Articles | Volume 22, issue 8
https://doi.org/10.5194/acp-22-5435-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-5435-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
25 Apr 2022
Research article |
| 25 Apr 2022
| 25 Apr 2022
Analyzing ozone variations and uncertainties at high latitudes during sudden stratospheric warming events using MERRA-2
Shima Bahramvash Shams
CORRESPONDING AUTHOR
Department of Civil and Environmental Engineering, Washington State University, Pullman, WA, United States
NCAR, National Center for Atmospheric Research, Boulder, CO, United
States
Von P. Walden
Department of Civil and Environmental Engineering, Washington State University, Pullman, WA, United States
James W. Hannigan
NCAR, National Center for Atmospheric Research, Boulder, CO, United
States
William J. Randel
NCAR, National Center for Atmospheric Research, Boulder, CO, United
States
Irina V. Petropavlovskikh
Cooperative Institute for Research in Environmental Sciences,
University of Colorado, Boulder, CO, USA
National Oceanic and Atmospheric Administration, Global Monitoring
Division, Boulder, CO, USA
Amy H. Butler
National Oceanic and Atmospheric Administration, Chemical Sciences
Laboratory, Boulder, CO, USA
Alvaro de la Cámara
Dept. Física de la Tierra y Astrofísica, Universidad
Complutense de Madrid, Madrid, Spain
Related authors
No articles found.
Roeland Van Malderen, Zhou Zang, Kai-Lan Chang, Robin Björklund, Owen R. Cooper, Jane Liu, Eliane Maillard Barras, Corinne Vigouroux, Irina Petropavlovskikh, Thierry Leblanc, Valérie Thouret, Pawel Wolff, Peter Effertz, Audrey Gaudel, David W. Tarasick, Herman G. J. Smit, Anne M. Thompson, Ryan M. Stauffer, Debra E. Kollonige, Deniz Poyraz, Gérard Ancellet, Marie-Renée De Backer, Matthias M. Frey, James W. Hannigan, José L. Hernandez, Bryan J. Johnson, Nicholas Jones, Rigel Kivi, Emmanuel Mahieu, Isamu Morino, Glen McConville, Katrin Müller, Isao Murata, Justus Notholt, Ankie Piters, Maxime Prignon, Richard Querel, Vincenzo Rizi, Dan Smale, Wolfgang Steinbrecht, Kimberly Strong, and Ralf Sussmann
Atmos. Chem. Phys., 25, 9905–9935, https://doi.org/10.5194/acp-25-9905-2025, https://doi.org/10.5194/acp-25-9905-2025, 2025
Short summary
Short summary
Tropospheric ozone is an important greenhouse gas and an air pollutant whose distribution and time variability are mainly governed by anthropogenic emissions and dynamics. In this paper, we assess regional trends of tropospheric ozone column amounts, based on two different approaches of merging or synthesizing ground-based observations and their trends within specific regions. Our findings clearly demonstrate regional trend differences but also consistently higher pre-COVID than post-COVID trends.
Yunqian Zhu, Hideharu Akiyoshi, Valentina Aquila, Elizabeth Asher, Ewa M. Bednarz, Slimane Bekki, Christoph Brühl, Amy H. Butler, Parker Case, Simon Chabrillat, Gabriel Chiodo, Margot Clyne, Peter R. Colarco, Sandip Dhomse, Lola Falletti, Eric Fleming, Ben Johnson, Andrin Jörimann, Mahesh Kovilakam, Gerbrand Koren, Ales Kuchar, Nicolas Lebas, Qing Liang, Cheng-Cheng Liu, Graham Mann, Michael Manyin, Marion Marchand, Olaf Morgenstern, Paul Newman, Luke D. Oman, Freja F. Østerstrøm, Yifeng Peng, David Plummer, Ilaria Quaglia, William Randel, Samuel Rémy, Takashi Sekiya, Stephen Steenrod, Timofei Sukhodolov, Simone Tilmes, Kostas Tsigaridis, Rei Ueyama, Daniele Visioni, Xinyue Wang, Shingo Watanabe, Yousuke Yamashita, Pengfei Yu, Wandi Yu, Jun Zhang, and Zhihong Zhuo
Geosci. Model Dev., 18, 5487–5512, https://doi.org/10.5194/gmd-18-5487-2025, https://doi.org/10.5194/gmd-18-5487-2025, 2025
Short summary
Short summary
To understand the climate impact of the 2022 Hunga volcanic eruption, we developed a climate model–observation comparison project. The paper describes the protocols and models that participate in the experiments. We designed several experiments to achieve our goals of this activity: (1) to evaluate the climate model performance and (2) to understand the Earth system responses to this eruption.
Ying Dai, Peter Hitchcock, Amy H. Butler, Chaim I. Garfinkel, and William J. M. Seviour
Weather Clim. Dynam., 6, 841–862, https://doi.org/10.5194/wcd-6-841-2025, https://doi.org/10.5194/wcd-6-841-2025, 2025
Short summary
Short summary
Using a new database of subseasonal to seasonal (S2S) forecasts, we find that with a successful forecast of the sudden stratospheric warming (SSW), S2S models can capture the European precipitation signals after the 2018 SSW several weeks in advance. The findings indicate that the stratosphere represents an important source of S2S predictability for precipitation over Europe and call for consideration of stratospheric variability in hydrological prediction at S2S timescales.
Blanca Ayarzagüena, Amy H. Butler, Peter Hitchcock, Chaim I. Garfinkel, Zac D. Lawrence, Wuhan Ning, Philip Rupp, Zheng Wu, Hilla Afargan-Gerstman, Natalia Calvo, Álvaro de la Cámara, Martin Jucker, Gerbrand Koren, Daniel De Maeseneire, Gloria L. Manney, Marisol Osman, Masakazu Taguchi, Cory Barton, Dong-Chang Hong, Yu-Kyung Hyun, Hera Kim, Jeff Knight, Piero Malguzzi, Daniele Mastrangelo, Jiyoung Oh, Inna Polichtchouk, Jadwiga H. Richter, Isla R. Simpson, Seok-Woo Son, Damien Specq, and Tim Stockdale
EGUsphere, https://doi.org/10.5194/egusphere-2025-3611, https://doi.org/10.5194/egusphere-2025-3611, 2025
This preprint is open for discussion and under review for Weather and Climate Dynamics (WCD).
Short summary
Short summary
Sudden Stratospheric Warmings (SSWs) are known to follow a sustained wave dissipation in the stratosphere, which depends on both the tropospheric and stratospheric states. However, the relative role of each state is still unclear. Using a new set of subseasonal to seasonal forecasts, we show that the stratospheric state does not drastically affect the precursors of three recent SSWs, but modulates the stratospheric wave activity, with impacts depending on SSW features.
Wanmin Gong, Stephen R. Beagley, Kenjiro Toyota, Henrik Skov, Jesper Heile Christensen, Alex Lupu, Diane Pendlebury, Junhua Zhang, Ulas Im, Yugo Kanaya, Alfonso Saiz-Lopez, Roberto Sommariva, Peter Effertz, John W. Halfacre, Nis Jepsen, Rigel Kivi, Theodore K. Koenig, Katrin Müller, Claus Nordstrøm, Irina Petropavlovskikh, Paul B. Shepson, William R. Simpson, Sverre Solberg, Ralf M. Staebler, David W. Tarasick, Roeland Van Malderen, and Mika Vestenius
Atmos. Chem. Phys., 25, 8355–8405, https://doi.org/10.5194/acp-25-8355-2025, https://doi.org/10.5194/acp-25-8355-2025, 2025
Short summary
Short summary
This study showed that the springtime O3 depletion plays a critical role in driving the surface O3 seasonal cycle in the central Arctic. The O3 depletion events, while occurring most notably within the lowest few hundred metres above the Arctic Ocean, can induce a 5–7 % loss in the pan-Arctic tropospheric O3 burden during springtime. The study also found enhancements in O3 and NOy (mostly peroxyacetyl nitrate) concentrations in the Arctic due to northern boreal wildfires, particularly at higher altitudes.
Roeland Van Malderen, Anne M. Thompson, Debra E. Kollonige, Ryan M. Stauffer, Herman G. J. Smit, Eliane Maillard Barras, Corinne Vigouroux, Irina Petropavlovskikh, Thierry Leblanc, Valérie Thouret, Pawel Wolff, Peter Effertz, David W. Tarasick, Deniz Poyraz, Gérard Ancellet, Marie-Renée De Backer, Stéphanie Evan, Victoria Flood, Matthias M. Frey, James W. Hannigan, José L. Hernandez, Marco Iarlori, Bryan J. Johnson, Nicholas Jones, Rigel Kivi, Emmanuel Mahieu, Glen McConville, Katrin Müller, Tomoo Nagahama, Justus Notholt, Ankie Piters, Natalia Prats, Richard Querel, Dan Smale, Wolfgang Steinbrecht, Kimberly Strong, and Ralf Sussmann
Atmos. Chem. Phys., 25, 7187–7225, https://doi.org/10.5194/acp-25-7187-2025, https://doi.org/10.5194/acp-25-7187-2025, 2025
Short summary
Short summary
Tropospheric ozone is an important greenhouse gas and is an air pollutant. The time variability of tropospheric ozone is mainly driven by anthropogenic emissions. In this paper, we study the distribution and time variability of ozone from harmonized ground-based observations from five different measurement techniques. Our findings provide clear standard references for atmospheric models and evolving tropospheric ozone satellite data for the 2000–2022 period.
Alexey Yu. Karpechko, Amy H. Butler, and Frederic Vitart
EGUsphere, https://doi.org/10.5194/egusphere-2025-2556, https://doi.org/10.5194/egusphere-2025-2556, 2025
Short summary
Short summary
We study how the knowledge of future tropical and stratospheric conditions could improve forecasts in winter remotely, via teleconnections, 3–6 weeks ahead. We find that the tropics improve forecasts of sea level pressure in subtropics, Europe, and North America. The stratosphere improves forecasts in high latitudes and Europe. Improvements are small for temperature and precipitation. Larger forecast ensembles than usually available for research are needed to predict teleconnection signals.
Ivan Ortega, James W. Hannigan, Bianca C. Baier, Kathryn McKain, and Dan Smale
Atmos. Meas. Tech., 18, 2353–2371, https://doi.org/10.5194/amt-18-2353-2025, https://doi.org/10.5194/amt-18-2353-2025, 2025
Short summary
Short summary
This study evaluates retrieval strategies for CH4 and N2O using high-resolution FTIR observations from Boulder, Colorado. By comparing results with independent AirCore and aircraft in situ measurements, the analysis validates retrieval accuracy and quantifies uncertainties. The findings highlight the benefits of updated spectroscopy and improved a priori profiles and highlight consistent agreement with in situ data.
Ewa M. Bednarz, Amy H. Butler, Xinyue Wang, Zhihong Zhuo, Wandi Yu, Georgiy Stenchikov, Matthew Toohey, and Yunqian Zhu
EGUsphere, https://doi.org/10.5194/egusphere-2025-1970, https://doi.org/10.5194/egusphere-2025-1970, 2025
Short summary
Short summary
Injection of sulfur and water vapour by the Hunga volcanic eruption significantly altered chemical composition and radiative budget of the stratosphere. Yet, whether the eruption could also affect surface climate, especially via indirect pathways, remains poorly understood. Here we investigate these effects using large ensembles of simulations with the CESM2(WACCM6) Earth system model.
