Articles | Volume 22, issue 19
https://doi.org/10.5194/acp-22-13115-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-22-13115-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
12 Oct 2022
Research article |
| 12 Oct 2022
| 12 Oct 2022
Size-resolved dust direct radiative effect efficiency derived from satellite observations
Qianqian Song
CORRESPONDING AUTHOR
Physics Department, UMBC, Baltimore, Maryland, USA
Goddard Earth Sciences Technology and Research II, UMBC, Baltimore,
Maryland, USA
Zhibo Zhang
Physics Department, UMBC, Baltimore, Maryland, USA
Goddard Earth Sciences Technology and Research II, UMBC, Baltimore,
Maryland, USA
Hongbin Yu
Climate and Radiation Laboratory, NASA Goddard Space Flight Center,
Greenbelt, Maryland, USA
Jasper F. Kok
Department of Atmospheric and Oceanic Sciences, University of California, Los Angeles, CA 90095, USA
Claudia Di Biagio
Université Paris Cité and Univ Paris Est Creteil, CNRS, LISA, 75013 Paris, France
Samuel Albani
Department of Environmental and Earth Sciences, University of
Milano–Bicocca, Milan, Italy
Jianyu Zheng
Physics Department, UMBC, Baltimore, Maryland, USA
Goddard Earth Sciences Technology and Research II, UMBC, Baltimore,
Maryland, USA
Jiachen Ding
Department of Atmospheric Sciences, Texas A&M University, College Station, Texas, USA
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Hongbin Yu, Qian Tan, Lillian Zhou, Yaping Zhou, Huisheng Bian, Mian Chin, Claire L. Ryder, Robert C. Levy, Yaswant Pradhan, Yingxi Shi, Qianqian Song, Zhibo Zhang, Peter R. Colarco, Dongchul Kim, Lorraine A. Remer, Tianle Yuan, Olga Mayol-Bracero, and Brent N. Holben
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Ramiro Checa-Garcia, Yves Balkanski, Samuel Albani, Tommi Bergman, Ken Carslaw, Anne Cozic, Chris Dearden, Beatrice Marticorena, Martine Michou, Twan van Noije, Pierre Nabat, Fiona M. O'Connor, Dirk Olivié, Joseph M. Prospero, Philippe Le Sager, Michael Schulz, and Catherine Scott
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Thousands of tons of dust are emitted into the atmosphere every year, producing important impacts on the Earth system. However, current global climate models are not yet able to reproduce dust emissions, transport and depositions with the desirable accuracy. Our study analyses five different Earth system models to report aspects to be improved to reproduce better available observations, increase the consistency between models and therefore decrease the current uncertainties.
Jasper F. Kok, Adeyemi A. Adebiyi, Samuel Albani, Yves Balkanski, Ramiro Checa-Garcia, Mian Chin, Peter R. Colarco, Douglas S. Hamilton, Yue Huang, Akinori Ito, Martina Klose, Danny M. Leung, Longlei Li, Natalie M. Mahowald, Ron L. Miller, Vincenzo Obiso, Carlos Pérez García-Pando, Adriana Rocha-Lima, Jessica S. Wan, and Chloe A. Whicker
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Jasper F. Kok, Adeyemi A. Adebiyi, Samuel Albani, Yves Balkanski, Ramiro Checa-Garcia, Mian Chin, Peter R. Colarco, Douglas S. Hamilton, Yue Huang, Akinori Ito, Martina Klose, Longlei Li, Natalie M. Mahowald, Ron L. Miller, Vincenzo Obiso, Carlos Pérez García-Pando, Adriana Rocha-Lima, and Jessica S. Wan
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We investigate how mid-Holocene dust reduction affects the Earth’s energetics from a suite of climate simulations. Our analyses confirm the peculiar role of the dust radiative effect over bright surfaces such as African deserts. We highlight a strong dependence on the dust pattern. The relative dust forcing between West Africa and the Middle East impacts the relative response of Indian and African monsoons and between the western tropical Atlantic and the Atlantic meridional circulation.
Longlei Li, Natalie M. Mahowald, Ron L. Miller, Carlos Pérez García-Pando, Martina Klose, Douglas S. Hamilton, Maria Gonçalves Ageitos, Paul Ginoux, Yves Balkanski, Robert O. Green, Olga Kalashnikova, Jasper F. Kok, Vincenzo Obiso, David Paynter, and David R. Thompson
Atmos. Chem. Phys., 21, 3973–4005, https://doi.org/10.5194/acp-21-3973-2021, https://doi.org/10.5194/acp-21-3973-2021, 2021
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For the first time, this study quantifies the range of the dust direct radiative effect due to uncertainty in the soil mineral abundance using all currently available information. We show that the majority of the estimated direct radiative effect range is due to uncertainty in the simulated mass fractions of iron oxides and thus their soil abundance, which is independent of the model employed. We therefore prove the necessity of considering mineralogy for understanding dust–climate interactions.
Zhibo Zhang, Qianqian Song, David B. Mechem, Vincent E. Larson, Jian Wang, Yangang Liu, Mikael K. Witte, Xiquan Dong, and Peng Wu
Atmos. Chem. Phys., 21, 3103–3121, https://doi.org/10.5194/acp-21-3103-2021, https://doi.org/10.5194/acp-21-3103-2021, 2021
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This study investigates the small-scale variations and covariations of cloud microphysical properties, namely, cloud liquid water content and cloud droplet number concentration, in marine boundary layer clouds based on in situ observation from the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) campaign. We discuss the dependence of cloud variations on vertical location in cloud and the implications for warm-rain simulations in the global climate models.
Clarissa Baldo, Paola Formenti, Sophie Nowak, Servanne Chevaillier, Mathieu Cazaunau, Edouard Pangui, Claudia Di Biagio, Jean-Francois Doussin, Konstantin Ignatyev, Pavla Dagsson-Waldhauserova, Olafur Arnalds, A. Robert MacKenzie, and Zongbo Shi
Atmos. Chem. Phys., 20, 13521–13539, https://doi.org/10.5194/acp-20-13521-2020, https://doi.org/10.5194/acp-20-13521-2020, 2020
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We showed that Icelandic dust has a fundamentally different chemical and mineralogical composition from low-latitude dust. In particular, magnetite is as high as 1 %–2 % of the total dust mass. Our results suggest that Icelandic dust may have an important impact on the radiation balance in the subpolar and polar regions.
Chenxi Wang, Steven Platnick, Kerry Meyer, Zhibo Zhang, and Yaping Zhou
Atmos. Meas. Tech., 13, 2257–2277, https://doi.org/10.5194/amt-13-2257-2020, https://doi.org/10.5194/amt-13-2257-2020, 2020
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A machine-learning (ML)-based approach that can be used for cloud mask and phase detection is developed. An all-day model that uses infrared (IR) observations and a daytime model that uses shortwave and IR observations from a passive instrument are trained separately for different surface types. The training datasets are selected by using reference pixel types from collocated space lidar. The ML approach is validated carefully and the overall performance is better than traditional methods.
Adeyemi A. Adebiyi, Jasper F. Kok, Yang Wang, Akinori Ito, David A. Ridley, Pierre Nabat, and Chun Zhao
Atmos. Chem. Phys., 20, 829–863, https://doi.org/10.5194/acp-20-829-2020, https://doi.org/10.5194/acp-20-829-2020, 2020
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Although atmospheric dust particles produce significant impacts on the Earth system, most climate models still have difficulty representing the basic processes that affect these particles. In this study, we present new constraints on dust properties that consistently outperform the conventional climate models, when compared to independent measurements. As a result, our constraints can be used to improve climate models or serve as an alternative in constraining dust impacts on the Earth system.
Claudia Di Biagio, Paola Formenti, Yves Balkanski, Lorenzo Caponi, Mathieu Cazaunau, Edouard Pangui, Emilie Journet, Sophie Nowak, Meinrat O. Andreae, Konrad Kandler, Thuraya Saeed, Stuart Piketh, David Seibert, Earle Williams, and Jean-François Doussin
Atmos. Chem. Phys., 19, 15503–15531, https://doi.org/10.5194/acp-19-15503-2019, https://doi.org/10.5194/acp-19-15503-2019, 2019
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This paper presents a new dataset of laboratory measurements of the shortwave (SW) spectral complex refractive index and single-scattering albedo (SSA) for global mineral dust aerosols of varying origin and composition. Our results show that the dust refractive index and SSA vary strongly from source to source, mostly due to particle iron content changes. We recommend that source-dependent values of the SW spectral refractive index and SSA be used in models and remote sensing applications.
Marc D. Mallet, Barbara D'Anna, Aurélie Même, Maria Chiara Bove, Federico Cassola, Giandomenico Pace, Karine Desboeufs, Claudia Di Biagio, Jean-Francois Doussin, Michel Maille, Dario Massabò, Jean Sciare, Pascal Zapf, Alcide Giorgio di Sarra, and Paola Formenti
Atmos. Chem. Phys., 19, 11123–11142, https://doi.org/10.5194/acp-19-11123-2019, https://doi.org/10.5194/acp-19-11123-2019, 2019
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We present findings from a summertime field campaign at the remote island of Lampedusa in the central Mediterranean Sea. We show that the aerosol loading is similar to coastal sites around the Mediterranean. We observe higher loadings of sulfate and aged organic aerosol from air masses transported over the central and eastern Mediterranean in comparison to those from the western Mediterranean. These results highlight the rarity of pristine air masses, even in remote marine environments.
Douglas S. Hamilton, Rachel A. Scanza, Yan Feng, Joseph Guinness, Jasper F. Kok, Longlei Li, Xiaohong Liu, Sagar D. Rathod, Jessica S. Wan, Mingxuan Wu, and Natalie M. Mahowald
Geosci. Model Dev., 12, 3835–3862, https://doi.org/10.5194/gmd-12-3835-2019, https://doi.org/10.5194/gmd-12-3835-2019, 2019
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MIMI v1.0 was designed for use within Earth system models to simulate the 3-D emission, atmospheric processing, and deposition of iron and its soluble fraction. Understanding the iron cycle is important due to its role as an essential micronutrient for ocean phytoplankton; its supply limits primary productivity in many of the world's oceans. Human activity has perturbed the iron cycle, and MIMI is capable of diagnosing many of these impacts; hence, it is important for future climate studies.
Antonio Di Noia, Otto P. Hasekamp, Bastiaan van Diedenhoven, and Zhibo Zhang
Atmos. Meas. Tech., 12, 1697–1716, https://doi.org/10.5194/amt-12-1697-2019, https://doi.org/10.5194/amt-12-1697-2019, 2019
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We present a neural network algorithm for the retrieval of cloud physical properties from multi-angle polarimetric measurements. We have trained the algorithm on a large dataset of synthetic measurements and applied it to a year of POLDER-3 data. A comparison against MODIS cloud products reveals that our algorithm is capable of performing cloud property retrievals on a global scale and possibly improves the estimates of cloud effective radius over land with respect to existing POLDER-3 products.
Yue Huang, Jasper F. Kok, Raleigh L. Martin, Nitzan Swet, Itzhak Katra, Thomas E. Gill, Richard L. Reynolds, and Livia S. Freire
Atmos. Chem. Phys., 19, 2947–2964, https://doi.org/10.5194/acp-19-2947-2019, https://doi.org/10.5194/acp-19-2947-2019, 2019
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This paper provides important insights on dust emission from sand dunes, which cover a large fraction of arid lands; produces the first in situ measurements for size-resolved dust emission from active sands that could improve the representation of dust cycle in climate models and remote sensing techniques; and shows that dust from active sands is likely significantly finer than thought, implying a greater effect of dust emission from active sands on downwind climate, hydrology, and human health.
Zhibo Zhang, Hua Song, Po-Lun Ma, Vincent E. Larson, Minghuai Wang, Xiquan Dong, and Jianwu Wang
Atmos. Chem. Phys., 19, 1077–1096, https://doi.org/10.5194/acp-19-1077-2019, https://doi.org/10.5194/acp-19-1077-2019, 2019
Peng Wu, Baike Xi, Xiquan Dong, and Zhibo Zhang
Atmos. Chem. Phys., 18, 17405–17420, https://doi.org/10.5194/acp-18-17405-2018, https://doi.org/10.5194/acp-18-17405-2018, 2018
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Prescribed autoconversion and accretion enhancement factors in GCM warm-rain parameterizations contribute partially to the too-frequent and too-light problem in precipitation simulation. The two factors should be regime- and resolution-dependent. A decreased autoconversion enhancement factor and increased accretion enhancement factor in the Morrison and Gettleman (2008) scheme can improve the simulated precipitation frequency and intensity. The two factors for other schemes are also suggested.
