Articles | Volume 19, issue 5
https://doi.org/10.5194/acp-19-3341-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-19-3341-2019
© Author(s) 2019. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
14 Mar 2019
Research article |
| 14 Mar 2019
| 14 Mar 2019
Lidar observations of pyrocumulonimbus smoke plumes in the UTLS over Tomsk (Western Siberia, Russia) from 2000 to 2017
Vladimir V. Zuev
Institute of Monitoring of Climatic and Ecological Systems SB RAS, Tomsk, 634055, Russia
Vladislav V. Gerasimov
CORRESPONDING AUTHOR
Institute of Monitoring of Climatic and Ecological Systems SB RAS, Tomsk, 634055, Russia
Faculty of Physics, Tomsk State University, Tomsk, 634050, Russia
Aleksei V. Nevzorov
V. E. Zuev Institute of Atmospheric Optics SB RAS, Tomsk, 634055, Russia
Ekaterina S. Savelieva
Institute of Monitoring of Climatic and Ecological Systems SB RAS, Tomsk, 634055, Russia
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The primary objective of the Complex Aerosol Experiment was measurement of microphysical, chemical, and optical properties of aerosol particles in the surface air layer and free atmosphere. The measurement data were used to retrieve the whole set of aerosol optical parameters, necessary for radiation calculations. Three measurement cycles were performed within the experiment during 2013: in spring, summer (July), and in late summer/early autumn.
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Subject: Aerosols | Research Activity: Remote Sensing | Altitude Range: Stratosphere | Science Focus: Physics (physical properties and processes)
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During the 2020 austral summer, the pristine atmosphere of the southwest Indian Ocean basin experienced significant perturbations. Numerical models indicated that the lower-stratospheric aerosol content was influenced by the intense and persistent stratospheric aerosol layer generated during the 2019–2020 extreme Australian bushfire events. Ground-based observations at Réunion confirmed the simultaneous presence of African and Australian aerosol layers.
Sandra Graßl, Christoph Ritter, Ines Tritscher, and Bärbel Vogel
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Arctic lidar data for 1 year are compared with global modeling of aerosol tracers in the stratosphere. A trend in the aerosol backscatter can be found. These observations are further compared with a model study to investigate the aerosol origin of the observed arctic aerosol. We found a correlation with increased backscatter signal during summer and early autumn and pathways from the Southeast Asian monsoon region and remains of the Asian tropopause aerosol layer in the Arctic.
Yun He, Dongzhe Jing, Zhenping Yin, Kevin Ohneiser, and Fan Yi
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We present a long-term ground-based lidar observation of stratospheric aerosols at a mid-latitude site, Wuhan in central China, from 2010 to 2021. We observed a stratospheric background period from 2013 to mid-2017 along with several perturbations from volcanic aerosols and wildfire-induced smoke. In summer, injected stratospheric aerosols are found to be captured by the Asian monsoon anticyclone, resulting in prolonged residence and regional transport in the mid-latitude of East Asia.
Jean-Paul Vernier, Thomas J. Aubry, Claudia Timmreck, Anja Schmidt, Lieven Clarisse, Fred Prata, Nicolas Theys, Andrew T. Prata, Graham Mann, Hyundeok Choi, Simon Carn, Richard Rigby, Susan C. Loughlin, and John A. Stevenson
Atmos. Chem. Phys., 24, 5765–5782, https://doi.org/10.5194/acp-24-5765-2024, https://doi.org/10.5194/acp-24-5765-2024, 2024
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Thomas Trickl, Hannes Vogelmann, Michael D. Fromm, Horst Jäger, Matthias Perfahl, and Wolfgang Steinbrecht
Atmos. Chem. Phys., 24, 1997–2021, https://doi.org/10.5194/acp-24-1997-2024, https://doi.org/10.5194/acp-24-1997-2024, 2024
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In 2023, the lidar team at Garmisch-Partenkirchen (Germany) celebrated its 50th year of aerosol profiling. The highlight of these activities has been the lidar measurements of stratospheric aerosol carried out since 1976. The observations since 2017 are characterized by severe smoke from several big fires in North America and Siberia and three volcanic eruptions. The sudden increase in the frequency of such strong fire events is difficult to understand.