Zhihong Zhuo, Xinyue Wang, Yunqian Zhu, Ewa M. Bednarz, Eric Fleming, Peter R. Colarco, Shingo Watanabe, David Plummer, Georgiy Stenchikov, William Randel, Adam Bourassa, Valentina Aquila, Takashi Sekiya, Mark R. Schoeberl, Simone Tilmes, Wandi Yu, Jun Zhang, Paul J. Kushner, and Francesco S. R. Pausata
EGUsphere, https://doi.org/10.5194/egusphere-2025-1505, https://doi.org/10.5194/egusphere-2025-1505, 2025
Short summary
Short summary
The 2022 Hunga eruption caused unprecedented stratospheric water injection, triggering unique atmospheric impacts. This study combines observations and model simulations, projecting a stratospheric water vapor anomaly lasting 4–7 years, with significant temperature variations and ozone depletion in the upper atmosphere lasting 7–10 years. These findings offer critical insights into the role of stratospheric water vapor in shaping climate and atmospheric chemistry.
Verónica Martínez-Andradas, Alvaro de la Cámara, Pablo Zurita-Gotor, François Lott, and Federico Serva
Weather Clim. Dynam., 6, 329–343, https://doi.org/10.5194/wcd-6-329-2025, https://doi.org/10.5194/wcd-6-329-2025, 2025
Short summary
Short summary
Global circulation model biases are present when simulating sudden stratospheric warmings (SSWs). These are important extreme phenomena that occur in the wintertime stratosphere, driven by the breaking of atmospheric waves. The present work shows that there is a large spread of the wave forcing during the development of SSWs in different models. In the mesosphere, gravity waves are found to force advection of the residual circulation, while planetary waves tend to decelerate the wind.
Irina Petropavlovskikh, Jeannette D. Wild, Kari Abromitis, Peter Effertz, Koji Miyagawa, Lawrence E. Flynn, Eliane Maillard Barras, Robert Damadeo, Glen McConville, Bryan Johnson, Patrick Cullis, Sophie Godin-Beekmann, Gerard Ancellet, Richard Querel, Roeland Van Malderen, and Daniel Zawada
Atmos. Chem. Phys., 25, 2895–2936, https://doi.org/10.5194/acp-25-2895-2025, https://doi.org/10.5194/acp-25-2895-2025, 2025
Short summary
Short summary
Observational records show that stratospheric ozone is recovering in accordance with the implementation of the Montreal Protocol and its amendments. Natural ozone variability complicates the detection of small trends. This study optimizes a statistical model fit in ground-station-based observational records by adding parameters that interpret seasonal and long-term changes in atmospheric circulation and airmass mixing, which reduces uncertainties in detecting the stratospheric ozone recovery.
Chaim I. Garfinkel, Zachary D. Lawrence, Amy H. Butler, Etienne Dunn-Sigouin, Irene Erner, Alexey Y. Karpechko, Gerbrand Koren, Marta Abalos, Blanca Ayarzagüena, David Barriopedro, Natalia Calvo, Alvaro de la Cámara, Andrew Charlton-Perez, Judah Cohen, Daniela I. V. Domeisen, Javier García-Serrano, Neil P. Hindley, Martin Jucker, Hera Kim, Robert W. Lee, Simon H. Lee, Marisol Osman, Froila M. Palmeiro, Inna Polichtchouk, Jian Rao, Jadwiga H. Richter, Chen Schwartz, Seok-Woo Son, Masakazu Taguchi, Nicholas L. Tyrrell, Corwin J. Wright, and Rachel W.-Y. Wu
Weather Clim. Dynam., 6, 171–195, https://doi.org/10.5194/wcd-6-171-2025, https://doi.org/10.5194/wcd-6-171-2025, 2025
Short summary
Short summary
Variability in the extratropical stratosphere and troposphere is coupled, and because of the longer timescales characteristic of the stratosphere, this allows for a window of opportunity for surface prediction. This paper assesses whether models used for operational prediction capture these coupling processes accurately. We find that most processes are too weak; however downward coupling from the lower stratosphere to the near surface is too strong.
Robin Björklund, Corinne Vigouroux, Peter Effertz, Omaira E. García, Alex Geddes, James Hannigan, Koji Miyagawa, Michael Kotkamp, Bavo Langerock, Gerald Nedoluha, Ivan Ortega, Irina Petropavlovskikh, Deniz Poyraz, Richard Querel, John Robinson, Hisako Shiona, Dan Smale, Penny Smale, Roeland Van Malderen, and Martine De Mazière
Atmos. Meas. Tech., 17, 6819–6849, https://doi.org/10.5194/amt-17-6819-2024, https://doi.org/10.5194/amt-17-6819-2024, 2024
Short summary
Short summary
Different ground-based ozone measurements from the last 2 decades at Lauder are compared to each other. We want to know why different trends have been observed in the stratosphere. Also, the quality and relevance of tropospheric datasets need to be evaluated. While remaining drifts are still present, our study explains roughly half of the differences in observed trends in previous studies and shows the necessity for continuous review and improvement of the measurements.
Thomas J. Ballinger, Kent Moore, Qinghua Ding, Amy H. Butler, James E. Overland, Richard L. Thoman, Ian Baxter, Zhe Li, and Edward Hanna
Weather Clim. Dynam., 5, 1473–1488, https://doi.org/10.5194/wcd-5-1473-2024, https://doi.org/10.5194/wcd-5-1473-2024, 2024
Short summary
Short summary
This study chronicles the meteorological conditions that led to the anomalous, tandem March 2023 ice melt event in the Labrador and Bering seas. A sudden stratospheric warming event initiated the development of an anticyclonic circulation pattern over the Greenland–Labrador region, while the La Niña background state supported ridging conditions over Alaska, both of which aided northward transport of warm, moist air and drove the concurrent sea ice melt extremes.
Kimberlee Dubé, Susann Tegtmeier, Adam Bourassa, Daniel Zawada, Douglas Degenstein, William Randel, Sean Davis, Michael Schwartz, Nathaniel Livesey, and Anne Smith
Atmos. Chem. Phys., 24, 12925–12941, https://doi.org/10.5194/acp-24-12925-2024, https://doi.org/10.5194/acp-24-12925-2024, 2024
Short summary
Short summary
Greenhouse gas emissions that warm the troposphere also result in stratospheric cooling. The cooling rate is difficult to quantify above 35 km due to a deficit of long-term observational data with high vertical resolution in this region. We use satellite observations from several instruments, including a new temperature product from OSIRIS, to show that the upper stratosphere, from 35–60 km, cooled by 0.5 to 1 K per decade over 2005–2021 and by 0.6 K per decade over 1979–2021.
Andrew O. Langford, Raul J. Alvarez II, Kenneth C. Aikin, Sunil Baidar, W. Alan Brewer, Steven S. Brown, Matthew M. Coggan, Patrick D. Cullis, Jessica Gilman, Georgios I. Gkatzelis, Detlev Helmig, Bryan J. Johnson, K. Emma Knowland, Rajesh Kumar, Aaron D. Lamplugh, Audra McClure-Begley, Brandi J. McCarty, Ann M. Middlebrook, Gabriele Pfister, Jeff Peischl, Irina Petropavlovskikh, Pamela S. Rickley, Andrew W. Rollins, Scott P. Sandberg, Christoph J. Senff, and Carsten Warneke
EGUsphere, https://doi.org/10.5194/egusphere-2024-1938, https://doi.org/10.5194/egusphere-2024-1938, 2024
Preprint withdrawn
Short summary
Short summary
High ozone (O3) formed by reactions of nitrogen oxides (NOx) and volatile organic compounds (VOCs) can harm human health and welfare. High O3 is usually associated with hot summer days, but under certain conditions, high O3 can also form under winter conditions. In this study, we describe a high O3 event that occurred in Colorado during the COVID-19 quarantine that was caused in part by the decrease in traffic, and in part by a shallow inversion created by descent of stratospheric air.
Zhongming Gao, Heping Liu, Dan Li, Bai Yang, Von Walden, Lei Li, and Ivan Bogoev
Atmos. Meas. Tech., 17, 4109–4120, https://doi.org/10.5194/amt-17-4109-2024, https://doi.org/10.5194/amt-17-4109-2024, 2024
Short summary
Short summary
Using data collected from three levels of a 62 m tower, we found that both the temperature variances and sensible heat flux obtained from sonic anemometers are consistently lower, by a few percent, compared to those from fine-wire thermocouples.
Luis F. Millán, Peter Hoor, Michaela I. Hegglin, Gloria L. Manney, Harald Boenisch, Paul Jeffery, Daniel Kunkel, Irina Petropavlovskikh, Hao Ye, Thierry Leblanc, and Kaley Walker
Atmos. Chem. Phys., 24, 7927–7959, https://doi.org/10.5194/acp-24-7927-2024, https://doi.org/10.5194/acp-24-7927-2024, 2024
Short summary
Short summary
In the Observed Composition Trends And Variability in the UTLS (OCTAV-UTLS) Stratosphere-troposphere Processes And their Role in Climate (SPARC) activity, we have mapped multiplatform ozone datasets into coordinate systems to systematically evaluate the influence of these coordinates on binned climatological variability. This effort unifies the work of studies that focused on individual coordinate system variability. Our goal was to create the most comprehensive assessment of this topic.
Kai-Lan Chang, Owen R. Cooper, Audrey Gaudel, Irina Petropavlovskikh, Peter Effertz, Gary Morris, and Brian C. McDonald
Atmos. Chem. Phys., 24, 6197–6218, https://doi.org/10.5194/acp-24-6197-2024, https://doi.org/10.5194/acp-24-6197-2024, 2024
Short summary
Short summary
A great majority of observational trend studies of free tropospheric ozone use sparsely sampled ozonesonde and aircraft measurements as reference data sets. A ubiquitous assumption is that trends are accurate and reliable so long as long-term records are available. We show that sampling bias due to sparse samples can persistently reduce the trend accuracy, and we highlight the importance of maintaining adequate frequency and continuity of observations.
Jean-François Müller, Trissevgeni Stavrakou, Glenn-Michael Oomen, Beata Opacka, Isabelle De Smedt, Alex Guenther, Corinne Vigouroux, Bavo Langerock, Carlos Augusto Bauer Aquino, Michel Grutter, James Hannigan, Frank Hase, Rigel Kivi, Erik Lutsch, Emmanuel Mahieu, Maria Makarova, Jean-Marc Metzger, Isamu Morino, Isao Murata, Tomoo Nagahama, Justus Notholt, Ivan Ortega, Mathias Palm, Amelie Röhling, Wolfgang Stremme, Kimberly Strong, Ralf Sussmann, Yao Té, and Alan Fried
Atmos. Chem. Phys., 24, 2207–2237, https://doi.org/10.5194/acp-24-2207-2024, https://doi.org/10.5194/acp-24-2207-2024, 2024
Short summary
Short summary
Formaldehyde observations from satellites can be used to constrain the emissions of volatile organic compounds, but those observations have biases. Using an atmospheric model, aircraft and ground-based remote sensing data, we quantify these biases, propose a correction to the data, and assess the consequence of this correction for the evaluation of emissions.
Victoria A. Flood, Kimberly Strong, Cynthia H. Whaley, Kaley A. Walker, Thomas Blumenstock, James W. Hannigan, Johan Mellqvist, Justus Notholt, Mathias Palm, Amelie N. Röhling, Stephen Arnold, Stephen Beagley, Rong-You Chien, Jesper Christensen, Makoto Deushi, Srdjan Dobricic, Xinyi Dong, Joshua S. Fu, Michael Gauss, Wanmin Gong, Joakim Langner, Kathy S. Law, Louis Marelle, Tatsuo Onishi, Naga Oshima, David A. Plummer, Luca Pozzoli, Jean-Christophe Raut, Manu A. Thomas, Svetlana Tsyro, and Steven Turnock
Atmos. Chem. Phys., 24, 1079–1118, https://doi.org/10.5194/acp-24-1079-2024, https://doi.org/10.5194/acp-24-1079-2024, 2024
Short summary
Short summary
It is important to understand the composition of the Arctic atmosphere and how it is changing. Atmospheric models provide simulations that can inform policy. This study examines simulations of CH4, CO, and O3 by 11 models. Model performance is assessed by comparing results matched in space and time to measurements from five high-latitude ground-based infrared spectrometers. This work finds that models generally underpredict the concentrations of these gases in the Arctic troposphere.