Stelios Myriokefalitakis, Akinori Ito, Maria Kanakidou, Athanasios Nenes, Maarten C. Krol, Natalie M. Mahowald, Rachel A. Scanza, Douglas S. Hamilton, Matthew S. Johnson, Nicholas Meskhidze, Jasper F. Kok, Cecile Guieu, Alex R. Baker, Timothy D. Jickells, Manmohan M. Sarin, Srinivas Bikkina, Rachel Shelley, Andrew Bowie, Morgane M. G. Perron, and Robert A. Duce
Biogeosciences, 15, 6659–6684, https://doi.org/10.5194/bg-15-6659-2018, https://doi.org/10.5194/bg-15-6659-2018, 2018
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The first atmospheric iron (Fe) deposition model intercomparison is presented in this study, as a result of the deliberations of the United Nations Joint Group of Experts on the Scientific Aspects of Marine Environmental Protection (GESAMP; http://www.gesamp.org/) Working Group 38. We conclude that model diversity over remote oceans reflects uncertainty in the Fe content parameterizations of dust aerosols, combustion aerosol emissions and the size distribution of transported aerosol Fe.
Benjamin S. Grandey, Daniel Rothenberg, Alexander Avramov, Qinjian Jin, Hsiang-He Lee, Xiaohong Liu, Zheng Lu, Samuel Albani, and Chien Wang
Atmos. Chem. Phys., 18, 15783–15810, https://doi.org/10.5194/acp-18-15783-2018, https://doi.org/10.5194/acp-18-15783-2018, 2018
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Anthropogenic emissions of aerosol particles likely cool the climate system. We investigate the uncertainty in the strength of the cooling effect by exploring the representation of aerosols in a global climate model. We conclude that the specific representation of aerosols in global climate models has important implications for climate modelling. Important factors include the representation of aerosol mixing state, size distribution, and optical properties.
Qianqian Song, Zhibo Zhang, Hongbin Yu, Seiji Kato, Ping Yang, Peter Colarco, Lorraine A. Remer, and Claire L. Ryder
Atmos. Chem. Phys., 18, 11303–11322, https://doi.org/10.5194/acp-18-11303-2018, https://doi.org/10.5194/acp-18-11303-2018, 2018
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Mineral dust is the most abundant atmospheric aerosol component in terms of dry mass. In this study, we integrate recent aircraft measurements of dust microphysical and optical properties with satellite retrievals of aerosol and radiative fluxes to quantify the dust direct radiative effects on the shortwave and longwave radiation at both the top of the atmosphere and the surface in the tropical North Atlantic during summer months.
Hua Song, Zhibo Zhang, Po-Lun Ma, Steven Ghan, and Minghuai Wang
Geosci. Model Dev., 11, 3147–3158, https://doi.org/10.5194/gmd-11-3147-2018, https://doi.org/10.5194/gmd-11-3147-2018, 2018
Daniel J. Miller, Zhibo Zhang, Steven Platnick, Andrew S. Ackerman, Frank Werner, Celine Cornet, and Kirk Knobelspiesse
Atmos. Meas. Tech., 11, 3689–3715, https://doi.org/10.5194/amt-11-3689-2018, https://doi.org/10.5194/amt-11-3689-2018, 2018
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Prior satellite comparisons of bispectral and polarimetric cloud droplet size retrievals exhibited systematic biases. However, similar airborne instrument retrievals have been found to be quite similar to one another. This study explains this discrepancy in terms of differing sensitivity to vertical profile, as well as spatial and angular resolution. This is accomplished by using a satellite retrieval simulator – an LES cloud model coupled to radiative transfer and cloud retrieval algorithms.
Masa Kageyama, Pascale Braconnot, Sandy P. Harrison, Alan M. Haywood, Johann H. Jungclaus, Bette L. Otto-Bliesner, Jean-Yves Peterschmitt, Ayako Abe-Ouchi, Samuel Albani, Patrick J. Bartlein, Chris Brierley, Michel Crucifix, Aisling Dolan, Laura Fernandez-Donado, Hubertus Fischer, Peter O. Hopcroft, Ruza F. Ivanovic, Fabrice Lambert, Daniel J. Lunt, Natalie M. Mahowald, W. Richard Peltier, Steven J. Phipps, Didier M. Roche, Gavin A. Schmidt, Lev Tarasov, Paul J. Valdes, Qiong Zhang, and Tianjun Zhou
Geosci. Model Dev., 11, 1033–1057, https://doi.org/10.5194/gmd-11-1033-2018, https://doi.org/10.5194/gmd-11-1033-2018, 2018
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The Paleoclimate Modelling Intercomparison Project (PMIP) takes advantage of the existence of past climate states radically different from the recent past to test climate models used for climate projections and to better understand these climates. This paper describes the PMIP contribution to CMIP6 (Coupled Model Intercomparison Project, 6th phase) and possible analyses based on PMIP results, as well as on other CMIP6 projects.
Heming Bai, Cheng Gong, Minghuai Wang, Zhibo Zhang, and Tristan L'Ecuyer
Atmos. Chem. Phys., 18, 1763–1783, https://doi.org/10.5194/acp-18-1763-2018, https://doi.org/10.5194/acp-18-1763-2018, 2018
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Precipitation susceptibility to aerosol perturbation plays a key role in understanding aerosol–cloud interactions and for constraining aerosol indirect effects. Here, multisensor aerosol and cloud products from A-Train satellites are analyzed to estimate precipitation susceptibility. Compared to precipitation intensity susceptibility, precipitation frequency susceptibility demonstrates relatively robust features across different retrieval products.
Masa Kageyama, Samuel Albani, Pascale Braconnot, Sandy P. Harrison, Peter O. Hopcroft, Ruza F. Ivanovic, Fabrice Lambert, Olivier Marti, W. Richard Peltier, Jean-Yves Peterschmitt, Didier M. Roche, Lev Tarasov, Xu Zhang, Esther C. Brady, Alan M. Haywood, Allegra N. LeGrande, Daniel J. Lunt, Natalie M. Mahowald, Uwe Mikolajewicz, Kerim H. Nisancioglu, Bette L. Otto-Bliesner, Hans Renssen, Robert A. Tomas, Qiong Zhang, Ayako Abe-Ouchi, Patrick J. Bartlein, Jian Cao, Qiang Li, Gerrit Lohmann, Rumi Ohgaito, Xiaoxu Shi, Evgeny Volodin, Kohei Yoshida, Xiao Zhang, and Weipeng Zheng
Geosci. Model Dev., 10, 4035–4055, https://doi.org/10.5194/gmd-10-4035-2017, https://doi.org/10.5194/gmd-10-4035-2017, 2017
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The Last Glacial Maximum (LGM, 21000 years ago) is an interval when global ice volume was at a maximum, eustatic sea level close to a minimum, greenhouse gas concentrations were lower, atmospheric aerosol loadings were higher than today, and vegetation and land-surface characteristics were different from today. This paper describes the implementation of the LGM numerical experiment for the PMIP4-CMIP6 modelling intercomparison projects and the associated sensitivity experiments.
Claudia Di Biagio, Paola Formenti, Mathieu Cazaunau, Edouard Pangui, Nicolas Marchand, and Jean-François Doussin
Atmos. Meas. Tech., 10, 2923–2939, https://doi.org/10.5194/amt-10-2923-2017, https://doi.org/10.5194/amt-10-2923-2017, 2017
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Mineral dust is one of the most abundant aerosol species at the global scale and an accurate estimation of its absorption at solar wavelengths is crucial to assess its impact on climate. In this work we provide an estimate of the Aethalometer multiple scattering correction for mineral dust aerosols at 450 and 660 nm. Our results suggest that the use of an optimized correction factor can lead to up to 11 % higher absorption coefficient and to 3 % higher single scattering albedo for mineral dust.
Lorenzo Caponi, Paola Formenti, Dario Massabó, Claudia Di Biagio, Mathieu Cazaunau, Edouard Pangui, Servanne Chevaillier, Gautier Landrot, Meinrat O. Andreae, Konrad Kandler, Stuart Piketh, Thuraya Saeed, Dave Seibert, Earle Williams, Yves Balkanski, Paolo Prati, and Jean-François Doussin
Atmos. Chem. Phys., 17, 7175–7191, https://doi.org/10.5194/acp-17-7175-2017, https://doi.org/10.5194/acp-17-7175-2017, 2017
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This paper presents new laboratory measurements of the shortwave mass absorption efficiency (MAE) used by climate models for mineral dust of different origin and at different sizes. We found that small particles are more efficient, by given mass, in absorbing radiation, particularly at shorter wavelength. Because dust has high concentrations in the atmosphere, light absorption by mineral dust can be competitive to other absorbing atmospheric aerosols such as black and brown carbon.
Molly B. Smith, Natalie M. Mahowald, Samuel Albani, Aaron Perry, Remi Losno, Zihan Qu, Beatrice Marticorena, David A. Ridley, and Colette L. Heald
Atmos. Chem. Phys., 17, 3253–3278, https://doi.org/10.5194/acp-17-3253-2017, https://doi.org/10.5194/acp-17-3253-2017, 2017
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Using different meteorology reanalyses to drive dust in climate modeling can produce dissimilar global dust distributions, especially in the Southern Hemisphere (SH). It may therefore not be advisable for SH dust studies to base results on simulations driven by one reanalysis. Northern Hemisphere dust varies mostly on seasonal timescales, while SH dust varies on interannual timescales. Dust is an important part of climate modeling, and we hope this contributes to understanding these simulations.
Giuliano Liuzzi, Guido Masiello, Carmine Serio, Daniela Meloni, Claudia Di Biagio, and Paola Formenti
Atmos. Meas. Tech., 10, 599–615, https://doi.org/10.5194/amt-10-599-2017, https://doi.org/10.5194/amt-10-599-2017, 2017
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In this work we have given a contribution to better understand some of the properties of the desert dust plumes in the western Mediterranean, using both direct measurements and satellite observations. This study has mainly evidenced that satellite observations can provide information about the geographical provenance of dust. This is important because such variability is reflected in the way in which dust interacts with atmosphere and impacts over the observed infrared radiation from satellites.
Claudia Di Biagio, Paola Formenti, Yves Balkanski, Lorenzo Caponi, Mathieu Cazaunau, Edouard Pangui, Emilie Journet, Sophie Nowak, Sandrine Caquineau, Meinrat O. Andreae, Konrad Kandler, Thuraya Saeed, Stuart Piketh, David Seibert, Earle Williams, and Jean-François Doussin
Atmos. Chem. Phys., 17, 1901–1929, https://doi.org/10.5194/acp-17-1901-2017, https://doi.org/10.5194/acp-17-1901-2017, 2017
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Modeling the interaction of dust with long-wave (LW) radiation is still a challenge due to the scarcity of information on their refractive index. In this paper, we present a unique dataset of dust refractive indices obtained from in situ measurements in a large smog chamber. Our results show that the dust LW refractive index varies strongly from source to source due to particle composition changes. We recommend taking this variability into account in climate and remote sensing applications.
Frank Werner, Galina Wind, Zhibo Zhang, Steven Platnick, Larry Di Girolamo, Guangyu Zhao, Nandana Amarasinghe, and Kerry Meyer
Atmos. Meas. Tech., 9, 5869–5894, https://doi.org/10.5194/amt-9-5869-2016, https://doi.org/10.5194/amt-9-5869-2016, 2016
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A research–level retrieval algorithm for cloud optical and microphysical properties is developed for the Advanced Spaceborne Thermal Emission and Reflection Radiometer (ASTER) aboard the Terra satellite. This yields reliable estimates of important cloud variables at a horizontal resolution of 30 m. Comparisons of the ASTER retrieval results with the operational cloud products from the Moderate Resolution Imaging Spectroradiometer (MODIS) show a high agreement for 48 example cloud fields.
David A. Ridley, Colette L. Heald, Jasper F. Kok, and Chun Zhao
Atmos. Chem. Phys., 16, 15097–15117, https://doi.org/10.5194/acp-16-15097-2016, https://doi.org/10.5194/acp-16-15097-2016, 2016
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Mineral dust aerosol affects climate through interaction with radiation and clouds, human health through contribution to particulate matter, and ecosystem health through nutrient transport and deposition. In this study, we use satellite and in situ retrievals to derive an observational estimate of the global dust AOD with which evaluate modeled dust AOD. Differences in the seasonality and regional distribution of dust AOD between observations and models are highlighted.
Claudia Di Biagio, Paola Formenti, Lionel Doppler, Cécile Gaimoz, Noel Grand, Gerard Ancellet, Jean-Luc Attié, Silvia Bucci, Philippe Dubuisson, Federico Fierli, Marc Mallet, and François Ravetta
Atmos. Chem. Phys., 16, 10591–10607, https://doi.org/10.5194/acp-16-10591-2016, https://doi.org/10.5194/acp-16-10591-2016, 2016
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Pollution aerosols strongly influence the composition of the Western Mediterranean, but at present little is known on their optical properties. Here, we report observations of pollution aerosols measured during the TRAQA airborne campaign in summer 2012. Data from this study indicate a large variability of the absorption for pollution particles. This variability strongly influences their direct radiative effect, with possible consequences on the hydrological cycle in this part of the basin.
