Articles | Volume 16, issue 11
https://doi.org/10.5194/acp-16-7251-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-16-7251-2016
© Author(s) 2016. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| 
10 Jun 2016
Research article |
| 10 Jun 2016
Derivation of physical and optical properties of mid-latitude cirrus ice crystals for a size-resolved cloud microphysics model
NASA Goddard Institute for Space Studies, 2880 Broadway, New York, NY, USA
Rachel Atlas
University of Chicago, Chicago, IL, USA
Bastiaan van Diedenhoven
NASA Goddard Institute for Space Studies, 2880 Broadway, New York, NY, USA
Columbia University, New York, NY, USA
Junshik Um
University of Illinois, Urbana-Champaign, IL, USA
Greg M. McFarquhar
University of Illinois, Urbana-Champaign, IL, USA
Andrew S. Ackerman
NASA Goddard Institute for Space Studies, 2880 Broadway, New York, NY, USA
Elisabeth J. Moyer
University of Chicago, Chicago, IL, USA
R. Paul Lawson
Spec Inc., Boulder, Colorado, USA
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EGUsphere, https://doi.org/10.5194/egusphere-2024-3462, https://doi.org/10.5194/egusphere-2024-3462, 2024
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The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCSs) when a large number of small ice particles with typical sizes of a few hundred micrometers is found at high altitudes. It was found that secondary ice production in the vicinity of the melting layer plays a key role in the formation and maintenance of HIWC. This study presents a conceptual model of the formation of HIWC in tropical MCSs based on in situ observations and numerical simulation.
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Atmos. Chem. Phys., 24, 11791–11805, https://doi.org/10.5194/acp-24-11791-2024, https://doi.org/10.5194/acp-24-11791-2024, 2024
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The measured aerosol size distribution modes reveal distinct properties characteristic of cold-air outbreaks in the Norwegian Arctic. We find higher sea spray number concentrations, smaller Hoppel minima, lower effective supersaturations, and accumulation-mode particle scavenging during cold-air outbreaks. These results advance our understanding of cold-air outbreak aerosol–cloud interactions in order to improve their accurate representation in models.
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Atmos. Chem. Phys., 24, 10793–10814, https://doi.org/10.5194/acp-24-10793-2024, https://doi.org/10.5194/acp-24-10793-2024, 2024
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Using computer simulations and real measurements, we discovered that storms over the Amazon were narrower but more intense during the dry periods, producing heavier rain and more ice particles in the clouds. Our research showed that cumulus bubbles played a key role in creating these intense storms. This study can improve the representation of the effect of continental and ocean environments on tropical regions' rainfall patterns in simulations.
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The evolution of cloud droplets, from the point they are activated by atmospheric aerosol to the formation of precipitation, is an important process relevant to understanding cloud-climate feedbacks. This study demonstrates a benchmark framework for using novel airborne measurements and retrievals to constrain high-resolution simulations of moderately deep cumulus clouds and pathways for scaling results to large-scale models and space-based observational platforms.
Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
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Human activities release copious amounts of small particles called aerosols into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate, whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
EGUsphere, https://doi.org/10.5194/egusphere-2024-778, https://doi.org/10.5194/egusphere-2024-778, 2024
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Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in drier, warmer air, which can lead to a reduction in cloud. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence had led us to conclude.
Kamil Mroz, Alessandro Battaglia, and Ann M. Fridlind
Atmos. Meas. Tech., 17, 1577–1597, https://doi.org/10.5194/amt-17-1577-2024, https://doi.org/10.5194/amt-17-1577-2024, 2024
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In this study, we examine the extent to which radar measurements from space can inform us about the properties of clouds and precipitation. Surprisingly, our analysis showed that the amount of ice turning into rain was lower than expected in the current product. To improve on this, we came up with a new way to extract information about the size and concentration of particles from radar data. As long as we use this method in the right conditions, we can even estimate how dense the ice is.
McKenna W. Stanford, Ann M. Fridlind, Israel Silber, Andrew S. Ackerman, Greg Cesana, Johannes Mülmenstädt, Alain Protat, Simon Alexander, and Adrian McDonald
Atmos. Chem. Phys., 23, 9037–9069, https://doi.org/10.5194/acp-23-9037-2023, https://doi.org/10.5194/acp-23-9037-2023, 2023
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Clouds play an important role in the Earth’s climate system as they modulate the amount of radiation that either reaches the surface or is reflected back to space. This study demonstrates an approach to robustly evaluate surface-based observations against a large-scale model. We find that the large-scale model precipitates too infrequently relative to observations, contrary to literature documentation suggesting otherwise based on satellite measurements.
Frederic Tridon, Israel Silber, Alessandro Battaglia, Stefan Kneifel, Ann Fridlind, Petros Kalogeras, and Ranvir Dhillon
Atmos. Chem. Phys., 22, 12467–12491, https://doi.org/10.5194/acp-22-12467-2022, https://doi.org/10.5194/acp-22-12467-2022, 2022
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The role of ice precipitation in the Earth water budget is not well known because ice particles are complex, and their formation involves intricate processes. Riming of ice crystals by supercooled water droplets is an efficient process, but little is known about its importance at high latitudes. In this work, by exploiting the deployment of an unprecedented number of remote sensing systems in Antarctica, we find that riming occurs at much lower temperatures compared with the mid-latitudes.
Michael S. Diamond, Pablo E. Saide, Paquita Zuidema, Andrew S. Ackerman, Sarah J. Doherty, Ann M. Fridlind, Hamish Gordon, Calvin Howes, Jan Kazil, Takanobu Yamaguchi, Jianhao Zhang, Graham Feingold, and Robert Wood
Atmos. Chem. Phys., 22, 12113–12151, https://doi.org/10.5194/acp-22-12113-2022, https://doi.org/10.5194/acp-22-12113-2022, 2022
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Smoke from southern Africa blankets the southeast Atlantic from June-October, overlying a major transition region between overcast and scattered clouds. The smoke affects Earth's radiation budget by absorbing sunlight and changing cloud properties. We investigate these effects in regional climate and large eddy simulation models based on international field campaigns. We find that large-scale circulation changes more strongly affect cloud transitions than smoke microphysical effects in our case.
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Atmos. Chem. Phys., 22, 711–724, https://doi.org/10.5194/acp-22-711-2022, https://doi.org/10.5194/acp-22-711-2022, 2022
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Florian Tornow, Andrew S. Ackerman, and Ann M. Fridlind
Atmos. Chem. Phys., 21, 12049–12067, https://doi.org/10.5194/acp-21-12049-2021, https://doi.org/10.5194/acp-21-12049-2021, 2021
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Cold air outbreaks affect the local energy budget by forming bright boundary layer clouds that, once it rains, evolve into dimmer, broken cloud fields that are depleted of condensation nuclei – an evolution consistent with closed-to-open cell transitions. We find that cloud ice accelerates this evolution, primarily via riming prior to rain onset, which (1) reduces liquid water, (2) reduces condensation nuclei, and (3) leads to early precipitation cooling and moistening below cloud.
Israel Silber, Ann M. Fridlind, Johannes Verlinde, Andrew S. Ackerman, Grégory V. Cesana, and Daniel A. Knopf
Atmos. Chem. Phys., 21, 3949–3971, https://doi.org/10.5194/acp-21-3949-2021, https://doi.org/10.5194/acp-21-3949-2021, 2021
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Long-term ground-based radar and sounding measurements over Alaska (Antarctica) indicate that more than 85 % (75 %) of supercooled clouds are precipitating at cloud base and that 75 % (50 %) are precipitating to the surface. Such high prevalence is reconciled with lesser spaceborne estimates by considering radar sensitivity. Results provide a strong observational constraint for polar cloud processes in large-scale models.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Alexei Korolev, Ivan Heckman, Mengistu Wolde, Andrew S. Ackerman, Ann M. Fridlind, Luis A. Ladino, R. Paul Lawson, Jason Milbrandt, and Earle Williams
Atmos. Chem. Phys., 20, 1391–1429, https://doi.org/10.5194/acp-20-1391-2020, https://doi.org/10.5194/acp-20-1391-2020, 2020
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This study attempts identification of mechanisms of secondary ice production (SIP) based on the observation of small faceted ice crystals. It was found that in both mesoscale convective systems and frontal clouds, SIP was observed right above the melting layer and extended to the higher altitudes with colder temperatures. A principal conclusion of this work is that the freezing drop shattering mechanism is plausibly accounting for the measured ice concentrations in the observed condition.
Ann M. Fridlind, Marcus van Lier-Walqui, Scott Collis, Scott E. Giangrande, Robert C. Jackson, Xiaowen Li, Toshihisa Matsui, Richard Orville, Mark H. Picel, Daniel Rosenfeld, Alexander Ryzhkov, Richard Weitz, and Pengfei Zhang
Atmos. Meas. Tech., 12, 2979–3000, https://doi.org/10.5194/amt-12-2979-2019, https://doi.org/10.5194/amt-12-2979-2019, 2019
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Weather radars are offering improved capabilities to investigate storm physics, which remain poorly understood. We investigate enhanced use of such data near Houston, Texas, where pollution sources often provide a convenient contrast between polluted and clean air. We conclude that Houston is a favorable location to conduct a future field campaign during June through September because isolated storms are common and tend to last an hour, allowing frequent observations of a full life cycle.
Grégory Cesana, Anthony D. Del Genio, Andrew S. Ackerman, Maxwell Kelley, Gregory Elsaesser, Ann M. Fridlind, Ye Cheng, and Mao-Sung Yao
Atmos. Chem. Phys., 19, 2813–2832, https://doi.org/10.5194/acp-19-2813-2019, https://doi.org/10.5194/acp-19-2813-2019, 2019
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The response of low clouds to climate change (i.e., cloud feedbacks) is still pointed out as being the largest source of uncertainty in climate models. Here we use CALIPSO observations to discriminate climate models that reproduce observed interannual change of cloud fraction with SST forcings, referred to as a present-day cloud feedback. Modeling moist processes in the planetary boundary layer is crucial to produce large stratocumulus decks and realistic present-day cloud feedbacks.
Katia Lamer, Ann M. Fridlind, Andrew S. Ackerman, Pavlos Kollias, Eugene E. Clothiaux, and Maxwell Kelley
Geosci. Model Dev., 11, 4195–4214, https://doi.org/10.5194/gmd-11-4195-2018, https://doi.org/10.5194/gmd-11-4195-2018, 2018
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Weather and climate predictions of cloud, rain, and snow occurrence remain uncertain, in part because guidance from observation is incomplete. We present a tool that transforms predictions into observations from ground-based remote sensors. Liquid water and ice occurrence errors associated with the transformation are below 8 %, with ~ 3 % uncertainty. This (GO)2-SIM forward-simulator tool enables better evaluation of cloud, rain, and snow occurrence predictions using available observations.
Xiaoli Zhou, Andrew S. Ackerman, Ann M. Fridlind, Robert Wood, and Pavlos Kollias
Atmos. Chem. Phys., 17, 12725–12742, https://doi.org/10.5194/acp-17-12725-2017, https://doi.org/10.5194/acp-17-12725-2017, 2017
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Shallow maritime clouds make a well-known transition from stratocumulus to trade cumulus with flow from the subtropics equatorward. Three-day large-eddy simulations that investigate the potential influence of overlying African biomass burning plumes during that transition indicate that cloud-related impacts are likely substantially cooling to negligible at the top of the atmosphere, with magnitude sensitive to background and perturbation aerosol and cloud properties.
Ann M. Fridlind, Xiaowen Li, Di Wu, Marcus van Lier-Walqui, Andrew S. Ackerman, Wei-Kuo Tao, Greg M. McFarquhar, Wei Wu, Xiquan Dong, Jingyu Wang, Alexander Ryzhkov, Pengfei Zhang, Michael R. Poellot, Andrea Neumann, and Jason M. Tomlinson
Atmos. Chem. Phys., 17, 5947–5972, https://doi.org/10.5194/acp-17-5947-2017, https://doi.org/10.5194/acp-17-5947-2017, 2017
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Understanding observed storm microphysics via computer simulation requires measurements of aerosol on which most hydrometeors form. We prepare aerosol input data for six storms observed over Oklahoma. We demonstrate their use in simulations of a case with widespread ice outflow well sampled by aircraft. Simulations predict too few ice crystals that are too large. We speculate that microphysics found in tropical storms occurred here, likely associated with poorly understood ice multiplication.
A. M. Fridlind, A. S. Ackerman, A. Grandin, F. Dezitter, M. Weber, J. W. Strapp, A. V. Korolev, and C. R. Williams
Atmos. Chem. Phys., 15, 11713–11728, https://doi.org/10.5194/acp-15-11713-2015, https://doi.org/10.5194/acp-15-11713-2015, 2015
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Airbus measurements at elevations circa 11 km within large storm systems near Darwin and Santiago indicate ice mass distributed over area-equivalent diameters of 100-500 µm. Profiler-observed radar reflectivity and mean Doppler velocity under similar conditions are found to be consistent with measurements and with 1D simulations of steady-state stratiform rain columns initialized with observed ice size distributions. Results motivate investigation of ice formation pathways in Part II.
A. S. Ackerman, A. M. Fridlind, A. Grandin, F. Dezitter, M. Weber, J. W. Strapp, and A. V. Korolev
Atmos. Chem. Phys., 15, 11729–11751, https://doi.org/10.5194/acp-15-11729-2015, https://doi.org/10.5194/acp-15-11729-2015, 2015
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An updraft parcel model with size-resolved microphysics is used to investigate microphysical pathways leading to ice water content > 2 g m-3 with mass median area-equivalent diameter of 200-300 micron reported at ~11 km in tropical deep convection. Parcel simulations require substantial source of small crystals at temperatures > ~-10 deg C growing by vapor deposition. Warm rain in weaker updrafts surprisingly leads to greater ice mass owing to reduced competition for available water vapor.
Florian Tornow, Ann Fridlind, George Tselioudis, Brian Cairns, Andrew Ackerman, Seethala Chellappan, David Painemal, Paquita Zuidema, Christiane Voigt, Simon Kirschler, and Armin Sorooshian
EGUsphere, https://doi.org/10.5194/egusphere-2024-3462, https://doi.org/10.5194/egusphere-2024-3462, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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The recent NASA campaign ACTIVATE (Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment) performed 71 tandem flights in mid-latitude marine cold-air outbreaks off the US Eastern seaboard. We provide meteorological and cloud transition stage context, allowing us to identify days that are most suitable for Lagrangian modeling and analysis. Surveyed cloud properties show signatures of cloud microphysical processes, such as cloud-top entrainment and secondary ice formation.
