Articles | Volume 20, issue 9
https://doi.org/10.5194/acp-20-5573-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/acp-20-5573-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Shipborne observations reveal contrasting Arctic marine, Arctic terrestrial and Pacific marine aerosol properties
Jiyeon Park
CORRESPONDING AUTHOR
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon 21990, South Korea
Manuel Dall'Osto
Institut de Ciències del Mar, CSIC, Pg. Marítim de la
Barceloneta 37-49, 08003, Barcelona, Catalonia, Spain
Kihong Park
School of Earth Science and Environmental Engineering, Gwangju Institute of Science and Technology (GIST), 123
Cheomdangwagi-ro, Buk-gu, Gwangju 61005, South Korea
Yeontae Gim
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon 21990, South Korea
Hyo Jin Kang
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon 21990, South Korea
University of Science and Technology (UST), 217 Gajeong-ro,
Yuseong-gu, Daejeon, 34113, South Korea
Eunho Jang
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon 21990, South Korea
University of Science and Technology (UST), 217 Gajeong-ro,
Yuseong-gu, Daejeon, 34113, South Korea
Ki-Tae Park
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon 21990, South Korea
Minsu Park
Department of Atmospheric Sciences, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul 03722, South Korea
Seong Soo Yum
Department of Atmospheric Sciences, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul 03722, South Korea
Jinyoung Jung
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon 21990, South Korea
Bang Yong Lee
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon 21990, South Korea
Young Jun Yoon
Korea Polar Research Institute, 26 Songdomirae-ro, Yeonsu-gu, Incheon 21990, South Korea
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Stephen M. Platt, Øystein Hov, Torunn Berg, Knut Breivik, Sabine Eckhardt, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Markus Fiebig, Rebecca Fisher, Georg Hansen, Hans-Christen Hansson, Jost Heintzenberg, Ove Hermansen, Dominic Heslin-Rees, Kim Holmén, Stephen Hudson, Roland Kallenborn, Radovan Krejci, Terje Krognes, Steinar Larssen, David Lowry, Cathrine Lund Myhre, Chris Lunder, Euan Nisbet, Pernilla B. Nizzetto, Ki-Tae Park, Christina A. Pedersen, Katrine Aspmo Pfaffhuber, Thomas Röckmann, Norbert Schmidbauer, Sverre Solberg, Andreas Stohl, Johan Ström, Tove Svendby, Peter Tunved, Kjersti Tørnkvist, Carina van der Veen, Stergios Vratolis, Young Jun Yoon, Karl Espen Yttri, Paul Zieger, Wenche Aas, and Kjetil Tørseth
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Dimitrios Bousiotis, Francis D. Pope, David C. S. Beddows, Manuel Dall'Osto, Andreas Massling, Jakob Klenø Nøjgaard, Claus Nordstrøm, Jarkko V. Niemi, Harri Portin, Tuukka Petäjä, Noemi Perez, Andrés Alastuey, Xavier Querol, Giorgos Kouvarakis, Nikos Mihalopoulos, Stergios Vratolis, Konstantinos Eleftheriadis, Alfred Wiedensohler, Kay Weinhold, Maik Merkel, Thomas Tuch, and Roy M. Harrison
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Congbo Song, Manuel Dall'Osto, Angelo Lupi, Mauro Mazzola, Rita Traversi, Silvia Becagli, Stefania Gilardoni, Stergios Vratolis, Karl Espen Yttri, David C. S. Beddows, Julia Schmale, James Brean, Agung Ghani Kramawijaya, Roy M. Harrison, and Zongbo Shi
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We present a cluster analysis of relatively long-term (2015–2019) aerosol aerodynamic volume size distributions up to 20 μm in the Arctic for the first time. The study found that anthropogenic and natural aerosols comprised 27 % and 73 % of the occurrence of the coarse-mode aerosols, respectively. Our study shows that about two-thirds of the coarse-mode aerosols are related to two sea-spray-related aerosol clusters, indicating that sea spray aerosol may more complex in the Arctic environment.
Sehyun Jang, Ki-Tae Park, Kitack Lee, Young Jun Yoon, Kitae Kim, Hyun Young Chung, Eunho Jang, Silvia Becagli, Bang Yong Lee, Rita Traversi, Konstantinos Eleftheriadis, Radovan Krejci, and Ove Hermansen
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This study provides comprehensive datasets encompassing seasonal and interannual variations in sulfate and MSA concentration in aerosol particles in the Arctic atmosphere. As oxidation products of DMS have important roles in new particle formation and growth, we focused on factors affecting their variability and the branching ratio of DMS oxidation. We found a strong correlation between the ratio and the light condition, chemical properties of particles, and biological activities near Svalbard.
Cited articles
Abbatt, J. P. D., Leaitch, W. R., Aliabadi, A. A., Bertram, A. K., Blanchet, J.-P., Boivin-Rioux, A., Bozem, H., Burkart, J., Chang, R. Y. W., Charette, J., Chaubey, J. P., Christensen, R. J., Cirisan, A., Collins, D. B., Croft, B., Dionne, J., Evans, G. J., Fletcher, C. G., Galí, M., Ghahremaninezhad, R., Girard, E., Gong, W., Gosselin, M., Gourdal, M., Hanna, S. J., Hayashida, H., Herber, A. B., Hesaraki, S., Hoor, P., Huang, L., Hussherr, R., Irish, V. E., Keita, S. A., Kodros, J. K., Köllner, F., Kolonjari, F., Kunkel, D., Ladino, L. A., Law, K., Levasseur, M., Libois, Q., Liggio, J., Lizotte, M., Macdonald, K. M., Mahmood, R., Martin, R. V., Mason, R. H., Miller, L. A., Moravek, A., Mortenson, E., Mungall, E. L., Murphy, J. G., Namazi, M., Norman, A.-L., O'Neill, N. T., Pierce, J. R., Russell, L. M., Schneider, J., Schulz, H., Sharma, S., Si, M., Staebler, R. M., Steiner, N. S., Thomas, J. L., von Salzen, K., Wentzell, J. J. B., Willis, M. D., Wentworth, G. R., Xu, J.-W., and Yakobi-Hancock, J. D.: Overview paper: New insights into aerosol and climate in the Arctic, Atmos. Chem. Phys., 19, 2527–2560, https://doi.org/10.5194/acp-19-2527-2019, 2019.
