Articles | Volume 18, issue 11
https://doi.org/10.5194/acp-18-7815-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Special issue:
https://doi.org/10.5194/acp-18-7815-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Radiative absorption enhancement of dust mixed with anthropogenic pollution over East Asia
Pengfei Tian
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou, China
Key Laboratory for Environmental Pollution Prediction and Control,
Gansu Province, College of Earth and Environmental Sciences, Lanzhou
University, Lanzhou, China
Lei Zhang
CORRESPONDING AUTHOR
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou, China
Jianmin Ma
Key Laboratory for Environmental Pollution Prediction and Control,
Gansu Province, College of Earth and Environmental Sciences, Lanzhou
University, Lanzhou, China
Laboratory for Earth Surface Processes, College of Urban and
Environmental Sciences, Peking University, Beijing, China
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou, China
Lili Xu
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou, China
Division of Geological and Planetary Sciences, California Institute of
Technology, Pasadena, CA 91125, USA
Xianjie Cao
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou, China
Jiening Liang
Key Laboratory for Semi-Arid Climate Change of the Ministry of
Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou, China
Yuemeng Ji
Department of Atmospheric Sciences, Texas A&M University, College
Station, TX 77843, USA
Jonathan H. Jiang
Jet Propulsion Laboratory, California Institute of Technology,
Pasadena, CA 91125, USA
Yuk L. Yung
Division of Geological and Planetary Sciences, California Institute of
Technology, Pasadena, CA 91125, USA
Renyi Zhang
Department of Atmospheric Sciences, Texas A&M University, College
Station, TX 77843, USA
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Jiarui Wu, Naifang Bei, Yuan Wang, Xia Li, Suixin Liu, Lang Liu, Ruonan Wang, Jiaoyang Yu, Tianhao Le, Min Zuo, Zhenxing Shen, Junji Cao, Xuexi Tie, and Guohui Li
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A source-oriented version of the WRF-Chem model is developed to conduct source identification of wintertime PM2.5 in the North China Plain. Trans-boundary transport of air pollutants generally dominates the haze pollution in Beijing and Tianjin. The air quality in Hebei, Shandong, and Shanxi is generally controlled by local emissions. Primary aerosol species, such as EC and POA, are generally controlled by local emissions, while secondary aerosol shows evident regional characteristics.
Yuan Wang, Xiaojian Zheng, Xiquan Dong, Baike Xi, Peng Wu, Timothy Logan, and Yuk L. Yung
Atmos. Chem. Phys., 20, 14741–14755, https://doi.org/10.5194/acp-20-14741-2020, https://doi.org/10.5194/acp-20-14741-2020, 2020
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A recent aircraft field campaign near the Azores in the summer of 2017 provides ample observations of aerosols and clouds with detailed vertical information. This study utilizes those observational data in combination with the aerosol-aware large-eddy simulations and aerosol reanalysis data to examine the significance of the long-range-transported aerosol effect on marine-boundary-layer clouds. It is the first time that the ACE-ENA aircraft campaign data are used for this topic.
Brigitte Rooney, Yuan Wang, Jonathan H. Jiang, Bin Zhao, Zhao-Cheng Zeng, and John H. Seinfeld
Atmos. Chem. Phys., 20, 14597–14616, https://doi.org/10.5194/acp-20-14597-2020, https://doi.org/10.5194/acp-20-14597-2020, 2020
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Wildfires have become increasingly prevalent. Intense smoke consisting of particulate matter (PM) leads to an increased risk of morbidity and mortality. The record-breaking Camp Fire ravaged Northern California for two weeks in 2018. Here, we employ a comprehensive chemical transport model along with ground-based and satellite observations to characterize the PM concentrations across Northern California and to investigate the pollution sensitivity predictions to key parameters of the model.
Cited articles
Ångström, A.: On the Atmospheric Transmission of Sun Radiation and
on Dust in the Air, Geogr. Ann., 11, 156–166, https://doi.org/10.2307/519399,
1929.
Bergstrom, R. W., Pilewskie, P., Russell, P. B., Redemann, J., Bond, T. C.,
Quinn, P. K., and Sierau, B.: Spectral absorption properties of atmospheric
aerosols, Atmos. Chem. Phys., 7, 5937–5943,
https://doi.org/10.5194/acp-7-5937-2007, 2007.