Jeonggyu Kim, Sungmin Park, Greg M. McFarquhar, Anthony J. Baran, Joo Wan Cha, Kyoungmi Lee, Seoung Soo Lee, Chang Hoon Jung, Kyo-Sun Sunny Lim, and Junshik Um
Atmos. Chem. Phys., 24, 12707–12726, https://doi.org/10.5194/acp-24-12707-2024, https://doi.org/10.5194/acp-24-12707-2024, 2024
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We developed idealized models to represent the shapes of ice particles found in deep convective clouds and calculated their single-scattering properties. By comparing these results with in situ measurements, we discovered that a mixture of shape models matches in situ measurements more closely than single-form models or aggregate models. This finding has important implications for enhancing the simulation of single-scattering properties of ice crystals in deep convective clouds.
Alexei Korolev, Zhipeng Qu, Jason Milbrandt, Ivan Heckman, Mélissa Cholette, Mengistu Wolde, Cuong Nguyen, Greg M. McFarquhar, Paul Lawson, and Ann M. Fridlind
Atmos. Chem. Phys., 24, 11849–11881, https://doi.org/10.5194/acp-24-11849-2024, https://doi.org/10.5194/acp-24-11849-2024, 2024
Short summary
Short summary
The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCSs) when a large number of small ice particles with typical sizes of a few hundred micrometers is found at high altitudes. It was found that secondary ice production in the vicinity of the melting layer plays a key role in the formation and maintenance of HIWC. This study presents a conceptual model of the formation of HIWC in tropical MCSs based on in situ observations and numerical simulation.
Abigail S. Williams, Jeramy L. Dedrick, Lynn M. Russell, Florian Tornow, Israel Silber, Ann M. Fridlind, Benjamin Swanson, Paul J. DeMott, Paul Zieger, and Radovan Krejci
Atmos. Chem. Phys., 24, 11791–11805, https://doi.org/10.5194/acp-24-11791-2024, https://doi.org/10.5194/acp-24-11791-2024, 2024
Short summary
Short summary
The measured aerosol size distribution modes reveal distinct properties characteristic of cold-air outbreaks in the Norwegian Arctic. We find higher sea spray number concentrations, smaller Hoppel minima, lower effective supersaturations, and accumulation-mode particle scavenging during cold-air outbreaks. These results advance our understanding of cold-air outbreak aerosol–cloud interactions in order to improve their accurate representation in models.
Toshi Matsui, Daniel Hernandez-Deckers, Scott E. Giangrande, Thiago S. Biscaro, Ann Fridlind, and Scott Braun
Atmos. Chem. Phys., 24, 10793–10814, https://doi.org/10.5194/acp-24-10793-2024, https://doi.org/10.5194/acp-24-10793-2024, 2024
Short summary
Short summary
Using computer simulations and real measurements, we discovered that storms over the Amazon were narrower but more intense during the dry periods, producing heavier rain and more ice particles in the clouds. Our research showed that cumulus bubbles played a key role in creating these intense storms. This study can improve the representation of the effect of continental and ocean environments on tropical regions' rainfall patterns in simulations.
Benjamin W. Clouser, Laszlo C. Sarkozy, Clare E. Singer, Carly C. KleinStern, Adrien Desmoulin, Dylan Gaeta, Sergey Khaykin, Stephen Gabbard, Stephen Shertz, and Elisabeth J. Moyer
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-98, https://doi.org/10.5194/amt-2024-98, 2024
Preprint under review for AMT
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The water molecule comes in several different varieties, which are nearly indistinguishable in daily life. However, slight differences between the water molecule types can be exploited to achieve better scientific understanding of parts of Earth's atmosphere. In this work we describe the design, construction, and operation of an instrument meant to measure these molecules aboard research aircraft up to altitudes of 20 kilometers.
McKenna Stanford, Ann Fridlind, Andrew Ackerman, Bastiaan van Diedenhoven, Qian Xiao, Jian Wang, Toshihisa Matsui, Daniel Hernandez-Deckers, and Paul Lawson
EGUsphere, https://doi.org/10.5194/egusphere-2024-2413, https://doi.org/10.5194/egusphere-2024-2413, 2024
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The evolution of cloud droplets, from the point they are activated by atmospheric aerosol to the formation of precipitation, is an important process relevant to understanding cloud-climate feedbacks. This study demonstrates a benchmark framework for using novel airborne measurements and retrievals to constrain high-resolution simulations of moderately deep cumulus clouds and pathways for scaling results to large-scale models and space-based observational platforms.
Kerry Meyer, Steven Platnick, G. Thomas Arnold, Nandana Amarasinghe, Daniel Miller, Jennifer Small-Griswold, Mikael Witte, Brian Cairns, Siddhant Gupta, Greg McFarquhar, and Joseph O'Brien
EGUsphere, https://doi.org/10.5194/egusphere-2024-2021, https://doi.org/10.5194/egusphere-2024-2021, 2024
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Satellite remote sensing retrievals of cloud droplet size are used to understand clouds and their interactions with aerosols and radiation but require many simplifying assumptions. Evaluation of these retrievals typically is done by comparing against direct measurements of droplets from airborne cloud probes. This paper details an evaluation of proxy airborne remote sensing droplet size retrievals against several cloud probes and explores the impact of key assumptions on retrieval agreement.
Johannes Mülmenstädt, Edward Gryspeerdt, Sudhakar Dipu, Johannes Quaas, Andrew S. Ackerman, Ann M. Fridlind, Florian Tornow, Susanne E. Bauer, Andrew Gettelman, Yi Ming, Youtong Zheng, Po-Lun Ma, Hailong Wang, Kai Zhang, Matthew W. Christensen, Adam C. Varble, L. Ruby Leung, Xiaohong Liu, David Neubauer, Daniel G. Partridge, Philip Stier, and Toshihiko Takemura
Atmos. Chem. Phys., 24, 7331–7345, https://doi.org/10.5194/acp-24-7331-2024, https://doi.org/10.5194/acp-24-7331-2024, 2024
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Human activities release copious amounts of small particles called aerosols into the atmosphere. These particles change how much sunlight clouds reflect to space, an important human perturbation of the climate, whose magnitude is highly uncertain. We found that the latest climate models show a negative correlation but a positive causal relationship between aerosols and cloud water. This means we need to be very careful when we interpret observational studies that can only see correlation.
Michie Vianca De Vera, Larry Di Girolamo, Guangyu Zhao, Robert M. Rauber, Stephen W. Nesbitt, and Greg M. McFarquhar
Atmos. Chem. Phys., 24, 5603–5623, https://doi.org/10.5194/acp-24-5603-2024, https://doi.org/10.5194/acp-24-5603-2024, 2024
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Tropical oceanic low clouds remain a dominant source of uncertainty in cloud feedback in climate models due to their macrophysical properties (fraction, size, height, shape, distribution) being misrepresented. High-resolution satellite imagery over the Philippine oceans is used here to characterize cumulus macrophysical properties and their relationship to meteorological variables. Such information can act as a benchmark for cloud models and can improve low-cloud generation in climate models.
Zihao Yuan, Guangliang Fu, Bastiaan van Diedenhoven, Hai Xiang Lin, Jan Willem Erisman, and Otto P. Hasekamp
Atmos. Meas. Tech., 17, 2595–2610, https://doi.org/10.5194/amt-17-2595-2024, https://doi.org/10.5194/amt-17-2595-2024, 2024
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Currently, aerosol properties from spaceborne multi-angle polarimeter (MAP) instruments can only be retrieved in cloud-free areas or in areas where an aerosol layer is located above a cloud. Therefore, it is important to be able to identify cloud-free pixels for which an aerosol retrieval algorithm can provide meaningful output. The developed neural network cloud screening demonstrates that cloud masking for MAP aerosol retrieval can be based on the MAP measurements themselves.
Johannes Mülmenstädt, Andrew S. Ackerman, Ann M. Fridlind, Meng Huang, Po-Lun Ma, Naser Mahfouz, Susanne E. Bauer, Susannah M. Burrows, Matthew W. Christensen, Sudhakar Dipu, Andrew Gettelman, L. Ruby Leung, Florian Tornow, Johannes Quaas, Adam C. Varble, Hailong Wang, Kai Zhang, and Youtong Zheng
EGUsphere, https://doi.org/10.5194/egusphere-2024-778, https://doi.org/10.5194/egusphere-2024-778, 2024
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Stratocumulus clouds play a large role in Earth's climate by reflecting incoming solar energy back to space. Turbulence at stratocumulus cloud top mixes in drier, warmer air, which can lead to a reduction in cloud. This process is challenging for coarse-resolution global models to represent. We show that global models nevertheless agree well with our process understanding. Global models also think the process is less important for the climate than other lines of evidence had led us to conclude.
Kamil Mroz, Alessandro Battaglia, and Ann M. Fridlind
Atmos. Meas. Tech., 17, 1577–1597, https://doi.org/10.5194/amt-17-1577-2024, https://doi.org/10.5194/amt-17-1577-2024, 2024
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In this study, we examine the extent to which radar measurements from space can inform us about the properties of clouds and precipitation. Surprisingly, our analysis showed that the amount of ice turning into rain was lower than expected in the current product. To improve on this, we came up with a new way to extract information about the size and concentration of particles from radar data. As long as we use this method in the right conditions, we can even estimate how dense the ice is.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Paul Konopka, Christian Rolf, Marc von Hobe, Sergey M. Khaykin, Benjamin Clouser, Elisabeth Moyer, Fabrizio Ravegnani, Francesco D'Amato, Silvia Viciani, Nicole Spelten, Armin Afchine, Martina Krämer, Fred Stroh, and Felix Ploeger
Atmos. Chem. Phys., 23, 12935–12947, https://doi.org/10.5194/acp-23-12935-2023, https://doi.org/10.5194/acp-23-12935-2023, 2023
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We studied water vapor in a critical region of the atmosphere, the Asian summer monsoon anticyclone, using rare in situ observations. Our study shows that extremely high water vapor values observed in the stratosphere within the Asian monsoon anticyclone still undergo significant freeze-drying and that water vapor concentrations set by the Lagrangian dry point are a better proxy for the stratospheric water vapor budget than rare observations of enhanced water mixing ratios.
Qian Xiao, Jiaoshi Zhang, Yang Wang, Luke D. Ziemba, Ewan Crosbie, Edward L. Winstead, Claire E. Robinson, Joshua P. DiGangi, Glenn S. Diskin, Jeffrey S. Reid, K. Sebastian Schmidt, Armin Sorooshian, Miguel Ricardo A. Hilario, Sarah Woods, Paul Lawson, Snorre A. Stamnes, and Jian Wang
Atmos. Chem. Phys., 23, 9853–9871, https://doi.org/10.5194/acp-23-9853-2023, https://doi.org/10.5194/acp-23-9853-2023, 2023
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Using recent airborne measurements, we show that the influences of anthropogenic emissions, transport, convective clouds, and meteorology lead to new particle formation (NPF) under a variety of conditions and at different altitudes in tropical marine environments. NPF is enhanced by fresh urban emissions in convective outflow but is suppressed in air masses influenced by aged urban emissions where reactive precursors are mostly consumed while particle surface area remains relatively high.
McKenna W. Stanford, Ann M. Fridlind, Israel Silber, Andrew S. Ackerman, Greg Cesana, Johannes Mülmenstädt, Alain Protat, Simon Alexander, and Adrian McDonald
Atmos. Chem. Phys., 23, 9037–9069, https://doi.org/10.5194/acp-23-9037-2023, https://doi.org/10.5194/acp-23-9037-2023, 2023
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Clouds play an important role in the Earth’s climate system as they modulate the amount of radiation that either reaches the surface or is reflected back to space. This study demonstrates an approach to robustly evaluate surface-based observations against a large-scale model. We find that the large-scale model precipitates too infrequently relative to observations, contrary to literature documentation suggesting otherwise based on satellite measurements.
Rose Marie Miller, Robert M. Rauber, Larry Di Girolamo, Matthew Rilloraza, Dongwei Fu, Greg M. McFarquhar, Stephen W. Nesbitt, Luke D. Ziemba, Sarah Woods, and Kenneth Lee Thornhill
Atmos. Chem. Phys., 23, 8959–8977, https://doi.org/10.5194/acp-23-8959-2023, https://doi.org/10.5194/acp-23-8959-2023, 2023
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The influence of human-produced aerosols on clouds remains one of the uncertainties in radiative forcing of Earth’s climate. Measurements of aerosol chemistry from sources around the Philippines illustrate the linkage between aerosol chemical composition and cloud droplet characteristics. Differences in aerosol chemical composition in the marine layer from biomass burning, industrial, ship-produced, and marine aerosols are shown to impact cloud microphysical structure just above cloud base.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Kara D. Lamb, Jerry Y. Harrington, Benjamin W. Clouser, Elisabeth J. Moyer, Laszlo Sarkozy, Volker Ebert, Ottmar Möhler, and Harald Saathoff
Atmos. Chem. Phys., 23, 6043–6064, https://doi.org/10.5194/acp-23-6043-2023, https://doi.org/10.5194/acp-23-6043-2023, 2023
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This study investigates how ice grows directly from vapor in cirrus clouds by comparing observations of populations of ice crystals growing in a cloud chamber against models developed in the context of single-crystal laboratory studies. We demonstrate that previous discrepancies between different experimental measurements do not necessarily point to different physical interpretations but are rather due to assumptions that were made in terms of how experiments were modeled in previous studies.
Seoung Soo Lee, Chang-Hoon Jung, Young Jun Yoon, Junshik Um, Youtong Zheng, Jianping Guo, Manguttathil G. Manoj, and Sang-Keun Song
EGUsphere, https://doi.org/10.5194/egusphere-2023-862, https://doi.org/10.5194/egusphere-2023-862, 2023
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This study is motivated by the fact that there are no general factors that represent the overall properties of mixed-phase clouds. The absence of these factors contributes to the high uncertainty in the prediction of climate change. Hence, this study finds a general factor that explains differences in the properties of different mixed-phase clouds, using a modeling tool. This factor is useful to develop a general way of using climate models to better predict climate change.
