights into the role of gravity waves in general atmospheric circulation and atmospheric processes.
Sören Johansson, Michael Höpfner, Felix Friedl-Vallon, Norbert Glatthor, Thomas Gulde, Vincent Huijnen, Anne Kleinert, Erik Kretschmer, Guido Maucher, Tom Neubert, Hans Nordmeyer, Christof Piesch, Peter Preusse, Martin Riese, Björn-Martin Sinnhuber, Jörn Ungermann, Gerald Wetzel, and Wolfgang Woiwode
Atmos. Chem. Phys., 24, 8125–8138, https://doi.org/10.5194/acp-24-8125-2024, https://doi.org/10.5194/acp-24-8125-2024, 2024
Short summary
Short summary
We present airborne infrared limb sounding GLORIA measurements of ammonia (NH3) in the upper troposphere of air masses within the Asian monsoon and of those connected with biomass burning. Comparing CAMS (Copernicus Atmosphere Monitoring Service) model data, we find that the model reproduces the measured enhanced NH3 within the Asian monsoon well but not that within biomass burning plumes, where no enhanced NH3 is measured in the upper troposphere but considerable amounts are simulated by CAMS.
Nelson Bègue, Alexandre Baron, Gisèle Krysztofiak, Gwenaël Berthet, Corinna Kloss, Fabrice Jégou, Sergey Khaykin, Marion Ranaivombola, Tristan Millet, Thierry Portafaix, Valentin Duflot, Philippe Keckhut, Hélène Vérèmes, Guillaume Payen, Mahesh Kumar Sha, Pierre-François Coheur, Cathy Clerbaux, Michaël Sicard, Tetsu Sakai, Richard Querel, Ben Liley, Dan Smale, Isamu Morino, Osamu Uchino, Tomohiro Nagai, Penny Smale, John Robinson, and Hassan Bencherif
Atmos. Chem. Phys., 24, 8031–8048, https://doi.org/10.5194/acp-24-8031-2024, https://doi.org/10.5194/acp-24-8031-2024, 2024
Short summary
Short summary
During the 2020 austral summer, the pristine atmosphere of the southwest Indian Ocean basin experienced significant perturbations. Numerical models indicated that the lower-stratospheric aerosol content was influenced by the intense and persistent stratospheric aerosol layer generated during the 2019–2020 extreme Australian bushfire events. Ground-based observations at Réunion confirmed the simultaneous presence of African and Australian aerosol layers.
Luis F. Millán, Peter Hoor, Michaela I. Hegglin, Gloria L. Manney, Harald Boenisch, Paul Jeffery, Daniel Kunkel, Irina Petropavlovskikh, Hao Ye, Thierry Leblanc, and Kaley Walker
Atmos. Chem. Phys., 24, 7927–7959, https://doi.org/10.5194/acp-24-7927-2024, https://doi.org/10.5194/acp-24-7927-2024, 2024
Short summary
Short summary
In the Observed Composition Trends And Variability in the UTLS (OCTAV-UTLS) Stratosphere-troposphere Processes And their Role in Climate (SPARC) activity, we have mapped multiplatform ozone datasets into coordinate systems to systematically evaluate the influence of these coordinates on binned climatological variability. This effort unifies the work of studies that focused on individual coordinate system variability. Our goal was to create the most comprehensive assessment of this topic.
Björn Linder, Peter Preusse, Qiuyu Chen, Ole Martin Christensen, Lukas Krasauskas, Linda Megner, Manfred Ern, and Jörg Gumbel
Atmos. Meas. Tech., 17, 3829–3841, https://doi.org/10.5194/amt-17-3829-2024, https://doi.org/10.5194/amt-17-3829-2024, 2024
Short summary
Short summary
The Swedish research satellite MATS (Mesospheric Airglow/Aerosol Tomography and Spectroscopy) is designed to study atmospheric waves in the mesosphere and lower thermosphere. These waves perturb the temperature field, and thus, by observing three-dimensional temperature fluctuations, their properties can be quantified. This pre-study uses synthetic MATS data generated from a general circulation model to investigate how well wave properties can be retrieved.
Fuzhen Shen, Michaela I. Hegglin, and Yue Yuan
Atmos. Chem. Phys., 24, 6539–6553, https://doi.org/10.5194/acp-24-6539-2024, https://doi.org/10.5194/acp-24-6539-2024, 2024
Short summary
Short summary
We attempt to use a novel structural self-organising map and machine learning models to identify a weather system and quantify the importance of each meteorological factor in driving the unexpected PM2.5 and O3 changes under the specific weather system during the COVID-19 lockdown in China. The result highlights that temperature under the double-centre high-pressure system plays the most crucial role in abnormal events.
Cristina Peña-Ortiz, Nuria Pilar Plaza, David Gallego, and Felix Ploeger
Atmos. Chem. Phys., 24, 5457–5478, https://doi.org/10.5194/acp-24-5457-2024, https://doi.org/10.5194/acp-24-5457-2024, 2024
Short summary
Short summary
Although water vapour (H2O) in the lower stratosphere is only a few molecules among 1 million air molecules, atmospheric radiative forcing and surface temperature are sensitive to changes in its concentration. Monsoon regions play a key role in H2O transport and its concentration in the lower stratosphere. We show how the quasi-biennial oscillation (QBO) has a major impact on H2O over the Asian monsoon during August through changes in temperature caused by QBO modulation of tropical clouds.
Martin Ebert, Ralf Weigel, Stephan Weinbruch, Lisa Schneider, Konrad Kandler, Stefan Lauterbach, Franziska Köllner, Felix Plöger, Gebhard Günther, Bärbel Vogel, and Stephan Borrmann
Atmos. Chem. Phys., 24, 4771–4788, https://doi.org/10.5194/acp-24-4771-2024, https://doi.org/10.5194/acp-24-4771-2024, 2024
Short summary
Short summary
Particles were collected during the flight campaign StratoClim 2017 within the Asian tropopause aerosol layer (ATAL). Refractory particles from seven different flights were characterized by scanning and transmission electron microscopy (SEM, TEM). The most abundant refractory particles are silicates and non-volatile organics. The most important sources are combustion processes at the ground and the agitation of soil material. During one flight, small cinnabar particles (HgS) were also detected.
Felix Ploeger, Thomas Birner, Edward Charlesworth, Paul Konopka, and Rolf Müller
Atmos. Chem. Phys., 24, 2033–2043, https://doi.org/10.5194/acp-24-2033-2024, https://doi.org/10.5194/acp-24-2033-2024, 2024
Short summary
Short summary
We present a novel mechanism of how regional anomalies in water vapour concentrations in the upper troposphere and lower stratosphere impact regional atmospheric circulation systems. These impacts include a displaced upper-level Asian monsoon circulation and strengthened prevailing westerlies in the Pacific region. Current climate models have biases in simulating these regional water vapour anomalies and circulation impacts, but the biases can be avoided by improving the model transport.
Igor Veselovskii, Qiaoyun Hu, Philippe Goloub, Thierry Podvin, William Boissiere, Mikhail Korenskiy, Nikita Kasianik, Sergey Khaykyn, and Robin Miri
Atmos. Meas. Tech., 17, 1023–1036, https://doi.org/10.5194/amt-17-1023-2024, https://doi.org/10.5194/amt-17-1023-2024, 2024
Short summary
Short summary
Measurements of transported smoke layers were performed with a lidar in Lille and a five-channel fluorescence lidar in Moscow. Results show the peak of fluorescence in the boundary layer is at 438 nm, while in the smoke layer it shifts to longer wavelengths. The fluorescence depolarization is 45 % to 55 %. The depolarization ratio of the water vapor channel is low (2 ± 0.5 %) in the absence of fluorescence and can be used to evaluate the contribution of fluorescence to water vapor signal.
Jan Clemens, Bärbel Vogel, Lars Hoffmann, Sabine Griessbach, Nicole Thomas, Suvarna Fadnavis, Rolf Müller, Thomas Peter, and Felix Ploeger
Atmos. Chem. Phys., 24, 763–787, https://doi.org/10.5194/acp-24-763-2024, https://doi.org/10.5194/acp-24-763-2024, 2024
Short summary
Short summary
The source regions of the Asian tropopause aerosol layer (ATAL) are debated. We use balloon-borne measurements of the layer above Nainital (India) in August 2016 and atmospheric transport models to find ATAL source regions. Most air originated from the Tibetan plateau. However, the measured ATAL was stronger when more air originated from the Indo-Gangetic Plain and weaker when more air originated from the Pacific. Hence, the results indicate important anthropogenic contributions to the ATAL.