Davide Putero, Paolo Cristofanelli, Kai-Lan Chang, Gaëlle Dufour, Gregory Beachley, Cédric Couret, Peter Effertz, Daniel A. Jaffe, Dagmar Kubistin, Jason Lynch, Irina Petropavlovskikh, Melissa Puchalski, Timothy Sharac, Barkley C. Sive, Martin Steinbacher, Carlos Torres, and Owen R. Cooper
Atmos. Chem. Phys., 23, 15693–15709, https://doi.org/10.5194/acp-23-15693-2023, https://doi.org/10.5194/acp-23-15693-2023, 2023
Short summary
Short summary
We investigated the impact of societal restriction measures during the COVID-19 pandemic on surface ozone at 41 high-elevation sites worldwide. Negative ozone anomalies were observed for spring and summer 2020 for all of the regions considered. In 2021, negative anomalies continued for Europe and partially for the eastern US, while western US sites showed positive anomalies due to wildfires. IASI satellite data and the Carbon Monitor supported emission reductions as a cause of the anomalies.
Ewa M. Bednarz, Amy H. Butler, Daniele Visioni, Yan Zhang, Ben Kravitz, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 13665–13684, https://doi.org/10.5194/acp-23-13665-2023, https://doi.org/10.5194/acp-23-13665-2023, 2023
Short summary
Short summary
We use a state-of-the-art Earth system model and a set of stratospheric aerosol injection (SAI) strategies to achieve the same level of global mean surface cooling through different combinations of location and/or timing of the injection. We demonstrate that the choice of SAI strategy can lead to contrasting impacts on stratospheric and tropospheric temperatures, circulation, and chemistry (including stratospheric ozone), thereby leading to different impacts on regional surface climate.
Yunqian Zhu, Robert W. Portmann, Douglas Kinnison, Owen Brian Toon, Luis Millán, Jun Zhang, Holger Vömel, Simone Tilmes, Charles G. Bardeen, Xinyue Wang, Stephanie Evan, William J. Randel, and Karen H. Rosenlof
Atmos. Chem. Phys., 23, 13355–13367, https://doi.org/10.5194/acp-23-13355-2023, https://doi.org/10.5194/acp-23-13355-2023, 2023
Short summary
Short summary
The 2022 Hunga Tonga eruption injected a large amount of water into the stratosphere. Ozone depletion was observed inside the volcanic plume. Chlorine and water vapor injected by this eruption exceeded the normal range, which made the ozone chemistry during this event occur at a higher temperature than polar ozone depletion. Unlike polar ozone chemistry where chlorine nitrate is more important, hypochlorous acid plays a large role in the in-plume chlorine balance and heterogeneous processes.
Kimberlee Dubé, Susann Tegtmeier, Adam Bourassa, Daniel Zawada, Douglas Degenstein, Patrick E. Sheese, Kaley A. Walker, and William Randel
Atmos. Chem. Phys., 23, 13283–13300, https://doi.org/10.5194/acp-23-13283-2023, https://doi.org/10.5194/acp-23-13283-2023, 2023
Short summary
Short summary
This paper presents a technique for understanding the causes of long-term changes in stratospheric composition. By using N2O as a proxy for stratospheric circulation in the model used to calculated trends, it is possible to separate the effects of dynamics and chemistry on observed trace gas trends. We find that observed HCl increases are due to changes in the stratospheric circulation, as are O3 decreases above 30 hPa in the Northern Hemisphere.
Vitali Fioletov, Xiaoyi Zhao, Ihab Abboud, Michael Brohart, Akira Ogyu, Reno Sit, Sum Chi Lee, Irina Petropavlovskikh, Koji Miyagawa, Bryan J. Johnson, Patrick Cullis, John Booth, Glen McConville, and C. Thomas McElroy
Atmos. Chem. Phys., 23, 12731–12751, https://doi.org/10.5194/acp-23-12731-2023, https://doi.org/10.5194/acp-23-12731-2023, 2023
Short summary
Short summary
Stratospheric ozone within the Southern Hemisphere springtime polar vortex has been a subject of intense research since the discovery of the Antarctic ozone hole. The wintertime ozone in the vortex is less studied. We show that the recent wintertime ozone values over the South Pole were about 12 % below the pre-1980s level; i.e., the decline there was nearly twice as large as that over southern midlatitudes. Thus, wintertime ozone there can be used as an indicator of the ozone layer state.
Luis F. Millán, Gloria L. Manney, Harald Boenisch, Michaela I. Hegglin, Peter Hoor, Daniel Kunkel, Thierry Leblanc, Irina Petropavlovskikh, Kaley Walker, Krzysztof Wargan, and Andreas Zahn
Atmos. Meas. Tech., 16, 2957–2988, https://doi.org/10.5194/amt-16-2957-2023, https://doi.org/10.5194/amt-16-2957-2023, 2023
Short summary
Short summary
The determination of atmospheric composition trends in the upper troposphere and lower stratosphere (UTLS) is still highly uncertain. We present the creation of dynamical diagnostics to map several ozone datasets (ozonesondes, lidars, aircraft, and satellite measurements) in geophysically based coordinate systems. The diagnostics can also be used to analyze other greenhouse gases relevant to surface climate and UTLS chemistry.
Dillon Elsbury, Amy H. Butler, John R. Albers, Melissa L. Breeden, and Andrew O'Neil Langford
Atmos. Chem. Phys., 23, 5101–5117, https://doi.org/10.5194/acp-23-5101-2023, https://doi.org/10.5194/acp-23-5101-2023, 2023
Short summary
Short summary
One of the global hotspots where stratosphere-to-troposphere transport (STT) of ozone takes place is over Pacific North America (PNA). However, we do not know how or if STT over PNA will change in response to climate change. Using climate model experiments forced with
worst-casescenario Representative Concentration Pathway 8.5 climate change, we find that changes in net chemical production and transport of ozone in the lower stratosphere increase STT of ozone over PNA in the future.
Bryan J. Johnson, Patrick Cullis, John Booth, Irina Petropavlovskikh, Glen McConville, Birgit Hassler, Gary A. Morris, Chance Sterling, and Samuel Oltmans
Atmos. Chem. Phys., 23, 3133–3146, https://doi.org/10.5194/acp-23-3133-2023, https://doi.org/10.5194/acp-23-3133-2023, 2023
Short summary
Short summary
In 1986, soon after the discovery of the Antarctic ozone hole, NOAA began year-round ozonesonde observations at South Pole Station to measure vertical profiles of ozone and temperature from the surface to 35 km. Balloon-borne ozonesondes launched at this unique site allow for tracking all phases of the yearly springtime ozone hole beginning in late winter and after sunrise, when rapid ozone depletion begins over the South Pole throughout the month of September.
Cynthia H. Whaley, Kathy S. Law, Jens Liengaard Hjorth, Henrik Skov, Stephen R. Arnold, Joakim Langner, Jakob Boyd Pernov, Garance Bergeron, Ilann Bourgeois, Jesper H. Christensen, Rong-You Chien, Makoto Deushi, Xinyi Dong, Peter Effertz, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Greg Huey, Ulas Im, Rigel Kivi, Louis Marelle, Tatsuo Onishi, Naga Oshima, Irina Petropavlovskikh, Jeff Peischl, David A. Plummer, Luca Pozzoli, Jean-Christophe Raut, Tom Ryerson, Ragnhild Skeie, Sverre Solberg, Manu A. Thomas, Chelsea Thompson, Kostas Tsigaridis, Svetlana Tsyro, Steven T. Turnock, Knut von Salzen, and David W. Tarasick
Atmos. Chem. Phys., 23, 637–661, https://doi.org/10.5194/acp-23-637-2023, https://doi.org/10.5194/acp-23-637-2023, 2023
Short summary
Short summary
This study summarizes recent research on ozone in the Arctic, a sensitive and rapidly warming region. We find that the seasonal cycles of near-surface atmospheric ozone are variable depending on whether they are near the coast, inland, or at high altitude. Several global model simulations were evaluated, and we found that because models lack some of the ozone chemistry that is important for the coastal Arctic locations, they do not accurately simulate ozone there.
Eliane Maillard Barras, Alexander Haefele, René Stübi, Achille Jouberton, Herbert Schill, Irina Petropavlovskikh, Koji Miyagawa, Martin Stanek, and Lucien Froidevaux
Atmos. Chem. Phys., 22, 14283–14302, https://doi.org/10.5194/acp-22-14283-2022, https://doi.org/10.5194/acp-22-14283-2022, 2022
Short summary
Short summary
Intercomparisons of three Dobson and three Brewer spectrophotometers at Arosa/Davos, Switzerland, are used for the homogenization of the longest Umkehr ozone profiles time series worldwide. Dynamic linear modeling (DLM) reveals a significant positive trend after 2004 in the upper stratosphere, a persistent negative trend between 25 and 30 km in the middle stratosphere, and a negative trend at 20 km in the lower stratosphere, with different levels of significance depending on the dataset.
Kimberlee Dubé, Daniel Zawada, Adam Bourassa, Doug Degenstein, William Randel, David Flittner, Patrick Sheese, and Kaley Walker
Atmos. Meas. Tech., 15, 6163–6180, https://doi.org/10.5194/amt-15-6163-2022, https://doi.org/10.5194/amt-15-6163-2022, 2022
Short summary
Short summary
Satellite observations are important for monitoring changes in atmospheric composition. Here we describe an improved version of the NO2 retrieval for the Optical Spectrograph and InfraRed Imager System. The resulting NO2 profiles are compared to those from the Atmospheric Chemistry Experiment – Fourier Transform Spectrometer and the Stratospheric Aerosol and Gas Experiment III on the International Space Station. All datasets agree within 20 % throughout the stratosphere.
John R. Albers, Amy H. Butler, Andrew O. Langford, Dillon Elsbury, and Melissa L. Breeden
Atmos. Chem. Phys., 22, 13035–13048, https://doi.org/10.5194/acp-22-13035-2022, https://doi.org/10.5194/acp-22-13035-2022, 2022
Short summary
Short summary
Ozone transported from the stratosphere contributes to background ozone concentrations in the free troposphere and to surface ozone exceedance events that affect human health. The physical processes whereby the El Niño–Southern Oscillation (ENSO) modulates North American stratosphere-to-troposphere ozone transport during spring are documented, and the usefulness of ENSO for predicting ozone events that may cause exceedances in surface air quality standards are assessed.
Kostas Eleftheratos, John Kapsomenakis, Ilias Fountoulakis, Christos S. Zerefos, Patrick Jöckel, Martin Dameris, Alkiviadis F. Bais, Germar Bernhard, Dimitra Kouklaki, Kleareti Tourpali, Scott Stierle, J. Ben Liley, Colette Brogniez, Frédérique Auriol, Henri Diémoz, Stana Simic, Irina Petropavlovskikh, Kaisa Lakkala, and Kostas Douvis
Atmos. Chem. Phys., 22, 12827–12855, https://doi.org/10.5194/acp-22-12827-2022, https://doi.org/10.5194/acp-22-12827-2022, 2022
Short summary
Short summary
We present the future evolution of DNA-active ultraviolet (UV) radiation in view of increasing greenhouse gases (GHGs) and decreasing ozone depleting substances (ODSs). It is shown that DNA-active UV radiation might increase after 2050 between 50° N–50° S due to GHG-induced reductions in clouds and ozone, something that is likely not to happen at high latitudes, where DNA-active UV radiation will continue its downward trend mainly due to stratospheric ozone recovery from the reduction in ODSs.