ACIA: Arctic Climate Impact Assessment, Chap. 2, 23, Cambridge University
Press, New York, USA, 2005.
Allan, J. D., Williams, P. I., Najera, J., Whitehead, J. D., Flynn, M. J., Taylor, J. W., Liu, D., Darbyshire, E., Carpenter, L. J., Chance, R., Andrews, S. J., Hackenberg, S. C., and McFiggans, G.: Iodine observed in new particle formation events in the Arctic atmosphere during ACCACIA, Atmos. Chem. Phys., 15, 5599–5609, https://doi.org/10.5194/acp-15-5599-2015, 2015.
Anttila, T., Brus, D., Jaatinen, A., Hyvärinen, A.-P., Kivekäs, N., Romakkaniemi, S., Komppula, M., and Lihavainen, H.: Relationships between particles, cloud condensation nuclei and cloud droplet activation during the third Pallas Cloud Experiment, Atmos. Chem. Phys., 12, 11435–11450, https://doi.org/10.5194/acp-12-11435-2012, 2012.
Asmi, E., Kondratyev, V., Brus, D., Laurila, T., Lihavainen, H., Backman, J., Vakkari, V., Aurela, M., Hatakka, J., Viisanen, Y., Uttal, T., Ivakhov, V., and Makshtas, A.: Aerosol size distribution seasonal characteristics measured in Tiksi, Russian Arctic, Atmos. Chem. Phys., 16, 1271–1287, https://doi.org/10.5194/acp-16-1271-2016, 2016.
Benner, R., Louchouarn, P., and Amon, R. M. W.: Terrigenous dissolved
organic matter in the Arctic Ocean and its transport to surface and deep
waters of the North Atlantic, Global Biogeochem. Cy., 19, GB2025,
https://doi.org/10.1029/2004GB002398, 2005.
Burkart, J., Willis, M. D., Bozem, H., Thomas, J. L., Law, K., Hoor, P., Aliabadi, A. A., Köllner, F., Schneider, J., Herber, A., Abbatt, J. P. D., and Leaitch, W. R.: Summertime observations of elevated levels of ultrafine particles in the high Arctic marine boundary layer, Atmos. Chem. Phys., 17, 5515–5535, https://doi.org/10.5194/acp-17-5515-2017, 2017a.
Burkart, J., Hodshire, A. L., Mungall, E. L., Pierce, J. R., Collins, D. B.,
Ladino, L. A., Lee, A. K. Y., Irish, V., Wentzell, J. J. B., Liggio, J.,
Papakyriakou, T., Murphy, J., and Abbatt, J.: Organic condensation and particle
growth to CCN sizes in the summertimemarine Arctic is driven by materials
more semivolatile than at continental sites, Geophys. Res. Lett., 44,
10725–10734, https://doi.org/10.1002/2017GL075671, 2017b.
Chang, R. Y.-W., Sjostedt, S. J., Pierce, J. R., Papakyriakou, T. N.,
Scarratt, M. G., Michaud, S., Levasseur, M., Leaitch, W. R., and Abbatt, J.
P. D.: Relating atmospheric and oceanic DMS levels to particle nucleation
events in the Canadian Arctic, J. Geophys. Res.-Atmos.,
116, D00S03, https://doi.org/10.1029/2011JD015926, 2011.
Chen, X., Zhang, X., Church, J. A., Watson, C. S., King, M. A., Monselesan,
D., Legresy, B., and Harig, C.: The increasing rate of global mean sea-level
rise during 1993–2014, Nat. Clim. Change, 7, 492, https://doi.org/10.1038/nclimate3325,
2017.
Ciuraru, R., Fine, L., van Pinxteren, M., D'Anna, B., Herrmann, H., and
George, C.: Photosensitized production of functionalized and unsaturated
organic compounds at the air-sea interface, Sci. Rep., 5, 12741,
https://doi.org/10.1038/srep12741, 2015.
Coble, P. G.: Marine Optical Biogeochemistry: The Chemistry of Ocean Color,
Chem. Rev., 107, 402–418, https://doi.org/10.1021/cr050350+, 2007.
Collins, D. B., Burkart, J., Chang, R. Y.-W., Lizotte, M., Boivin-Rioux, A., Blais, M., Mungall, E. L., Boyer, M., Irish, V. E., Massé, G., Kunkel, D., Tremblay, J.-É., Papakyriakou, T., Bertram, A. K., Bozem, H., Gosselin, M., Levasseur, M., and Abbatt, J. P. D.: Frequent ultrafine particle formation and growth in Canadian Arctic marine and coastal environments, Atmos. Chem. Phys., 17, 13119–13138, https://doi.org/10.5194/acp-17-13119-2017, 2017.
Croft, B., Martin, R. V., Leaitch, W. R., Tunved, P., Breider, T. J., D'Andrea, S. D., and Pierce, J. R.: Processes controlling the annual cycle of Arctic aerosol number and size distributions, Atmos. Chem. Phys., 16, 3665–3682, https://doi.org/10.5194/acp-16-3665-2016, 2016.