Pasquale Sellitto, Redha Belhadji, Juan Cuesta, Aurélien Podglajen, and Bernard Legras
Atmos. Chem. Phys., 23, 15523–15535, https://doi.org/10.5194/acp-23-15523-2023, https://doi.org/10.5194/acp-23-15523-2023, 2023
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Johan Friberg, Bengt G. Martinsson, and Moa K. Sporre
Atmos. Chem. Phys., 23, 12557–12570, https://doi.org/10.5194/acp-23-12557-2023, https://doi.org/10.5194/acp-23-12557-2023, 2023
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We study the short- and long-term stratospheric impact of smoke from the massive Australian wildfires in Dec 2019–Jan 2020 using four satellite sensors. Smoke entered the stratosphere rapidly via transport by firestorms, as well as weeks after the fires. The smoke particle properties evolved over time together with rapidly decreasing stratospheric aerosol load, suggesting photolytic loss of organics in the smoke particles. The depletion rate was estimated to a half-life (e folding) of 10 (14) d.
Larry W. Thomason and Travis Knepp
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We examine space-based observations of stratospheric aerosol to infer the presence of episodic smoke perturbations. We find that smoke's optical properties often show a consistent behavior but vary somewhat from event to event. We also find that the rate of smoke events observed in the 1984–2005 period is about half the rate of similar observations in the period from 2017 to the present; however, with such low overall rates, inferring change between the periods is difficult.
Felix Wrana, Ulrike Niemeier, Larry W. Thomason, Sandra Wallis, and Christian von Savigny
Atmos. Chem. Phys., 23, 9725–9743, https://doi.org/10.5194/acp-23-9725-2023, https://doi.org/10.5194/acp-23-9725-2023, 2023
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The stratospheric aerosol layer is a naturally occurring and permanent layer of aerosol, in this case very small droplets of mostly sulfuric acid and water, that has a cooling effect on our climate. To quantify this effect and for our general understanding of stratospheric microphysical processes, knowledge of the size of those aerosol particles is needed. Using satellite measurements and atmospheric models we show that some volcanic eruptions can lead to on average smaller aerosol sizes.
Bianca Lauster, Steffen Dörner, Carl-Fredrik Enell, Udo Frieß, Myojeong Gu, Janis Puķīte, Uwe Raffalski, and Thomas Wagner
Atmos. Chem. Phys., 22, 15925–15942, https://doi.org/10.5194/acp-22-15925-2022, https://doi.org/10.5194/acp-22-15925-2022, 2022
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Polar stratospheric clouds (PSCs) are an important component in ozone chemistry. Here, we use two differential optical absorption spectroscopy (DOAS) instruments in the Antarctic and Arctic to investigate the occurrence of PSCs based on the colour index, i.e. the colour of the zenith sky. Additionally using radiative transfer simulations, the variability and the seasonal cycle of PSC occurrence are analysed and an unexpectedly high signal during spring suggests the influence of volcanic aerosol.
Feiyue Mao, Ruixing Shi, Daniel Rosenfeld, Zengxin Pan, Lin Zang, Yannian Zhu, and Xin Lu
Atmos. Chem. Phys., 22, 10589–10602, https://doi.org/10.5194/acp-22-10589-2022, https://doi.org/10.5194/acp-22-10589-2022, 2022
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Previous studies generally ignored the faint aerosols undetected by the CALIPSO layer detection algorithm because they are too optically thin. Here, we retrieved the faint aerosol extinction based on instantaneous CALIPSO observations with the constraint of SAGE data. The correlation and normalized root-mean-square error of the retrievals with independent SAGE data are 0.66 and 100.6 %, respectively. The minimum retrieved extinction at night can be extended to 10-4 km-1 with 125 % uncertainty.