Robert Raiswell, Jon R. Hawkings, Liane G. Benning, Alex R. Baker, Ros Death, Samuel Albani, Natalie Mahowald, Michael D. Krom, Simon W. Poulton, Jemma Wadham, and Martyn Tranter
Biogeosciences, 13, 3887–3900, https://doi.org/10.5194/bg-13-3887-2016, https://doi.org/10.5194/bg-13-3887-2016, 2016
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Iron is an essential nutrient for plankton growth. One important source of iron is wind-blown dust. The polar oceans are remote from dust sources but melting icebergs supply sediment that contains iron which is potentially available to plankton. We show that iceberg sediments contain more potentially bioavailable iron than wind-blown dust. Iceberg sources will become increasingly important with climate change and increased plankton growth can remove more carbon dioxide from the atmosphere.
Zhibo Zhang, Kerry Meyer, Hongbin Yu, Steven Platnick, Peter Colarco, Zhaoyan Liu, and Lazaros Oreopoulos
Atmos. Chem. Phys., 16, 2877–2900, https://doi.org/10.5194/acp-16-2877-2016, https://doi.org/10.5194/acp-16-2877-2016, 2016
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The frequency of occurrence and shortwave direct radiative effects (DRE) of above-cloud aerosols (ACAs) over global oceans are investigated using 8 years of collocated CALIOP and MODIS observations. We estimated that ACAs have a global ocean annual mean diurnally averaged cloudy-sky DRE of 0.015 W m−2 (range of −0.03 to 0.06 W m−2) at TOA. The DREs at surface and within atmosphere are −0.15 W m−2 (range of −0.09 to −0.21 W m−2), and 0.17 W m−2 (range of 0.11 to 0.24 W m−2), respectively.
Y. Zhang, N. Mahowald, R. A. Scanza, E. Journet, K. Desboeufs, S. Albani, J. F. Kok, G. Zhuang, Y. Chen, D. D. Cohen, A. Paytan, M. D. Patey, E. P. Achterberg, J. P. Engelbrecht, and K. W. Fomba
Biogeosciences, 12, 5771–5792, https://doi.org/10.5194/bg-12-5771-2015, https://doi.org/10.5194/bg-12-5771-2015, 2015
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A new technique to determine a size-fractionated global soil elemental emission inventory based on a global soil and mineralogical data set is introduced. Spatial variability of mineral dust elemental fractions (8 elements, e.g., Ca, Fe, Al) is identified on a global scale, particularly for Ca. The Ca/Al ratio ranged between 0.1 and 5.0 and is confirmed as an indicator of dust source regions by a global dust model. Total and soluble dust element fluxes into different ocean basins are estimated.
C. Di Biagio, L. Doppler, C. Gaimoz, N. Grand, G. Ancellet, J.-C. Raut, M. Beekmann, A. Borbon, K. Sartelet, J.-L. Attié, F. Ravetta, and P. Formenti
Atmos. Chem. Phys., 15, 9611–9630, https://doi.org/10.5194/acp-15-9611-2015, https://doi.org/10.5194/acp-15-9611-2015, 2015
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Observations from this study indicate that continental pollution largely affects the atmospheric composition and structure of the western Mediterranean basin. Pollution plumes reach 3000-4000 m in altitude and present a very complex and highly stratified structure, characterized by fresh and aged layers both in the boundary layer and in the free troposphere. Also we report the observations of high levels of ultrafine particles over the basin, possibly linked to new particle formation events.
S. Albani, N. M. Mahowald, G. Winckler, R. F. Anderson, L. I. Bradtmiller, B. Delmonte, R. François, M. Goman, N. G. Heavens, P. P. Hesse, S. A. Hovan, S. G. Kang, K. E. Kohfeld, H. Lu, V. Maggi, J. A. Mason, P. A. Mayewski, D. McGee, X. Miao, B. L. Otto-Bliesner, A. T. Perry, A. Pourmand, H. M. Roberts, N. Rosenbloom, T. Stevens, and J. Sun
Clim. Past, 11, 869–903, https://doi.org/10.5194/cp-11-869-2015, https://doi.org/10.5194/cp-11-869-2015, 2015
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We propose an innovative framework to organize paleodust records, formalized in a publicly accessible database, and discuss the emerging properties of the global dust cycle during the Holocene by integrating our analysis with simulations performed with the Community Earth System Model. We show how the size distribution of dust is intrinsically related to the dust mass accumulation rates and that only considering a consistent size range allows for a consistent analysis of the global dust cycle.
P. Nabat, S. Somot, M. Mallet, M. Michou, F. Sevault, F. Driouech, D. Meloni, A. di Sarra, C. Di Biagio, P. Formenti, M. Sicard, J.-F. Léon, and M.-N. Bouin
Atmos. Chem. Phys., 15, 3303–3326, https://doi.org/10.5194/acp-15-3303-2015, https://doi.org/10.5194/acp-15-3303-2015, 2015
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This paper uses an original approach based on a coupled regional aerosol--atmosphere--ocean model to study the dust radiative effects over the Mediterranean in summer 2012. After an evaluation of the prognostic aerosol scheme, the dust aerosol daily variability is shown to improve the simulated surface radiation and temperature at the daily scale. It has also a significant impact on the summer average, thus highlighting the importance of a relevant representation of aerosols in climate models.
R. A. Scanza, N. Mahowald, S. Ghan, C. S. Zender, J. F. Kok, X. Liu, Y. Zhang, and S. Albani
Atmos. Chem. Phys., 15, 537–561, https://doi.org/10.5194/acp-15-537-2015, https://doi.org/10.5194/acp-15-537-2015, 2015
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The main purpose of this study was to build a framework in the Community Atmosphere Models version 4 and 5 within the Community Earth System Model to simulate dust aerosols as their component minerals. With this framework, we investigate the direct radiative forcing that results from the mineral speciation. We find that adding mineralogy results in a small positive forcing at the top of the atmosphere, while simulations without mineralogy have a small negative forcing.
J. F. Kok, N. M. Mahowald, G. Fratini, J. A. Gillies, M. Ishizuka, J. F. Leys, M. Mikami, M.-S. Park, S.-U. Park, R. S. Van Pelt, and T. M. Zobeck
Atmos. Chem. Phys., 14, 13023–13041, https://doi.org/10.5194/acp-14-13023-2014, https://doi.org/10.5194/acp-14-13023-2014, 2014
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We developed an improved model for the emission of dust particulates ("aerosols") emitted by wind erosion from the world's deserts. The implementation of our improved dust emission model into a climate model improves its agreement against measurements. We furthermore find that dust emissions are substantially more sensitive to the soil state than most current climate models account for.
C. Di Biagio, H. Boucher, S. Caquineau, S. Chevaillier, J. Cuesta, and P. Formenti
Atmos. Chem. Phys., 14, 11093–11116, https://doi.org/10.5194/acp-14-11093-2014, https://doi.org/10.5194/acp-14-11093-2014, 2014
Z. Zhang, K. Meyer, S. Platnick, L. Oreopoulos, D. Lee, and H. Yu
Atmos. Meas. Tech., 7, 1777–1789, https://doi.org/10.5194/amt-7-1777-2014, https://doi.org/10.5194/amt-7-1777-2014, 2014
S. Schüpbach, U. Federer, P. R. Kaufmann, S. Albani, C. Barbante, T. F. Stocker, and H. Fischer
Clim. Past, 9, 2789–2807, https://doi.org/10.5194/cp-9-2789-2013, https://doi.org/10.5194/cp-9-2789-2013, 2013
C. Zhao, S. Chen, L. R. Leung, Y. Qian, J. F. Kok, R. A. Zaveri, and J. Huang
Atmos. Chem. Phys., 13, 10733–10753, https://doi.org/10.5194/acp-13-10733-2013, https://doi.org/10.5194/acp-13-10733-2013, 2013
A. Arola, T. F. Eck, J. Huttunen, K. E. J. Lehtinen, A. V. Lindfors, G. Myhre, A. Smirnov, S. N. Tripathi, and H. Yu
Atmos. Chem. Phys., 13, 7895–7901, https://doi.org/10.5194/acp-13-7895-2013, https://doi.org/10.5194/acp-13-7895-2013, 2013
P. Stier, N. A. J. Schutgens, N. Bellouin, H. Bian, O. Boucher, M. Chin, S. Ghan, N. Huneeus, S. Kinne, G. Lin, X. Ma, G. Myhre, J. E. Penner, C. A. Randles, B. Samset, M. Schulz, T. Takemura, F. Yu, H. Yu, and C. Zhou
Atmos. Chem. Phys., 13, 3245–3270, https://doi.org/10.5194/acp-13-3245-2013, https://doi.org/10.5194/acp-13-3245-2013, 2013
W. J. Collins, M. M. Fry, H. Yu, J. S. Fuglestvedt, D. T. Shindell, and J. J. West
Atmos. Chem. Phys., 13, 2471–2485, https://doi.org/10.5194/acp-13-2471-2013, https://doi.org/10.5194/acp-13-2471-2013, 2013
C. A. Randles, S. Kinne, G. Myhre, M. Schulz, P. Stier, J. Fischer, L. Doppler, E. Highwood, C. Ryder, B. Harris, J. Huttunen, Y. Ma, R. T. Pinker, B. Mayer, D. Neubauer, R. Hitzenberger, L. Oreopoulos, D. Lee, G. Pitari, G. Di Genova, J. Quaas, F. G. Rose, S. Kato, S. T. Rumbold, I. Vardavas, N. Hatzianastassiou, C. Matsoukas, H. Yu, F. Zhang, H. Zhang, and P. Lu
Atmos. Chem. Phys., 13, 2347–2379, https://doi.org/10.5194/acp-13-2347-2013, https://doi.org/10.5194/acp-13-2347-2013, 2013
L. Zhu, J. V. Martins, and H. Yu
Atmos. Meas. Tech., 5, 3055–3067, https://doi.org/10.5194/amt-5-3055-2012, https://doi.org/10.5194/amt-5-3055-2012, 2012
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Troposphere | Science Focus: Physics (physical properties and processes)
Improved simulations of biomass burning aerosol optical properties and lifetimes in the NASA GEOS Model during the ORACLES-I campaign
Sharp increase in Saharan dust intrusions over the western Euro-Mediterranean in February–March 2020–2022 and associated atmospheric circulation
Temporal and spatial variations in dust activity in Australia based on remote sensing and reanalysis datasets
Sensitivity of global direct aerosol shortwave radiative forcing to uncertainties in aerosol optical properties
Molecular-level study on the role of methanesulfonic acid in iodine oxoacid nucleation
Regional to global distributions, trends, and drivers of biogenic volatile organic compound emission from 2001 to 2020
Impacts of ice-nucleating particles on cirrus clouds and radiation derived from global model simulations with MADE3 in EMAC
Seasonal characteristics of emission, distribution, and radiative effect of marine organic aerosols over the western Pacific Ocean: an investigation with a coupled regional climate aerosol model
Fire–precipitation interactions amplify the quasi-biennial variability in fires over southern Mexico and Central America
Improved estimates of smoke exposure during Australia fire seasons: importance of quantifying plume injection heights
New particle formation induced by anthropogenic–biogenic interactions on the southeastern Tibetan Plateau
Investigation of observed dust trends over the Middle East region in NASA Goddard Earth Observing System (GEOS) model simulations
A new process-based and scale-aware desert dust emission scheme for global climate models – Part II: Evaluation in the Community Earth System Model version 2 (CESM2)
Aerosols in the central Arctic cryosphere: Satellite and model integrated insights during Arctic spring and summer
How well do Earth system models reproduce the observed aerosol response to rapid emission reductions? A COVID-19 case study
Observationally constrained analysis of sulfur cycle in the marine atmosphere with NASA ATom measurements and AeroCom model simulations
Impact of acidity and surface-modulated acid dissociation on cloud response to organic aerosol
The contribution of residential wood combustion to the PM2.5 concentrations in the Helsinki metropolitan area
Analysis of atmospheric particle growth based on vapor concentrations measured at the high-altitude GAW station Chacaltaya in the Bolivian Andes
Expanding the simulation of East Asian super dust storms: physical transport mechanisms impacting the western Pacific
Improving 3-day deterministic air pollution forecasts using machine learning algorithms
Opinion: The importance of historical and paleoclimate aerosol radiative effects
Assessing the assimilation of Himawari-8 observations on aerosol forecasts and radiative effects during pollution transport from South Asia to the Tibetan Plateau
Aerosol–meteorology feedback diminishes the transboundary transport of black carbon into the Tibetan Plateau
Associations of interannual variation in summer tropospheric ozone with the Western Pacific Subtropical High in China from 1999 to 2017
Climate intervention using marine cloud brightening (MCB) compared with stratospheric aerosol injection (SAI) in the UKESM1 climate model
Comparison of six approaches to predicting droplet activation of surface active aerosol – Part 2: Strong surfactants
Increased importance of aerosol–cloud interactions for surface PM2.5 pollution relative to aerosol–radiation interactions in China with the anthropogenic emission reductions
The role of temporal scales in extracting dominant meteorological drivers of major airborne pollutants
Biomass-burning smoke's properties and its interactions with marine stratocumulus clouds in WRF-CAM5 and southeastern Atlantic field campaigns
Air pollution trapping in the Dresden Basin from gray-zone scale urban modeling
The effect of atmospherically relevant aminium salts on water uptake
Droplet collection efficiencies estimated from satellite retrievals constrain effective radiative forcing of aerosol-cloud interactions
Intercomparison of Aerosol Optical Depths from four reanalyses and their multi-reanalysis-consensus
The impact of aerosols on stratiform clouds over southern West Africa: a large-eddy-simulation study
Numerical simulation and evaluation of global ultrafine particle concentrations at the Earth's surface
Rapid Iodine Oxoacids Nucleation Enhanced by Dimethylamine in Broad Marine Regions
Comparing the simulated influence of biomass burning plumes on low-level clouds over the southeastern Atlantic under varying smoke conditions
Global aviation contrail climate effects from 2019 to 2021
Global aerosol typing classification using a new hybrid algorithm utilizing Aerosol Robotic Network data
Diagnosing uncertainties in global biomass burning emission inventories and their impact on modeled air pollutants
The underappreciated role of transboundary pollution in future air quality and health improvements in China
The export of African mineral dust across the Atlantic and its impact over the Amazon Basin
Assimilation of POLDER observations to estimate aerosol emissions
Role of atmospheric aerosols in severe winter fog over Indo Gangetic Plains of India: a case study
Effect of radiation interaction and aerosol processes on ventilation and aerosol concentrations in a real urban neighbourhood in Helsinki
Numerical evidence that the impact of CCN and INP concentrations on mixed-phase clouds is observable with cloud radars
Atlantic Multidecadal Oscillation modulates the relationship between El Niño–Southern Oscillation and fire weather in Australia
Phase state and viscosity of secondary organic aerosols over China simulated by WRF-Chem
Identifying climate model structural inconsistencies allows for tight constraint of aerosol radiative forcing
Sampa Das, Peter R. Colarco, Huisheng Bian, and Santiago Gassó
Atmos. Chem. Phys., 24, 4421–4449, https://doi.org/10.5194/acp-24-4421-2024, https://doi.org/10.5194/acp-24-4421-2024, 2024
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The smoke aerosols emitted from vegetation burning can alter the regional energy budget via multiple pathways. We utilized detailed observations from the NASA ORACLES airborne campaign based in Namibia during September 2016 to improve the representation of smoke aerosol properties and lifetimes in our GEOS Earth system model. The improved model simulations are for the first time able to capture the observed changes in the smoke absorption during long-range plume transport.