Croft, B., Martin, R. V., Leaitch, W. R., Burkart, J., Chang, R. Y.-W., Collins, D. B., Hayes, P. L., Hodshire, A. L., Huang, L., Kodros, J. K., Moravek, A., Mungall, E. L., Murphy, J. G., Sharma, S., Tremblay, S., Wentworth, G. R., Willis, M. D., Abbatt, J. P. D., and Pierce, J. R.: Arctic marine secondary organic aerosol contributes significantly to summertime particle size distributions in the Canadian Arctic Archipelago, Atmos. Chem. Phys., 19, 2787–2812, https://doi.org/10.5194/acp-19-2787-2019, 2019.
Dall'Osto, M., Ceburnis, D., Martucci, G., Bialek, J., Dupuy, R., Jennings, S. G., Berresheim, H., Wenger, J., Healy, R., Facchini, M. C., Rinaldi, M., Giulianelli, L., Finessi, E., Worsnop, D., Ehn, M., Mikkilä, J., Kulmala, M., and O'Dowd, C. D.: Aerosol properties associated with air masses arriving into the North East Atlantic during the 2008 Mace Head EUCAARI intensive observing period: an overview, Atmos. Chem. Phys., 10, 8413–8435, https://doi.org/10.5194/acp-10-8413-2010, 2010.
Dall'Osto, M., Beddows, D. C. S., Tunved, P., Krejci, R.,
Ström, J., Hansson, H. C., Yoon, Y. J., Park, K.-T., Becagli, S.,
Udisti, R., Onasch, T., O'Dowd, C. D., Simó, R., and
Harrison, R. M.: Arctic sea ice melt leads to atmospheric new particle
formation, Sci. Rep., 7, 3318, https://doi.org/10.1038/s41598-017-03328-1, 2017.
Dall'Osto, M., Beddows, D. C. S., Tunved, P., Harrison, R. M., Lupi, A., Vitale, V., Becagli, S., Traversi, R., Park, K.-T., Yoon, Y. J., Massling, A., Skov, H., Lange, R., Strom, J., and Krejci, R.: Simultaneous measurements of aerosol size distributions at three sites in the European high Arctic, Atmos. Chem. Phys., 19, 7377–7395, https://doi.org/10.5194/acp-19-7377-2019, 2019.
Dal Maso, M.: Condensation and coagulation sinks and formation of nucleation
mode particles in coastal and boreal forest boundary layers, J. Geophys.
Res., 107, 8097, https://doi.org/10.1029/2001jd001053, 2002.
Dal Maso, M., Kulmala, M., Riipinen, I., Wagner, R., Hussein, T., Aalto, P.
P., and Lehtinen, K. E. J.: Formation and growth of fresh atmospheric
aerosols: Eight years of aerosol size distribution data from SMEAR II,
Hyytiälä, Finland, Boreal Environ. Res., 10, 323–336, 2005.
Dong, X., Xi, B., Crosby, K., Long, C. N., Stone, R. S., and Shupe, M.: A 10
year climatology of Arctic cloud fraction and radiative forcing at Barrow,
Alaska, J. Geophys. Res.-Atmos., 115, D17212, https://doi.org/10.1029/2009JD013489,
2010.
Ehn, M., Vuollekoski, H., Petäjä, T., Kerminen, V.-M., Vana, M.,
Aalto, P., de Leeuw, G., Ceburnis, D., Dupuy, R., O'Dowd, C. D., and
Kulmala, M.: Growth rates during coastal and marine new particle formation
in western Ireland, J. Geophys. Res.-Atmos., 115, D18218, https://doi.org/10.1029/2010JD014292,
2010.
Faubert, P., Tiiva, P., Rinnan, Å., Michelsen, A., Holopainen, J. K.,
and Rinnan, R.: Doubled volatile organic compound emissions from subarctic
tundra under simulated climate warming, New Phytol., 187, 199–208,
https://doi.org/10.1111/j.1469-8137.2010.03270.x, 2010.
Fichot, C. G., Kaiser, K., Hooker, S. B., Amon, R. M. W., Babin, M.,
Bélanger, S., Walker, S. A., and Benner, R.: Pan-Arctic distributions of
continental runoff in the Arctic Ocean, Sci. Rep., 3, 1053,
https://doi.org/10.1038/srep01053, 2013.
Freud, E., Krejci, R., Tunved, P., Leaitch, R., Nguyen, Q. T., Massling, A., Skov, H., and Barrie, L.: Pan-Arctic aerosol number size distributions: seasonality and transport patterns, Atmos. Chem. Phys., 17, 8101–8128, https://doi.org/10.5194/acp-17-8101-2017, 2017.
Frossard, A. A., Russell, L. M., Burrows, S. M., Elliott, S. M., Bates, T.
S., and Quinn, P. K.: Sources and composition of submicron organic mass in
marine aerosol particles, J. Geophys. Res.-Atmos., 119, 12977–913003, https://doi.org/10.1002/2014jd021913, 2014.
Fu, P., Kawamura, K., Chen, J., Qin, M., Ren, L., Sun, Y., Wang, Z., Barrie,
L. A., Tachibana, E., Ding, A., and Yamashita, Y.: Fluorescent water-soluble
organic aerosols in the High Arctic atmosphere, Sci. Rep., 5, 9845,
https://doi.org/10.1038/srep09845, 2015.
Furutani, H., Dall’osto, M., Roberts, G. C., and Prather, K. A.:
Assessment of the relative importance of atmospheric aging on CCN activity derived from field observations, Atmos. Environ., 42, 3130–3142, 2008.
Giamarelou, M., Eleftheriadis, K., Nyeki, S., Tunved, P., Torseth, K., and
Biskos, G.: Indirect evidence of the composition of nucleation mode
atmospheric particles in the high Arctic, J. Geophys. Res.-Atmos., 121,
965–975, https://doi.org/10.1002/2015JD023646, 2016.