Bi, J., Huang, J., Shi, J., Hu, Z., Zhou, T., Zhang, G., Huang, Z., Wang, X.,
and Jin, H.: Measurement of scattering and absorption properties of dust
aerosol in a Gobi farmland region of northwestern China – a potential
anthropogenic influence, Atmos. Chem. Phys., 17, 7775–7792,
https://doi.org/10.5194/acp-17-7775-2017, 2017.
Bond, T. C. and Bergstrom, R. W.: Light Absorption by Carbonaceous Particles:
An Investigative Review, Aerosol Sci. Tech., 40, 27–67,
https://doi.org/10.1080/02786820500421521, 2006.
Cai, W., Li, K., Liao, H., Wang, H., and Wu, L.: Weather conditions conducive
to Beijing severe haze more frequent under climate change, Nat. Clim. Change,
7, 257–262, https://doi.org/10.1038/nclimate3249, 2017.
Charlson, R. J., Schwartz, S. E., Hales, J. M., Cess, R. D., Coakley, J. A.,
Hansen, J. E., and Hofmann, D. J.: Climate Forcing by Anthropogenic Aerosols,
Science, 255, 423–430, https://doi.org/10.1126/science.255.5043.423, 1992.
Chen, W., Tang, H., Zhao, H., and Yan, L.: Analysis of Aerosol Properties in
Beijing Based on Ground-Based Sun Photometer and Air Quality Monitoring
Observations from 2005 to 2014, Remote Sens., 8, 110,
https://doi.org/10.3390/rs8020110, 2016.
Cui, X., Wang, X., Yang, L., Chen, B., Chen, J., Andersson, A., and
Gustafsson, Ö.: Radiative absorption enhancement from coatings on black
carbon aerosols, Sci. Total Environ., 551–552, 51–56, 2016.
Derimian, Y., Léon, J. F., Dubovik, O., Chiapello, I., Tanré, D.,
Sinyuk, A., Auriol, F., Podvin, T., Brogniez, G., and Holben, B. N.:
Radiative properties of aerosol mixture observed during the dry season 2006
over M'Bour, Senegal (African Monsoon Multidisciplinary Analysis campaign),
J. Geophys. Res.-Atmos., 113, D00C09, https://doi.org/10.1029/2008JD009904, 2008.
Derimian, Y., Dubovik, O., Huang, X., Lapyonok, T., Litvinov, P., Kostinski,
A. B., Dubuisson, P., and Ducos, F.: Comprehensive tool for calculation of
radiative fluxes: illustration of shortwave aerosol radiative effect
sensitivities to the details in aerosol and underlying surface
characteristics, Atmos. Chem. Phys., 16, 5763–5780,
https://doi.org/10.5194/acp-16-5763-2016, 2016.
Ding, A. J., Huang, X., Nie, W., Sun, J. N., Kerminen, V. M., Petäjä,
T., Su, H., Cheng, Y. F., Yang, X. Q., Wang, M. H., Chi, X. G., Wang, J. P.,
Virkkula, A., Guo, W. D., Yuan, J., Wang, S. Y., Zhang, R. J., Wu, Y. F.,
Song, Y., Zhu, T., Zilitinkevich, S., Kulmala, M., and Fu, C. B.: Enhanced
haze pollution by black carbon in megacities in China, Geophys. Res. Lett.,
43, 2873–2879, https://doi.org/10.1002/2016GL067745, 2016.
Dubovik, O. and King, M. D.: A flexible inversion algorithm for retrieval of
aerosol optical properties from Sun and sky radiance measurements, J.
Geophys. Res.-Atmos., 105, 20673–20696, https://doi.org/10.1029/2000JD900282, 2000.
Eck, T. F., Holben, B. N., Sinyuk, A., Pinker, R. T., Goloub, P., Chen, H.,
Chatenet, B., Li, Z., Singh, R. P., Tripathi, S. N., Reid, J. S., Giles, D.
M., Dubovik, O., O'Neill, N. T., Smirnov, A., Wang, P., and Xia, X.:
Climatological aspects of the optical properties of fine/coarse mode aerosol
mixtures, J. Geophys. Res.-Atmos., 115, D19205, https://doi.org/10.1029/2010JD014002,
2010.