Bärbel Vogel, C. Michael Volk, Johannes Wintel, Valentin Lauther, Jan Clemens, Jens-Uwe Grooß, Gebhard Günther, Lars Hoffmann, Johannes C. Laube, Rolf Müller, Felix Ploeger, and Fred Stroh
Atmos. Chem. Phys., 24, 317–343, https://doi.org/10.5194/acp-24-317-2024, https://doi.org/10.5194/acp-24-317-2024, 2024
Short summary
Short summary
Over the Indian subcontinent, polluted air is rapidly uplifted to higher altitudes during the Asian monsoon season. We present an assessment of vertical transport in this region using different wind data provided by the European Centre for Medium-Range Weather Forecasts (ECMWF), as well as high-resolution aircraft measurements. In general, our findings confirm that the newest ECMWF reanalysis product, ERA5, yields a better representation of transport compared to the predecessor, ERA-Interim.
Konstantin Ntokas, Jörn Ungermann, Martin Kaufmann, Tom Neubert, and Martin Riese
Atmos. Meas. Tech., 16, 5681–5696, https://doi.org/10.5194/amt-16-5681-2023, https://doi.org/10.5194/amt-16-5681-2023, 2023
Short summary
Short summary
A nanosatellite was developed to obtain 1-D vertical temperature profiles in the mesosphere and lower thermosphere, which can be used to derive wave parameters needed for atmospheric models. A new processing method is shown, which allows one to extract two 1-D temperature profiles. The location of the two profiles is analyzed, as it is needed for deriving wave parameters. We show that this method is feasible, which however will increase the requirements of an accurate calibration and processing.
Francesco Cairo, Martina Krämer, Armin Afchine, Guido Di Donfrancesco, Luca Di Liberto, Sergey Khaykin, Lorenza Lucaferri, Valentin Mitev, Max Port, Christian Rolf, Marcel Snels, Nicole Spelten, Ralf Weigel, and Stephan Borrmann
Atmos. Meas. Tech., 16, 4899–4925, https://doi.org/10.5194/amt-16-4899-2023, https://doi.org/10.5194/amt-16-4899-2023, 2023
Short summary
Short summary
Cirrus clouds have been observed over the Himalayan region between 10 km and the tropopause at 17–18 km. Data from backscattersonde, hygrometers, and particle cloud spectrometers have been compared to assess their consistency. Empirical relationships between optical parameters accessible with remote sensing lidars and cloud microphysical parameters (such as ice water content, particle number and surface area density, and particle aspherical fraction) have been established.
Paul Konopka, Christian Rolf, Marc von Hobe, Sergey M. Khaykin, Benjamin Clouser, Elisabeth Moyer, Fabrizio Ravegnani, Francesco D'Amato, Silvia Viciani, Nicole Spelten, Armin Afchine, Martina Krämer, Fred Stroh, and Felix Ploeger
Atmos. Chem. Phys., 23, 12935–12947, https://doi.org/10.5194/acp-23-12935-2023, https://doi.org/10.5194/acp-23-12935-2023, 2023
Short summary
Short summary
We studied water vapor in a critical region of the atmosphere, the Asian summer monsoon anticyclone, using rare in situ observations. Our study shows that extremely high water vapor values observed in the stratosphere within the Asian monsoon anticyclone still undergo significant freeze-drying and that water vapor concentrations set by the Lagrangian dry point are a better proxy for the stratospheric water vapor budget than rare observations of enhanced water mixing ratios.
Frederik Harzer, Hella Garny, Felix Ploeger, Harald Bönisch, Peter Hoor, and Thomas Birner
Atmos. Chem. Phys., 23, 10661–10675, https://doi.org/10.5194/acp-23-10661-2023, https://doi.org/10.5194/acp-23-10661-2023, 2023
Short summary
Short summary
We study the statistical relation between year-by-year fluctuations in winter-mean ozone and the strength of the stratospheric polar vortex. In the latitude–pressure plane, regression analysis shows that anomalously weak polar vortex years are associated with three pronounced local ozone maxima over the polar cap relative to the winter climatology. These response maxima primarily reflect the non-trivial combination of different ozone transport processes with varying relative contributions.
Manfred Ern, Mohamadou A. Diallo, Dina Khordakova, Isabell Krisch, Peter Preusse, Oliver Reitebuch, Jörn Ungermann, and Martin Riese
Atmos. Chem. Phys., 23, 9549–9583, https://doi.org/10.5194/acp-23-9549-2023, https://doi.org/10.5194/acp-23-9549-2023, 2023
Short summary
Short summary
Quasi-biennial oscillation (QBO) of the stratospheric tropical winds is an important mode of climate variability but is not well reproduced in free-running climate models. We use the novel global wind observations by the Aeolus satellite and radiosondes to show that the QBO is captured well in three modern reanalyses (ERA-5, JRA-55, and MERRA-2). Good agreement is also found also between Aeolus and reanalyses for large-scale tropical wave modes in the upper troposphere and lower stratosphere.
Sebastian Rhode, Peter Preusse, Manfred Ern, Jörn Ungermann, Lukas Krasauskas, Julio Bacmeister, and Martin Riese
Atmos. Chem. Phys., 23, 7901–7934, https://doi.org/10.5194/acp-23-7901-2023, https://doi.org/10.5194/acp-23-7901-2023, 2023
Short summary
Short summary
Gravity waves (GWs) transport energy vertically and horizontally within the atmosphere and thereby affect wind speeds far from their sources. Here, we present a model that identifies orographic GW sources and predicts the pathways of the excited GWs through the atmosphere for a better understanding of horizontal GW propagation. We use this model to explain physical patterns in satellite observations (e.g., low GW activity above the Himalaya) and predict seasonal patterns of GW propagation.
Mathieu Ratynski, Sergey Khaykin, Alain Hauchecorne, Robin Wing, Jean-Pierre Cammas, Yann Hello, and Philippe Keckhut
Atmos. Meas. Tech., 16, 997–1016, https://doi.org/10.5194/amt-16-997-2023, https://doi.org/10.5194/amt-16-997-2023, 2023
Short summary
Short summary
Aeolus is the first spaceborne wind lidar providing global wind measurements since 2018. This study offers a comprehensive analysis of Aeolus instrument performance, using ground-based wind lidars and meteorological radiosondes, at tropical and mid-latitudes sites. The analysis allows assessing the long-term evolution of the satellite's performance for more than 3 years. The results will help further elaborate the understanding of the error sources and the behavior of the Doppler wind lidar.
Fayçal Lamraoui, Martina Krämer, Armin Afchine, Adam B. Sokol, Sergey Khaykin, Apoorva Pandey, and Zhiming Kuang
Atmos. Chem. Phys., 23, 2393–2419, https://doi.org/10.5194/acp-23-2393-2023, https://doi.org/10.5194/acp-23-2393-2023, 2023
Short summary
Short summary
Cirrus in the tropical tropopause layer (TTL) can play a key role in vertical transport. We investigate the role of different cloud regimes and the associated ice habits in regulating the properties of the TTL. We use high-resolution numerical experiments at the scales of large-eddy simulations (LESs) and aircraft measurements. We found that LES-scale parameterizations that predict ice shape are crucial for an accurate representation of TTL cirrus and thus the associated (de)hydration process.
Reimar Bauer, Jens-Uwe Grooß, Jörn Ungermann, May Bär, Markus Geldenhuys, and Lars Hoffmann
Geosci. Model Dev., 15, 8983–8997, https://doi.org/10.5194/gmd-15-8983-2022, https://doi.org/10.5194/gmd-15-8983-2022, 2022
Short summary
Short summary
The Mission Support System (MSS) is an open source software package that has been used for planning flight tracks of scientific aircraft in multiple measurement campaigns during the last decade. Here, we describe the MSS software and its use during the SouthTRAC measurement campaign in 2019. As an example for how the MSS software is used in conjunction with many datasets, we describe the planning of a single flight probing orographic gravity waves propagating up into the lower mesosphere.
