Articles | Volume 21, issue 21
https://doi.org/10.5194/acp-21-16575-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-16575-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Nov 2021
Research article |
| 12 Nov 2021
| 12 Nov 2021
A weather regime characterisation of winter biomass aerosol transport from southern Africa
Université de Paris and Université Paris Est Creteil, CNRS,
LISA, 75013 Paris, France
Scuola Universitaria Superiore IUSS, Pavia, Italy
Benjamin Pohl
CRC/Biogéosciences, UMR6282 CNRS/Université de Bourgogne
Franche-Comté, Dijon, France
Maria del Carmen Alvarez Castro
Physical, Chemical and Natural Systems department, University Pablo de Olavide (UPO), Seville, 41013, Spain
Mediterranean Center of Climate Change (CMCC), Climate Simulation and Prediction Division, Bologna, 40126, Italy
Cyrille Flamant
Institut Pierre Simon Laplace, Laboratoire Atmosphères, Milieux, Observations Spatiales, UMR CNRS 8190, Sorbonne Université,
Université Versailles Saint Quentin, Paris, France
Paola Formenti
Université de Paris and Université Paris Est Creteil, CNRS,
LISA, 75013 Paris, France
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We present a comparison between concentrations of dissolved trace metals in pairs of total suspended particulate (TSP) and fog samples collected in Henties Bay, Namibia, during the AErosols, Radiation and CLOuds in southern Africa (AEROCLO-sA) field campaign. We found enhanced concentrations of dissolved metals in fog samples, which we attributed to metal–ligand complex formation in the early stages of particle activation into droplets that can then remain in a kinetically stable form in fog or lead to the formation of colloidal nanoparticles.
Aurélien Royer, Julien Crétat, Rémi Laffont, Sara Gamboa, Belén Luna, Iris Menéndez, Benjamin Pohl, Sophie Montuire, and Manuel Hernández Fernández
Clim. Past, 21, 1821–1851, https://doi.org/10.5194/cp-21-1821-2025, https://doi.org/10.5194/cp-21-1821-2025, 2025
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Continental-scale temperature maps have been generated based on rodent associations and spatial generalized linear mixed model for six different periods (Last Glacial Maximum, Heinrich Stadial, Bølling, Allerød, Younger Dryas and present-day conditions). Their reliability was assessed by comparing them with general circulation models, showing similar estimates, but slightly colder values in western Europe and warmer ones in eastern Europe for past periods.
Francesco Battaglia, Paola Formenti, Chiara Giorio, Mathieu Cazaunau, Edouard Pangui, Antonin Bergé, Aline Gratien, Diana L. Pereira, Thomas Bertin, Joel F. de Brito, Manolis N. Romanias, Vincent Michoud, Clarissa Baldo, Servanne Chevaillier, Gael Noyalet, Philippe Decorse, Bénédicte Picquet-Varrault, and Jean-François Doussin
Atmos. Chem. Phys., 25, 12409–12431, https://doi.org/10.5194/acp-25-12409-2025, https://doi.org/10.5194/acp-25-12409-2025, 2025
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This paper presents an experimental investigation of the interactions between glyoxal, an important volatile organic compound, and mineral dust particles of size and composition typical of natural conditions. We show that their interactions modify, in a definitive way, the concentrations of the gas phase and the surface properties of the dust, which could have important implications for the atmospheric composition and the Earth's climate.
Tanguy Jonville, Maurus Borne, Cyrille Flamant, Juan Cuesta, Olivier Bock, Pierre Bosser, Christophe Lavaysse, Andreas Fink, and Peter Knippertz
Atmos. Chem. Phys., 25, 9765–9786, https://doi.org/10.5194/acp-25-9765-2025, https://doi.org/10.5194/acp-25-9765-2025, 2025
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Tropical waves structure the atmosphere. Four types of tropical waves (equatorial Rossby – ER, Kelvin, MRG-TD1, and MRG-TD2 – mixed Rossby gravity–tropical depressions) are studied using filters, satellite measurements, and in situ data from the Clouds–Atmosphere Dynamics–Dust Interaction in West Africa (CADDIWA) campaign held in September 2021 in Cabo Verde. ER waves impact temperature and humidity above 2500 m, MRG-TD1 around 3500 m, and MRG-TD2 around 2000 m. Interactions between these waves favor tropical cyclone formation.
Daniele Zannoni, Hans Christian Steen-Larsen, Harald Sodemann, Iris Thurnherr, Cyrille Flamant, Patrick Chazette, Julien Totems, Martin Werner, and Myriam Raybaut
Atmos. Chem. Phys., 25, 9471–9495, https://doi.org/10.5194/acp-25-9471-2025, https://doi.org/10.5194/acp-25-9471-2025, 2025
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High-resolution airborne observations reveal that mixing between the free troposphere and surface evapotranspiration flux primarily modulates the water vapor isotopic composition in the lower troposphere. Water vapor isotope structure variations occur on the scale of hundreds of meters, underlining the utility of stable isotopes for studying microscale atmospheric dynamics. This study also provides the basis for better validation of water vapor isotope remote sensing retrievals with surface observations.
Mégane Ventura, Fabien Waquet, Isabelle Chiapello, Gérard Brogniez, Frédéric Parol, Frédérique Auriol, Rodrigue Loisil, Cyril Delegove, Luc Blarel, Oleg Dubovik, Marc Mallet, Cyrille Flamant, and Paola Formenti
Atmos. Meas. Tech., 18, 4005–4024, https://doi.org/10.5194/amt-18-4005-2025, https://doi.org/10.5194/amt-18-4005-2025, 2025
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Biomass-burning aerosols (BBAs) from Central Africa are transported above stratocumulus clouds. The absorption of solar energy by aerosols induces warming, altering the cloud dynamics. We developed an approach that combines polarimeter and lidar to quantify this. This methodology is assessed during the AEROCLO-sA (AErosol RadiatiOn and CLOud in Southern Africa) campaign. To validate it, we used irradiance measurements acquired during aircraft spiral descents. A major perspective is the generalization of this method to the global level.
Abdulaziz T. Yakubu, Danitza Klopper, Henno Havenga, Roelof Burger, Paola Formenti, and Stuart J. Piketh
EGUsphere, https://doi.org/10.5194/egusphere-2025-1827, https://doi.org/10.5194/egusphere-2025-1827, 2025
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Low-level inversions experienced along the Namibia coast and adjacent ocean have implications for air pollutant dispersion and low clouds. These affect air quality, human health, radiative forcing and climate change. We used reanalysis and satellite datasets to understand inversion properties over the region. The result shows inversion prominence at night and in winter, seasonally influences pollutant trapping and initiates stratocumulus clouds formation, but is not liable for their extent.
Johannes Heuser, Claudia Di Biagio, Jérôme Yon, Mathieu Cazaunau, Antonin Bergé, Edouard Pangui, Marco Zanatta, Laura Renzi, Angela Marinoni, Satoshi Inomata, Chenjie Yu, Vera Bernardoni, Servanne Chevaillier, Daniel Ferry, Paolo Laj, Michel Maillé, Dario Massabò, Federico Mazzei, Gael Noyalet, Hiroshi Tanimoto, Brice Temime-Roussel, Roberta Vecchi, Virginia Vernocchi, Paola Formenti, Bénédicte Picquet-Varrault, and Jean-François Doussin
Atmos. Chem. Phys., 25, 6407–6428, https://doi.org/10.5194/acp-25-6407-2025, https://doi.org/10.5194/acp-25-6407-2025, 2025
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The spectral optical properties of combustion soot aerosols with varying black (BC) and brown carbon (BrC) content were studied in an atmospheric simulation chamber. Measurements of the mass spectral absorption cross section (MAC), supplemented by literature data, allowed us to establish a generalised exponential relationship between the spectral absorption and the elemental-to-total-carbon ratio (EC / TC) in soot. This relationship can provide a useful tool for modelling the properties of soot.
