Articles | Volume 15, issue 12
https://doi.org/10.5194/acp-15-6689-2015
https://doi.org/10.5194/acp-15-6689-2015
Research article
 | 
17 Jun 2015
Research article |  | 17 Jun 2015

Formaldehyde (HCHO) in air, snow, and interstitial air at Concordia (East Antarctic Plateau) in summer

S. Preunkert, M. Legrand, M. M. Frey, A. Kukui, J. Savarino, H. Gallée, M. King, B. Jourdain, W. Vicars, and D. Helmig

Related authors

Measurement Report: Changes of ammonia emissions since the 18th century in south-eastern Europe inferred from an Elbrus (Caucasus, Russia) ice core record
Michel Legrand, Mstislav Vorobyev, Daria Bokuchava, Stanislav Kutuzov, Andreas Plach, Andreas Stohl, Alexandra Khairedinova, Vladimir Mikhalenko, Maria Vinogradova, Sabine Eckhardt, and Susanne Preunkert
EGUsphere, https://doi.org/10.5194/egusphere-2024-1381,https://doi.org/10.5194/egusphere-2024-1381, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Impact of subsurface crevassing on the depth–age relationship of high-Alpine ice cores extracted at Col du Dôme between 1994 and 2012
Susanne Preunkert, Pascal Bohleber, Michel Legrand, Adrien Gilbert, Tobias Erhardt, Roland Purtschert, Lars Zipf, Astrid Waldner, Joseph R. McConnell, and Hubertus Fischer
The Cryosphere, 18, 2177–2194, https://doi.org/10.5194/tc-18-2177-2024,https://doi.org/10.5194/tc-18-2177-2024, 2024
Short summary
Accumulation rates over the past 260 years archived in Elbrus ice core, Caucasus
Vladimir Mikhalenko, Stanislav Kutuzov, Pavel Toropov, Michel Legrand, Sergey Sokratov, Gleb Chernyakov, Ivan Lavrentiev, Susanne Preunkert, Anna Kozachek, Mstislav Vorobiev, Aleksandra Khairedinova, and Vladimir Lipenkov
Clim. Past, 20, 237–255, https://doi.org/10.5194/cp-20-237-2024,https://doi.org/10.5194/cp-20-237-2024, 2024
Short summary
Consistent histories of anthropogenic western European air pollution preserved in different Alpine ice cores
Anja Eichler, Michel Legrand, Theo M. Jenk, Susanne Preunkert, Camilla Andersson, Sabine Eckhardt, Magnuz Engardt, Andreas Plach, and Margit Schwikowski
The Cryosphere, 17, 2119–2137, https://doi.org/10.5194/tc-17-2119-2023,https://doi.org/10.5194/tc-17-2119-2023, 2023
Short summary
Factors controlling atmospheric DMS and its oxidation products (MSA and nssSO42−) in the aerosol at Terra Nova Bay, Antarctica
Silvia Becagli, Elena Barbaro, Simone Bonamano, Laura Caiazzo, Alcide di Sarra, Matteo Feltracco, Paolo Grigioni, Jost Heintzenberg, Luigi Lazzara, Michel Legrand, Alice Madonia, Marco Marcelli, Chiara Melillo, Daniela Meloni, Caterina Nuccio, Giandomenico Pace, Ki-Tae Park, Suzanne Preunkert, Mirko Severi, Marco Vecchiato, Roberta Zangrando, and Rita Traversi
Atmos. Chem. Phys., 22, 9245–9263, https://doi.org/10.5194/acp-22-9245-2022,https://doi.org/10.5194/acp-22-9245-2022, 2022
Short summary

