Articles | Volume 21, issue 18
https://doi.org/10.5194/acp-21-14371-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-21-14371-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
28 Sep 2021
Research article |
| 28 Sep 2021
| 28 Sep 2021
The outflow of Asian biomass burning carbonaceous aerosol into the upper troposphere and lower stratosphere in spring: radiative effects seen in a global model
Prashant Chavan
Indian Institute of Tropical Meteorology, Center for climate change,
MoES, India
Department of Atmospheric and Space Sciences, Savitribai Phule Pune University, Pune, India
Indian Institute of Tropical Meteorology, Center for climate change,
MoES, India
Tanusri Chakroborty
Indian Institute of Tropical Meteorology, Center for climate change,
MoES, India
Christopher E. Sioris
Air Quality Research Division, Environment and Climate Change,
Toronto, Canada
Sabine Griessbach
Forschungszentrum Jülich GmbH, Jülich Supercomputing Center,
Jülich, Germany
Rolf Müller
Forschungszentrum Jülich GmbH, IEK7, Jülich, Germany
Related authors
Suvarna Fadnavis, Prashant Chavan, Akash Joshi, Sunil M. Sonbawne, Asutosh Acharya, Panuganti C. S. Devara, Alexandru Rap, Felix Ploeger, and Rolf Müller
Atmos. Chem. Phys., 22, 7179–7191, https://doi.org/10.5194/acp-22-7179-2022, https://doi.org/10.5194/acp-22-7179-2022, 2022
Short summary
Short summary
We show that large amounts of anthropogenic aerosols are transported from South Asia to the northern Indian Ocean. These aerosols are then lifted into the UTLS by the ascending branch of the Hadley circulation. They are further transported to the Southern Hemisphere and downward via westerly ducts over the tropical Atlantic and Pacific. These aerosols increase tropospheric heating, resulting in an increase in water vapor, which is then transported to the UTLS.
Yiran Zhang-Liu, Rolf Müller, Jens-Uwe Grooß, Sabine Robrecht, Bärbel Vogel, Abdul Mannan Zafar, and Ralph Lehmann
Atmos. Chem. Phys., 24, 12557–12574, https://doi.org/10.5194/acp-24-12557-2024, https://doi.org/10.5194/acp-24-12557-2024, 2024
Short summary
Short summary
HCl null cycles in Antarctica are important for maintaining high values of ozone-destroying chlorine in Antarctic spring. These HCl null cycles are not affected by (1) using the most recent recommendations of chemical kinetics (compared to older recommendations), (2) accounting for dehydration in the Antarctic winter vortex, and (3) considering the observed (but unexplained) depletion of HCl in mid-winter in the Antarctic vortex throughout Antarctic winter.
Yasin Elshorbany, Jerald R. Ziemke, Sarah Strode, Hervé Petetin, Kazuyuki Miyazaki, Isabelle De Smedt, Kenneth Pickering, Rodrigo J. Seguel, Helen Worden, Tamara Emmerichs, Domenico Taraborrelli, Maria Cazorla, Suvarna Fadnavis, Rebecca R. Buchholz, Benjamin Gaubert, Néstor Y. Rojas, Thiago Nogueira, Thérèse Salameh, and Min Huang
Atmos. Chem. Phys., 24, 12225–12257, https://doi.org/10.5194/acp-24-12225-2024, https://doi.org/10.5194/acp-24-12225-2024, 2024
Short summary
Short summary
We investigated tropospheric ozone spatial variability and trends from 2005 to 2019 and related those to ozone precursors on global and regional scales. We also investigate the spatiotemporal characteristics of the ozone formation regime in relation to ozone chemical sources and sinks. Our analysis is based on remote sensing products of the tropospheric column of ozone and its precursors, nitrogen dioxide, formaldehyde, and total column CO, as well as ozonesonde data and model simulations.
Ling Zou, Reinhold Spang, Sabine Griessbach, Lars Hoffmann, Farahnaz Khosrawi, Rolf Müller, and Ines Tritscher
Atmos. Chem. Phys., 24, 11759–11774, https://doi.org/10.5194/acp-24-11759-2024, https://doi.org/10.5194/acp-24-11759-2024, 2024
Short summary
Short summary
This study provided estimates of the occurrence of ice polar stratospheric clouds (PSCs) observed by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) and their connection with temperatures above the frost point (Tice) using a Lagrangian model derived from ERA5. We found that ice PSCs above Tice with temperature fluctuations along the backward trajectory are 33 % in the Arctic and 9 % in the Antarctic. This quantitative assessment enhances our understanding of ice PSCs.
Suvarna Fadnavis, Yasin Elshorbany, Jerald Ziemke, Brice Barret, Alexandru Rap, P. R. Satheesh Chandran, Richard Pope, Vijay Sagar, Domenico Taraborrelli, Eric Le Flochmoen, Juan Cuesta, Catherine Wespes, Folkert Boersma, Isolde Glissenaar, Isabelle De Smedt, Michel Van Roozendael, Hervé Petetin, and Isidora Anglou
EGUsphere, https://doi.org/10.5194/egusphere-2024-3050, https://doi.org/10.5194/egusphere-2024-3050, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Satellites and model simulations show enhancement in tropospheric ozone, which is highly impacted by human-produced Nitrous oxides compared to volatile organic compounds. The increased amount of ozone enhances ozone radiative forcing. The ozone enhancement and associated radiative forcing are highest over South and East Asia. The emissions of Nitrous oxides show a higher influence in shifting ozone photochemical regimes than volatile organic compounds.
Mingzhao Liu, Lars Hoffmann, Jens-Uwe Grooß, Zhongyin Cai, Sabine Grießbach, and Yi Heng
EGUsphere, https://doi.org/10.5194/egusphere-2024-2596, https://doi.org/10.5194/egusphere-2024-2596, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
We studied the transport and chemical decomposition of volcanic SO2, focusing on the 2019 Raikoke event. By comparing two different chemistry modeling schemes, we found that including complex chemical reactions leads to a more accurate prediction of how long SO2 stays in the atmosphere. This research helps improve our understanding of volcanic pollution and its impact on air quality and climate, providing better tools for scientists to track and predict the movement of these pollutants.
Astrid Kerkweg, Timo Kirfel, Doung H. Do, Sabine Griessbach, Patrick Jöckel, and Domenico Taraborrelli
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-117, https://doi.org/10.5194/gmd-2024-117, 2024
Revised manuscript under review for GMD
Short summary
Short summary
This article introduces the MESSy DWARF. Usually, the Modular Earth Submodel System (MESSy) is linked to full dynamical models to build chemistry climate models. However, due to the modular concept of MESSy, and the newly developed DWARF component, it is now possible to create simplified models containing just one or some process descriptions. This renders very useful for technical optimisation (e.g., GPU porting) and can be used to create less complex models, e.g., a chemical box model.
Jayanarayanan Kuttippurath, Gopalakrishna Pillai Gopikrishnan, Rolf Müller, Sophie Godin-Beekmann, and Jerome Brioude
Atmos. Chem. Phys., 24, 6743–6756, https://doi.org/10.5194/acp-24-6743-2024, https://doi.org/10.5194/acp-24-6743-2024, 2024
Short summary
Short summary
The current understanding and observational evidence do not provide any support for the possibility of an ozone hole occurring outside Antarctica today with respect to the present-day stratospheric halogen levels.
Jan Clemens, Lars Hoffmann, Bärbel Vogel, Sabine Grießbach, and Nicole Thomas
Geosci. Model Dev., 17, 4467–4493, https://doi.org/10.5194/gmd-17-4467-2024, https://doi.org/10.5194/gmd-17-4467-2024, 2024
Short summary
Short summary
Lagrangian transport models simulate the transport of air masses in the atmosphere. For example, one model (CLaMS) is well suited to calculating transport as it uses a special coordinate system and special vertical wind. However, it only runs inefficiently on modern supercomputers. Hence, we have implemented the benefits of CLaMS into a new model (MPTRAC), which is already highly efficient on modern supercomputers. Finally, in extensive tests, we showed that CLaMS and MPTRAC agree very well.
Felix Ploeger, Thomas Birner, Edward Charlesworth, Paul Konopka, and Rolf Müller
Atmos. Chem. Phys., 24, 2033–2043, https://doi.org/10.5194/acp-24-2033-2024, https://doi.org/10.5194/acp-24-2033-2024, 2024
Short summary
Short summary
We present a novel mechanism of how regional anomalies in water vapour concentrations in the upper troposphere and lower stratosphere impact regional atmospheric circulation systems. These impacts include a displaced upper-level Asian monsoon circulation and strengthened prevailing westerlies in the Pacific region. Current climate models have biases in simulating these regional water vapour anomalies and circulation impacts, but the biases can be avoided by improving the model transport.
Reinhold Spang, Rolf Müller, and Alexandru Rap
Atmos. Chem. Phys., 24, 1213–1230, https://doi.org/10.5194/acp-24-1213-2024, https://doi.org/10.5194/acp-24-1213-2024, 2024
Short summary
Short summary
Cirrus clouds play an important role in the radiation budget of the Earth. Despite recent progress in their observation, the radiative impact of ultra-thin cirrus clouds (UTC) in the tropopause region and in the lowermost stratosphere remains poorly constrained. Sensitivity model simulations with different ice parameters provide an uncertainty range for the radiative effect of UTCs. There is a need for better observed UTCs to enable the simulation of their potentially large effect on climate.
Jan Clemens, Bärbel Vogel, Lars Hoffmann, Sabine Griessbach, Nicole Thomas, Suvarna Fadnavis, Rolf Müller, Thomas Peter, and Felix Ploeger
Atmos. Chem. Phys., 24, 763–787, https://doi.org/10.5194/acp-24-763-2024, https://doi.org/10.5194/acp-24-763-2024, 2024
Short summary
Short summary
The source regions of the Asian tropopause aerosol layer (ATAL) are debated. We use balloon-borne measurements of the layer above Nainital (India) in August 2016 and atmospheric transport models to find ATAL source regions. Most air originated from the Tibetan plateau. However, the measured ATAL was stronger when more air originated from the Indo-Gangetic Plain and weaker when more air originated from the Pacific. Hence, the results indicate important anthropogenic contributions to the ATAL.
Bärbel Vogel, C. Michael Volk, Johannes Wintel, Valentin Lauther, Jan Clemens, Jens-Uwe Grooß, Gebhard Günther, Lars Hoffmann, Johannes C. Laube, Rolf Müller, Felix Ploeger, and Fred Stroh
Atmos. Chem. Phys., 24, 317–343, https://doi.org/10.5194/acp-24-317-2024, https://doi.org/10.5194/acp-24-317-2024, 2024
Short summary
Short summary
Over the Indian subcontinent, polluted air is rapidly uplifted to higher altitudes during the Asian monsoon season. We present an assessment of vertical transport in this region using different wind data provided by the European Centre for Medium-Range Weather Forecasts (ECMWF), as well as high-resolution aircraft measurements. In general, our findings confirm that the newest ECMWF reanalysis product, ERA5, yields a better representation of transport compared to the predecessor, ERA-Interim.
Rolf Müller, Ulrich Pöschl, Thomas Koop, Thomas Peter, and Ken Carslaw
Atmos. Chem. Phys., 23, 15445–15453, https://doi.org/10.5194/acp-23-15445-2023, https://doi.org/10.5194/acp-23-15445-2023, 2023
Short summary
Short summary
Paul J. Crutzen was a pioneer in atmospheric sciences and a kind-hearted, humorous person with empathy for the private lives of his colleagues and students. He made fundamental scientific contributions to a wide range of scientific topics in all parts of the atmosphere. Paul was among the founders of the journal Atmospheric Chemistry and Physics. His work will continue to be a guide for generations of scientists and environmental policymakers to come.
Suvarna Fadnavis, Bernd Heinold, T. P. Sabin, Anne Kubin, Katty Huang, Alexandru Rap, and Rolf Müller
Atmos. Chem. Phys., 23, 10439–10449, https://doi.org/10.5194/acp-23-10439-2023, https://doi.org/10.5194/acp-23-10439-2023, 2023
Short summary
Short summary
The influence of the COVID-19 lockdown on the Himalayas caused increases in snow cover and a decrease in runoff, ultimately leading to an enhanced snow water equivalent. Our findings highlight that, out of the two processes causing a retreat of Himalayan glaciers – (1) slow response to global climate change and (2) fast response to local air pollution – a policy action on the latter is more likely to be within the reach of possible policy action to help billions of people in southern Asia.
Mingzhao Liu, Lars Hoffmann, Sabine Griessbach, Zhongyin Cai, Yi Heng, and Xue Wu
Geosci. Model Dev., 16, 5197–5217, https://doi.org/10.5194/gmd-16-5197-2023, https://doi.org/10.5194/gmd-16-5197-2023, 2023
Short summary
Short summary
We introduce new and revised chemistry and physics modules in the Massive-Parallel Trajectory Calculations (MPTRAC) Lagrangian transport model aiming to improve the representation of volcanic SO2 transport and depletion. We test these modules in a case study of the Ambae eruption in July 2018 in which the SO2 plume underwent wet removal and convection. The lifetime of SO2 shows highly variable and complex dependencies on the atmospheric conditions at different release heights.
Liubov Poshyvailo-Strube, Rolf Müller, Stephan Fueglistaler, Michaela I. Hegglin, Johannes C. Laube, C. Michael Volk, and Felix Ploeger
Atmos. Chem. Phys., 22, 9895–9914, https://doi.org/10.5194/acp-22-9895-2022, https://doi.org/10.5194/acp-22-9895-2022, 2022
Short summary
Short summary
Brewer–Dobson circulation (BDC) controls the composition of the stratosphere, which in turn affects radiation and climate. As the BDC cannot be measured directly, it is necessary to infer its strength and trends indirectly. In this study, we test in the
model worlddifferent methods for estimating the mean age of air trends based on a combination of stratospheric water vapour and methane data. We also provide simple practical advice of a more reliable estimation of the mean age of air trends.
William G. Read, Gabriele Stiller, Stefan Lossow, Michael Kiefer, Farahnaz Khosrawi, Dale Hurst, Holger Vömel, Karen Rosenlof, Bianca M. Dinelli, Piera Raspollini, Gerald E. Nedoluha, John C. Gille, Yasuko Kasai, Patrick Eriksson, Christopher E. Sioris, Kaley A. Walker, Katja Weigel, John P. Burrows, and Alexei Rozanov
Atmos. Meas. Tech., 15, 3377–3400, https://doi.org/10.5194/amt-15-3377-2022, https://doi.org/10.5194/amt-15-3377-2022, 2022
Short summary
Short summary
This paper attempts to provide an assessment of the accuracy of 21 satellite-based instruments that remotely measure atmospheric humidity in the upper troposphere of the Earth's atmosphere. The instruments made their measurements from 1984 to the present time; however, most of these instruments began operations after 2000, and only a few are still operational. The objective of this study is to quantify the accuracy of each satellite humidity data set.
Suvarna Fadnavis, Prashant Chavan, Akash Joshi, Sunil M. Sonbawne, Asutosh Acharya, Panuganti C. S. Devara, Alexandru Rap, Felix Ploeger, and Rolf Müller
Atmos. Chem. Phys., 22, 7179–7191, https://doi.org/10.5194/acp-22-7179-2022, https://doi.org/10.5194/acp-22-7179-2022, 2022
Short summary
Short summary
We show that large amounts of anthropogenic aerosols are transported from South Asia to the northern Indian Ocean. These aerosols are then lifted into the UTLS by the ascending branch of the Hadley circulation. They are further transported to the Southern Hemisphere and downward via westerly ducts over the tropical Atlantic and Pacific. These aerosols increase tropospheric heating, resulting in an increase in water vapor, which is then transported to the UTLS.
Zhongyin Cai, Sabine Griessbach, and Lars Hoffmann
Atmos. Chem. Phys., 22, 6787–6809, https://doi.org/10.5194/acp-22-6787-2022, https://doi.org/10.5194/acp-22-6787-2022, 2022
Short summary
Short summary
Using AIRS and TROPOMI sulfur dioxide retrievals and the Lagrangian transport model MPTRAC, we present an improved reconstruction of injection parameters of the 2019 Raikoke eruption. Reconstructions agree well between using AIRS nighttime and TROPOMI daytime retrievals, showing the potential of our approach to create a long-term volcanic sulfur dioxide inventory from nearly 20 years of AIRS retrievals.