Pasquale Sellitto, Redha Belhadji, Corinna Kloss, and Bernard Legras
Atmos. Chem. Phys., 22, 9299–9311, https://doi.org/10.5194/acp-22-9299-2022, https://doi.org/10.5194/acp-22-9299-2022, 2022
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As a consequence of extreme heat and drought, record-breaking wildfires ravaged south-eastern Australia during the fire season in 2019–2020. Fires injected a smoke plume very high up to the stratosphere, which dispersed quite quickly to the whole Southern Hemisphere and interacted with solar radiation, reflecting and absorbing part of it – thus producing impacts on the climate system. Here we estimate this impact on radiation and we study how it depends on the properties and ageing of the plume.
Kevin Ohneiser, Albert Ansmann, Bernd Kaifler, Alexandra Chudnovsky, Boris Barja, Daniel A. Knopf, Natalie Kaifler, Holger Baars, Patric Seifert, Diego Villanueva, Cristofer Jimenez, Martin Radenz, Ronny Engelmann, Igor Veselovskii, and Félix Zamorano
Atmos. Chem. Phys., 22, 7417–7442, https://doi.org/10.5194/acp-22-7417-2022, https://doi.org/10.5194/acp-22-7417-2022, 2022
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We present and discuss 2 years of long-term lidar observations of the largest stratospheric perturbation by wildfire smoke ever observed. The smoke originated from the record-breaking Australian fires in 2019–2020 and affects climate conditions and even the ozone layer in the Southern Hemisphere. The obvious link between dense smoke occurrence in the stratosphere and strong ozone depletion found in the Arctic and in the Antarctic in 2020 can be regarded as a new aspect of climate change.
Bengt G. Martinsson, Johan Friberg, Oscar S. Sandvik, and Moa K. Sporre
Atmos. Chem. Phys., 22, 3967–3984, https://doi.org/10.5194/acp-22-3967-2022, https://doi.org/10.5194/acp-22-3967-2022, 2022
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Large amounts of wildfire smoke reached the stratosphere in 2017. The literature on stratospheric aerosol is mainly based on horizontally viewing sensors that saturate in dense smoke. Using also a vertically viewing sensor with orders of magnitude shorter path in the smoke, we show that the horizontally viewing sensors miss a dramatic exponential decline of the aerosol load with a half-life of 10 d, where 80 %–90 % of smoke is lost. We attribute the decline to photolytic loss of organic aerosol.
Kevin Ohneiser, Albert Ansmann, Alexandra Chudnovsky, Ronny Engelmann, Christoph Ritter, Igor Veselovskii, Holger Baars, Henriette Gebauer, Hannes Griesche, Martin Radenz, Julian Hofer, Dietrich Althausen, Sandro Dahlke, and Marion Maturilli
Atmos. Chem. Phys., 21, 15783–15808, https://doi.org/10.5194/acp-21-15783-2021, https://doi.org/10.5194/acp-21-15783-2021, 2021
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The highlight of the lidar measurements during the 1-year MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition of the German icebreaker Polarstern (October 2019–October 2020) was the detection of a persistent, 10 km deep Siberian wildfire smoke layer in the upper troposphere and lower stratosphere (UTLS) from about 7–8 km to 17–18 km height that could potentially have impacted the record-breaking ozone depletion over the Arctic in the spring of 2020.
Elizaveta Malinina, Alexei Rozanov, Ulrike Niemeier, Sandra Wallis, Carlo Arosio, Felix Wrana, Claudia Timmreck, Christian von Savigny, and John P. Burrows
Atmos. Chem. Phys., 21, 14871–14891, https://doi.org/10.5194/acp-21-14871-2021, https://doi.org/10.5194/acp-21-14871-2021, 2021
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In the paper, changes in the stratospheric aerosol loading after the 2018 Ambae eruption were analyzed using OMPS-LP observations. The eruption was also simulated with the MAECHAM5-HAM global climate model. Generally, the model and observations agree very well. We attribute the good consistency of the results to a precisely determined altitude and mass of the volcanic injection, as well as nudging of the meteorological data. The radiative forcing from the eruption was estimated to be −0.13 W m−2.