Fan, J., Zhang, R., Li, G., and Tao, W. K.: Effects of aerosols and relative
humidity on cumulus clouds, J. Geophys. Res.-Atmos., 112,
D14204, https://doi.org/10.1029/2006JD008136, 2007.
García, O. E., Díaz, J. P., Expósito, F. J., Díaz, A. M.,
Dubovik, O., Derimian, Y., Dubuisson, P., and Roger, J.-C.: Shortwave
radiative forcing and efficiency of key aerosol types using AERONET data,
Atmos. Chem. Phys., 12, 5129–5145, https://doi.org/10.5194/acp-12-5129-2012,
2012.
Giles, D. M., Holben, B. N., Eck, T. F., Sinyuk, A., Smirnov, A., Slutsker,
I., Dickerson, R. R., Thompson, A. M., and Schafer, J. S.: An analysis of
AERONET aerosol absorption properties and classifications representative of
aerosol source regions, J. Geophys. Res.-Atmos., 117, D17203,
https://doi.org/10.1029/2012JD018127, 2012.
Guo, J., Lou, M., Miao, Y., Wang, Y., Zeng, Z., Liu, H., He, J., Xu, H.,
Wang, F., and Min, M.: Trans-Pacific transport of dust aerosols from East
Asia: Insights gained from multiple observations and modeling, Environ.
Pollut., 230, 1030–1039, 2017.
Guo, S., Hu, M., Zamora, M. L., Peng, J., Shang, D., Zheng, J., Du, Z., Wu,
Z., Shao, M., Zeng, L., Molina, M. J., and Zhang, R.: Elucidating severe
urban haze formation in China, P. Natl. Acad. Sci. USA, 111, 17373–17378,
https://doi.org/10.1073/pnas.1419604111, 2014.
Hara, Y., Nishizawa, T., Sugimoto, N., Matsui, I., Pan, X., Kobayashi, H.,
Osada, K., and Uno, I.: Optical properties of mixed aerosol layers over Japan
derived with multi-wavelength Mie–Raman lidar system, J. Quant. Spectrosc.
Ra., 188, 20–27, 2017.
Haywood, J. and Boucher, O.: Estimates of the direct and indirect radiative
forcing due to tropospheric aerosols: A review, Rev. Geophys., 38, 513–543,
2000.
He, C., Liou, K.-N., Takano, Y., Zhang, R., Levy Zamora, M., Yang, P., Li,
Q., and Leung, L. R.: Variation of the radiative properties during black
carbon aging: theoretical and experimental intercomparison, Atmos. Chem.
Phys., 15, 11967–11980, https://doi.org/10.5194/acp-15-11967-2015,
2015.
Holben, B. N., Eck, T. F., Slutsker, I., Tanré, D., Buis, J. P., Setzer,
A., Vermote, E., Reagan, J. A., Kaufman, Y. J., Nakajima, T., Lavenu, F.,
Jankowiak, I., and Smirnov, A.: AERONET – A Federated Instrument Network and
Data Archive for Aerosol Characterization, Remote Sens. Environ., 66, 1–16,
https://doi.org/10.1016/S0034-4257(98)00031-5, 1998.
Hsu, W. P. and Matijević, E.: Optical properties of monodispersed
hematite hydrosols, Appl. Optics, 24, 1623–1630, https://doi.org/10.1364/AO.24.001623,
1985.
Huang, J., Wang, T., Wang, W., Li, Z., and Yan, H.: Climate effects of dust
aerosols over East Asian arid and semiarid regions, J. Geophys. Res.-Atmos.,
119, 11398–311416, https://doi.org/10.1002/2014JD021796, 2014.
Huang, K., Zhuang, G., Li, J., Wang, Q., Sun, Y., Lin, Y., and Fu, J. S.:
Mixing of Asian dust with pollution aerosol and the transformation of
aerosol components during the dust storm over China in spring 2007, J.
Geophys. Res.-Atmos., 115, D00K13, https://doi.org/10.1029/2009JD013145, 2010.
Huang, Z., Huang, J., Hayasaka, T., Wang, S., Zhou, T., and Jin, H.:
Short-cut transport path for Asian dust directly to the Arctic: a case study,
Environ. Res. Lett., 10, 114018, https://doi.org/10.1088/1748-9326/10/11/114018,
2015.