Ling Zou, Sabine Griessbach, Lars Hoffmann, and Reinhold Spang
Atmos. Chem. Phys., 22, 6677–6702, https://doi.org/10.5194/acp-22-6677-2022, https://doi.org/10.5194/acp-22-6677-2022, 2022
Short summary
Short summary
Ice clouds in the stratosphere (SICs) greatly affect the water vapor balance and radiation budget in the upper troposphere and lower stratosphere (UTLS). We quantified the global SICs and analyzed their relationships with tropopause temperature, double tropopauses, UTLS clouds, gravity waves, and stratospheric aerosols. The correlations between SICs and all abovementioned processes indicate that the occurrence of and variability in SICs are spatiotemporally dependent on different processes.
Lars Hoffmann, Paul F. Baumeister, Zhongyin Cai, Jan Clemens, Sabine Griessbach, Gebhard Günther, Yi Heng, Mingzhao Liu, Kaveh Haghighi Mood, Olaf Stein, Nicole Thomas, Bärbel Vogel, Xue Wu, and Ling Zou
Geosci. Model Dev., 15, 2731–2762, https://doi.org/10.5194/gmd-15-2731-2022, https://doi.org/10.5194/gmd-15-2731-2022, 2022
Short summary
Short summary
We describe the new version (2.2) of the Lagrangian transport model MPTRAC, which has been ported for application on GPUs. The model was verified by comparing kinematic trajectories and synthetic tracer simulations for the free troposphere and stratosphere from GPUs and CPUs. Benchmarking showed a speed-up of a factor of 16 of GPU-enabled simulations compared to CPU-only runs, indicating the great potential of applying GPUs for Lagrangian transport simulations on upcoming HPC systems.
Valentin Lauther, Bärbel Vogel, Johannes Wintel, Andrea Rau, Peter Hoor, Vera Bense, Rolf Müller, and C. Michael Volk
Atmos. Chem. Phys., 22, 2049–2077, https://doi.org/10.5194/acp-22-2049-2022, https://doi.org/10.5194/acp-22-2049-2022, 2022
Short summary
Short summary
We show airborne in situ measurements of the very short-lived ozone-depleting substances CH2Cl2 and CHCl3, revealing particularly high concentrations of both species in the lower stratosphere. Back-trajectory calculations and 3D model simulations show that the air masses with high concentrations originated in the Asian boundary layer and were transported via the Asian summer monsoon. We also identify a fast transport pathway into the stratosphere via the North American monsoon and by hurricanes.
Dina Khordakova, Christian Rolf, Jens-Uwe Grooß, Rolf Müller, Paul Konopka, Andreas Wieser, Martina Krämer, and Martin Riese
Atmos. Chem. Phys., 22, 1059–1079, https://doi.org/10.5194/acp-22-1059-2022, https://doi.org/10.5194/acp-22-1059-2022, 2022
Short summary
Short summary
Extreme storms transport humidity from the troposphere to the stratosphere. Here it has a strong impact on the climate. With ongoing global warming, we expect more storms and, hence, an enhancement of this effect. A case study was performed in order to measure the impact of the direct injection of water vapor into the lower stratosphere. The measurements displayed a significant transport of water vapor into the lower stratosphere, and this was supported by satellite and reanalysis data.
Jayanarayanan Kuttippurath, Wuhu Feng, Rolf Müller, Pankaj Kumar, Sarath Raj, Gopalakrishna Pillai Gopikrishnan, and Raina Roy
Atmos. Chem. Phys., 21, 14019–14037, https://doi.org/10.5194/acp-21-14019-2021, https://doi.org/10.5194/acp-21-14019-2021, 2021
Short summary
Short summary
The Arctic winter/spring 2020 was one of the coldest with a strong and long-lasting vortex, high chlorine activation, severe denitrification, and unprecedented ozone loss. The loss was even equal to the levels of some of the warm Antarctic winters. Total column ozone values below 220 DU for several weeks and ozone loss saturation were observed during the period. These results show an unusual meteorology and warrant dedicated studies on the impact of climate change on ozone loss.
Paul A. Makar, Ayodeji Akingunola, Jack Chen, Balbir Pabla, Wanmin Gong, Craig Stroud, Christopher Sioris, Kerry Anderson, Philip Cheung, Junhua Zhang, and Jason Milbrandt
Atmos. Chem. Phys., 21, 10557–10587, https://doi.org/10.5194/acp-21-10557-2021, https://doi.org/10.5194/acp-21-10557-2021, 2021
Short summary
Short summary
We have examined the effects of airborne particles on absorption and scattering of incoming sunlight by the particles themselves via cloud formation. We used an advanced, combined high-resolution weather forecast and chemical transport computer model, for western North America, and simulations with and without the connections between particles and weather enabled. Feedbacks improved weather and air pollution forecasts and changed cloud behaviour and forest-fire pollutant amount and height.
Ling Zou, Lars Hoffmann, Sabine Griessbach, Reinhold Spang, and Lunche Wang
Atmos. Chem. Phys., 21, 10457–10475, https://doi.org/10.5194/acp-21-10457-2021, https://doi.org/10.5194/acp-21-10457-2021, 2021
Short summary
Short summary
Ice clouds in the lowermost stratosphere (SICs) have important impacts on the radiation budget and climate change. We quantified the occurrence of SICs over North America and analysed its relations with convective systems and gravity waves to investigate potential formation mechanisms of SICs. Deep convection is proved to be the primary factor linked to the occurrence of SICs over North America.
Michaela I. Hegglin, Susann Tegtmeier, John Anderson, Adam E. Bourassa, Samuel Brohede, Doug Degenstein, Lucien Froidevaux, Bernd Funke, John Gille, Yasuko Kasai, Erkki T. Kyrölä, Jerry Lumpe, Donal Murtagh, Jessica L. Neu, Kristell Pérot, Ellis E. Remsberg, Alexei Rozanov, Matthew Toohey, Joachim Urban, Thomas von Clarmann, Kaley A. Walker, Hsiang-Jui Wang, Carlo Arosio, Robert Damadeo, Ryan A. Fuller, Gretchen Lingenfelser, Christopher McLinden, Diane Pendlebury, Chris Roth, Niall J. Ryan, Christopher Sioris, Lesley Smith, and Katja Weigel
Earth Syst. Sci. Data, 13, 1855–1903, https://doi.org/10.5194/essd-13-1855-2021, https://doi.org/10.5194/essd-13-1855-2021, 2021
Short summary
Short summary
An overview of the SPARC Data Initiative is presented, to date the most comprehensive assessment of stratospheric composition measurements spanning 1979–2018. Measurements of 26 chemical constituents obtained from an international suite of space-based limb sounders were compiled into vertically resolved, zonal monthly mean time series. The quality and consistency of these gridded datasets are then evaluated using a climatological validation approach and a range of diagnostics.
Irene Bartolome Garcia, Reinhold Spang, Jörn Ungermann, Sabine Griessbach, Martina Krämer, Michael Höpfner, and Martin Riese
Atmos. Meas. Tech., 14, 3153–3168, https://doi.org/10.5194/amt-14-3153-2021, https://doi.org/10.5194/amt-14-3153-2021, 2021
Short summary
Short summary
Cirrus clouds contribute to the general radiation budget of the Earth. Measuring optically thin clouds is challenging but the IR limb sounder GLORIA possesses the necessary technical characteristics to make it possible. This study analyses data from the WISE campaign obtained with GLORIA. We developed a cloud detection method and derived characteristics of the observed cirrus-like cloud top, cloud bottom or position with respect to the tropopause.
Christoph Kalicinsky, Sabine Griessbach, and Reinhold Spang
Atmos. Meas. Tech., 14, 1893–1915, https://doi.org/10.5194/amt-14-1893-2021, https://doi.org/10.5194/amt-14-1893-2021, 2021
Short summary
Short summary
For an airborne viewing geometry, radiative transfer simulations of infrared limb emission spectra in the presence of polar stratospheric clouds – nitric acid trihydrate (NAT), supercooled ternary solution, ice, and mixtures – were used to develop a size-sensitive NAT detection algorithm. Characteristic size-dependent spectral features in the 810–820 cm−1 region were exploited to subgroup the NAT into three size regimes: small NAT (≤ 1.0 μm), medium NAT (1.5–4.0 μm), and large NAT (≥ 3.5 μm).
Sabine Robrecht, Bärbel Vogel, Simone Tilmes, and Rolf Müller
Atmos. Chem. Phys., 21, 2427–2455, https://doi.org/10.5194/acp-21-2427-2021, https://doi.org/10.5194/acp-21-2427-2021, 2021
Short summary
Short summary
Column ozone protects life on Earth from radiation damage. Stratospheric chlorine compounds cause immense ozone loss in polar winter. Whether similar loss processes can occur in the lower stratosphere above North America today or in future is a matter of debate. We show that these ozone loss processes are very unlikely today or in future independently of whether sulfate geoengineering is applied and that less than 0.1 % of column ozone would be destroyed by this process in any future scenario.
Teresa Jorge, Simone Brunamonti, Yann Poltera, Frank G. Wienhold, Bei P. Luo, Peter Oelsner, Sreeharsha Hanumanthu, Bhupendra B. Singh, Susanne Körner, Ruud Dirksen, Manish Naja, Suvarna Fadnavis, and Thomas Peter
Atmos. Meas. Tech., 14, 239–268, https://doi.org/10.5194/amt-14-239-2021, https://doi.org/10.5194/amt-14-239-2021, 2021
Short summary
Short summary
Balloon-borne frost point hygrometers are crucial for the monitoring of water vapour in the upper troposphere and lower stratosphere. We found that when traversing a mixed-phase cloud with big supercooled droplets, the intake tube of the instrument collects on its inner surface a high percentage of these droplets. The newly formed ice layer will sublimate at higher levels and contaminate the measurement. The balloon is also a source of contamination, but only at higher levels during the ascent.
Jörn Ungermann, Irene Bartolome, Sabine Griessbach, Reinhold Spang, Christian Rolf, Martina Krämer, Michael Höpfner, and Martin Riese
Atmos. Meas. Tech., 13, 7025–7045, https://doi.org/10.5194/amt-13-7025-2020, https://doi.org/10.5194/amt-13-7025-2020, 2020
Short summary
Short summary
This study examines the potential of new IR limb imager instruments and tomographic methods for cloud detection purposes. Simple color-ratio-based methods are examined and compared against more involved nonlinear convex optimization. In a second part, 3-D measurements of the airborne limb sounder GLORIA taken during the Wave-driven ISentropic Exchange campaign are used to exemplarily derive the location and extent of small-scale cirrus clouds with high spatial accuracy.
Sreeharsha Hanumanthu, Bärbel Vogel, Rolf Müller, Simone Brunamonti, Suvarna Fadnavis, Dan Li, Peter Ölsner, Manish Naja, Bhupendra Bahadur Singh, Kunchala Ravi Kumar, Sunil Sonbawne, Hannu Jauhiainen, Holger Vömel, Beiping Luo, Teresa Jorge, Frank G. Wienhold, Ruud Dirkson, and Thomas Peter
Atmos. Chem. Phys., 20, 14273–14302, https://doi.org/10.5194/acp-20-14273-2020, https://doi.org/10.5194/acp-20-14273-2020, 2020
Short summary
Short summary
During boreal summer, anthropogenic sources yield the Asian Tropopause Aerosol Layer (ATAL), found in Asia between about 13 and 18 km altitude. Balloon-borne measurements of the ATAL conducted in northern India in 2016 show the strong variability of the ATAL. To explain its observed variability, model simulations are performed to deduce the origin of air masses on the Earth's surface, which is important to develop recommendations for regulations of anthropogenic surface emissions of the ATAL.
Joram J. D. Hooghiem, Maria Elena Popa, Thomas Röckmann, Jens-Uwe Grooß, Ines Tritscher, Rolf Müller, Rigel Kivi, and Huilin Chen
Atmos. Chem. Phys., 20, 13985–14003, https://doi.org/10.5194/acp-20-13985-2020, https://doi.org/10.5194/acp-20-13985-2020, 2020
Short summary
Short summary
Wildfires release a large quantity of pollutants that can reach the stratosphere through pyro-convection events. In September 2017, a stratospheric plume was accidentally sampled during balloon soundings in northern Finland. The source of the plume was identified to be wildfire smoke based on in situ measurements of carbon monoxide (CO) and stable isotope analysis of CO. Furthermore, the age of the plume was estimated using backwards transport modelling to be ~24 d, with its origin in Canada.
Ling Zou, Sabine Griessbach, Lars Hoffmann, Bing Gong, and Lunche Wang
Atmos. Chem. Phys., 20, 9939–9959, https://doi.org/10.5194/acp-20-9939-2020, https://doi.org/10.5194/acp-20-9939-2020, 2020
Short summary
Short summary
Cirrus clouds appearing in the upper troposphere and lower stratosphere have important impacts on the radiation budget and climate change. We revisited global stratospheric cirrus clouds with CALIPSO and for the first time with MIPAS satellite observations. Stratospheric cirrus clouds related to deep convection are frequently detected in the tropics. At middle latitudes, MIPAS detects more than twice as many stratospheric cirrus clouds due to higher detection sensitivity.
Rocco Sedona, Lars Hoffmann, Reinhold Spang, Gabriele Cavallaro, Sabine Griessbach, Michael Höpfner, Matthias Book, and Morris Riedel
Atmos. Meas. Tech., 13, 3661–3682, https://doi.org/10.5194/amt-13-3661-2020, https://doi.org/10.5194/amt-13-3661-2020, 2020
Short summary
Short summary
Polar stratospheric clouds (PSCs) play a key role in polar ozone depletion in the stratosphere. In this paper, we explore the potential of applying machine learning (ML) methods to classify PSC observations of infrared spectra to classify PSC types. ML methods have proved to reach results in line with those obtained using well-established approaches. Among the considered ML methods, random forest (RF) seems to be the most promising one, being able to produce explainable classification results.
Dan Li, Bärbel Vogel, Rolf Müller, Jianchun Bian, Gebhard Günther, Felix Ploeger, Qian Li, Jinqiang Zhang, Zhixuan Bai, Holger Vömel, and Martin Riese
Atmos. Chem. Phys., 20, 4133–4152, https://doi.org/10.5194/acp-20-4133-2020, https://doi.org/10.5194/acp-20-4133-2020, 2020
Short summary
Short summary
Low ozone and low water vapour signatures in the UTLS were investigated using balloon-borne measurements and trajectory calculations. The results show that deep convection in tropical cyclones over the western Pacific transports boundary air parcels with low ozone into the tropopause region. Subsequently, these air parcels are dehydrated when passing the lowest temperature region (< 190 K) during quasi-horizontal advection.
Debora Griffin, Christopher Sioris, Jack Chen, Nolan Dickson, Andrew Kovachik, Martin de Graaf, Swadhin Nanda, Pepijn Veefkind, Enrico Dammers, Chris A. McLinden, Paul Makar, and Ayodeji Akingunola
Atmos. Meas. Tech., 13, 1427–1445, https://doi.org/10.5194/amt-13-1427-2020, https://doi.org/10.5194/amt-13-1427-2020, 2020
Short summary
Short summary
This study looks into validating the aerosol layer height product from the recently launched TROPOspheric Monitoring Instrument (TROPOMI) for forest fire plume through comparisons with two other satellite products, and interpreting differences due to the individual measurement techniques. These satellite observations are compared to predicted plume heights from Environment and Climate Change's air quality forecast model.
Sabine Griessbach, Lars Hoffmann, Reinhold Spang, Peggy Achtert, Marc von Hobe, Nina Mateshvili, Rolf Müller, Martin Riese, Christian Rolf, Patric Seifert, and Jean-Paul Vernier
Atmos. Meas. Tech., 13, 1243–1271, https://doi.org/10.5194/amt-13-1243-2020, https://doi.org/10.5194/amt-13-1243-2020, 2020
Short summary
Short summary
In this paper we study the cloud top height derived from MIPAS measurements. Previous studies showed contradictory results with respect to MIPAS, both underestimating and overestimating cloud top height. We used simulations and found that overestimation and/or underestimation depend on cloud extinction. To support our findings we compared MIPAS cloud top heights of volcanic sulfate aerosol with measurements from CALIOP, ground-based lidar, and ground-based twilight measurements.