Albert Ansmann, Kevin Ohneiser, Rodanthi-Elisavet Mamouri, Daniel A. Knopf, Igor Veselovskii, Holger Baars, Ronny Engelmann, Andreas Foth, Cristofer Jimenez, Patric Seifert, and Boris Barja
Atmos. Chem. Phys., 21, 9779–9807, https://doi.org/10.5194/acp-21-9779-2021, https://doi.org/10.5194/acp-21-9779-2021, 2021
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We present retrievals of tropospheric and stratospheric height profiles of particle mass, volume, surface area concentration of wildfire smoke layers, and related cloud condensation nuclei (CCN) and ice-nucleating particle (INP) concentrations. The new analysis scheme is applied to ground-based lidar observations of stratospheric Australian smoke over southern South America and to spaceborne lidar observations of tropospheric North American smoke.
Marcel Snels, Francesco Colao, Francesco Cairo, Ilir Shuli, Andrea Scoccione, Mauro De Muro, Michael Pitts, Lamont Poole, and Luca Di Liberto
Atmos. Chem. Phys., 21, 2165–2178, https://doi.org/10.5194/acp-21-2165-2021, https://doi.org/10.5194/acp-21-2165-2021, 2021
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A total of 5 years of polar stratospheric cloud (PSC) observations by ground-based lidar at Concordia station (Antarctica) are presented. These data have been recorded in coincidence with the overpasses of the CALIOP lidar on the CALIPSO satellite. First we demonstrate that both lidars observe essentially the same thing, in terms of detection and composition of the PSCs. Then we use both datasets to study seasonal and interannual variations in the formation temperature of NAT mixtures.
Larry W. Thomason, Mahesh Kovilakam, Anja Schmidt, Christian von Savigny, Travis Knepp, and Landon Rieger
Atmos. Chem. Phys., 21, 1143–1158, https://doi.org/10.5194/acp-21-1143-2021, https://doi.org/10.5194/acp-21-1143-2021, 2021
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Measurements of the impact of volcanic eruptions on stratospheric aerosol loading by space-based instruments show show a fairly well-behaved relationship between the magnitude and the apparent changes to aerosol size over several orders of magnitude. This directly measured relationship provides a unique opportunity to verify the performance of interactive aerosol models used in climate models.
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Felix Ploeger, Ghassan Taha, Mariam Tidiga, Maxim Eremenko, Adriana Bossolasco, Fabrice Jégou, Jean-Baptiste Renard, and Bernard Legras
Atmos. Chem. Phys., 21, 535–560, https://doi.org/10.5194/acp-21-535-2021, https://doi.org/10.5194/acp-21-535-2021, 2021
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The year 2019 was particularly rich for the stratospheric aerosol layer due to two volcanic eruptions (at Raikoke and Ulawun) and wildfire events. With satellite observations and models, we describe the exceptionally complex situation following the Raikoke eruption. The respective plume overwhelmed the Northern Hemisphere stratosphere in terms of aerosol load and resulted in the highest climate impact throughout the past decade.
Anna Gialitaki, Alexandra Tsekeri, Vassilis Amiridis, Romain Ceolato, Lucas Paulien, Anna Kampouri, Antonis Gkikas, Stavros Solomos, Eleni Marinou, Moritz Haarig, Holger Baars, Albert Ansmann, Tatyana Lapyonok, Anton Lopatin, Oleg Dubovik, Silke Groß, Martin Wirth, Maria Tsichla, Ioanna Tsikoudi, and Dimitris Balis
Atmos. Chem. Phys., 20, 14005–14021, https://doi.org/10.5194/acp-20-14005-2020, https://doi.org/10.5194/acp-20-14005-2020, 2020
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Stratospheric smoke particles are found to significantly depolarize incident light, while this effect is also accompanied by a strong spectral dependence. We utilize scattering simulations to show that this behaviour can be attributed to the near-spherical shape of the particles. We also examine whether an extension of the current AERONET scattering model to include the near-spherical shapes could be of benefit to the AERONET retrieval for stratospheric smoke associated with enhanced PLDR.