Simone T. Andersen, Rolf Sander, Patrick Dewald, Laura Wüst, Tobias Seubert, Gunther N. T. E. Türk, Jan Schuladen, Max R. McGillen, Chaoyang Xue, Abdelwahid Mellouki, Alexandre Kukui, Vincent Michoud, Manuela Cirtog, Mathieu Cazaunau, Astrid Bauville, Hichem Bouzidi, Paola Formenti, Cyrielle Denjean, Jean-Claude Etienne, Olivier Garrouste, Christopher Cantrell, Jos Lelieveld, and John N. Crowley
Atmos. Chem. Phys., 25, 5893–5909, https://doi.org/10.5194/acp-25-5893-2025, https://doi.org/10.5194/acp-25-5893-2025, 2025
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Measurements and modelling of reactive nitrogen gases observed in a suburban temperate forest in Rambouillet, France, circa 50 km southwest of Paris in 2022 indicate that the biosphere rapidly scavenges organic nitrates of mixed biogenic and anthropogenic origin, resulting in short lifetimes for, for example, alkyl nitrates and peroxy nitrates.
Ludovico Di Antonio, Matthias Beekmann, Guillaume Siour, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Joel F. de Brito, Paola Formenti, Cecile Gaimoz, Olivier Garret, Aline Gratien, Valérie Gros, Martial Haeffelin, Lelia N. Hawkins, Simone Kotthaus, Gael Noyalet, Diana L. Pereira, Jean-Eudes Petit, Eva Drew Pronovost, Véronique Riffault, Chenjie Yu, Gilles Foret, Jean-François Doussin, and Claudia Di Biagio
Atmos. Chem. Phys., 25, 4803–4831, https://doi.org/10.5194/acp-25-4803-2025, https://doi.org/10.5194/acp-25-4803-2025, 2025
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The summer of 2022 has been considered a proxy for future climate scenarios due to its hot and dry conditions. In this paper, we use the measurements from the Atmospheric Chemistry of the Suburban Forest (ACROSS) campaign, conducted in the Paris area in June–July 2022, along with observations from existing networks, to evaluate a 3D chemistry transport model (WRF–CHIMERE) simulation. Results are shown to be satisfactory, allowing us to explain the gas and aerosol variability at the campaign sites.
Diana L. Pereira, Chiara Giorio, Aline Gratien, Alexander Zherebker, Gael Noyalet, Servanne Chevaillier, Stéphanie Alage, Elie Almarj, Antonin Bergé, Thomas Bertin, Mathieu Cazaunau, Patrice Coll, Ludovico Di Antonio, Sergio Harb, Johannes Heuser, Cécile Gaimoz, Oscar Guillemant, Brigitte Language, Olivier Lauret, Camilo Macias, Franck Maisonneuve, Bénédicte Picquet-Varrault, Raquel Torres, Sylvain Triquet, Pascal Zapf, Lelia Hawkins, Drew Pronovost, Sydney Riley, Pierre-Marie Flaud, Emilie Perraudin, Pauline Pouyes, Eric Villenave, Alexandre Albinet, Olivier Favez, Robin Aujay-Plouzeau, Vincent Michoud, Christopher Cantrell, Manuela Cirtog, Claudia Di Biagio, Jean-François Doussin, and Paola Formenti
Atmos. Chem. Phys., 25, 4885–4905, https://doi.org/10.5194/acp-25-4885-2025, https://doi.org/10.5194/acp-25-4885-2025, 2025
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In order to study aerosols in environments influenced by anthropogenic and biogenic emissions, we performed analyses of samples collected during the ACROSS (Atmospheric Chemistry Of the Suburban Forest) campaign in summer 2022 in the greater Paris area. After analysis of the chemical composition by means of total carbon determination and high-resolution mass spectrometry, this work highlights the influence of anthropogenic inputs on the chemical composition of both urban and forested areas.
Ludovico Di Antonio, Claudia Di Biagio, Paola Formenti, Aline Gratien, Vincent Michoud, Christopher Cantrell, Astrid Bauville, Antonin Bergé, Mathieu Cazaunau, Servanne Chevaillier, Manuela Cirtog, Patrice Coll, Barbara D'Anna, Joel F. de Brito, David O. De Haan, Juliette R. Dignum, Shravan Deshmukh, Olivier Favez, Pierre-Marie Flaud, Cecile Gaimoz, Lelia N. Hawkins, Julien Kammer, Brigitte Language, Franck Maisonneuve, Griša Močnik, Emilie Perraudin, Jean-Eudes Petit, Prodip Acharja, Laurent Poulain, Pauline Pouyes, Eva Drew Pronovost, Véronique Riffault, Kanuri I. Roundtree, Marwa Shahin, Guillaume Siour, Eric Villenave, Pascal Zapf, Gilles Foret, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 25, 3161–3189, https://doi.org/10.5194/acp-25-3161-2025, https://doi.org/10.5194/acp-25-3161-2025, 2025
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The spectral complex refractive index (CRI) and single scattering albedo were retrieved from submicron aerosol measurements at three sites within the greater Paris area during the ACROSS field campaign (June–July 2022). Measurements revealed urban emission impact on surrounding areas. CRI full period averages at 520 nm were 1.41 – 0.037i (urban), 1.52 – 0.038i (peri-urban), and 1.50 – 0.025i (rural). Organic aerosols dominated the aerosol mass and contributed up to 22 % of absorption at 370 nm.
Alexandre Mass, Hendrik Andersen, Jan Cermak, Paola Formenti, Eva Pauli, and Julian Quinting
Atmos. Chem. Phys., 25, 491–510, https://doi.org/10.5194/acp-25-491-2025, https://doi.org/10.5194/acp-25-491-2025, 2025
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This study investigates the interaction between smoke aerosols and fog and low clouds (FLCs) in the Namib Desert between June and October. Here, a satellite-based dataset of FLCs, reanalysis data and machine learning are used to systematically analyze FLC persistence under different aerosol loadings. Aerosol plumes are shown to modify local thermodynamics, which increase FLC persistence. But fully disentangling aerosol effects from meteorological ones remains a challenge.
Cedric G. Ngoungue Langue, Christophe Lavaysse, and Cyrille Flamant
Nat. Hazards Earth Syst. Sci., 25, 147–168, https://doi.org/10.5194/nhess-25-147-2025, https://doi.org/10.5194/nhess-25-147-2025, 2025
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The present study addresses the predictability of heat waves at subseasonal timescales in West African cities over the period 2001–2020. Two models, the European Centre for Medium-Range Weather Forecasts (ECMWF) and the UK Met Office models, were evaluated using two reanalyses: ERA5 and MERRA. The results suggest that at subseasonal timescales, the forecast models provide a better forecast than climatology, but the hit rate and false alarm rate are sub-optimal.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Junying Sun, Ye Kuang, Paola Formenti, and Steven G. Howell
Atmos. Chem. Phys., 24, 13849–13864, https://doi.org/10.5194/acp-24-13849-2024, https://doi.org/10.5194/acp-24-13849-2024, 2024
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Using airborne measurements over the southeast Atlantic Ocean, we examined how much moisture aerosols take up during Africa’s biomass burning season. Our study revealed the important role of organic aerosols and introduced a predictive model for moisture uptake, accounting for organics, sulfate, and black carbon, summarizing results from various campaigns. These findings improve our understanding of aerosol–moisture interactions and their radiative effects in this climatically critical region.
Laura T. Massano, Giorgia Fosser, Marco Gaetani, and Cécile Caillaud
Nat. Hazards Earth Syst. Sci., 24, 4293–4315, https://doi.org/10.5194/nhess-24-4293-2024, https://doi.org/10.5194/nhess-24-4293-2024, 2024
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Traditional wine-growing regions are threatened by expected climate change. Climate models and observations are used to calculate bioclimatic indices based on both temperature and precipitation. These indices are correlated with grape productivity in two wine-growing regions in Italy. This analysis paves the way for using climate models to study how climate change will affect wine production in the future.