IPCC: Climate Change 2007: The Physical Science Basis. Contribution of
Working Group I to the Fourth Assessment Report of the Intergovernmental
Panel on Climate Change, edited by: Solomon, S., Qin, D., Manning, M., Chen,
Z., Marquis, M., Averyt, K. B., Tignor, M., and Miller, H. L., Cambridge
University Press, Cambridge, United Kingdom and New York, NY, USA, 996 pp.,
2007.
IPCC: Climate Change 2013: The Physical Science Basis. Contribution of
Working Group I to the Fifth Assessment Report of the Intergovernmental Panel
on Climate Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K.,
Tignor, M., Allen, S. K., Boschung, J., Nauels, A., Xia, Y., Bex, V., and
Midgley, P. M., Cambridge University Press, Cambridge, United Kingdom and New
York, NY, USA, 1535 pp., 2013.
Jacobson, M. Z.: Strong radiative heating due to the mixing state of black
carbon in atmospheric aerosols, Nature, 409, 695–697, 2001.
Khalizov, A. F., Zhang, R., Zhang, D., Xue, H., Pagels, J., and Mcmurry, P.
H.: Formation of highly hygroscopic soot aerosols upon internal mixing with
sulfuric acid vapor, J. Geophys. Res.-Atmos., 114, D05208, https://doi.org/10.1029/2008JD010595, 2009a.
Khalizov, A. F., Xue, H., Wang, L., Zheng, J., and Zhang, R.: Enhanced Light
Absorption and Scattering by Carbon Soot Aerosol Internally Mixed with
Sulfuric Acid, J. Phys. Chem. A, 113, 1066–1074, 2009b.
Khatri, P., Takamura, T., Shimizu, A., and Sugimoto, N.: Observation of low
single scattering albedo of aerosols in the downwind of the East Asian desert
and urban areas during the inflow of dust aerosols, J. Geophys. Res.-Atmos.,
119, 787–802, https://doi.org/10.1002/2013JD019961, 2014.
Kim, D.-H., Sohn, B. J., Nakajima, T., and Takamura, T.: Aerosol radiative
forcing over east Asia determined from ground-based solar radiation
measurements, J. Geophys. Res.-Atmos., 110, D10S22,
https://doi.org/10.1029/2004JD004678, 2005.
Kok, J. F., Ridley, D. A., Zhou, Q., Miller, R. L., Zhao, C., Heald, C. L.,
Ward, D. S., Albani, S., and Haustein, K.: Smaller desert dust cooling effect
estimated from analysis of dust size and abundance, Nat. Geosci., 10,
274–278, https://doi.org/10.1038/ngeo2912, 2017.
Li, G., Bei, N., Cao, J., Huang, R., Wu, J., Feng, T., Wang, Y., Liu, S.,
Zhang, Q., Tie, X., and Molina, L. T.: A possible pathway for rapid growth of
sulfate during haze days in China, Atmos. Chem. Phys., 17, 3301–3316,
https://doi.org/10.5194/acp-17-3301-2017, 2017.
Li, J., Carlson, B. E., and Lacis, A. A.: Using single-scattering albedo
spectral curvature to characterize East Asian aerosol mixtures, J. Geophys.
Res.-Atmos., 120, 2037–2052, https://doi.org/10.1002/2014JD022433, 2015.
Li, W., Shao, L., Shi, Z., Chen, J., Yang, L., Yuan, Q., Yan, C., Zhang, X.,
Wang, Y., Sun, J., Zhang, Y., Shen, X., Wang, Z., and Wang, W.: Mixing state
and hygroscopicity of dust and haze particles before leaving Asian continent,
J. Geophys. Res.-Atmos., 119, 1044–1059, https://doi.org/10.1002/2013JD021003, 2014.
Li, Z., Lee, K.-H., Wang, Y., Xin, J., and Hao, W.-M.: First
observation-based estimates of cloud-free aerosol radiative forcing across
China, J. Geophys. Res.-Atmos., 115, D00K18, https://doi.org/10.1029/2009JD013306, 2010.
Li, Z., Guo, J., Ding, A., Liao, H., Liu, J., Sun, Y., Wang, T., Xue, H.,
Zhang, H., and Zhu, B.: Aerosol and Boundary-Layer Interactions and Impact on
Air Quality, Natl. Sci. Rev., 4, 810–833, https://doi.org/10.1093/nsr/nwx117, 2017.