Emilio Cuevas-Agulló, David Barriopedro, Rosa Delia García, Silvia Alonso-Pérez, Juan Jesús González-Alemán, Ernest Werner, David Suárez, Juan José Bustos, Gerardo García-Castrillo, Omaira García, África Barreto, and Sara Basart
Atmos. Chem. Phys., 24, 4083–4104, https://doi.org/10.5194/acp-24-4083-2024, https://doi.org/10.5194/acp-24-4083-2024, 2024
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During February–March (FM) 2020–2022, unusually intense dust storms from northern Africa hit the western Euro-Mediterranean (WEM). Using dust products from satellites and atmospheric reanalysis for 2003–2022, results show that cut-off lows and European blocking are key drivers of FM dust intrusions over the WEM. A higher frequency of cut-off lows associated with subtropical ridges is observed in the late 2020–2022 period.
Yahui Che, Bofu Yu, and Katherine Bracco
Atmos. Chem. Phys., 24, 4105–4128, https://doi.org/10.5194/acp-24-4105-2024, https://doi.org/10.5194/acp-24-4105-2024, 2024
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Dust events occur more frequently during the Austral spring and summer in dust regions, including central Australia, the southwest of Western Australia, and the northern and southern regions of eastern Australia using remote sensing and reanalysis datasets. High-concentration dust is distributed around central Australia and in the downwind northern and southern Australia. Typically, around 50 % of the dust lifted settles on Australian land, with the remaining half being deposited in the ocean.
Jonathan Elsey, Nicolas Bellouin, and Claire Ryder
Atmos. Chem. Phys., 24, 4065–4081, https://doi.org/10.5194/acp-24-4065-2024, https://doi.org/10.5194/acp-24-4065-2024, 2024
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Aerosols influence the Earth's energy balance. The uncertainty in this radiative forcing is large depending partly on uncertainty in measurements of aerosol optical properties. We have developed a freely available new framework of millions of radiative transfer simulations spanning aerosol uncertainty and assess the impact on radiative forcing uncertainty. We find that reducing these uncertainties would reduce radiative forcing uncertainty, but non-aerosol uncertainties must also be considered.
Jing Li, Nan Wu, Biwu Chu, An Ning, and Xiuhui Zhang
Atmos. Chem. Phys., 24, 3989–4000, https://doi.org/10.5194/acp-24-3989-2024, https://doi.org/10.5194/acp-24-3989-2024, 2024
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Iodic acid (HIO3) nucleates with iodous acid (HIO2) efficiently in marine areas; however, whether methanesulfonic acid (MSA) can synergistically participate in the HIO3–HIO2-based nucleation is unclear. We provide molecular-level evidence that MSA can efficiently promote the formation of HIO3–HIO2-based clusters using a theoretical approach. The proposed MSA-enhanced iodine nucleation mechanism may help us to deeply understand marine new particle formation events with bursts of iodine particles.
Hao Wang, Xiaohong Liu, Chenglai Wu, and Guangxing Lin
Atmos. Chem. Phys., 24, 3309–3328, https://doi.org/10.5194/acp-24-3309-2024, https://doi.org/10.5194/acp-24-3309-2024, 2024
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We quantified different global- and regional-scale drivers of biogenic volatile organic compound (BVOC) emission trends over the past 20 years. The results show that global greening trends significantly boost BVOC emissions and deforestation reduces BVOC emissions in South America and Southeast Asia. Elevated temperature in Europe and increased soil moisture in East and South Asia enhance BVOC emissions. The results deepen our understanding of long-term BVOC emission trends in hotspots.
Christof G. Beer, Johannes Hendricks, and Mattia Righi
Atmos. Chem. Phys., 24, 3217–3240, https://doi.org/10.5194/acp-24-3217-2024, https://doi.org/10.5194/acp-24-3217-2024, 2024
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Ice-nucleating particles (INPs) have important influences on cirrus clouds and the climate system; however, the understanding of their global impacts is still uncertain. We perform numerical simulations with a global aerosol–climate model to analyse INP-induced cirrus changes and the resulting climate impacts. We evaluate various sources of uncertainties, e.g. the ice-nucleating ability of INPs and the role of model dynamics, and provide a new estimate for the global INP–cirrus effect.
Jiawei Li, Zhiwei Han, Pingqing Fu, Xiaohong Yao, and Mingjie Liang
Atmos. Chem. Phys., 24, 3129–3161, https://doi.org/10.5194/acp-24-3129-2024, https://doi.org/10.5194/acp-24-3129-2024, 2024
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Organic aerosols of marine origin are important for aerosol climatic effects but are poorly understood. For the first time, an online coupled regional chemistry–climate model is applied to explore the characteristics of emission, distribution, and direct and indirect radiative effects of marine organic aerosols over the western Pacific, which reveals an important role of marine organic aerosols in perturbing cloud and radiation and promotes understanding of global aerosol climatic impact.
Yawen Liu, Yun Qian, Philip J. Rasch, Kai Zhang, Lai-yung Ruby Leung, Yuhang Wang, Minghuai Wang, Hailong Wang, Xin Huang, and Xiu-Qun Yang
Atmos. Chem. Phys., 24, 3115–3128, https://doi.org/10.5194/acp-24-3115-2024, https://doi.org/10.5194/acp-24-3115-2024, 2024
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Fire management has long been a challenge. Here we report that spring-peak fire activity over southern Mexico and Central America (SMCA) has a distinct quasi-biennial signal by measuring multiple fire metrics. This signal is initially driven by quasi-biennial variability in precipitation and is further amplified by positive feedback of fire–precipitation interaction at short timescales. This work highlights the importance of fire–climate interactions in shaping fires on an interannual scale.
Xu Feng, Loretta J. Mickley, Michelle L. Bell, Tianjia Liu, Jenny A. Fisher, and Maria Val Martin
Atmos. Chem. Phys., 24, 2985–3007, https://doi.org/10.5194/acp-24-2985-2024, https://doi.org/10.5194/acp-24-2985-2024, 2024
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During severe wildfire seasons, smoke can have a significant impact on air quality in Australia. Our study demonstrates that characterization of the smoke plume injection fractions greatly affects estimates of surface smoke PM2.5. Using the plume behavior predicted by the machine learning method leads to the best model agreement with observed surface PM2.5 in key cities across Australia, with smoke PM2.5 accounting for 5 %–52 % of total PM2.5 on average during fire seasons from 2009 to 2020.
Shiyi Lai, Ximeng Qi, Xin Huang, Sijia Lou, Xuguang Chi, Liangduo Chen, Chong Liu, Yuliang Liu, Chao Yan, Mengmeng Li, Tengyu Liu, Wei Nie, Veli-Matti Kerminen, Tuukka Petäjä, Markku Kulmala, and Aijun Ding
Atmos. Chem. Phys., 24, 2535–2553, https://doi.org/10.5194/acp-24-2535-2024, https://doi.org/10.5194/acp-24-2535-2024, 2024
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By combining in situ measurements and chemical transport modeling, this study investigates new particle formation (NPF) on the southeastern Tibetan Plateau. We found that the NPF was driven by the presence of biogenic gases and the transport of anthropogenic precursors. The NPF was vertically heterogeneous and shaped by the vertical mixing. This study highlights the importance of anthropogenic–biogenic interactions and meteorological dynamics in NPF in this climate-sensitive region.
Adriana Rocha-Lima, Peter R. Colarco, Anton S. Darmenov, Edward P. Nowottnick, Arlindo M. da Silva, and Luke D. Oman
Atmos. Chem. Phys., 24, 2443–2464, https://doi.org/10.5194/acp-24-2443-2024, https://doi.org/10.5194/acp-24-2443-2024, 2024
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Observations show an increasing aerosol optical depth trend in the Middle East between 2003–2012. We evaluate the NASA Goddard Earth Observing System (GEOS) model's ability to capture these trends and examine the meteorological and surface parameters driving dust emissions. Our results highlight the importance of data assimilation for long-term trends of atmospheric aerosols and support the hypothesis that vegetation cover loss may have contributed to increasing dust emissions in the period.
Danny M. Leung, Jasper F. Kok, Longlei Li, Natalie M. Mahowald, David M. Lawrence, Simone Tilmes, Erik Kluzek, Martina Klose, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 24, 2287–2318, https://doi.org/10.5194/acp-24-2287-2024, https://doi.org/10.5194/acp-24-2287-2024, 2024
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This study uses a premier Earth system model to evaluate a new desert dust emission scheme proposed in our companion paper. We show that our scheme accounts for more dust emission physics, hence matching better against observations than other existing dust emission schemes do. Our scheme's dust emissions also couple tightly with meteorology, hence likely improving the modeled dust sensitivity to climate change. We believe this work is vital for improving dust representation in climate models.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-440, https://doi.org/10.5194/egusphere-2024-440, 2024
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Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW AOD data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine understanding of aerosol effects on cloud microphysics, ice nucleation and radiative forcing under evolving AA.
Ruth A. R. Digby, Nathan P. Gillett, Adam H. Monahan, Knut von Salzen, Antonis Gkikas, Qianqian Song, and Zhibo Zhang
Atmos. Chem. Phys., 24, 2077–2097, https://doi.org/10.5194/acp-24-2077-2024, https://doi.org/10.5194/acp-24-2077-2024, 2024
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The COVID-19 lockdowns reduced aerosol emissions. We ask whether these reductions affected regional aerosol optical depth (AOD) and compare the observed changes to predictions from Earth system models. Only India has an observed AOD reduction outside of typical variability. Models overestimate the response in some regions, but when key biases have been addressed, the agreement is improved. Our results suggest that current models can realistically predict the effects of future emission changes.
Huisheng Bian, Mian Chin, Peter R. Colarco, Eric C. Apel, Donald R. Blake, Karl Froyd, Rebecca S. Hornbrook, Jose Jimenez, Pedro Campuzano Jost, Michael Lawler, Mingxu Liu, Marianne Tronstad Lund, Hitoshi Matsui, Benjamin A. Nault, Joyce E. Penner, Andrew W. Rollins, Gregory Schill, Ragnhild B. Skeie, Hailong Wang, Lu Xu, Kai Zhang, and Jialei Zhu
Atmos. Chem. Phys., 24, 1717–1741, https://doi.org/10.5194/acp-24-1717-2024, https://doi.org/10.5194/acp-24-1717-2024, 2024
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This work studies sulfur in the remote troposphere at global and seasonal scales using aircraft measurements and multi-model simulations. The goal is to understand the sulfur cycle over remote oceans, spread of model simulations, and observation–model discrepancies. Such an understanding and comparison with real observations are crucial to narrow down the uncertainties in model sulfur simulations and improve understanding of the sulfur cycle in atmospheric air quality, climate, and ecosystems.