Paola Formenti and Claudia Di Biagio
Earth Syst. Sci. Data, 16, 4995–5007, https://doi.org/10.5194/essd-16-4995-2024, https://doi.org/10.5194/essd-16-4995-2024, 2024
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Particles from deserts and semi-vegetated areas (mineral dust) are important for Earth's climate and human health, notably depending on their size. In this paper we collect and make a synthesis of a body of these observations since 1972 in order to provide researchers modeling Earth's climate and developing satellite observations from space with a simple way of confronting their results and understanding their validity.
Marco Gaetani, Gabriele Messori, Francesco S. R. Pausata, Shivangi Tiwari, M. Carmen Alvarez Castro, and Qiong Zhang
Clim. Past, 20, 1735–1759, https://doi.org/10.5194/cp-20-1735-2024, https://doi.org/10.5194/cp-20-1735-2024, 2024
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Palaeoclimate reconstructions suggest that, around 6000 years ago, a greening of the Sahara took place, accompanied by climate changes in the Northern Hemisphere at middle to high latitudes. In this study, a climate model is used to investigate how this drastic environmental change in the Sahara impacted remote regions. Specifically, climate simulations reveal significant modifications in atmospheric circulation over the North Atlantic, affecting North American and European climates.
Chenjie Yu, Edouard Pangui, Kevin Tu, Mathieu Cazaunau, Maxime Feingesicht, Landsheere Xavier, Thierry Bourrianne, Vincent Michoud, Christopher Cantrell, Timothy B. Onasch, Andrew Freedman, and Paola Formenti
Atmos. Meas. Tech., 17, 3419–3437, https://doi.org/10.5194/amt-17-3419-2024, https://doi.org/10.5194/amt-17-3419-2024, 2024
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To meet the requirements for measuring aerosol optical properties on airborne platforms and conducting dual-wavelength measurements, we introduced A2S2, an airborne dual-wavelength cavity-attenuated phase-shift single monitor. This study reports the results in the laboratory and an aircraft campaign over Paris and its surrounding regions. The results demonstrate A2S2's reliability in measuring aerosol optical properties at both wavelengths and its suitability for future aircraft campaigns.
Vincenzo Obiso, María Gonçalves Ageitos, Carlos Pérez García-Pando, Jan P. Perlwitz, Gregory L. Schuster, Susanne E. Bauer, Claudia Di Biagio, Paola Formenti, Kostas Tsigaridis, and Ron L. Miller
Atmos. Chem. Phys., 24, 5337–5367, https://doi.org/10.5194/acp-24-5337-2024, https://doi.org/10.5194/acp-24-5337-2024, 2024
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We calculate the dust direct radiative effect (DRE) in an Earth system model accounting for regionally varying soil mineralogy through a new observationally constrained method. Linking dust absorption at solar wavelengths to the varying amount of specific minerals (i.e., iron oxides) improves the modeled range of dust single scattering albedo compared to observations and increases the global cooling by dust. Our results may contribute to improved estimates of the dust DRE and its climate impact.
Cyrille Flamant, Jean-Pierre Chaboureau, Marco Gaetani, Kerstin Schepanski, and Paola Formenti
Atmos. Chem. Phys., 24, 4265–4288, https://doi.org/10.5194/acp-24-4265-2024, https://doi.org/10.5194/acp-24-4265-2024, 2024
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In the austral dry season, the atmospheric composition over southern Africa is dominated by biomass burning aerosols and terrigenous aerosols (so-called mineral dust). This study suggests that the radiative effect of biomass burning aerosols needs to be taken into account to properly forecast dust emissions in Namibia.
Anil Kumar Mandariya, Junteng Wu, Anne Monod, Paola Formenti, Bénédicte Picquet-Varrault, Mathieu Cazaunau, Stephan Mertes, Laurent Poulain, Antonin Berge, Edouard Pangui, Andreas Tilgner, Thomas Schaefer, Liang Wen, Hartmut Herrmann, and Jean-François Doussin
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-206, https://doi.org/10.5194/amt-2023-206, 2024
Publication in AMT not foreseen
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An optimized and controlled protocol for generating quasi-adiabatic expansion clouds under simulated dark and light conditions was presented. The irradiated clouds clearly showed a gradual activation of seed particles into droplets. In contrast, non-irradiated clouds faced a flash activation. This paper will lay the foundation for multiphase photochemical studies implying water-soluble volatile organic compounds and particulate matter formation during cloud formation-evaporation cycles.
Claudio Stefanini, Giovanni Macelloni, Marion Leduc-Leballeur, Vincent Favier, Benjamin Pohl, and Ghislain Picard
The Cryosphere, 18, 593–608, https://doi.org/10.5194/tc-18-593-2024, https://doi.org/10.5194/tc-18-593-2024, 2024
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Local and large-scale meteorological conditions have been considered in order to explain some peculiar changes of snow grains on the East Antarctic Plateau from 2000 to 2022, by using remote sensing observations and reanalysis. We identified some extreme grain size events on the highest ice divide, resulting from a combination of conditions of low wind speed and low temperature. Moreover, the beginning of seasonal grain growth has been linked to the occurrence of atmospheric rivers.
Karine Desboeufs, Paola Formenti, Raquel Torres-Sánchez, Kerstin Schepanski, Jean-Pierre Chaboureau, Hendrik Andersen, Jan Cermak, Stefanie Feuerstein, Benoit Laurent, Danitza Klopper, Andreas Namwoonde, Mathieu Cazaunau, Servanne Chevaillier, Anaïs Feron, Cécile Mirande-Bret, Sylvain Triquet, and Stuart J. Piketh
Atmos. Chem. Phys., 24, 1525–1541, https://doi.org/10.5194/acp-24-1525-2024, https://doi.org/10.5194/acp-24-1525-2024, 2024
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This study investigates the fractional solubility of iron (Fe) in dust particles along the coast of Namibia, a critical region for the atmospheric Fe supply of the South Atlantic Ocean. Our results suggest a possible two-way interplay whereby marine biogenic emissions from the coastal marine ecosystems into the atmosphere would increase the solubility of Fe-bearing dust by photo-reduction processes. The subsequent deposition of soluble Fe could act to further enhance marine biogenic emissions.
Maurus Borne, Peter Knippertz, Martin Weissmann, Benjamin Witschas, Cyrille Flamant, Rosimar Rios-Berrios, and Peter Veals
Atmos. Meas. Tech., 17, 561–581, https://doi.org/10.5194/amt-17-561-2024, https://doi.org/10.5194/amt-17-561-2024, 2024
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This study assesses the quality of Aeolus wind measurements over the tropical Atlantic. The results identified the accuracy and precision of the Aeolus wind measurements and the potential source of errors. For instance, the study revealed atmospheric conditions that can deteriorate the measurement quality, such as weaker laser signal in cloudy or dusty conditions, and confirmed the presence of an orbital-dependant bias. These results can help to improve the Aeolus wind measurement algorithm.
Gaëlle de Coëtlogon, Adrien Deroubaix, Cyrille Flamant, Laurent Menut, and Marco Gaetani
Atmos. Chem. Phys., 23, 15507–15521, https://doi.org/10.5194/acp-23-15507-2023, https://doi.org/10.5194/acp-23-15507-2023, 2023
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Using a numerical atmospheric model, we found that cooling sea surface temperatures along the southern coast of West Africa in July cause the “little dry season”. This effect reduces humidity and pollutant transport inland, potentially enhancing West Africa's synoptic and seasonal forecasting.