Kevin Ohneiser, Albert Ansmann, Holger Baars, Patric Seifert, Boris Barja, Cristofer Jimenez, Martin Radenz, Audrey Teisseire, Athina Floutsi, Moritz Haarig, Andreas Foth, Alexandra Chudnovsky, Ronny Engelmann, Félix Zamorano, Johannes Bühl, and Ulla Wandinger
Atmos. Chem. Phys., 20, 8003–8015, https://doi.org/10.5194/acp-20-8003-2020, https://doi.org/10.5194/acp-20-8003-2020, 2020
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Unique lidar observations of a strong perturbation in stratospheric aerosol conditions in the Southern Hemisphere caused by the extreme Australian bushfires in 2019–2020 are presented. One of the main goals of this article is to provide the CALIPSO and Aeolus spaceborne lidar science teams with basic input parameters (lidar ratios, depolarization ratios) for a trustworthy documentation of this record-breaking event.
Fernando Chouza, Thierry Leblanc, John Barnes, Mark Brewer, Patrick Wang, and Darryl Koon
Atmos. Chem. Phys., 20, 6821–6839, https://doi.org/10.5194/acp-20-6821-2020, https://doi.org/10.5194/acp-20-6821-2020, 2020
Holger Baars, Albert Ansmann, Kevin Ohneiser, Moritz Haarig, Ronny Engelmann, Dietrich Althausen, Ingrid Hanssen, Michael Gausa, Aleksander Pietruczuk, Artur Szkop, Iwona S. Stachlewska, Dongxiang Wang, Jens Reichardt, Annett Skupin, Ina Mattis, Thomas Trickl, Hannes Vogelmann, Francisco Navas-Guzmán, Alexander Haefele, Karen Acheson, Albert A. Ruth, Boyan Tatarov, Detlef Müller, Qiaoyun Hu, Thierry Podvin, Philippe Goloub, Igor Veselovskii, Christophe Pietras, Martial Haeffelin, Patrick Fréville, Michaël Sicard, Adolfo Comerón, Alfonso Javier Fernández García, Francisco Molero Menéndez, Carmen Córdoba-Jabonero, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Daniele Bortoli, Maria João Costa, Davide Dionisi, Gian Luigi Liberti, Xuan Wang, Alessia Sannino, Nikolaos Papagiannopoulos, Antonella Boselli, Lucia Mona, Giuseppe D'Amico, Salvatore Romano, Maria Rita Perrone, Livio Belegante, Doina Nicolae, Ivan Grigorov, Anna Gialitaki, Vassilis Amiridis, Ourania Soupiona, Alexandros Papayannis, Rodanthi-Elisaveth Mamouri, Argyro Nisantzi, Birgit Heese, Julian Hofer, Yoav Y. Schechner, Ulla Wandinger, and Gelsomina Pappalardo
Atmos. Chem. Phys., 19, 15183–15198, https://doi.org/10.5194/acp-19-15183-2019, https://doi.org/10.5194/acp-19-15183-2019, 2019
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Felix Ploeger, Silvia Bucci, Sergey Khaykin, Fabrice Jégou, Ghassan Taha, Larry W. Thomason, Brice Barret, Eric Le Flochmoen, Marc von Hobe, Adriana Bossolasco, Nelson Bègue, and Bernard Legras
Atmos. Chem. Phys., 19, 13547–13567, https://doi.org/10.5194/acp-19-13547-2019, https://doi.org/10.5194/acp-19-13547-2019, 2019
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With satellite measurements and transport models, we show that a plume resulting from strong Canadian fires in July/August 2017 was not only distributed throughout the northern/higher latitudes, but also reached the faraway tropics, aided by the circulation of Asian monsoon anticyclone. The regional climate impact in the wider Asian monsoon area in September exceeds the impact of the Asian tropopause aerosol layer by a factor of ~ 3 and compares to that of an advected moderate volcanic eruption.
Qiaoyun Hu, Philippe Goloub, Igor Veselovskii, Juan-Antonio Bravo-Aranda, Ioana Elisabeta Popovici, Thierry Podvin, Martial Haeffelin, Anton Lopatin, Oleg Dubovik, Christophe Pietras, Xin Huang, Benjamin Torres, and Cheng Chen
Atmos. Chem. Phys., 19, 1173–1193, https://doi.org/10.5194/acp-19-1173-2019, https://doi.org/10.5194/acp-19-1173-2019, 2019
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Smoke plumes generated in Canadian fire activities were elevated to the lower stratosphere and transported from North America to Europe. The smoke plumes were observed by three lidar systems in northern France. This study provides a comprehensive characterization for aged smoke aerosols at high altitude using lidar observations. It presents that fire activities on the Earth's surface can be an important contributor of stratospheric aerosols and impact the Earth's radiation budget.