Gargi Sengupta, Minjie Zheng, and Nønne L. Prisle
Atmos. Chem. Phys., 24, 1467–1487, https://doi.org/10.5194/acp-24-1467-2024, https://doi.org/10.5194/acp-24-1467-2024, 2024
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The effect of organic acid aerosol on sulfur chemistry and cloud properties was investigated in an atmospheric model. Organic acid dissociation was considered using both bulk and surface-related properties. We found that organic acid dissociation leads to increased hydrogen ion concentrations and sulfate aerosol mass in aqueous aerosols, increasing cloud formation. This could be important in large-scale climate models as many organic aerosol components are both acidic and surface-active.
Leena Kangas, Jaakko Kukkonen, Mari Kauhaniemi, Kari Riikonen, Mikhail Sofiev, Anu Kousa, Jarkko V. Niemi, and Ari Karppinen
Atmos. Chem. Phys., 24, 1489–1507, https://doi.org/10.5194/acp-24-1489-2024, https://doi.org/10.5194/acp-24-1489-2024, 2024
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Residential wood combustion is a major source of fine particulate matter. This study has evaluated the contribution of residential wood combustion to fine particle concentrations and its year-to-year and seasonal variation in te Helsinki metropolitan area. The average concentrations attributed to wood combustion in winter were up to 10- or 15-fold compared to summer. Wood combustion caused 12 % to 14 % of annual fine particle concentrations. In winter, the contribution ranged from 16 % to 21 %.
Arto Heitto, Cheng Wu, Diego Aliaga, Luis Blacutt, Xuemeng Chen, Yvette Gramlich, Liine Heikkinen, Wei Huang, Radovan Krejci, Paolo Laj, Isabel Moreno, Karine Sellegri, Fernando Velarde, Kay Weinhold, Alfred Wiedensohler, Qiaozhi Zha, Federico Bianchi, Marcos Andrade, Kari E. J. Lehtinen, Claudia Mohr, and Taina Yli-Juuti
Atmos. Chem. Phys., 24, 1315–1328, https://doi.org/10.5194/acp-24-1315-2024, https://doi.org/10.5194/acp-24-1315-2024, 2024
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Particle growth at the Chacaltaya station in Bolivia was simulated based on measured vapor concentrations and ambient conditions. Major contributors to the simulated growth were low-volatility organic compounds (LVOCs). Also, sulfuric acid had major role when volcanic activity was occurring in the area. This study provides insight on nanoparticle growth at this high-altitude Southern Hemispheric site and hence contributes to building knowledge of early growth of atmospheric particles.
Steven Soon-Kai Kong, Saginela Ravindra Babu, Sheng-Hsiang Wang, Stephen M. Griffith, Jackson Hian-Wui Chang, Ming-Tung Chuang, Guey-Rong Sheu, and Neng-Huei Lin
Atmos. Chem. Phys., 24, 1041–1058, https://doi.org/10.5194/acp-24-1041-2024, https://doi.org/10.5194/acp-24-1041-2024, 2024
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In this study, we combined ground observations from 7-SEAS Dongsha Experiment, MERRA-2 reanalysis, and MODIS satellite images for evaluation and improvement of the CMAQ dust model for cases of East Asian Dust reaching the Taiwan region, including Dongsha in the western Pacific. We proposed a better CMAQ dust treatment over East Asia and for the first time revealed the impact of typhoons on dust transport.
Zhiguo Zhang, Christer Johansson, Magnuz Engardt, Massimo Stafoggia, and Xiaoliang Ma
Atmos. Chem. Phys., 24, 807–851, https://doi.org/10.5194/acp-24-807-2024, https://doi.org/10.5194/acp-24-807-2024, 2024
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Up-to-date information on present and near-future air quality help people avoid exposure to high levels of air pollution. We apply different machine learning models to significantly improve traditional forecasts of PM10, NOx, and O3 in Stockholm, Sweden. It is shown that forecasts of all air pollutants are improved by the input of lagged measurements and taking calendar information into account. The final modelled errors are substantially smaller than uncertainties in the measurements.
Natalie M. Mahowald, Longlei Li, Samuel Albani, Douglas S. Hamilton, and Jasper F. Kok
Atmos. Chem. Phys., 24, 533–551, https://doi.org/10.5194/acp-24-533-2024, https://doi.org/10.5194/acp-24-533-2024, 2024
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Estimating past aerosol radiative effects and their uncertainties is an important topic in climate science. Aerosol radiative effects propagate into large uncertainties in estimates of how present and future climate evolves with changing greenhouse gas emissions. A deeper understanding of how aerosols interacted with the atmospheric energy budget under past climates is hindered in part by a lack of relevant paleo-observations and in part because less attention has been paid to the problem.
Min Zhao, Tie Dai, Daisuke Goto, Hao Wang, and Guangyu Shi
Atmos. Chem. Phys., 24, 235–258, https://doi.org/10.5194/acp-24-235-2024, https://doi.org/10.5194/acp-24-235-2024, 2024
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During a springtime pollution input from South Asia to the Tibetan Plateau, we combined atmospheric chemistry modeling and data assimilation methods to assimilate and forecast aerosols from South Asia and the Tibetan Plateau. Assimilation of observations over a whole time window leads to a more reasonable distribution of daily variations in the aerosol forecast field. We also find that aerosol assimilation can improve the surface solar energy forecast in the Tibetan Plateau region.
Yuling Hu, Haipeng Yu, Shichang Kang, Junhua Yang, Mukesh Rai, Xiufeng Yin, Xintong Chen, and Pengfei Chen
Atmos. Chem. Phys., 24, 85–107, https://doi.org/10.5194/acp-24-85-2024, https://doi.org/10.5194/acp-24-85-2024, 2024
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The Tibetan Plateau (TP) saw a record-breaking aerosol pollution event from April 20 to May 10, 2016. We studied the impact of aerosol–meteorology feedback on the transboundary transport flux of black carbon (BC) during this severe pollution event. It was found that the aerosol–meteorology feedback decreases the transboundary transport flux of BC from the central and western Himalayas towards the TP. This study is of great significance for the protection of the ecological environment of the TP.
Xiaodong Zhang, Ruiyu Zhugu, Xiaohu Jian, Xinrui Liu, Kaijie Chen, Shu Tao, Junfeng Liu, Hong Gao, Tao Huang, and Jianmin Ma
Atmos. Chem. Phys., 23, 15629–15642, https://doi.org/10.5194/acp-23-15629-2023, https://doi.org/10.5194/acp-23-15629-2023, 2023
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WRF-Chem modeling was conducted to assess impacts of Western Pacific Subtropical High Pressure (WPSH) on interannual fluctuations of O3 pollution in China. We find that, while precursor emissions dominated the long-term trend and magnitude of O3 from 1999 to 2017, WPSH determined interannual variation of summer O3. The response of O3 pollution to WPSH in major urban clusters depended on the proximity of these urban areas to WPSH. The results could help long-term O3 pollution mitigation planning.
Jim M. Haywood, Andy Jones, Anthony C. Jones, Paul Halloran, and Philip J. Rasch
Atmos. Chem. Phys., 23, 15305–15324, https://doi.org/10.5194/acp-23-15305-2023, https://doi.org/10.5194/acp-23-15305-2023, 2023
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The difficulties in ameliorating global warming and the associated climate change via conventional mitigation are well documented, with all climate model scenarios exceeding 1.5 °C above the preindustrial level in the near future. There is therefore a growing interest in geoengineering to reflect a greater proportion of sunlight back to space and offset some of the global warming. We use a state-of-the-art Earth-system model to investigate two of the most prominent geoengineering strategies.
Sampo Vepsäläinen, Silvia M. Calderón, and Nønne L. Prisle
Atmos. Chem. Phys., 23, 15149–15164, https://doi.org/10.5194/acp-23-15149-2023, https://doi.org/10.5194/acp-23-15149-2023, 2023
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Atmospheric aerosols act as seeds for cloud formation. Many aerosols contain surface active material that accumulates at the surface of growing droplets. This can affect cloud droplet activation, but the broad significance of the effect and the best way to model it are still debated. We compare predictions of six models to surface activity of strongly surface active aerosol and find significant differences between the models, especially with large fractions of surfactant in the dry particles.
Da Gao, Bin Zhao, Shuxiao Wang, Yuan Wang, Brian Gaudet, Yun Zhu, Xiaochun Wang, Jiewen Shen, Shengyue Li, Yicong He, Dejia Yin, and Zhaoxin Dong
Atmos. Chem. Phys., 23, 14359–14373, https://doi.org/10.5194/acp-23-14359-2023, https://doi.org/10.5194/acp-23-14359-2023, 2023
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Surface PM2.5 concentrations can be enhanced by aerosol–radiation interactions (ARIs) and aerosol–cloud interactions (ACIs). In this study, we found PM2.5 enhancement induced by ACIs shows a significantly smaller decrease ratio than that induced by ARIs in China with anthropogenic emission reduction from 2013 to 2021, making ACIs more important for enhancing PM2.5 concentrations. ACI-induced PM2.5 enhancement needs to be emphatically considered to meet the national PM2.5 air quality standard.
Miaoqing Xu, Jing Yang, Manchun Li, Xiao Chen, Qiancheng Lv, Qi Yao, Bingbo Gao, and Ziyue Chen
Atmos. Chem. Phys., 23, 14065–14076, https://doi.org/10.5194/acp-23-14065-2023, https://doi.org/10.5194/acp-23-14065-2023, 2023
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Although the temporal-scale effects on PM2.5–meteorology associations have been discussed, no quantitative evidence has proved this before. Based on rare 3 h meteorology data, we revealed that the dominant meteorological factor for PM2.5 concentrations across China extracted at the 3 h and 24 h scales presented large variations. This research suggests that data sources of different temporal scales should be comprehensively considered for better attribution and prevention of airborne pollution.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Michael Weger and Bernd Heinold
Atmos. Chem. Phys., 23, 13769–13790, https://doi.org/10.5194/acp-23-13769-2023, https://doi.org/10.5194/acp-23-13769-2023, 2023
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This study investigates the effects of complex terrain on air pollution trapping using a numerical model which simulates the dispersion of emissions under real meteorological conditions. The additionally simulated aerosol age allows us to distinguish areas that accumulate aerosol over time from areas that are more influenced by fresh emissions. The Dresden Basin, a widened section of the Elbe Valley in eastern Germany, is selected as the target area in a case study to demonstrate the concept.
Noora Hyttinen
Atmos. Chem. Phys., 23, 13809–13817, https://doi.org/10.5194/acp-23-13809-2023, https://doi.org/10.5194/acp-23-13809-2023, 2023
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Water activity in aerosol particles describes how particles respond to variations in relative humidity. Here, water activities were calculated for a set of 80 salts that may be present in aerosol particles using a state-of-the-art quantum-chemistry-based method. The effect of the dissociated salt on water activity varies with both the cation and anion. Most of the studied salts increase water uptake compared to pure water-soluble organic particles.
Charlotte M. Beall, Po-Lun Ma, Matthew W. Christensen, Johannes Mülmenstädt, Adam Varble, Kentaroh Suzuki, and Takuro Michibata
EGUsphere, https://doi.org/10.5194/egusphere-2023-2161, https://doi.org/10.5194/egusphere-2023-2161, 2023
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Single-layer warm liquid clouds cover nearly one-third of the earth's surface, and uncertainties regarding the impact of aerosols on their radiative properties pose a significant challenge to climate prediction. Here, we demonstrate how satellite observations can be used to constrain Earth Systems Model estimates of the radiative forcing due to the interactions of aerosols with clouds due to warm rain processes.
Peng Xian, Jeffrey S. Reid, Melanie Ades, Angela Benedettie, Peter R. Colarco, Arlindo da Silva, Tom F. Eck, Johannes Flemming, Edward J. Hyer, Zak Kipling, Samuel Rémy, Tsuyoshi Thomas Sekiyama, Taichu Tanaka, Keiya Yumimoto, and Jianglong Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2023-2354, https://doi.org/10.5194/egusphere-2023-2354, 2023
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The study compares and evaluates the monthly aerosol optical depth of four reanalyses (RA) and their consensus. The basic verification characteristics of these RA versus both AERONET and MODIS retrievals are presented. The study discusses the strength of each RA and identifies regions where diversity and challenges are prominent. The RA consensus usually performs very well on a global scale in terms of how well it matches the observational data, making it a good choice for various applications.
Lambert Delbeke, Chien Wang, Pierre Tulet, Cyrielle Denjean, Maurin Zouzoua, Nicolas Maury, and Adrien Deroubaix
Atmos. Chem. Phys., 23, 13329–13354, https://doi.org/10.5194/acp-23-13329-2023, https://doi.org/10.5194/acp-23-13329-2023, 2023
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Low-level stratiform clouds (LLSCs) appear frequently over southern West Africa during the West African monsoon. Local and remote aerosol sources (biomass burning aerosols from central Africa) play a significant role in the LLSC life cycle. Based on measurements by the DACCIWA campaign, large-eddy simulation (LES) was conducted using different aerosol scenarios. The results show that both indirect and semi-direct effects can act individually or jointly to influence the life cycles of LLSCs.