Leonie Villiger, Marina Dütsch, Sandrine Bony, Marie Lothon, Stephan Pfahl, Heini Wernli, Pierre-Etienne Brilouet, Patrick Chazette, Pierre Coutris, Julien Delanoë, Cyrille Flamant, Alfons Schwarzenboeck, Martin Werner, and Franziska Aemisegger
Atmos. Chem. Phys., 23, 14643–14672, https://doi.org/10.5194/acp-23-14643-2023, https://doi.org/10.5194/acp-23-14643-2023, 2023
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This study evaluates three numerical simulations performed with an isotope-enabled weather forecast model and investigates the coupling between shallow trade-wind cumulus clouds and atmospheric circulations on different scales. We show that the simulations reproduce key characteristics of shallow trade-wind clouds as observed during the field experiment EUREC4A and that the spatial distribution of stable-water-vapour isotopes is shaped by the overturning circulation associated with these clouds.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Junying Sun, Ye Kuang, and Paola Formenti
EGUsphere, https://doi.org/10.5194/egusphere-2023-2319, https://doi.org/10.5194/egusphere-2023-2319, 2023
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Our study examined the interaction between atmospheric particles and moisture over the south-eastern Atlantic Ocean during the biomass burning seasons in Africa. We found that organic components of these particles play a more important role in aerosol-moisture interactions than previously expected. This discovery is important as such interactions impact radiation and climate. Current climate models might need better representations of the moisture-absorbing properties of organic aerosols.
Ludovico Di Antonio, Claudia Di Biagio, Gilles Foret, Paola Formenti, Guillaume Siour, Jean-François Doussin, and Matthias Beekmann
Atmos. Chem. Phys., 23, 12455–12475, https://doi.org/10.5194/acp-23-12455-2023, https://doi.org/10.5194/acp-23-12455-2023, 2023
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Long-term (2000–2021) 1 km resolution satellite data have been used to investigate the climatological aerosol optical depth (AOD) variability and trends at different scales in Europe. Average enhancements of the local-to-regional AOD ratio at 550 nm of 57 %, 55 %, 39 % and 32 % are found for large metropolitan areas such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions.
Valerian Hahn, Ralf Meerkötter, Christiane Voigt, Sonja Gisinger, Daniel Sauer, Valéry Catoire, Volker Dreiling, Hugh Coe, Cyrille Flamant, Stefan Kaufmann, Jonas Kleine, Peter Knippertz, Manuel Moser, Philip Rosenberg, Hans Schlager, Alfons Schwarzenboeck, and Jonathan Taylor
Atmos. Chem. Phys., 23, 8515–8530, https://doi.org/10.5194/acp-23-8515-2023, https://doi.org/10.5194/acp-23-8515-2023, 2023
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During the DACCIWA campaign in West Africa, we found a 35 % increase in the cloud droplet concentration that formed in a polluted compared with a less polluted environment and a decrease of 17 % in effective droplet diameter. Radiative transfer simulations, based on the measured cloud properties, reveal that these low-level polluted clouds radiate only 2.6 % more energy back to space, compared with a less polluted cloud. The corresponding additional decrease in temperature is rather small.
Clarissa Baldo, Paola Formenti, Claudia Di Biagio, Gongda Lu, Congbo Song, Mathieu Cazaunau, Edouard Pangui, Jean-Francois Doussin, Pavla Dagsson-Waldhauserova, Olafur Arnalds, David Beddows, A. Robert MacKenzie, and Zongbo Shi
Atmos. Chem. Phys., 23, 7975–8000, https://doi.org/10.5194/acp-23-7975-2023, https://doi.org/10.5194/acp-23-7975-2023, 2023
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This paper presents new shortwave spectral complex refractive index and single scattering albedo data for Icelandic dust. Our results show that the imaginary part of the complex refractive index of Icelandic dust is at the upper end of the range of low-latitude dust. Furthermore, we observed that Icelandic dust is more absorbing towards the near-infrared, which we attribute to its high magnetite content. These findings are important for modeling dust aerosol radiative effects in the Arctic.
Michail Mytilinaios, Sara Basart, Sergio Ciamprone, Juan Cuesta, Claudio Dema, Enza Di Tomaso, Paola Formenti, Antonis Gkikas, Oriol Jorba, Ralph Kahn, Carlos Pérez García-Pando, Serena Trippetta, and Lucia Mona
Atmos. Chem. Phys., 23, 5487–5516, https://doi.org/10.5194/acp-23-5487-2023, https://doi.org/10.5194/acp-23-5487-2023, 2023
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Multiscale Online Non-hydrostatic AtmospheRe CHemistry model (MONARCH) dust reanalysis provides a high-resolution 3D reconstruction of past dust conditions, allowing better quantification of climate and socioeconomic dust impacts. We assess the performance of the reanalysis needed to reproduce dust optical depth using dust-related products retrieved from satellite and ground-based observations and show that it reproduces the spatial distribution and seasonal variability of atmospheric dust well.
Cedric Gacial Ngoungue Langue, Christophe Lavaysse, Mathieu Vrac, and Cyrille Flamant
Nat. Hazards Earth Syst. Sci., 23, 1313–1333, https://doi.org/10.5194/nhess-23-1313-2023, https://doi.org/10.5194/nhess-23-1313-2023, 2023
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Heat waves (HWs) are climatic hazards that affect the planet. We assess here uncertainties encountered in the process of HW detection and analyse their recent trends in West Africa using reanalysis data. Three types of uncertainty have been investigated. We identified 6 years with higher frequency of HWs, possibly due to higher sea surface temperatures in the equatorial Atlantic. We noticed an increase in HW characteristics during the last decade, which could be a consequence of climate change.
Michael John Weston, Stuart John Piketh, Frédéric Burnet, Stephen Broccardo, Cyrielle Denjean, Thierry Bourrianne, and Paola Formenti
Atmos. Chem. Phys., 22, 10221–10245, https://doi.org/10.5194/acp-22-10221-2022, https://doi.org/10.5194/acp-22-10221-2022, 2022
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An aerosol-aware microphysics scheme is evaluated for fog cases in Namibia. AEROCLO-sA campaign observations are used to access and parameterise the model. The model cloud condensation nuclei activation is lower than the observations. The scheme is designed for clouds with updrafts, while fog typically forms in stable conditions. A pseudo updraft speed assigned to the lowest model levels helps achieve more realistic cloud droplet number concentration and size distribution in the model.
N. Hempelmann, C. Ehbrecht, E. Plesiat, G. Hobona, J. Simoes, D. Huard, T. J. Smith, U. S. McKnight, I. G. Pechlivanidis, and C. Alvarez-Castro
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLVIII-4-W1-2022, 187–194, https://doi.org/10.5194/isprs-archives-XLVIII-4-W1-2022-187-2022, https://doi.org/10.5194/isprs-archives-XLVIII-4-W1-2022-187-2022, 2022
Núria Pérez-Zanón, Louis-Philippe Caron, Silvia Terzago, Bert Van Schaeybroeck, Llorenç Lledó, Nicolau Manubens, Emmanuel Roulin, M. Carmen Alvarez-Castro, Lauriane Batté, Pierre-Antoine Bretonnière, Susana Corti, Carlos Delgado-Torres, Marta Domínguez, Federico Fabiano, Ignazio Giuntoli, Jost von Hardenberg, Eroteida Sánchez-García, Verónica Torralba, and Deborah Verfaillie
Geosci. Model Dev., 15, 6115–6142, https://doi.org/10.5194/gmd-15-6115-2022, https://doi.org/10.5194/gmd-15-6115-2022, 2022
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CSTools (short for Climate Service Tools) is an R package that contains process-based methods for climate forecast calibration, bias correction, statistical and stochastic downscaling, optimal forecast combination, and multivariate verification, as well as basic and advanced tools to obtain tailored products. In addition to describing the structure and methods in the package, we also present three use cases to illustrate the seasonal climate forecast post-processing for specific purposes.