Qiuyu Chen, Konstantin Ntokas, Björn Linder, Lukas Krasauskas, Manfred Ern, Peter Preusse, Jörn Ungermann, Erich Becker, Martin Kaufmann, and Martin Riese
Atmos. Meas. Tech., 15, 7071–7103, https://doi.org/10.5194/amt-15-7071-2022, https://doi.org/10.5194/amt-15-7071-2022, 2022
Short summary
Short summary
Observations of phase speed and direction spectra as well as zonal mean net gravity wave momentum flux are required to understand how gravity waves reach the mesosphere–lower thermosphere and how they there interact with background flow. To this end we propose flying two CubeSats, each deploying a spatial heterodyne spectrometer for limb observation of the airglow. End-to-end simulations demonstrate that individual gravity waves are retrieved faithfully for the expected instrument performance.
Manfred Ern, Peter Preusse, and Martin Riese
Atmos. Chem. Phys., 22, 15093–15133, https://doi.org/10.5194/acp-22-15093-2022, https://doi.org/10.5194/acp-22-15093-2022, 2022
Short summary
Short summary
Based on data from the HIRDLS and SABER infrared limb sounding satellite instruments, we investigate the intermittency of global distributions of gravity wave (GW) potential energies and GW momentum fluxes in the stratosphere and mesosphere using probability distribution functions (PDFs) and Gini coefficients. We compare GW intermittency in different regions, seasons, and altitudes. These results can help to improve GW parameterizations and the distributions of GWs resolved in models.
Markus Jesswein, Rafael P. Fernandez, Lucas Berná, Alfonso Saiz-Lopez, Jens-Uwe Grooß, Ryan Hossaini, Eric C. Apel, Rebecca S. Hornbrook, Elliot L. Atlas, Donald R. Blake, Stephen Montzka, Timo Keber, Tanja Schuck, Thomas Wagenhäuser, and Andreas Engel
Atmos. Chem. Phys., 22, 15049–15070, https://doi.org/10.5194/acp-22-15049-2022, https://doi.org/10.5194/acp-22-15049-2022, 2022
Short summary
Short summary
This study presents the global and seasonal distribution of the two major brominated short-lived substances CH2Br2 and CHBr3 in the upper troposphere and lower stratosphere based on observations from several aircraft campaigns. They show similar seasonality for both hemispheres, except in the respective hemispheric autumn lower stratosphere. A comparison with the TOMCAT and CAM-Chem models shows good agreement in the annual mean but larger differences in the seasonal consideration.
Bernard Legras, Clair Duchamp, Pasquale Sellitto, Aurélien Podglajen, Elisa Carboni, Richard Siddans, Jens-Uwe Grooß, Sergey Khaykin, and Felix Ploeger
Atmos. Chem. Phys., 22, 14957–14970, https://doi.org/10.5194/acp-22-14957-2022, https://doi.org/10.5194/acp-22-14957-2022, 2022
Short summary
Short summary
The long-duration atmospheric impact of the Tonga eruption in January 2022 is a plume of water and sulfate aerosols in the stratosphere that persisted for more than 6 months. We study this evolution using several satellite instruments and analyse the unusual behaviour of this plume as sulfates and water first moved down rapidly and then separated into two layers. We also report the self-organization in compact and long-lived patches.
Paul Konopka, Mengchu Tao, Marc von Hobe, Lars Hoffmann, Corinna Kloss, Fabrizio Ravegnani, C. Michael Volk, Valentin Lauther, Andreas Zahn, Peter Hoor, and Felix Ploeger
Geosci. Model Dev., 15, 7471–7487, https://doi.org/10.5194/gmd-15-7471-2022, https://doi.org/10.5194/gmd-15-7471-2022, 2022
Short summary
Short summary
Pure trajectory-based transport models driven by meteorology derived from reanalysis products (ERA5) take into account only the resolved, advective part of transport. That means neither mixing processes nor unresolved subgrid-scale advective processes like convection are included. The Chemical Lagrangian Model of the Stratosphere (CLaMS) includes these processes. We show that isentropic mixing dominates unresolved transport. The second most important transport process is unresolved convection.
Clare E. Singer, Benjamin W. Clouser, Sergey M. Khaykin, Martina Krämer, Francesco Cairo, Thomas Peter, Alexey Lykov, Christian Rolf, Nicole Spelten, Armin Afchine, Simone Brunamonti, and Elisabeth J. Moyer
Atmos. Meas. Tech., 15, 4767–4783, https://doi.org/10.5194/amt-15-4767-2022, https://doi.org/10.5194/amt-15-4767-2022, 2022
Short summary
Short summary
In situ measurements of water vapor in the upper troposphere are necessary to study cloud formation and hydration of the stratosphere but challenging due to cold–dry conditions. We compare measurements from three water vapor instruments from the StratoClim campaign in 2017. In clear sky (clouds), point-by-point differences were <1.5±8 % (<1±8 %). This excellent agreement allows detection of fine-scale structures required to understand the impact of convection on stratospheric water vapor.
Liubov Poshyvailo-Strube, Rolf Müller, Stephan Fueglistaler, Michaela I. Hegglin, Johannes C. Laube, C. Michael Volk, and Felix Ploeger
Atmos. Chem. Phys., 22, 9895–9914, https://doi.org/10.5194/acp-22-9895-2022, https://doi.org/10.5194/acp-22-9895-2022, 2022
Short summary
Short summary
Brewer–Dobson circulation (BDC) controls the composition of the stratosphere, which in turn affects radiation and climate. As the BDC cannot be measured directly, it is necessary to infer its strength and trends indirectly. In this study, we test in the
model worlddifferent methods for estimating the mean age of air trends based on a combination of stratospheric water vapour and methane data. We also provide simple practical advice of a more reliable estimation of the mean age of air trends.
Suvarna Fadnavis, Prashant Chavan, Akash Joshi, Sunil M. Sonbawne, Asutosh Acharya, Panuganti C. S. Devara, Alexandru Rap, Felix Ploeger, and Rolf Müller
Atmos. Chem. Phys., 22, 7179–7191, https://doi.org/10.5194/acp-22-7179-2022, https://doi.org/10.5194/acp-22-7179-2022, 2022
Short summary
Short summary
We show that large amounts of anthropogenic aerosols are transported from South Asia to the northern Indian Ocean. These aerosols are then lifted into the UTLS by the ascending branch of the Hadley circulation. They are further transported to the Southern Hemisphere and downward via westerly ducts over the tropical Atlantic and Pacific. These aerosols increase tropospheric heating, resulting in an increase in water vapor, which is then transported to the UTLS.
Felix Ploeger and Hella Garny
Atmos. Chem. Phys., 22, 5559–5576, https://doi.org/10.5194/acp-22-5559-2022, https://doi.org/10.5194/acp-22-5559-2022, 2022
Short summary
Short summary
We investigate hemispheric asymmetries in stratospheric circulation changes in the last 2 decades in model simulations and atmospheric observations. We find that observed trace gas changes can be explained by a structural circulation change related to a deepening circulation in the Northern Hemisphere relative to the Southern Hemisphere. As this asymmetric signal is small compared to internal variability observed circulation trends over the recent past are not in contradiction to climate models.
Jan Clemens, Felix Ploeger, Paul Konopka, Raphael Portmann, Michael Sprenger, and Heini Wernli
Atmos. Chem. Phys., 22, 3841–3860, https://doi.org/10.5194/acp-22-3841-2022, https://doi.org/10.5194/acp-22-3841-2022, 2022
Short summary
Short summary
Highly polluted air flows from the surface to higher levels of the atmosphere during the Asian summer monsoon. At high levels, the air is trapped within eddies. Here, we study how air masses can leave the eddy within its cutoff, how they distribute, and how their chemical composition changes. We found evidence for transport from the eddy to higher latitudes over the North Pacific and even Alaska. During transport, trace gas concentrations within cutoffs changed gradually, showing steady mixing.
Helmut Ziereis, Peter Hoor, Jens-Uwe Grooß, Andreas Zahn, Greta Stratmann, Paul Stock, Michael Lichtenstern, Jens Krause, Vera Bense, Armin Afchine, Christian Rolf, Wolfgang Woiwode, Marleen Braun, Jörn Ungermann, Andreas Marsing, Christiane Voigt, Andreas Engel, Björn-Martin Sinnhuber, and Hermann Oelhaf
Atmos. Chem. Phys., 22, 3631–3654, https://doi.org/10.5194/acp-22-3631-2022, https://doi.org/10.5194/acp-22-3631-2022, 2022
Short summary
Short summary
Airborne observations were conducted in the lowermost Arctic stratosphere during the winter of 2015/2016. The observed distribution of reactive nitrogen shows clear indications of nitrification in mid-winter and denitrification in late winter. This was caused by the formation of polar stratospheric cloud particles, which were observed during several flights. The sedimentation and evaporation of these particles and the descent of air masses cause a redistribution of reactive nitrogen.