Ruhi S. Humphries, Melita D. Keywood, Jason P. Ward, James Harnwell, Simon P. Alexander, Andrew R. Klekociuk, Keiichiro Hara, Ian M. McRobert, Alain Protat, Joel Alroe, Luke T. Cravigan, Branka Miljevic, Zoran D. Ristovski, Robyn Schofield, Stephen R. Wilson, Connor J. Flynn, Gourihar R. Kulkarni, Gerald G. Mace, Greg M. McFarquhar, Scott D. Chambers, Alastair G. Williams, and Alan D. Griffiths
Atmos. Chem. Phys., 23, 3749–3777, https://doi.org/10.5194/acp-23-3749-2023, https://doi.org/10.5194/acp-23-3749-2023, 2023
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Observations of aerosols in pristine regions are rare but are vital to constraining the natural baseline from which climate simulations are calculated. Here we present recent seasonal observations of aerosols from the Southern Ocean and contrast them with measurements from Antarctica, Australia and regionally relevant voyages. Strong seasonal cycles persist, but striking differences occur at different latitudes. This study highlights the need for more long-term observations in remote regions.
Andrew M. Sayer, Luca Lelli, Brian Cairns, Bastiaan van Diedenhoven, Amir Ibrahim, Kirk D. Knobelspiesse, Sergey Korkin, and P. Jeremy Werdell
Atmos. Meas. Tech., 16, 969–996, https://doi.org/10.5194/amt-16-969-2023, https://doi.org/10.5194/amt-16-969-2023, 2023
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This paper presents a method to estimate the height of the top of clouds above Earth's surface using satellite measurements. It is based on light absorption by oxygen in Earth's atmosphere, which darkens the signal that a satellite will see at certain wavelengths of light. Clouds "shield" the satellite from some of this darkening, dependent on cloud height (and other factors), because clouds scatter light at these wavelengths. The method will be applied to the future NASA PACE mission.
Seoung Soo Lee, Junshik Um, Won Jun Choi, Kyung-Ja Ha, Chang Hoon Jung, Jianping Guo, and Youtong Zheng
Atmos. Chem. Phys., 23, 273–286, https://doi.org/10.5194/acp-23-273-2023, https://doi.org/10.5194/acp-23-273-2023, 2023
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This paper elaborates on process-level mechanisms regarding how the interception of radiation by aerosols interacts with the surface heat fluxes and atmospheric instability in warm cumulus clouds. This paper elucidates how these mechanisms vary with the location or altitude of an aerosol layer. This elucidation indicates that the location of aerosol layers should be taken into account for parameterizations of aerosol–cloud interactions.
Bastiaan van Diedenhoven, Otto P. Hasekamp, Brian Cairns, Gregory L. Schuster, Snorre Stamnes, Michael Shook, and Luke Ziemba
Atmos. Meas. Tech., 15, 7411–7434, https://doi.org/10.5194/amt-15-7411-2022, https://doi.org/10.5194/amt-15-7411-2022, 2022
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The strong variability in the chemistry of atmospheric particulate matter affects the amount of water aerosols absorb and their effect on climate. We present a remote sensing method to determine the amount of water in particulate matter. Its application to airborne instruments indicates that the observed aerosols have rather low water contents and low fractions of soluble particles. Future satellites will be able to yield global aerosol water uptake data.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Ian Chang, Lan Gao, Feng Xu, and Jens Redemann
Atmos. Chem. Phys., 22, 12923–12943, https://doi.org/10.5194/acp-22-12923-2022, https://doi.org/10.5194/acp-22-12923-2022, 2022
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The ability of NASA’s Terra and Aqua satellites to retrieve cloud properties and estimate the changes in cloud properties due to aerosol–cloud interactions (ACI) was examined. There was good agreement between satellite retrievals and in situ measurements over the southeast Atlantic Ocean. This suggests that, combined with information on aerosol properties, satellite retrievals of cloud properties can be used to study ACI over larger domains and longer timescales in the absence of in situ data.
Frederic Tridon, Israel Silber, Alessandro Battaglia, Stefan Kneifel, Ann Fridlind, Petros Kalogeras, and Ranvir Dhillon
Atmos. Chem. Phys., 22, 12467–12491, https://doi.org/10.5194/acp-22-12467-2022, https://doi.org/10.5194/acp-22-12467-2022, 2022
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The role of ice precipitation in the Earth water budget is not well known because ice particles are complex, and their formation involves intricate processes. Riming of ice crystals by supercooled water droplets is an efficient process, but little is known about its importance at high latitudes. In this work, by exploiting the deployment of an unprecedented number of remote sensing systems in Antarctica, we find that riming occurs at much lower temperatures compared with the mid-latitudes.
Zhipeng Qu, Alexei Korolev, Jason A. Milbrandt, Ivan Heckman, Yongjie Huang, Greg M. McFarquhar, Hugh Morrison, Mengistu Wolde, and Cuong Nguyen
Atmos. Chem. Phys., 22, 12287–12310, https://doi.org/10.5194/acp-22-12287-2022, https://doi.org/10.5194/acp-22-12287-2022, 2022
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Secondary ice production (SIP) is an important physical phenomenon that results in an increase in the cloud ice particle concentration and can have a significant impact on the evolution of clouds. Here, idealized simulations of a tropical convective system were conducted. Agreement between the simulations and observations highlights the impacts of SIP on the maintenance of tropical convection in nature and the importance of including the modelling of SIP in numerical weather prediction models.
Michael S. Diamond, Pablo E. Saide, Paquita Zuidema, Andrew S. Ackerman, Sarah J. Doherty, Ann M. Fridlind, Hamish Gordon, Calvin Howes, Jan Kazil, Takanobu Yamaguchi, Jianhao Zhang, Graham Feingold, and Robert Wood
Atmos. Chem. Phys., 22, 12113–12151, https://doi.org/10.5194/acp-22-12113-2022, https://doi.org/10.5194/acp-22-12113-2022, 2022
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Smoke from southern Africa blankets the southeast Atlantic from June-October, overlying a major transition region between overcast and scattered clouds. The smoke affects Earth's radiation budget by absorbing sunlight and changing cloud properties. We investigate these effects in regional climate and large eddy simulation models based on international field campaigns. We find that large-scale circulation changes more strongly affect cloud transitions than smoke microphysical effects in our case.
Clare E. Singer, Benjamin W. Clouser, Sergey M. Khaykin, Martina Krämer, Francesco Cairo, Thomas Peter, Alexey Lykov, Christian Rolf, Nicole Spelten, Armin Afchine, Simone Brunamonti, and Elisabeth J. Moyer
Atmos. Meas. Tech., 15, 4767–4783, https://doi.org/10.5194/amt-15-4767-2022, https://doi.org/10.5194/amt-15-4767-2022, 2022
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In situ measurements of water vapor in the upper troposphere are necessary to study cloud formation and hydration of the stratosphere but challenging due to cold–dry conditions. We compare measurements from three water vapor instruments from the StratoClim campaign in 2017. In clear sky (clouds), point-by-point differences were <1.5±8 % (<1±8 %). This excellent agreement allows detection of fine-scale structures required to understand the impact of convection on stratospheric water vapor.
Seoung Soo Lee, Jinho Choi, Goun Kim, Kyung-Ja Ha, Kyong-Hwan Seo, Chang Hoon Jung, Junshik Um, Youtong Zheng, Jianping Guo, Sang-Keun Song, Yun Gon Lee, and Nobuyuki Utsumi
Atmos. Chem. Phys., 22, 9059–9081, https://doi.org/10.5194/acp-22-9059-2022, https://doi.org/10.5194/acp-22-9059-2022, 2022
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This study investigates how aerosols affect clouds and precipitation and how the aerosol effects vary with varying types of clouds that are characterized by cloud depth in two metropolitan areas in East Asia. As cloud depth increases, the enhancement of precipitation amount transitions to no changes in precipitation amount with increasing aerosol concentrations. This indicates that cloud depth needs to be considered for a comprehensive understanding of aerosol-cloud interactions.
Dongwei Fu, Larry Di Girolamo, Robert M. Rauber, Greg M. McFarquhar, Stephen W. Nesbitt, Jesse Loveridge, Yulan Hong, Bastiaan van Diedenhoven, Brian Cairns, Mikhail D. Alexandrov, Paul Lawson, Sarah Woods, Simone Tanelli, Sebastian Schmidt, Chris Hostetler, and Amy Jo Scarino
Atmos. Chem. Phys., 22, 8259–8285, https://doi.org/10.5194/acp-22-8259-2022, https://doi.org/10.5194/acp-22-8259-2022, 2022
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Satellite-retrieved cloud microphysics are widely used in climate research because of their central role in water and energy cycles. Here, we provide the first detailed investigation of retrieved cloud drop sizes from in situ and various satellite and airborne remote sensing techniques applied to real cumulus cloud fields. We conclude that the most widely used passive remote sensing method employed in climate research produces high biases of 6–8 µm (60 %–80 %) caused by 3-D radiative effects.
Matthew S. Norgren, John Wood, K. Sebastian Schmidt, Bastiaan van Diedenhoven, Snorre A. Stamnes, Luke D. Ziemba, Ewan C. Crosbie, Michael A. Shook, A. Scott Kittelman, Samuel E. LeBlanc, Stephen Broccardo, Steffen Freitag, and Jeffrey S. Reid
Atmos. Meas. Tech., 15, 1373–1394, https://doi.org/10.5194/amt-15-1373-2022, https://doi.org/10.5194/amt-15-1373-2022, 2022
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A new spectral instrument (SPN-S), with the ability to partition solar radiation into direct and diffuse components, is used in airborne settings to study the optical properties of aerosols and cirrus. It is a low-cost and mechanically simple system but has higher measurement uncertainty than existing standards. This challenge is overcome by utilizing the unique measurement capabilities to develop new retrieval techniques. Validation is done with data from two NASA airborne research campaigns.
Sergey M. Khaykin, Elizabeth Moyer, Martina Krämer, Benjamin Clouser, Silvia Bucci, Bernard Legras, Alexey Lykov, Armin Afchine, Francesco Cairo, Ivan Formanyuk, Valentin Mitev, Renaud Matthey, Christian Rolf, Clare E. Singer, Nicole Spelten, Vasiliy Volkov, Vladimir Yushkov, and Fred Stroh
Atmos. Chem. Phys., 22, 3169–3189, https://doi.org/10.5194/acp-22-3169-2022, https://doi.org/10.5194/acp-22-3169-2022, 2022
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The Asian monsoon anticyclone is the key contributor to the global annual maximum in lower stratospheric water vapour. We investigate the impact of deep convection on the lower stratospheric water using a unique set of observations aboard the high-altitude M55-Geophysica aircraft deployed in Nepal in summer 2017 within the EU StratoClim project. We find that convective plumes of wet air can persist within the Asian anticyclone for weeks, thereby enhancing the occurrence of high-level clouds.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, Michael R. Poellot, David J. Delene, Rose M. Miller, and Jennifer D. Small Griswold
Atmos. Chem. Phys., 22, 2769–2793, https://doi.org/10.5194/acp-22-2769-2022, https://doi.org/10.5194/acp-22-2769-2022, 2022
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This study evaluates the impact of biomass burning aerosols on precipitation in marine stratocumulus clouds using observations from the NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign over the Southeast Atlantic. Instances of contact and separation between aerosol and cloud layers show polluted clouds have a lower precipitation rate and a lower precipitation susceptibility. This information will help improve cloud representation in Earth system models.
Yongjie Huang, Wei Wu, Greg M. McFarquhar, Ming Xue, Hugh Morrison, Jason Milbrandt, Alexei V. Korolev, Yachao Hu, Zhipeng Qu, Mengistu Wolde, Cuong Nguyen, Alfons Schwarzenboeck, and Ivan Heckman
Atmos. Chem. Phys., 22, 2365–2384, https://doi.org/10.5194/acp-22-2365-2022, https://doi.org/10.5194/acp-22-2365-2022, 2022
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Numerous small ice crystals in tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. Previous numerical simulations failed to reproduce this phenomenon and hypothesized that key microphysical processes are still lacking in current models to realistically simulate the phenomenon. This study uses numerical experiments to confirm the dominant role of secondary ice production in the formation of these large numbers of small ice crystals.
Israel Silber, Robert C. Jackson, Ann M. Fridlind, Andrew S. Ackerman, Scott Collis, Johannes Verlinde, and Jiachen Ding
Geosci. Model Dev., 15, 901–927, https://doi.org/10.5194/gmd-15-901-2022, https://doi.org/10.5194/gmd-15-901-2022, 2022
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The Earth Model Column Collaboratory (EMC2) is an open-source ground-based (and air- or space-borne) lidar and radar simulator and subcolumn generator designed for large-scale models, in particular climate models, applicable also for high-resolution models. EMC2 emulates measurements while remaining faithful to large-scale models' physical assumptions implemented in their cloud or radiation schemes. We demonstrate the use of EMC2 to compare AWARE measurements with the NASA GISS ModelE3 and LES.
Daniel Hernandez-Deckers, Toshihisa Matsui, and Ann M. Fridlind
Atmos. Chem. Phys., 22, 711–724, https://doi.org/10.5194/acp-22-711-2022, https://doi.org/10.5194/acp-22-711-2022, 2022
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We investigate how the concentration of aerosols (small particles that serve as seeds for cloud droplets) affect the dynamics of simulated clouds using two different frameworks, i.e., the traditional selection of cloudy rising grid points and tracking small-scale coherent rising features (cumulus thermals). By doing so, we find that these cumulus thermals reveal useful information about the coupling between internal cloud circulations and cloud droplet and raindrop formation.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Seoung Soo Lee, Kyung-Ja Ha, Manguttathil Gopalakrishnan Manoj, Mohammad Kamruzzaman, Hyungjun Kim, Nobuyuki Utsumi, Youtong Zheng, Byung-Gon Kim, Chang Hoon Jung, Junshik Um, Jianping Guo, Kyoung Ock Choi, and Go-Un Kim
Atmos. Chem. Phys., 21, 16843–16868, https://doi.org/10.5194/acp-21-16843-2021, https://doi.org/10.5194/acp-21-16843-2021, 2021
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Using a modeling framework, a midlatitude stratocumulus cloud system is simulated. It is found that cloud mass in the system becomes very low due to interactions between ice and liquid particles compared to that in the absence of ice particles. It is also found that interactions between cloud mass and aerosols lead to a reduction in cloud mass in the system, and this is contrary to an aerosol-induced increase in cloud mass in the absence of ice particles.