Sophie Godin-Beekmann, Niramson Azouz, Viktoria F. Sofieva, Daan Hubert, Irina Petropavlovskikh, Peter Effertz, Gérard Ancellet, Doug A. Degenstein, Daniel Zawada, Lucien Froidevaux, Stacey Frith, Jeannette Wild, Sean Davis, Wolfgang Steinbrecht, Thierry Leblanc, Richard Querel, Kleareti Tourpali, Robert Damadeo, Eliane Maillard Barras, René Stübi, Corinne Vigouroux, Carlo Arosio, Gerald Nedoluha, Ian Boyd, Roeland Van Malderen, Emmanuel Mahieu, Dan Smale, and Ralf Sussmann
Atmos. Chem. Phys., 22, 11657–11673, https://doi.org/10.5194/acp-22-11657-2022, https://doi.org/10.5194/acp-22-11657-2022, 2022
Short summary
Short summary
An updated evaluation up to 2020 of stratospheric ozone profile long-term trends at extrapolar latitudes based on satellite and ground-based records is presented. Ozone increase in the upper stratosphere is confirmed, with significant trends at most latitudes. In this altitude region, a very good agreement is found with trends derived from chemistry–climate model simulations. Observed and modelled trends diverge in the lower stratosphere, but the differences are non-significant.
Heather Guy, David D. Turner, Von P. Walden, Ian M. Brooks, and Ryan R. Neely
Atmos. Meas. Tech., 15, 5095–5115, https://doi.org/10.5194/amt-15-5095-2022, https://doi.org/10.5194/amt-15-5095-2022, 2022
Short summary
Short summary
Fog formation is highly sensitive to near-surface temperatures and humidity profiles. Passive remote sensing instruments can provide continuous measurements of the vertical temperature and humidity profiles and liquid water content, which can improve fog forecasts. Here we compare the performance of collocated infrared and microwave remote sensing instruments and demonstrate that the infrared instrument is especially sensitive to the onset of thin radiation fog.
Zachary D. Lawrence, Marta Abalos, Blanca Ayarzagüena, David Barriopedro, Amy H. Butler, Natalia Calvo, Alvaro de la Cámara, Andrew Charlton-Perez, Daniela I. V. Domeisen, Etienne Dunn-Sigouin, Javier García-Serrano, Chaim I. Garfinkel, Neil P. Hindley, Liwei Jia, Martin Jucker, Alexey Y. Karpechko, Hera Kim, Andrea L. Lang, Simon H. Lee, Pu Lin, Marisol Osman, Froila M. Palmeiro, Judith Perlwitz, Inna Polichtchouk, Jadwiga H. Richter, Chen Schwartz, Seok-Woo Son, Irene Erner, Masakazu Taguchi, Nicholas L. Tyrrell, Corwin J. Wright, and Rachel W.-Y. Wu
Weather Clim. Dynam., 3, 977–1001, https://doi.org/10.5194/wcd-3-977-2022, https://doi.org/10.5194/wcd-3-977-2022, 2022
Short summary
Short summary
Forecast models that are used to predict weather often struggle to represent the Earth’s stratosphere. This may impact their ability to predict surface weather weeks in advance, on subseasonal-to-seasonal (S2S) timescales. We use data from many S2S forecast systems to characterize and compare the stratospheric biases present in such forecast models. These models have many similar stratospheric biases, but they tend to be worse in systems with low model tops located within the stratosphere.
Peter Hitchcock, Amy Butler, Andrew Charlton-Perez, Chaim I. Garfinkel, Tim Stockdale, James Anstey, Dann Mitchell, Daniela I. V. Domeisen, Tongwen Wu, Yixiong Lu, Daniele Mastrangelo, Piero Malguzzi, Hai Lin, Ryan Muncaster, Bill Merryfield, Michael Sigmond, Baoqiang Xiang, Liwei Jia, Yu-Kyung Hyun, Jiyoung Oh, Damien Specq, Isla R. Simpson, Jadwiga H. Richter, Cory Barton, Jeff Knight, Eun-Pa Lim, and Harry Hendon
Geosci. Model Dev., 15, 5073–5092, https://doi.org/10.5194/gmd-15-5073-2022, https://doi.org/10.5194/gmd-15-5073-2022, 2022
Short summary
Short summary
This paper describes an experimental protocol focused on sudden stratospheric warmings to be carried out by subseasonal forecast modeling centers. These will allow for inter-model comparisons of these major disruptions to the stratospheric polar vortex and their impacts on the near-surface flow. The protocol will lead to new insights into the contribution of the stratosphere to subseasonal forecast skill and new approaches to the dynamical attribution of extreme events.
Noah Bernays, Daniel A. Jaffe, Irina Petropavlovskikh, and Peter Effertz
Atmos. Meas. Tech., 15, 3189–3192, https://doi.org/10.5194/amt-15-3189-2022, https://doi.org/10.5194/amt-15-3189-2022, 2022
Short summary
Short summary
Ozone is an important pollutant that impacts millions of people worldwide. It is therefore important to ensure accurate measurements. A recent surge in wildfire activity in the USA has resulted in significant enhancements in ozone concentration. However given the nature of wildfire smoke, there are questions about our ability to accurately measure ozone. In this comment, we discuss possible biases in the UV measurements of ozone in the presence of smoke.
Irina Petropavlovskikh, Koji Miyagawa, Audra McClure-Beegle, Bryan Johnson, Jeannette Wild, Susan Strahan, Krzysztof Wargan, Richard Querel, Lawrence Flynn, Eric Beach, Gerard Ancellet, and Sophie Godin-Beekmann
Atmos. Meas. Tech., 15, 1849–1870, https://doi.org/10.5194/amt-15-1849-2022, https://doi.org/10.5194/amt-15-1849-2022, 2022
Short summary
Short summary
The Montreal Protocol and its amendments assure the recovery of the stratospheric ozone layer that protects the Earth from harmful ultraviolet radiation. To monitor ozone recovery, multiple satellites and ground-based observational platforms collect ozone data. The changes in instruments can influence the continuation of the ozone data. We discuss a method to remove instrumental artifacts from ozone records to improve the internal consistency among multiple observational records.
Adam A. Scaife, Mark P. Baldwin, Amy H. Butler, Andrew J. Charlton-Perez, Daniela I. V. Domeisen, Chaim I. Garfinkel, Steven C. Hardiman, Peter Haynes, Alexey Yu Karpechko, Eun-Pa Lim, Shunsuke Noguchi, Judith Perlwitz, Lorenzo Polvani, Jadwiga H. Richter, John Scinocca, Michael Sigmond, Theodore G. Shepherd, Seok-Woo Son, and David W. J. Thompson
Atmos. Chem. Phys., 22, 2601–2623, https://doi.org/10.5194/acp-22-2601-2022, https://doi.org/10.5194/acp-22-2601-2022, 2022
Short summary
Short summary
Great progress has been made in computer modelling and simulation of the whole climate system, including the stratosphere. Since the late 20th century we also gained a much clearer understanding of how the stratosphere interacts with the lower atmosphere. The latest generation of numerical prediction systems now explicitly represents the stratosphere and its interaction with surface climate, and here we review its role in long-range predictions and projections from weeks to decades ahead.
Andrew O. Langford, Christoph J. Senff, Raul J. Alvarez II, Ken C. Aikin, Sunil Baidar, Timothy A. Bonin, W. Alan Brewer, Jerome Brioude, Steven S. Brown, Joel D. Burley, Dani J. Caputi, Stephen A. Conley, Patrick D. Cullis, Zachary C. J. Decker, Stéphanie Evan, Guillaume Kirgis, Meiyun Lin, Mariusz Pagowski, Jeff Peischl, Irina Petropavlovskikh, R. Bradley Pierce, Thomas B. Ryerson, Scott P. Sandberg, Chance W. Sterling, Ann M. Weickmann, and Li Zhang
Atmos. Chem. Phys., 22, 1707–1737, https://doi.org/10.5194/acp-22-1707-2022, https://doi.org/10.5194/acp-22-1707-2022, 2022
Short summary
Short summary
The Fires, Asian, and Stratospheric Transport–Las Vegas Ozone Study (FAST-LVOS) combined lidar, aircraft, and in situ measurements with global models to investigate the contributions of stratospheric intrusions, regional and Asian pollution, and wildfires to background ozone in the southwestern US during May and June 2017 and demonstrated that these processes contributed to background ozone levels that exceeded 70 % of the US National Ambient Air Quality Standard during the 6-week campaign.
William J. Randel, Fei Wu, Alison Ming, and Peter Hitchcock
Atmos. Chem. Phys., 21, 18531–18542, https://doi.org/10.5194/acp-21-18531-2021, https://doi.org/10.5194/acp-21-18531-2021, 2021
Short summary
Short summary
Balloon and satellite observations show strong coupling between large-scale ozone and temperature fields in the tropical lower stratosphere, spanning timescales of days to years. We present a simple interpretation of this behavior based on an idealized model of transport by the tropical stratospheric circulation, and good quantitative agreement with observations demonstrates that this is a useful simplification. The results provide simple understanding of observed atmospheric behavior.
Heather Guy, Ian M. Brooks, Ken S. Carslaw, Benjamin J. Murray, Von P. Walden, Matthew D. Shupe, Claire Pettersen, David D. Turner, Christopher J. Cox, William D. Neff, Ralf Bennartz, and Ryan R. Neely III
Atmos. Chem. Phys., 21, 15351–15374, https://doi.org/10.5194/acp-21-15351-2021, https://doi.org/10.5194/acp-21-15351-2021, 2021
Short summary
Short summary
We present the first full year of surface aerosol number concentration measurements from the central Greenland Ice Sheet. Aerosol concentrations here have a distinct seasonal cycle from those at lower-altitude Arctic sites, which is driven by large-scale atmospheric circulation. Our results can be used to help understand the role aerosols might play in Greenland surface melt through the modification of cloud properties. This is crucial in a rapidly changing region where observations are sparse.
Mahesh Kumar Sha, Bavo Langerock, Jean-François L. Blavier, Thomas Blumenstock, Tobias Borsdorff, Matthias Buschmann, Angelika Dehn, Martine De Mazière, Nicholas M. Deutscher, Dietrich G. Feist, Omaira E. García, David W. T. Griffith, Michel Grutter, James W. Hannigan, Frank Hase, Pauli Heikkinen, Christian Hermans, Laura T. Iraci, Pascal Jeseck, Nicholas Jones, Rigel Kivi, Nicolas Kumps, Jochen Landgraf, Alba Lorente, Emmanuel Mahieu, Maria V. Makarova, Johan Mellqvist, Jean-Marc Metzger, Isamu Morino, Tomoo Nagahama, Justus Notholt, Hirofumi Ohyama, Ivan Ortega, Mathias Palm, Christof Petri, David F. Pollard, Markus Rettinger, John Robinson, Sébastien Roche, Coleen M. Roehl, Amelie N. Röhling, Constantina Rousogenous, Matthias Schneider, Kei Shiomi, Dan Smale, Wolfgang Stremme, Kimberly Strong, Ralf Sussmann, Yao Té, Osamu Uchino, Voltaire A. Velazco, Corinne Vigouroux, Mihalis Vrekoussis, Pucai Wang, Thorsten Warneke, Tyler Wizenberg, Debra Wunch, Shoma Yamanouchi, Yang Yang, and Minqiang Zhou
Atmos. Meas. Tech., 14, 6249–6304, https://doi.org/10.5194/amt-14-6249-2021, https://doi.org/10.5194/amt-14-6249-2021, 2021
Short summary
Short summary
This paper presents, for the first time, Sentinel-5 Precursor methane and carbon monoxide validation results covering a period from November 2017 to September 2020. For this study, we used global TCCON and NDACC-IRWG network data covering a wide range of atmospheric and surface conditions across different terrains. We also show the influence of a priori alignment, smoothing uncertainties and the sensitivity of the validation results towards the application of advanced co-location criteria.
