Articles | Volume 24, issue 2
https://doi.org/10.5194/acp-24-891-2024
https://doi.org/10.5194/acp-24-891-2024
Research article
 | 
22 Jan 2024
Research article |  | 22 Jan 2024

Contribution of intermediate-volatility organic compounds from on-road transport to secondary organic aerosol levels in Europe

Stella E. I. Manavi and Spyros N. Pandis

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A lumped species approach for the simulation of secondary organic aerosol production from intermediate-volatility organic compounds (IVOCs): application to road transport in PMCAMx-iv (v1.0)
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Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
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Cited articles

An, J., Huang, C., Huang, D., Qin, M., Liu, H., Yan, R., Qiao, L., Zhou, M., Li, Y., Zhu, S., Wang, Q., and Wang, H.: Sources of organic aerosols in eastern China: a modeling study with high-resolution intermediate-volatility and semivolatile organic compound emissions, Atmos. Chem. Phys., 23, 323–344, https://doi.org/10.5194/acp-23-323-2023, 2023. 
Barsanti, K. C., Carlton, A. G., and Chung, S. H.: Analyzing experimental data and model parameters: implications for predictions of SOA using chemical transport models, Atmos. Chem. Phys., 13, 12073–12088, https://doi.org/10.5194/acp-13-12073-2013, 2013. 
Carter, W. P. L.: SAPRC-99 mechanism files and associated programs and examples, https://intra.cert.ucr.edu/~carter/SAPRC99/index.htm (last access: 6 July 2023), 2010. 
Chan, A. W. H., Kautzman, K. E., Chhabra, P. S., Surratt, J. D., Chan, M. N., Crounse, J. D., Kürten, A., Wennberg, P. O., Flagan, R. C., and Seinfeld, J. H.: Secondary organic aerosol formation from photooxidation of naphthalene and alkylnaphthalenes: implications for oxidation of intermediate volatility organic compounds (IVOCs), Atmos. Chem. Phys., 9, 3049–3060, https://doi.org/10.5194/acp-9-3049-2009, 2009. 
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Organic vapors of intermediate volatility have often been neglected as sources of atmospheric organic aerosol. In this work we use a new approach for their simulation and quantify the contribution of these compounds emitted by transportation sources (gasoline and diesel vehicles) to particulate matter over Europe. The estimated secondary organic aerosol levels are on average 60 % higher than predicted by previous approaches. However, these estimates are probably lower limits.
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