Gunsch, M. J., Kirpes, R. M., Kolesar, K. R., Barrett, T. E., China, S., Sheesley, R. J., Laskin, A., Wiedensohler, A., Tuch, T., and Pratt, K. A.: Contributions of transported Prudhoe Bay oil field emissions to the aerosol population in Utqiaġvik, Alaska, Atmos. Chem. Phys., 17, 10879–10892, https://doi.org/10.5194/acp-17-10879-2017, 2017.
Heintzenberg, J., Leck, C., and Tunved, P.: Potential source regions and processes of aerosol in the summer Arctic, Atmos. Chem. Phys., 15, 6487–6502, https://doi.org/10.5194/acp-15-6487-2015, 2015.
Heintzenberg, J., Tunved, P., Galí, M., and Leck, C.: New particle formation in the Svalbard region 2006–2015, Atmos. Chem. Phys., 17, 6153–6175, https://doi.org/10.5194/acp-17-6153-2017, 2017.
Hinds, W. C.: Aerosol Technology: Properties, Behavior, and Measurement of
Airborne Particles, 2nd edn., Wiley-Interscience, New York, 1999.
Hoppel, W. A., Frick, G. M., Fitzgerald, J. W., and Larson, R. E.: Marine
boundary layer measurements of new particle formation and the effects
nonprecipitating clouds have on aerosol size distribution, J. Geophys. Res.-Atmos., 99, 14443–14459,
https://doi.org/10.1029/94jd00797, 1994.
Hudson, J. G. and Yum, S. S.: Cloud condensation nuclei spectra and
polluted and clean clouds over the Indian Ocean, J. Geophys. Res.-Atmos., 107, INX221-21–INX2221-12, https://doi.org/10.1029/2001jd000829, 2002.
IPCC: Climate change 2013: The physical science basis, Intergovernmental
panel on Climate Change, Cambridge University Press, New York, USA, 571–740,
2013.
Jang, E., Park, K.-T., Yoon, Y. J., Kim, T.-W., Hong, S.-B., Becagli, S., Traversi, R., Kim, J., and Gim, Y.: New particle formation events observed at the King Sejong Station, Antarctic Peninsula – Part 2: Link with the oceanic biological activities, Atmos. Chem. Phys., 19, 7595–7608, https://doi.org/10.5194/acp-19-7595-2019, 2019.
Jung, C. H., Yoon, Y. J., Kang, H. J., Gim, Y., Lee, B. Y., Ström, J.,
Krejci, R., and Tunved, P.: The seasonal characteristics of cloud
condensation nuclei (CCN) in the arctic lower troposphere, Tellus B:
Chem. Phys. Meteorol., 70, 1–13, https://doi.org/10.1080/16000889.2018.1513291,
2018.
Kalivitis, N., Kerminen, V.-M., Kouvarakis, G., Stavroulas, I., Bougiatioti, A., Nenes, A., Manninen, H. E., Petäjä, T., Kulmala, M., and Mihalopoulos, N.: Atmospheric new particle formation as a source of CCN in the eastern Mediterranean marine boundary layer, Atmos. Chem. Phys., 15, 9203–9215, https://doi.org/10.5194/acp-15-9203-2015, 2015.
Kerminen, V.-M., Chen, X., Vakkari, V., Petäjä, T., Kulmala, M., and
Bianchi, F.: Atmospheric new particle formation and growth: review of field
observations, Environ. Res. Lett., 13, 103003,
https://doi.org/10.1088/1748-9326/aadf3c, 2018.
Kim, G., Cho, H.-j., Seo, A., Kim, D., Gim, Y., Lee, B. Y., Yoon, Y. J., and
Park, K.: Comparison of Hygroscopicity, Volatility, and Mixing State of
Submicrometer Particles between Cruises over the Arctic Ocean and the
Pacific Ocean, Environ. Sci. Technol., 49, 12024–12035,
https://doi.org/10.1021/acs.est.5b01505, 2015.
Kim, J., Yoon, Y. J., Gim, Y., Kang, H. J., Choi, J. H., Park, K.-T., and Lee, B. Y.: Seasonal variations in physical characteristics of aerosol particles at the King Sejong Station, Antarctic Peninsula, Atmos. Chem. Phys., 17, 12985–12999, https://doi.org/10.5194/acp-17-12985-2017, 2017.
Kim, J., Yoon, Y. J., Gim, Y., Choi, J. H., Kang, H. J., Park, K.-T., Park, J., and Lee, B. Y.: New particle formation events observed at King Sejong Station, Antarctic Peninsula – Part 1: Physical characteristics and contribution to cloud condensation nuclei, Atmos. Chem. Phys., 19, 7583–7594, https://doi.org/10.5194/acp-19-7583-2019, 2019.
Kolesar, K. R., Cellini, J., Peterson, P. K., Jefferson, A., Tuch, T.,
Birmili, W., Wiedensohler, A., and Pratt, K. A.: Effect of Prudhoe Bay
emissions on atmospheric aerosol growth events observed in Utqiagvik
(Barrow), Alaska, Atmos. Environ., 152, 146–155,
https://doi.org/10.1016/j.atmosenv.2016.12.019, 2017.
Kulmala, M., Vehkamäki, H., Petäjä, T., Dal Maso, M., Lauri, A.,
Kerminen, V. M., Birmili, W., and McMurry, P. H.: Formation and growth rates
of ultrafine atmospheric particles: a review of observations, J.
Aerosol Sci., 35, 143–176, https://doi.org/10.1016/j.jaerosci.2003.10.003, 2004.