Caroline Dang, Michal Segal-Rozenhaimer, Haochi Che, Lu Zhang, Paola Formenti, Jonathan Taylor, Amie Dobracki, Sara Purdue, Pui-Shan Wong, Athanasios Nenes, Arthur Sedlacek III, Hugh Coe, Jens Redemann, Paquita Zuidema, Steven Howell, and James Haywood
Atmos. Chem. Phys., 22, 9389–9412, https://doi.org/10.5194/acp-22-9389-2022, https://doi.org/10.5194/acp-22-9389-2022, 2022
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Transmission electron microscopy was used to analyze aged African smoke particles and how the smoke interacts with the marine atmosphere. We found that the volatility of organic aerosol increases with biomass burning plume age, that black carbon is often mixed with potassium salts and that the marine atmosphere can incorporate Na and Cl into smoke particles. Marine salts are more processed when mixed with smoke plumes, and there are interesting Cl-rich yet Na-absent marine particles.
Lu Zhang, Michal Segal-Rozenhaimer, Haochi Che, Caroline Dang, Arthur J. Sedlacek III, Ernie R. Lewis, Amie Dobracki, Jenny P. S. Wong, Paola Formenti, Steven G. Howell, and Athanasios Nenes
Atmos. Chem. Phys., 22, 9199–9213, https://doi.org/10.5194/acp-22-9199-2022, https://doi.org/10.5194/acp-22-9199-2022, 2022
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Widespread biomass burning (BB) events occur annually in Africa and contribute ~ 1 / 3 of global BB emissions, which contain a large family of light-absorbing organics, known as brown carbon (BrC), whose absorption of incident radiation is difficult to estimate, leading to large uncertainties in the global radiative forcing estimation. This study quantifies the BrC absorption of aged BB particles and highlights the potential presence of absorbing iron oxides in this climatically important region.
Jean-Pierre Chaboureau, Laurent Labbouz, Cyrille Flamant, and Alma Hodzic
Atmos. Chem. Phys., 22, 8639–8658, https://doi.org/10.5194/acp-22-8639-2022, https://doi.org/10.5194/acp-22-8639-2022, 2022
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Ground-based, spaceborne and rare airborne observations of biomass burning aerosols (BBAs) during the AEROCLO-sA field campaign in 2017 are complemented with convection-permitting simulations with online trajectories. The results show that the radiative effect of the BBA accelerates the southern African easterly jet and generates upward motions that transport the BBAs to higher altitudes and farther southwest.
Enza Di Tomaso, Jerónimo Escribano, Sara Basart, Paul Ginoux, Francesca Macchia, Francesca Barnaba, Francesco Benincasa, Pierre-Antoine Bretonnière, Arnau Buñuel, Miguel Castrillo, Emilio Cuevas, Paola Formenti, María Gonçalves, Oriol Jorba, Martina Klose, Lucia Mona, Gilbert Montané Pinto, Michail Mytilinaios, Vincenzo Obiso, Miriam Olid, Nick Schutgens, Athanasios Votsis, Ernest Werner, and Carlos Pérez García-Pando
Earth Syst. Sci. Data, 14, 2785–2816, https://doi.org/10.5194/essd-14-2785-2022, https://doi.org/10.5194/essd-14-2785-2022, 2022
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MONARCH reanalysis of desert dust aerosols extends the existing observation-based information for mineral dust monitoring by providing 3-hourly upper-air, surface and total column key geophysical variables of the dust cycle over Northern Africa, the Middle East and Europe, at a 0.1° horizontal resolution in a rotated grid, from 2007 to 2016. This work provides evidence of the high accuracy of this data set and its suitability for air quality and health and climate service applications.
Cyrille Flamant, Marco Gaetani, Jean-Pierre Chaboureau, Patrick Chazette, Juan Cuesta, Stuart John Piketh, and Paola Formenti
Atmos. Chem. Phys., 22, 5701–5724, https://doi.org/10.5194/acp-22-5701-2022, https://doi.org/10.5194/acp-22-5701-2022, 2022
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Rivers of smoke extend from tropical southern Africa towards the Indian Ocean during the winter fire season, controlled by the interaction of tropical easterly waves, and westerly waves at mid latitudes. During the AEROCLO-sA field campaign in 2017, a river of smoke was directly observed over Namibia. In this paper, the evolution and atmospheric drivers of the river of smoke are described, and the role of a mid-latitude cut-off low in lifting the smoke to the upper troposphere is highlighted.
Sandrine Bony, Marie Lothon, Julien Delanoë, Pierre Coutris, Jean-Claude Etienne, Franziska Aemisegger, Anna Lea Albright, Thierry André, Hubert Bellec, Alexandre Baron, Jean-François Bourdinot, Pierre-Etienne Brilouet, Aurélien Bourdon, Jean-Christophe Canonici, Christophe Caudoux, Patrick Chazette, Michel Cluzeau, Céline Cornet, Jean-Philippe Desbios, Dominique Duchanoy, Cyrille Flamant, Benjamin Fildier, Christophe Gourbeyre, Laurent Guiraud, Tetyana Jiang, Claude Lainard, Christophe Le Gac, Christian Lendroit, Julien Lernould, Thierry Perrin, Frédéric Pouvesle, Pascal Richard, Nicolas Rochetin, Kevin Salaün, Alfons Schwarzenboeck, Guillaume Seurat, Bjorn Stevens, Julien Totems, Ludovic Touzé-Peiffer, Gilles Vergez, Jessica Vial, Leonie Villiger, and Raphaela Vogel
Earth Syst. Sci. Data, 14, 2021–2064, https://doi.org/10.5194/essd-14-2021-2022, https://doi.org/10.5194/essd-14-2021-2022, 2022
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The French ATR42 research aircraft participated in the EUREC4A international field campaign that took place in 2020 over the tropical Atlantic, east of Barbados. We present the extensive instrumentation of the aircraft, the research flights and the different measurements. We show that the ATR measurements of humidity, wind, aerosols and cloudiness in the lower atmosphere are robust and consistent with each other. They will make it possible to advance understanding of cloud–climate interactions.
Adrien Deroubaix, Laurent Menut, Cyrille Flamant, Peter Knippertz, Andreas H. Fink, Anneke Batenburg, Joel Brito, Cyrielle Denjean, Cheikh Dione, Régis Dupuy, Valerian Hahn, Norbert Kalthoff, Fabienne Lohou, Alfons Schwarzenboeck, Guillaume Siour, Paolo Tuccella, and Christiane Voigt
Atmos. Chem. Phys., 22, 3251–3273, https://doi.org/10.5194/acp-22-3251-2022, https://doi.org/10.5194/acp-22-3251-2022, 2022
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During the summer monsoon in West Africa, pollutants emitted in urbanized areas modify cloud cover and precipitation patterns. We analyze these patterns with the WRF-CHIMERE model, integrating the effects of aerosols on meteorology, based on the numerous observations provided by the Dynamics-Aerosol-Climate-Interactions campaign. This study adds evidence to recent findings that increased pollution levels in West Africa delay the breakup time of low-level clouds and reduce precipitation.
Patrick Chazette, Alexandre Baron, and Cyrille Flamant
Atmos. Chem. Phys., 22, 1271–1292, https://doi.org/10.5194/acp-22-1271-2022, https://doi.org/10.5194/acp-22-1271-2022, 2022
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Within the framework of the international EUREC4A project, horizontal lidar measurements were carried out over Barbados from the French research aircraft ATR-42. These measurements highlighted the strong heterogeneity of the aerosol field (mainly dust and biomass burning aerosols) and therefore of the associated optical properties. This heterogeneity varies according to meteorological conditions and could significantly modulate the climatic impact of aerosols trapped over the tropical Atlantic.