Amy H. Butler and Daniela I. V. Domeisen
Weather Clim. Dynam., 2, 453–474, https://doi.org/10.5194/wcd-2-453-2021, https://doi.org/10.5194/wcd-2-453-2021, 2021
Short summary
Short summary
We classify by wave geometry the stratospheric polar vortex during the final warming that occurs every spring in both hemispheres due to a combination of radiative and dynamical processes. We show that the shape of the vortex, as well as the timing of the seasonal transition, is linked to total column ozone prior to and surface weather following the final warming. These results have implications for prediction and our understanding of stratosphere–troposphere coupling processes in springtime.
John R. Albers, Amy H. Butler, Melissa L. Breeden, Andrew O. Langford, and George N. Kiladis
Weather Clim. Dynam., 2, 433–452, https://doi.org/10.5194/wcd-2-433-2021, https://doi.org/10.5194/wcd-2-433-2021, 2021
Short summary
Short summary
Weather variability controls the transport of ozone from the stratosphere to the Earth’s surface and water vapor from oceanic source regions to continental land masses. Forecasting these types of transport has high societal value because of the negative impacts of ozone on human health and the role of water vapor in governing precipitation variability. We use upper-level wind forecasts to assess the potential for predicting ozone and water vapor transport 3–6 weeks ahead of time.
Antara Banerjee, Amy H. Butler, Lorenzo M. Polvani, Alan Robock, Isla R. Simpson, and Lantao Sun
Atmos. Chem. Phys., 21, 6985–6997, https://doi.org/10.5194/acp-21-6985-2021, https://doi.org/10.5194/acp-21-6985-2021, 2021
Short summary
Short summary
We find that simulated stratospheric sulfate geoengineering could lead to warmer Eurasian winters alongside a drier Mediterranean and wetting to the north. These effects occur due to the strengthening of the Northern Hemisphere stratospheric polar vortex, which shifts the North Atlantic Oscillation to a more positive phase. We find the effects in our simulations to be much more significant than the wintertime effects of large tropical volcanic eruptions which inject much less sulfate aerosol.
Melissa L. Breeden, Amy H. Butler, John R. Albers, Michael Sprenger, and Andrew O'Neil Langford
Atmos. Chem. Phys., 21, 2781–2794, https://doi.org/10.5194/acp-21-2781-2021, https://doi.org/10.5194/acp-21-2781-2021, 2021
Short summary
Short summary
Prior research has found a maximum in deep stratosphere-to-troposphere mass/ozone transport over the western United States in boreal spring, which can enhance surface ozone concentrations, reducing air quality. We find that the winter-to-summer evolution of the north Pacific jet increases the frequency of stratospheric intrusions that drive transport, helping explain the observed maximum. The El Niño–Southern Oscillation affects the timing of the spring jet transition and therefore transport.
Thomas Blumenstock, Frank Hase, Axel Keens, Denis Czurlok, Orfeo Colebatch, Omaira Garcia, David W. T. Griffith, Michel Grutter, James W. Hannigan, Pauli Heikkinen, Pascal Jeseck, Nicholas Jones, Rigel Kivi, Erik Lutsch, Maria Makarova, Hamud K. Imhasin, Johan Mellqvist, Isamu Morino, Tomoo Nagahama, Justus Notholt, Ivan Ortega, Mathias Palm, Uwe Raffalski, Markus Rettinger, John Robinson, Matthias Schneider, Christian Servais, Dan Smale, Wolfgang Stremme, Kimberly Strong, Ralf Sussmann, Yao Té, and Voltaire A. Velazco
Atmos. Meas. Tech., 14, 1239–1252, https://doi.org/10.5194/amt-14-1239-2021, https://doi.org/10.5194/amt-14-1239-2021, 2021
Short summary
Short summary
This study investigates the level of channeling (optical resonances) of each FTIR spectrometer within the Network for the Detection of Atmospheric Composition Change (NDACC). Since the air gap of the beam splitter is a significant source of channeling, we propose new beam splitters with an increased wedge of the air gap. This study shows the potential for reducing channeling in the FTIR spectrometers operated by the NDACC, thereby increasing the quality of recorded spectra across the network.
Kimberlee Dubé, Adam Bourassa, Daniel Zawada, Douglas Degenstein, Robert Damadeo, David Flittner, and William Randel
Atmos. Meas. Tech., 14, 557–566, https://doi.org/10.5194/amt-14-557-2021, https://doi.org/10.5194/amt-14-557-2021, 2021
Short summary
Short summary
SAGE III/ISS measures profiles of NO2; however the algorithm to convert raw measurements to NO2 concentration neglects variations caused by changes in chemistry over the course of a day. We devised a procedure to account for these diurnal variations and assess their impact on NO2 measurements from SAGE III/ISS. We find that the new NO2 concentration is more than 10 % lower than NO2 from the standard algorithm below 30 km, showing that this effect is important to consider at lower altitudes.
Xin Yang, Anne-M. Blechschmidt, Kristof Bognar, Audra McClure-Begley, Sara Morris, Irina Petropavlovskikh, Andreas Richter, Henrik Skov, Kimberly Strong, David W. Tarasick, Taneil Uttal, Mika Vestenius, and Xiaoyi Zhao
Atmos. Chem. Phys., 20, 15937–15967, https://doi.org/10.5194/acp-20-15937-2020, https://doi.org/10.5194/acp-20-15937-2020, 2020
Short summary
Short summary
This is a modelling-based study on Arctic surface ozone, with a particular focus on spring ozone depletion events (i.e. with concentrations < 10 ppbv). Model experiments show that model runs with blowing-snow-sourced sea salt aerosols implemented as a source of reactive bromine can reproduce well large-scale ozone depletion events observed in the Arctic. This study supplies modelling evidence of the proposed mechanism of reactive-bromine release from blowing snow on sea ice (Yang et al., 2008).
Erik Lutsch, Kimberly Strong, Dylan B. A. Jones, Thomas Blumenstock, Stephanie Conway, Jenny A. Fisher, James W. Hannigan, Frank Hase, Yasuko Kasai, Emmanuel Mahieu, Maria Makarova, Isamu Morino, Tomoo Nagahama, Justus Notholt, Ivan Ortega, Mathias Palm, Anatoly V. Poberovskii, Ralf Sussmann, and Thorsten Warneke
Atmos. Chem. Phys., 20, 12813–12851, https://doi.org/10.5194/acp-20-12813-2020, https://doi.org/10.5194/acp-20-12813-2020, 2020
Short summary
Short summary
This paper describes the use of a network of 10 Arctic and midlatitude ground-based FTIR measurement sites to detect enhancements of the wildfire tracers carbon monoxide, hydrogen cyanide, and ethane from 2003 to 2018. A tagged CO GEOS-Chem simulation is used for source attribution and to evaluate the relative contribution of CO sources to the FTIR measurements. The use of FTIR measurements allowed for the emission ratios of hydrogen cyanide and ethane to be quantified.
Li Zhang, Meiyun Lin, Andrew O. Langford, Larry W. Horowitz, Christoph J. Senff, Elizabeth Klovenski, Yuxuan Wang, Raul J. Alvarez II, Irina Petropavlovskikh, Patrick Cullis, Chance W. Sterling, Jeff Peischl, Thomas B. Ryerson, Steven S. Brown, Zachary C. J. Decker, Guillaume Kirgis, and Stephen Conley
Atmos. Chem. Phys., 20, 10379–10400, https://doi.org/10.5194/acp-20-10379-2020, https://doi.org/10.5194/acp-20-10379-2020, 2020
Short summary
Short summary
Measuring and quantifying the sources of elevated springtime ozone in the southwestern US is challenging but relevant to the implications for control policy. Here we use intensive field measurements and two global models to study ozone sources in the region. We find that ozone from the stratosphere, wildfires, and Asia is an important source of high-ozone events in the region. Our analysis also helps understand the uncertainties in ozone simulations with individual models.
Cited articles
Albers, J. R., Perlwitz, J., Butler, A. H., Birner, T., Kiladis, G. N.,
Lawrence, Z. D., Manney, G. L., Langford, A. O., and Dias, J.: Mechanisms
Governing Interannual Variability of Stratosphere-to-Troposphere Ozone
Transport, J. Geophys. Res., 123, 234–260,
https://doi.org/10.1002/2017jd026890, 2018.
Ancellet, G., Daskalakis, N., Raut, J. C., Tarasick, D., Hair, J., Quennehen, B., Ravetta, F., Schlager, H., Weinheimer, A. J., Thompson, A. M., Johnson, B., Thomas, J. L., and Law, K. S.: Analysis of the latitudinal variability of tropospheric ozone in the Arctic using the large number of aircraft and ozonesonde observations in early summer 2008, Atmos. Chem. Phys., 16, 13341–13358, https://doi.org/10.5194/acp-16-13341-2016, 2016.
Andrews, D. G., Holton, J. R., and Leovy, C. B.: Middle atmosphere dynamics,
Academic Press, edited by: Holton, J. R. and Dmowska, R., ISBN 13: 9780120585762, 1987.
Anstey, J. A. and Shepherd, T. G.: High-latitude influence of the
quasi-biennial oscillation, Q. J. Roy. Meteor. Soc., 1, 1–21,
https://doi.org/10.1002/qj.2132, 2014.
Ayarzagüena, B., Polvani, L. M., Langematz, U., Akiyoshi, H., Bekki, S., Butchart, N., Dameris, M., Deushi, M., Hardiman, S. C., Jöckel, P., Klekociuk, A., Marchand, M., Michou, M., Morgenstern, O., O'Connor, F. M., Oman, L. D., Plummer, D. A., Revell, L., Rozanov, E., Saint-Martin, D., Scinocca, J., Stenke, A., Stone, K., Yamashita, Y., Yoshida, K., and Zeng, G.: No robust evidence of future changes in major stratospheric sudden warmings: a multi-model assessment from CCMI, Atmos. Chem. Phys., 18, 11277–11287, https://doi.org/10.5194/acp-18-11277-2018, 2018.
Ayarzagüena, B., Charlton-Perez, A. J., Butler, A. H., Hitchcock, P.,
Simpson, I. R., Polvani, L. M., Butchart, N., Gerber, E. P., Gray, L.,
Hassler, B., Lin, P., Lott, F., Manzini, E., Mizuta, R., Orbe, C., Osprey,
S., Saint-Martin, D., Sigmond, M., Taguchi, M., Volodin, E. M., and
Watanabe, S.: Uncertainty in the Response of Sudden Stratospheric Warmings
and Stratosphere-Troposphere Coupling to Quadrupled CO2 Concentrations in
CMIP6 Models, J Geophys. Res.-Atmos., 125, e2019JD032345, https://doi.org/10.1029/2019jd032345, 2020.
Bahramvash Shams, S., Walden, V. P., Petropavlovskikh, I., Tarasick, D., Kivi, R., Oltmans, S., Johnson, B., Cullis, P., Sterling, C. W., Thölix, L., and Errera, Q.: Variations in the vertical profile of ozone at four high-latitude Arctic sites from 2005 to 2017, Atmos. Chem. Phys., 19, 9733–9751, https://doi.org/10.5194/acp-19-9733-2019, 2019.