Logan, T., Xi, B., Dong, X., Li, Z., and Cribb, M.: Classification and
investigation of Asian aerosol absorptive properties, Atmos. Chem. Phys., 13,
2253–2265, https://doi.org/10.5194/acp-13-2253-2013, 2013.
Ma, Q., Liu, Y., Liu, C., Ma, J., and He, H.: A case study of Asian dust
storm particles: Chemical composition, reactivity to SO2 and
hygroscopic properties, J. Environ. Sci., 24, 62–71, 2012.
Noh, Y., Müller, D., Lee, H., Lee, K., Kim, K., Shin, S., and Kim, Y. J.:
Estimation of radiative forcing by the dust and non-dust content in mixed
East Asian pollution plumes on the basis of depolarization ratios measured
with lidar, Atmos. Environ., 61, 221–231, 2012.
Noh, Y., Müller, D., Lee, K., Kim, K., Lee, K., Shimizu, A., Sano, I.,
and Park, C. B.: Depolarization ratios retrieved by AERONET sun–sky
radiometer data and comparison to depolarization ratios measured with lidar,
Atmos. Chem. Phys., 17, 6271–6290, https://doi.org/10.5194/acp-17-6271-2017,
2017.
Obregón, M. A., Pereira, S., Salgueiro, V., Costa, M. J., Silva, A. M.,
Serrano, A., and Bortoli, D.: Aerosol radiative effects during two desert
dust events in August 2012 over the Southwestern Iberian Peninsula, Atmos.
Res., 153, 404–415, 2015.
Pagels, J., Khalizov, A. F., McMurry, P. H., and Zhang, R. Y.: Processing of
Soot by Controlled Sulphuric Acid and Water Condensation – Mass and Mobility
Relationship, Aerosol Sci. Tech., 43, 629–640, 2009.
Pan, X., Uno, I., Wang, Z., Nishizawa, T., Sugimoto, N., Yamamoto, S.,
Kobayashi, H., Sun, Y., Fu, P., Tang, X., and Wang, Z.: Real-time
observational evidence of changing Asian dust morphology with the mixing of
heavy anthropogenic pollution, Sci. Rep., 7, 335,
https://doi.org/10.1038/s41598-017-00444-w, 2017.
Peng, J., Hu, M., Guo, S., Du, Z., Zheng, J., Shang, D., Levy Zamora, M.,
Zeng, L., Shao, M., Wu, Y.-S., Zheng, J., Wang, Y., Glen, C. R., Collins, D.
R., Molina, M. J., and Zhang, R.: Markedly enhanced absorption and direct
radiative forcing of black carbon under polluted urban environments, P. Natl.
Acad. Sci. USA, 113, 4266–4271, https://doi.org/10.1073/pnas.1602310113, 2016.
Qiu, C., Wang, L., Lal, V., Khalizov, A. F., and Zhang, R.: Heterogeneous
reactions of alkylamines with ammonium sulfate and ammonium bisulfate,
Environ. Sci. Technol., 45, 4748–4755, 2011.
Ramanathan, V. and Carmichael, G.: Global and regional climate changes due to
black carbon, Nat. Geosci., 1, 221–227, 2008.
Ricchiazzi, P., Yang, S. R., Gautier, C., and Sowle, D.: SBDART: A research
and teaching software tool for plane-parallell radiative transfer in the
Earth's atmosphere, B. Am. Meteorol. Soc., 79, 2101–2114,
https://doi.org/10.1175/1520-0477(1998)079<2101:SARATS>2.0.CO;2, 1998.
Schuster, G. L., Dubovik, O., and Arola, A.: Remote sensing of soot carbon –
Part 1: Distinguishing different absorbing aerosol species, Atmos. Chem.
Phys., 16, 1565–1585, https://doi.org/10.5194/acp-16-1565-2016, 2016.
Seinfeld, J. H., Carmichael, G. R., Arimoto, R., Conant, W. C., Brechtel, F.
J., Bates, T. S., Cahill, T. A., Clarke, A. D., Doherty, S. J., Flatau, P.
J., Huebert, B. J., Kim, J., Markowicz, K. M., Quinn, P. K., Russell, L. M.,
Russell, P. B., Shimizu, A., Shinozuka, Y., Song, C. H., Tang, Y., Uno, I.,
Vogelmann, A. M., Weber, R. J., Woo, J.-H., and Zhang, X. Y.: ACE-ASIA:
Regional Climatic and Atmospheric Chemical Effects of Asian Dust and
Pollution, B. Am. Meteorol. Soc., 85, 367–380, https://doi.org/10.1175/bams-85-3-367,
2004.