Law, K. S. and Stohl, A.: Arctic Air Pollution: Origins and Impacts,
Science, 315, 1537–1540, https://doi.org/10.1126/science.1137695, 2007.
Leaitch, W. R., Sharma, S., Huang, L., Toom-Sauntry, D., Chivulescu, A.,
Macdonald, A. M., von Salzen, K., Pierce, J. R., Bertram, A. K., Schroder,
J. C., Shantz, N. C., Chang, R. Y.-W., and Norman, A.-L.: Dimethyl sulfide
control of the clean summertime Arctic aerosol and cloud, Elem. Sci. Anth.,
1, 000017, https://doi.org/10.12952/journal.elementa.000017, 2013.
Leck, C., Norman, M., Bigg, E. K., and Hillamo, R.: Chemical composition and
sources of the high Arctic aerosol relevant for cloud formation, 107, AAC1-1–AAC1-17, https://doi.org/10.1029/2001jd001463, 2002.
Levasseur, M.: Impact of Arctic meltdown on the microbial cycling of
sulphur, Nat. Geosci., 6, 691, https://doi.org/10.1038/ngeo1910, 2013.
Lindwall, F., Schollert, M., Michelsen, A., Blok, D., and Rinnan, R.:
Fourfold higher tundra volatile emissions due to arctic summer warming, 121,
895–902, https://doi.org/10.1002/2015jg003295, 2016.
Mann, P. J., Spencer, R. G. M., Hernes, P. J., Six, J., Aiken, G. R., Tank,
S. E., McClelland, J. W., Butler, K. D., Dyda, R. Y., and Holmes, R. M.:
Pan-Arctic Trends in Terrestrial Dissolved Organic Matter from Optical
Measurements, Front. Earth Sci., 4, 25, https://doi.org/10.3389/feart.2016.00025, 2016.
Martin, M., Chang, R. Y.-W., Sierau, B., Sjogren, S., Swietlicki, E., Abbatt, J. P. D., Leck, C., and Lohmann, U.: Cloud condensation nuclei closure study on summer arctic aerosol, Atmos. Chem. Phys., 11, 11335–11350, https://doi.org/10.5194/acp-11-11335-2011, 2011.
Massicotte, P., Asmala, E., Stedmon, C., and Markager, S.: Global
distribution of dissolved organic matter along the aquatic continuum: Across
rivers, lakes and oceans, Sci. Total Environ., 609, 180–191,
https://doi.org/10.1016/j.scitotenv.2017.07.076, 2017.
Mauritsen, T., Sedlar, J., Tjernström, M., Leck, C., Martin, M., Shupe, M., Sjogren, S., Sierau, B., Persson, P. O. G., Brooks, I. M., and Swietlicki, E.: An Arctic CCN-limited cloud-aerosol regime, Atmos. Chem. Phys., 11, 165–173, https://doi.org/10.5194/acp-11-165-2011, 2011.
Merikanto, J., Spracklen, D. V., Mann, G. W., Pickering, S. J., and Carslaw, K. S.: Impact of nucleation on global CCN, Atmos. Chem. Phys., 9, 8601–8616, https://doi.org/10.5194/acp-9-8601-2009, 2009.
Mungall, E. L., Croft, B., Lizotte, M., Thomas, J. L., Murphy, J. G., Levasseur, M., Martin, R. V., Wentzell, J. J. B., Liggio, J., and Abbatt, J. P. D.: Dimethyl sulfide in the summertime Arctic atmosphere: measurements and source sensitivity simulations, Atmos. Chem. Phys., 16, 6665–6680, https://doi.org/10.5194/acp-16-6665-2016, 2016.
Németh, Z. and Salma, I.: Spatial extension of nucleating air masses in the Carpathian Basin, Atmos. Chem. Phys., 14, 8841–8848, https://doi.org/10.5194/acp-14-8841-2014, 2014.
Nguyen, Q. T., Glasius, M., Sørensen, L. L., Jensen, B., Skov, H., Birmili, W., Wiedensohler, A., Kristensson, A., Nøjgaard, J. K., and Massling, A.: Seasonal variation of atmospheric particle number concentrations, new particle formation and atmospheric oxidation capacity at the high Arctic site Villum Research Station, Station Nord, Atmos. Chem. Phys., 16, 11319–11336, https://doi.org/10.5194/acp-16-11319-2016, 2016.
O'Dowd, C., Ceburnis, D., Ovadnevaite, J., Vaishya, A., Rinaldi, M., and Facchini, M. C.: Do anthropogenic, continental or coastal aerosol sources impact on a marine aerosol signature at Mace Head?, Atmos. Chem. Phys., 14, 10687–10704, https://doi.org/10.5194/acp-14-10687-2014, 2014.
O'Dowd, C. D., Jimenez, J. L., Bahreini, R., Flagan, R. C., Seinfeld, J. H.,
Hämeri, K., Pirjola, L., Kulmala, M., Jennings, S. G., and Hoffmann, T.:
Marine aerosol formation from biogenic iodine emissions, Nature, 417, 632,
https://doi.org/10.1038/nature00775, 2002.
Oziel, L., Neukermans, G., Ardyna, M., Lancelot, C., Tison, J.-L., Wassmann,
P., Sirven, J., Ruiz-Pino, D., and Gascard, J.-C.: Role for Atlantic inflows
and sea ice loss on shifting phytoplankton blooms in the Barents Sea, J. Geophys. Res.-Oceans, 122,
5121–5139, https://doi.org/10.1002/2016jc012582, 2017.
Pang, X., Pu, J., Zhao, X., Ji, Q., Qu, M., and Cheng, Z.: Comparison
between AMSR2 Sea Ice Concentration Products and Pseudo-Ship Observations of
the Arctic and Antarctic Sea Ice Edge on Cloud-Free Days, Remote Sens., 10, 317, 2018.