Rose M. Miller, Greg M. McFarquhar, Robert M. Rauber, Joseph R. O'Brien, Siddhant Gupta, Michal Segal-Rozenhaimer, Amie N. Dobracki, Arthur J. Sedlacek, Sharon P. Burton, Steven G. Howell, Steffen Freitag, and Caroline Dang
Atmos. Chem. Phys., 21, 14815–14831, https://doi.org/10.5194/acp-21-14815-2021, https://doi.org/10.5194/acp-21-14815-2021, 2021
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A large stratocumulus cloud deck resides off the west coast of central Africa. Biomass burning in Africa produces a large plume of aerosol that is carried by the wind over this stratocumulus cloud deck. This paper shows that particles with sizes from 0.01 to 1 mm reside within this plume. Past studies have shown that biomass burning produces such particles, but this is the first study to show that they can be transported westward, over long distances, to the Atlantic stratocumulus cloud deck.
Ruhi S. Humphries, Melita D. Keywood, Sean Gribben, Ian M. McRobert, Jason P. Ward, Paul Selleck, Sally Taylor, James Harnwell, Connor Flynn, Gourihar R. Kulkarni, Gerald G. Mace, Alain Protat, Simon P. Alexander, and Greg McFarquhar
Atmos. Chem. Phys., 21, 12757–12782, https://doi.org/10.5194/acp-21-12757-2021, https://doi.org/10.5194/acp-21-12757-2021, 2021
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The Southern Ocean region is one of the most pristine in the world and serves as an important proxy for the pre-industrial atmosphere. Improving our understanding of the natural processes in this region is likely to result in the largest reductions in the uncertainty of climate and earth system models. In this paper we present a statistical summary of the latitudinal gradient of aerosol and cloud condensation nuclei concentrations obtained from five voyages spanning the Southern Ocean.
Youssef Wehbe, Sarah A. Tessendorf, Courtney Weeks, Roelof Bruintjes, Lulin Xue, Roy Rasmussen, Paul Lawson, Sarah Woods, and Marouane Temimi
Atmos. Chem. Phys., 21, 12543–12560, https://doi.org/10.5194/acp-21-12543-2021, https://doi.org/10.5194/acp-21-12543-2021, 2021
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The role of dust aerosols as ice-nucleating particles is well established in the literature, whereas their role as cloud condensation nuclei is less understood, particularly in polluted desert environments. We analyze coincident aerosol size distributions and cloud particle imagery collected over the UAE with a research aircraft. Despite the presence of ultra-giant aerosol sizes associated with dust, an active collision–coalescence process is not observed within the limited depths of warm cloud.
Florian Tornow, Andrew S. Ackerman, and Ann M. Fridlind
Atmos. Chem. Phys., 21, 12049–12067, https://doi.org/10.5194/acp-21-12049-2021, https://doi.org/10.5194/acp-21-12049-2021, 2021
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Cold air outbreaks affect the local energy budget by forming bright boundary layer clouds that, once it rains, evolve into dimmer, broken cloud fields that are depleted of condensation nuclei – an evolution consistent with closed-to-open cell transitions. We find that cloud ice accelerates this evolution, primarily via riming prior to rain onset, which (1) reduces liquid water, (2) reduces condensation nuclei, and (3) leads to early precipitation cooling and moistening below cloud.
Yongjie Huang, Wei Wu, Greg M. McFarquhar, Xuguang Wang, Hugh Morrison, Alexander Ryzhkov, Yachao Hu, Mengistu Wolde, Cuong Nguyen, Alfons Schwarzenboeck, Jason Milbrandt, Alexei V. Korolev, and Ivan Heckman
Atmos. Chem. Phys., 21, 6919–6944, https://doi.org/10.5194/acp-21-6919-2021, https://doi.org/10.5194/acp-21-6919-2021, 2021
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Numerous small ice crystals in the tropical convective storms are difficult to detect and could be potentially hazardous for commercial aircraft. This study evaluated the numerical models against the airborne observations and investigated the potential cloud processes that could lead to the production of these large numbers of small ice crystals. It is found that key microphysical processes are still lacking or misrepresented in current numerical models to realistically simulate the phenomenon.
Andrew M. Dzambo, Tristan L'Ecuyer, Kenneth Sinclair, Bastiaan van Diedenhoven, Siddhant Gupta, Greg McFarquhar, Joseph R. O'Brien, Brian Cairns, Andrzej P. Wasilewski, and Mikhail Alexandrov
Atmos. Chem. Phys., 21, 5513–5532, https://doi.org/10.5194/acp-21-5513-2021, https://doi.org/10.5194/acp-21-5513-2021, 2021
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This work highlights a new algorithm using data collected from the 2016–2018 NASA ORACLES field campaign. This algorithm synthesizes cloud and rain measurements to attain estimates of cloud and precipitation properties over the southeast Atlantic Ocean. Estimates produced by this algorithm compare well against in situ estimates. Increased rain fractions and rain rates are found in regions of atmospheric instability. This dataset can be used to explore aerosol–cloud–precipitation interactions.
Siddhant Gupta, Greg M. McFarquhar, Joseph R. O'Brien, David J. Delene, Michael R. Poellot, Amie Dobracki, James R. Podolske, Jens Redemann, Samuel E. LeBlanc, Michal Segal-Rozenhaimer, and Kristina Pistone
Atmos. Chem. Phys., 21, 4615–4635, https://doi.org/10.5194/acp-21-4615-2021, https://doi.org/10.5194/acp-21-4615-2021, 2021
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Observations from the 2016 NASA ObseRvations of Aerosols above CLouds and their intEractionS (ORACLES) field campaign examine how biomass burning aerosols from southern Africa affect marine stratocumulus cloud decks over the Southeast Atlantic. Instances of contact and separation between aerosols and clouds are examined to quantify the impact of aerosol mixing into cloud top on cloud drop numbers and sizes. This information is needed for improving Earth system models and satellite retrievals.
Israel Silber, Ann M. Fridlind, Johannes Verlinde, Andrew S. Ackerman, Grégory V. Cesana, and Daniel A. Knopf
Atmos. Chem. Phys., 21, 3949–3971, https://doi.org/10.5194/acp-21-3949-2021, https://doi.org/10.5194/acp-21-3949-2021, 2021
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Long-term ground-based radar and sounding measurements over Alaska (Antarctica) indicate that more than 85 % (75 %) of supercooled clouds are precipitating at cloud base and that 75 % (50 %) are precipitating to the surface. Such high prevalence is reconciled with lesser spaceborne estimates by considering radar sensitivity. Results provide a strong observational constraint for polar cloud processes in large-scale models.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Martina Krämer, Christian Rolf, Nicole Spelten, Armin Afchine, David Fahey, Eric Jensen, Sergey Khaykin, Thomas Kuhn, Paul Lawson, Alexey Lykov, Laura L. Pan, Martin Riese, Andrew Rollins, Fred Stroh, Troy Thornberry, Veronika Wolf, Sarah Woods, Peter Spichtinger, Johannes Quaas, and Odran Sourdeval
Atmos. Chem. Phys., 20, 12569–12608, https://doi.org/10.5194/acp-20-12569-2020, https://doi.org/10.5194/acp-20-12569-2020, 2020
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To improve the representations of cirrus clouds in climate predictions, extended knowledge of their properties and geographical distribution is required. This study presents extensive airborne in situ and satellite remote sensing climatologies of cirrus and humidity, which serve as a guide to cirrus clouds. Further, exemplary radiative characteristics of cirrus types and also in situ observations of tropical tropopause layer cirrus and humidity in the Asian monsoon anticyclone are shown.
Kirk Knobelspiesse, Henrique M. J. Barbosa, Christine Bradley, Carol Bruegge, Brian Cairns, Gao Chen, Jacek Chowdhary, Anthony Cook, Antonio Di Noia, Bastiaan van Diedenhoven, David J. Diner, Richard Ferrare, Guangliang Fu, Meng Gao, Michael Garay, Johnathan Hair, David Harper, Gerard van Harten, Otto Hasekamp, Mark Helmlinger, Chris Hostetler, Olga Kalashnikova, Andrew Kupchock, Karla Longo De Freitas, Hal Maring, J. Vanderlei Martins, Brent McBride, Matthew McGill, Ken Norlin, Anin Puthukkudy, Brian Rheingans, Jeroen Rietjens, Felix C. Seidel, Arlindo da Silva, Martijn Smit, Snorre Stamnes, Qian Tan, Sebastian Val, Andrzej Wasilewski, Feng Xu, Xiaoguang Xu, and John Yorks
Earth Syst. Sci. Data, 12, 2183–2208, https://doi.org/10.5194/essd-12-2183-2020, https://doi.org/10.5194/essd-12-2183-2020, 2020
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The Aerosol Characterization from Polarimeter and Lidar (ACEPOL) field campaign is a resource for the next generation of spaceborne multi-angle polarimeter (MAP) and lidar missions. Conducted in the fall of 2017 from the Armstrong Flight Research Center in Palmdale, California, four MAP instruments and two lidars were flown on the high-altitude ER-2 aircraft over a variety of scene types and ground assets. Data are freely available to the public and useful for algorithm development and testing.
James A. Franke, Christoph Müller, Joshua Elliott, Alex C. Ruane, Jonas Jägermeyr, Abigail Snyder, Marie Dury, Pete D. Falloon, Christian Folberth, Louis François, Tobias Hank, R. Cesar Izaurralde, Ingrid Jacquemin, Curtis Jones, Michelle Li, Wenfeng Liu, Stefan Olin, Meridel Phillips, Thomas A. M. Pugh, Ashwan Reddy, Karina Williams, Ziwei Wang, Florian Zabel, and Elisabeth J. Moyer
Geosci. Model Dev., 13, 3995–4018, https://doi.org/10.5194/gmd-13-3995-2020, https://doi.org/10.5194/gmd-13-3995-2020, 2020
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Improving our understanding of the impacts of climate change on crop yields will be critical for global food security in the next century. The models often used to study the how climate change may impact agriculture are complex and costly to run. In this work, we describe a set of global crop model emulators (simplified models) developed under the Agricultural Model Intercomparison Project. Crop model emulators make agricultural simulations more accessible to policy or decision makers.
Daniel J. Miller, Michal Segal-Rozenhaimer, Kirk Knobelspiesse, Jens Redemann, Brian Cairns, Mikhail Alexandrov, Bastiaan van Diedenhoven, and Andrzej Wasilewski
Atmos. Meas. Tech., 13, 3447–3470, https://doi.org/10.5194/amt-13-3447-2020, https://doi.org/10.5194/amt-13-3447-2020, 2020
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A neural network (NN) is developed and used to retrieve cloud microphysical properties from multiangular and multispectral polarimetric remote sensing observations. The NN is applied to research scanning polarimeter (RSP) observations obtained during the ORACLES field campaign and compared to other co-located remote sensing retrievals of cloud effective radius and optical thickness. A NN approach can advance more complex iterative search retrieval algorithms by providing a quick initial guess.
James A. Franke, Christoph Müller, Joshua Elliott, Alex C. Ruane, Jonas Jägermeyr, Juraj Balkovic, Philippe Ciais, Marie Dury, Pete D. Falloon, Christian Folberth, Louis François, Tobias Hank, Munir Hoffmann, R. Cesar Izaurralde, Ingrid Jacquemin, Curtis Jones, Nikolay Khabarov, Marian Koch, Michelle Li, Wenfeng Liu, Stefan Olin, Meridel Phillips, Thomas A. M. Pugh, Ashwan Reddy, Xuhui Wang, Karina Williams, Florian Zabel, and Elisabeth J. Moyer
Geosci. Model Dev., 13, 2315–2336, https://doi.org/10.5194/gmd-13-2315-2020, https://doi.org/10.5194/gmd-13-2315-2020, 2020
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Concerns about food security under climate change motivate efforts to better understand future changes in crop yields. Crop models, which represent plant biology, are necessary tools for this purpose since they allow representing future climate, farmer choices, and new agricultural geographies. The Global Gridded Crop Model Intercomparison (GGCMI) Phase 2 experiment, under the Agricultural Model Intercomparison and Improvement Project (AgMIP), is designed to evaluate and improve crop models.
Seoung Soo Lee, George Kablick III, Zhanqing Li, Chang Hoon Jung, Yong-Sang Choi, Junshik Um, and Won Jun Choi
Atmos. Chem. Phys., 20, 3357–3371, https://doi.org/10.5194/acp-20-3357-2020, https://doi.org/10.5194/acp-20-3357-2020, 2020
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This paper examines a thunderstorm-type cloud that is triggered by wildfire. This paper shows that this cloud has a substantial impact on air components such as water vapor that act as a global warming agent together with carbon dioxide. This paper also shows that that impact is strongly dependent on fire intensity. This raises a possibility that clouds, which are triggered by fire, act as a modulator of climate changes and this function as a modulator is altered by how intense fire is.
Alexei Korolev, Ivan Heckman, Mengistu Wolde, Andrew S. Ackerman, Ann M. Fridlind, Luis A. Ladino, R. Paul Lawson, Jason Milbrandt, and Earle Williams
Atmos. Chem. Phys., 20, 1391–1429, https://doi.org/10.5194/acp-20-1391-2020, https://doi.org/10.5194/acp-20-1391-2020, 2020
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This study attempts identification of mechanisms of secondary ice production (SIP) based on the observation of small faceted ice crystals. It was found that in both mesoscale convective systems and frontal clouds, SIP was observed right above the melting layer and extended to the higher altitudes with colder temperatures. A principal conclusion of this work is that the freezing drop shattering mechanism is plausibly accounting for the measured ice concentrations in the observed condition.
Benjamin W. Clouser, Kara D. Lamb, Laszlo C. Sarkozy, Jan Habig, Volker Ebert, Harald Saathoff, Ottmar Möhler, and Elisabeth J. Moyer
Atmos. Chem. Phys., 20, 1089–1103, https://doi.org/10.5194/acp-20-1089-2020, https://doi.org/10.5194/acp-20-1089-2020, 2020
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Previous measurements of water vapor in the upper troposphere and lower stratosphere (UT/LS) have shown unexpectedly high concentrations of water vapor in ice clouds, which may be due to an incomplete understanding of the structure of ice and the behavior of ice growth in this part of the atmosphere. Water vapor measurements during the 2013 IsoCloud campaign at the AIDA cloud chamber show no evidence of this
anomalous supersaturationin conditions similar to the real atmosphere.
