Articles | Volume 21, issue 13
Atmos. Chem. Phys., 21, 9955–9976, 2021
https://doi.org/10.5194/acp-21-9955-2021
Atmos. Chem. Phys., 21, 9955–9976, 2021
https://doi.org/10.5194/acp-21-9955-2021
Research article
02 Jul 2021
Research article | 02 Jul 2021

Secondary aerosol formation from dimethyl sulfide – improved mechanistic understanding based on smog chamber experiments and modelling

Robin Wollesen de Jonge et al.

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Hygroscopicity and CCN potential of DMS derived aerosol particles
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Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-188,https://doi.org/10.5194/acp-2022-188, 2022
Revised manuscript accepted for ACP
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This study presents a detailed analysis of the OH-initiated oxidation of dimethyl sulfide (DMS) based on experiments performed in the Aarhus University Research on Aerosol (AURA) smog chamber and the gas- and particle-phase chemistry kinetic multilayer model (ADCHAM). We capture the formation, growth and chemical composition of aerosols in the chamber setup by an improved multiphase oxidation mechanism and utilize our results to reproduce the important role of DMS in the marine boundary layer.
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