Park, J. and Yoon, Y. J.: Concentration of Black Carbon on ARAON, Arctic Cruise, 2017, https://doi.org/10.22663/KOPRI-KPDC-00001140.4, 2020a.
Park, J. and Yoon, Y. J.: Condensation Particle Counter concentration (CPC3776, CPC3772) on ARAON 2017 Arctic Cruise, https://doi.org/10.22663/KOPRI-KPDC-00001137.4, 2020b.
Park, J. and Yoon, Y. J.: Concentration for each diameter (nano and normal SMPS) Data on ARAON Arctic Cruise, 2017, https://doi.org/10.22663/KOPRI-KPDC-00001136.5, 2020c.
Park, J. and Yoon, Y. J.: Concentration of Optical Particle Counter for each diameter on ARAON, Arctic ocean, 2017, https://doi.org/10.22663/KOPRI-KPDC-00001138.4, 2020d.
Park, J. and Yoon, Y. J.: Cloud Condensation Nuclei concentration of 2017 Arctic Cruise, ARAON, 2017, https://doi.org/10.22663/KOPRI-KPDC-00001141.5, 2020e.
Park, J., Dall'Osto, M., Park, K., Kim, J.-H., Park, J., Park, K.-T., Hwang,
C. Y., Jang, G. I., Gim, Y., Kang, S., Park, S., Jin, Y. K., Yum, S. S.,
Simó, R., and Yoon, Y. J.: Arctic Primary Aerosol Production Strongly
Influenced by Riverine Organic Matter, Environ. Sci.
Technol., 53, 8621–8630, https://doi.org/10.1021/acs.est.9b03399, 2019.
Park, K.-T., Jang, S., Lee, K., Yoon, Y. J., Kim, M.-S., Park, K., Cho, H.-J., Kang, J.-H., Udisti, R., Lee, B.-Y., and Shin, K.-H.: Observational evidence for the formation of DMS-derived aerosols during Arctic phytoplankton blooms, Atmos. Chem. Phys., 17, 9665–9675, https://doi.org/10.5194/acp-17-9665-2017, 2017.
Park, K.-T., Lee, K., Kim, T.-W., Yoon, Y. J., Jang, E.-H., Jang, S., Lee,
B.-Y., and Hermansen, O.: Atmospheric DMS in the Arctic Ocean and Its
Relation to Phytoplankton Biomass, Global Biogeochem. Cy., 32, 351–359, https://doi.org/10.1002/2017gb005805, 2018.
Peñuelas, J. and Staudt, M.: BVOCs and global change, Trend. Plant
Sci., 15, 133–144, https://doi.org/10.1016/j.tplants.2009.12.005, 2010.
Peters, G. P., Nilssen, T. B., Lindholt, L., Eide, M. S., Glomsrød, S., Eide, L. I., and Fuglestvedt, J. S.: Future emissions from shipping and petroleum activities in the Arctic, Atmos. Chem. Phys., 11, 5305–5320, https://doi.org/10.5194/acp-11-5305-2011, 2011.
Peterson, B. J., Holmes, R. M., McClelland, J. W., Vörösmarty, C.
J., Lammers, R. B., Shiklomanov, A. I., Shiklomanov, I. A., and Rahmstorf,
S.: Increasing River Discharge to the Arctic Ocean, Science, 298, 2171–2173,
https://doi.org/10.1126/science.1077445, 2002.
Pierce, J. R., Leaitch, W. R., Liggio, J., Westervelt, D. M., Wainwright, C. D., Abbatt, J. P. D., Ahlm, L., Al-Basheer, W., Cziczo, D. J., Hayden, K. L., Lee, A. K. Y., Li, S.-M., Russell, L. M., Sjostedt, S. J., Strawbridge, K. B., Travis, M., Vlasenko, A., Wentzell, J. J. B., Wiebe, H. A., Wong, J. P. S., and Macdonald, A. M.: Nucleation and condensational growth to CCN sizes during a sustained pristine biogenic SOA event in a forested mountain valley, Atmos. Chem. Phys., 12, 3147–3163, https://doi.org/10.5194/acp-12-3147-2012, 2012.
Pierce, J. R., Westervelt, D. M., Atwood, S. A., Barnes, E. A., and Leaitch, W. R.: New-particle formation, growth and climate-relevant particle production in Egbert, Canada: analysis from 1 year of size-distribution observations, Atmos. Chem. Phys., 14, 8647–8663, https://doi.org/10.5194/acp-14-8647-2014, 2014.
Potosnak, M. J., Baker, B. M., LeStourgeon, L., Disher, S. M., Griffin, K. L., Bret-Harte, M. S., and Starr, G.: Isoprene emissions from a tundra ecosystem, Biogeosciences, 10, 871–889, https://doi.org/10.5194/bg-10-871-2013, 2013.
Quinn, P. K. and Bates, T. S.: The case against climate regulation via
oceanic phytoplankton sulphur emissions, Nature, 480, 51–56,
https://doi.org/10.1038/nature10580, 2011.
Quinn, P. K., Collins, D. B., Grassian, V. H., Prather, K. A., and Bates, T.
S.: Chemistry and Related Properties of Freshly Emitted Sea Spray Aerosol,
Chem. Rev., 115, 4383–4399, https://doi.org/10.1021/cr500713g, 2015.
Raso, A. R. W., Custard, K. D., May, N. W., Tanner, D., Newburn, M. K.,
Walker, L., Moore, R. J., Huey, L. G., Alexander, L., Shepson, P. B., and
Pratt, K. A.: Active molecular iodine photochemistry in the Arctic,
P. Natl. Acad. Sci. USA, 114, 10053–10058,
https://doi.org/10.1073/pnas.1702803114, 2017.