Stevens, B. and Bony, S.: What Are Climate Models Missing?, Science, 340,
1053–1054, https://doi.org/10.1126/science.1237554, 2013.
Sugimoto, N., Nishizawa, T., Shimizu, A., Matsui, I., and Kobayashi, H.:
Detection of internally mixed Asian dust with air pollution aerosols using a
polarization optical particle counter and a polarization-sensitive
two-wavelength lidar, J. Quant. Spectrosc. Ra., 150, 107–113, 2015.
Taylor, M., Kazadzis, S., Amiridis, V., and Kahn, R. A.: Global aerosol
mixtures and their multiyear and seasonal characteristics, Atmos. Environ.,
116, 112–129, 2015.
Tian, P., Cao, X., Zhang, L., Wang, H., Shi, J., Huang, Z., Zhou, T., and
Liu, H.: Observation and simulation study of atmospheric aerosol
nonsphericity over the Loess Plateau in northwest China, Atmos. Environ.,
117, 212–219, 2015.
Tian, P., Cao, X., Zhang, L., Sun, N., Sun, L., Logan, T., Shi, J., Wang, Y.,
Ji, Y., Lin, Y., Huang, Z., Zhou, T., Shi, Y., and Zhang, R.: Aerosol
vertical distribution and optical properties over China from long-term
satellite and ground-based remote sensing, Atmos. Chem. Phys., 17,
2509–2523, https://doi.org/10.5194/acp-17-2509-2017, 2017.
Tian, P., Zhang, L., Cao, X., Sun, N., Mo, X., Liang, J., Li, X., Gao, X.,
and Zhang, B.: Enhanced Bottom-of-the-Atmosphere Cooling and Atmosphere
Heating Efficiency by Mixed-Type Aerosols: A Classification Based on Aerosol
Nonsphericity, J. Atmos. Sci., 75, 113–124, https://doi.org/10.1175/JAS-D-17-0019.1,
2018.
Twomey, S.: The Influence of Pollution on the Shortwave Albedo of Clouds, J.
Atmos. Sci., 34, 1149–1152, 1977.
Tobo, Y., Zhang, D., Matsuki, A., and Iwasaka, Y.: Asian dust particles
converted into aqueous droplets under remote marine atmospheric conditions,
P. Natl. Acad. Sci. USA, 107, 17905–17910, https://doi.org/10.1073/pnas.1008235107,
2010.
Wang, G., Zhang, R., Gomez, M. E., Yang, L., Levy Zamora, M., Hu, M., Lin,
Y., Peng, J., Guo, S., Meng, J., Li, J., Cheng, C., Hu, T., Ren, Y., Wang,
Y., Gao, J., Cao, J., An, Z., Zhou, W., Li, G., Wang, J., Tian, P.,
Marrero-Ortiz, W., Secrest, J., Du, Z., Zheng, J., Shang, D., Zeng, L., Shao,
M., Wang, W., Huang, Y., Wang, Y., Zhu, Y., Li, Y., Hu, J., Pan, B., Cai, L.,
Cheng, Y., Ji, Y., Zhang, F., Rosenfeld, D., Liss, P. S., Duce, R. A., Kolb,
C. E., and Molina, M. J.: Persistent sulfate formation from London Fog to
Chinese haze, P. Natl. Acad. Sci. USA, 113, 13630–13635,
https://doi.org/10.1073/pnas.1616540113, 2016.
Wang, R., Tao, S., Wang, W., Liu, J., Shen, H., Shen, G., Wang, B., Liu, X.,
Li, W., Huang, Y., Zhang, Y., Lu, Y., Chen, H., Chen, Y., Wang, C., Zhu, D.,
Wang, X., Li, B., Liu, W., and Ma, J.: Black Carbon Emissions in China from
1949 to 2050, Environ. Sci. Technol., 46, 7595–7603, https://doi.org/10.1021/es3003684,
2012.