Sergey M. Khaykin, Elizabeth Moyer, Martina Krämer, Benjamin Clouser, Silvia Bucci, Bernard Legras, Alexey Lykov, Armin Afchine, Francesco Cairo, Ivan Formanyuk, Valentin Mitev, Renaud Matthey, Christian Rolf, Clare E. Singer, Nicole Spelten, Vasiliy Volkov, Vladimir Yushkov, and Fred Stroh
Atmos. Chem. Phys., 22, 3169–3189, https://doi.org/10.5194/acp-22-3169-2022, https://doi.org/10.5194/acp-22-3169-2022, 2022
Short summary
Short summary
The Asian monsoon anticyclone is the key contributor to the global annual maximum in lower stratospheric water vapour. We investigate the impact of deep convection on the lower stratospheric water using a unique set of observations aboard the high-altitude M55-Geophysica aircraft deployed in Nepal in summer 2017 within the EU StratoClim project. We find that convective plumes of wet air can persist within the Asian anticyclone for weeks, thereby enhancing the occurrence of high-level clouds.
Dina Khordakova, Christian Rolf, Jens-Uwe Grooß, Rolf Müller, Paul Konopka, Andreas Wieser, Martina Krämer, and Martin Riese
Atmos. Chem. Phys., 22, 1059–1079, https://doi.org/10.5194/acp-22-1059-2022, https://doi.org/10.5194/acp-22-1059-2022, 2022
Short summary
Short summary
Extreme storms transport humidity from the troposphere to the stratosphere. Here it has a strong impact on the climate. With ongoing global warming, we expect more storms and, hence, an enhancement of this effect. A case study was performed in order to measure the impact of the direct injection of water vapor into the lower stratosphere. The measurements displayed a significant transport of water vapor into the lower stratosphere, and this was supported by satellite and reanalysis data.
Abhinna K. Behera, Emmanuel D. Rivière, Sergey M. Khaykin, Virginie Marécal, Mélanie Ghysels, Jérémie Burgalat, and Gerhard Held
Atmos. Chem. Phys., 22, 881–901, https://doi.org/10.5194/acp-22-881-2022, https://doi.org/10.5194/acp-22-881-2022, 2022
Short summary
Short summary
Deep convection overshooting the stratosphere's contribution to the global stratospheric water budget is still being quantified. We ran three different cloud-resolving simulations of an observed case of overshoots in Bauru during the TRO-Pico balloon campaign in the context of upscaling the impact of overshoots at a large scale. These simulations, which have been validated with balloon-borne and S-band radar measurements, shed light on the local-scale variability and composition of overshoots.
Manuel Baumgartner, Christian Rolf, Jens-Uwe Grooß, Julia Schneider, Tobias Schorr, Ottmar Möhler, Peter Spichtinger, and Martina Krämer
Atmos. Chem. Phys., 22, 65–91, https://doi.org/10.5194/acp-22-65-2022, https://doi.org/10.5194/acp-22-65-2022, 2022
Short summary
Short summary
An important mechanism for the appearance of ice particles in the upper troposphere at low temperatures is homogeneous nucleation. This process is commonly described by the
Koop line, predicting the humidity at freezing. However, laboratory measurements suggest that the freezing humidities are above the Koop line, motivating the present study to investigate the influence of different physical parameterizations on the homogeneous freezing with the help of a detailed numerical model.
Cornelia Strube, Peter Preusse, Manfred Ern, and Martin Riese
Atmos. Chem. Phys., 21, 18641–18668, https://doi.org/10.5194/acp-21-18641-2021, https://doi.org/10.5194/acp-21-18641-2021, 2021
Short summary
Short summary
High gravity wave (GW) momentum fluxes in the lower stratospheric southern polar vortex around 60° S are still poorly understood. Few GW sources are found at these latitudes. We present a ray tracing case study on waves resolved in high-resolution global model temperatures southeast of New Zealand. We show that lateral propagation of more than 1000 km takes place below 20 km altitude, and a variety of orographic and non-orographic sources located north of 50° S generate the wave field.
Meike K. Rotermund, Vera Bense, Martyn P. Chipperfield, Andreas Engel, Jens-Uwe Grooß, Peter Hoor, Tilman Hüneke, Timo Keber, Flora Kluge, Benjamin Schreiner, Tanja Schuck, Bärbel Vogel, Andreas Zahn, and Klaus Pfeilsticker
Atmos. Chem. Phys., 21, 15375–15407, https://doi.org/10.5194/acp-21-15375-2021, https://doi.org/10.5194/acp-21-15375-2021, 2021
Short summary
Short summary
Airborne total bromine (Brtot) and tracer measurements suggest Brtot-rich air masses persistently protruded into the lower stratosphere (LS), creating a high Brtot region over the North Atlantic in fall 2017. The main source is via isentropic transport by the Asian monsoon and to a lesser extent transport across the extratropical tropopause as quantified by a Lagrange model. The transport of Brtot via Central American hurricanes is also observed. Lastly, the impact of Brtot on LS O3 is assessed.
Christoph Mahnke, Ralf Weigel, Francesco Cairo, Jean-Paul Vernier, Armin Afchine, Martina Krämer, Valentin Mitev, Renaud Matthey, Silvia Viciani, Francesco D'Amato, Felix Ploeger, Terry Deshler, and Stephan Borrmann
Atmos. Chem. Phys., 21, 15259–15282, https://doi.org/10.5194/acp-21-15259-2021, https://doi.org/10.5194/acp-21-15259-2021, 2021
Short summary
Short summary
In 2017, in situ aerosol measurements were conducted aboard the M55 Geophysica in the Asian monsoon region. The vertical particle mixing ratio profiles show a distinct layer (15–18.5 km), the Asian tropopause aerosol layer (ATAL). The backscatter ratio (BR) was calculated based on the aerosol size distributions and compared with the BRs detected by a backscatter probe and a lidar aboard M55, and by the CALIOP lidar. All four methods show enhanced BRs in the ATAL altitude range (max. at 17.5 km).
Cited articles
Abalos, M., Ploeger, F., Konopka, P., Randel, W. J., and Serrano, E.: Ozone seasonality above the tropical tropopause: reconciling the Eulerian and Lagrangian perspectives of transport processes, Atmos. Chem. Phys., 13, 10787–10794, https://doi.org/10.5194/acp-13-10787-2013, 2013. a, b
Andrews, D. G., Holton, J. R., and Leovy, C. B.: Middle Atmosphere Dynamics,
vol. 40 of International Geophysics Series, Academic Press, San
Diego, USA, 1987. a
Anstey, J. A., Banyard, T. P., Butchart, N., Coy, L., Newman, P. A., Osprey,
S., and Wright, C. J.: Quasi-biennial oscillation disrupted by abnormal
Southern Hemisphere stratosphere, Earth and Space Science Open Archive,
https://doi.org/10.1002/essoar.10503358.1, 2020. a
Anstey, J. A., Banyard, T. P., Butchart, N., Coy, L., Newman, P. A., Osprey,
S., and Wright, C. J.: Prospect of increased disruption to the QBO in a
changing climate, Geophys. Res. Lett., 48, e2021GL093058, https://doi.org/10.1029/2021GL093058,
2021. a, b
Baldwin, M. P., Gray, L. J., Dunkerton, T. J., Hamilton, K., Haynes, P. H.,
Randel, W. J., Holton, J. R., Alexander, M. J., Hirota, I., Horinouchi, T.,
Jones, D. B. A., Kinnersley, J. S., Marquardt, C., Sato, K., and Takahashi,
M.: The quasi-biennial oscillation, Rev. Geophys., 39, 179–229,
https://doi.org/10.1029/1999RG000073, 2001. a
Barton, C. A. and McCormack, J. P.: Origin of the 2016 QBO Disruption and Its
Relationship to Extreme El Niño Events, Geophys. Res. Lett., 44, 11150–11157,
https://doi.org/10.1002/2017GL075576, 2017. a, b
Brewer, A.: Evidence for a world circulation provided by the measurements of
helium and water vapour distribution in the stratosphere, Q. J. R. Meteorol.