Matthias Kohl, Jos Lelieveld, Sourangsu Chowdhury, Sebastian Ehrhart, Disha Sharma, Yafang Cheng, Sachchida Nand Tripathi, Mathew Sebastian, Govindan Pandithurai, Hongli Wang, and Andrea Pozzer
Atmos. Chem. Phys., 23, 13191–13215, https://doi.org/10.5194/acp-23-13191-2023, https://doi.org/10.5194/acp-23-13191-2023, 2023
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Knowledge on atmospheric ultrafine particles (UFPs) with a diameter smaller than 100 nm is crucial for public health and the hydrological cycle. We present a new global dataset of UFP concentrations at the Earth's surface derived with a comprehensive chemistry–climate model and evaluated with ground-based observations. The evaluation results are combined with high-resolution primary emissions to downscale UFP concentrations to an unprecedented horizontal resolution of 0.1° × 0.1°.
Haotian Zu, Biwu Chu, Yiqun Lu, Ling Liu, and Xiuhui Zhang
EGUsphere, https://doi.org/10.5194/egusphere-2023-1774, https://doi.org/10.5194/egusphere-2023-1774, 2023
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The nucleation process of iodic acid (HIO3) and iodous acid (HIO2) was proved to be critical in marine areas. However, HIO3-HIO2 nucleation cannot effectively derive the observed rapid new particle formation in broad marine areas. We show the extensive participation of dimethylamine (DMA) in HIO3-HIO2 nucleation and find a significant enhancement of DMA on the HIO3-HIO2 nucleation, which establishes reasonable connections between the iodine oxoacids nucleation and the rapid marine new particles.
Alejandro Baró Pérez, Michael S. Diamond, Frida A.-M. Bender, Abhay Devasthale, Matthias Schwarz, Julien Savre, Juha Tonttila, Harri Kokkola, Hyunho Lee, David Painemal, and Annica M. L. Ekman
EGUsphere, https://doi.org/10.5194/egusphere-2023-2070, https://doi.org/10.5194/egusphere-2023-2070, 2023
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We use a numerical model to study interactions between humid light-absorbing aerosol plumes, clouds, and radiation over the Southeast Atlantic. We find that the warming produced by the aerosols reduces cloud cover, especially in highly polluted situations. Aerosol impacts on drizzle play a minor role. However, aerosol effects on cloud reflectivity and moisture-induced changes in cloud cover dominate the climatic response and lead to an overall cooling by the biomass-burning plumes.
Roger Teoh, Zebediah Engberg, Ulrich Schumann, Christiane Voigt, Marc Shapiro, Susanne Rohs, and Marc Stettler
EGUsphere, https://doi.org/10.5194/egusphere-2023-1859, https://doi.org/10.5194/egusphere-2023-1859, 2023
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The radiative forcing attributable to aviation contrails is estimated for 2019–21. We estimate a global contrail net RF that is approximately half the best estimate of a previous study. Contrail climate impacts have not scaled proportionally with air traffic growth due to higher growth in regions where contrails are less likely to form. There are significant opportunities to mitigate contrail impacts as only 2 % of all flights globally account for 80 % of the annual contrail energy forcing.
Xiaoli Wei, Qian Cui, Leiming Ma, Feng Zhang, Wenwen Li, and Peng Liu
EGUsphere, https://doi.org/10.5194/egusphere-2023-1754, https://doi.org/10.5194/egusphere-2023-1754, 2023
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A new aerosol-type classification algorithm was proposed. It includes an optical database building by Mie scattering and a complex refractive index working as a baseline to identify different aerosol types. The new algorithm shows high accuracy and efficiency. Hence, a global map of aerosol types was generated using the new algorithm to characterize aerosol types across the five continents. It will help improve the accuracy of aerosol inversion and determine the sources of aerosol pollution.
Wenxuan Hua, Sijia Lou, Xin Huang, Lian Xue, Ke Ding, Zilin Wang, and Aijun Ding
EGUsphere, https://doi.org/10.5194/egusphere-2023-1822, https://doi.org/10.5194/egusphere-2023-1822, 2023
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In this study, we diagnose uncertainties in CO and OC emissions from four inventories for seven majorwildfire-prone regions. Uncertainties in vegetation classification methods, fire detection products, and cloud obscuration effects lead to bias in these biomass burning (BB) emission inventories. By comparing simulations with measurements, we provide certain inventory recommendations. Our study has implications for reducing uncertainties in emissions in further studies.
Jun-Wei Xu, Jintai Lin, Dan Tong, and Lulu Chen
Atmos. Chem. Phys., 23, 10075–10089, https://doi.org/10.5194/acp-23-10075-2023, https://doi.org/10.5194/acp-23-10075-2023, 2023
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This study highlights the necessity of a low-carbon pathway in foreign countries for China to achieve air quality goals and to protect public health. We find that adopting the low-carbon instead of the fossil-fuel-intensive pathway in foreign countries would prevent 63 000–270 000 transboundary PM2.5-associated mortalities in China in 2060. Our study provides direct evidence of the necessity of inter-regional cooperation for air quality improvement.
Xurong Wang, Qiaoqiao Wang, Maria Prass, Christopher Pöhlker, Daniel Moran-Zuloaga, Paulo Artaxo, Jianwei Gu, Ning Yang, Xiajie Yang, Jiangchuan Tao, Juan Hong, Nan Ma, Yafang Cheng, Hang Su, and Meinrat O. Andreae
Atmos. Chem. Phys., 23, 9993–10014, https://doi.org/10.5194/acp-23-9993-2023, https://doi.org/10.5194/acp-23-9993-2023, 2023
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In this work, with an optimized particle mass size distribution, we captured observed aerosol optical depth (AOD) and coarse aerosol concentrations over source and/or receptor regions well, demonstrating good performance in simulating export of African dust toward the Amazon Basin. In addition to factors controlling the transatlantic transport of African dust, the study investigated the impact of African dust over the Amazon Basin, including the nutrient inputs associated with dust deposition.
Athanasios Tsikerdekis, Otto P. Hasekamp, Nick A. J. Schutgens, and Qirui Zhong
Atmos. Chem. Phys., 23, 9495–9524, https://doi.org/10.5194/acp-23-9495-2023, https://doi.org/10.5194/acp-23-9495-2023, 2023
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Aerosols are tiny particles of different substances (species) that can be emitted into the atmosphere by natural processes or by anthropogenic activities. However, the actual aerosol emission amount per species is highly uncertain. Thus in this work we correct the aerosol emissions used to drive a global aerosol–climate model using satellite observations through a process called data assimilation. These more accurate aerosol emissions can lead to a more accurate weather and climate prediction.
Chandrakala Bharali, Mary Barth, Rajesh Kumar, Sachin D. Ghude, Vinayak Sinha, and Baerbel Sinha
EGUsphere, https://doi.org/10.5194/egusphere-2023-1686, https://doi.org/10.5194/egusphere-2023-1686, 2023
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This study examines the role of atmospheric aerosols in winter fog over the Indo-Gangetic Plains of India using the WRF-Chem model. The increase in RH with aerosol-radiation feedback (ARF) is found to be important for fog formation as it promoted the growth of aerosol and increased aerosol activation in the polluted environment. ARF and aqueous phase chemistry affected the timing of fog formation by ~1–2 hours and the fog intensity by modulating the meteorology and aerosol concentration.
Jani Strömberg, Xiaoyu Li, Mona Kurppa, Heino Kuuluvainen, Liisa Pirjola, and Leena Järvi
Atmos. Chem. Phys., 23, 9347–9364, https://doi.org/10.5194/acp-23-9347-2023, https://doi.org/10.5194/acp-23-9347-2023, 2023
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We conclude that with low wind speeds, solar radiation has a larger decreasing effect (53 %) on pollutant concentrations than aerosol processes (18 %). Additionally, our results showed that with solar radiation included, pollutant concentrations were closer to observations (−13 %) than with only aerosol processes (+98 %). This has implications when planning simulations under calm conditions such as in our case and when deciding whether or not simulations need to include these processes.
Junghwa Lee, Patric Seifert, Tempei Hashino, Maximilian Maahn, Fabian Senf, and Oswald Knoth
EGUsphere, https://doi.org/10.5194/egusphere-2023-1887, https://doi.org/10.5194/egusphere-2023-1887, 2023
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Spectral-bin model simulations of an idealized supercooled stratiform cloud were performed with the AMPS model for variable CCN and INP concentrations. We performed radar forward simulations with PAMTRA to transfer the simulations into radar observational space. The derived radar reflectivity factors were compared to observational studies of stratiform mixed-phase clouds. These studies report a similar response of the radar reflectivity factor to aerosol perturbations as we found in our study.
Guanyu Liu, Jing Li, and Tong Ying
Atmos. Chem. Phys., 23, 9217–9228, https://doi.org/10.5194/acp-23-9217-2023, https://doi.org/10.5194/acp-23-9217-2023, 2023
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Fires in Australia are positively correlated with the El Niño–Southern Oscillation (ENSO). However, the correlation between ENSO and the Australian Fire Weather Index (FWI) increases from 0.17 to 0.70 when the Atlantic Multidecadal Oscillation (AMO) shifts from a negative to positive phase. This is explained by the teleconnection effect through which the warmer AMO generates Rossby wave trains and results in high pressures and a weather condition conducive to wildfires.
Zhiqiang Zhang, Ying Li, Haiyan Ran, Junling An, Yu Qu, Wei Zhou, Weiqi Xu, Weiwei Hu, Hongbin Xie, Zifa Wang, Yele Sun, and Manabu Shiraiwa
EGUsphere, https://doi.org/10.5194/egusphere-2023-1444, https://doi.org/10.5194/egusphere-2023-1444, 2023
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Secondary organic aerosols (SOA) can exist in liquid, semi-solid or amorphous solid states, which are rarely accounted for in current chemical transport models. We predict the phase state of SOA particles over China and find that in the northwestern China SOA particles are mostly highly viscous or glassy solid. Our results indicate that the particle phase state should be considered in SOA formation in chemical transport models for more accurate prediction of SOA mass concentrations.
Leighton A. Regayre, Lucia Deaconu, Daniel P. Grosvenor, David M. H. Sexton, Christopher Symonds, Tom Langton, Duncan Watson-Paris, Jane P. Mulcahy, Kirsty J. Pringle, Mark Richardson, Jill S. Johnson, John W. Rostron, Hamish Gordon, Grenville Lister, Philip Stier, and Ken S. Carslaw
Atmos. Chem. Phys., 23, 8749–8768, https://doi.org/10.5194/acp-23-8749-2023, https://doi.org/10.5194/acp-23-8749-2023, 2023
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Aerosol forcing of Earth’s energy balance has persisted as a major cause of uncertainty in climate simulations over generations of climate model development. We show that structural deficiencies in a climate model are exposed by comprehensively exploring parametric uncertainty and that these deficiencies limit how much the model uncertainty can be reduced through observational constraint. This provides a future pathway towards building models with greater physical realism and lower uncertainty.
Cited articles
Adebiyi, A. A. and Kok, J. F.: Climate models miss most of the coarse dust
in the atmosphere, Sci. Adv., 6, eaaz9507,
https://doi.org/10.1126/sciadv.aaz9507, 2020.
Adebiyi, A. A., Kok, J. F., Wang, Y., Ito, A., Ridley, D. A., Nabat, P., and Zhao, C.: Dust Constraints from joint Observational-Modelling-experiMental analysis (DustCOMM): comparison with measurements and model simulations, Atmos. Chem. Phys., 20, 829–863, https://doi.org/10.5194/acp-20-829-2020, 2020.
Albrecht, B. A.: Aerosols, Cloud Microphysics, and Fractional Cloudiness,
Science, 80, 1227–1230, https://doi.org/10.1126/science.245.4923.1227, 1989.
Balkanski, Y., Schulz, M., Claquin, T., and Guibert, S.: Reevaluation of Mineral aerosol radiative forcings suggests a better agreement with satellite and AERONET data, Atmos. Chem. Phys., 7, 81–95, https://doi.org/10.5194/acp-7-81-2007, 2007.
Brindley, H. E. and Russell, J. E.: An assessment of Saharan dust loading
and the corresponding cloud-free longwave direct radiative effect from
geostationary satellite observations, J. Geophys. Res.-Atmos., 114, D23201,
https://doi.org/10.1029/2008JD011635, 2009.
Choobari, O. A., Zawar-Reza, P., and Sturman, A.: The global distribution of
mineral dust and its impacts on the climate system: A review, Atmos. Res.,
138, 152–165, https://doi.org/10.1016/j.atmosres.2013.11.007, 2014.
Colarco, P. R., Nowottnick, E. P., Randles, C. A., Yi, B. Q., Yang, P., Kim,
K. M., Smith, J. A., and Bardeen, C. G.: Impact of radiatively interactive
dust aerosols in the NASA GEOS-5 climate model: Sensitivity to dust particle
shape and refractive index, J. Geophys. Res., 119, 753–786,
https://doi.org/10.1002/2013jd020046, 2014.