Marcel Snels, Andrea Scoccione, Luca Di Liberto, Francesco Colao, Michael Pitts, Lamont Poole, Terry Deshler, Francesco Cairo, Chiara Cagnazzo, and Federico Fierli
Atmos. Chem. Phys., 19, 955–972, https://doi.org/10.5194/acp-19-955-2019, https://doi.org/10.5194/acp-19-955-2019, 2019
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Polar stratospheric clouds are important for stratospheric chemistry and ozone depletion. Here we statistically compare ground-based and satellite-borne lidar measurements at McMurdo (Antarctica) in order to better understand the differences between ground-based and satellite-borne observations. The satellite observations have also been compared to models used in CCMVAL-2 and CCMI studies, with the goal of testing different diagnostic methods for comparing observations with model outputs.
Albert Ansmann, Holger Baars, Alexandra Chudnovsky, Ina Mattis, Igor Veselovskii, Moritz Haarig, Patric Seifert, Ronny Engelmann, and Ulla Wandinger
Atmos. Chem. Phys., 18, 11831–11845, https://doi.org/10.5194/acp-18-11831-2018, https://doi.org/10.5194/acp-18-11831-2018, 2018
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Extremely large light extinction coefficients of 500 Mm-1, about 20 times higher than after the Pinatubo volcanic eruptions in 1991, were observed by EARLINET lidars in the stratosphere over central Europe from 21 to 22 August, 2017. This paper provides an overview based on ground-based (lidar, AERONET) and satellite (MODIS, OMI) remote sensing.
Moritz Haarig, Albert Ansmann, Holger Baars, Cristofer Jimenez, Igor Veselovskii, Ronny Engelmann, and Dietrich Althausen
Atmos. Chem. Phys., 18, 11847–11861, https://doi.org/10.5194/acp-18-11847-2018, https://doi.org/10.5194/acp-18-11847-2018, 2018
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The worldwide only triple-wavelength polarization/Raman lidar was used to measure optical, microphysical, and morphological properties of aged Canadian wildfire smoke occurring in the troposphere and stratosphere over Leipzig, Germany, in August 2017. A strong contrast between the tropospheric and stratospheric smoke properties was found.
Johan Friberg, Bengt G. Martinsson, Sandra M. Andersson, and Oscar S. Sandvik
Atmos. Chem. Phys., 18, 11149–11169, https://doi.org/10.5194/acp-18-11149-2018, https://doi.org/10.5194/acp-18-11149-2018, 2018
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During 2006–2015 volcanism contributed 40 % of the stratospheric aerosol load. We compute the AOD (aerosol optical depth) of the stratosphere (from the tropopause to 35 km altitude) using new techniques of handling CALIOP data. Regional and global AODs are presented for the entire stratosphere in relation to transport patterns, and the AOD is presented for three stratospheric layers: the LMS, the potential temperature range of 380 to 470 K, and altitudes above the 470 K isentrope.
Reinhold Spang, Lars Hoffmann, Rolf Müller, Jens-Uwe Grooß, Ines Tritscher, Michael Höpfner, Michael Pitts, Andrew Orr, and Martin Riese
Atmos. Chem. Phys., 18, 5089–5113, https://doi.org/10.5194/acp-18-5089-2018, https://doi.org/10.5194/acp-18-5089-2018, 2018
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This paper represents an unprecedented pole-covering day- and nighttime climatology of the polar stratospheric clouds (PSCs) based on satellite measurements, their spatial distribution, and composition of different particle types. The climatology has a high potential for the validation and improvement of PSC schemes in chemical transport and chemistry–climate models, which is important for a better prediction of future polar ozone loss in a changing climate.