Paola Formenti, Claudia Di Biagio, Yue Huang, Jasper Kok, Marc Daniel Mallet, Damien Boulanger, and Mathieu Cazaunau
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2021-403, https://doi.org/10.5194/amt-2021-403, 2021
Publication in AMT not foreseen
Short summary
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This paper provides with standardized correction factors for the measurements of the most common instruments used in the atmosphere to measure the concentration per size of aerosol particles. These correction factors are provided to users with supplementary information for their use.
Cited articles
Abel, S. J., Haywood, J. M., Highwood, E. J., Li, J., and Buseck, P. R.:
Evolution of biomass burning aerosol properties from an agricultural fire in
southern Africa, Geophys. Res. Lett., 30, 1783,
https://doi.org/10.1029/2003GL017342, 2003.
Adebiyi, A. A. and Zuidema, P.: The role of the southern African easterly
jet in modifying the southeast Atlantic aerosol and cloud environments, Q.
J. R. Meteorol. Soc., 142, 1574–1589, https://doi.org/10.1002/qj.2765, 2016.
Adebiyi, A. A. and Zuidema, P.: Low Cloud Cover Sensitivity to
Biomass-Burning Aerosols and Meteorology over the Southeast Atlantic, J.
Climate, 31, 4329–4346, https://doi.org/10.1175/JCLI-D-17-0406.1, 2018.
Baker, A. R., Lesworth, T., Adams, C., Jickells, T. D., and Ganzeveld, L.:
Estimation of atmospheric nutrient inputs to the Atlantic Ocean from
50∘ N to 50∘ S based on large-scale field sampling:
Fixed nitrogen and dry deposition of phosphorus, Global Biogeochem. Cycles,
24, GB3006, https://doi.org/10.1029/2009GB003634, 2010.
Baldwin, M. P.: Annular modes in global daily surface pressure, Geophys.
Res. Lett., 28, 4115–4118, https://doi.org/10.1029/2001GL013564, 2001.
Barkley, A. E., Prospero, J. M., Mahowald, N., Hamilton, D. S., Popendorf,
K. J., Oehlert, A. M., Pourmand, A., Gatineau, A., Panechou-Pulcherie, K.,
Blackwelder, P., and Gaston, C. J.: African biomass burning is a substantial
source of phosphorus deposition to the Amazon, Tropical Atlantic Ocean, and
Southern Ocean, Proc. Natl. Acad. Sci. USA, 116, 16216–16221,
https://doi.org/10.1073/pnas.1906091116, 2019.
Bellouin, N., Quaas, J., Gryspeerdt, E., Kinne, S., Stier, P.,
Watson-Parris, D., Boucher, O., Carslaw, K. S., Christensen, M., Daniau, A.-L., Dufresne, J.-L., Feingold, G., Fiedler, S., Forster, P., Gettelman,
A., Haywood, J. M., Lohmann, U., Malavelle, F., Mauritsen, T., McCoy, D. T.,
Myhre, G., Mülmenstädt, J., Neubauer, D., Possner, A., Rugenstein,
M., Sato, Y., Schulz, M., Schwartz, S. E., Sourdeval, O., Storelvmo, T.,
Toll, V., Winker, D., and Stevens, B.: Bounding Global Aerosol Radiative
Forcing of Climate Change, Rev. Geophys., 58, e2019RG000660,
https://doi.org/10.1029/2019RG000660, 2020.
Boening, C., Willis, J. K., Landerer, F. W., Nerem, R. S., and Fasullo, J.:
The 2011 La Niña: So strong, the oceans fell, Geophys. Res. Lett.,
39, L19602, https://doi.org/10.1029/2012GL053055, 2012.
Chen, G.: Revisit to atmospheric oscillations over global oceans: a combined
climatology/modality approach, Int. J. Climatol., 34, 2715–2729,
https://doi.org/10.1002/joc.3870, 2014.
Crétat, J., Pohl, B., Dieppois, B., Berthou, S., and Pergaud, J.: The
Angola Low: relationship with southern African rainfall and ENSO, Clim.
Dynam., 52, 1783–1803, https://doi.org/10.1007/s00382-018-4222-3, 2019.
Diab, R. D., Jury, M. R., Combrink, J., and Sokolic, F.: A comparison of
anticyclone and trough influences on the vertical distribution of ozone and
meteorological conditions during SAFARI-92, J. Geophys. Res.-Atmos.,
101, 23809–23821, https://doi.org/10.1029/95JD01844, 1996.
Dieppois, B., Pohl, B., Rouault, M., New, M., Lawler, D., and Keenlyside, N.:
Interannual to interdecadal variability of winter and summer southern
African rainfall, and their teleconnections, J. Geophys. Res.-Atmos.,
121, 6215–6239, https://doi.org/10.1002/2015JD024576, 2016.
Eck, T. F., Holben, B. N., Reid, J. S., Dubovik, O., Smirnov, A., O'Neill,
N. T., Slutsker, I., and Kinne, S.: Wavelength dependence of the optical
depth of biomass burning, urban, and desert dust aerosols, J. Geophys. Res.-Atmos., 104, 31333–31349, https://doi.org/10.1029/1999JD900923, 1999.
Eck, T. F., Holben, B. N., Ward, D. E., Mukelabai, M. M., Dubovik, O.,
Smirnov, A., Schafer, J. S., Hsu, N. C., Piketh, S. J., Queface, A., Le Roux,
J., Swap, R. J., and Slutsker, I.: Variability of biomass burning aerosol
optical characteristics in southern Africa during the SAFARI 2000 dry season
campaign and a comparison of single scattering albedo estimates from
radiometric measurements, J. Geophys. Res.-Atmos., 108, 8477,
https://doi.org/10.1029/2002JD002321, 2003.
Fauchereau, N., Pohl, B., Reason, C. J. C., Rouault, M., and Richard, Y.:
Recurrent daily OLR patterns in the Southern Africa/Southwest Indian Ocean
region, implications for South African rainfall and teleconnections, Clim.
Dynam., 32, 575–591, https://doi.org/10.1007/s00382-008-0426-2, 2009.
Formenti, P., Elbert, W., Maenhaut, W., Haywood, J., Osborne, S., and
Andreae, M. O.: Inorganic and carbonaceous aerosols during the Southern
African Regional Science Initiative (SAFARI 2000) experiment: Chemical
characteristics, physical properties, and emission data for smoke from
African biomass burning, J. Geophys. Res.-Atmos., 108, 8488,
https://doi.org/10.1029/2002JD002408, 2003.
Formenti, P., D'Anna, B., Flamant, C., Mallet, M., Piketh, S. J.,
Schepanski, K., Waquet, F., Auriol, F., Brogniez, G., Burnet, F.,
Chaboureau, J.-P., Chauvigné, A., Chazette, P., Denjean, C., Desboeufs,
K., Doussin, J.-F., Elguindi, N., Feuerstein, S., Gaetani, M., Giorio, C.,
Klopper, D., Mallet, M. D., Nabat, P., Monod, A., Solmon, F., Namwoonde, A.,
Chikwililwa, C., Mushi, R., Welton, E. J., and Holben, B.: The Aerosols,
Radiation and Clouds in Southern Africa Field Campaign in Namibia: Overview,
Illustrative Observations, and Way Forward, B. Am. Meteorol. Soc.,
100, 1277–1298, https://doi.org/10.1175/BAMS-D-17-0278.1, 2019.
Gao, Y., Yu, S., Sherrell, R. M., Fan, S., Bu, K., and Anderson, J. R.:
Particle-Size Distributions and Solubility of Aerosol Iron Over the
Antarctic Peninsula During Austral Summer, J. Geophys. Res.-Atmos., 125,
e2019JD032082, https://doi.org/10.1029/2019JD032082, 2020.
Garstang, M., Tyson, P. D., Swap, R., Edwards, M., Kållberg, P., and
Lindesay, J. A.: Horizontal and vertical transport of air over southern
Africa, J. Geophys. Res.-Atmos., 101, 23721–23736,
https://doi.org/10.1029/95JD00844, 1996.