Di Biagio, C., Formenti, P., Balkanski, Y., Caponi, L., Cazaunau, M., Pangui, E., Journet, E., Nowak, S., Caquineau, S., Andreae, M. O., Kandler, K., Saeed, T., Piketh, S., Seibert, D., Williams, E., and Doussin, J.-F.: Global scale variability of the mineral dust long-wave refractive index: a new dataset of in situ measurements for climate modeling and remote sensing, Atmos. Chem. Phys., 17, 1901–1929, https://doi.org/10.5194/acp-17-1901-2017, 2017.
Di Biagio, C., Formenti, P., Balkanski, Y., Caponi, L., Cazaunau, M., Pangui, E., Journet, E., Nowak, S., Andreae, M. O., Kandler, K., Saeed, T., Piketh, S., Seibert, D., Williams, E., and Doussin, J.-F.: Complex refractive indices and single-scattering albedo of global dust aerosols in the shortwave spectrum and relationship to size and iron content, Atmos. Chem. Phys., 19, 15503–15531, https://doi.org/10.5194/acp-19-15503-2019, 2019.
Di Biagio, C., Balkanski, Y., Albani, S., Boucher, O., and Formenti, P.:
Direct Radiative Effect by Mineral Dust Aerosols Constrained by New
Microphysical and Spectral Optical Data, Geophys. Res. Lett., 47,
e2019GL086186, https://doi.org/https://doi.org/10.1029/2019GL086186, 2020.
Drakaki, E., Amiridis, V., Tsekeri, A., Gkikas, A., Proestakis, E., Mallios, S., Solomos, S., Spyrou, C., Marinou, E., Ryder, C. L., Bouris, D., and Katsafados, P.: Modeling coarse and giant desert dust particles, Atmos. Chem. Phys., 22, 12727–12748, https://doi.org/10.5194/acp-22-12727-2022, 2022.
Dubovik, O., Sinyuk, A., Lapyonok, T., Holben, B. N., Mishchenko, M., Yang,
P., Eck, T. F., Volten, H., Munoz, O., Veihelmann, B., van der Zande, W. J.,
Leon, J. F., Sorokin, M., and Slutsker, I.: Application of spheroid models
to account for aerosol particle nonsphericity in remote sensing of desert
dust, J. Geophys. Res., 111, D11208, https://doi.org/10.1029/2005jd006619, 2006.
Dufresne, J. L., Gautier, C., and Ricchiazzi, P.: Longwave scattering
effects of mineral aerosols, J. Atmos. Sci., 59, 1959–1966,
https://doi.org/10.1175/1520-0469(2002)059<1959:LSEOMA>2.0.CO;2, 2002.
García, O. E., Díez, A. M., Expósito, F. J., Díaz, J. P.,
Dubovik, O., Dubuisson, P., Roger, J. C., Eck, T. F., Sinyuk, A., Derimian,
Y., Dutton, E. G., Schafer, J. S., Holben, B., and García, C. A.:
Validation of AERONET estimates of atmospheric solar fluxes and aerosol
radiative forcing by ground-based broadband measurements, J. Geophys. Res.-Atmos., 113, D21207, https://doi.org/10.1029/2008JD010211, 2008.
Gelaro, R., McCarty, W., Suárez, M. J., Todling, R., Molod, A., Takacs,
L., Randles, C. A., Darmenov, A., Bosilovich, M. G., Reichle, R., Wargan,
K., Coy, L., Cullather, R., Draper, C., Akella, S., Buchard, V., Conaty, A.,
da Silva, A. M., Gu, W., Kim, G. K., Koster, R., Lucchesi, R., Merkova, D.,
Nielsen, J. E., Partyka, G., Pawson, S., Putman, W., Rienecker, M.,
Schubert, S. D., Sienkiewicz, M., and Zhao, B.: The modern-era retrospective
analysis for research and applications, version 2 (MERRA-2), J. Climate, 30,
5419–5454, https://doi.org/10.1175/JCLI-D-16-0758.1, 2017.
Ginoux, P., Prospero, J. M., Gill, T. E., Hsu, N. C., and Zhao, M.:
Global-scale attribution of anthropogenic and natural dust sources and their
emission rates based on MODIS Deep Blue aerosol products, Rev. Geophys., 50, RG3005,
https://doi.org/10.1029/2012RG000388, 2012.
Gkikas, A., Proestakis, E., Amiridis, V., Kazadzis, S., Di Tomaso, E., Tsekeri, A., Marinou, E., Hatzianastassiou, N., and Pérez García-Pando, C.: ModIs Dust AeroSol (MIDAS): a global fine-resolution dust optical depth data set, Atmos. Meas. Tech., 14, 309–334, https://doi.org/10.5194/amt-14-309-2021, 2021.
Hansell, R. A., Tsay, S. C., Ji, Q., Hsu, N. C., Jeong, M. J., Wang, S. H.,
Reid, J. S., Liou, K. N., and Ou, S. C.: An assessment of the surface
longwave direct radiative effect of airborne Saharan dust during the NAMMA
field campaign, J. Atmos. Sci., 67, 1048–1065,
https://doi.org/10.1175/2009JAS3257.1, 2010.
Hsu, N. C., Jeong, M.-J., Bettenhausen, C., Sayer, A. M., Hansell, R.,
Seftor, C. S., Huang, J., and Tsay, S.-C.: Enhanced Deep Blue aerosol
retrieval algorithm: The second generation, J. Geophys. Res.-Atmos., 118,
9296–9315, https://doi.org/https://doi.org/10.1002/jgrd.50712, 2013.
Huang, X. L., Chen, X. H., Zhou, D. K., and Liu, X.: An Observationally Based Global Band-by-Band Surface Emissivity Dataset for Climate and Weather Simulations, J. Atmos. Sci., 73, 3541–3555, https://doi.org/10.1175/Jas-D-15-0355.1, 2016.
Huang, Y., Kok, J. F., Kandler, K., Lindqvist, H., Nousiainen, T., Sakai,
T., Adebiyi, A., and Jokinen, O.: Climate Models and Remote Sensing
Retrievals Neglect Substantial Desert Dust Asphericity, Geophys. Res. Lett.,
47, e2019GL086592, https://doi.org/10.1029/2019GL086592, 2020.
Huneeus, N., Schulz, M., Balkanski, Y., Griesfeller, J., Prospero, J., Kinne, S., Bauer, S., Boucher, O., Chin, M., Dentener, F., Diehl, T., Easter, R., Fillmore, D., Ghan, S., Ginoux, P., Grini, A., Horowitz, L., Koch, D., Krol, M. C., Landing, W., Liu, X., Mahowald, N., Miller, R., Morcrette, J.-J., Myhre, G., Penner, J., Perlwitz, J., Stier, P., Takemura, T., and Zender, C. S.: Global dust model intercomparison in AeroCom phase I, Atmos. Chem. Phys., 11, 7781–7816, https://doi.org/10.5194/acp-11-7781-2011, 2011.
Kato, S., Rose, F. G., Sun-Mack, S., Miller, W. F., Chen, Y., Rutan, D. A.,
Stephens, G. L., Loeb, N. G., Minnis, P., Wielicki, B. A., Winker, D. M.,
Charlock, T. P., Stackhouse, P. W., Xu, K. M., and Collins, W. D.:
Improvements of top-of-atmosphere and surface irradiance computations with
CALIPSO-, CloudSat-, and MODIS-derived cloud and aerosol properties, J.
Geophys. Res., 116, D19209, https://doi.org/10.1029/2011jd016050, 2011.
Kaufman, Y. J., Koren, I., Remer, L. A., Tanré, D., Ginoux, P., and Fan,
S.: Dust transport and deposition observed from the Terra-Moderate
Resolution Imaging Spectroradiometer (MODIS) spacecraft over the Atlantic
Ocean, J. Geophys. Res.-Atmos., 110, 1–16,
https://doi.org/10.1029/2003JD004436, 2005.
Koffi, B., Schulz, M., Bréon, F. M., Griesfeller, J., Winker, D.,
Balkanski, Y., Bauer, S., Berntsen, T., Chin, M., Collins, W. D., Dentener,
F., Diehl, T., Easter, R., Ghan, S., Ginoux, P., Gong, S., Horowitz, L. W.,
Iversen, T., Kirkevg, A., Koch, D., Krol, M., Myhre, G., Stier, P., and
Takemura, T.: Application of the CALIOP layer product to evaluate the
vertical distribution of aerosols estimated by global models: AeroCom phase
i results, J. Geophys. Res.-Atmos., 117, D10201, https://doi.org/10.1029/2011JD016858, 2012.
Kok, J. F., Ridley, D. A., Zhou, Q., Miller, R. L., Zhao, C., Heald, C. L.,
Ward, D. S., Albani, S., and Haustein, K.: Smaller desert dust cooling
effect estimated from analysis of dust size and abundance, Nat. Geosci., 10,
274–278, https://doi.org/10.1038/Ngeo2912, 2017.
Li, F., Vogelmann, A. M., and Ramanathan, V.: Saharan dust aerosol radiative
forcing measured from space, J. Climate, 17, 2558–2571, https://doi.org/10.1175/1520-0442(2004)017<2558:Sdarfm>2.0.Co;2, 2004.
Mahowald, N., Albani, S., Kok, J. F., Engelstaeder, S., Scanza, R., Ward, D.
S., and Flanner, M. G.: The size distribution of desert dust aerosols and
its impact on the Earth system, Aeolian Res., 15, 53–71,
https://doi.org/10.1016/j.aeolia.2013.09.002, 2014.
Meloni, D., di Sarra, A., Di Iorio, T., and Fiocco, G.: Influence of the
vertical profile of Saharan dust on the visible direct radiative forcing, J.
Quant. Spectrosc. Ra. Transf., 93, 397–413,
https://doi.org/10.1016/j.jqsrt.2004.08.035, 2005.
Meloni, D., Junkermann, W., di Sarra, A., Cacciani, M., De Silvestri, L., Di
Iorio, T., Estellés, V., Gómez-Amo, J. L., Pace, G., and Sferlazzo,
D. M.: Altitude-resolved shortwave and longwave radiative effects of desert
dust in the Mediterranean during the GAMARF campaign: Indications of a net
daily cooling in the dust layer, J. Geophys. Res., 120, 3386–3407,
https://doi.org/10.1002/2014JD022312, 2015.
Meng, Z. K., Yang, P., Kattawar, G. W., Bi, L., Liou, K. N., and Laszlo, I.:
Single-scattering properties of tri-axial ellipsoidal mineral dust aerosols:
A database for application to radiative transfer calculations, J. Aerosol
Sci., 41, 501–512, https://doi.org/10.1016/j.jaerosci.2010.02.008, 2010.
Meng, J., Huang, Y., Leung, D. M., Li, L., Adebiyi, A. A., Ryder, C. L., Mahowald, N. M., and Kok, J. F.: Improved parameterization for the size distribution of emitted dust aerosols reduces model underestimation of super coarse dust, Geophys. Res. Lett., 49, e2021GL097287, https://doi.org/10.1029/2021GL097287, 2022.
Mlawer, E. J. and Clough, S. A.: Shortwave and longwave enhancements in the
rapid radiative transfer model, Proc. Seventh Atmos. Radiat. Meas. Sci. Team
Meet., 409–413, 1998.
Mlawer, E. J., Taubman, S. J., Brown, P. D., Iacono, M. J., and Clough, S.
A.: Radiative transfer for inhomogeneous atmospheres: RRTM, a validated
correlated-k model for the longwave, J. Geophys. Res.-Atmos., 102,
16663–16682, https://doi.org/10.1029/97jd00237, 1997.
Myhre, G., Grini, A., Haywood, J. M., Stordal, F., Chatenet, B., Tanre, D.,
Sundet, J. K., and Isaksen, I. S. A.: Modeling the radiative impact of
mineral dust during the Saharan Dust Experiment (SHADE) campaign, J.
Geophys. Res., 108, 8579, https://doi.org/10.1029/2002jd002566, 2003.
Myhre, G., Samset, B. H., Mohr, C. W., Alterskjær, K., Balkanski, Y., Bellouin, N., Chin, M., Haywood, J., Hodnebrog, Ø., Kinne, S., Lin, G., Lund, M. T., Penner, J. E., Schulz, M., Schutgens, N., Skeie, R. B., Stier, P., Takemura, T., and Zhang, K.: Cloudy-sky contributions to the direct aerosol effect, Atmos. Chem. Phys., 20, 8855–8865, https://doi.org/10.5194/acp-20-8855-2020, 2020.
Patadia, F., Yang, E. S., and Christopher, S. A.: Does dust change the clear
sky top of atmosphere shortwave flux over high surface reflectance regions?,
Geophys. Res. Lett., 36, L15825, https://doi.org/10.1029/2009GL039092, 2009.
Pu, B. and Ginoux, P.: How reliable are CMIP5 models in simulating dust optical depth?, Atmos. Chem. Phys., 18, 12491–12510, https://doi.org/10.5194/acp-18-12491-2018, 2018.
Raisanen, P., Haapanala, P., Chung, C. E., Kahnert, M., Makkonen, R.,
Tonttila, J., and Nousiainen, T.: Impact of dust particle non-sphericity on
climate simulations, Q. J. Roy. Meteorol. Soc., 139, 2222–2232,
https://doi.org/10.1002/qj.2084, 2013.