Alyn Lambert and Michelle L. Santee
Atmos. Chem. Phys., 18, 1945–1975, https://doi.org/10.5194/acp-18-1945-2018, https://doi.org/10.5194/acp-18-1945-2018, 2018
Andrew T. Prata, Stuart A. Young, Steven T. Siems, and Michael J. Manton
Atmos. Chem. Phys., 17, 8599–8618, https://doi.org/10.5194/acp-17-8599-2017, https://doi.org/10.5194/acp-17-8599-2017, 2017
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We have studied the optical properties of ash-rich and sulfate-rich volcanic aerosols by analysing satellite observations of three different volcanic eruptions. Our results indicate that ash particles have distinctive optical properties when compared to sulfates. We expect our results will improve space-borne lidar detection of volcanic aerosols and provide new insight into their interaction with the atmosphere and solar radiation.
Vladimir V. Zuev, Vladimir D. Burlakov, Aleksei V. Nevzorov, Vladimir L. Pravdin, Ekaterina S. Savelieva, and Vladislav V. Gerasimov
Atmos. Chem. Phys., 17, 3067–3081, https://doi.org/10.5194/acp-17-3067-2017, https://doi.org/10.5194/acp-17-3067-2017, 2017
Sergey M. Khaykin, Sophie Godin-Beekmann, Philippe Keckhut, Alain Hauchecorne, Julien Jumelet, Jean-Paul Vernier, Adam Bourassa, Doug A. Degenstein, Landon A. Rieger, Christine Bingen, Filip Vanhellemont, Charles Robert, Matthew DeLand, and Pawan K. Bhartia
Atmos. Chem. Phys., 17, 1829–1845, https://doi.org/10.5194/acp-17-1829-2017, https://doi.org/10.5194/acp-17-1829-2017, 2017
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The article is devoted to the long-term evolution and variability of stratospheric aerosol, which plays an important role in climate change and the ozone layer. We use 22-year long continuous observations using laser radar soundings in southern France and satellite-based observations to distinguish between natural aerosol variability (caused by volcanic eruptions) and human-induced change in aerosol concentration. An influence of growing pollution above Asia on stratospheric aerosol is found.
Alyn Lambert, Michelle L. Santee, and Nathaniel J. Livesey
Atmos. Chem. Phys., 16, 15219–15246, https://doi.org/10.5194/acp-16-15219-2016, https://doi.org/10.5194/acp-16-15219-2016, 2016
Wolfgang Woiwode, Michael Höpfner, Lei Bi, Michael C. Pitts, Lamont R. Poole, Hermann Oelhaf, Sergej Molleker, Stephan Borrmann, Marcus Klingebiel, Gennady Belyaev, Andreas Ebersoldt, Sabine Griessbach, Jens-Uwe Grooß, Thomas Gulde, Martina Krämer, Guido Maucher, Christof Piesch, Christian Rolf, Christian Sartorius, Reinhold Spang, and Johannes Orphal
Atmos. Chem. Phys., 16, 9505–9532, https://doi.org/10.5194/acp-16-9505-2016, https://doi.org/10.5194/acp-16-9505-2016, 2016
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The analysis of spectral signatures of a polar stratospheric cloud in airborne infrared remote sensing observations in the Arctic in combination with further collocated measurements supports the view that the observed cloud consisted of highly aspherical nitric acid trihydrate particles. A characteristic "shoulder-like" spectral signature may be exploited for identification of large, highly aspherical nitric acid trihydrate particles involved in denitrification of the polar winter stratosphere.
T. Grigas, M. Hervo, G. Gimmestad, H. Forrister, P. Schneider, J. Preißler, L. Tarrason, and C. O'Dowd
Atmos. Chem. Phys., 15, 12179–12191, https://doi.org/10.5194/acp-15-12179-2015, https://doi.org/10.5194/acp-15-12179-2015, 2015
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The expedited near-real-time Level 1.5 Cloud-Aerosol Lidar with Orthogonal Polarization version 3 products were evaluated against data from the ground-based European Aerosol Research Lidar Network. The statistical framework and results of the 3-year evaluation of 48 CALIOP overpasses with ground tracks within a 100km distance from operating EARLINET stations are presented.