Bahramvash Shams, S.: Analyzing Ozone and dynamical transport variables in middle stratosphere using MERRA-2 data (Jupiter notebook), Zenodo [code], https://doi.org/10.5281/zenodo.6466540, 2022.
Baldwin, M. P. and Dunkerton, T. J.: Stratospheric Harbingers of Anomalous
Weather Regimes, Science, 294, 581–584,
https://doi.org/10.1126/science.1063315, 2001.
Baldwin, M. P., Ayarzagüena, B., Birner, T., Butchart, N., Butler, A.
H., Charlton-Perez, A. J., Domeisen, D. I. V., Garfinkel, C. I., Garny, H.,
Gerber, E. P., Hegglin, M. I., Langematz, U., and Pedatella, N. M.: Sudden
Stratospheric Warmings, Rev. Geophys., 59, 27.1–37,
https://doi.org/10.1029/2020rg000708, 2021.
Bognar, K., Zhao, X., Strong, K., Boone, C. D., Bourassa, A. E., Degenstein,
D. A., Drummond, J. R., Duff, A., Goutail, F., Griffin, D., Jeffery, P. S.,
Lutsch, E., Manney, G. L., McElroy, C. T., McLinden, C. A., Millán, L.
F., Pazmiño, A., Sioris, C. E., Walker, K. A., and Zou, J.: Updated
validation of ACE and OSIRIS ozone and NO2 measurements in the Arctic using
ground-based instruments at Eureka, Canada, J. Quant. Spectrosc. Ra., 238, 106571, https://doi.org/10.1016/j.jqsrt.2019.07.014, 2019.
Butler, A. H. and Domeisen, D. I. V.: The wave geometry of final stratospheric warming events, Weather Clim. Dynam., 2, 453–474, https://doi.org/10.5194/wcd-2-453-2021, 2021.
Butler, A. H., Seidel, D. J., Hardiman, S. C., Butchart, N., Birner, T., and
Match, A.: Defining Sudden Stratospheric Warmings, B. Am. Meteor. Soc.,
96, 1913–1928, https://doi.org/10.1175/bams-d-13-00173.1, 2015.
Butler, A. H., Sjoberg, J. P., Seidel, D. J., and Rosenlof, K. H.: A sudden stratospheric warming compendium, Earth Syst. Sci. Data, 9, 63–76, https://doi.org/10.5194/essd-9-63-2017, 2017.
Butler, A. H., Charlton-Perez, A., Domeisen, D. I. V., Garfinkel, C., Gerber, E. P., Hitchcock, P., Karpechko, A.-Y., Maycock, A. C., Sigmond, M., Simpson, I., and Son, S.-W.: Sub-seasonal Predictability and the Stratosphere, in: Chapter 11, The Gap Between Weather and Climate Forecasting, 223–241, https://doi.org/10.1016/B978-0-12-811714-9.00011-5, 2019.
Butler, A. H., Lawrence, Z. D., Lee, S. H., Lillo, S. P., and Long, C. S.:
Differences between the 2018 and 2019 stratospheric polar vortex split
events, Q. J. Roy. Meteor. Soc., 146, 3503–3521,
https://doi.org/10.1002/qj.3858, 2020.
Cagnazzo, C. and E. Manzini.: Impact of the Stratosphere on the Winter
Tropospheric Teleconnections between ENSO and the North Atlantic and
European Region, J. Climate, 22, 1223–1238, https://doi.org/10.1175/2008JCLI2549.1, 2009.
Calvo, N., Polvani, L. M., and Solomon, S.: On the surface impact of Arctic
stratospheric ozone extremes, Environ. Res. Lett., 10, 094003,
https://doi.org/10.1088/1748-9326/10/9/094003, 2015.
de la Cámara, A., Abalos, M., and Hitchcock, P.: Changes in
Stratospheric Transport and Mixing During Sudden Stratospheric Warmings, J.
Geophys. Res., 123, 3356–3373, https://doi.org/10.1002/2017jd028007, 2018a.
de la Cámara, A., Abalos, M., Hitchcock, P., Calvo, N., and Garcia, R. R.: Response of Arctic ozone to sudden stratospheric warmings, Atmos. Chem. Phys., 18, 16499–16513, https://doi.org/10.5194/acp-18-16499-2018, 2018b.
de la Cámara, A., Birner, T., and Albers, J. R.: Are Sudden
Stratospheric Warmings Preceded by Anomalous Tropospheric Wave Activity?, J.
Climate, 32, 7173–7189, https://doi.org/10.1175/jcli-d-19-0269.1, 2019.
Charlton, A. J. and Polvani, L. M.: A New Look at Stratospheric Sudden
Warmings. Part I: Climatology and Modeling Benchmarks, J. Climate, 20,
449–469, https://doi.org/10.1175/jcli3996.1, 2007.
Charlton-Perez, A. J., Ferranti, L., and Lee, R. W.: The influence of the
stratospheric state on North Atlantic weather regimes, Q. J. Roy. Meteor.
Soc., 144, 1140–1151, https://doi.org/10.1002/qj.3280, 2018.
Coy, L., Wargan, K., Molod, A. M., McCarty, W. R., and Pawson, S.: Structure
and Dynamics of the Quasi-Biennial Oscillation in MERRA-2, J. Climate, 29,
5339–5354, https://doi.org/10.1175/jcli-d-15-0809.1, 2016.
Davis, S. M., Hegglin, M. I., Fujiwara, M., Dragani, R., Harada, Y., Kobayashi, C., Long, C., Manney, G. L., Nash, E. R., Potter, G. L., Tegtmeier, S., Wang, T., Wargan, K., and Wright, J. S.: Assessment of upper tropospheric and stratospheric water vapor and ozone in reanalyses as part of S-RIP, Atmos. Chem. Phys., 17, 12743–12778, https://doi.org/10.5194/acp-17-12743-2017, 2017.
Dickinson, R. E.: Method of parameterization for infrared cooling between
altitudes of 30 and 70 kilometers, J. Geophys. Res., 78, 4451–4457,
https://doi.org/10.1029/jc078i021p04451, 1973.
Flury, T., Hocke, K., Haefele, A., Kämpfer, N., and Lehmann, R.: Ozone
depletion, water vapor increase, and PSC generation at midlatitudes by the
2008 major stratospheric warming, J. Geophys. Res., 114, 7903–14,
https://doi.org/10.1029/2009jd011940, 2009.
Fritts, D. C. and Alexander, M. J.: Gravity wave dynamics and effects in the
middle atmosphere, Rev. Geophys., 41, 1003,
https://doi.org/10.1029/2001rg000106, 2003.
Fusco, A. C. and Salby, M. L.: Interannual Variations of Total Ozone and
Their Relationship to Variations of Planetary Wave Activity, J. Climate, 12,
1619–1629, https://doi.org/10.1175/1520-0442(1999)012<1619:ivotoa>2.0.co;2, 1999.
García, O. E., Schneider, M., Redondas, A., González, Y., Hase, F., Blumenstock, T., and Sepúlveda, E.: Investigating the long-term evolution of subtropical ozone profiles applying ground-based FTIR spectrometry, Atmos. Meas. Tech., 5, 2917–2931, https://doi.org/10.5194/amt-5-2917-2012, 2012.
Gaudel, A., Ancellet, G., and Godin-Beekmann, S.: Analysis of 20 Years of
tropospheric ozone vertical profiles by lidar and ecc at observatoire de
Haute Provence (OHP) at 44∘ N, 6.7∘ E, Atmos. Environ., 113, 78–89,
https://doi.org/10.1016/j.atmosenv.2015.04.028, 2015.
Gelaro, R., McCarty, W., Suárez, M. J., Todling, R., Molod, A., Takacs,
L., Randles, C. A., Darmenov, A., Bosilovich, M. G., Reichle, R., Wargan,
K., Coy, L., Cullather, R., Draper, C., Akella, S., Buchard, V., Conaty, A.,
Silva, A. M. da, Gu, W., Kim, G.-K., Koster, R., Lucchesi, R., Merkova, D.,
Nielsen, J. E., Partyka, G., Pawson, S., Putman, W., Rienecker, M.,
Schubert, S. D., Sienkiewicz, M., and Zhao, B.: The Modern-Era Retrospective
Analysis for Research and Applications, Version 2 (MERRA-2), J. Climate, 30,
5419–5454, https://doi.org/10.1175/jcli-d-16-0758.1, 2017.
Global Modeling and Assimilation Office (GMAO), MERRA-2
inst3_3d_asm_Nv:
3d,3-Hourly,Instantaneous,Model-Level,Assimilation,Assimilated
Meteorological Fields V5.12.4, Greenbelt, MD, USA, Goddard Earth Sciences
Data and Information Services Center (GES DISC), https://doi.org/10.5067/WWQSXQ8IVFW8, 2015a.
Global Modeling and Assimilation Office (GMAO), MERRA-2 inst3_3d_asm_Np:
3d,3-Hourly,Instantaneous,Pressure-Level,Assimilation,Assimilated
Meteorological Fields V5.12.4, Greenbelt, MD, USA, Goddard Earth Sciences
Data and Information Services Center (GES DISC), https://doi.org/10.5067/QBZ6MG944HW0,
2015b.
Goncharenko, L. and Zhang, S.-R.: Ionospheric signatures of sudden
stratospheric warming: Ion temperature at middle latitude, Geophys. Res.
Lett., 35, L15804-4, https://doi.org/10.1029/2008gl035684, 2008.
Greening, K. and Hodgson, A.: Atmospheric analysis of the cold late February
and early March 2018 over the UK, Weather, 74, 79–85,
https://doi.org/10.1002/wea.3467, 2019.
Haigh, J. D.: The role of stratospheric ozone in modulating the solar
radiative forcing of climate, Nature, 370, 544–546,
https://doi.org/10.1038/370544a0, 1994.
Harada, Y., G. Atsushi, H. Hiroshi, and N. Fujikawa: A major stratospheric sudden warming event in January 2009, J. Atmos. Sci., 67, 2052–2069, https://doi.org/10.1175/2009JAS3320.1, 2010.
Hitchcock, P. and Simpson, I. R.: The Downward Influence of Stratospheric
Sudden Warmings, J. Atmos. Sci., 71, 3856–3876,
https://doi.org/10.1175/jas-d-14-0012.1, 2014.
Holton, J. R. and Lindzen, R. S.: An Updated Theory for the Quasi-Biennial
Cycle of the Tropical Stratosphere, J. Atmos. Sci., 29, 1076–1080,
https://doi.org/10.1175/1520-0469(1972)029<1076:autftq>2.0.co;2, 1972.
Holton, J. R., Haynes, P. H., McIntyre, M. E., Douglass, A. R., Rood, R. B.,
and Pfister, L.: Stratosphere-troposphere exchange, Rev. Geophys., 33,
403–439, https://doi.org/10.1029/95rg02097, 1995.
Houghton, J. T.: The stratosphere and mesosphere, Q. J. Roy. Meteor. Soc.,
104, 1–29, https://doi.org/10.1002/qj.49710443902, 1978.
Ineson, S., and A. A. Scaife.: The role of the stratosphere in the European
climate response to El Niño, Nat. Geosci., 2, 32–36, https://doi.org/10.1038/ngeo381, 2008.
Jaegleì, L., Wood, R., and Wargan, K.: Multiyear composite view of ozone
enhancements and stratosphere-to-troposphere transport in dry intrusions of
northern hemisphere extratropical cyclones, J. Geophys. Res.-Atmos.,
122, 13436–13457, https://doi.org/10.1002/2017JD027656, 2017.