Schmale, J., Arnold, S. R., Law, K. S., Thorp, T., Anenberg, S., Simpson, W.
R., Mao, J., and Pratt, K. A.: Local Arctic Air Pollution: A Neglected but
Serious Problem, Earth's Future, 6, 1385–1412, https://doi.org/10.1029/2018ef000952, 2018a.
Schmale, J., Henning, S., Decesari, S., Henzing, B., Keskinen, H., Sellegri, K., Ovadnevaite, J., Pöhlker, M. L., Brito, J., Bougiatioti, A., Kristensson, A., Kalivitis, N., Stavroulas, I., Carbone, S., Jefferson, A., Park, M., Schlag, P., Iwamoto, Y., Aalto, P., Äijälä, M., Bukowiecki, N., Ehn, M., Frank, G., Fröhlich, R., Frumau, A., Herrmann, E., Herrmann, H., Holzinger, R., Kos, G., Kulmala, M., Mihalopoulos, N., Nenes, A., O'Dowd, C., Petäjä, T., Picard, D., Pöhlker, C., Pöschl, U., Poulain, L., Prévôt, A. S. H., Swietlicki, E., Andreae, M. O., Artaxo, P., Wiedensohler, A., Ogren, J., Matsuki, A., Yum, S. S., Stratmann, F., Baltensperger, U., and Gysel, M.: Long-term cloud condensation nuclei number concentration, particle number size distribution and chemical composition measurements at regionally representative observatories, Atmos. Chem. Phys., 18, 2853–2881, https://doi.org/10.5194/acp-18-2853-2018, 2018b.
Schollert, M., Burchard, S., Faubert, P., Michelsen, A., and Rinnan, R. J.
P. B.: Biogenic volatile organic compound emissions in four vegetation types
in high arctic Greenland, Polar Biol., 37, 237–249, https://doi.org/10.1007/s00300-013-1427-0, 2014.
Sellegri, K., O'Dowd, C. D., Yoon, Y. J., Jennings, S. G., and Leeuw, G. d.:
Surfactants and submicron sea spray generation, J. Geophys.
Res.-Atmos., 111, D22215, https://doi.org/10.1029/2005JD006658, 2006.
Shen, Y., Fichot, C. G., and Benner, R.: Dissolved organic matter composition and bioavailability reflect ecosystem productivity in the Western Arctic Ocean, Biogeosciences, 9, 4993–5005, https://doi.org/10.5194/bg-9-4993-2012, 2012.
Shiklomanov, I. A., Shiklomanov, A. I., Lammers, R. B., Peterson, B. J., and
Vorosmarty, C. J.: The Dynamics of River Water Inflow to the Arctic Ocean,
in: The Freshwater Budget of the Arctic Ocean, edited by: Lewis, E. L.,
Jones, E. P., Lemke, P., Prowse, T. D., and Wadhams, P., Springer
Netherlands, Dordrecht, 281–296, 2000.
Spracklen, D. V., Carslaw, K. S., Kulmala, M., Kerminen, V.-M., Sihto,
S.-L., Riipinen, I., Merikanto, J., Mann, G. W., Chipperfield, M. P.,
Wiedensohler, A., Birmili, W., and Lihavainen, H.: Contribution of particle
formation to global cloud condensation nuclei concentrations, Geophys.
Res. Lett., 35, L06808, https://doi.org/10.1029/2007GL033038, 2008.
Steinke, M., Hodapp, B., Subhan, R., Bell, T. G., and Martin-Creuzburg, D.:
Flux of the biogenic volatiles isoprene and dimethyl sulfide from an
oligotrophic lake, Sci. Rep., 8, 630, https://doi.org/10.1038/s41598-017-18923-5,
2018.
Stier, P., Seinfeld, J. H., Kinne, S., and Boucher, O.: Aerosol absorption and radiative forcing, Atmos. Chem. Phys., 7, 5237–5261, https://doi.org/10.5194/acp-7-5237-2007, 2007.
Stroeve, J. C., Serreze, M. C., Holland, M. M., Kay, J. E., Malanik, J., and
Barrett, A. P.: The Arctic's rapidly shrinking sea ice cover: a research
synthesis, Clim. Change, 110, 1005–1027, https://doi.org/10.1007/s10584-011-0101-1, 2012.
Ström, J., Umegård, J., Tørseth, K., Tunved, P., Hansson, H. C.,
Holmén, K., Wismann, V., Herber, A., and König-Langlo, G.: One year
of particle size distribution and aerosol chemical composition measurements
at the Zeppelin Station, Svalbard, March 2000–March 2001, Phys.
Chem. Earth, Parts A/B/C, 28, 1181–1190, https://doi.org/10.1016/j.pce.2003.08.058, 2003.
Suni, T., Kulmala, M., Hirsikko, A., Bergman, T., Laakso, L., Aalto, P. P., Leuning, R., Cleugh, H., Zegelin, S., Hughes, D., van Gorsel, E., Kitchen, M., Vana, M., Hõrrak, U., Mirme, S., Mirme, A., Sevanto, S., Twining, J., and Tadros, C.: Formation and characteristics of ions and charged aerosol particles in a native Australian Eucalypt forest, Atmos. Chem. Phys., 8, 129–139, https://doi.org/10.5194/acp-8-129-2008, 2008.
Svenningsson, B., Arneth, A., Hayward, S., Holst, T., Massling, A.,
Swietlicki, E., Hirsikko, A., Junninen, H., Riipinen, I., Vana, M., Maso, M.
D., Hussein, T., and Kulmala, M.: Aerosol particle formation events and
analysis of high growth rates observed above a subarctic wetland–forest
mosaic, Tellus B: Chem. Phys. Meteorol., 60, 353–364,
https://doi.org/10.1111/j.1600-0889.2008.00351.x, 2008.