M. J. M. Penning de Vries, S. Dörner, J. Puķīte, C. Hörmann, M. D. Fromm, and T. Wagner
Atmos. Chem. Phys., 14, 8149–8163, https://doi.org/10.5194/acp-14-8149-2014, https://doi.org/10.5194/acp-14-8149-2014, 2014
T. D. Fairlie, J.-P. Vernier, M. Natarajan, and K. M. Bedka
Atmos. Chem. Phys., 14, 7045–7057, https://doi.org/10.5194/acp-14-7045-2014, https://doi.org/10.5194/acp-14-7045-2014, 2014
I. A. Mironova and I. G. Usoskin
Atmos. Chem. Phys., 13, 8543–8550, https://doi.org/10.5194/acp-13-8543-2013, https://doi.org/10.5194/acp-13-8543-2013, 2013
M. C. Pitts, L. R. Poole, A. Lambert, and L. W. Thomason
Atmos. Chem. Phys., 13, 2975–2988, https://doi.org/10.5194/acp-13-2975-2013, https://doi.org/10.5194/acp-13-2975-2013, 2013
O. Uchino, T. Sakai, T. Nagai, K. Nakamae, I. Morino, K. Arai, H. Okumura, S. Takubo, T. Kawasaki, Y. Mano, T. Matsunaga, and T. Yokota
Atmos. Chem. Phys., 12, 11975–11984, https://doi.org/10.5194/acp-12-11975-2012, https://doi.org/10.5194/acp-12-11975-2012, 2012
L. W. Thomason
Atmos. Chem. Phys., 12, 8177–8188, https://doi.org/10.5194/acp-12-8177-2012, https://doi.org/10.5194/acp-12-8177-2012, 2012
I. A. Mironova, I. G. Usoskin, G. A. Kovaltsov, and S. V. Petelina
Atmos. Chem. Phys., 12, 769–778, https://doi.org/10.5194/acp-12-769-2012, https://doi.org/10.5194/acp-12-769-2012, 2012
A. E. Bourassa, L. A. Rieger, N. D. Lloyd, and D. A. Degenstein
Atmos. Chem. Phys., 12, 605–614, https://doi.org/10.5194/acp-12-605-2012, https://doi.org/10.5194/acp-12-605-2012, 2012
F. Vanhellemont, D. Fussen, N. Mateshvili, C. Tétard, C. Bingen, E. Dekemper, N. Loodts, E. Kyrölä, V. Sofieva, J. Tamminen, A. Hauchecorne, J.-L. Bertaux, F. Dalaudier, L. Blanot, O. Fanton d'Andon, G. Barrot, M. Guirlet, T. Fehr, and L. Saavedra
Atmos. Chem. Phys., 10, 7997–8009, https://doi.org/10.5194/acp-10-7997-2010, https://doi.org/10.5194/acp-10-7997-2010, 2010
D. Wurl, R. G. Grainger, A. J. McDonald, and T. Deshler
Atmos. Chem. Phys., 10, 4295–4317, https://doi.org/10.5194/acp-10-4295-2010, https://doi.org/10.5194/acp-10-4295-2010, 2010
C. David, P. Keckhut, A. Armetta, J. Jumelet, M. Snels, M. Marchand, and S. Bekki
Atmos. Chem. Phys., 10, 3813–3825, https://doi.org/10.5194/acp-10-3813-2010, https://doi.org/10.5194/acp-10-3813-2010, 2010
L. W. Thomason, J. R. Moore, M. C. Pitts, J. M. Zawodny, and E. W. Chiou
Atmos. Chem. Phys., 10, 2159–2173, https://doi.org/10.5194/acp-10-2159-2010, https://doi.org/10.5194/acp-10-2159-2010, 2010
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Short summary
Massive wildfires sometimes generate pyrocumulonimbus clouds (pyroCbs), inside of which combustion products can ascend to the upper troposphere or even lower stratosphere (UTLS). Smoke plumes from pyroCbs occurred in North America can spread in the UTLS for long distances and be observed in the UTLS over Europe and even over Russia. In this work, we analyzed aerosol layers detected in the UTLS over Tomsk (Russia) that could be smoke plumes from such pyroCbs that occurred in the 2000–2017 period.
Massive wildfires sometimes generate pyrocumulonimbus clouds (pyroCbs), inside of which...
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