Mark W. Shephard, Enrico Dammers, Karen E. Cady-Pereira, Shailesh K. Kharol, Jesse Thompson, Yonatan Gainariu-Matz, Junhua Zhang, Chris A. McLinden, Andrew Kovachik, Michael Moran, Shabtai Bittman, Christopher E. Sioris, Debora Griffin, Matthew J. Alvarado, Chantelle Lonsdale, Verica Savic-Jovcic, and Qiong Zheng
Atmos. Chem. Phys., 20, 2277–2302, https://doi.org/10.5194/acp-20-2277-2020, https://doi.org/10.5194/acp-20-2277-2020, 2020
Short summary
Short summary
Presented is a description and survey demonstrating the capabilities of the CrIS ammonia product for monitoring, air quality forecast model evaluation, dry deposition estimates, and emission estimates of an agricultural hotspot.
Xiaolu Yan, Paul Konopka, Felix Ploeger, Aurélien Podglajen, Jonathon S. Wright, Rolf Müller, and Martin Riese
Atmos. Chem. Phys., 19, 15629–15649, https://doi.org/10.5194/acp-19-15629-2019, https://doi.org/10.5194/acp-19-15629-2019, 2019
Short summary
Short summary
The Asian and North American summer monsoons (ASM and NASM) have considerable influence on stratospheric chemistry and physics. More air mass is transported from the monsoon regions to the tropical stratosphere when the tracers are released clearly below the tropopause than when they are released close to the tropopause. Results for different altitudes of air origin reveal two transport pathways (monsoon and tropical) from the upper troposphere over the monsoon regions to the tropical pipe.
Suvarna Fadnavis, Rolf Müller, Gayatry Kalita, Matthew Rowlinson, Alexandru Rap, Jui-Lin Frank Li, Blaž Gasparini, and Anton Laakso
Atmos. Chem. Phys., 19, 9989–10008, https://doi.org/10.5194/acp-19-9989-2019, https://doi.org/10.5194/acp-19-9989-2019, 2019
Short summary
Short summary
This paper highlights the impact of Asian anthropogenic emission changes in SO2 on sulfate loading in the Asian upper troposphere–lower stratosphere from a global chemistry–climate model and satellite remote sensing. Estimated seasonal mean direct radiative forcing at the top of the atmosphere induced by the increase in Indian SO2 is −0.2–−1.5 W m2 over India. Chinese SO2 emission reduction leads to a positive radiative forcing of ~0.6–6 W m2 over China. It will likely decrease Indian rainfall.
Dan Weaver, Kimberly Strong, Kaley A. Walker, Chris Sioris, Matthias Schneider, C. Thomas McElroy, Holger Vömel, Michael Sommer, Katja Weigel, Alexei Rozanov, John P. Burrows, William G. Read, Evan Fishbein, and Gabriele Stiller
Atmos. Meas. Tech., 12, 4039–4063, https://doi.org/10.5194/amt-12-4039-2019, https://doi.org/10.5194/amt-12-4039-2019, 2019
Short summary
Short summary
This work assesses water vapour profiles acquired by Atmospheric Chemistry Experiment (ACE) satellite instruments in the upper troposphere and lower stratosphere (UTLS) using comparisons to radiosondes and ground-based Fourier transform infrared spectrometer measurements acquired at a Canadian high Arctic measurement site in Eureka, Nunavut. Additional comparisons are made between these Eureka measurements and other water vapour satellite datasets for context, including AIRS, MLS, and others.
Stefan Lossow, Farahnaz Khosrawi, Michael Kiefer, Kaley A. Walker, Jean-Loup Bertaux, Laurent Blanot, James M. Russell, Ellis E. Remsberg, John C. Gille, Takafumi Sugita, Christopher E. Sioris, Bianca M. Dinelli, Enzo Papandrea, Piera Raspollini, Maya García-Comas, Gabriele P. Stiller, Thomas von Clarmann, Anu Dudhia, William G. Read, Gerald E. Nedoluha, Robert P. Damadeo, Joseph M. Zawodny, Katja Weigel, Alexei Rozanov, Faiza Azam, Klaus Bramstedt, Stefan Noël, John P. Burrows, Hideo Sagawa, Yasuko Kasai, Joachim Urban, Patrick Eriksson, Donal P. Murtagh, Mark E. Hervig, Charlotta Högberg, Dale F. Hurst, and Karen H. Rosenlof
Atmos. Meas. Tech., 12, 2693–2732, https://doi.org/10.5194/amt-12-2693-2019, https://doi.org/10.5194/amt-12-2693-2019, 2019
Bärbel Vogel, Rolf Müller, Gebhard Günther, Reinhold Spang, Sreeharsha Hanumanthu, Dan Li, Martin Riese, and Gabriele P. Stiller
Atmos. Chem. Phys., 19, 6007–6034, https://doi.org/10.5194/acp-19-6007-2019, https://doi.org/10.5194/acp-19-6007-2019, 2019
Short summary
Short summary
We identified the transport pathways of air masses from the region of the Asian monsoon (e.g. pollution and greenhouse gases caused by increasing population and growing industries in Asia) into the lower stratosphere. Even small changes of the chemical composition of the lower stratosphere have an impact on surface climate (e.g. surface temperatures). Therefore, it is important to identify transport pathways to the stratosphere to allow potential environmental risks to be assessed.
Sabine Robrecht, Bärbel Vogel, Jens-Uwe Grooß, Karen Rosenlof, Troy Thornberry, Andrew Rollins, Martina Krämer, Lance Christensen, and Rolf Müller
Atmos. Chem. Phys., 19, 5805–5833, https://doi.org/10.5194/acp-19-5805-2019, https://doi.org/10.5194/acp-19-5805-2019, 2019
Short summary
Short summary
The potential destruction of stratospheric ozone in the mid-latitudes has been discussed recently. We analysed this ozone loss mechanism and its sensitivities. In a certain temperature range, we found a threshold in water vapour, which has to be exceeded for ozone loss to occur. We show the dependence of this water vapour threshold on temperature, sulfate content and air composition. This study provides a basis to estimate the impact of potential sulphate geoengineering on stratospheric ozone.
Lars Hoffmann, Gebhard Günther, Dan Li, Olaf Stein, Xue Wu, Sabine Griessbach, Yi Heng, Paul Konopka, Rolf Müller, Bärbel Vogel, and Jonathon S. Wright
Atmos. Chem. Phys., 19, 3097–3124, https://doi.org/10.5194/acp-19-3097-2019, https://doi.org/10.5194/acp-19-3097-2019, 2019
Short summary
Short summary
ECMWF's new ERA5 reanalysis provides higher spatiotemporal resolution, yielding an improved representation of meso- and synoptic-scale features of the atmosphere. We assessed the impact of this challenging new data set on Lagrangian trajectory calculations for the free troposphere and stratosphere. Key findings are considerable transport deviations between the ERA5 and ERA-Interim simulations as well as significantly improved conservation of potential temperature in the stratosphere for ERA5.
Ines Tritscher, Jens-Uwe Grooß, Reinhold Spang, Michael C. Pitts, Lamont R. Poole, Rolf Müller, and Martin Riese
Atmos. Chem. Phys., 19, 543–563, https://doi.org/10.5194/acp-19-543-2019, https://doi.org/10.5194/acp-19-543-2019, 2019
Short summary
Short summary
We present Lagrangian simulations of polar stratospheric clouds (PSCs) for the Arctic winter 2009/2010 and the Antarctic winter 2011 using the Chemical Lagrangian Model of the Stratosphere (CLaMS). The paper comprises a detailed model description with ice PSCs and related dehydration being the focus of this study. Comparisons between our simulations and observations from different satellites on season-long and vortex-wide scales as well as for single PSC events show an overall good agreement.
Mohamadou Diallo, Paul Konopka, Michelle L. Santee, Rolf Müller, Mengchu Tao, Kaley A. Walker, Bernard Legras, Martin Riese, Manfred Ern, and Felix Ploeger
Atmos. Chem. Phys., 19, 425–446, https://doi.org/10.5194/acp-19-425-2019, https://doi.org/10.5194/acp-19-425-2019, 2019
Short summary
Short summary
This paper assesses the structural changes in the shallow and transition branches of the BDC induced by El Nino using the Lagrangian model simulations driven by ERAi and JRA-55 combined with MLS observations. We found a clear evidence of a weakening of the transition branch due to an upward shift in the dissipation height of the planetary and gravity waves and a strengthening of the shallow branch due to enhanced GW breaking in the tropics–subtropics and PW breaking at high latitudes.
Dan Li, Bärbel Vogel, Rolf Müller, Jianchun Bian, Gebhard Günther, Qian Li, Jinqiang Zhang, Zhixuan Bai, Holger Vömel, and Martin Riese
Atmos. Chem. Phys., 18, 17979–17994, https://doi.org/10.5194/acp-18-17979-2018, https://doi.org/10.5194/acp-18-17979-2018, 2018
Short summary
Short summary
Balloon-borne measurements performed over Lhasa in August 2013 are investigated using CLaMS trajectory calculations. Here, we focus on high ozone mixing ratios in the free troposphere. Our findings demonstrate that both stratospheric intrusions and convective transport of air pollution play a major role in enhancing middle and upper tropospheric ozone.
Simone Brunamonti, Teresa Jorge, Peter Oelsner, Sreeharsha Hanumanthu, Bhupendra B. Singh, K. Ravi Kumar, Sunil Sonbawne, Susanne Meier, Deepak Singh, Frank G. Wienhold, Bei Ping Luo, Maxi Boettcher, Yann Poltera, Hannu Jauhiainen, Rijan Kayastha, Jagadishwor Karmacharya, Ruud Dirksen, Manish Naja, Markus Rex, Suvarna Fadnavis, and Thomas Peter
Atmos. Chem. Phys., 18, 15937–15957, https://doi.org/10.5194/acp-18-15937-2018, https://doi.org/10.5194/acp-18-15937-2018, 2018
Short summary
Short summary
Based on balloon-borne measurements performed in India and Nepal in 2016–2017, we infer the vertical distributions of water vapor, ozone and aerosols in the atmosphere, from the surface to 30 km altitude. Our measurements show that the atmospheric dynamics of the Asian summer monsoon system over the polluted Indian subcontinent lead to increased concentrations of water vapor and aerosols in the high atmosphere (approximately 14–20 km altitude), which can have an important effect on climate.
Xue Wu, Sabine Griessbach, and Lars Hoffmann
Atmos. Chem. Phys., 18, 15859–15877, https://doi.org/10.5194/acp-18-15859-2018, https://doi.org/10.5194/acp-18-15859-2018, 2018
Short summary
Short summary
Volcanic aerosol is an important source of sulfur for Antarctica, where local sources of sulfur are rare. Midlatitude and high-latitude volcanism can directly influence the aerosol budget of the polar stratosphere, but tropical volcanic eruptions can also enhance polar aerosols by transport. Our study investigates pathway and transport processes of volcanic aerosol from the tropics to the lower stratosphere over Antarctica by combining Lagrangian transport simulation and satellite observations.
Mohamadou Diallo, Martin Riese, Thomas Birner, Paul Konopka, Rolf Müller, Michaela I. Hegglin, Michelle L. Santee, Mark Baldwin, Bernard Legras, and Felix Ploeger
Atmos. Chem. Phys., 18, 13055–13073, https://doi.org/10.5194/acp-18-13055-2018, https://doi.org/10.5194/acp-18-13055-2018, 2018
Short summary
Short summary
The unprecedented timing of an El Niño event aligned with the disrupted QBO in 2015–2016 caused a perturbation to the stratospheric circulation, affecting trace gases. This paper resolves the puzzling response of the lower stratospheric water vapor by showing that the QBO disruption reversed the lower stratosphere moistening triggered by the alignment of the El Niño event with a westerly QBO in early boreal winter.
Suvarna Fadnavis, Chaitri Roy, Rajib Chattopadhyay, Christopher E. Sioris, Alexandru Rap, Rolf Müller, K. Ravi Kumar, and Raghavan Krishnan
Atmos. Chem. Phys., 18, 11493–11506, https://doi.org/10.5194/acp-18-11493-2018, https://doi.org/10.5194/acp-18-11493-2018, 2018
Short summary
Short summary
Rapid industrialization, traffic growth and urbanization resulted in a significant increase in the tropospheric trace gases over Asia. There is global concern about rising levels of these trace gases. The monsoon convection transports these gases to the upper-level-anticyclone. In this study, we show transport of these gases to the extratropics via eddy-shedding from the anticyclone. We also deliberate on changes in ozone heating rates due to the transport of Asian trace gases.
Farahnaz Khosrawi, Stefan Lossow, Gabriele P. Stiller, Karen H. Rosenlof, Joachim Urban, John P. Burrows, Robert P. Damadeo, Patrick Eriksson, Maya García-Comas, John C. Gille, Yasuko Kasai, Michael Kiefer, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Alexei Rozanov, Christopher E. Sioris, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 11, 4435–4463, https://doi.org/10.5194/amt-11-4435-2018, https://doi.org/10.5194/amt-11-4435-2018, 2018
Short summary
Short summary
Time series of stratospheric and lower mesospheric water vapour using 33 data sets from 15 satellite instruments were compared in the framework of the second SPARC water vapour assessment. We find that most data sets can be considered in observational and modelling studies addressing, e.g. stratospheric and lower mesospheric water vapour variability and trends if data-set-specific characteristics (e.g. a drift) and restrictions (e.g. temporal and spatial coverage) are taken into account.
Jens-Uwe Grooß, Rolf Müller, Reinhold Spang, Ines Tritscher, Tobias Wegner, Martyn P. Chipperfield, Wuhu Feng, Douglas E. Kinnison, and Sasha Madronich
Atmos. Chem. Phys., 18, 8647–8666, https://doi.org/10.5194/acp-18-8647-2018, https://doi.org/10.5194/acp-18-8647-2018, 2018
Short summary
Short summary
We investigate a discrepancy between model simulations and observations of HCl in the dark polar stratosphere. In early winter, the less-well-studied period of the onset of chlorine activation, observations show a much faster depletion of HCl than simulations of three models. This points to some unknown process that is currently not represented in the models. Various hypotheses for potential causes are investigated that partly reduce the discrepancy. The impact on polar ozone depletion is low.
Liubov Poshyvailo, Rolf Müller, Paul Konopka, Gebhard Günther, Martin Riese, Aurélien Podglajen, and Felix Ploeger
Atmos. Chem. Phys., 18, 8505–8527, https://doi.org/10.5194/acp-18-8505-2018, https://doi.org/10.5194/acp-18-8505-2018, 2018
Short summary
Short summary
Water vapour (H2O) in the UTLS is a key player for global radiation, which is critical for predictions of future climate change. We investigate the effects of current uncertainties in tropopause temperature, horizontal transport and small-scale mixing on simulated H2O, using the Chemical Lagrangian Model of the Stratosphere. Our sensitivity studies provide new insights into the leading processes controlling stratospheric H2O, important for assessing and improving climate model projections.
Xiaolu Yan, Paul Konopka, Felix Ploeger, Mengchu Tao, Rolf Müller, Michelle L. Santee, Jianchun Bian, and Martin Riese
Atmos. Chem. Phys., 18, 8079–8096, https://doi.org/10.5194/acp-18-8079-2018, https://doi.org/10.5194/acp-18-8079-2018, 2018
Short summary
Short summary
Many works investigate the impact of ENSO on the troposphere. However, only a few works check the impact of ENSO at higher altitudes.
Here, we analyse the impact of ENSO on the vicinity of the tropopause using reanalysis, satellite, in situ and model data. We find that ENSO shows the strongest signal in winter, but its impact can last until early the next summer. The ENSO anomaly is insignificant in late summer. Our study can help to understand the atmosphere propagation after ENSO.