Remer, L. A., Kaufman, Y. J., Tanré, D., Mattoo, S., Chu, D. A.,
Martins, J. V, Li, R. R., Ichoku, C., Levy, R. C., Kleidman, R. G., Eck, T.
F., Vermote, E., and Holben, B. N.: The MODIS aerosol algorithm, products,
and validation, J. Atmos. Sci., 62, 947–973,
https://doi.org/10.1175/JAS3385.1, 2005.
Ryder, C. L., Highwood, E. J., Lai, T. M., Sodemann, H., and Marsham, J. H.:
Impact of atmospheric transport on the evolution of microphysical and
optical properties of Saharan dust, Geophys. Res. Lett., 40, 2433–2438,
https://doi.org/10.1002/grl.50482, 2013a.
Ryder, C. L., Highwood, E. J., Rosenberg, P. D., Trembath, J., Brooke, J. K., Bart, M., Dean, A., Crosier, J., Dorsey, J., Brindley, H., Banks, J., Marsham, J. H., McQuaid, J. B., Sodemann, H., and Washington, R.: Optical properties of Saharan dust aerosol and contribution from the coarse mode as measured during the Fennec 2011 aircraft campaign, Atmos. Chem. Phys., 13, 303–325, https://doi.org/10.5194/acp-13-303-2013, 2013b.
Ryder, C. L., Marenco, F., Brooke, J. K., Estelles, V., Cotton, R., Formenti, P., McQuaid, J. B., Price, H. C., Liu, D., Ausset, P., Rosenberg, P. D., Taylor, J. W., Choularton, T., Bower, K., Coe, H., Gallagher, M., Crosier, J., Lloyd, G., Highwood, E. J., and Murray, B. J.: Coarse-mode mineral dust size distributions, composition and optical properties from AER-D aircraft measurements over the tropical eastern Atlantic, Atmos. Chem. Phys., 18, 17225–17257, https://doi.org/10.5194/acp-18-17225-2018, 2018.
Ryder, C. L., Highwood, E. J., Walser, A., Seibert, P., Philipp, A., and Weinzierl, B.: Coarse and giant particles are ubiquitous in Saharan dust export regions and are radiatively significant over the Sahara, Atmos. Chem. Phys., 19, 15353–15376, https://doi.org/10.5194/acp-19-15353-2019, 2019.
Sakai, T., Nagai, T., Zaizen, Y., and Mano, Y.: Backscattering linear
depolarization ratio measurements of mineral, sea-salt, and ammonium sulfate
particles simulated in a laboratory chamber, Appl. Opt., 49, 4441–4449,
2010.
Satheesh, S. K. and Ramanathan, V.: Large differences in tropical aerosol
forcing at the top of the atmosphere and Earth's surface, Nature, 405,
60–63, https://doi.org/10.1038/35011039, 2000.
Sinyuk, A., Torres, O., and Dubovik, O.: Combined use of satellite and
surface observations to infer the imaginary part of refractive index of
Saharan dust, Geophys. Res. Lett., 30, 1081, https://doi.org/10.1029/2002GL016189,
2003.
Sokolik, I. N., Toon, O. B., and Bergstrom, R. W.: Modeling the radiative
characteristics of airborne mineral aerosols at infrared wavelengths, J.
Geophys. Res., 103, 8813–8826, https://doi.org/10.1029/98jd00049, 1998.
Song, Q., Zhang, Z., Yu, H., Kato, S., Yang, P., Colarco, P., Remer, L. A., and Ryder, C. L.: Net radiative effects of dust in the tropical North Atlantic based on integrated satellite observations and in situ measurements, Atmos. Chem. Phys., 18, 11303–11322, https://doi.org/10.5194/acp-18-11303-2018, 2018.
Song, Q., Zhang, Z., Yu, H., Ginoux, P., and Shen, J.: Global dust optical depth climatology derived from CALIOP and MODIS aerosol retrievals on decadal timescales: regional and interannual variability, Atmos. Chem. Phys., 21, 13369–13395, https://doi.org/10.5194/acp-21-13369-2021, 2021.
Stamnes, K., Tsay, S.-C., Wiscombe, W., and Jayaweera, K.: Numerically
stable algorithm for discrete-ordinate-method radiative transfer in multiple
scattering and emitting layered media, Appl. Opt., 27, 2502,
https://doi.org/10.1364/ao.27.002502, 1988.
Tegen, I. and Lacis, A. A.: Modeling of particle size distribution and its
influence on the radiative properties of mineral dust aerosol, J. Geophys.
Res.-Atmos., 101, 19237–19244, https://doi.org/10.1029/95jd03610, 1996.
Tegen, I., Lacis, A. A., and Fung, I.: The influence on climate forcing of
mineral aerosols from disturbed soils, Nature, 380, 419–422,
https://doi.org/10.1038/380419a0, 1996.
Textor, C., Schulz, M., Guibert, S., Kinne, S., Balkanski, Y., Bauer, S., Berntsen, T., Berglen, T., Boucher, O., Chin, M., Dentener, F., Diehl, T., Easter, R., Feichter, H., Fillmore, D., Ghan, S., Ginoux, P., Gong, S., Grini, A., Hendricks, J., Horowitz, L., Huang, P., Isaksen, I., Iversen, I., Kloster, S., Koch, D., Kirkevåg, A., Kristjansson, J. E., Krol, M., Lauer, A., Lamarque, J. F., Liu, X., Montanaro, V., Myhre, G., Penner, J., Pitari, G., Reddy, S., Seland, Ø., Stier, P., Takemura, T., and Tie, X.: Analysis and quantification of the diversities of aerosol life cycles within AeroCom, Atmos. Chem. Phys., 6, 1777–1813, https://doi.org/10.5194/acp-6-1777-2006, 2006.
Twomey, S.: The influence of pollution on the shortwave albedo of clouds, J.
Atmos. Sci., 34, 1149–1152, 1977.
van de Hulst, H. C.: Light scattering by small particles, Wiley, Hoboken, NJ, 103–113, ISBN 0-486-64228-3,
1957.
Van Der Does, M., Knippertz, P., Zschenderlein, P., Harrison, R. G., and
Stuut, J.-B. W.: The mysterious long-range transport of giant mineral dust
particles, Sci. Adv., 4, 1–9, 2018.
Voss, K. K. and Evan, A. T.: A New Satellite-Based Global Climatology of
Dust Aerosol Optical Depth, J. Appl. Meteorol. Climatol., 59, 83–102,
https://doi.org/10.1175/JAMC-D-19-0194.1, 2020.
VOUK, V.: Projected Area of Convex Bodies, Nature, 162, 330–331,
https://doi.org/10.1038/162330a0, 1948.
Weinzierl, B., Ansmann, A., Prospero, J. M., Althausen, D., Benker, N.,
Chouza, F., Dollner, M., Farrell, D., Fomba, W. K., Freudenthaler, V.,
Gasteiger, J., Gross, S., Haarig, M., Heinold, B., Kandler, K., Kristensen,
T. B., Mayol-Bracero, O. L., Muller, T., Reitebuch, O., Sauer, D., Schafler,
A., Schepanski, K., Spanu, A., Tegen, I., Toledano, C., and Walser, A.: THE
SAHARAN AEROSOL LONG-RANGE TRANSPORT AND AEROSOL-CLOUD-INTERACTION
EXPERIMENT Overview and Selected Highlights, B. Am. Meteorol. Soc., 98,
1427–1451, https://doi.org/10.1175/Bams-D-15-00142.1, 2017.
Winker, D. M., Vaughan, M. A., Omar, A., Hu, Y., Powell, K. A., Liu, Z.,
Hunt, W. H., and Young, S. A.: Overview of the CALIPSO mission and CALIOP
data processing algorithms, J. Atmos. Ocean. Technol., 26, 2310–2323,
https://doi.org/10.1175/2009JTECHA1281.1, 2009.
Wiscombe, W. J.: Improved Mie Scattering Algorithms, Appl. Opt., 19,
1505–1509, https://doi.org/10.1364/Ao.19.001505, 1980.
Wu, M., Liu, X., Yu, H., Wang, H., Shi, Y., Yang, K., Darmenov, A., Wu, C., Wang, Z., Luo, T., Feng, Y., and Ke, Z.: Understanding processes that control dust spatial distributions with global climate models and satellite observations, Atmos. Chem. Phys., 20, 13835–13855, https://doi.org/10.5194/acp-20-13835-2020, 2020.
Yu, H., Kaufman, Y. J., Chin, M., Feingold, G., Remer, L. A., Anderson, T. L., Balkanski, Y., Bellouin, N., Boucher, O., Christopher, S., DeCola, P., Kahn, R., Koch, D., Loeb, N., Reddy, M. S., Schulz, M., Takemura, T., and Zhou, M.: A review of measurement-based assessments of the aerosol direct radiative effect and forcing, Atmos. Chem. Phys., 6, 613–666, https://doi.org/10.5194/acp-6-613-2006, 2006.
Yu, H., Chin, M., Remer, L. A., Kleidman, R. G., Bellouin, N., Bian, H., and
Diehl, T.: Variability of marine aerosol fine-mode fraction and estimates of
anthropogenic aerosol component over cloud-free oceans from the Moderate
Resolution Imaging Spectroradiometer (MODIS), J. Geophys. Res.-Atmos., 114,
D10206, https://doi.org/10.1029/2008JD010648, 2009.
Yu, H., Chin, M., Winker, D. M., Omar, A. H., Liu, Z., Kittaka, C., and
Diehl, T.: Global view of aerosol vertical distributions from CALIPSO lidar
measurements and GOCART simulations: Regional and seasonal variations, J.
Geophys. Res.-Atmos., 115, 1–19, https://doi.org/10.1029/2009JD013364,
2010.
Yu, H., Tan, Q., Chin, M., Remer, L. A., Kahn, R. A., Bian, H., Kim, D.,
Zhang, Z., Yuan, T., Omar, A. H., Winker, D. M., Levy, R. C., Kalashnikova,
O., Crepeau, L., Capelle, V., and Chédin, A.: Estimates of African Dust
Deposition Along the Trans-Atlantic Transit Using the Decadelong Record of
Aerosol Measurements from CALIOP, MODIS, MISR, and IASI, J. Geophys. Res.-Atmos., 124, 7975–7996, https://doi.org/10.1029/2019JD030574, 2019.
Yu, H., Yang, Y., Wang, H., Tan, Q., Chin, M., Levy, R. C., Remer, L. A., Smith, S. J., Yuan, T., and Shi, Y.: Interannual variability and trends of combustion aerosol and dust in major continental outflows revealed by MODIS retrievals and CAM5 simulations during 2003–2017, Atmos. Chem. Phys., 20, 139–161, https://doi.org/10.5194/acp-20-139-2020, 2020.
Zhang, J. L. and Christopher, S. A.: Longwave radiative forcing of Saharan
dust aerosols estimated from MODIS, MISR, and CERES observations on Terra,
Geophys. Res. Lett., 30, 2188, https://doi.org/10.1029/2003gl018479,
2003.
Zhang, Z., Meyer, K., Yu, H., Platnick, S., Colarco, P., Liu, Z., and Oreopoulos, L.: Shortwave direct radiative effects of above-cloud aerosols over global oceans derived from 8 years of CALIOP and MODIS observations, Atmos. Chem. Phys., 16, 2877–2900, https://doi.org/10.5194/acp-16-2877-2016, 2016.
Zhao, C., Liu, X., Leung, L. R., Johnson, B., McFarlane, S. A., Gustafson Jr., W. I., Fast, J. D., and Easter, R.: The spatial distribution of mineral dust and its shortwave radiative forcing over North Africa: modeling sensitivities to dust emissions and aerosol size treatments, Atmos. Chem. Phys., 10, 8821–8838, https://doi.org/10.5194/acp-10-8821-2010, 2010.
Zheng, J., Zhang, Z., Garnier, A., Yu, H., Song, Q., Wang, C., Dubuisson,
P., and Di Biagio, C.: The thermal infrared optical depth of mineral dust
retrieved from integrated CALIOP and IIR observations, Remote Sens.
Environ., 270, 112841, https://doi.org/10.1016/j.rse.2021.112841, 2022.
Zhou, M., Yu, H., Dickinson, R. E., Dubovik, O., and Holben, B. N.: A
normalized description of the direct effect of key aerosol types on solar
radiation as estimated from Aerosol Robotic Network aerosols and Moderate
Resolution Imaging Spectroradiometer albedos, J. Geophys. Res.-Atmos.,
110, 1–10, https://doi.org/10.1029/2005JD005909, 2005.
Short summary
This study developed a dataset that enables us to efficiently calculate dust direct radiative effect (DRE, i.e., cooling or warming our planet) for any given dust size distribution in addition to three sets of dust mineral components and two dust shapes. We demonstrate and validate the method of using this dataset to calculate dust DRE. Moreover, using this dataset we found that dust mineral composition is a more important factor in determining dust DRE than dust size and shape.
This study developed a dataset that enables us to efficiently calculate dust direct radiative...
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