Soc., 75, 351–363, 1949. a
Brinkop, S., Dameris, M., Jöckel, P., Garny, H., Lossow, S., and Stiller, G.: The millennium water vapour drop in chemistry–climate model simulations, Atmos. Chem. Phys., 16, 8125–8140, https://doi.org/10.5194/acp-16-8125-2016, 2016. a, b
Butchart, N.: The Brewer-Dobson circulation, Rev. Geophys., 52, 157–184,
https://doi.org/10.1002/2013RG000448, 2014. a, b
Butchart, N. and Scaife, A. A.: Removal of chlorofluorocarbons by increased
mass exchange between the stratosphere and troposphere in a changing
climate., Nature, 410, 799–802, https://doi.org/10.1038/35071047, 2001. a
Cai, W., Borlace, S., Lengaigne, M., van Rensch, P., Collins, M., Vecchi, G.,
Timmermann, A., Santoso, A., McPhaden, M. J., Wu, L., England, M. H., Wang,
G., Guilyardi, E., and Jin, F.-F.: Increasing frequency of extreme El Niño
events due to greenhouse warming, Nat. Clim. Change, 4, 111–116,
https://doi.org/10.1038/nclimate2100, 2014. a
Christiansen, B., Yang, S., and Madsen, M. S.: Do strong warm ENSO events
control the phase of the stratospheric QBO?, Geophys. Res. Lett., 43,
10489–10495, https://doi.org/10.1002/2016GL070751, 2016. a, b
Cicerone, R. J.: Changes in stratospheric ozone, Science, 237, 35–42,
https://doi.org/10.1126/science.237.4810.35, 1987. a
Coy, L., Newman, P. A., Pawson, S., and Lait, L. R.: Dynamics of the Disrupted
2015/16 Quasi-Biennial Oscillation, J. Clim., 30, 5661–5674,
https://doi.org/10.1175/JCLI-D-16-0663.1, 2017. a, b
DallaSanta, K., Orbe, C., Rind, D., Nazarenko, L., and Jonas, J.: Response of
the Quasi-Biennial Oscillation to Historical Volcanic Eruptions, Geophys.
Res. Lett., 48, e2021GL095412,
https://doi.org/10.1029/2021GL095412, 2021. a, b
Damadeo, R. P., Zawodny, J. M., and Thomason, L. W.: Reevaluation of stratospheric ozone trends from SAGE II data using a simultaneous temporal and spatial analysis, Atmos. Chem. Phys., 14, 13455–13470, https://doi.org/10.5194/acp-14-13455-2014, 2014. a
Dessler, A. E., Schoeberl, M. R., Wang, T., Davis, S. M., and Rosenlof, K. H.:
Stratospheric water vapor feedback, P. Natl. Acad. Sci. USA, 110,
18087–18091, https://doi.org/10.1073/pnas.1310344110, 2013. a
Dessler, A. E., Schoeberl, M. R., Wang, T., Davis, S. M., Rosenlof, K. H., and
Vernier, J.-P.: Variations of stratospheric water vapor over the past three
decades, J. Geophys. Res.-Atmos., 119, 12588–12598,
https://doi.org/10.1002/2014JD021712, 2014. a
Diallo, M., Ploeger, F., Konopka, P., Birner, T., Müller, R., Riese, M.,
Garny, H., Legras, B., Ray, E., Berthet, G., and Jegou, F.: Significant
Contributions of Volcanic Aerosols to Decadal Changes in the Stratospheric
Circulation, Geophys. Res. Lett., 44, 10780–10791,
https://doi.org/10.1002/2017GL074662, 2017. a, b
Diallo, M., Riese, M., Birner, T., Konopka, P., Müller, R., Hegglin, M. I., Santee, M. L., Baldwin, M., Legras, B., and Ploeger, F.: Response of stratospheric water vapor and ozone to the unusual timing of El Niño and the QBO disruption in 2015–2016, Atmos. Chem. Phys., 18, 13055–13073, https://doi.org/10.5194/acp-18-13055-2018, 2018. a, b, c, d, e, f, g, h, i, j, k
Diallo, M., Konopka, P., Santee, M. L., Müller, R., Tao, M., Walker, K. A., Legras, B., Riese, M., Ern, M., and Ploeger, F.: Structural changes in the shallow and transition branch of the Brewer–Dobson circulation induced by El Niño, Atmos. Chem. Phys., 19, 425–446, https://doi.org/10.5194/acp-19-425-2019, 2019. a, b
Diallo, M., Ern, M., and Ploeger, F.: The advective Brewer–Dobson circulation in the ERA5 reanalysis: climatology, variability, and trends, Atmos. Chem. Phys., 21, 7515–7544, https://doi.org/10.5194/acp-21-7515-2021, 2021. a, b, c, d
Dunkerton, T. J.: A Lagrangian mean theory of wave, mean-Flow interaction with
applications to nonacceleration and its breakdown, Rev. Geophys., 18,
387–400, https://doi.org/10.1029/RG018i002p00387, 1980. a
Dunkerton, T. J.: The quasi-biennial oscillation of 2015–2016: Hiccup or
death spiral?, Geophys. Res. Lett., 43, 10547–10552,
https://doi.org/10.1002/2016GL070921, 2016. a, b
Ern, M., Ploeger, F., Preusse, P., Gille, J. C., Gray, L. J., Kalisch, S.,
Mlynczak, M. G., Russell, J. M., and Riese, M.: Interaction of gravity waves
with the QBO: A satellite perspective, J. Geophys. Res.-Atmos., 119,
2329–2355, https://doi.org/10.1002/2013JD020731, 2014. a, b, c
Ern, M., Diallo, M., Preusse, P., Mlynczak, M. G., Schwartz, M. J., Wu, Q., and Riese, M.: The semiannual oscillation (SAO) in the tropical middle atmosphere and its gravity wave driving in reanalyses and satellite observations, Atmos. Chem. Phys., 21, 13763–13795, https://doi.org/10.5194/acp-21-13763-2021, 2021. a, b
Forster, P. M. and Shine, K. P.: Stratospheric water vapour changes as a
possible contributor to observed stratospheric cooling, Geophys. Res. Lett.,
26, 3309–3312, https://doi.org/10.1029/1999GL010487, 1999. a, b
Forster, P. M. and Shine, K. P.: Assessing the climate impact of trends in
stratospheric water vapor, Geophys. Res. Lett., 29, 10-1–10-4,
https://doi.org/10.1029/2001GL013909, 2002. a
Friston, K., Ashburner, J., Kiebel, S. J., Nichols, T. E., and Penny, W. D.,
eds.: Statistical Parametric Mapping: The Analysis of Functional Brain
Images, Academic Press,
http://store.elsevier.com/product.jsp?isbn=9780123725608 (last access: 27 October 2022),
2007. a
Fueglistaler, S., Dessler, A. E., Dunkerton, T. J., Folkins, I., Fu,
Q., and Mote, P. W.: Tropical Tropopause Layer, Rev. Geophys., 47, G1004+,
https://doi.org/10.1029/2008RG000267, 2009. a
Fujiwara, M., Suzuki, J., Gettelman, A., Hegglin, M. I., Akiyoshi, H., and
Shibata, K.: Wave activity in the tropical tropopause layer in seven
reanalysis and four chemistry climate model data sets, J. Geophys. Res.-Atmos., 117, https://doi.org/10.1029/2011JD016808, 2012. a
Garfinkel, C. I., Hurwitz, M. M., Oman, L. D., and Waugh, D. W.: Contrasting
Effects of Central Pacific and Eastern Pacific El Niño on stratospheric
water vapor, Geophys. Res. Lett., 40, 4115–4120, https://doi.org/10.1002/grl.50677,
2013. a
Geller, M. A., Zhou, X., and Zhang, M.: Simulations of the Interannual
Variability of Stratospheric Water Vapor, J. Atmos. Sci., 59, 1076–1085,
https://doi.org/10.1175/1520-0469(2002)059<1076:SOTIVO>2.0.CO;2, 2002. a
Gettelman, A., Hoor, P., Pan, L. L., Randel, W. J., Hegglin, M. I., and Birner,
T.: The extratropical upper troposphere and lower stratosphere, Rev.