Wang, Y., Wan, Q., Meng, W., Liao, F., Tan, H., and Zhang, R.: Long-term
impacts of aerosols on precipitation and lightning over the Pearl River Delta
megacity area in China, Atmos. Chem. Phys., 11, 12421–12436,
https://doi.org/10.5194/acp-11-12421-2011, 2011.
Wang, Z., Pan, X., Uno, I., Li, J., Wang, Z., Chen, X., Fu, P., Yang, T.,
Kobayashi, H., Shimizu, A., Sugimoto, N., and Yamamoto, S.: Significant
impacts of heterogeneous reactions on the chemical composition and mixing
state of dust particles: A case study during dust events over northern China,
Atmos. Environ., 159, 83–91, 2017.
Wu, G., Li, Z., Fu, C., Zhang, X., Zhang, R., Zhang, R., Zhou, T., Li, J.,
Li, J., Zhou, D., Wu, L., Zhou, L., He, B., and Huang, R.: Advances in
studying interactions between aerosols and monsoon in China, Sci. China Earth
Sci., 59, 1–16, https://doi.org/10.1007/s11430-015-5198-z,
2016.
Wu, Y., Zhu, J., Che, H., Xia, X., and Zhang, R.: Column-integrated aerosol
optical properties and direct radiative forcing based on sun photometer
measurements at a semi-arid rural site in Northeast China, Atmos. Res., 157,
56–65, 2015.
Xin, J., Gong, C., Wang, S., and Wang, Y.: Aerosol direct radiative forcing
in desert and semi-desert regions of northwestern China, Atmos. Res., 171,
56–65, 2016.
Xue, H., Khalizov, A. F., Wang, L., Zheng, J., and Zhang, R.: Effects of
dicarboxylic acid coating on the optical properties of soot, Phys. Chem.
Chem. Phys., 11, 7869–7875, 2009.
Yu, X., Lü, R., Kumar, K. R., Ma, J., Zhang, Q., Jiang, Y., Kang, N.,
Yang, S., Wang, J., and Li, M.: Dust aerosol properties and radiative forcing
observed in spring during 2001–2014 over urban Beijing, China, Environ. Sci.
Pollut. R., 23, 15432–15442, https://doi.org/10.1007/s11356-016-6727-9, 2016.
Zhang, D. and Zhang, R.: Laboratory Investigation of Heterogeneous
Interaction of Sulfuric Acid with Soot, Environ. Sci. Technol., 39,
5722–5728, https://doi.org/10.1021/es050372d, 2005.
Zhang, M., Wang, L., Gong, W., Ma, Y., and Liu, B.: Aerosol Optical
Properties and Direct Radiative Effects over Central China, Remote Sens., 9,
997, https://doi.org/10.3390/rs9100997, 2017.
Zhang, R., Mingtaun Leu, A., and Keyser, L. F.: Heterogeneous Chemistry of
HONO on Liquid Sulfuric Acid:? A New Mechanism of Chlorine Activation on
Stratospheric Sulfate Aerosols, J. Phys. Chem., 100, 339–345, 1996.
Zhang, R., Khalizov, A. F., Pagels, J., Zhang, D., Xue, H., and McMurry, P.
H.: Variability in morphology, hygroscopicity, and optical properties of soot
aerosols during atmospheric processing, P. Natl. Acad. Sci. USA, 105,
10291–10296, https://doi.org/10.1073/pnas.0804860105, 2008.
Zhang, R., Wang, G., Guo, S., Zamora, M. L., Ying, Q., Lin, Y., Wang, W., Hu,
M., and Wang, Y.: Formation of Urban Fine Particulate Matter, Chem. Rev.,
115, 3803–3855, https://doi.org/10.1021/acs.chemrev.5b00067, 2015.
Zhao, C., Tie, X., and Lin, Y.: A possible positive feedback of reduction of
precipitation and increase in aerosols over eastern central China, Geophys.
Res. Lett., 33, L11814, https://doi.org/10.1029/2006GL025959, 2006.
Short summary
The mixing of dust and anthropogenic pollution over East Asia plays a significant yet poorly quantified role in aerosol radiative effects. We have found that radiative absorption of the East Asian aerosol mixtures are significantly enhanced. Our results show that the interaction between dust and anthropogenic pollution not only represents a viable aerosol formation pathway but also results in unfavorable dispersion conditions, both exacerbating the regional air pollution in East Asia.
The mixing of dust and anthropogenic pollution over East Asia plays a significant yet poorly...
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