Tape, K., Sturm, M., and Racine, C.: The evidence for shrub expansion in
Northern Alaska and the Pan-Arctic, Glob. Change Biol., 12, 686–702,
https://doi.org/10.1111/j.1365-2486.2006.01128.x, 2006.
Tremblay, S., Picard, J.-C., Bachelder, J. O., Lutsch, E., Strong, K., Fogal, P., Leaitch, W. R., Sharma, S., Kolonjari, F., Cox, C. J., Chang, R. Y.-W., and Hayes, P. L.: Characterization of aerosol growth events over Ellesmere Island during the summers of 2015 and 2016, Atmos. Chem. Phys., 19, 5589–5604, https://doi.org/10.5194/acp-19-5589-2019, 2019.
Tunved, P., Ström, J., and Krejci, R.: Arctic aerosol life cycle: linking aerosol size distributions observed between 2000 and 2010 with air mass transport and precipitation at Zeppelin station, Ny-Ålesund, Svalbard, Atmos. Chem. Phys., 13, 3643–3660, https://doi.org/10.5194/acp-13-3643-2013, 2013.
Twomey, S.: Pollution and the planetary albedo, Atmos. Environ., 8, 1251–1256, https://doi.org/10.1016/0004-6981(74)90004-3, 1974.
Väänänen, R., Kyrö, E.-M., Nieminen, T., Kivekäs, N., Junninen, H., Virkkula, A., Dal Maso, M., Lihavainen, H., Viisanen, Y., Svenningsson, B., Holst, T., Arneth, A., Aalto, P. P., Kulmala, M., and Kerminen, V.-M.: Analysis of particle size distribution changes between three measurement sites in northern Scandinavia, Atmos. Chem. Phys., 13, 11887–11903, https://doi.org/10.5194/acp-13-11887-2013, 2013.
Vana, M., Kulmala, M., Dal Maso, M., Hõrrak, U., and Tamm, E.:
Comparative study of nucleation mode aerosol particles and intermediate air
ions formation events at three sites, J. Geophys. Res.-Atmos., 109, D17201, https://doi.org/10.1029/2003jd004413, 2004.
Vehkamäki, H., Dal Maso, M., Hussein, T., Flanagan, R., Hyvärinen, A., Lauros, J., Merikanto, P., Mönkkönen, M., Pihlatie, K., Salminen, K., Sogacheva, L., Thum, T., Ruuskanen, T. M., Keronen, P., Aalto, P. P., Hari, P., Lehtinen, K. E. J., Rannik, Ü., and Kulmala, M.: Atmospheric particle formation events at Värriö measurement station in Finnish Lapland 1998–2002, Atmos. Chem. Phys., 4, 2015–2023, https://doi.org/10.5194/acp-4-2015-2004, 2004.
Wang, M. and Overland, J. E.: A sea ice free summer Arctic within 30
years?, Geophys. Res. Lett., 36, L07502, https://doi.org/10.1029/2009GL037820, 2009.
Watson, J. G., Chow, J. C., Sodeman, D. A., Lowenthal, D. H., Chang, M. C.
O., Park, K., and Wang, X.: Comparison of four scanning mobility particle
sizers at the Fresno Supersite, Particuology, 9, 204–209, 2011.
Westervelt, D. M., Pierce, J. R., and Adams, P. J.: Analysis of feedbacks between nucleation rate, survival probability and cloud condensation nuclei formation, Atmos. Chem. Phys., 14, 5577–5597, https://doi.org/10.5194/acp-14-5577-2014, 2014.
Willis, M. D., Burkart, J., Thomas, J. L., Köllner, F., Schneider, J., Bozem, H., Hoor, P. M., Aliabadi, A. A., Schulz, H., Herber, A. B., Leaitch, W. R., and Abbatt, J. P. D.: Growth of nucleation mode particles in the summertime Arctic: a case study, Atmos. Chem. Phys., 16, 7663–7679, https://doi.org/10.5194/acp-16-7663-2016, 2016.
Willis, M. D., Leaitch, W. R., and Abbatt, J. P. D.: Processes Controlling
the Composition and Abundance of Arctic Aerosol, Rev. Geophys., 56, 621–671,
https://doi.org/10.1029/2018rg000602, 2018.
Yum, S. S., Hudson, J. G., and Xie, Y.: Comparisons of cloud microphysics
with cloud condensation nuclei spectra over the summertime Southern Ocean, J. Geophys. Res.-Atmos.,
103, 16625–16636, https://doi.org/10.1029/98jd01513, 1998.
Zhang, R., Khalizov, A., Wang, L., Hu, M., and Xu, W.: Nucleation and Growth
of Nanoparticles in the Atmosphere, Chem. Rev., 112, 1957–2011,
https://doi.org/10.1021/cr2001756, 2012.
Ziemba, L. D., Dibb, J. E., Griffin, R. J., Huey, L. G., and Beckman, P.:
Observations of particle growth at a remote, Arctic site, Atmos. Environ.,
44, 1649–1657, https://doi.org/10.1016/j.atmosenv.2010.01.032, 2010.
Short summary
The physical properties of aerosol particles throughout the Arctic Ocean and Pacific Ocean were measured aboard the Korean icebreaker R/V Araon during the summer of 2017. A number of new particle formation (NPF) events and growth were frequently observed in both Arctic terrestrial and Arctic marine air masses. This suggests that terrestrial ecosystems – including river outflows and tundra – strongly affect aerosol emissions in the Arctic coastal areas, affecting
radiative forcing.
The physical properties of aerosol particles throughout the Arctic Ocean and Pacific Ocean were...
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