Reinhold Spang, Lars Hoffmann, Rolf Müller, Jens-Uwe Grooß, Ines Tritscher, Michael Höpfner, Michael Pitts, Andrew Orr, and Martin Riese
Atmos. Chem. Phys., 18, 5089–5113, https://doi.org/10.5194/acp-18-5089-2018, https://doi.org/10.5194/acp-18-5089-2018, 2018
Short summary
Short summary
This paper represents an unprecedented pole-covering day- and nighttime climatology of the polar stratospheric clouds (PSCs) based on satellite measurements, their spatial distribution, and composition of different particle types. The climatology has a high potential for the validation and improvement of PSC schemes in chemical transport and chemistry–climate models, which is important for a better prediction of future polar ozone loss in a changing climate.
Rolf Müller, Jens-Uwe Grooß, Abdul Mannan Zafar, Sabine Robrecht, and Ralph Lehmann
Atmos. Chem. Phys., 18, 2985–2997, https://doi.org/10.5194/acp-18-2985-2018, https://doi.org/10.5194/acp-18-2985-2018, 2018
Short summary
Short summary
This paper revisits the chemistry leading to strong ozone depletion in the Antarctic. We focus on the heart of the ozone layer in the lowermost stratosphere in the core of the vortex. We argue that chemical cycles (referred to as HCl null cycles) that have hitherto been largely neglected counteract the deactivation of chlorine and are therefore key to ozone depletion in the core of the Antarctic vortex. The key process to full activation of chlorine is the photolysis of formaldehyde.
Christian Rolf, Bärbel Vogel, Peter Hoor, Armin Afchine, Gebhard Günther, Martina Krämer, Rolf Müller, Stefan Müller, Nicole Spelten, and Martin Riese
Atmos. Chem. Phys., 18, 2973–2983, https://doi.org/10.5194/acp-18-2973-2018, https://doi.org/10.5194/acp-18-2973-2018, 2018
Short summary
Short summary
The Asian monsoon is a pronounced circulation system linked to rapid vertical transport of surface air from India and east Asia in the summer months. We found, based on aircraft measurements, higher concentration of water vapor in the lowermost stratosphere caused by the Asian monsoon. Enrichment of water vapor concentrations in the lowermost stratosphere impacts the radiation budget and thus climate. Understanding those variations in water vapor is important for climate projections.
Annika Günther, Michael Höpfner, Björn-Martin Sinnhuber, Sabine Griessbach, Terry Deshler, Thomas von Clarmann, and Gabriele Stiller
Atmos. Chem. Phys., 18, 1217–1239, https://doi.org/10.5194/acp-18-1217-2018, https://doi.org/10.5194/acp-18-1217-2018, 2018
Short summary
Short summary
Satellite-borne data of sulfur dioxide and a new data set of sulfate aerosol volume densities, as retrieved from MIPAS measurements, are studied in the upper-troposphere–lower-stratosphere region. General patterns of enhanced aerosol are in agreement with SO2. Via chemical transport model simulations for two volcanic eruptions in the Northern Hemisphere midlatitudes, we show that the volcanic enhancements in MIPAS SO2 and sulfate aerosol are consistent in terms of mass and transport patterns.
Xue Wu, Sabine Griessbach, and Lars Hoffmann
Atmos. Chem. Phys., 17, 13439–13455, https://doi.org/10.5194/acp-17-13439-2017, https://doi.org/10.5194/acp-17-13439-2017, 2017
Short summary
Short summary
This study is focused on the Sarychev eruption in 2009. Based on Lagrangian model simulations and satellite data, the equatorward transport of the plume and aerosol from the Sarychev eruption is confirmed, and the transport is facilitated by the Asian summer monsoon anticyclonic circulations. The aerosol transported to the tropics remained for months and dispersed upward, which could make the Sarychev eruption have a similar global climate impact as a tropical volcanic eruption.
Suvarna Fadnavis, Gayatry Kalita, K. Ravi Kumar, Blaž Gasparini, and Jui-Lin Frank Li
Atmos. Chem. Phys., 17, 11637–11654, https://doi.org/10.5194/acp-17-11637-2017, https://doi.org/10.5194/acp-17-11637-2017, 2017
Short summary
Short summary
In this study, the model simulations show that monsoon convection over the Bay of Bengal, the South China Sea and southern flanks of the Himalayas transports Asian carbonaceous aerosol into the UTLS. Carbonaceous aerosol induces enhancement in heating rate, vertical velocity and water vapor transport in the UTLS. Doubling of carbonaceous aerosols creates an anomalous warming over the TP. It generates monsoon Hadley circulation and thus increases precipitation over India and northeast China.
Dan Weaver, Kimberly Strong, Matthias Schneider, Penny M. Rowe, Chris Sioris, Kaley A. Walker, Zen Mariani, Taneil Uttal, C. Thomas McElroy, Holger Vömel, Alessio Spassiani, and James R. Drummond
Atmos. Meas. Tech., 10, 2851–2880, https://doi.org/10.5194/amt-10-2851-2017, https://doi.org/10.5194/amt-10-2851-2017, 2017
Short summary
Short summary
We have compared techniques used by several PEARL instruments to measure atmospheric water vapour. No single instrument can comprehensively map the atmosphere. We documented how well these techniques perform and quantified the agreement and biases between them. This work showed that new FTIR datasets at PEARL capture accurate measurements of High Arctic water vapour.
Cristen Adams, Adam E. Bourassa, Chris A. McLinden, Chris E. Sioris, Thomas von Clarmann, Bernd Funke, Landon A. Rieger, and Douglas A. Degenstein
Atmos. Chem. Phys., 17, 8063–8080, https://doi.org/10.5194/acp-17-8063-2017, https://doi.org/10.5194/acp-17-8063-2017, 2017
Short summary
Short summary
We measured the relationship between volcanic aerosol and trace gases in the stratosphere using the OSIRIS and MIPAS satellite instruments between 2002 and 2014. We found that levels of stratospheric NO2 and N2O5 both decreased significantly in the presence of volcanic aerosol. These decreases were consistent with the modeling results.
Shailesh K. Kharol, Chris A. McLinden, Christopher E. Sioris, Mark W. Shephard, Vitali Fioletov, Aaron van Donkelaar, Sajeev Philip, and Randall V. Martin
Atmos. Chem. Phys., 17, 5921–5929, https://doi.org/10.5194/acp-17-5921-2017, https://doi.org/10.5194/acp-17-5921-2017, 2017
Dan Li, Bärbel Vogel, Jianchun Bian, Rolf Müller, Laura L. Pan, Gebhard Günther, Zhixuan Bai, Qian Li, Jinqiang Zhang, Qiujun Fan, and Holger Vömel
Atmos. Chem. Phys., 17, 4657–4672, https://doi.org/10.5194/acp-17-4657-2017, https://doi.org/10.5194/acp-17-4657-2017, 2017
Short summary
Short summary
High-resolution ozone and water vapour profiles over Lhasa, China, were measured in August 2013. The correlations between ozone and water vapour profiles show a strong variability in the upper troposphere. These relationships were investigated using CLaMS trajectory calculations. The model results demonstrate that three tropical cyclones (Jebi, Utor, and Trami), occurring over the western Pacific, had a strong impact on the vertical structure of ozone and water vapour profiles.
Christopher E. Sioris, Landon A. Rieger, Nicholas D. Lloyd, Adam E. Bourassa, Chris Z. Roth, Douglas A. Degenstein, Claude Camy-Peyret, Klaus Pfeilsticker, Gwenaël Berthet, Valéry Catoire, Florence Goutail, Jean-Pierre Pommereau, and Chris A. McLinden
Atmos. Meas. Tech., 10, 1155–1168, https://doi.org/10.5194/amt-10-1155-2017, https://doi.org/10.5194/amt-10-1155-2017, 2017
Short summary
Short summary
A new OSIRIS NO2 retrieval algorithm is described and validated using > 40 balloon-based profile measurements. The validation results indicate a slight improvement relative to the existing operational algorithm in terms of the bias versus the balloon data, particularly in the lower stratosphere. The implication is that this new algorithm should replace the operational one. The motivation was to combine spectral fitting and the SaskTRAN radiative transfer model to achieve an improved product.
Stefan Lossow, Farahnaz Khosrawi, Gerald E. Nedoluha, Faiza Azam, Klaus Bramstedt, John. P. Burrows, Bianca M. Dinelli, Patrick Eriksson, Patrick J. Espy, Maya García-Comas, John C. Gille, Michael Kiefer, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Gabriele P. Stiller, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 10, 1111–1137, https://doi.org/10.5194/amt-10-1111-2017, https://doi.org/10.5194/amt-10-1111-2017, 2017
Christopher E. Sioris, Chris A. McLinden, Mark W. Shephard, Vitali E. Fioletov, and Ihab Abboud
Atmos. Chem. Phys., 17, 1931–1943, https://doi.org/10.5194/acp-17-1931-2017, https://doi.org/10.5194/acp-17-1931-2017, 2017
Short summary
Short summary
The contribution of the oil sands region to the local aerosol optical depth (AOD) is sought. Satellite data are used since they provide spatial coverage over many years. Satellites measure AOD with high correlation and small biases relative to coincident AERONET AODs. Trends are determined using annual mean AODs, and an increasing trend is found near the Shell mines. Spatially variable and high surface albedo is challenging for some sensors. Measuring polarization appears to be an asset.
Chaitri Roy, Suvarna Fadnavis, Rolf Müller, D. C. Ayantika, Felix Ploeger, and Alexandru Rap
Atmos. Chem. Phys., 17, 1297–1311, https://doi.org/10.5194/acp-17-1297-2017, https://doi.org/10.5194/acp-17-1297-2017, 2017
Short summary
Short summary
In the monsoon season, Asian NOx emissions are rapidly transported to the UTLS and can impact ozone in the UTLS. From chemistry–climate model simulations, we show that increasing Asian NOx emissions have enhanced ozone radiative forcing over Southeast Asia, which leads to significant warming over the Tibetan Plateau and increase precipitation over India. However, a further increase in NOx emissions elicited negative precipitation due to reversal of monsoon Hadley circulation.
Bärbel Vogel, Gebhard Günther, Rolf Müller, Jens-Uwe Grooß, Armin Afchine, Heiko Bozem, Peter Hoor, Martina Krämer, Stefan Müller, Martin Riese, Christian Rolf, Nicole Spelten, Gabriele P. Stiller, Jörn Ungermann, and Andreas Zahn
Atmos. Chem. Phys., 16, 15301–15325, https://doi.org/10.5194/acp-16-15301-2016, https://doi.org/10.5194/acp-16-15301-2016, 2016
Short summary
Short summary
The identification of transport pathways from the Asian monsoon anticyclone into the lower stratosphere is unclear. Global simulations with the CLaMS model demonstrate that source regions in Asia and in the Pacific Ocean have a significant impact on the chemical composition of the lower stratosphere of the Northern Hemisphere by flooding the extratropical lower stratosphere with young moist air masses. Two main horizontal transport pathways from the Asian monsoon anticyclone are identified.
Sabine Griessbach, Lars Hoffmann, Reinhold Spang, Marc von Hobe, Rolf Müller, and Martin Riese
Atmos. Meas. Tech., 9, 4399–4423, https://doi.org/10.5194/amt-9-4399-2016, https://doi.org/10.5194/amt-9-4399-2016, 2016
Short summary
Short summary
A new method for detecting aerosol in the UTLS based on infrared limb emission measurements is presented. The method was developed using radiative transfer simulations (including scattering) and Envisat MIPAS measurements. Results are presented for volcanic ash and sulfate aerosol originating from the Grimsvötn (Iceland), Puyehue–Cordon Caulle (Chile), and Nabro (Eritrea) eruptions in 2011 and compared with AIRS volcanic ash and SO2 measurements.
Reinhold Spang, Lars Hoffmann, Michael Höpfner, Sabine Griessbach, Rolf Müller, Michael C. Pitts, Andrew M. W. Orr, and Martin Riese
Atmos. Meas. Tech., 9, 3619–3639, https://doi.org/10.5194/amt-9-3619-2016, https://doi.org/10.5194/amt-9-3619-2016, 2016
Short summary
Short summary
We present a new classification approach for different polar stratospheric cloud types. The so-called Bayesian classifier estimates the most likely probability that one of the three PSC types (ice, NAT, or STS) dominates the characteristics of a measured infrared spectrum. The entire measurement period of the satellite instrument MIPAS from July 2002 to April 2013 is processed using the new classifier.
Wolfgang Woiwode, Michael Höpfner, Lei Bi, Michael C. Pitts, Lamont R. Poole, Hermann Oelhaf, Sergej Molleker, Stephan Borrmann, Marcus Klingebiel, Gennady Belyaev, Andreas Ebersoldt, Sabine Griessbach, Jens-Uwe Grooß, Thomas Gulde, Martina Krämer, Guido Maucher, Christof Piesch, Christian Rolf, Christian Sartorius, Reinhold Spang, and Johannes Orphal
Atmos. Chem. Phys., 16, 9505–9532, https://doi.org/10.5194/acp-16-9505-2016, https://doi.org/10.5194/acp-16-9505-2016, 2016
Short summary
Short summary
The analysis of spectral signatures of a polar stratospheric cloud in airborne infrared remote sensing observations in the Arctic in combination with further collocated measurements supports the view that the observed cloud consisted of highly aspherical nitric acid trihydrate particles. A characteristic "shoulder-like" spectral signature may be exploited for identification of large, highly aspherical nitric acid trihydrate particles involved in denitrification of the polar winter stratosphere.
Jörn Ungermann, Mandfred Ern, Martin Kaufmann, Rolf Müller, Reinhold Spang, Felix Ploeger, Bärbel Vogel, and Martin Riese
Atmos. Chem. Phys., 16, 8389–8403, https://doi.org/10.5194/acp-16-8389-2016, https://doi.org/10.5194/acp-16-8389-2016, 2016
Short summary
Short summary
This paper presents an analysis of temperature and the trace gases PAN and O3 in
the Asian Summer Monsoon (ASM) region. The positive PAN anomaly consisting of
polluted air is confined vertically within the main ASM anticyclone, whereas a
recently shed eddy exhibits enhanced PAN VMRs for 1 to 2 km above the thermal
tropopause. This implies that eddy shedding provides a very rapid horizontal
transport pathway of Asian pollution into the extratropical lowermost
stratosphere.
Charlotte Marinke Hoppe, Felix Ploeger, Paul Konopka, and Rolf Müller
Atmos. Chem. Phys., 16, 6223–6239, https://doi.org/10.5194/acp-16-6223-2016, https://doi.org/10.5194/acp-16-6223-2016, 2016
Yi Heng, Lars Hoffmann, Sabine Griessbach, Thomas Rößler, and Olaf Stein
Geosci. Model Dev., 9, 1627–1645, https://doi.org/10.5194/gmd-9-1627-2016, https://doi.org/10.5194/gmd-9-1627-2016, 2016
Short summary
Short summary
A new inverse modeling and simulation system is developed to enable efficient and reliable transport simulations of volcanic SO2 at large scale. The complex time- and altitude-dependent volcanic emission pattern of the Nabro eruption is identified by our inversion algorithm. The simulation results show good agreements with different satellite observations in terms of SO2 horizontal distributions, and help to further reveal the complex transport processes such as the Asian monsoon circulation.
Stefan Noël, Klaus Bramstedt, Michael Hilker, Patricia Liebing, Johannes Plieninger, Max Reuter, Alexei Rozanov, Christopher E. Sioris, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 9, 1485–1503, https://doi.org/10.5194/amt-9-1485-2016, https://doi.org/10.5194/amt-9-1485-2016, 2016
Short summary
Short summary
Stratospheric methane (CH4) and carbon dioxide (CO2) profiles have been derived from solar occultation measurements of the SCIAMACHY satellite instrument. The accuracy of these profiles is estimated to be about 5–10 % for CH4 and 2–3 % for CO2, mainly limited by unexpected vertical oscillations. Results are available for August 2002 to April 2012 and latitudes between about 50 and 70° N. From these, time series trends have been estimated, which are in reasonable agreement with total column trends.