Johnson, B. J., Oltmans, S. J., Vömel, H., Smit, H. G. J., Deshler, T.,
and Kröger, C.: Electrochemical concentration cell (ECC) ozonesonde pump
efficiency measurements and tests on the sensitivity to ozone of buffered
and unbuffered ECC sensor cathode solutions, J. Geophys. Res., 107, 7881,
https://doi.org/10.1029/2001jd000557, 2002.
Johnson, B. J., Cullis, P. D., and NOAA ESRL: Earth System Research Laboratory Ozone Water Vapor Group Ozonesonde Measurements, Version 1, NOAA National Centers for Environmental Information, https://doi.org/10.7289/V5CC0XZ1, 2018.
Karpechko, A. Y., Perlwitz, J., and Manzini, E.: A model study of
tropospheric impacts of the Arctic ozone depletion 2011, J. Geophys. Res.,
119, 7999–8014, https://doi.org/10.1002/2013jd021350, 2014.
Karpechko, A. Y., Perez, A. C., Balmaseda, M., Tyrrell, N., and Vitart, F.:
Predicting Sudden Stratospheric Warming 2018 and Its Climate Impacts With a
Multimodel Ensemble, Geophys. Res. Lett., 45, 13538–12546,
https://doi.org/10.1029/2018gl081091, 2018.
Kidston, J., Scaife, A. A., Hardiman, S. C., Mitchell, D. M., Butchart, N.,
Baldwin, M. P., and Gray, L. J.: Stratospheric influence on tropospheric jet
streams, storm tracks and surface weather, Nat. Geosci., 8, 1–8,
https://doi.org/10.1038/ngeo2424, 2015.
Knowland, K. E., Ott, L. E., Duncan, B. N., and Wargan, K.: Stratospheric
Intrusion-Influenced Ozone Air Quality Exceedances Investigated in the NASA
MERRA-2 Reanalysis, Geophys. Res. Lett., 44, 10691–10701,
https://doi.org/10.1002/2017gl074532, 2017.
Komhyr, W. D.: Operations handbook-ozone measurements to 40-km altitude with
Model 4A Electrochemical Concentration Cell (ECC) ozonesonaes (used with
1680-MHz radiosondes), U.S. Dept. of Commerce, National Oceanic and Atmospheric Administration, Environmental Research Laboratories, Air Resources Laboratory, 1986.
Korenkov, Y. N., Klimenko, V. V., Klimenko, M. V., Bessarab, F. S.,
Korenkova, N. A., Ratovsky, K. G., Chernigovskaya, M. A., Shcherbakov, A.
A., Sahai, Y., Fagundes, P. R., Jesus, R. de, Abreu, A. J. de, and Condor,
P.: The global thermospheric and ionospheric response to the 2008 minor
sudden stratospheric warming event, J. Geophys. Res., 117, A10309, https://doi.org/10.1029/2012ja018018, 2012.
Lawrence, Z. D. and Manney, G. L.: Does the Arctic Stratospheric Polar
Vortex Exhibit Signs of Preconditioning Prior to Sudden Stratospheric
Warmings?, J. Atmos. Sci., 77, 611–632,
https://doi.org/10.1175/jas-d-19-0168.1, 2020.
Lee, S. H. and Butler, A. H.: The 2018–2019 Arctic stratospheric polar vortex, Weather, 75, 52–57, 2020.
Limpasuvan, V., Richter, J. H., Orsolini, Y. J., Stordal, F., and Kvissel,
O.-K.: The roles of planetary and gravity waves during a major stratospheric
sudden warming as characterized in WACCM, J. Atmos. Sol.-Terr. Phys.,
78–79, 84–98, https://doi.org/10.1016/j.jastp.2011.03.004, 2012.
Lindzen, R. S. and Holton, J. R.: A Theory of the Quasi-Biennial
Oscillation, J. Atmos. Sci., 25, 1095–1107,
https://doi.org/10.1175/1520-0469(1968)025<1095:atotqb>2.0.co;2, 1968.
Logan, J. A.: Trends in the vertical distribution of ozone: An analysis of
ozonesonde data, J. Geophys. Res., 99, 25,
https://doi.org/10.1029/94jd02333, 1994.
Logan, J. A., Megretskaia, I. A., Miller, A. J., Tiao, G. C., Choi, D.,
Zhang, L., Stolarski, R. S., Labow, G. J., Hollandsworth, S. M., Bodeker, G.
E., Claude, H., Muer, D. de, Kerr, J. B., Tarasick, D. W., Oltmans, S. J.,
Johnson, B., Schmidlin, F., Staehelin, J., Viatte, P., and Uchino, O.:
Trends in the vertical distribution of ozone: A comparison of two analyses
of ozonesonde data, J. Geophys. Res., 104, 26,
https://doi.org/10.1029/1999jd900300, 1999.
Manney, G. L., Krüger, K., Pawson, S., Minschwaner, K., Schwartz, M. J.,
Daffer, W. H., Livesey, N. J., Mlynczak, M. G., Remsberg, E. E., Russel III, J. M., and Waters, J. W.: The evolution of the stratopause during the 2006
major warming: Satellite data and assimilated meteorological analyses, J.
Geophys. Res., 113, D11115, https://doi.org/10.1029/2007jd009097, 2008a.
Manney, G. L., Daffer, W. H., Strawbridge, K. B., Walker, K. A., Boone, C. D., Bernath, P. F., Kerzenmacher, T., Schwartz, M. J., Strong, K., Sica, R. J., Krüger, K., Pumphrey, H. C., Lambert, A., Santee, M. L., Livesey, N. J., Remsberg, E. E., Mlynczak, M. G., and Russell III, J. R.: The high Arctic in extreme winters: vortex, temperature, and MLS and ACE-FTS trace gas evolution, Atmos. Chem. Phys., 8, 505–522, https://doi.org/10.5194/acp-8-505-2008, 2008b.
Manney, G. L., Schwartz, M. J., Krüger, K., Santee, M. L., Pawson, S.,
Lee, J. N., Daffer, W. H., Fuller, R. A., and Livesey, N. J.: Aura Microwave
Limb Sounder observations of dynamics and transport during the
record-breaking 2009 Arctic stratospheric major warming, Geophys. Res.
Lett., 36, L12815, https://doi.org/10.1029/2009gl038586, 2009a.
Manney, G. L., Harwood, R. S., MacKenzie, I. A., Minschwaner, K., Allen, D. R., Santee, M. L., Walker, K. A., Hegglin, M. I., Lambert, A., Pumphrey, H. C., Bernath, P. F., Boone, C. D., Schwartz, M. J., Livesey, N. J., Daffer, W. H., and Fuller, R. A.: Satellite observations and modeling of transport in the upper troposphere through the lower mesosphere during the 2006 major stratospheric sudden warming, Atmos. Chem. Phys., 9, 4775–4795, https://doi.org/10.5194/acp-9-4775-2009, 2009b.
Manney, G. L., Lawrence, Z. D., Santee, M. L., Livesey, N. J., Lambert, A., and Pitts, M. C.: Polar processing in a split vortex: Arctic ozone loss in early winter 2012/2013, Atmos. Chem. Phys., 15, 5381–5403, https://doi.org/10.5194/acp-15-5381-2015, 2015.
Marsh, D. R., Mills, M. J., Kinnison, D. E., Lamarque, J.-F., Calvo, N., and
Polvani, L. M.: Climate Change from 1850 to 2005 Simulated in CESM1(WACCM),
J. Climate, 26, 7372–7391, https://doi.org/10.1175/jcli-d-12-00558.1, 2013.
Martineau, P., Wright, J. S., Zhu, N., and Fujiwara, M.: Zonal-mean data set of global atmospheric reanalyses on pressure levels, Earth Syst. Sci. Data, 10, 1925–1941, https://doi.org/10.5194/essd-10-1925-2018, 2018.
Matsuno, T.: A dynamical model of the stratospheric sudden warming, J.
Atmos. Sci., 28, 1479–1494, https://doi.org/10.1175/1520-0469(1971)028<1479:ADMOTS>2.0.CO;2, 1971.
McDonald, M. K., Turnbull, D. N., and Donovan, D. P.: Steller Brewer,
ozonesonde, and DIAL measurements of Arctic O3 column over Eureka, N.W.T.
during 1996 winter/spring, Geophys. Res. Lett., 26, 2383–2386,
https://doi.org/10.1029/1999gl900506, 1999.
Molod, A., Takacs, L., Suarez, M., and Bacmeister, J.: Development of the GEOS-5 atmospheric general circulation model: evolution from MERRA to MERRA2, Geosci. Model Dev., 8, 1339–1356, https://doi.org/10.5194/gmd-8-1339-2015, 2015.
Nakamura, N.: Two-Dimensional Mixing, Edge Formation, and Permeability
Diagnosed in an Area Coordinate, J. Atmos. Sci., 53, 1524–1537, https://doi.org/10.1175/1520-0469(1996)053<1524:TDMEFA>2.0.CO;2, 1996.
Network for the Detection of Atmospheric Composition Change (NDACC): FTIR ozone retrievals, http://www.ndaccdemo.org/, last access: 18 April 2022.
Nowack, P. J., Abraham, N. L., Maycock, A. C., Braesicke, P., Gregory, J.
M., Joshi, M. M., Osprey, A., and Pyle, J. A.: A large ozone-circulation
feedback and its implications for global warming assessments, Nat. Clim.
Chang., 5, 41–45, https://doi.org/10.1038/nclimate2451, 2015.
Palmeiro, F. M., Barriopedro, D., García-Herrera, R., and Calvo, N.:
Comparing Sudden Stratospheric Warming Definitions in Reanalysis Data, J.
Climate, 28, 6823–6840, https://doi.org/10.1175/jcli-d-15-0004.1, 2015.
Polvani, L. M. and Waugh, D. W.: Upward Wave Activity Flux as a Precursor to
Extreme Stratospheric Events and Subsequent Anomalous Surface Weather
Regimes., J. Climate, 17, 3548–3554,
https://doi.org/10.1175/1520-0442(2004)017<3548:uwafaa>2.0.co;2, 2004.
Ramaswamy, V., Schwarzkopf, M. D., and Randel, W. J.: Fingerprint of ozone
depletion in the spatial and temporal pattern of recent lower-stratospheric
cooling, Nature, 382, 616–618, https://doi.org/10.1038/382616a0, 1996.
Randel, W. J.: Global variations of zonal mean ozone during strarospheric
warming events, J. Atmos. Sci., 50, 3308–3321, 1993.
Randel, W. J., Wu, F., and Stolarski, R.: Changes in Column Ozone Correlated
with the Stratospheric EP Flux, J. Meteorol. Soc. Jpn. Ser. II, 80,
849–862, https://doi.org/10.2151/jmsj.80.849, 2002.
Rao, J., Ren, R., Chen, H., Yu, Y., and Zhou, Y.: The Stratospheric Sudden
Warming Event in February 2018 and its Prediction by a Climate System Model,
J. Geophys. Res., 123, 13332–13345, https://doi.org/10.1029/2018jd028908, 2018.
Rao, J., Garfinkel, C. I., Chen, H., and White, I. P.: The 2019 New Year
Stratospheric Sudden Warming and Its Real-Time Predictions in Multiple S2S
Models, J. Geophys. Res., 124, 11155–11174,
https://doi.org/10.1029/2019jd030826, 2019.
Rao, T. N.: Climatology of UTLS ozone and the ratio of ozone and potential
vorticity over northern Europe, J. Geophys. Res., 108, 4703,
https://doi.org/10.1029/2003jd003860, 2003.
Rao, T. N., Arvelius, J., Kirkwood, S., and Gathen, P. von der: Climatology
of ozone in the troposphere and lower stratosphere over the European Arctic,
Adv. Space Res., 34, 754–758, https://doi.org/10.1016/j.asr.2003.05.055,
2004.