Kristina Pistone, Jens Redemann, Sarah Doherty, Paquita Zuidema, Sharon Burton, Brian Cairns, Sabrina Cochrane, Richard Ferrare, Connor Flynn, Steffen Freitag, Steven G. Howell, Meloë Kacenelenbogen, Samuel LeBlanc, Xu Liu, K. Sebastian Schmidt, Arthur J. Sedlacek III, Michal Segal-Rozenhaimer, Yohei Shinozuka, Snorre Stamnes, Bastiaan van Diedenhoven, Gerard Van Harten, and Feng Xu
Atmos. Chem. Phys., 19, 9181–9208, https://doi.org/10.5194/acp-19-9181-2019, https://doi.org/10.5194/acp-19-9181-2019, 2019
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Understanding how smoke particles interact with sunlight is important in calculating their effects on climate, since some smoke is more scattering (cooling) and some is more absorbing (heating). Knowing this proportion is important for both satellite observations and climate models. We measured smoke properties in a recent aircraft-based field campaign off the west coast of Africa and present a comparison of these properties as measured using the six different, independent techniques available.
Ann M. Fridlind, Marcus van Lier-Walqui, Scott Collis, Scott E. Giangrande, Robert C. Jackson, Xiaowen Li, Toshihisa Matsui, Richard Orville, Mark H. Picel, Daniel Rosenfeld, Alexander Ryzhkov, Richard Weitz, and Pengfei Zhang
Atmos. Meas. Tech., 12, 2979–3000, https://doi.org/10.5194/amt-12-2979-2019, https://doi.org/10.5194/amt-12-2979-2019, 2019
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Weather radars are offering improved capabilities to investigate storm physics, which remain poorly understood. We investigate enhanced use of such data near Houston, Texas, where pollution sources often provide a convenient contrast between polluted and clean air. We conclude that Houston is a favorable location to conduct a future field campaign during June through September because isolated storms are common and tend to last an hour, allowing frequent observations of a full life cycle.
Matz A. Haugen, Michael L. Stein, Ryan L. Sriver, and Elisabeth J. Moyer
Adv. Stat. Clim. Meteorol. Oceanogr., 5, 37–55, https://doi.org/10.5194/ascmo-5-37-2019, https://doi.org/10.5194/ascmo-5-37-2019, 2019
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This work uses current temperature observations combined with climate models to project future temperature estimates, e.g., 100 years into the future. We accomplish this by modeling temperature as a smooth function of time both in the seasonal variation as well as in the annual trend. These smooth functions are estimated at multiple quantiles that are all projected into the future. We hope that this work can be used as a template for how other climate variables can be projected into the future.
Joseph A. Finlon, Greg M. McFarquhar, Stephen W. Nesbitt, Robert M. Rauber, Hugh Morrison, Wei Wu, and Pengfei Zhang
Atmos. Chem. Phys., 19, 3621–3643, https://doi.org/10.5194/acp-19-3621-2019, https://doi.org/10.5194/acp-19-3621-2019, 2019
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A new approach describing the relationship between ice crystal mass (m) and dimension (D) is derived, characterizing it as a set of
equally realizableparameters based on the natural variability in cloud conditions observed by aircraft over the Great Plains. Results from this approach address shortcomings of microphysical parameterization schemes and remote sensing retrievals that employ a single m–D relation for a given ice species or environment.
Antonio Di Noia, Otto P. Hasekamp, Bastiaan van Diedenhoven, and Zhibo Zhang
Atmos. Meas. Tech., 12, 1697–1716, https://doi.org/10.5194/amt-12-1697-2019, https://doi.org/10.5194/amt-12-1697-2019, 2019
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We present a neural network algorithm for the retrieval of cloud physical properties from multi-angle polarimetric measurements. We have trained the algorithm on a large dataset of synthetic measurements and applied it to a year of POLDER-3 data. A comparison against MODIS cloud products reveals that our algorithm is capable of performing cloud property retrievals on a global scale and possibly improves the estimates of cloud effective radius over land with respect to existing POLDER-3 products.
Grégory Cesana, Anthony D. Del Genio, Andrew S. Ackerman, Maxwell Kelley, Gregory Elsaesser, Ann M. Fridlind, Ye Cheng, and Mao-Sung Yao
Atmos. Chem. Phys., 19, 2813–2832, https://doi.org/10.5194/acp-19-2813-2019, https://doi.org/10.5194/acp-19-2813-2019, 2019
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The response of low clouds to climate change (i.e., cloud feedbacks) is still pointed out as being the largest source of uncertainty in climate models. Here we use CALIPSO observations to discriminate climate models that reproduce observed interannual change of cloud fraction with SST forcings, referred to as a present-day cloud feedback. Modeling moist processes in the planetary boundary layer is crucial to produce large stratocumulus decks and realistic present-day cloud feedbacks.
Junshik Um, Greg M. McFarquhar, Jeffrey L. Stith, Chang Hoon Jung, Seoung Soo Lee, Ji Yi Lee, Younghwan Shin, Yun Gon Lee, Yiseok Isaac Yang, Seong Soo Yum, Byung-Gon Kim, Joo Wan Cha, and A-Reum Ko
Atmos. Chem. Phys., 18, 16915–16930, https://doi.org/10.5194/acp-18-16915-2018, https://doi.org/10.5194/acp-18-16915-2018, 2018
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During the 2012 Deep Convective Clouds and Chemistry experiment upper anvils of two storms were sampled. The occurrence of well-defined pristine crystals was low in the anvils, while single frozen droplets and frozen droplet aggregates (FDAs) were the dominant habits. A new algorithm was developed to automatically identify the number, size, and relative position of element frozen droplets within FDAs. The morphological characteristics of FDAs were compared with those of black carbon aggregates.
Emma Järvinen, Olivier Jourdan, David Neubauer, Bin Yao, Chao Liu, Meinrat O. Andreae, Ulrike Lohmann, Manfred Wendisch, Greg M. McFarquhar, Thomas Leisner, and Martin Schnaiter
Atmos. Chem. Phys., 18, 15767–15781, https://doi.org/10.5194/acp-18-15767-2018, https://doi.org/10.5194/acp-18-15767-2018, 2018
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Using light diffraction it is possible to detect microscopic features within ice particles that have not yet been fully characterized. Here, this technique was applied in airborne measurements, where it was found that majority of atmospheric ice particles have features that significantly change the way ice particles interact with solar light. The microscopic features make ice-containing clouds more reflective than previously thought, which could have consequences for predicting our climate.
Katia Lamer, Ann M. Fridlind, Andrew S. Ackerman, Pavlos Kollias, Eugene E. Clothiaux, and Maxwell Kelley
Geosci. Model Dev., 11, 4195–4214, https://doi.org/10.5194/gmd-11-4195-2018, https://doi.org/10.5194/gmd-11-4195-2018, 2018
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Weather and climate predictions of cloud, rain, and snow occurrence remain uncertain, in part because guidance from observation is incomplete. We present a tool that transforms predictions into observations from ground-based remote sensors. Liquid water and ice occurrence errors associated with the transformation are below 8 %, with ~ 3 % uncertainty. This (GO)2-SIM forward-simulator tool enables better evaluation of cloud, rain, and snow occurrence predictions using available observations.
Seoung Soo Lee, Byung-Gon Kim, Zhanqing Li, Yong-Sang Choi, Chang-Hoon Jung, Junshik Um, Jungbin Mok, and Kyong-Hwan Seo
Atmos. Chem. Phys., 18, 12531–12550, https://doi.org/10.5194/acp-18-12531-2018, https://doi.org/10.5194/acp-18-12531-2018, 2018
Armin Afchine, Christian Rolf, Anja Costa, Nicole Spelten, Martin Riese, Bernhard Buchholz, Volker Ebert, Romy Heller, Stefan Kaufmann, Andreas Minikin, Christiane Voigt, Martin Zöger, Jessica Smith, Paul Lawson, Alexey Lykov, Sergey Khaykin, and Martina Krämer
Atmos. Meas. Tech., 11, 4015–4031, https://doi.org/10.5194/amt-11-4015-2018, https://doi.org/10.5194/amt-11-4015-2018, 2018
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The ice water content (IWC) of cirrus clouds is an essential parameter that determines their radiative properties and is thus important for climate simulations. Experimental investigations of IWCs measured on board research aircraft reveal that their accuracy is influenced by the sampling position. IWCs detected at the aircraft roof deviate significantly from wing, side or bottom IWCs. The reasons are deflections of the gas streamlines and ice particle trajectories behind the aircraft cockpit.
Daniel J. Miller, Zhibo Zhang, Steven Platnick, Andrew S. Ackerman, Frank Werner, Celine Cornet, and Kirk Knobelspiesse
Atmos. Meas. Tech., 11, 3689–3715, https://doi.org/10.5194/amt-11-3689-2018, https://doi.org/10.5194/amt-11-3689-2018, 2018
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Prior satellite comparisons of bispectral and polarimetric cloud droplet size retrievals exhibited systematic biases. However, similar airborne instrument retrievals have been found to be quite similar to one another. This study explains this discrepancy in terms of differing sensitivity to vertical profile, as well as spatial and angular resolution. This is accomplished by using a satellite retrieval simulator – an LES cloud model coupled to radiative transfer and cloud retrieval algorithms.
Seoung Soo Lee, Zhanqing Li, Yuwei Zhang, Hyelim Yoo, Seungbum Kim, Byung-Gon Kim, Yong-Sang Choi, Jungbin Mok, Junshik Um, Kyoung Ock Choi, and Danhong Dong
Atmos. Chem. Phys., 18, 13–29, https://doi.org/10.5194/acp-18-13-2018, https://doi.org/10.5194/acp-18-13-2018, 2018
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This paper compares the contribution of resolutions with that of parameterizations to errors in the simulations of clouds, precipitation, and their interactions with aerosol in numerical weather prediction (NWP) models. This comparison shows that resolutions contribute to errors to a much greater degree than microphysics parameterizations. This finding provides a useful guideline for how to develop NWP models and has not been discussed in previous studies.
Antonio Di Noia, Otto P. Hasekamp, Lianghai Wu, Bastiaan van Diedenhoven, Brian Cairns, and John E. Yorks
Atmos. Meas. Tech., 10, 4235–4252, https://doi.org/10.5194/amt-10-4235-2017, https://doi.org/10.5194/amt-10-4235-2017, 2017
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In this paper an algorithm for the retrieval of aerosol properties from NASA Research Scanning Polarimeter (RSP) data is presented. An artificial neural network is used to produce a first estimate of the aerosol properties, which is then improved using an iterative retrieval scheme based on Phillips–Tikhonov regularization. Using the neural network retrievals as a first guess for the Phillips–Tikhonov improved the retrieval convergence, confirming results previously found on ground-based data.
Xiaoli Zhou, Andrew S. Ackerman, Ann M. Fridlind, Robert Wood, and Pavlos Kollias
Atmos. Chem. Phys., 17, 12725–12742, https://doi.org/10.5194/acp-17-12725-2017, https://doi.org/10.5194/acp-17-12725-2017, 2017
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Shallow maritime clouds make a well-known transition from stratocumulus to trade cumulus with flow from the subtropics equatorward. Three-day large-eddy simulations that investigate the potential influence of overlying African biomass burning plumes during that transition indicate that cloud-related impacts are likely substantially cooling to negligible at the top of the atmosphere, with magnitude sensitive to background and perturbation aerosol and cloud properties.
Kenneth Sinclair, Bastiaan van Diedenhoven, Brian Cairns, John Yorks, Andrzej Wasilewski, and Matthew McGill
Atmos. Meas. Tech., 10, 2361–2375, https://doi.org/10.5194/amt-10-2361-2017, https://doi.org/10.5194/amt-10-2361-2017, 2017
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We present a multi-angular contrast approach to retrieve cloud top height (CTH) using photogrammetry. We demonstrate the method’s ability to retrieve heights of multiple cloud layers within single footprints, using the multiple views available for each footprint. This paper provides an in-depth description and performance analysis of the CTH retrieval technique and the retrieved cloud heights are evaluated using collocated data from the Cloud Physics Lidar.
Andrew Poppick, Elisabeth J. Moyer, and Michael L. Stein
Adv. Stat. Clim. Meteorol. Oceanogr., 3, 33–53, https://doi.org/10.5194/ascmo-3-33-2017, https://doi.org/10.5194/ascmo-3-33-2017, 2017
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We show that ostensibly empirical methods of analyzing trends in the global mean temperature record, which appear to de-emphasize assumptions, can nevertheless produce misleading inferences about trends and associated uncertainty. We illustrate how a simple but physically motivated trend model can provide better-fitting and more broadly applicable results, and show the importance of adequately characterizing internal variability for estimating trend uncertainty.
Ann M. Fridlind, Xiaowen Li, Di Wu, Marcus van Lier-Walqui, Andrew S. Ackerman, Wei-Kuo Tao, Greg M. McFarquhar, Wei Wu, Xiquan Dong, Jingyu Wang, Alexander Ryzhkov, Pengfei Zhang, Michael R. Poellot, Andrea Neumann, and Jason M. Tomlinson
Atmos. Chem. Phys., 17, 5947–5972, https://doi.org/10.5194/acp-17-5947-2017, https://doi.org/10.5194/acp-17-5947-2017, 2017
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Understanding observed storm microphysics via computer simulation requires measurements of aerosol on which most hydrometeors form. We prepare aerosol input data for six storms observed over Oklahoma. We demonstrate their use in simulations of a case with widespread ice outflow well sampled by aircraft. Simulations predict too few ice crystals that are too large. We speculate that microphysics found in tropical storms occurred here, likely associated with poorly understood ice multiplication.
Whitney K. Huang, Michael L. Stein, David J. McInerney, Shanshan Sun, and Elisabeth J. Moyer
Adv. Stat. Clim. Meteorol. Oceanogr., 2, 79–103, https://doi.org/10.5194/ascmo-2-79-2016, https://doi.org/10.5194/ascmo-2-79-2016, 2016
L. M. Zamora, R. A. Kahn, M. J. Cubison, G. S. Diskin, J. L. Jimenez, Y. Kondo, G. M. McFarquhar, A. Nenes, K. L. Thornhill, A. Wisthaler, A. Zelenyuk, and L. D. Ziemba
Atmos. Chem. Phys., 16, 715–738, https://doi.org/10.5194/acp-16-715-2016, https://doi.org/10.5194/acp-16-715-2016, 2016
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Based on extensive aircraft campaigns, we quantify how biomass burning smoke affects subarctic and Arctic liquid cloud microphysical properties. Enhanced cloud albedo may decrease short-wave radiative flux by between 2 and 4 Wm2 or more in some subarctic conditions. Smoke halved average cloud droplet diameter. In one case study, it also appeared to limit droplet formation. Numerous Arctic background Aitken particles can also interact with combustion particles, perhaps affecting their properties.