Christopher E. Sioris, Jason Zou, David A. Plummer, Chris D. Boone, C. Thomas McElroy, Patrick E. Sheese, Omid Moeini, and Peter F. Bernath
Atmos. Chem. Phys., 16, 3265–3278, https://doi.org/10.5194/acp-16-3265-2016, https://doi.org/10.5194/acp-16-3265-2016, 2016
Short summary
Short summary
The AM (annular mode) is the most important internal mode of climatic variability at high latitudes. Upper tropospheric water vapour (UTWV) at high latitudes increases by up to ~ 50 % during the negative phase of the AMs. The response of water vapour to the AMs vanishes above the tropopause. The ultimate goal of the study was to improve UTWV trend uncertainties by explaining shorter-term variability, and this was achieved by accounting for the AM-related response in a multiple linear regression.
Christopher E. Sioris, Jason Zou, C. Thomas McElroy, Chris D. Boone, Patrick E. Sheese, and Peter F. Bernath
Atmos. Chem. Phys., 16, 2207–2219, https://doi.org/10.5194/acp-16-2207-2016, https://doi.org/10.5194/acp-16-2207-2016, 2016
Short summary
Short summary
This paper shows that volcanic eruptions occurring at higher latitudes in windy environments can lead to significant perturbations to upper tropospheric (UT) humidity mostly due to entrainment of lower tropospheric moisture by wind-blown plumes.
This research was performed for the purpose of determining long-term trends in high-latitude UT water vapour. The steps involve building a monthly climatology and using it to deseasonalize the time series. Large observed anomalies are then studied.
Suvarna Fadnavis, K. Ravi Kumar, Yogesh K. Tiwari, and Luca Pozzoli
Ann. Geophys., 34, 279–291, https://doi.org/10.5194/angeo-34-279-2016, https://doi.org/10.5194/angeo-34-279-2016, 2016
Short summary
Short summary
Analysis of 10 years (2000–2009) of Carbon Tracker (CT-2010) model CO2 fluxes gives insights into the regional variation of CO2 fluxes over the Indian land mass. CO2 emission hot spots overlap with locations of densely clustered thermal power plants, coal mines, and other industrial and urban centres. CO2 sink regions coincide with locations of dense forests with less industrial centres. CO2 fossil fuel emissions show good agreement with two bottom-up inventories REAS v1.11 and EDGAR v4.2.
B. Vogel, G. Günther, R. Müller, J.-U. Grooß, and M. Riese
Atmos. Chem. Phys., 15, 13699–13716, https://doi.org/10.5194/acp-15-13699-2015, https://doi.org/10.5194/acp-15-13699-2015, 2015
Short summary
Short summary
The Asian summer monsoon circulation is an important global circulation system associated with strong upward transport of tropospheric source gases. We show that the contribution of different boundary source regions to the Asian monsoon anticyclone strongly depends on its intra-seasonal variability and that emissions from Asia have a significant impact on the chemical compositions of the lowermost stratosphere of the Northern Hemisphere at the end of the monsoon season in Sep./Oct. 2012.
F. Ploeger, C. Gottschling, S. Griessbach, J.-U. Grooß, G. Guenther, P. Konopka, R. Müller, M. Riese, F. Stroh, M. Tao, J. Ungermann, B. Vogel, and M. von Hobe
Atmos. Chem. Phys., 15, 13145–13159, https://doi.org/10.5194/acp-15-13145-2015, https://doi.org/10.5194/acp-15-13145-2015, 2015
Short summary
Short summary
The Asian summer monsoon provides an important pathway of tropospheric source gases and pollution into the lower stratosphere. This transport is characterized by deep convection and steady upwelling, combined with confinement inside a large-scale anticyclonic circulation in the upper troposphere and lower stratosphere. In this paper, we show that a barrier to horizontal transport in the monsoon can be determined from a local maximum in the gradient of potential vorticity.
S. Fadnavis, K. Semeniuk, M. G. Schultz, M. Kiefer, A. Mahajan, L. Pozzoli, and S. Sonbawane
Atmos. Chem. Phys., 15, 11477–11499, https://doi.org/10.5194/acp-15-11477-2015, https://doi.org/10.5194/acp-15-11477-2015, 2015
Short summary
Short summary
The model and MIPAS satellite data show that there are three regions which contribute substantial pollution to the south Asian UTLS: the Asian summer monsoon (ASM), the North American monsoon (NAM) and the West African monsoon (WAM). However, penetration due to ASM convection reaches deeper into the UTLS compared to NAM and WAM outflow. Simulations show that westerly winds drive North American and European pollutants eastward where they can become part of the ASM and lifted to LS.
N. R. P. Harris, B. Hassler, F. Tummon, G. E. Bodeker, D. Hubert, I. Petropavlovskikh, W. Steinbrecht, J. Anderson, P. K. Bhartia, C. D. Boone, A. Bourassa, S. M. Davis, D. Degenstein, A. Delcloo, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, N. Jones, M. J. Kurylo, E. Kyrölä, M. Laine, S. T. Leblanc, J.-C. Lambert, B. Liley, E. Mahieu, A. Maycock, M. de Mazière, A. Parrish, R. Querel, K. H. Rosenlof, C. Roth, C. Sioris, J. Staehelin, R. S. Stolarski, R. Stübi, J. Tamminen, C. Vigouroux, K. A. Walker, H. J. Wang, J. Wild, and J. M. Zawodny
Atmos. Chem. Phys., 15, 9965–9982, https://doi.org/10.5194/acp-15-9965-2015, https://doi.org/10.5194/acp-15-9965-2015, 2015
Short summary
Short summary
Trends in the vertical distribution of ozone are reported for new and recently revised data sets. The amount of ozone-depleting compounds in the stratosphere peaked in the second half of the 1990s. We examine the trends before and after that peak to see if any change in trend is discernible. The previously reported decreases are confirmed. Furthermore, the downward trend in upper stratospheric ozone has not continued. The possible significance of any increase is discussed in detail.
S. D. Bansod, S. Fadnavis, and S. P. Ghanekar
Ann. Geophys., 33, 1051–1058, https://doi.org/10.5194/angeo-33-1051-2015, https://doi.org/10.5194/angeo-33-1051-2015, 2015
Short summary
Short summary
In this paper inter-annual variability of tropospheric air temperature over the Asian summer monsoon region during the pre-monsoon months is examined in relation to Indian summer monsoon rainfall (ISMR; June to September total rainfall). The results indicate a strong and significant northwest–southeast dipole structure in the spatial correlations over the Indian region with highly significant positive (negative) correlations over the regions of north India and the western Tibetan Plateau region.
M. Tao, P. Konopka, F. Ploeger, J.-U. Grooß, R. Müller, C. M. Volk, K. A. Walker, and M. Riese
Atmos. Chem. Phys., 15, 8695–8715, https://doi.org/10.5194/acp-15-8695-2015, https://doi.org/10.5194/acp-15-8695-2015, 2015
Short summary
Short summary
A remarkable major stratospheric sudden warming during the boreal winter 2008/09 is studied with the Chemical Lagrangian Model of the Stratosphere (CLaMS). We investigate how mixing triggered by this event correlates the wave forcing and how transport and mixing affect the composition of the whole stratosphere in the Northern Hemisphere, by using the tracer-tracer correlation technique.
O. Kirner, R. Müller, R. Ruhnke, and H. Fischer
Atmos. Chem. Phys., 15, 2019–2030, https://doi.org/10.5194/acp-15-2019-2015, https://doi.org/10.5194/acp-15-2019-2015, 2015
Short summary
Short summary
We use multi-year simulations of the chemistry--climate model EMAC to investigate
the impact that the various types of PSCs have on Antarctic chlorine activation and ozone loss. Heterogeneous chemistry on liquid particles is responsible for more than 90% of the ozone depletion in Antarctic spring in the model simulations. In high southern latitudes, heterogeneous chemistry on ice particles causes only up to 5 DU of additional ozone depletion and chemistry on NAT particles less than 0.5 DU.
R. Spang, G. Günther, M. Riese, L. Hoffmann, R. Müller, and S. Griessbach
Atmos. Chem. Phys., 15, 927–950, https://doi.org/10.5194/acp-15-927-2015, https://doi.org/10.5194/acp-15-927-2015, 2015
Short summary
Short summary
Here we present observations of the Cryogenic Infrared Spectrometers and Telescopes for the Atmosphere (CRISTA) of cirrus cloud and water vapour in August 1997 in the upper troposphere and lower stratosphere (UTLS) region. The observations indicate a considerable flux of moisture from the upper tropical troposphere into the extra-tropical lowermost stratosphere (LMS), resulting in the occurrence of high-altitude optically thin cirrus clouds in the LMS.
R. Pommrich, R. Müller, J.-U. Grooß, P. Konopka, F. Ploeger, B. Vogel, M. Tao, C. M. Hoppe, G. Günther, N. Spelten, L. Hoffmann, H.-C. Pumphrey, S. Viciani, F. D'Amato, C. M. Volk, P. Hoor, H. Schlager, and M. Riese
Geosci. Model Dev., 7, 2895–2916, https://doi.org/10.5194/gmd-7-2895-2014, https://doi.org/10.5194/gmd-7-2895-2014, 2014
Short summary
Short summary
A version of the chemical transport model CLaMS is presented, which features a simplified (numerically inexpensive) chemistry scheme. The model results using this version of CLaMS show a good representation of anomaly fields of CO, CH4, N2O, and CFC-11 in the lower stratosphere. CO measurements of three instruments (COLD, HAGAR, and Falcon-CO) in the lower tropical stratosphere (during the campaign TROCCINOX in 2005) have been compared and show a good agreement within the error bars.
B. Vogel, G. Günther, R. Müller, J.-U. Grooß, P. Hoor, M. Krämer, S. Müller, A. Zahn, and M. Riese
Atmos. Chem. Phys., 14, 12745–12762, https://doi.org/10.5194/acp-14-12745-2014, https://doi.org/10.5194/acp-14-12745-2014, 2014
Short summary
Short summary
Enhanced tropospheric trace gases (e.g. pollutants) were measured in situ in
the lowermost stratosphere over Northern Europe on 26 September 2012
during the TACTS aircraft campaign. We found that the combination of rapid uplift by a typhoon and eastward eddy shedding from the Asian monsoon anticyclone is a novel fast transport pathway
that may carry boundary emissions from Southeast
Asia/western Pacific within approximately 5 weeks to the lowermost
stratosphere in Northern Europe.
S. Fadnavis, M. G. Schultz, K. Semeniuk, A. S. Mahajan, L. Pozzoli, S. Sonbawne, S. D. Ghude, M. Kiefer, and E. Eckert
Atmos. Chem. Phys., 14, 12725–12743, https://doi.org/10.5194/acp-14-12725-2014, https://doi.org/10.5194/acp-14-12725-2014, 2014
Short summary
Short summary
The Asian summer monsoon transports pollutants from local emission sources to the upper troposphere and lower stratosphere (UTLS). The increasing trend of these pollutants may have climatic impact. This study addresses the impact of convectively lifted Indian and Chinese emissions on the ULTS. Sensitivity experiments with emission changes in particular regions show that Chinese emissions have a greater impact on the concentrations of NOY species than Indian emissions.
L. Hoffmann, C. M. Hoppe, R. Müller, G. S. Dutton, J. C. Gille, S. Griessbach, A. Jones, C. I. Meyer, R. Spang, C. M. Volk, and K. A. Walker
Atmos. Chem. Phys., 14, 12479–12497, https://doi.org/10.5194/acp-14-12479-2014, https://doi.org/10.5194/acp-14-12479-2014, 2014
Short summary
Short summary
Stratospheric lifetimes determine the global warming and ozone depletion potentials of chlorofluorocarbons. We present new estimates of the CFC-11/CFC-12 lifetime ratio from satellite and model data (ACE-FTS, HIRDLS, MIPAS, and EMAC/CLaMS). Our estimates of 0.46+/-0.04 (satellites) and 0.48+/-0.07 (model) are in excellent agreement with the recent SPARC reassessment. Having smaller uncertainties than other studies, our results can help to better constrain future CFC lifetime recommendations.