Giles, D. M., Sinyuk, A., Sorokin, M. G., Schafer, J. S., Smirnov, A., Slutsker, I., Eck, T. F., Holben, B. N., Lewis, J. R., Campbell, J. R., Welton, E. J., Korkin, S. V., and Lyapustin, A. I.: Advancements in the Aerosol Robotic Network (AERONET) Version 3 database – automated near-real-time quality control algorithm with improved cloud screening for Sun photometer aerosol optical depth (AOD) measurements, Atmos. Meas. Tech., 12, 169–209, https://doi.org/10.5194/amt-12-169-2019, 2019.
Haywood, J. M., Osborne, S. R., Francis, P. N., Keil, A., Formenti, P.,
Andreae, M. O., and Kaye, P. H.: The mean physical and optical properties of
regional haze dominated by biomass burning aerosol measured from the C-130
aircraft during SAFARI 2000, J. Geophys. Res.-Atmos., 108, 8473,
https://doi.org/10.1029/2002JD002226, 2003.
Haywood, J. M., Abel, S. J., Barrett, P. A., Bellouin, N., Blyth, A., Bower,
K. N., Brooks, M., Carslaw, K., Che, H., Coe, H., Cotterell, M. I.,
Crawford, I., Cui, Z., Davies, N., Dingley, B., Field, P., Formenti, P.,
Gordon, H., de Graaf, M., Herbert, R., Johnson, B., Jones, A. C., Langridge,
J. M., Malavelle, F., Partridge, D. G., Peers, F., Redemann, J., Stier, P.,
Szpek, K., Taylor, J. W., Watson-Parris, D., Wood, R., Wu, H., and Zuidema,
P.: The CLoud–Aerosol–Radiation Interaction and Forcing: Year 2017
(CLARIFY-2017) measurement campaign, Atmos. Chem. Phys., 21, 1049–1084,
https://doi.org/10.5194/acp-21-1049-2021, 2021.
Hersbach, H., Bell, B., Berrisford, P., Biavati, G., Horányi, A., Muñoz Sabater, J., Nicolas, J., Peubey, C., Radu, R., Rozum, I., Schepers, D., Simmons, A., Soci, C., Dee, D., and Thépaut, J.-N.: ERA5 hourly data on pressure levels from 1979 to present, Copernicus Climate Change Service (C3S) Climate Data Store (CDS) [data set], https://doi.org/10.24381/cds.bd0915c6, 2018.
Inness, A., Ades, M., Agustí-Panareda, A., Barré, J., Benedictow, A., Blechschmidt, A., Dominguez, J., Engelen, R., Eskes, H., Flemming, J., Huijnen, V., Jones, L., Kipling, Z., Massart, S., Parrington, M., Peuch, V.-H., Razinger, M., Remy, S., Schulz, M., and Suttie, M.: CAMS global reanalysis (EAC4), Copernicus Atmosphere Monitoring Service (CAMS) Atmosphere Data Store (ADS) [data set], https://ads.atmosphere.copernicus.eu/cdsapp#!/dataset/cams-global-reanalysis-eac4?tab=overview (last access: 24 July 2020), 2019.
Horowitz, H. M., Garland, R. M., Thatcher, M., Landman, W. A., Dedekind, Z.,
van der Merwe, J., and Engelbrecht, F. A.: Evaluation of climate model
aerosol seasonal and spatial variability over Africa using AERONET, Atmos.
Chem. Phys., 17, 13999–14023, https://doi.org/10.5194/acp-17-13999-2017, 2017.
Hoskins, B. J. and Ambrizzi, T.: Rossby Wave Propagation on a Realistic
Longitudinally Varying Flow, J. Atmos. Sci., 50, 1661–1671,
https://doi.org/10.1175/1520-0469(1993)050<1661:RWPOAR>2.0.CO;2,
1993.
Hu, S. and Fedorov, A. V.: The extreme El Niño of 2015–2016 and the end
of global warming hiatus, Geophys. Res. Lett., 44, 3816–3824,
https://doi.org/10.1002/2017GL072908, 2017.
Huang, B., Thorne, P. W., Banzon, V. F., Boyer, T., Chepurin, G., Lawrimore,
J. H., Menne, M. J., Smith, T. M., Vose, R. S., and Zhang, H.-M.: Extended
Reconstructed Sea Surface Temperature, Version 5 (ERSSTv5): Upgrades,
Validations, and Intercomparisons, J. Climate, 30, 8179–8205,
https://doi.org/10.1175/JCLI-D-16-0836.1, 2017.
Limpasuvan, V. and Hartmann, D. L.: Eddies and the annular modes of climate
variability, Geophys. Res. Lett., 26, 3133–3136,
https://doi.org/10.1029/1999GL010478, 1999.
Lindesay, J. A., Andreae, M. O., Goldammer, J. G., Harris, G., Annegarn, H.
J., Garstang, M., Scholes, R. J., and van Wilgen, B. W.: International
geosphere-biosphere programme/international global atmospheric chemistry
SAFARI-92 field experiment: Background and overview, J. Geophys. Res.-Atmos., 101, 23521–23530, https://doi.org/10.1029/96JD01512, 1996.
Macron, C., Pohl, B., Richard, Y., and Bessafi, M.: How do Tropical Temperate
Troughs Form and Develop over Southern Africa?, J. Clim., 27, 1633–1647,
https://doi.org/10.1175/JCLI-D-13-00175.1, 2014.
Mallet, M., Solmon, F., Nabat, P., Elguindi, N., Waquet, F., Bouniol, D.,
Sayer, A. M., Meyer, K., Roehrig, R., Michou, M., Zuidema, P., Flamant, C.,
Redemann, J., and Formenti, P.: Direct and semi-direct radiative forcing of
biomass-burning aerosols over the southeast Atlantic (SEA) and its
sensitivity to absorbing properties: a regional climate modeling study,
Atmos. Chem. Phys., 20, 13191–13216, https://doi.org/10.5194/acp-20-13191-2020,
2020.
McMillan, W. W., McCourt, M. L., Revercomb, H. E., Knuteson, R. O.,
Christian, T. J., Doddridge, B. G., Hobbs, P. V., Lukovich, J. V., Novelli,
P. C., Piketh, S. J., Sparling, L., Stein, D., Swap, R. J., and Yokelson, R.
J.: Tropospheric carbon monoxide measurements from the Scanning
High-Resolution Interferometer Sounder on 7 September 2000 in southern
Africa during SAFARI 2000, J. Geophys. Res.-Atmos., 108, 8492,
https://doi.org/10.1029/2002JD002335, 2003.
Michelangeli, P. A., Vautard, R., and Legras, B.: Weather regimes: recurrence
and quasi stationarity, J. Atmos. Sci., 52, 1237–1256,
https://doi.org/10.1175/1520-0469(1995)052<1237:WRRAQS>2.0.CO;2,
1995.
NASA Goddard Space Flight Center: AERONET station data, NASA [data set], https://aeronet.gsfc.nasa.gov/, 2021.
NOAA Climate Prediction Center: SAM daily index, NOAA [data set], https://www.cpc.ncep.noaa.gov/, 2021.
Pistone, K., Redemann, J., Doherty, S., Zuidema, P., Burton, S., Cairns, B., Cochrane, S., Ferrare, R., Flynn, C., Freitag, S., Howell, S. G., Kacenelenbogen, M., LeBlanc, S., Liu, X., Schmidt, K. S., Sedlacek III, A. J., Segal-Rozenhaimer, M., Shinozuka, Y., Stamnes, S., van Diedenhoven, B., Van Harten, G., and Xu, F.: Intercomparison of biomass burning aerosol optical properties from in situ and remote-sensing instruments in ORACLES-2016, Atmos. Chem. Phys., 19, 9181–9208, https://doi.org/10.5194/acp-19-9181-2019, 2019.