Geophys., 49, RG3003, https://doi.org/10.1029/2011RG000355, 2011. a
Grimshaw, R.: Wave Action and Wave–Mean Flow Interaction, with Application to
Stratified Shear Flows, Annual Rev. of Fluid Mech., 16, 11–44,
https://doi.org/10.1146/annurev.fl.16.010184.000303, 1984. a
Hartmann, D. L., Holton, J. R., and Fu, Q.: The heat balance of the tropical
tropopause, cirrus, and stratospheric dehydration, Geophys. Res. Lett., 28,
1969–1972, https://doi.org/10.1029/2000GL012833, 2001. a
Haynes, P. H. and Shuckburgh, E.: Effective diffusivity as a diagnostic of
atmospheric transport 2. Troposphere and lower stratosphere,
J. Geophys. Res., 105, 22795–22810, https://doi.org/10.1029/2000JD900092, 2000. a
Haynes, P. H., McIntyre, M. E., Shepherd, T. G., Marks, C. J., and Shine,
K. P.: On the “Downward Control” of Extratropical Diabatic Circulations by
Eddy-Induced Mean Zonal Forces, J. Atmos. Sci., 48, 651–678,
https://doi.org/10.1175/1520-0469(1991)048<0651:OTCOED>2.0.CO;2, 1991. a
Hegglin, M. I., Tegtmeier, S., Anderson, J., Froidevaux, L., Fuller, R., Funke,
B., Jones, A., Lingenfelser, G., Lumpe, J., Pendlebury, D., Remsberg, E.,
Rozanov, A., Toohey, M., Urban, J., Clarmann, T., Walker, K. A., Wang, R.,
and Weigel, K.: SPARC Data Initiative: Comparison of water vapor
climatologies from international satellite limb sounders, J. Geophys. Res.-Atmos., 118, 11824–11846, https://doi.org/10.1002/jgrd.50752, 2013. a
Hegglin, M. I., Tegtmeier, S., Anderson, J., Bourassa, A. E., Brohede, S., Degenstein, D., Froidevaux, L., Funke, B., Gille, J., Kasai, Y., Kyrölä, E. T., Lumpe, J., Murtagh, D., Neu, J. L., Pérot, K., Remsberg, E. E., Rozanov, A., Toohey, M., Urban, J., von Clarmann, T., Walker, K. A., Wang, H.-J., Arosio, C., Damadeo, R., Fuller, R. A., Lingenfelser, G., McLinden, C., Pendlebury, D., Roth, C., Ryan, N. J., Sioris, C., Smith, L., and Weigel, K.: Overview and update of the SPARC Data Initiative: comparison of stratospheric composition measurements from satellite limb sounders, Earth Syst. Sci. Data, 13, 1855–1903, https://doi.org/10.5194/essd-13-1855-2021, 2021. a
Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A.,
Muñoz-Sabater, J., Nicolas, J., Peubey, C., Radu, R., Schepers, D., Simmons,
A., Soci, C., Abdalla, S., Abellan, X., Balsamo, G., Bechtold, P., Biavati,
G., Bidlot, J., Bonavita, M., De Chiara, G., Dahlgren, P., Dee, D.,
Diamantakis, M., Dragani, R., Flemming, J., Forbes, R., Fuentes, M., Geer,
A., Haimberger, L., Healy, S., Hogan, R. J., Hólm, E., Janisková, M.,
Keeley, S., Laloyaux, P., Lopez, P., Lupu, C., Radnoti, G., de Rosnay, P.,
Rozum, I., Vamborg, F., Villaume, S., and Thépaut, J.-N.: The ERA5 Global
Reanalysis, Q. J. R. Meteorol. Soc., 146, 1999–2049, https://doi.org/10.1002/qj.3803, 2020. a, b
Hitchcock, P., Haynes, P. H., Randel, W. J., and Birner, T.: The Emergence of
Shallow Easterly Jets within QBO Westerlies, J. Atmos. Sci., 75, 21–40,
https://doi.org/10.1175/JAS-D-17-0108.1, 2018. a
Holton, J. R.: Equatorial Wave-Mean Flow Interaction: A Numerical Study of the
Role of Latitudinal Shear, J. Atmos. Sci., 36, 1030–1040,
https://doi.org/10.1175/1520-0469(1979)036<1030:EWMFIA>2.0.CO;2, 1979. a
Holton, J. R. and Gettelman, A.: Horizontal transport and the dehydration of
the stratosphere, Geophys. Res. Lett., 28, 2799–2802,
https://doi.org/10.1029/2001GL013148, 2001. a, b, c
Holton, J. R. and Tan, H.-C.: The Influence of the Equatorial Quasi-Biennial
Oscillation on the Global Circulation at 50 mb, J. Atmos.
Sci., 37, 2200–2208,
https://doi.org/10.1175/1520-0469(1980)037<2200:TIOTEQ>2.0.CO;2, 1980. a
Hu, D., Tian, W., Guan, Z., Guo, Y., and Dhomse, S.: Longitudinal Asymmetric
Trends of Tropical Cold-Point Tropopause Temperature and Their Link to
Strengthened Walker Circulation, J. Clim., 29, 7755–7771,
https://doi.org/10.1175/JCLI-D-15-0851.1, 2016. a, b
Iglesias-Suarez, F., Wild, O., Kinnison, D. E., Garcia, R. R., Marsh, D. R.,
Lamarque, J.-F., Ryan, E. M., Davis, S. M., Eichinger, R., Saiz-Lopez, A.,
and Young, P. J.: Tropical Stratospheric Circulation and Ozone Coupled to
Pacific Multi-Decadal Variability, Geophys. Res. Lett., 48,
e2020GL092162, https://doi.org/10.1029/2020GL092162, 2021. a
Ihara, C., Kushnir, Y., and Cane, M. A.: Warming Trend of the Indian Ocean SST
and Indian Ocean Dipole from 1880 to 2004, J. Clim., 21, 2035–2046,
https://doi.org/10.1175/2007JCLI1945.1, 2008. a
Jensen, E. J., Toon, O. B., Pfister, L., and Selkirk, H. B.: Dehydration of
the upper troposphere and lower stratosphere by subvisible cirrus clouds near
the tropical tropopause, Geophys. Res. Lett., 23, 825–828,
https://doi.org/10.1029/96GL00722, 1996. a
Jia, J. Y., Preusse, P., Ern, M., Chun, H.-Y., Gille, J. C., Eckermann, S. D., and Riese, M.: Sea surface temperature as a proxy for convective gravity wave excitation: a study based on global gravity wave observations in the middle atmosphere, Ann. Geophys., 32, 1373–1394, https://doi.org/10.5194/angeo-32-1373-2014, 2014. a
Kang, M.-J. and Chun, H.-Y.: Contributions of equatorial waves and small-scale convective gravity waves to the 2019/20 quasi-biennial oscillation (QBO) disruption, Atmos. Chem. Phys., 21, 9839–9857, https://doi.org/10.5194/acp-21-9839-2021, 2021. a, b, c, d
Kang, M.-J., Chun, H.-Y., and Garcia, R. R.: Role of equatorial waves and convective gravity waves in the 2015/16 quasi-biennial oscillation disruption, Atmos. Chem. Phys., 20, 14669–14693, https://doi.org/10.5194/acp-20-14669-2020, 2020. a, b, c, d
Kawatani, Y. and Hamilton, K.: Weakened stratospheric quasibiennial
oscillation driven by increased tropical mean upwelling, Nature, 497,
478–481, https://doi.org/10.1038/nature12140, 2013. a, b
Kawatani, Y., Hamilton, K., and Watanabe, S.: The Quasi-Biennial Oscillation
in a Double CO2 Climate, J. Atmos. Sci., 68, 265–283,
https://doi.org/10.1175/2010JAS3623.1, 2011. a
Kawatani, Y., Hamilton, K., Miyazaki, K., Fujiwara, M., and Anstey, J. A.: Representation of the tropical stratospheric zonal wind in global atmospheric reanalyses, Atmos. Chem. Phys., 16, 6681–6699, https://doi.org/10.5194/acp-16-6681-2016, 2016. a
Khaykin, S., Legras, B., and Bucci, S., Sellitto, P.,
Isaksen, L., Tencé, F., Bekki, S., Bourassa, A., Rieger, L., Zawada, D., and Jumelet, J.: The 2019/20 Australian wildfires
generated a persistent smoket charged vortex rising up to 35 km altitude,
Commun. Earth Environ., 1, 22, https://doi.org/10.1038/s43247-020-00022-5, 2020. a, b, c, d, e
Kim, J. and Son, S.-W.: Tropical Cold-Point Tropopause: Climatology, Seasonal
Cycle, and Intraseasonal Variability Derived from COSMIC GPS Radio
Occultation Measurements, J. Clim., 25, 5343–5360,
https://doi.org/10.1175/JCLI-D-11-00554.1, 2012. a
Kim, Y.-H. and Chun, H.-Y.: Momentum forcing of the quasi-biennial oscillation by equatorial waves in recent reanalyses, Atmos. Chem. Phys., 15, 6577–6587, https://doi.org/10.5194/acp-15-6577-2015, 2015. a, b
Kroll, C. A., Dacie, S., Azoulay, A., Schmidt, H., and Timmreck, C.: The impact of volcanic eruptions of different magnitude on stratospheric water vapor in the tropics, Atmos. Chem. Phys., 21, 6565–6591, https://doi.org/10.5194/acp-21-6565-2021, 2021. a, b
Langematz, U.: Stratospheric ozone: down and up through the anthropocene,
ChemTexts, 5, 8, https://doi.org/10.1007/s40828-019-0082-7, 2019. a
Lambert, A., Read, W. and Livesey, N.: MLS/Aura Level 2 Water Vapor (H2O) Mixing Ratio V005, Greenbelt, MD, USA, Goddard Earth Sciences Data and Information Services Center (GES DISC) [data set], https://doi.org/10.5067/Aura/MLS/DATA2508, 2020. a
Liess, S. and Geller, M. A.: On the relationship between QBO and distribution
of tropical deep convection, J. Geophys. Res.-Atmos., 117, D03108,
https://doi.org/10.1029/2011JD016317, 2012. a
Lin, P. and Fu, Q.: Changes in various branches of the Brewer–Dobson
circulation from an ensemble of chemistry climate models, J. Geophys. Res.-Atmos., 118, 73–84, https://doi.org/10.1029/2012JD018813, 2013. a
Lin, P., Held, I., and Ming, Y.: The Early Development of the 2015/16
Quasi-Biennial Oscillation Disruption, J. Atmos.-Sci.,
76, 821–836, https://doi.org/10.1175/JAS-D-18-0292.1, 2019. a
Lindzen, R. S.: Equatorial Planetary Waves in Shear. Part I, J. Atmos.