C. M. Hoppe, L. Hoffmann, P. Konopka, J.-U. Grooß, F. Ploeger, G. Günther, P. Jöckel, and R. Müller
Geosci. Model Dev., 7, 2639–2651, https://doi.org/10.5194/gmd-7-2639-2014, https://doi.org/10.5194/gmd-7-2639-2014, 2014
A. Kunz, N. Spelten, P. Konopka, R. Müller, R. M. Forbes, and H. Wernli
Atmos. Chem. Phys., 14, 10803–10822, https://doi.org/10.5194/acp-14-10803-2014, https://doi.org/10.5194/acp-14-10803-2014, 2014
S. Molleker, S. Borrmann, H. Schlager, B. Luo, W. Frey, M. Klingebiel, R. Weigel, M. Ebert, V. Mitev, R. Matthey, W. Woiwode, H. Oelhaf, A. Dörnbrack, G. Stratmann, J.-U. Grooß, G. Günther, B. Vogel, R. Müller, M. Krämer, J. Meyer, and F. Cairo
Atmos. Chem. Phys., 14, 10785–10801, https://doi.org/10.5194/acp-14-10785-2014, https://doi.org/10.5194/acp-14-10785-2014, 2014
S. Fadnavis, K. Semeniuk, M. G. Schultz, A. Mahajan, L. Pozzoli, S. Sonbawane, and M. Kiefer
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-20159-2014, https://doi.org/10.5194/acpd-14-20159-2014, 2014
Revised manuscript not accepted
C. E. Sioris, C. D. Boone, R. Nassar, K. J. Sutton, I. E. Gordon, K. A. Walker, and P. F. Bernath
Atmos. Meas. Tech., 7, 2243–2262, https://doi.org/10.5194/amt-7-2243-2014, https://doi.org/10.5194/amt-7-2243-2014, 2014
A. E. Bourassa, D. A. Degenstein, W. J. Randel, J. M. Zawodny, E. Kyrölä, C. A. McLinden, C. E. Sioris, and C. Z. Roth
Atmos. Chem. Phys., 14, 6983–6994, https://doi.org/10.5194/acp-14-6983-2014, https://doi.org/10.5194/acp-14-6983-2014, 2014
S. Griessbach, L. Hoffmann, R. Spang, and M. Riese
Atmos. Meas. Tech., 7, 1487–1507, https://doi.org/10.5194/amt-7-1487-2014, https://doi.org/10.5194/amt-7-1487-2014, 2014
C. E. Sioris, C. A. McLinden, V. E. Fioletov, C. Adams, J. M. Zawodny, A. E. Bourassa, C. Z. Roth, and D. A. Degenstein
Atmos. Chem. Phys., 14, 3479–3496, https://doi.org/10.5194/acp-14-3479-2014, https://doi.org/10.5194/acp-14-3479-2014, 2014
J.-U. Grooß, I. Engel, S. Borrmann, W. Frey, G. Günther, C. R. Hoyle, R. Kivi, B. P. Luo, S. Molleker, T. Peter, M. C. Pitts, H. Schlager, G. Stiller, H. Vömel, K. A. Walker, and R. Müller
Atmos. Chem. Phys., 14, 1055–1073, https://doi.org/10.5194/acp-14-1055-2014, https://doi.org/10.5194/acp-14-1055-2014, 2014
C. Adams, A. E. Bourassa, V. Sofieva, L. Froidevaux, C. A. McLinden, D. Hubert, J.-C. Lambert, C. E. Sioris, and D. A. Degenstein
Atmos. Meas. Tech., 7, 49–64, https://doi.org/10.5194/amt-7-49-2014, https://doi.org/10.5194/amt-7-49-2014, 2014
J. Liu, D. W. Tarasick, V. E. Fioletov, C. McLinden, T. Zhao, S. Gong, C. Sioris, J. J. Jin, G. Liu, and O. Moeini
Atmos. Chem. Phys., 13, 11441–11464, https://doi.org/10.5194/acp-13-11441-2013, https://doi.org/10.5194/acp-13-11441-2013, 2013
M. von Hobe, S. Bekki, S. Borrmann, F. Cairo, F. D'Amato, G. Di Donfrancesco, A. Dörnbrack, A. Ebersoldt, M. Ebert, C. Emde, I. Engel, M. Ern, W. Frey, S. Genco, S. Griessbach, J.-U. Grooß, T. Gulde, G. Günther, E. Hösen, L. Hoffmann, V. Homonnai, C. R. Hoyle, I. S. A. Isaksen, D. R. Jackson, I. M. Jánosi, R. L. Jones, K. Kandler, C. Kalicinsky, A. Keil, S. M. Khaykin, F. Khosrawi, R. Kivi, J. Kuttippurath, J. C. Laube, F. Lefèvre, R. Lehmann, S. Ludmann, B. P. Luo, M. Marchand, J. Meyer, V. Mitev, S. Molleker, R. Müller, H. Oelhaf, F. Olschewski, Y. Orsolini, T. Peter, K. Pfeilsticker, C. Piesch, M. C. Pitts, L. R. Poole, F. D. Pope, F. Ravegnani, M. Rex, M. Riese, T. Röckmann, B. Rognerud, A. Roiger, C. Rolf, M. L. Santee, M. Scheibe, C. Schiller, H. Schlager, M. Siciliani de Cumis, N. Sitnikov, O. A. Søvde, R. Spang, N. Spelten, F. Stordal, O. Sumińska-Ebersoldt, A. Ulanovski, J. Ungermann, S. Viciani, C. M. Volk, M. vom Scheidt, P. von der Gathen, K. Walker, T. Wegner, R. Weigel, S. Weinbruch, G. Wetzel, F. G. Wienhold, I. Wohltmann, W. Woiwode, I. A. K. Young, V. Yushkov, B. Zobrist, and F. Stroh
Atmos. Chem. Phys., 13, 9233–9268, https://doi.org/10.5194/acp-13-9233-2013, https://doi.org/10.5194/acp-13-9233-2013, 2013
S. Fadnavis, K. Semeniuk, L. Pozzoli, M. G. Schultz, S. D. Ghude, S. Das, and R. Kakatkar
Atmos. Chem. Phys., 13, 8771–8786, https://doi.org/10.5194/acp-13-8771-2013, https://doi.org/10.5194/acp-13-8771-2013, 2013
K. Minschwaner, L. Hoffmann, A. Brown, M. Riese, R. Müller, and P. F. Bernath
Atmos. Chem. Phys., 13, 4253–4263, https://doi.org/10.5194/acp-13-4253-2013, https://doi.org/10.5194/acp-13-4253-2013, 2013
F. Khosrawi, R. Müller, J. Urban, M. H. Proffitt, G. Stiller, M. Kiefer, S. Lossow, D. Kinnison, F. Olschewski, M. Riese, and D. Murtagh
Atmos. Chem. Phys., 13, 3619–3641, https://doi.org/10.5194/acp-13-3619-2013, https://doi.org/10.5194/acp-13-3619-2013, 2013
Related subject area
Subject: Aerosols | Research Activity: Atmospheric Modelling and Data Analysis | Altitude Range: Stratosphere | Science Focus: Chemistry (chemical composition and reactions)
Analysis of the global atmospheric background sulfur budget in a multi-model framework
Stratospheric ozone depletion inside the volcanic plume shortly after the 2022 Hunga Tonga eruption
Effects of denitrification on the distributions of trace gas abundances in the polar regions: a comparison of WACCM with observations
Reconstructing volcanic radiative forcing since 1990, using a comprehensive emission inventory and spatially resolved sulfur injections from satellite data in a chemistry-climate model
Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes
Stratospheric ozone response to sulfate aerosol and solar dimming climate interventions based on the G6 Geoengineering Model Intercomparison Project (GeoMIP) simulations
Mountain-wave-induced polar stratospheric clouds and their representation in the global chemistry model ICON-ART
Co-emission of volcanic sulfur and halogens amplifies volcanic effective radiative forcing
Potential of future stratospheric ozone loss in the midlatitudes under global warming and sulfate geoengineering
Evaluating the simulated radiative forcings, aerosol properties, and stratospheric warmings from the 1963 Mt Agung, 1982 El Chichón, and 1991 Mt Pinatubo volcanic aerosol clouds
The impact of recent changes in Asian anthropogenic emissions of SO2 on sulfate loading in the upper troposphere and lower stratosphere and the associated radiative changes
Mechanism of ozone loss under enhanced water vapour conditions in the mid-latitude lower stratosphere in summer
Multi-model comparison of the volcanic sulfate deposition from the 1815 eruption of Mt. Tambora
Impacts of Mt Pinatubo volcanic aerosol on the tropical stratosphere in chemistry–climate model simulations using CCMI and CMIP6 stratospheric aerosol data
Potential impact of carbonaceous aerosol on the upper troposphere and lower stratosphere (UTLS) and precipitation during Asian summer monsoon in a global model simulation
Vortex-wide chlorine activation by a mesoscale PSC event in the Arctic winter of 2009/10
Solar geoengineering using solid aerosol in the stratosphere
Lagrangian analysis of microphysical and chemical processes in the Antarctic stratosphere: a case study
Aerosol microphysics simulations of the Mt.~Pinatubo eruption with the UM-UKCA composition-climate model
Modeling of 2008 Kasatochi volcanic sulfate direct radiative forcing: assimilation of OMI SO2 plume height data and comparison with MODIS and CALIOP observations
Microphysical simulations of sulfur burdens from stratospheric sulfur geoengineering
The role of carbonyl sulphide as a source of stratospheric sulphate aerosol and its impact on climate
Christina V. Brodowsky, Timofei Sukhodolov, Gabriel Chiodo, Valentina Aquila, Slimane Bekki, Sandip S. Dhomse, Michael Höpfner, Anton Laakso, Graham W. Mann, Ulrike Niemeier, Giovanni Pitari, Ilaria Quaglia, Eugene Rozanov, Anja Schmidt, Takashi Sekiya, Simone Tilmes, Claudia Timmreck, Sandro Vattioni, Daniele Visioni, Pengfei Yu, Yunqian Zhu, and Thomas Peter
Atmos. Chem. Phys., 24, 5513–5548, https://doi.org/10.5194/acp-24-5513-2024, https://doi.org/10.5194/acp-24-5513-2024, 2024
Short summary
Short summary
The aerosol layer is an essential part of the climate system. We characterize the sulfur budget in a volcanically quiescent (background) setting, with a special focus on the sulfate aerosol layer using, for the first time, a multi-model approach. The aim is to identify weak points in the representation of the atmospheric sulfur budget in an intercomparison of nine state-of-the-art coupled global circulation models.
Yunqian Zhu, Robert W. Portmann, Douglas Kinnison, Owen Brian Toon, Luis Millán, Jun Zhang, Holger Vömel, Simone Tilmes, Charles G. Bardeen, Xinyue Wang, Stephanie Evan, William J. Randel, and Karen H. Rosenlof
Atmos. Chem. Phys., 23, 13355–13367, https://doi.org/10.5194/acp-23-13355-2023, https://doi.org/10.5194/acp-23-13355-2023, 2023
Short summary
Short summary
The 2022 Hunga Tonga eruption injected a large amount of water into the stratosphere. Ozone depletion was observed inside the volcanic plume. Chlorine and water vapor injected by this eruption exceeded the normal range, which made the ozone chemistry during this event occur at a higher temperature than polar ozone depletion. Unlike polar ozone chemistry where chlorine nitrate is more important, hypochlorous acid plays a large role in the in-plume chlorine balance and heterogeneous processes.
Michael Weimer, Douglas E. Kinnison, Catherine Wilka, and Susan Solomon
Atmos. Chem. Phys., 23, 6849–6861, https://doi.org/10.5194/acp-23-6849-2023, https://doi.org/10.5194/acp-23-6849-2023, 2023
Short summary
Short summary
We investigate the influence of the number density of nitric acid trihydrate (NAT) particles on associated trace gases in the lower stratosphere using data from a satellite, ozonesondes and simulations by a community chemistry climate model. By comparing probability density functions between observations and the model, we find that the standard NAT number density should be reduced for future simulations with the model.
Jennifer Schallock, Christoph Brühl, Christine Bingen, Michael Höpfner, Landon Rieger, and Jos Lelieveld
Atmos. Chem. Phys., 23, 1169–1207, https://doi.org/10.5194/acp-23-1169-2023, https://doi.org/10.5194/acp-23-1169-2023, 2023
Short summary
Short summary
We characterized the influence of volcanic aerosols for the period 1990–2019 and established a volcanic SO2 emission inventory that includes more than 500 eruptions. From limb-based satellite observations of SO2 and extinction, we derive 3D plumes of SO2 perturbations and injected mass by a novel method. We calculate instantaneous radiative forcing with a comprehensive chemisty climate model. Our results show that smaller eruptions can also contribute to the stratospheric aerosol forcing.
Daniele Visioni, Ewa M. Bednarz, Walker R. Lee, Ben Kravitz, Andy Jones, Jim M. Haywood, and Douglas G. MacMartin
Atmos. Chem. Phys., 23, 663–685, https://doi.org/10.5194/acp-23-663-2023, https://doi.org/10.5194/acp-23-663-2023, 2023
Short summary
Short summary
The paper constitutes Part 1 of a study performing a first systematic inter-model comparison of the atmospheric responses to stratospheric sulfate aerosol injections (SAIs) at various latitudes as simulated by three state-of-the-art Earth system models. We identify similarities and differences in the modeled aerosol burden, investigate the differences in the aerosol approaches between the models, and ultimately show the differences produced in surface climate, temperature and precipitation.
Simone Tilmes, Daniele Visioni, Andy Jones, James Haywood, Roland Séférian, Pierre Nabat, Olivier Boucher, Ewa Monica Bednarz, and Ulrike Niemeier
Atmos. Chem. Phys., 22, 4557–4579, https://doi.org/10.5194/acp-22-4557-2022, https://doi.org/10.5194/acp-22-4557-2022, 2022
Short summary
Short summary
This study assesses the impacts of climate interventions, using stratospheric sulfate aerosol and solar dimming on stratospheric ozone, based on three Earth system models with interactive stratospheric chemistry. The climate interventions have been applied to a high emission (baseline) scenario in order to reach global surface temperatures of a medium emission scenario. We find significant increases and decreases in total column ozone, depending on regions and seasons.
Michael Weimer, Jennifer Buchmüller, Lars Hoffmann, Ole Kirner, Beiping Luo, Roland Ruhnke, Michael Steiner, Ines Tritscher, and Peter Braesicke
Atmos. Chem. Phys., 21, 9515–9543, https://doi.org/10.5194/acp-21-9515-2021, https://doi.org/10.5194/acp-21-9515-2021, 2021
Short summary
Short summary
We show that we are able to directly simulate polar stratospheric clouds formed locally in a mountain wave and represent their effect on the ozone chemistry with the global atmospheric chemistry model ICON-ART. Thus, we show the first simulations that close the gap between directly resolved mountain-wave-induced polar stratospheric clouds and their representation at coarse global resolutions.
John Staunton-Sykes, Thomas J. Aubry, Youngsub M. Shin, James Weber, Lauren R. Marshall, Nathan Luke Abraham, Alex Archibald, and Anja Schmidt
Atmos. Chem. Phys., 21, 9009–9029, https://doi.org/10.5194/acp-21-9009-2021, https://doi.org/10.5194/acp-21-9009-2021, 2021
Sabine Robrecht, Bärbel Vogel, Simone Tilmes, and Rolf Müller
Atmos. Chem. Phys., 21, 2427–2455, https://doi.org/10.5194/acp-21-2427-2021, https://doi.org/10.5194/acp-21-2427-2021, 2021
Short summary
Short summary
Column ozone protects life on Earth from radiation damage. Stratospheric chlorine compounds cause immense ozone loss in polar winter. Whether similar loss processes can occur in the lower stratosphere above North America today or in future is a matter of debate. We show that these ozone loss processes are very unlikely today or in future independently of whether sulfate geoengineering is applied and that less than 0.1 % of column ozone would be destroyed by this process in any future scenario.
Sandip S. Dhomse, Graham W. Mann, Juan Carlos Antuña Marrero, Sarah E. Shallcross, Martyn P. Chipperfield, Kenneth S. Carslaw, Lauren Marshall, N. Luke Abraham, and Colin E. Johnson
Atmos. Chem. Phys., 20, 13627–13654, https://doi.org/10.5194/acp-20-13627-2020, https://doi.org/10.5194/acp-20-13627-2020, 2020
Short summary
Short summary
We confirm downward adjustment of SO2 emission to simulate the Pinatubo aerosol cloud with aerosol microphysics models. Similar adjustment is also needed to simulate the El Chichón and Agung volcanic cloud, indicating potential missing removal or vertical redistribution process in models. Important inhomogeneities in the CMIP6 forcing datasets after Agung and El Chichón eruptions are difficult to reconcile. Quasi-biennial oscillation plays an important role in modifying stratospheric warming.
Suvarna Fadnavis, Rolf Müller, Gayatry Kalita, Matthew Rowlinson, Alexandru Rap, Jui-Lin Frank Li, Blaž Gasparini, and Anton Laakso
Atmos. Chem. Phys., 19, 9989–10008, https://doi.org/10.5194/acp-19-9989-2019, https://doi.org/10.5194/acp-19-9989-2019, 2019
Short summary
Short summary
This paper highlights the impact of Asian anthropogenic emission changes in SO2 on sulfate loading in the Asian upper troposphere–lower stratosphere from a global chemistry–climate model and satellite remote sensing. Estimated seasonal mean direct radiative forcing at the top of the atmosphere induced by the increase in Indian SO2 is −0.2–−1.5 W m2 over India. Chinese SO2 emission reduction leads to a positive radiative forcing of ~0.6–6 W m2 over China. It will likely decrease Indian rainfall.
Sabine Robrecht, Bärbel Vogel, Jens-Uwe Grooß, Karen Rosenlof, Troy Thornberry, Andrew Rollins, Martina Krämer, Lance Christensen, and Rolf Müller
Atmos. Chem. Phys., 19, 5805–5833, https://doi.org/10.5194/acp-19-5805-2019, https://doi.org/10.5194/acp-19-5805-2019, 2019
Short summary
Short summary
The potential destruction of stratospheric ozone in the mid-latitudes has been discussed recently. We analysed this ozone loss mechanism and its sensitivities. In a certain temperature range, we found a threshold in water vapour, which has to be exceeded for ozone loss to occur. We show the dependence of this water vapour threshold on temperature, sulfate content and air composition. This study provides a basis to estimate the impact of potential sulphate geoengineering on stratospheric ozone.
Lauren Marshall, Anja Schmidt, Matthew Toohey, Ken S. Carslaw, Graham W. Mann, Michael Sigl, Myriam Khodri, Claudia Timmreck, Davide Zanchettin, William T. Ball, Slimane Bekki, James S. A. Brooke, Sandip Dhomse, Colin Johnson, Jean-Francois Lamarque, Allegra N. LeGrande, Michael J. Mills, Ulrike Niemeier, James O. Pope, Virginie Poulain, Alan Robock, Eugene Rozanov, Andrea Stenke, Timofei Sukhodolov, Simone Tilmes, Kostas Tsigaridis, and Fiona Tummon
Atmos. Chem. Phys., 18, 2307–2328, https://doi.org/10.5194/acp-18-2307-2018, https://doi.org/10.5194/acp-18-2307-2018, 2018
Short summary
Short summary
We use four global aerosol models to compare the simulated sulfate deposition from the 1815 Mt. Tambora eruption to ice core records. Inter-model volcanic sulfate deposition differs considerably. Volcanic sulfate deposited on polar ice sheets is used to estimate the atmospheric sulfate burden and subsequently radiative forcing of historic eruptions. Our results suggest that deriving such relationships from model simulations may be associated with greater uncertainties than previously thought.
Laura E. Revell, Andrea Stenke, Beiping Luo, Stefanie Kremser, Eugene Rozanov, Timofei Sukhodolov, and Thomas Peter
Atmos. Chem. Phys., 17, 13139–13150, https://doi.org/10.5194/acp-17-13139-2017, https://doi.org/10.5194/acp-17-13139-2017, 2017
Short summary
Short summary
Compiling stratospheric aerosol data sets after a major volcanic eruption is difficult as the stratosphere becomes too optically opaque for satellite instruments to measure accurately. We performed ensemble chemistry–climate model simulations with two stratospheric aerosol data sets compiled for two international modelling activities and compared the simulated volcanic aerosol-induced effects from the 1991 Mt Pinatubo eruption on tropical stratospheric temperature and ozone with observations.