Rienecker, M. M., Suárez, M. J., Gelaro, R., Todling, R., Bacmeister,
J., Liu, E., Bosilovich, M. G., Schubert, S. D., Takacs, L., Kim, G.-K.,
Bloom, S., Chen, J., Collins, D., Conaty, A., Silva, A. da, Gu, W., Joiner,
J., Koster, R. D., Lucchesi, R., Molod, A., Owens, T., Pawson, S., Pegion,
P., Redder, C. R., Reichle, R., Robertson, F. R., Ruddick, A. G.,
Sienkiewicz, M., and Woollen, J.: MERRA: NASA's Modern-Era Retrospective
Analysis for Research and Applications, J. Climate, 24, 3624–3648,
https://doi.org/10.1175/jcli-d-11-00015.1, 2011.
Rodgers, C. D.: Inverse Methods for Atmospheric Sounding – Theory and
Practice, Oxford, Series on Atmospheric Oceanic and Planetary Physics,
https://doi.org/10.1142/9789812813718, 2000.
Rodgers, C. D. and Connor, B. J.: Intercomparison of remote sounding
instruments, J. Geophys. Res., 108, 4116,
https://doi.org/10.1029/2002jd002299, 2003.
Romanowsky, E., Handorf, D., Jaiser, R., Wohltmann, I., Dorn,
W., Ukita, J., Cohen, J., Dethloff, K., and Rex, M.: The role of
stratospheric ozone for Arctic-midlatitude linkages, Sci. Rep., 9,
1–7, https://doi.org/10.1038/s41598-019-43823-1, 2019.
Rothman, L. S., Gordon, I. E., Barbe, A., Benner, D. C., Bernath, P. F.,
Birk, M., Boudon, V., Brown, L. R., Campargue, A., Champion, J. P., Chance,
K., Coudert, L. H., Dana, V., Devi, V. M., Fally, S., Flaud, J. M., Gamache,
R. R., Goldman, A., Jacquemart, D., Kleiner, I., Lacome, N., Lafferty, W.
J., Mandin, J. Y., Massie, S. T., Mikhailenko, S. N., Miller, C. E.,
Moazzen-Ahmadi, N., Naumenko, O. V., Nikitin, A. V., Orphal, J., Perevalov,
V. I., Perrin, A., Predoi-Cross, A., Rinsland, C. P., Rotger, M.,
Šimečková, M., Smith, M. A. H., Sung, K., Tashkun, S. A.,
Tennyson, J., Toth, R. A., Vandaele, A. C., and Auwera, J. V.: The HITRAN
2008 molecular spectroscopic database, J. Quant. Spectrosc. Ra., 110, 533–572, https://doi.org/10.1016/j.jqsrt.2009.02.013, 2009.
Scheiben, D., Straub, C., Hocke, K., Forkman, P., and Kämpfer, N.: Observations of middle atmospheric H2O and O3 during the 2010 major sudden stratospheric warming by a network of microwave radiometers, Atmos. Chem. Phys., 12, 7753–7765, https://doi.org/10.5194/acp-12-7753-2012, 2012.
Scherhag, R.: Die explosionsartige Stratosphärenerwärmung des Spätwinters,
Ber. Det. Wetterdienstes, 38, 51–63, 1952.
Schoeberl, M. R.: Stratospheric Warmings: Observations and Theory, 16, 521,
https://doi.org/10.1029/rg016i004p00521, 1978.
Schranz, F., Hagen, J., Stober, G., Hocke, K., Murk, A., and Kämpfer, N.: Small-scale variability of stratospheric ozone during the sudden stratospheric warming 2018/2019 observed at Ny-Ålesund, Svalbard, Atmos. Chem. Phys., 20, 10791–10806, https://doi.org/10.5194/acp-20-10791-2020, 2020.
Scott, R. K. and Polvani, L. M.: Stratospheric control of upward wave flux
near the tropopause, Geophys. Res. Lett., 31, L02115,
https://doi.org/10.1029/2003gl017965, 2004.
Shangguan, M., Wang, W., and Jin, S.: Variability of temperature and ozone in the upper troposphere and lower stratosphere from multi-satellite observations and reanalysis data, Atmos. Chem. Phys., 19, 6659–6679, https://doi.org/10.5194/acp-19-6659-2019, 2019.
Siskind, D. E., Eckermann, S. D., Coy, L., McCormack, J. P., and Randall, C.
E.: On recent interannual variability of the Arctic winter mesosphere:
Implications for tracer descent, Geophys. Res. Lett., 34, 498–5,
https://doi.org/10.1029/2007gl029293, 2007.
Smit, H. G. J., Straeter, W., Johnson, B. J., Oltmans, S. J., Davies, J.,
Tarasick, D. W., Hoegger, B., Stubi, R., Schmidlin, F. J., Northam, T.,
Thompson, A. M., Witte, J. C., Boyd, I., and Posny, F.: Assessment of the
performance of ECC-ozonesondes under quasi-flight conditions in the
environmental simulation chamber: Insights from the Juelich Ozone Sonde
Intercomparison Experiment (JOSIE), J. Geophys. Res., 112, D19306,
https://doi.org/10.1029/2006jd007308, 2007.
Smith, K. L. and Polvani, L. M.: The surface impacts of Arctic stratospheric
ozone anomalies, Environ. Res. Lett., 9, 074015,
https://doi.org/10.1088/1748-9326/9/7/074015, 2014.
Sterling, C. W., Johnson, B. J., Oltmans, S. J., Smit, H. G. J., Jordan, A. F., Cullis, P. D., Hall, E. G., Thompson, A. M., and Witte, J. C.: Homogenizing and estimating the uncertainty in NOAA's long-term vertical ozone profile records measured with the electrochemical concentration cell ozonesonde, Atmos. Meas. Tech., 11, 3661–3687, https://doi.org/10.5194/amt-11-3661-2018, 2018.
Stolarski, R. S.: History of the Study of Atmospheric Ozone, Ozone Science
Engineering, 23, 421–428, https://doi.org/10.1080/01919510108962025, 2001.
Strahan, S. E., Douglass, A. R., and Steenrod, S. D.: Chemical and dynamical impacts of stratospheric sudden warmings on Arctic ozone variability, J. Geophys. Res.-Atmos, 121, 11836–11851, https://doi.org/10.1002/2016JD025128, 2016.
Tao, M., Konopka, P., Ploeger, F., Grooß, J.-U., Müller, R., Volk, C. M., Walker, K. A., and Riese, M.: Impact of the 2009 major sudden stratospheric warming on the composition of the stratosphere, Atmos. Chem. Phys., 15, 8695–8715, https://doi.org/10.5194/acp-15-8695-2015, 2015.
Tarasick, D. W. and Bottenheim, J. W.: Surface ozone depletion episodes in the Arctic and Antarctic from historical ozonesonde records, Atmos. Chem. Phys., 2, 197–205, https://doi.org/10.5194/acp-2-197-2002, 2002.
Tarasick, D. W., Davies, J., Smit, H. G. J., and Oltmans, S. J.: A re-evaluated Canadian ozonesonde record: measurements of the vertical distribution of ozone over Canada from 1966 to 2013, Atmos. Meas. Tech., 9, 195–214, https://doi.org/10.5194/amt-9-195-2016, 2016.
Thurairajah, B., Collins, R. L., Harvey, V. L., Lieberman, R. S., Gerding,
M., Mizutani, K., and Livingston, J. M.: Gravity wave activity in the Arctic
stratosphere and mesosphere during the 2007–2008 and 2008–2009
stratospheric sudden warming events, J. Geophys. Res., 115, D00N06,
https://doi.org/10.1029/2010jd014125, 2010.
Tiao, G. C., Reinsel, G. C., Pedrick, J. H., Allenby, G. M., Mateer, C. L.,
Miller, A. J., and DeLuisi, J. J.: A statistical trend analysis of
ozonesonde data, J. Geophys. Res., 91, 13121–13136,
https://doi.org/10.1029/jd091id12p13121, 1986.
Tripathi, O. P., Baldwin, M., Perez, A. C., Charron, M., Eckermann, S. D.,
Gerber, E., Harrison, R. G., Jackson, D. R., Kim, B.-M., Kuroda, Y., Lang,
A., Mahmood, S., Mizuta, R., Roff, G., Sigmond, M., and Son, S.-W.: The
predictability of the extratropical stratosphere on monthly time-scales and
its impact on the skill of tropospheric forecasts, Q. J. Roy. Meteor. Soc.,
141, 987–1003, https://doi.org/10.1002/qj.2432, 2015.
Vigouroux, C., De Mazière, M., Demoulin, P., Servais, C., Hase, F., Blumenstock, T., Kramer, I., Schneider, M., Mellqvist, J., Strandberg, A., Velazco, V., Notholt, J., Sussmann, R., Stremme, W., Rockmann, A., Gardiner, T., Coleman, M., and Woods, P.: Evaluation of tropospheric and stratospheric ozone trends over Western Europe from ground-based FTIR network observations, Atmos. Chem. Phys., 8, 6865–6886, https://doi.org/10.5194/acp-8-6865-2008, 2008.
Vigouroux, C., Blumenstock, T., Coffey, M., Errera, Q., García, O., Jones, N. B., Hannigan, J. W., Hase, F., Liley, B., Mahieu, E., Mellqvist, J., Notholt, J., Palm, M., Persson, G., Schneider, M., Servais, C., Smale, D., Thölix, L., and De Mazière, M.: Trends of ozone total columns and vertical distribution from FTIR observations at eight NDACC stations around the globe, Atmos. Chem. Phys., 15, 2915–2933, https://doi.org/10.5194/acp-15-2915-2015, 2015.
Wallace, J. M.: General circulation of the tropical lower stratosphere, Rev.
Geophys., 11, 191–222, https://doi.org/10.1029/rg011i002p00191, 1973.
Wargan, K., Labow, G., Frith, S., Pawson, S., Livesey, N., and Partyka, G.:
Evaluation of the Ozone Fields in NASA's MERRA-2 Reanalysis, J. Climate, 30,
2961–2988, https://doi.org/10.1175/jcli-d-16-0699.1, 2017.
Wargan, K., Orbe, C., Pawson, S., Ziemke, J. R., Oman, L. D., Olsen, M. A.,
Coy, L., and Knowland, K. E.: Recent Decline in Extratropical Lower
Stratospheric Ozone Attributed to Circulation Changes, Geophys. Res. Lett.,
45, 5166–5176, https://doi.org/10.1029/2018gl077406, 2018.
WMO/GAW Ozone Monitoring Community: World Meteorological Organization-Global Atmosphere Watch Program (WMO-GAW)/World Ozone and Ultraviolet Radiation Data Centre (WOUDC), [data set], retrieved 24 October 2013, from https://woudc.org, https://doi.org/10.14287/10000001, 2013.
Xie, F., Li, J., Tian, W., Fu, Q., Jin, F.-F., Hu, Y., Zhang, J., Wang, W.,
Sun, C., Feng, J., Yang, Y., and Ding, R.: A connection from Arctic
stratospheric ozone to El Niño-Southern oscillation, Environ. Res.
Lett., 11, 124026–12, https://doi.org/10.1088/1748-9326/11/12/124026, 2016.
Short summary
Large-scale atmospheric circulation has a strong influence on ozone in the Arctic, and certain anomalous dynamical events, such as sudden stratospheric warmings, cause dramatic alterations of the large-scale circulation. A reanalysis model is evaluated and then used to investigate the impact of sudden stratospheric warmings on mid-atmospheric ozone. Results show that the position of the cold jet stream over the Arctic before these events influences the variability of ozone.
Large-scale atmospheric circulation has a strong influence on ozone in the Arctic, and certain...
Altmetrics
Final-revised paper
Preprint