Related subject area

Subject: Gases | Research Activity: Field Measurements | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Deciphering anthropogenic and biogenic contributions to selected non-methane volatile organic compound emissions in an urban area
Arianna Peron, Martin Graus, Marcus Striednig, Christian Lamprecht, Georg Wohlfahrt, and Thomas Karl
Atmos. Chem. Phys., 24, 7063–7083, https://doi.org/10.5194/acp-24-7063-2024,https://doi.org/10.5194/acp-24-7063-2024, 2024
Short summary
Emission characteristics of reactive organic gases (ROGs) from industrial volatile chemical products (VCPs) in the Pearl River Delta (PRD), China
Sihang Wang, Bin Yuan, Xianjun He, Ru Cui, Xin Song, Yubin Chen, Caihong Wu, Chaomin Wang, Yibo Huangfu, Xiao-Bing Li, Boguang Wang, and Min Shao
Atmos. Chem. Phys., 24, 7101–7121, https://doi.org/10.5194/acp-24-7101-2024,https://doi.org/10.5194/acp-24-7101-2024, 2024
Short summary
Measurement report: Enhanced photochemical formation of formic and isocyanic acids in urban regions aloft – insights from tower-based online gradient measurements
Qing Yang, Xiao-Bing Li, Bin Yuan, Xiaoxiao Zhang, Yibo Huangfu, Lei Yang, Xianjun He, Jipeng Qi, and Min Shao
Atmos. Chem. Phys., 24, 6865–6882, https://doi.org/10.5194/acp-24-6865-2024,https://doi.org/10.5194/acp-24-6865-2024, 2024
Short summary
Sources of organic gases and aerosol particles and their roles in nighttime particle growth at a rural forested site in southwest Germany
Junwei Song, Harald Saathoff, Feng Jiang, Linyu Gao, Hengheng Zhang, and Thomas Leisner
Atmos. Chem. Phys., 24, 6699–6717, https://doi.org/10.5194/acp-24-6699-2024,https://doi.org/10.5194/acp-24-6699-2024, 2024
Short summary
Surface snow bromide and nitrate at Eureka, Canada, in early spring and implications for polar boundary layer chemistry
Xin Yang, Kimberly Strong, Alison S. Criscitiello, Marta Santos-Garcia, Kristof Bognar, Xiaoyi Zhao, Pierre Fogal, Kaley A. Walker, Sara M. Morris, and Peter Effertz
Atmos. Chem. Phys., 24, 5863–5886, https://doi.org/10.5194/acp-24-5863-2024,https://doi.org/10.5194/acp-24-5863-2024, 2024
Short summary

Cited articles

Albert, M. R. and Shultz, E. F.: Snow and firn properties and air–snow transport processes at Summit, Greenland, Atmos. Environ., 36, 2789–2797, https://doi.org/10.1016/S1352-2310(02)00119-X, 2002.
Atkinson, R., Baulch, D. L., Cox, R. A., Crowley, J. N., Hampson, R. F., Hynes, R. G., Jenkin, M. E., Rossi, M. J., Troe, J., and IUPAC Subcommittee: Evaluated kinetic and photochemical data for atmospheric chemistry: Volume II – gas phase reactions of organic species, Atmos. Chem. Phys., 6, 3625–4055, https://doi.org/10.5194/acp-6-3625-2006, 2006.
Atkinson, R., Baulch, D. L., Cox, R. A., Crowley, J. N., Hampson, R. F., Hynes, R. G., Jenkin, M. E., Rossi, M. J., and Troe, J.: Evaluated kinetic and photochemical data for atmospheric chemistry: Volume III – gas phase reactions of inorganic halogens, Atmos. Chem. Phys., 7, 981–1191, https://doi.org/10.5194/acp-7-981-2007, 2007.
Atkinson, R., Baulch, D. L., Cox, R. A., Crowley, J. N., Hampson, R. F., Hynes, R. G., Jenkin, M. E., Rossi, M. J., Troe, J., and Wallington, T. J.: Evaluated kinetic and photochemical data for atmospheric chemistry: Volume IV – gas phase reactions of organic halogen species, Atmos. Chem. Phys., 8, 4141–4496, https://doi.org/10.5194/acp-8-4141-2008, 2008.
Barret, M., Houdier, S., and Domine, F.: Thermodynamics of the Formaldehyde-Water and Formaldehyde-Ice Systems for atmospheric implications, J. Phys. Chem. A, 115, 307–317, https://doi.org/10.1021/jp108907u, 2011a.
Download
Short summary
During two austral summers HCHO was investigated in air, snow, and interstitial air at the Concordia site located on the East Antarctic Plateau. Snow emission fluxes were estimated to be around 1 to 2 and 3 to 5 x 10^12 molecules m-2 s-1 at night and at noon, respectively. Shading experiments suggest that the photochemical HCHO production in the snowpack at Concordia remains negligible. The mean HCHO level of 130pptv observed at 1m above the surface is quite well reproduced by 1-D simulations.
Altmetrics
Final-revised paper
Preprint