A. M. Fridlind, A. S. Ackerman, A. Grandin, F. Dezitter, M. Weber, J. W. Strapp, A. V. Korolev, and C. R. Williams
Atmos. Chem. Phys., 15, 11713–11728, https://doi.org/10.5194/acp-15-11713-2015, https://doi.org/10.5194/acp-15-11713-2015, 2015
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Airbus measurements at elevations circa 11 km within large storm systems near Darwin and Santiago indicate ice mass distributed over area-equivalent diameters of 100-500 µm. Profiler-observed radar reflectivity and mean Doppler velocity under similar conditions are found to be consistent with measurements and with 1D simulations of steady-state stratiform rain columns initialized with observed ice size distributions. Results motivate investigation of ice formation pathways in Part II.
A. S. Ackerman, A. M. Fridlind, A. Grandin, F. Dezitter, M. Weber, J. W. Strapp, and A. V. Korolev
Atmos. Chem. Phys., 15, 11729–11751, https://doi.org/10.5194/acp-15-11729-2015, https://doi.org/10.5194/acp-15-11729-2015, 2015
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An updraft parcel model with size-resolved microphysics is used to investigate microphysical pathways leading to ice water content > 2 g m-3 with mass median area-equivalent diameter of 200-300 micron reported at ~11 km in tropical deep convection. Parcel simulations require substantial source of small crystals at temperatures > ~-10 deg C growing by vapor deposition. Warm rain in weaker updrafts surprisingly leads to greater ice mass owing to reduced competition for available water vapor.
M. Ottaviani, B. van Diedenhoven, and B. Cairns
The Cryosphere, 9, 1933–1942, https://doi.org/10.5194/tc-9-1933-2015, https://doi.org/10.5194/tc-9-1933-2015, 2015
L. Wu, O. Hasekamp, B. van Diedenhoven, and B. Cairns
Atmos. Meas. Tech., 8, 2625–2638, https://doi.org/10.5194/amt-8-2625-2015, https://doi.org/10.5194/amt-8-2625-2015, 2015
J. Um, G. M. McFarquhar, Y. P. Hong, S.-S. Lee, C. H. Jung, R. P. Lawson, and Q. Mo
Atmos. Chem. Phys., 15, 3933–3956, https://doi.org/10.5194/acp-15-3933-2015, https://doi.org/10.5194/acp-15-3933-2015, 2015
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Dimensions of ice crystals increased with an increase in temperature and the L-W relationships of crystals with a given L depended heavily on temperature, whereas the aspect ratio depended only weakly on temperature. The relative frequency of occurrence of plates was much larger in anvil clouds compared to that of columnar crystals (i.e., columns and bullet rosettes), whereas the relative occurrence frequency of columnar crystals was much larger in non-anvil clouds.
K. Knobelspiesse, B. van Diedenhoven, A. Marshak, S. Dunagan, B. Holben, and I. Slutsker
Atmos. Meas. Tech., 8, 1537–1554, https://doi.org/10.5194/amt-8-1537-2015, https://doi.org/10.5194/amt-8-1537-2015, 2015
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We test if ground-based sun photometers/radiometers like those in the Aerosol Robotic Network (AERONET) can use the polarization sensitivity of some instruments for improved cloud optical property retrieval. Our radiative transfer simulations show that the direction of linear polarization indicates cloud thermodynamic phase for optically thin clouds. In practice, data analysis shows a weak response with AERONET instruments, most likely due to noise and orientation/calibration ambiguity.
W. B. Leeds, E. J. Moyer, and M. L. Stein
Adv. Stat. Clim. Meteorol. Oceanogr., 1, 1–14, https://doi.org/10.5194/ascmo-1-1-2015, https://doi.org/10.5194/ascmo-1-1-2015, 2015
J. L. Stith, L. M. Avallone, A. Bansemer, B. Basarab, S. W. Dorsi, B. Fuchs, R. P. Lawson, D. C. Rogers, S. Rutledge, and D. W. Toohey
Atmos. Chem. Phys., 14, 1973–1985, https://doi.org/10.5194/acp-14-1973-2014, https://doi.org/10.5194/acp-14-1973-2014, 2014
M. Bolot, B. Legras, and E. J. Moyer
Atmos. Chem. Phys., 13, 7903–7935, https://doi.org/10.5194/acp-13-7903-2013, https://doi.org/10.5194/acp-13-7903-2013, 2013
B. van Diedenhoven, B. Cairns, A. M. Fridlind, A. S. Ackerman, and T. J. Garrett
Atmos. Chem. Phys., 13, 3185–3203, https://doi.org/10.5194/acp-13-3185-2013, https://doi.org/10.5194/acp-13-3185-2013, 2013
Related subject area
Subject: Clouds and Precipitation | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
The presence of clouds lowers climate sensitivity in the MPI-ESM1.2 climate model
Diurnal variation in an amplified canopy urban heat island during heat wave periods in the megacity of Beijing: roles of mountain–valley breeze and urban morphology
Diurnal evolution of non-precipitating marine stratocumuli in a large-eddy simulation ensemble
High ice water content in tropical mesoscale convective systems (a conceptual model)
Evolution of cloud droplet temperature and lifetime in spatiotemporally varying subsaturated environments with implications for ice nucleation at cloud edges
Effect of secondary ice production processes on the simulation of ice pellets using the Predicted Particle Properties microphysics scheme
Simulated particle evolution within a winter storm: contributions of riming to radar moments and precipitation fallout
A thermal-driven graupel generation process to explain dry-season convective vigor over the Amazon
Modeling homogeneous ice nucleation from drop-freezing experiments: impact of droplet volume dispersion and cooling rates
Cloud water adjustments to aerosol perturbations are buffered by solar heating in non-precipitating marine stratocumuli
Glaciation of mixed-phase clouds: insights from bulk model and bin-microphysics large-eddy simulation informed by laboratory experiment
Microphysical processes involving the vapour phase dominate in simulated low-level Arctic clouds
Understanding aerosol–cloud interactions using a single-column model for a cold-air outbreak case during the ACTIVATE campaign
On the sensitivity of aerosol–cloud interactions to changes in sea surface temperature in radiative–convective equilibrium
The role of ascent timescale for WCB moisture transport into the UTLS
Exploring aerosol–cloud interactions in liquid-phase clouds over eastern China and its adjacent ocean using the WRF-Chem–SBM model
Estimating the concentration of silver iodide needed to detect unambiguous signatures of glaciogenic cloud seeding
The impact of mesh size and microphysics scheme on the representation of mid-level clouds in the ICON model in hilly and complex terrain
Finite domains cause bias in measured and modeled distributions of cloud sizes
A systematic evaluation of high-cloud controlling factors
Tracking precipitation features and associated large-scale environments over southeastern Texas
Revisiting the evolution of downhill thunderstorms over Beijing: a new perspective from a radar wind profiler mesonet
How well can persistent contrails be predicted? An update
Potential impacts of marine fuel regulations on Arctic clouds and radiative feedbacks
Present-day correlations are insufficient to predict cloud albedo change by anthropogenic aerosols in E3SM v2
Simulations of primary and secondary ice production during an Arctic mixed-phase cloud case from the Ny-Ålesund Aerosol Cloud Experiment (NASCENT) campaign
Microphysical characteristics of precipitation within convective overshooting over East China observed by GPM DPR and ERA5
The Impact of Aerosol on Cloud Water: A Heuristic Perspective
Effects of radiative cooling on advection fog over the northwest Pacific Ocean: observations and large-eddy simulations
Evaluating the Wegener–Bergeron–Findeisen process in ICON in large-eddy mode with in situ observations from the CLOUDLAB project
Aerosol-induced closure of marine cloud cells: enhanced effects in the presence of precipitation
Ice-nucleating particle concentration impacts cloud properties over Dronning Maud Land, East Antarctica, in COSMO-CLM2
Impact of ice multiplication on the cloud electrification of a cold-season thunderstorm: a numerical case study
Developing a climatological simplification of aerosols to enter the cloud microphysics of a global climate model
Interactions between trade wind clouds and local forcings over the Great Barrier Reef: a case study using convection-permitting simulations
Variability in the properties of the distribution of the relative humidity with respect to ice: implications for contrail formation
Simulating the seeder–feeder impacts on cloud ice and precipitation over the Alps
Can pollen affect precipitation?
Cloud response to co-condensation of water and organic vapors over the boreal forest
Distribution and morphology of non-persistent contrail and persistent contrail formation areas in ERA5
Connection of Surface Snowfall Bias to Cloud Phase Bias – Satellite Observations, ERA5, and CMIP6
Above-cloud concentrations of cloud condensation nuclei help to sustain some Arctic low-level clouds
WRF-SBM Numerical Simulation of Aerosol Effects on Stratiform Warm Clouds in Jiangxi, China
Contrail formation on ambient aerosol particles for aircraft with hydrogen combustion: a box model trajectory study
Effects of intermittent aerosol forcing on the stratocumulus-to-cumulus transition
Cloud properties and their projected changes in CMIP models with low to high climate sensitivity
Water isotopic characterisation of the cloud–circulation coupling in the North Atlantic trades – Part 2: The imprint of the atmospheric circulation at different scales
Impact of urban land use on mean and heavy rainfall during the Indian summer monsoon
Towards a more reliable forecast of ice supersaturation: concept of a one-moment ice-cloud scheme that avoids saturation adjustment
Opinion: Tropical cirrus – from micro-scale processes to climate-scale impacts
Andrea Mosso, Thomas Hocking, and Thorsten Mauritsen
Atmos. Chem. Phys., 24, 12793–12806, https://doi.org/10.5194/acp-24-12793-2024, https://doi.org/10.5194/acp-24-12793-2024, 2024
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Clouds play a crucial role in the Earth's energy balance, as they can either warm up or cool down the area they cover depending on their height and depth. They are expected to alter their behaviour under climate change, affecting the warming generated by greenhouse gases. This paper proposes a new method to estimate their overall effect on this warming by simulating a climate where clouds are transparent. Results show that with the model used, clouds have a stabilising effect on climate.
Tao Shi, Yuanjian Yang, Ping Qi, and Simone Lolli
Atmos. Chem. Phys., 24, 12807–12822, https://doi.org/10.5194/acp-24-12807-2024, https://doi.org/10.5194/acp-24-12807-2024, 2024
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This paper explored the formation mechanisms of the amplified canopy urban heat island intensity (ΔCUHII) during heat wave (HW) periods in the megacity of Beijing from the perspectives of mountain–valley breeze and urban morphology. During the mountain breeze phase, high-rise buildings with lower sky view factors (SVFs) had a pronounced effect on the ΔCUHII. During the valley breeze phase, high-rise buildings exerted a dual influence on the ΔCUHII.
Yao-Sheng Chen, Jianhao Zhang, Fabian Hoffmann, Takanobu Yamaguchi, Franziska Glassmeier, Xiaoli Zhou, and Graham Feingold
Atmos. Chem. Phys., 24, 12661–12685, https://doi.org/10.5194/acp-24-12661-2024, https://doi.org/10.5194/acp-24-12661-2024, 2024
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Marine stratocumulus cloud is a type of shallow cloud that covers the vast areas of Earth's surface. It plays an important role in Earth's energy balance by reflecting solar radiation back to space. We used numerical models to simulate a large number of marine stratocumuli with different characteristics. We found that how the clouds develop throughout the day is affected by the level of humidity in the air above the clouds and how closely the clouds connect to the ocean surface.
Alexei Korolev, Zhipeng Qu, Jason Milbrandt, Ivan Heckman, Mélissa Cholette, Mengistu Wolde, Cuong Nguyen, Greg M. McFarquhar, Paul Lawson, and Ann M. Fridlind
Atmos. Chem. Phys., 24, 11849–11881, https://doi.org/10.5194/acp-24-11849-2024, https://doi.org/10.5194/acp-24-11849-2024, 2024
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The phenomenon of high ice water content (HIWC) occurs in mesoscale convective systems (MCSs) when a large number of small ice particles with typical sizes of a few hundred micrometers is found at high altitudes. It was found that secondary ice production in the vicinity of the melting layer plays a key role in the formation and maintenance of HIWC. This study presents a conceptual model of the formation of HIWC in tropical MCSs based on in situ observations and numerical simulation.
Puja Roy, Robert M. Rauber, and Larry Di Girolamo
Atmos. Chem. Phys., 24, 11653–11678, https://doi.org/10.5194/acp-24-11653-2024, https://doi.org/10.5194/acp-24-11653-2024, 2024
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Cloud droplet temperature and lifetime impact cloud microphysical processes such as the activation of ice-nucleating particles. We investigate the thermal and radial evolution of supercooled cloud droplets and their surrounding environments with an aim to better understand observed enhanced ice formation at supercooled cloud edges. This analysis shows that the magnitude of droplet cooling during evaporation is greater than estimated from past studies, especially for drier environments.
Mathieu Lachapelle, Mélissa Cholette, and Julie M. Thériault
Atmos. Chem. Phys., 24, 11285–11304, https://doi.org/10.5194/acp-24-11285-2024, https://doi.org/10.5194/acp-24-11285-2024, 2024
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Hazardous precipitation types such as ice pellets and freezing rain are difficult to predict because they are associated with complex microphysical processes. Using Predicted Particle Properties (P3), this work shows that secondary ice production processes increase the amount of ice pellets simulated while decreasing the amount of freezing rain. Moreover, the properties of the simulated precipitation compare well with those that were measured.
Andrew DeLaFrance, Lynn A. McMurdie, Angela K. Rowe, and Andrew J. Heymsfield
Atmos. Chem. Phys., 24, 11191–11206, https://doi.org/10.5194/acp-24-11191-2024, https://doi.org/10.5194/acp-24-11191-2024, 2024
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Using a numerical model, the process whereby falling ice crystals accumulate supercooled liquid water droplets is investigated to elucidate its effects on radar-based measurements and surface precipitation. We demonstrate that this process accounted for 55% of the precipitation during a wintertime storm and is uniquely discernable from other ice crystal growth processes in Doppler velocity measurements. These results have implications for measurements from airborne and spaceborne platforms.