Sci., 28, 609–622, https://doi.org/10.1175/1520-0469(1971)028<0609:EPWISP>2.0.CO;2,
1971. a
Livesey, N. J., Read, W. G., Wagner, P. A., Froidevaux, L., Lambert, A.,
Manney, G. L., Millán Valle, L. F., Pumphrey, H. C., Santee, M. L.,
Schwartz, M. J., Wang, S., Fuller, R. A., Jarnot, R. F., Knosp, B. W., and
Martinez, E.: Aura Microwave Limb Sounder (MLS) Version 4.2x Level 2 data
quality and description document, Tech. Rep. JPL D-33509 Rev. C, 1–169,
https://mls.jpl.nasa.gov/data/v4-2_data_quality_document.pdf (last access: 4 November 2022), 2017. a, b
Match, A. and Fueglistaler, S.: Anomalous Dynamics of QBO Disruptions Explained
by 1D Theory with External Triggering, J. Atmos. Sci.,
78, 373–383, https://doi.org/10.1175/JAS-D-20-0172.1, 2021. a, b, c
Mote, P. W., Rosenlof, K. H., M. Mclntyre, M. E., Carr, E. S., Gille, J. C.,
Holton, J. R., Kinnersley, J. S., Pumphrey, H. C., Russell III, J. M., and
Waters, J. W.: An atmospheric tape recorder: The imprint of
tropical tropopause temperatures on stratospheric water vapor, J. Geophys.
Res., 101, 3989–4006, 1996. a
Newman, P. A. and Nash, E. R.: Quantifying the wave driving of the
stratosphere, J. Geophys. Res.-Atmos., 105, 12485–12497,
https://doi.org/10.1029/1999JD901191, 2000. a
Newman, P. A., Coy, L., Pawson, S., and Lait, L. R.: The anomalous change in
the QBO in 2015–2016, Geophys. Res. Lett., 43, 8791–8797,
https://doi.org/10.1002/2016GL070373, 2016. a, b
Niwano, M., Yamazaki, K., and Shiotani, M.: Seasonal and QBO variations of
ascent rate in the tropical lower stratosphere as inferred from UARS HALOE
trace gas data, J. Geophys. Res., 108, 4794, https://doi.org/10.1029/2003JD003871, 2003. a
Nowack, P., Abraham, N., Maycock, A., Braesicke, P., Gregory, J., Joshi, M.,
Osprey, A., and Pyle, J.: A large ozone-circulation feedback and its
implications for global warming assessments, Nat. Clim. Change, 5,
41–45, https://doi.org/10.1038/NCLIMATE2451, 2015. a
Osprey, S. M., Butchart, N., Knight, J. R., Scaife, A. A., Hamilton, K.,
Anstey, J. A., Schenzinger, V., and Zhang, C.: An unexpected disruption of
the atmospheric quasi-biennial oscillation, Science, 353, 1424–1427,
https://doi.org/10.1126/science.aah4156, 2016. a, b, c, d
Peterson, D. A., Fromm, M. D., McRae, R. H. D., Campbell, J. R., Hyer, Edward
J. Taha, G., Camacho, C. P., Kablick, G. P., Schmidt, C. C., and DeLand,
M. T.: Australia’s Black Summer pyrocumulonimbus super outbreak reveals
potential for increasingly extreme stratospheric smoke events, npj Clima.
Atmos. Sci., 4, 2397–3722, https://doi.org/10.1038/s41612-021-00192-9, 2021. a, b, c, d
Plumb, R. A.: The Interaction of Two Internal Waves with the Mean Flow:
Implications for the Theory of the Quasi-Biennial Oscillation, J.
Atmos. Sci., 34, 1847–1858,
https://doi.org/10.1175/1520-0469(1977)034<1847:TIOTIW>2.0.CO;2, 1977. a
Plumb, R. A.: Stratospheric transport, J. Meteor. Soc. Jpn., 80, 793–809,
2002. a
Plumb, R. A. and Bell, R. C.: A model of the quasi-biennial oscillation on an
equatorial beta-plane, Q. J. Roy. Meteorol. Soc.,
108, 335–352, https://doi.org/10.1002/qj.49710845604, 1982. a, b, c
Randel, W. and Park, M.: Diagnosing Observed Stratospheric Water Vapor
Relationships to the Cold Point Tropical Tropopause, J. Geophys. Res.-Atmos., 124, 7018–7033, https://doi.org/10.1029/2019JD030648, 2019. a, b
Randel, W. J. and Thompson, A. M.: Interannual variability and trends in
tropical ozone derived from SAGE II satellite data and SHADOZ ozonesondes,
J. Geophys. Res.-Atmos., 116, D07303,
https://doi.org/10.1029/2010JD015195, 2011. a
Randel, W. J., Wu, F., Vömel, H., Nedoluha, G. E., and Forster, P.:
Decreases in stratospheric water vapor after 2001: Links to changes in the
tropical tropopause and the Brewer-Dobson circulation, J. Geophys. Res.,
111, 12312, https://doi.org/10.1029/2005JD006744, 2006. a
Randel, W. J., Park, M., Wu, F., and Livesey, N.: A Large Annual Cycle in
Ozone above the Tropical Tropopause Linked to the Brewer Dobson Circulation,
J. Atmos. Sci., 64, 4479–4488, https://doi.org/10.1175/2007JAS2409.1, 2007. a
Ray, E. A., Portmann, R. W., Yu, P., Daniel, J.,
Montzka, S. A., Dutton, G. S., Hall, B. D., Moore, F. L., and Rosenlof,
K. H.: The influence of the
stratospheric Quasi-Biennial Oscillation on trace gas levels at the Earth’s
surface, Nat. Geosci., 13, 1752–0908, https://doi.org/10.1038/s41561-019-0507-3,
2020. a
Renaud, A., Nadeau, L.-P., and Venaille, A.: Periodicity Disruption of a Model
Quasibiennial Oscillation of Equatorial Winds, Phys. Rev. Lett., 122,
214504, https://doi.org/10.1103/PhysRevLett.122.214504, 2019. a
Riese, M., Ploeger, F., Rap, A., Vogel, B., Konopka, P., Dameris, M., and
Forster, P.: Impact of uncertainties in atmospheric mixing on simulated UTLS
composition and related radiative effects, J. Geophys. Res., 117, D16305,
https://doi.org/10.1029/2012JD017751, 2012. a, b
Rosenlof, K. and Holton, J.: Estimates of the stratospheric residual
circulation using the downward control principle, J. Geophys. Res., 98,
10465–10479, 1993. a
Saji, N., Goswami, B., Vinayachandran, P., and Yamagata, T.: A dipole mode in
the tropical Indian Ocean, Nature, 401, 360—363, https://doi.org/10.1038/43854, 1999. a
Santee, M. L., Manney, G. L., Livesey, N. J., Schwartz, M. J., Neu, J. L., and
Read, W. G.: A comprehensive overview of the climatological composition of
the Asian summer monsoon anticyclone based on 10 years of Aura Microwave Limb
Sounder measurements, J. Geophys. Res.-Atmos., 122, 5491–5514,
https://doi.org/10.1002/2016JD026408, 2017. a
Saravanan, R.: A Multiwave Model of the Quasi-biennial Oscillation, J. Atmos.