Suvarna Fadnavis, Gayatry Kalita, K. Ravi Kumar, Blaž Gasparini, and Jui-Lin Frank Li
Atmos. Chem. Phys., 17, 11637–11654, https://doi.org/10.5194/acp-17-11637-2017, https://doi.org/10.5194/acp-17-11637-2017, 2017
Short summary
Short summary
In this study, the model simulations show that monsoon convection over the Bay of Bengal, the South China Sea and southern flanks of the Himalayas transports Asian carbonaceous aerosol into the UTLS. Carbonaceous aerosol induces enhancement in heating rate, vertical velocity and water vapor transport in the UTLS. Doubling of carbonaceous aerosols creates an anomalous warming over the TP. It generates monsoon Hadley circulation and thus increases precipitation over India and northeast China.
Tobias Wegner, Michael C. Pitts, Lamont R. Poole, Ines Tritscher, Jens-Uwe Grooß, and Hideaki Nakajima
Atmos. Chem. Phys., 16, 4569–4577, https://doi.org/10.5194/acp-16-4569-2016, https://doi.org/10.5194/acp-16-4569-2016, 2016
Short summary
Short summary
Satellite observations are used to constrain areas with large backscatter values areas inside the polar vortex. Surface area is derived from these observations and used in heterogeneous modeling. Satellite gas species observations show a decrease in HCl downwind of areas with large surface area density indicating heterogeneous processing inside these areas. This decrease can only be simulated if a realistic surface area is assumed demonstrating the importance of polar stratospheric cloud.
D. K. Weisenstein, D. W. Keith, and J. A. Dykema
Atmos. Chem. Phys., 15, 11835–11859, https://doi.org/10.5194/acp-15-11835-2015, https://doi.org/10.5194/acp-15-11835-2015, 2015
Short summary
Short summary
We investigate stratospheric aerosol geoengineering with solid particle injection by modeling the fractal structure of alumina aerosols and their interaction with background sulfate. We analyze the efficacy (W m^-2 of radiative forcing per megaton of injection) and risks (ozone loss, s) for both alumina and diamond particles as a function of injected monomer radius, finding 240nm alumina and 160nm diamond optimal. We discuss the limitations of our 2-D model study and associated uncertainties.
L. Di Liberto, R. Lehmann, I. Tritscher, F. Fierli, J. L. Mercer, M. Snels, G. Di Donfrancesco, T. Deshler, B. P. Luo, J-U. Grooß, E. Arnone, B. M. Dinelli, and F. Cairo
Atmos. Chem. Phys., 15, 6651–6665, https://doi.org/10.5194/acp-15-6651-2015, https://doi.org/10.5194/acp-15-6651-2015, 2015
Short summary
Short summary
We investigated chemical and microphysical processes in the late winter Antarctic stratosphere, for the first time (to our knowledge) coupling a detailed microphysical box model to a chemistry model.
Model results have been compared with in situ and remote sensing measurements of particles along trajectories.
Our goal is to contribute to the most recent discussion of the relative role of PSC and liquid (background) aerosol in the ozone depletion.
S. S. Dhomse, K. M. Emmerson, G. W. Mann, N. Bellouin, K. S. Carslaw, M. P. Chipperfield, R. Hommel, N. L. Abraham, P. Telford, P. Braesicke, M. Dalvi, C. E. Johnson, F. O'Connor, O. Morgenstern, J. A. Pyle, T. Deshler, J. M. Zawodny, and L. W. Thomason
Atmos. Chem. Phys., 14, 11221–11246, https://doi.org/10.5194/acp-14-11221-2014, https://doi.org/10.5194/acp-14-11221-2014, 2014
J. Wang, S. Park, J. Zeng, C. Ge, K. Yang, S. Carn, N. Krotkov, and A. H. Omar
Atmos. Chem. Phys., 13, 1895–1912, https://doi.org/10.5194/acp-13-1895-2013, https://doi.org/10.5194/acp-13-1895-2013, 2013
J. M. English, O. B. Toon, and M. J. Mills
Atmos. Chem. Phys., 12, 4775–4793, https://doi.org/10.5194/acp-12-4775-2012, https://doi.org/10.5194/acp-12-4775-2012, 2012
C. Brühl, J. Lelieveld, P. J. Crutzen, and H. Tost
Atmos. Chem. Phys., 12, 1239–1253, https://doi.org/10.5194/acp-12-1239-2012, https://doi.org/10.5194/acp-12-1239-2012, 2012
Cited articles
Abdou, W. A., Diner, D. J., Martonchik, J. V., Bruegge, C. J., Kahn, R. A.,
Gaitley, B. J., Crean, K. A., Remer, L. A., and Holben, B.: Comparison of
coincident Multiangle Imaging Spectroradiometer and Moderate Resolution
Imaging Spectroradiometer aerosol optical depths over land and ocean scenes
containing Aerosol Robotic Network sites, J. Geophys. Res., 110, D10S07,
https://doi.org/10.1029/2004JD004693, 2005.
Andreae, M. O.: Emission of trace gases and aerosols from biomass burning – an updated assessment, Atmos. Chem. Phys., 19, 8523–8546, https://doi.org/10.5194/acp-19-8523-2019, 2019.
Banerjee A., Chiodo, G., Previdi, M., Ponater, M., Conley, A. J., and Polvani, L.
M.: Stratospheric water vapor: an important climate feedback, Clim. Dynam.,
53, 1697–1710, https://doi.org/10.1007/s00382-019-04721-4,
2019.
Bhardwaj, P., Naja, M., Kumar, R., and Chandola, H. C.: Seasonal, interannual, and long-term variabilities in biomass burning activity over South Asia, Environ. Sci. Pollut. R., 23, 4397–4410, https://doi.org/10.1007/s11356-015-5629-6, 2016.
Bond, T. C., Doherty, S. J., Fahey, D. W., Forster, P. M., Berntsen, T., Deangelo, B. J., Flanner, M. G., Ghan, S., Kärcher, B., Koch, D., Kinne, S., Kondo, Y., Quinn, P. K., Sarofim, M. C., Schultz, M. G., Schulz, M., Venkataraman, C., Zhang, H., Zhang, S., Bellouin, N., Guttikunda, S. K., Hopke, P. K., Jacobson, M. Z., Kaiser, J. W., Klimont, Z., Lohmann, U., Schwarz, J. P., Shindell, D., Storelvmo, T., Warren, S. G., and Zender, C. S.: Bounding the role of black carbon in the climate system: A scientific assessment, J. Geophys. Res.-Atmos., 118, 5380–5552, https://doi.org/10.1002/jgrd.50171, 2013.
Bourassa, A. E., Rieger, L. A., Lloyd, N. D., and Degenstein, D. A.: Odin-OSIRIS stratospheric aerosol data product and SAGE III intercomparison, Atmos. Chem. Phys., 12, 605–614, https://doi.org/10.5194/acp-12-605-2012, 2012.
Brunamonti, S., Jorge, T., Oelsner, P., Hanumanthu, S., Singh, B. B., Kumar, K. R., Sonbawne, S., Meier, S., Singh, D., Wienhold, F. G., Luo, B. P., Boettcher, M., Poltera, Y., Jauhiainen, H., Kayastha, R., Karmacharya, J., Dirksen, R., Naja, M., Rex, M., Fadnavis, S., and Peter, T.: Balloon-borne measurements of temperature, water vapor, ozone and aerosol backscatter on the southern slopes of the Himalayas during StratoClim 2016–2017, Atmos. Chem. Phys., 18, 15937–15957, https://doi.org/10.5194/acp-18-15937-2018, 2018.
Chang, C. P., Zhuo, W., John, M., and Ching-Hwang, L.: Annual Cycle of Southeast Asia – Maritime Continent Rainfall and the Asymmetric Monsoon Transition, J. Climate, 18, 287–301, https://doi.org/10.1175/JCLI-3257.1, 2005.
Chen, J. C., Li, Z., Ristovski, A., Milic, Y., Gu, M., S., Islam, S., Wang,
J., Hao, H., Zhang, C., He, H., Guo, H., Fu, B., Miljevic, L., Morawska, P.,
Thai, Y., Fat LAM, G., Pereira, A., Ding, X., Huang, and Dumka, U. C.: A
review of biomass burning: Emissions and impacts on air quality, health and
climate in China, Sci. Total Environ., 579, 1000–1034, 2017.
Cheng, Y. F., Berghof, M., Garland, R. M., Wiedensohler, A., Wehner, B., Müller, T., Su, H., Zhang, Y. H., Achtert, P., Nowak, A., Pöschl, U., Zhu, T., Hu, M., and Zeng, L. M.: Influence of soot mixing state on aerosol light absorption and single scattering albedo during air mass aging at a polluted regional site in northeastern China, J. Geophys. Res.-Atmos., 114, D00G10, https://doi.org/10.1029/2008JD010883, 2009.
Choi, M., Lim, H., Kim, J., Lee, S., Eck, T. F., Holben, B. N., Garay, M. J., Hyer, E. J., Saide, P. E., and Liu, H.: Validation, comparison, and integration of GOCI, AHI, MODIS, MISR, and VIIRS aerosol optical depth over East Asia during the 2016 KORUS-AQ campaign, Atmos. Meas. Tech., 12, 4619–4641, https://doi.org/10.5194/amt-12-4619-2019, 2019.
Dentener, F., Kinne, S., Bond, T., Boucher, O., Cofala, J., Generoso, S., Ginoux, P., Gong, S., Hoelzemann, J. J., Ito, A., Marelli, L., Penner, J. E., Putaud, J.-P., Textor, C., Schulz, M., van der Werf, G. R., and Wilson, J.: Emissions of primary aerosol and precursor gases in the years 2000 and 1750 prescribed data-sets for AeroCom, Atmos. Chem. Phys., 6, 4321–4344, https://doi.org/10.5194/acp-6-4321-2006, 2006.
Dessler, A. E., Schoeberl, M. R., Wang, T., Davis, S. M., and Rosenlof, K. H.:
Stratospheric Water Vapor Feedback, P. Natl. Acad. Sci. USA, 110,
18087–18091, https://doi.org/10.1073/pnas.1310344110, 2013.
Dong, X. and Fu, J. S.: Understanding interannual variations of biomass burning from Peninsular Southeast Asia, part II: Variability and different influencesin lower and higher atmosphere levels, Atmos. Environ., 115, 9–18, https://doi.org/10.1016/j.atmosenv.2015.05.052, 2015.
Fadnavis, S., Semeniuk, K., Pozzoli, L., Schultz, M. G., Ghude, S. D., Das, S., and Kakatkar, R.: Transport of aerosols into the UTLS and their impact on the Asian monsoon region as seen in a global model simulation, Atmos. Chem. Phys., 13, 8771–8786, https://doi.org/10.5194/acp-13-8771-2013, 2013.
Fadnavis, S., Kalita, G., Kumar, K. R., Gasparini, B., and Li, J.-L. F.: Potential impact of carbonaceous aerosol on the upper troposphere and lower stratosphere (UTLS) and precipitation during Asian summer monsoon in a global model simulation, Atmos. Chem. Phys., 17, 11637–11654, https://doi.org/10.5194/acp-17-11637-2017, 2017a.
Fadnavis, S., Roy, C., Sabin, T. P., Ayantika, D. C., and Karumuri, A.:
Potential modulations of pre-monsoon aerosols during El Niño: impact on
Indian summer monsoon, Clim. Dynam., 49, 2279–2290, https://doi.org/10.1007/s00382-016-3451-6, 2017b.
Fadnavis, S., Müller, R., Kalita, G., Rowlinson, M., Rap, A., Li, J.-L. F., Gasparini, B., and Laakso, A.: The impact of recent changes in Asian anthropogenic emissions of SO2 on sulfate loading in the upper troposphere and lower stratosphere and the associated radiative changes, Atmos. Chem. Phys., 19, 9989–10008, https://doi.org/10.5194/acp-19-9989-2019, 2019.
Fadnavis, S., Sabin, T. P., Rap, A., Müller, R., Kubin, A., and Heinold,
B.: The impact of COVID-19 lockdown measures on the Indian summer monsoon,
Environ. Res. Lett., 16, 074054, https://doi.org/10.1088/1748-9326/ac109c, 2021a.
Fadnavis, S., Sioris, C. E., Wagh, N., Chattopadhyay, R., Tao, M., Chavan,
P., and Chakroborty, T.: A rising trend of double tropopause s over South Asia
in a warming environment: Implications for moistening of the lower
stratosphere, Int. J. Climatol., 41, E200–E215, https://doi.org/10.1002/joc.6677,
2021b.
Fisher, J. A., Jacob, D. J., Wang, Q., Bahreini, R., Carouge, C. C., Cubison, M. J., Dibb, J. E., Diehl, T., Jimenez, J. L., Leibensperger, E. M., Lu, Z., Meinders, M. B. J., Pye, H. O. T., Quinn, P. K., Sharma, S., Streets, D. G., van Donkelaar, A., and Yantosca, R. M.: Sources, distribution, and acidity of sulfate-ammonium aerosol in the Arctic in winter–spring, Atmos. Environ., 45, 7301–7318, https://doi.org/10.1016/j.atmosenv.2011.08.030, 2011.
Gettelman, A., Piers, P. M., Fujiwara, M., Fu, Q., Vömel, H., Gohar, L. K., Johanson, C., and Ammerman, M.: Radiation balance of the tropical tropopause layer, J. Geophys. Res.-Atmos., 109, 1–12, https://doi.org/10.1029/2003jd004190, 2004.
Giglio, L., Descloitres, J., Justice, C. O., and Kaufman, Y. J.: An Enhanced
Contextual Fire Detection Algorithm for MODIS, Remote Sens. Environ.,
87, 273–282, 2003.
Giglio, L., Schroeder, W., and Justice, C. O.: The collection 6 MODIS active fire detection algorithm and fire products, Remote Sens. Environ., 178, 31–41, https://doi.org/10.1016/j.rse.2016.02.054, 2016.
Guenther, A.: A global model of natural volatile organic compound emissions, J. Geophys. Res., 100, 8873–8892, https://doi.org/10.1029/94JD02950, 1995.
Guha, A., Kumar De, B., Dhar, P., Banik, T., Chakraborty, M., Roy, R., Choudhury, A., Gogoi, M. M., Suresh Babu, S., and Krishna Moorthy, K.: Seasonal characteristics of aerosol black carbon in relation to long range transport over Tripura in Northeast India, Aerosol Air Qual. Res., 15, 786–798, https://doi.org/10.4209/aaqr.2014.02.0029, 2015.
Guhathakurta, P. and Rajeevan, M.: Trends in the rainfall pattern over India, Int. J. Climatol., 28, 1453–1469, https://doi.org/10.1002/joc.1640, 2008.
Hooghiem, J. J. D., Popa, M. E., Röckmann, T., Grooß, J.-U., Tritscher, I., Müller, R., Kivi, R., and Chen, H.: Wildfire smoke in the lower stratosphere identified by in situ CO observations, Atmos. Chem. Phys., 20, 13985–14003, https://doi.org/10.5194/acp-20-13985-2020, 2020.
Hanumanthu, S., Vogel, B., Müller, R., Brunamonti, S., Fadnavis, S., Li, D., Ölsner, P., Naja, M., Singh, B. B., Kumar, K. R., Sonbawne, S., Jauhiainen, H., Vömel, H., Luo, B., Jorge, T., Wienhold, F. G., Dirkson, R., and Peter, T.: Strong day-to-day variability of the Asian Tropopause Aerosol Layer (ATAL) in August 2016 at the Himalayan foothills, Atmos. Chem. Phys., 20, 14273–14302, https://doi.org/10.5194/acp-20-14273-2020, 2020.
Khaykin, S., Legras, B., Bucci, S., Sellitto, P., Isaksen, L., Tencé, F., Bekki, S., Bourassa, A., Rieger, L., Zawada, D., Jumelet, J., and Godin-Beekmann, S.: The 2019/20 Australian wildfires generated a persistent smoke-charged vortex rising up to 35 km altitude, Commun. Earth Environ., 1, 22, https://doi.org/10.1038/s43247-020-00022-5, 2020.