Toshi Matsui, Daniel Hernandez-Deckers, Scott E. Giangrande, Thiago S. Biscaro, Ann Fridlind, and Scott Braun
Atmos. Chem. Phys., 24, 10793–10814, https://doi.org/10.5194/acp-24-10793-2024, https://doi.org/10.5194/acp-24-10793-2024, 2024
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Using computer simulations and real measurements, we discovered that storms over the Amazon were narrower but more intense during the dry periods, producing heavier rain and more ice particles in the clouds. Our research showed that cumulus bubbles played a key role in creating these intense storms. This study can improve the representation of the effect of continental and ocean environments on tropical regions' rainfall patterns in simulations.
Ravi Kumar Reddy Addula, Ingrid de Almeida Ribeiro, Valeria Molinero, and Baron Peters
Atmos. Chem. Phys., 24, 10833–10848, https://doi.org/10.5194/acp-24-10833-2024, https://doi.org/10.5194/acp-24-10833-2024, 2024
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Ice nucleation from supercooled droplets is important in many weather and climate modeling efforts. For experiments where droplets are steadily supercooled from the freezing point, our work combines nucleation theory and survival probability analysis to predict the nucleation spectrum, i.e., droplet freezing probabilities vs. temperature. We use the new framework to extract approximately consistent rate parameters from experiments with different cooling rates and droplet sizes.
Jianhao Zhang, Yao-Sheng Chen, Takanobu Yamaguchi, and Graham Feingold
Atmos. Chem. Phys., 24, 10425–10440, https://doi.org/10.5194/acp-24-10425-2024, https://doi.org/10.5194/acp-24-10425-2024, 2024
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Quantifying cloud response to aerosol perturbations presents a major challenge in understanding the human impact on climate. Using a large number of process-resolving simulations of marine stratocumulus, we show that solar heating drives a negative feedback mechanism that buffers the persistent negative trend in cloud water adjustment after sunrise. This finding has implications for the dependence of the cloud cooling effect on the timing of deliberate aerosol perturbations.
Aaron Wang, Steve Krueger, Sisi Chen, Mikhail Ovchinnikov, Will Cantrell, and Raymond A. Shaw
Atmos. Chem. Phys., 24, 10245–10260, https://doi.org/10.5194/acp-24-10245-2024, https://doi.org/10.5194/acp-24-10245-2024, 2024
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We employ two methods to examine a laboratory experiment on clouds with both ice and liquid phases. The first assumes well-mixed properties; the second resolves the spatial distribution of turbulence and cloud particles. Results show that while the trends in mean properties generally align, when turbulence is resolved, liquid droplets are not fully depleted by ice due to incomplete mixing. This underscores the threshold of ice mass fraction in distinguishing mixed-phase clouds from ice clouds.
Theresa Kiszler, Davide Ori, and Vera Schemann
Atmos. Chem. Phys., 24, 10039–10053, https://doi.org/10.5194/acp-24-10039-2024, https://doi.org/10.5194/acp-24-10039-2024, 2024
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Microphysical processes impact the phase-partitioning of clouds. In this study we evaluate these processes while focusing on low-level Arctic clouds. To achieve this we used an extensive simulation set in combination with a new diagnostic tool. This study presents our findings on the relevance of these processes and their behaviour under different thermodynamic regimes.
Shuaiqi Tang, Hailong Wang, Xiang-Yu Li, Jingyi Chen, Armin Sorooshian, Xubin Zeng, Ewan Crosbie, Kenneth L. Thornhill, Luke D. Ziemba, and Christiane Voigt
Atmos. Chem. Phys., 24, 10073–10092, https://doi.org/10.5194/acp-24-10073-2024, https://doi.org/10.5194/acp-24-10073-2024, 2024
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We examined marine boundary layer clouds and their interactions with aerosols in the E3SM single-column model (SCM) for a case study. The SCM shows good agreement when simulating the clouds with high-resolution models. It reproduces the relationship between cloud droplet and aerosol particle number concentrations as produced in global models. However, the relationship between cloud liquid water and droplet number concentration is different, warranting further investigation.
Suf Lorian and Guy Dagan
Atmos. Chem. Phys., 24, 9323–9338, https://doi.org/10.5194/acp-24-9323-2024, https://doi.org/10.5194/acp-24-9323-2024, 2024
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We examine the combined effect of aerosols and sea surface temperature (SST) on clouds under equilibrium conditions in cloud-resolving radiative–convective equilibrium simulations. We demonstrate that the aerosol–cloud interaction's effect on top-of-atmosphere energy gain strongly depends on the underlying SST, while the shortwave part of the spectrum is significantly more sensitive to SST. Furthermore, increasing aerosols influences upper-troposphere stability and thus anvil cloud fraction.
Cornelis Schwenk and Annette Miltenberger
EGUsphere, https://doi.org/10.5194/egusphere-2024-2402, https://doi.org/10.5194/egusphere-2024-2402, 2024
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Warm conveyor belts (WCBs) transport moisture into the upper atmosphere, where it acts as a greenhouse gas. This transport is not well understood, and the role of rapidly rising air is unclear. We simulate a WCB and look at fast and slow rising air to see how moisture is (differently) transported. We find that for fast ascending air more ice particles reach higher into the atmosphere, and that frozen cloud particles are removed differently than during slow ascent, which has more water vapour.
Jianqi Zhao, Xiaoyan Ma, Johannes Quaas, and Hailing Jia
Atmos. Chem. Phys., 24, 9101–9118, https://doi.org/10.5194/acp-24-9101-2024, https://doi.org/10.5194/acp-24-9101-2024, 2024
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We explore aerosol–cloud interactions in liquid-phase clouds over eastern China and its adjacent ocean in winter based on the WRF-Chem–SBM model, which couples a spectral-bin microphysics scheme and an online aerosol module. Our study highlights the differences in aerosol–cloud interactions between land and ocean and between precipitation clouds and non-precipitation clouds, and it differentiates and quantifies their underlying mechanisms.
Jing Yang, Jiaojiao Li, Meilian Chen, Xiaoqin Jing, Yan Yin, Bart Geerts, Zhien Wang, Yubao Liu, Baojun Chen, Shaofeng Hua, Hao Hu, Xiaobo Dong, Ping Tian, Qian Chen, and Yang Gao
EGUsphere, https://doi.org/10.5194/egusphere-2024-2301, https://doi.org/10.5194/egusphere-2024-2301, 2024
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Detecting unambiguous signatures is vital to investigate cloud seeding impacts, but in many cases seeding signature is immersed in natural variability. In this study, the reflectivity change induced by glaciogenic seeding using different AgI concentrations is investigated under various conditions, and a method is developed to estimate the AgI concentration needed to detect unambiguous seeding signatures. The results are helpful in operational seeding decision making of the AgI amount dispersed.
Nadja Omanovic, Brigitta Goger, and Ulrike Lohmann
EGUsphere, https://doi.org/10.5194/egusphere-2024-1989, https://doi.org/10.5194/egusphere-2024-1989, 2024
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We evaluated the numerical weather model ICON in two horizontal resolutions with two bulk microphysics schemes over hilly and complex terrain in Switzerland and Austria, respectively. We focused on the model's ability of simulating mid-level clouds in summer and winter. By combining observational data from two different field campaigns we show that both an increase in horizontal resolution and a more advanced cloud microphysics scheme is strongly beneficial for the cloud representation.
Thomas D. DeWitt and Timothy J. Garrett
Atmos. Chem. Phys., 24, 8457–8472, https://doi.org/10.5194/acp-24-8457-2024, https://doi.org/10.5194/acp-24-8457-2024, 2024
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There is considerable disagreement on mathematical parameters that describe the number of clouds of different sizes as well as the size of the largest clouds. Both are key defining characteristics of Earth's atmosphere. A previous study provided an incorrect explanation for the disagreement. Instead, the disagreement may be explained by prior studies not properly accounting for the size of their measurement domain. We offer recommendations for how the domain size can be accounted for.
Sarah Wilson Kemsley, Paulo Ceppi, Hendrik Andersen, Jan Cermak, Philip Stier, and Peer Nowack
Atmos. Chem. Phys., 24, 8295–8316, https://doi.org/10.5194/acp-24-8295-2024, https://doi.org/10.5194/acp-24-8295-2024, 2024
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Aiming to inform parameter selection for future observational constraint analyses, we incorporate five candidate meteorological drivers specifically targeting high clouds into a cloud controlling factor framework within a range of spatial domain sizes. We find a discrepancy between optimal domain size for predicting locally and globally aggregated cloud radiative anomalies and identify upper-tropospheric static stability as an important high-cloud controlling factor.
Ye Liu, Yun Qian, Larry K. Berg, Zhe Feng, Jianfeng Li, Jingyi Chen, and Zhao Yang
Atmos. Chem. Phys., 24, 8165–8181, https://doi.org/10.5194/acp-24-8165-2024, https://doi.org/10.5194/acp-24-8165-2024, 2024
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Deep convection under various large-scale meteorological patterns (LSMPs) shows distinct precipitation features. In southeastern Texas, mesoscale convective systems (MCSs) contribute significantly to precipitation year-round, while isolated deep convection (IDC) is prominent in summer and fall. Self-organizing maps (SOMs) reveal convection can occur without large-scale lifting or moisture convergence. MCSs and IDC events have distinct life cycles influenced by specific LSMPs.
Xiaoran Guo, Jianping Guo, Tianmeng Chen, Ning Li, Fan Zhang, and Yuping Sun
Atmos. Chem. Phys., 24, 8067–8083, https://doi.org/10.5194/acp-24-8067-2024, https://doi.org/10.5194/acp-24-8067-2024, 2024
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The prediction of downhill thunderstorms (DSs) remains elusive. We propose an objective method to identify DSs, based on which enhanced and dissipated DSs are discriminated. A radar wind profiler (RWP) mesonet is used to derive divergence and vertical velocity. The mid-troposphere divergence and prevailing westerlies enhance the intensity of DSs, whereas low-level divergence is observed when the DS dissipates. The findings highlight the key role that an RWP mesonet plays in the evolution of DSs.
Sina Hofer, Klaus Gierens, and Susanne Rohs
Atmos. Chem. Phys., 24, 7911–7925, https://doi.org/10.5194/acp-24-7911-2024, https://doi.org/10.5194/acp-24-7911-2024, 2024
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We try to improve the forecast of ice supersaturation (ISS) and potential persistent contrails using data on dynamical quantities in addition to temperature and relative humidity in a modern kind of regression model. Although the results are improved, they are not good enough for flight routing. The origin of the problem is the strong overlap of probability densities conditioned on cases with and without ice-supersaturated regions (ISSRs) in the important range of 70–100 %.
Luís Filipe Escusa dos Santos, Hannah C. Frostenberg, Alejandro Baró Pérez, Annica M. L. Ekman, Luisa Ickes, and Erik S. Thomson
EGUsphere, https://doi.org/10.5194/egusphere-2024-1891, https://doi.org/10.5194/egusphere-2024-1891, 2024
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The Arctic is experiencing enhanced surface warming. The observed decline in Arctic sea-ice extent is projected to lead to an increase in Arctic shipping activity which may lead to further climatic feedbacks. We investigate, using an atmospheric model and results from marine engine experiments which focused on fuel sulfur content reduction and exhaust wet scrubbing, how ship exhaust particles influence the properties of Arctic clouds. Implications for radiative surface processes are discussed.
Naser Mahfouz, Johannes Mülmenstädt, and Susannah Burrows
Atmos. Chem. Phys., 24, 7253–7260, https://doi.org/10.5194/acp-24-7253-2024, https://doi.org/10.5194/acp-24-7253-2024, 2024
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Climate models are our primary tool to probe past, present, and future climate states unlike the more recent observation record. By constructing a hypothetical model configuration, we show that present-day correlations are insufficient to predict a persistent uncertainty in climate projection (how much sun because clouds will reflect in a changing climate). We hope our result will contribute to the scholarly conversation on better utilizing observations to constrain climate uncertainties.
Britta Schäfer, Robert Oscar David, Paraskevi Georgakaki, Julie Thérèse Pasquier, Georgia Sotiropoulou, and Trude Storelvmo
Atmos. Chem. Phys., 24, 7179–7202, https://doi.org/10.5194/acp-24-7179-2024, https://doi.org/10.5194/acp-24-7179-2024, 2024
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Mixed-phase clouds, i.e., clouds consisting of ice and supercooled water, are very common in the Arctic. However, how these clouds form is often not correctly represented in standard weather models. We show that both ice crystal concentrations in the cloud and precipitation from the cloud can be improved in the model when aerosol concentrations are prescribed from observations and when more processes for ice multiplication, i.e., the production of new ice particles from existing ice, are added.
Nan Sun, Gaopeng Lu, and Yunfei Fu
Atmos. Chem. Phys., 24, 7123–7135, https://doi.org/10.5194/acp-24-7123-2024, https://doi.org/10.5194/acp-24-7123-2024, 2024
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Microphysical characteristics of convective overshooting are essential but poorly understood, and we examine them by using the latest data. (1) Convective overshooting events mainly occur over NC (Northeast China) and northern MEC (Middle and East China). (2) Radar reflectivity of convective overshooting over NC accounts for a higher proportion below the zero level, while the opposite is the case for MEC and SC (South China). (3) Droplets of convective overshooting are large but sparse.
Fabian Hoffmann, Franziska Glassmeier, and Graham Feingold
EGUsphere, https://doi.org/10.5194/egusphere-2024-1725, https://doi.org/10.5194/egusphere-2024-1725, 2024
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Clouds constitute a major cooling influence on Earth's climate system by reflecting a large fraction of the incident solar radiation back to space. This ability is controlled by the number of cloud droplets, which is governed by the number of aerosol particles in the atmosphere, laying out the foundation for so-called aerosol-cloud-climate interactions. In this study, a simple model to understand the effect of aerosol on cloud water is developed and applied.