Pohl, B., Dieppois, B., Crétat, J., Lawler, D., and Rouault, M.: From
synoptic to interdecadal variability in southern African rainfall: Toward a
unified view across time scales, J. Climate, 31, 5845–5872,
https://doi.org/10.1175/JCLI-D-17-0405.1, 2018.
Rayner, N. A., Parker, D. E., Horton, E. B., Folland, C. K., Alexander, L.
V., Rowell, D. P., Kent, E. C., and Kaplan, A.: Global analyses of sea
surface temperature, sea ice, and night marine air temperature since the
late nineteenth century, J. Geophys. Res.-Atmos., 108, 4407,
https://doi.org/10.1029/2002jd002670, 2003.
Redemann, J., Wood, R., Zuidema, P., Doherty, S. J., Luna, B., LeBlanc, S. E., Diamond, M. S., Shinozuka, Y., Chang, I. Y., Ueyama, R., Pfister, L., Ryoo, J.-M., Dobracki, A. N., da Silva, A. M., Longo, K. M., Kacenelenbogen, M. S., Flynn, C. J., Pistone, K., Knox, N. M., Piketh, S. J., Haywood, J. M., Formenti, P., Mallet, M., Stier, P., Ackerman, A. S., Bauer, S. E., Fridlind, A. M., Carmichael, G. R., Saide, P. E., Ferrada, G. A., Howell, S. G., Freitag, S., Cairns, B., Holben, B. N., Knobelspiesse, K. D., Tanelli, S., L'Ecuyer, T. S., Dzambo, A. M., Sy, O. O., McFarquhar, G. M., Poellot, M. R., Gupta, S., O'Brien, J. R., Nenes, A., Kacarab, M., Wong, J. P. S., Small-Griswold, J. D., Thornhill, K. L., Noone, D., Podolske, J. R., Schmidt, K. S., Pilewskie, P., Chen, H., Cochrane, S. P., Sedlacek, A. J., Lang, T. J., Stith, E., Segal-Rozenhaimer, M., Ferrare, R. A., Burton, S. P., Hostetler, C. A., Diner, D. J., Seidel, F. C., Platnick, S. E., Myers, J. S., Meyer, K. G., Spangenberg, D. A., Maring, H., and Gao, L.: An overview of the ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) project: aerosol–cloud–radiation interactions in the southeast Atlantic basin, Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, 2021.
Stein, D. C., Swap, R. J., Greco, S., Piketh, S. J., Macko, S. A.,
Doddridge, B. G., Elias, T., and Bruintjes, R. T.: Haze layer
characterization and associated meteorological controls along the eastern
coastal region of southern Africa, J. Geophys. Res.-Atmos., 108,
8506, https://doi.org/10.1029/2002JD003237, 2003.
Stier, P., Schutgens, N. A. J., Bellouin, N., Bian, H., Boucher, O., Chin,
M., Ghan, S., Huneeus, N., Kinne, S., Lin, G., Ma, X., Myhre, G., Penner, J.
E., Randles, C. A., Samset, B., Schulz, M., Takemura, T., Yu, F., Yu, H., and
Zhou, C.: Host model uncertainties in aerosol radiative forcing estimates:
Results from the AeroCom Prescribed intercomparison study, Atmos. Chem.
Phys., 13, 3245–3270, https://doi.org/10.5194/acp-13-3245-2013, 2013.
Swap, R., Garstang, M., Macko, S. A., Tyson, P. D., Maenhaut, W., Artaxo,
P., Kållberg, P., and Talbot, R.: The long-range transport of southern
African aerosols to the tropical South Atlantic, J. Geophys. Res.-Atmos.,
101, 23777–23791, https://doi.org/10.1029/95JD01049, 1996.
Swap, R. J., Annegarn, H. J., Suttles, J. T., King, M. D., Platnick, S.,
Privette, J. L., and Scholes, R. J.: Africa burning: A thematic analysis of
the Southern African Regional Science Initiative (SAFARI 2000), J. Geophys.
Res.-Atmos., 108, 8465, https://doi.org/10.1029/2003JD003747, 2003.
Tang, C., Morel, B., Wild, M., Pohl, B., Abiodun, B., and Bessafi, M.:
Numerical simulation of surface solar radiation over Southern Africa. Part
1: Evaluation of regional and global climate models, Clim. Dyn., 52,
457–477, https://doi.org/10.1007/s00382-018-4143-1, 2019.
Tyson, P. D.: Atmospheric transport of aerosols and trace gases over
southern Africa, Prog. Phys. Geogr. Earth Environ., 21, 79–101,
https://doi.org/10.1177/030913339702100105, 1997.
van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., Mu, M.,
Kasibhatla, P. S., Morton, D. C., DeFries, R. S., Jin, Y., and van Leeuwen,
T. T.: Global fire emissions and the contribution of deforestation, savanna,
forest, agricultural, and peat fires (1997–2009), Atmos. Chem. Phys.,
10, 11707–11735, https://doi.org/10.5194/acp-10-11707-2010, 2010.
van der Werf, G. R., Randerson, J. T., Giglio, L., van Leeuwen, T. T., Chen,
Y., Rogers, B. M., Mu, M., van Marle, M. J. E., Morton, D. C., Collatz, G.
J., Yokelson, R. J., and Kasibhatla, P. S.: Global fire emissions estimates
during 1997–2016, Earth Syst. Sci. Data, 9, 697–720,
https://doi.org/10.5194/essd-9-697-2017, 2017.
Vigaud, N., Pohl, B., and Crétat, J.: Tropical-temperate interactions
over southern Africa simulated by a regional climate model, Clim. Dynam.,
39, 2895–2916, https://doi.org/10.1007/s00382-012-1314-3, 2012.
von Storch, H. and Zwiers, F. W.: Statistical Analysis in Climate Research, Cambridge University Press, Cambridge, ISBN 978-0-5116-1233-6, https://doi.org/10.1017/CBO9780511612336, 1999.
Wai, K. M., Wu, S., Kumar, A., and Liao, H.: Seasonal variability and
long-term evolution of tropospheric composition in the tropics and Southern
Hemisphere, Atmos. Chem. Phys., 14, 4859–4874,
https://doi.org/10.5194/acp-14-4859-2014, 2014.
Wu, H., Taylor, J. W., Szpek, K., Langridge, J. M., Williams, P. I., Flynn,
M., Allan, J. D., Abel, S. J., Pitt, J., Cotterell, M. I., Fox, C., Davies,
N. W., Haywood, J., and Coe, H.: Vertical variability of the properties of
highly aged biomass burning aerosol transported over the southeast Atlantic
during CLARIFY-2017, Atmos. Chem. Phys., 20, 12697–12719,
https://doi.org/10.5194/acp-20-12697-2020, 2020.
Zuidema, P., Chang, P., Medeiros, B., Kirtman, B. P., Mechoso, R.,
Schneider, E. K., Toniazzo, T., Richter, I., Small, R. J., Bellomo, K.,
Brandt, P., De Szoeke, S., Farrar, J. T., Jung, E., Kato, S., Li, M.,
Patricola, C., Wang, Z., Wood, R., and Xu, Z.: Challenges and prospects for
reducing coupled climate model sst biases in the eastern tropical atlantic
and pacific oceans: The U.S. Clivar eastern tropical oceans synthesis
working group, B. Am. Meteorol. Soc., 97, 2305–2327,
https://doi.org/10.1175/BAMS-D-15-00274.1, 2016.
Short summary
During the dry austral winter, biomass fires in tropical Africa emit large amounts of smoke in the atmosphere, with large impacts on climate and air quality. The study of the relationship between atmospheric circulation and smoke transport shows that midlatitude atmospheric disturbances may deflect the smoke from tropical Africa towards southern Africa. Understanding the distribution of the smoke in the region is crucial for climate modelling and air quality monitoring.
During the dry austral winter, biomass fires in tropical Africa emit large amounts of smoke in...
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