Lamarque, J.-F., Bond, T. C., Eyring, V., Granier, C., Heil, A., Klimont, Z., Lee, D., Liousse, C., Mieville, A., Owen, B., Schultz, M. G., Shindell, D., Smith, S. J., Stehfest, E., Van Aardenne, J., Cooper, O. R., Kainuma, M., Mahowald, N., McConnell, J. R., Naik, V., Riahi, K., and van Vuuren, D. P.: Historical (1850–2000) gridded anthropogenic and biomass burning emissions of reactive gases and aerosols: methodology and application, Atmos. Chem. Phys., 10, 7017–7039, https://doi.org/10.5194/acp-10-7017-2010, 2010.
Lau, K. M., Kim, M. K., and Kim, K. M.: Asian summer monsoon anomalies induced by aerosol direct forcing: The role of the Tibetan Plateau, Clim. Dynam., 26, 855–864, https://doi.org/10.1007/s00382-006-0114-z, 2006.
Lestrelin, H., Legras, B., Podglajen, A., and Salihoglu, M.: Smoke-charged vortices in the stratosphere generated by wildfires and their behaviour in both hemispheres: comparing Australia 2020 to Canada 2017, Atmos. Chem. Phys., 21, 7113–7134, https://doi.org/10.5194/acp-21-7113-2021, 2021.
Lin, C. Y., Zhao, C., Liu, X., Lin, N. H., and Chen, W. N.: Modelling of long-range transport of Southeast Asia biomass-burning aerosols to Taiwan and their radiative forcings over East Asia, Tellus B, 66, 1, https://doi.org/10.3402/tellusb.v66.23733, 2014.
Li, Z., Yang, S., He, B., and Hu, C.: Intensified Springtime Deep Convection
over the South China Sea and the Philippine Sea Dries Southern China, Sci.
Rep.-UK, 6, 30470, https://doi.org/10.3402/tellusb.v66.23733, 2016.
Matson, M. and Dozier, J.: Identification of Subresolution High
Temperature Sources Using a Thermal IR Sensor, Photogramm. Eng. Remote
Sens., 47, 1311–1318, 1981.
Maycock, A. C., Joshi, M. M., Shine, K. P., and Scaife, A. A.: The Circulation
Response to Idealized Changes in Stratospheric Water Vapor, J. Climate, 26,
545–561, https://doi.org/10.1175/JCLI-D-12-00155.1, 2013.
Meehl, G. A., Arblaster, J., and Collins, W. D.: Effects of Black Carbon
Aerosols on the Indian Monsoon, J. Climate, 21, 2869–2882, https://doi.org/10.1175/2007JCLI1777.1, 2008.
Mhawish, A., Banerjee, T., Sorek-Hamer, M., Lyapustin, A., Broday, D. M., and Chatfield, R.: Comparison and Evaluation of MODIS Multi-Angle Implementation
of Atmospheric Correction (MAIAC) Aerosol Product over South Asia, Remote
Sens. Environ., 224, 12–28, https://doi.org/10.1016/j.rse.2019.01.033, 2019.
Murugavel, P., Pawar, S. D., and Gopalakrishnan, V.: Trends of Convective Available Potential Energy over the Indian region and its effect on rainfall, Int. J. Climatol., 32, 1362–1372, https://doi.org/10.1002/joc.2359, 2012.
NASA: Resolution Imaging Spectrodiometer (MODIS), Fire Information for Resource Management System [data set], available at: https://firms.modaps.eosdis.nasa.gov/download, last access: 1 January 2021a.
NASA: MODATML2, LAADS DAAC [data set], available at: https://ladsweb.modaps.eosdis.nasa.gov/archive/allData/61/MODATML2/, last access: 1 January 2021b.
NASA: Multi-angle Imaging SpectroRadiometer (MISR), available at: https://misr.jpl.nasa.gov/getData/accessData/, last access: 1 January 2021c.
NASA: Aerosol Robotic NETwork (AERONET), available at: https://aeronet.gsfc.nasa.gov/, last access: 1 January 2021d.
Nguyen, H. N., Martinsson, B. G., Wagner, J. B., Carlemalm, E., Ebert, M., Weinbruch, S., Brenninkmeijer, C. A. M., Heintzenberg, J., Hermann, M., Schuck, T., van Velthoven, P. F. J., and Zahn, A.: Chemical composition and morphology of individual aerosol particles from a CARIBIC flight at 10 km altitude between 50∘ N and 30∘ S, J. Geophys. Res.-Atmos., 113, D23209, https://doi.org/10.1029/2008JD009956, 2008.
Ni, H., Huang, R.-J., Cao, J., Guo, J., Deng, H., and Dusek, U.: Sources and formation of carbonaceous aerosols in Xi'an, China: primary emissions and secondary formation constrained by radiocarbon, Atmos. Chem. Phys., 19, 15609–15628, https://doi.org/10.5194/acp-19-15609-2019, 2019.
NOAA/OAR/ESRL PSL: NCEP-DOE Reanalysis 2: Pressure Level, Physical Sciences Laboratory [data set], available at: https://psl.noaa.gov/data/gridded/data.ncep.reanalysis2.pressure.html, last access: 1 January 2021.
Oman, L., Waugh, D. W., Pawson, S., Stolarski, R. S., and Nielsen, J. E.: Understanding the changes of stratospheric water vapor in coupled chemistry-climate model simulations, J. Atmos. Sci., 65, 3278–3291, https://doi.org/10.1175/2008JAS2696.1, 2008.
Oshima, N., Kondo, Y., Moteki, N., Takegawa, N., Koike, M., Kita, K., Matsui, H., Kajino, M., Nakamura, H., Jung, J. S., and Kim, Y. J.: Wet removal of black carbon in Asian outflow: Aerosol Radiative Forcing in East Asia (A-FORCE) aircraft campaign, J. Geophys. Res.-Atmos., 117, D03204, https://doi.org/10.1029/2011JD016552, 2012.
Peterson, D. A., Campbell, J. R., Hyer, E. J., Fromm, M. D., Kablick, G. P., Cossuth, J. H., and DeLand, M. T.: Wildfire-driven thunderstorms cause a volcano-like stratospheric injection of smoke, npj Clim. Atmos. Sci., 1, 30, https://doi.org/10.1038/s41612-018-0039-3, 2018.
Pozzoli, L., Bey, I., Rast, S., Schultz, M. G., Stier, P., and Feichter, J.: Trace gas and aerosol interactions in the fully coupled model of aerosol-chemistry-climate ECHAM5-HAMMOZ: 1. Model
description and insights from the spring 2001 TRACE-P
experiment, J. Geophys. Res., 113, D07308, https://doi.org/10.1029/2007JD009007, 2008.
Randel, W. J., Park, M., Emmons, L., Kinnison, D., Bernath, P., Walker, K. A., Boone, C., and Pumphrey, H.: Asian monsoon transport of pollution to the stratosphere, Science, 328, 611–613, https://doi.org/10.1126/science.1182274, 2010.
Rieger, L. A., Malinina, E. P., Rozanov, A. V., Burrows, J. P., Bourassa, A. E., and Degenstein, D. A.: A study of the approaches used to retrieve aerosol extinction, as applied to limb observations made by OSIRIS and SCIAMACHY, Atmos. Meas. Tech., 11, 3433–3445, https://doi.org/10.5194/amt-11-3433-2018, 2018.
Riese, M., Ploeger, F., Rap, A., Vogel, B., Konopka, P., Dameris, M., and
Forster, P.: Impact of uncertainties in atmospheric mixing on simulated UTLS
composition and related radiative effects, J. Geophys. Res., 117, D16305,
https://doi.org/10.1029/2012JD017751, 2012.
Schill, G. P., Froyd, K. D., Bian, H., Kupc, A., Williamson, C., Brock, C. A., Ray, E., Hornbrook, R. S., Hills, A. J., Apel, E. C., Chin, M., Colarco, P. R., and Murphy, D. M.: Widespread biomass burning smoke throughout the remote troposphere, Nat. Geosci., 13, 422–427, https://doi.org/10.1038/s41561-020-0586-1, 2020.
Sherwood, S., Dixit, V., and Salomez, C.: The Global Warming Potential of
Near-Surface Emitted Water Vapour, Environ. Res. Lett., 13, 104006, https://doi.org/10.1088/1748-9326/aae018,
2018.
Shindell, D. T., Chin, M., Dentener, F., Doherty, R. M., Faluvegi, G., Fiore, A. M., Hess, P., Koch, D. M., MacKenzie, I. A., Sanderson, M. G., Schultz, M. G., Schulz, M., Stevenson, D. S., Teich, H., Textor, C., Wild, O., Bergmann, D. J., Bey, I., Bian, H., Cuvelier, C., Duncan, B. N., Folberth, G., Horowitz, L. W., Jonson, J., Kaminski, J. W., Marmer, E., Park, R., Pringle, K. J., Schroeder, S., Szopa, S., Takemura, T., Zeng, G., Keating, T. J., and Zuber, A.: A multi-model assessment of pollution transport to the Arctic, Atmos. Chem. Phys., 8, 5353–5372, https://doi.org/10.5194/acp-8-5353-2008, 2008.
Singh, N., Murari, V., Kumar, M., Barman, S. C., and Banerjee, T.: Fine particulates over South Asia: Review and meta-analysis of PM2.5 source apportionment through receptor model, Environ. Pollut., 223, 121–136, https://doi.org/10.1016/j.envpol.2016.12.071, 2017.
Singh, P., Sarawade, P., and Adhikary, B.: Carbonaceous aerosol from open burning and its impact on regional weather in South Asia, Aerosol Air Qual. Res., 20, 419–431, https://doi.org/10.4209/aaqr.2019.03.0146, 2020a.
Singh, P., Sarawade, P., and Adhikary, B.: Transport of black carbon from planetary boundary layer to free troposphere during the summer monsoon over South Asia, Atmos. Res., 235, 104761, https://doi.org/10.1016/j.atmosres.2019.104761, 2020b.
Stier, P., Feichter, J., Kinne, S., Kloster, S., Vignati, E., Wilson, J., Ganzeveld, L., Tegen, I., Werner, M., Balkanski, Y., Schulz, M., Boucher, O., Minikin, A., and Petzold, A.: The aerosol-climate model ECHAM5-HAM, Atmos. Chem. Phys., 5, 1125–1156, https://doi.org/10.5194/acp-5-1125-2005, 2005.
Streets, D. G., Yarber, K. F., Woo, J. H., and Carmichael, G. R.: Biomass
Burning in Asia: Annual and Seasonal Estimates and Atmospheric Emissions,
Global Biogeochem. Cy., 17, 1099, https://doi.org/10.1029/2003GB002040, 2003.
Talukdar, S., Jana, S., Maitra, A., and Gogoi, M. M.: Characteristics of black carbon concentration at a metropolitan city located near land-ocean boundary in Eastern India, Atmos. Res., 153, 526–534, https://doi.org/10.1016/j.atmosres.2014.10.014, 2015.
Tegen, I., Neubauer, D., Ferrachat, S., Siegenthaler-Le Drian, C., Bey, I., Schutgens, N., Stier, P., Watson-Parris, D., Stanelle, T., Schmidt, H., Rast, S., Kokkola, H., Schultz, M., Schroeder, S., Daskalakis, N., Barthel, S., Heinold, B., and Lohmann, U.: The global aerosol–climate model ECHAM6.3–HAM2.3 – Part 1: Aerosol evaluation, Geosci. Model Dev., 12, 1643–1677, https://doi.org/10.5194/gmd-12-1643-2019, 2019.
Thomas, A., Sarangi, C., and Kanawade, V. P.: Recent Increase in Winter Hazy Days over Central India and the Arabian Sea, Sci. Rep., 9, 17406, https://doi.org/10.1038/s41598-019-53630-3, 2019.
University of Saskatchewan: OSIRIS on Odin, available at: https://psl.noaa.gov/data/gridded/data.ncep.reanalysis2.pressure.html, last access: 1 January 2021.
Val Martin, M., Logan, J. A., Kahn, R. A., Leung, F.-Y., Nelson, D. L., and Diner, D. J.: Smoke injection heights from fires in North America: analysis of 5 years of satellite observations, Atmos. Chem. Phys., 10, 1491–1510, https://doi.org/10.5194/acp-10-1491-2010, 2010.
van Vuuren, D. P., Edmonds, J., Kainuma, M., Riahi, K., Thomson, A., Hibbard, K., Hurtt, G. C., Kram, T., Krey, V., Lamarque, J. F., Masui, T., Meinshausen, M., Nakicenovic, N., Smith, S. J., and Rose, S. K.: The representative concentration pathways: An overview, Clim. Change, 109, 5–31, https://doi.org/10.1007/s10584-011-0148-z, 2011.
Wang, S. H., Lin, N. H., Chou, M. D., and Woo, J. H.: Estimate of radiative forcing of Asian biomass-burning aerosols during the period of TRACE-P, J. Geophys. Res.-Atmos., 112, D10222, https://doi.org/10.1029/2006JD007564, 2007.
Wang, S. H., Welton, E. J., Holben, B. N., Tsay, S. C., Lin, N. H., Giles, D., Stewart, S. A., Janjai, S., Nguyen, X. A., Hsiao, T. C., Chen, W. N., Lin, T. H., Buntoung, S., Chantara, S., and Wiriya, W.: Vertical distribution and columnar optical properties of springtime biomass-burning aerosols over Northern Indochina during 2014 7-SEAS Campaign, Aerosol Air Qual. Res., 15, 2037–2050, https://doi.org/10.4209/aaqr.2015.05.0310, 2015.
Wang, X. and Dessler, A. E.: The response of stratospheric water vapor to climate change driven by different forcing agents, Atmos. Chem. Phys., 20, 13267–13282, https://doi.org/10.5194/acp-20-13267-2020, 2020.
Weigel, R., Mahnke, C., Baumgartner, M., Dragoneas, A., Vogel, B., Ploeger, F., Viciani, S., D'Amato, F., Bucci, S., Legras, B., Luo, B., and Borrmann, S.: In situ observation of new particle formation (NPF) in the tropical tropopause layer of the 2017 Asian monsoon anticyclone – Part 1: Summary of StratoClim results, Atmos. Chem. Phys., 21, 11689–11722, https://doi.org/10.5194/acp-21-11689-2021, 2021.
Wu, J., Kong, S., Wu, F., Cheng, Y., Zheng, S., Yan, Q., Zheng, H., Yang, G., Zheng, M., Liu, D., Zhao, D., and Qi, S.: Estimating the open biomass burning emissions in central and eastern China from 2003 to 2015 based on satellite observation, Atmos. Chem. Phys., 18, 11623–11646, https://doi.org/10.5194/acp-18-11623-2018, 2018.
Xie, F., Tian, W., Zhou, X., Zhang, J., Xia, Y., and Lu, J.: Increase in
Lower Stratospheric Water Vapor in the Past 100 Years Related to Tropical
Atlantic Warming, Geophys. Res. Lett., 47, e2020GL090539, https://doi.org/10.1029/2020GL090539, 2020.
Zhang, X., Liu, J., Han, H., Zhang, Y., Jiang, Z., Wang, H., Meng, L., Li,
Y. C., and Liu, Y.: Satellite-Observed Variations and Trends in Carbon
Monoxide over Asia and Their Sensitivities to Biomass Burning, Remote Sens.
12, 830, https://doi.org/10.3390/rs12050830, 2020.
Short summary
Biomass burning (BB) over Asia is a strong source of carbonaceous aerosols during spring. Here, we show an outflow of Asian BB carbonaceous aerosols into the UTLS. These aerosols enhance atmospheric heating and produce circulation changes that lead to the enhancement of water vapor in the UTLS over the tropics. In the stratosphere, water vapor is further transported to the South Pole by the Brewer–Dobson circulation. Enhancement of water vapor in the UTLS has implications for climate change.
Biomass burning (BB) over Asia is a strong source of carbonaceous aerosols during spring. Here,...
Altmetrics
Final-revised paper
Preprint