Liu Yang, Saisai Ding, Jing-Wu Liu, and Su-Ping Zhang
Atmos. Chem. Phys., 24, 6809–6824, https://doi.org/10.5194/acp-24-6809-2024, https://doi.org/10.5194/acp-24-6809-2024, 2024
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Advection fog occurs when warm and moist air moves over a cold sea surface. In this situation, the temperature of the foggy air usually drops below the sea surface temperature (SST), particularly at night. High-resolution simulations show that the cooling effect of longwave radiation from the top of the fog layer permeates through the fog, resulting in a cooling of the surface air below SST. This study emphasizes the significance of monitoring air temperature to enhance sea fog forecasting.
Nadja Omanovic, Sylvaine Ferrachat, Christopher Fuchs, Jan Henneberger, Anna J. Miller, Kevin Ohneiser, Fabiola Ramelli, Patric Seifert, Robert Spirig, Huiying Zhang, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 6825–6844, https://doi.org/10.5194/acp-24-6825-2024, https://doi.org/10.5194/acp-24-6825-2024, 2024
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We present simulations with a high-resolution numerical weather prediction model to study the growth of ice crystals in low clouds following glaciogenic seeding. We show that the simulated ice crystals grow slower than observed and do not consume as many cloud droplets as measured in the field. This may have implications for forecasting precipitation, as the ice phase is crucial for precipitation at middle and high latitudes.
Matthew W. Christensen, Peng Wu, Adam C. Varble, Heng Xiao, and Jerome D. Fast
Atmos. Chem. Phys., 24, 6455–6476, https://doi.org/10.5194/acp-24-6455-2024, https://doi.org/10.5194/acp-24-6455-2024, 2024
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Clouds are essential to keep Earth cooler by reflecting sunlight back to space. We show that an increase in aerosol concentration suppresses precipitation in clouds, causing them to accumulate water and expand in a polluted environment with stronger turbulence and radiative cooling. This process enhances their reflectance by 51 %. It is therefore prudent to account for cloud fraction changes in assessments of aerosol–cloud interactions to improve predictions of climate change.
Florian Sauerland, Niels Souverijns, Anna Possner, Heike Wex, Preben Van Overmeiren, Alexander Mangold, Kwinten Van Weverberg, and Nicole van Lipzig
EGUsphere, https://doi.org/10.5194/egusphere-2024-1341, https://doi.org/10.5194/egusphere-2024-1341, 2024
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We use a regional climate model, COSMO-CLM², enhanced with a module resolving aerosol processes, to study Antarctic clouds. We prescribe INP concentrations from observations at Princess Elisabeth Station and other sites to the model. We assess how Antarctic clouds respond to INP concentration changes, validating results with cloud observations from the station. Our results show that aerosol-cloud interactions vary with temperature, providing valuable insights into Antarctic cloud dynamics.
Jing Yang, Shiye Huang, Tianqi Yang, Qilin Zhang, Yuting Deng, and Yubao Liu
Atmos. Chem. Phys., 24, 5989–6010, https://doi.org/10.5194/acp-24-5989-2024, https://doi.org/10.5194/acp-24-5989-2024, 2024
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This study contributes to filling the dearth of understanding the impacts of different secondary ice production (SIP) processes on the cloud electrification in cold-season thunderstorms. The results suggest that SIP, especially the rime-splintering process and the shattering of freezing drops, has significant impacts on the charge structure of the storm. In addition, the modeled radar composite reflectivity and flash rate are improved after implementing the SIP processes in the model.
Ulrike Proske, Sylvaine Ferrachat, and Ulrike Lohmann
Atmos. Chem. Phys., 24, 5907–5933, https://doi.org/10.5194/acp-24-5907-2024, https://doi.org/10.5194/acp-24-5907-2024, 2024
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Climate models include treatment of aerosol particles because these influence clouds and radiation. Over time their representation has grown increasingly detailed. This complexity may hinder our understanding of model behaviour. Thus here we simplify the aerosol representation of our climate model by prescribing mean concentrations, which saves run time and helps to discover unexpected model behaviour. We conclude that simplifications provide a new perspective for model study and development.
Wenhui Zhao, Yi Huang, Steven Siems, Michael Manton, and Daniel Harrison
Atmos. Chem. Phys., 24, 5713–5736, https://doi.org/10.5194/acp-24-5713-2024, https://doi.org/10.5194/acp-24-5713-2024, 2024
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We studied how shallow clouds and rain behave over the Great Barrier Reef (GBR) using a detailed weather model. We found that the shape of the land, especially mountains, and particles in the air play big roles in influencing these clouds. Surprisingly, the sea's temperature had a smaller effect. Our research helps us understand the GBR's climate and how various factors can influence it, where the importance of the local cloud in thermal coral bleaching has recently been identified.
Sidiki Sanogo, Olivier Boucher, Nicolas Bellouin, Audran Borella, Kevin Wolf, and Susanne Rohs
Atmos. Chem. Phys., 24, 5495–5511, https://doi.org/10.5194/acp-24-5495-2024, https://doi.org/10.5194/acp-24-5495-2024, 2024
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Relative humidity relative to ice (RHi) is a key variable in the formation of cirrus clouds and contrails. This study shows that the properties of the probability density function of RHi differ between the tropics and higher latitudes. In line with RHi and temperature variability, aircraft are likely to produce more contrails with bioethanol and liquid hydrogen as fuel. The impact of this fuel change decreases with decreasing pressure levels but increases from high latitudes to the tropics.
Zane Dedekind, Ulrike Proske, Sylvaine Ferrachat, Ulrike Lohmann, and David Neubauer
Atmos. Chem. Phys., 24, 5389–5404, https://doi.org/10.5194/acp-24-5389-2024, https://doi.org/10.5194/acp-24-5389-2024, 2024
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Ice particles precipitating into lower clouds from an upper cloud, the seeder–feeder process, can enhance precipitation. A numerical modeling study conducted in the Swiss Alps found that 48 % of observed clouds were overlapping, with the seeder–feeder process occurring in 10 % of these clouds. Inhibiting the seeder–feeder process reduced the surface precipitation and ice particle growth rates, which were further reduced when additional ice multiplication processes were included in the model.
Marje Prank, Juha Tonttila, Xiaoxia Shang, Sami Romakkaniemi, and Tomi Raatikainen
EGUsphere, https://doi.org/10.5194/egusphere-2024-876, https://doi.org/10.5194/egusphere-2024-876, 2024
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Large primary bioparticles such as pollen can be abundant in the atmosphere. In humid conditions pollens can rupture and release a large number of fine sub-pollen particles (SPPs). The paper investigates what kind of birch pollen concentrations are needed for the pollen and SPPs to start playing a noticeable role in cloud processes and alter precipitation formation. In the studied cases only the largest observed pollen concentrations were able to noticeably alter the precipitation formation.
Liine Heikkinen, Daniel G. Partridge, Sara Blichner, Wei Huang, Rahul Ranjan, Paul Bowen, Emanuele Tovazzi, Tuukka Petäjä, Claudia Mohr, and Ilona Riipinen
Atmos. Chem. Phys., 24, 5117–5147, https://doi.org/10.5194/acp-24-5117-2024, https://doi.org/10.5194/acp-24-5117-2024, 2024
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The organic vapor condensation with water vapor (co-condensation) in rising air below clouds is modeled in this work over the boreal forest because the forest air is rich in organic vapors. We show that the number of cloud droplets can increase by 20 % if considering co-condensation. The enhancements are even larger if the air contains many small, naturally produced aerosol particles. Such conditions are most frequently met in spring in the boreal forest.
Kevin Wolf, Nicolas Bellouin, and Olivier Boucher
Atmos. Chem. Phys., 24, 5009–5024, https://doi.org/10.5194/acp-24-5009-2024, https://doi.org/10.5194/acp-24-5009-2024, 2024
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The contrail formation potential and its tempo-spatial distribution are estimated for the North Atlantic flight corridor. Meteorological conditions of temperature and relative humidity are taken from the ERA5 re-analysis and IAGOS. Based on IAGOS flight tracks, crossing length, size, orientation, frequency of occurrence, and overlap of persistent contrail formation areas are determined. The presented conclusions might provide a guide for statistical flight track optimization to reduce contrails.
Franziska Hellmuth, Tim Carlsen, Anne Sophie Daloz, Robert Oscar David, and Trude Storelvmo
EGUsphere, https://doi.org/10.5194/egusphere-2024-754, https://doi.org/10.5194/egusphere-2024-754, 2024
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This article compares the occurrence of supercooled liquid-containing clouds (sLCCs) and their link to surface snowfall in CloudSat-CALIPSO, ERA5, and CMIP6 models. Significant discrepancies were found, with ERA5 and CMIP6 consistently overestimating sLCC and snowfall frequency. This bias is likely due to cloud microphysics parameterization. This conclusion has implications for accurately representing cloud phase and snowfall in future climate projections.
Lucas J. Sterzinger and Adele L. Igel
Atmos. Chem. Phys., 24, 3529–3540, https://doi.org/10.5194/acp-24-3529-2024, https://doi.org/10.5194/acp-24-3529-2024, 2024
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Using idealized large eddy simulations, we find that clouds forming in the Arctic in environments with low concentrations of aerosol particles may be sustained by mixing in new particles through the cloud top. Observations show that higher concentrations of these particles regularly exist above cloud top in concentrations that are sufficient to promote this sustenance.
Yi Li, Xiaoli Liu, and Hengjia Cai
EGUsphere, https://doi.org/10.5194/egusphere-2023-2644, https://doi.org/10.5194/egusphere-2023-2644, 2024
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Different aerosol modes' influence on cloud processes remains controversial. As a result, we modified the aerosol spectrum and concentration to simulated a warm stratiform cloud process in Jiangxi, China by WRF-SBM scheme. Research shows that: different aerosol spectra have diverse effects on cloud droplet spectra, cloud development, and correlation between dispersion (ε) and cloud physics quantities. Compared to cloud droplet concentration, ε is more sensitive to the volume radius.
Andreas Bier, Simon Unterstrasser, Josef Zink, Dennis Hillenbrand, Tina Jurkat-Witschas, and Annemarie Lottermoser
Atmos. Chem. Phys., 24, 2319–2344, https://doi.org/10.5194/acp-24-2319-2024, https://doi.org/10.5194/acp-24-2319-2024, 2024
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Using hydrogen as aviation fuel affects contrails' climate impact. We study contrail formation behind aircraft with H2 combustion. Due to the absence of soot emissions, contrail ice crystals are assumed to form only on ambient particles mixed into the plume. The ice crystal number, which strongly varies with temperature and aerosol number density, is decreased by more than 80 %–90 % compared to kerosene contrails. However H2 contrails can form at lower altitudes due to higher H2O emissions.
Prasanth Prabhakaran, Fabian Hoffmann, and Graham Feingold
Atmos. Chem. Phys., 24, 1919–1937, https://doi.org/10.5194/acp-24-1919-2024, https://doi.org/10.5194/acp-24-1919-2024, 2024
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In this study, we explore the impact of deliberate aerosol perturbation in the northeast Pacific region using large-eddy simulations. Our results show that cloud reflectivity is sensitive to the aerosol sprayer arrangement in the pristine system, whereas in the polluted system it is largely proportional to the total number of aerosol particles injected. These insights would aid in assessing the efficiency of various aerosol injection strategies for climate intervention applications.
Lisa Bock and Axel Lauer
Atmos. Chem. Phys., 24, 1587–1605, https://doi.org/10.5194/acp-24-1587-2024, https://doi.org/10.5194/acp-24-1587-2024, 2024
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Climate model simulations still show a large range of effective climate sensitivity (ECS) with high uncertainties. An important contribution to ECS is cloud climate feedback. We investigate the representation of cloud physical and radiative properties from Coupled Model Intercomparison Project models grouped by ECS. We compare the simulated cloud properties of today’s climate from three ECS groups and quantify how the projected changes in cloud properties and cloud radiative effects differ.
Leonie Villiger and Franziska Aemisegger
Atmos. Chem. Phys., 24, 957–976, https://doi.org/10.5194/acp-24-957-2024, https://doi.org/10.5194/acp-24-957-2024, 2024
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Three numerical simulations performed with an isotope-enabled weather forecast model are used to investigate the cloud–circulation coupling between shallow trade-wind cumulus clouds and atmospheric circulations on different scales. It is shown that stable water isotopes near cloud base in the tropics reflect (1) the diel cycle of the atmospheric circulation, which drives the formation and dissipation of clouds, and (2) changes in the large-scale circulation over the North Atlantic.
Renaud Falga and Chien Wang
Atmos. Chem. Phys., 24, 631–647, https://doi.org/10.5194/acp-24-631-2024, https://doi.org/10.5194/acp-24-631-2024, 2024
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The impact of urban land use on regional meteorology and rainfall during the Indian summer monsoon has been assessed in this study. Using a cloud-resolving model centered around Kolkata, we have shown that the urban heat island effect led to a rainfall enhancement via the amplification of convective activity, especially during the night. Furthermore, the results demonstrated that the kinetic effect of the city induced the initiation of a nighttime storm.
Dario Sperber and Klaus Gierens
Atmos. Chem. Phys., 23, 15609–15627, https://doi.org/10.5194/acp-23-15609-2023, https://doi.org/10.5194/acp-23-15609-2023, 2023
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A significant share of aviation's climate impact is due to persistent contrails. Avoiding their creation is a step toward sustainable air transportation. For this purpose, a reliable forecast of so-called ice-supersaturated regions is needed, which then allows one to plan aircraft routes without persistent contrails. Here, we propose a method that leads to the better prediction of ice-supersaturated regions.
Blaž Gasparini, Sylvia C. Sullivan, Adam B. Sokol, Bernd Kärcher, Eric Jensen, and Dennis L. Hartmann
Atmos. Chem. Phys., 23, 15413–15444, https://doi.org/10.5194/acp-23-15413-2023, https://doi.org/10.5194/acp-23-15413-2023, 2023
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Tropical cirrus clouds are essential for climate, but our understanding of these clouds is limited due to their dependence on a wide range of small- and large-scale climate processes. In this opinion paper, we review recent advances in the study of tropical cirrus clouds, point out remaining open questions, and suggest ways to resolve them.
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Short summary
Images of crystals within mid-latitude cirrus clouds are used to derive consistent ice physical and optical properties for a detailed cloud microphysics model, including size-dependent mass, projected area, and fall speed. Based on habits found, properties are derived for bullet rosettes, their aggregates, and crystals with irregular shapes. Derived bullet rosette fall speeds are substantially greater than reported in past studies, owing to differences in mass, area, or diameter representation.
Images of crystals within mid-latitude cirrus clouds are used to derive consistent ice physical...
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