Sci., 47, 2465–2474,
https://doi.org/10.1175/1520-0469(1990)047<2465:AMMOTQ>2.0.CO;2, 1990. a
Schirber, S.: Influence of ENSO on the QBO: Results from an ensemble of
idealized simulations, J. Geophys. Res.-Atmos., 120,
1109–1122, https://doi.org/10.1002/2014JD022460, 2015. a, b
Schoeberl, M. R. and Dessler, A. E.: Dehydration of the stratosphere, Atmos. Chem. Phys., 11, 8433–8446, https://doi.org/10.5194/acp-11-8433-2011, 2011. a
Schwartz, M. J., Read, W. G., Santee, M. L., Livesey, N. J., Froidevaux, L.,
Lambert, A., and Manney, G. L.: Convectively injected water vapor in the
North American summer lowermost stratosphere, Geophys. Res. Lett., 40,
2316–2321, https://doi.org/10.1002/grl.50421, 2013. a
Schwartz, M., Froidevaux, L., Livesey, N., and Read, W.: MLS/Aura Level 2 Ozone (O3)
Mixing Ratio V005, Greenbelt, MD, USA, Goddard Earth Sciences Data and Information Services
Center (GES DISC) [data set], https://doi.org/10.5067/Aura/MLS/DATA2516, 2020. a
Shepherd, T. G.: Transport in the Middle Atmosphere, J. Meteorol. Soc.
Jpn. Ser. II, 85B, 165–191, https://doi.org/10.2151/jmsj.85B.165, 2007. a
Shepherd, T. G. and McLandress, C.: A Robust Mechanism for Strengthening of the
Brewer–Dobson Circulation in Response to Climate Change: Critical-Layer
Control of Subtropical Wave Breaking, J. Atmos. Sci., 68, 784–797,
https://doi.org/10.1175/2010JAS3608.1, 2011. a
Smith, J. W., Haynes, P. H., Maycock, A. C., Butchart, N., and Bushell, A. C.: Sensitivity of stratospheric water vapour to variability in tropical tropopause temperatures and large-scale transport, Atmos. Chem. Phys., 21, 2469–2489, https://doi.org/10.5194/acp-21-2469-2021, 2021. a
Solomon, S., Rosenlof, K. H., Portmann, R. W., Daniel, J. S. Davis, S. M.,
Sanford, T., and Plattner, G.-K.: Contributions of Stratospheric Water Vapor
to Decadal Changes in the Rate of Global Warming, Science, 327, 1219–1223,
https://doi.org/10.1126/science.1182488, 2010. a, b
Son, S.-W., Lim, Y., Yoo, C., Hendon, H. H., and Kim, J.: Stratospheric Control
of the Madden–Julian Oscillation, J. Climate, 30, 1909–1922,
https://doi.org/10.1175/JCLI-D-16-0620.1, 2017. a
Stolarski, R. S., Waugh, D. W., Wang, L., Oman, L. D., Douglass, A. R., and
Newman, P. A.: Seasonal variation of ozone in the tropical lower
stratosphere: Southern tropics are different from northern tropics, J.
Geophys. Res.-Atmos., 119, 6196–6206,
https://doi.org/10.1002/2013JD021294, 2014. a, b
Tao, M., Konopka, P., Ploeger, F., Yan, X., Wright, J. S., Diallo, M., Fueglistaler, S., and Riese, M.: Multitimescale variations in modeled stratospheric water vapor derived from three modern reanalysis products, Atmos. Chem. Phys., 19, 6509–6534, https://doi.org/10.5194/acp-19-6509-2019, 2019.
a, b
Thomason, L. W., Ernest, N., Millán, L., Rieger, L., Bourassa, A., Vernier, J.-P., Manney, G., Luo, B., Arfeuille, F., and Peter, T.: A global space-based stratospheric aerosol climatology: 1979–2016, Earth Syst. Sci. Data, 10, 469–492, https://doi.org/10.5194/essd-10-469-2018, 2018. a
Tian, E. W., Su, H., Tian, B., and Jiang, J. H.: Interannual variations of water vapor in the tropical upper troposphere and the lower and middle stratosphere and their connections to ENSO and QBO, Atmos. Chem. Phys., 19, 9913–9926, https://doi.org/10.5194/acp-19-9913-2019, 2019. a
Timmermann, A., Oberhuber, J., Bacher, A., Esch, M., Latif, M., and Roeckner,
E.: El Niño, La Nina, and the Southern Oscillation, Nature, 398,
904–905, https://doi.org/10.1038/19505, 1999. a
Tweedy, O. V., Kramarova, N. A., Strahan, S. E., Newman, P. A., Coy, L., Randel, W. J., Park, M., Waugh, D. W., and Frith, S. M.: Response of trace gases to the disrupted 2015–2016 quasi-biennial oscillation, Atmos. Chem. Phys., 17, 6813–6823, https://doi.org/10.5194/acp-17-6813-2017, 2017. a, b
von Storch, H. and Zwiers, F. W.: Statistical analysis in climate research,
Cambridge Unv. Press, https://doi.org/10.1017/CBO9780511612336, 1999. a
Watanabe, S., Hamilton, K., Osprey, S., Kawatani, Y., and Nishimoto, E.: First
Successful Hindcasts of the 2016 Disruption of the Stratospheric
Quasi-biennial Oscillation, Geophys. Res. Lett., 45, 1602–1610,
https://doi.org/10.1002/2017GL076406, 2018. a
Weber, M., Dikty, S., Burrows, J. P., Garny, H., Dameris, M., Kubin, A., Abalichin, J., and Langematz, U.: The Brewer-Dobson circulation and total ozone from seasonal to decadal time scales, Atmos. Chem. Phys., 11, 11221–11235, https://doi.org/10.5194/acp-11-11221-2011, 2011. a
Wolter, K. and Timlin, M. S.: El Nino/Southern Oscillation behaviour since
1871 as diagnosed in an extended multivariate ENSO index (MEI.ext), Int. J.
Climatol., 31, 1074–1087, https://doi.org/10.1002/joc.2336, 2011. a
Yu, P., Davis, S. M., Toon, O. B., Portmann, R. W., Bardeen, C. G., Barnes,
J. E., Telg, H., Maloney, C., and Rosenlof, K. H.: Persistent Stratospheric
Warming Due to 2019-2020 Australian Wildfire Smoke, Geophys. Res. Lett., 48,
e2021GL092609, https://doi.org/10.1029/2021GL092609, 2021. a, b, c, d
Short summary
The quasi-biennial oacillation disruption events in both 2016 and 2020 decreased lower-stratospheric water vapour and ozone. Differences in the strength and depth of the anomalous lower-stratospheric circulation and ozone are due to differences in tropical upwelling and cold-point temperature induced by lower-stratospheric planetary and gravity wave breaking. The differences in water vapour are due to higher cold-point temperature in 2020 induced by Australian wildfire.
The quasi-biennial oacillation disruption events in both 2016 and 2020 decreased...
Altmetrics
Final-revised paper
Preprint